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At least 325 records · Page 18
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Nature of polariton transport in a Fabry-Perot cavity

Fabry-Perot microcavities can strongly enhance interactions between light and molecules, leading to the formation of hybrid light-matter states known as polaritons. Polaritons possess much smaller effective masses and much larger group velocities when the molecules are resonant with cavity modes that have finite (nonzero) in-plane wave vectors, giving rise to the possibilities of long-range and ultrafast ballistic transport. In this paper, we present the results of numerical simulations of the ultrafast ballistic transport phenomenon in real space and time during and after initialization with a short, spatially localized pulse. Here, we address this problem with two approaches: the standard transfer-matrix method (TMM) for planar structures and a second simulation based on the numerical solution of the Maxwell-Bloch equations that can be used for general configurations (complex metasurfaces, for instance) and excitation modes. The agreement between the TMM and the full numerical calculation with the Maxwell-Bloch equations when applied to multilayer planar configurations provides proof of the validity of both approaches for the present analyses. Overall, we find that the transport of the molecular excitons inside the cavity synchronize with the evolution of the enhanced electromagnetic field inside the cavity. Moreover, the synchronized transport rate is in good agreement with the group velocities predicted from a calculated dispersion relation across a wide range of frequencies. Finally, we relate the group velocity to the Hopfield coefficient obtained from quantum modeling and suggest that the dependence of light-matter coupling on the in-plane wave vector can be an important but overlooked factor for understanding the transport behavior of polaritons. These simulations provide an intuitive tool for understanding the collective motion of light and excitons and helps us to better understand how experimental observations of polaritons should be interpreted.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Fundamental studies of thermal and electrical transport in microporous metal-organic frameworks

In this work, we established porous metal-organic frameworks (MOFs) as designer conductors of electrons and ions relevant to fundamental research and technological applications. MOFs are porous, crystalline materials composed of organic linkers and inorganic nodes. While most MOFs are insulating with respect to ionic and electronic charge carriers, a number of exceptions have been reported in recent years. Electrically conductive MOFs are highly attractive for applications including electrical energy storage, chemiresistive sensing, and optoelectronics because of their high surface areas and tunable chemical properties. Ion-conducting MOFs are desirable for the synthetically tunable size, shape, and polarity of their pore environments, allowing for the tailored development of solid state electrolytes for metal-ion batteries. We developed systematic strategies for the design of MOFs that conduct ions and electrons. For each objective, we leveraged the versatile chemistry of these materials to obtain frameworks with targeted properties towards electronic or ionic charge carriers. We studied the factors that govern electrical transport in MOFs in order to gain fundamental knowledge of this emerging class of materials. We took several approaches to tackle this problem from multiple angles. Namely, we synthesized and characterized new frameworks, investigated post-synthetic modifications to enhance conductivity, and correlated theory and experiment to uncover new mechanistic findings. These results, which put forth new design principles for conductive MOFs, move the field toward one of the DOE Basic Energy Sciences Grand Challenges: to “design and perfect atom- and energy-efficient synthesis of revolutionary new forms of matter with tailored properties.” In addition to investigating the movement of electrons in MOFs, we also studied the movement of other charged species in MOFs, such as protons, lithium, and magnesium. Proton-conducting frameworks could be appealing materials for solid state electrolytes in fuel cells. In addition, they contain crystallographically defined proton-conducting channels, in contrast with state-of-the-art polymer membranes such as Nafion, which are amorphous. Controlling pore size and polarity in MOFs can thus shed light on proton and other ion transport mechanisms, ultimately enabling the design of more advanced electrolyte materials and potentially novel electrical energy storage materials.

36 MATERIALS SCIENCE↗
NASA NTRS1991

HST observations of 3C 66B - A double-stranded optical jet

The central region of the synchrotron jet in 3C 66B imaged with ultrahigh spatial resolution by the Faint Object Camera on the HST is discussed. A close correspondence between the general characteristics of the smoothed optical image and the radio map is observed, implying that the young and old relativistic particles occupy similar regions to within about 130 pc. Focus is placed on the double-stranded filamentary nature of the jet, and it is speculated that this could reflect edge-brightening effects due to enhanced radiation from a skinlike structure surrounding the jet. It is noted that the similarity of optical and radio morphologies points to the fact that localized particle acceleration occurs along the jet; however, the filamentary structure and a low filling factor of radiation agree with a model in which the electrons are accelerated within the nucleus and are transported along the jet in a channel having low magnetic field.

Macchetto, F.↗
DOE OSTI2026

Suppression and enhancement of electromagnetic pulses from laser–target interactions by strong magnetic fields

Laser–target interactions generate intense electromagnetic pulses (EMPs) that can interfere with measurements and damage equipment. In this paper we show that applying a magnetic field to nanosecond pulse laser–target interactions decreases the magnitude of EMPs. We demonstrate this effect in two experiments with different geometries (spherical versus planar), laser intensities ( ∼10 13 versus ∼10 15 W/cm 2 ) and applied field strength (12 versus 0.1 T) that both observed suppression of EMPs in approximately the 1 GHz band (by factors of 0.65× and 0.32×, respectively). We then observe the opposite effect at high intensities with a picosecond pulse: for planar experiments with laser intensities of approximately 10 19 W/cm 2 and magnetic fields of 6–10 T, the magnitude of EMPs is increased by a factor of 1.75×. These results provide a benchmark for models of EMP generation, but suggest that magnetic fields are not a viable solution for mitigating EMPs in the high-intensity laser facilities where they are most damaging.

electromagnetic pulse↗
DOE OSTI2024

Constraining effects of aerosol-cloud interaction by accounting for coupling between cloud and land surface

Aerosol-cloud interactions (ACIs) are vital for regulating Earth’s climate by influencing energy and water cycles. Yet, effects of ACI bear large uncertainties, evidenced by systematic discrepancies between observed and modeled estimates. This study quantifies a major bias in ACI determinations, stemming from conventional surface or space measurements that fail to capture aerosol at the cloud level unless the cloud is coupled with land surface. We introduce an advanced approach to determine radiative forcing of ACI by accounting for cloud-surface coupling. By integrating field observations, satellite data, and model simulations, this approach reveals a drastic alteration in aerosol vertical transport and ACI effects caused by cloud coupling. In coupled regimes, aerosols enhance cloud droplet number concentration across the boundary layer more homogeneously than in decoupled conditions, under which aerosols from the free atmosphere predominantly affect cloud properties, leading to marked cooling effects. Our findings spotlight cloud-surface coupling as a key factor for ACI quantification, hinting at potential underassessments in traditional estimates.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Measuring Impact: Evaluating Thermal Zoning Simplification on Energy Efficiency Measures Analysis

Building Energy Modeling (BEM) is a versatile tool for designing, retrofitting, ensuring code compliance, obtaining certifications, qualifying for incentives, and enabling real-time building control. However, capturing all the details of building geometry for thermal zoning can be time-consuming, costly, and sometimes computationally challenging. As a result, modelers have been applying zoning simplification based on factors such as space functions and internal loads, as well as relying on their experience and judgment while adhering to zoning rules outlined in industry standards. Despite the prevalence of this common practice, a notable gap exists in the literature regarding studies quantifying the influence of simplified thermal zoning on the evaluation of Energy Efficiency Measures (EEMs). Recognizing this gap, this paper seeks to contribute to the field by enhancing the understanding of how the simplification of thermal zoning influences the evaluation of EEMs against a baseline design. The study utilized a medium office prototype model with a detailed floor plan featuring over 20 zones per floor covering diverse functional spaces with varying internal loads and occupancy schedules. A standard thermal zoning strategy outlined in ASHRAE Standard 90.1 Appendix G was employed as the simplified zoning method. This strategy condenses the zoning into a core zone and four perimeter zones per floor. It was compared with the detailed zoning approach, which involves one zone per space. Common Energy EEMs, such as enhanced envelope, high-efficiency appliances and equipment, and HVAC controls, were individually implemented and evaluated. The results indicate that the performance comparison between the two zoning methods varies depending on the type of measures considered. Basic measures, such as adding wall insulation, demonstrate similar energy impacts, while advanced HVAC control measures, such as static pressure reset, exhibit a more substantial difference that cannot be overlooked.

Xie, Jiarong↗
NASA NTRS1993

Appendix A: Proposed statement of work, 1994

This NRA effort is devoted to developing new techniques and methodologies which utilize and/or provide support to Integrated Vehicle Health Management (IVHM) concepts and techniques, modern design processes, and open architectures to realize an avionics system architecture that relieves the flight control system (FCS) of the requirement of maintaining intimate knowledge and control of the vehicle subsystems (for instance, the reaction control system (RCS)). The benefit of this architecture is that future upgrades and enhancements to the system(s) or to individual components within the system(s) are greatly simplified. This approach also allows a much more straightforward treatment of failure analysis, system diagnosis, and the design of fault containment domains. This NRA effort is also devoted to realizing capabilities to provide an available avionics system (and subsystem(s)) at minimum operational cost. This thrust provides a direct benefit to NASA in that it seeks to accelerate the design cycle to allow state of the art components and designs to actually appear in the fielded system rather than merely in the initial design. To achieve this, this effort is intended to benefit from efforts already underway at Lockheed and other major contractors. For instance, Lockheed Sanders is currently engaged in a major DoD funded development program which has the goal of cutting design cycle time of high performance electronics by a factor of four while simultaneously improving quality also by a factor of four. The early work on this program was used to enable the rapid prototyping of the Reaction Jet Drive Controller which was accomplished in 1993. Similarly, maximum leverage will be derived from recent NASA and DoD efforts to increase the content of high quality commercial grade electronic components in systems for aerospace applications. Both of these goals result in a system with enhanced cost effectiveness, increased reliability, and greatly increased performance compared to a system developed using a more conventional approach.

Source record↗
DOE OSTI2022

Field-Deployable Quantum Memory for Quantum Networking

High-performance quantum memories are an essential component for regulating temporal events in quantum networks. As a component in quantum-repeaters, they have the potential to support the distribution of entanglement beyond the physical limitations of fiber loss. This will enable key applications such as quantum key distribution, network-enhanced quantum sensing, and distributed quantum computing. Here, we present a quantum memory engineered to meet real-world deployment and scaling challenges. The memory technology utilizes a warm rubidium vapor as the storage medium, and operates at room temperature, without the need for vacuum- and/or cryogenic- support. Here, we demonstrate performance specifications of high-fidelity retrieval (95%) and low operation error (10 –2 ) at a storage time of 160 µs for single-photon level quantum memory operations. We further show a substantially improved storage time (with classical-level light) of up to 1ms by suppressing atomic diffusions. The device is housed in an enclosure with a standard 2U rackmount form factor, and can robustly operate on a day scale in a noisy environment. This result marks an important step toward implementing quantum networks in the field.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Magneto-Optical Sensing Beyond the Shot Noise Limit

Magneto-optical sensors including spin noise spectroscopies and magneto-optical Kerr effect microscopies are now ubiquitous tools for materials characterization that can provide new understanding of spin dynamics, hyperfine interactions, spin-orbit interactions, and charge-carrier g-factors. Both interferometric and intensity-difference measurements can provide photon-shot-noise-limited sensitivity, but further improvements in sensitivity with classical resources require either increased laser power that can induce unwanted heating and electronic perturbations or increased measurement times that can obscure out-of-equilibrium dynamics and slow experimental throughput. Proof-of-principle measurements have already demonstrated quantum enhanced spin noise measurements with a squeezed readout field that are likely to be critical to the nonperturbative characterization of spin excitations in quantum materials that emerge at low temperatures. Here, a truncated nonlinear interferometric readout for low-temperature magneto-optical Kerr effect and related magneto-optical microscopies that is accessible with today's quantum optical resources is proposed. 10 nrad/$\sqrt{Hz}$ sensitivity is achievable with optical power as small as 1 µW. As a result, measurements may be performed at temperatures as low as 83 mK in commercially available dilution refrigerators. This combination of high sensitivity and low operating temperature is impossible to achieve with any classical measurement. The quantum advantage for the proposed measurements persists even in the limit of large loss and small squeezing parameters.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1975

Some early results from the ATS-6 radio beacon experiment

The multifrequency satellite radio beacon enables the measurement of the columnar electron content of the ionosphere and plasmasphere along the ray path and its spatial and temporal structure. Measurements include modulation phase, Faraday rotation, and amplitude. The characteristics of the beacon transmitter and its design are presented together with the design of the Boulder receiver and antennas and the calibration procedures. A shape factor F is defined which depends on the electron density and geomagnetic field distributions. It is found that F varies by about 30% from day to night. It is shown that the ratio of the plasmaspheric content to total content varies from about 0.08 during the day to about 0.35 at night. Other examples which are presented to illustrate the uses of the radio beacon include sunrise effects, solar flare enhancements of total content, and the ionospheric storms of early July 1974.

Davies, K.↗
NASA NTRS1999

Microwave Induced Direct Bonding of Single Crystal Silicon Wafers

We have heated polished doped single-crystal silicon wafers in a single mode microwave cavity to temperatures where surface to surface bonding occurred. The absorption of microwaves and heating of the wafers is attributed to the inclusion of n-type or p-type impurities into these substrates. A cylindrical cavity TM (sub 010) standing wave mode was used to irradiate samples of various geometry's at positions of high magnetic field. This process was conducted in vacuum to exclude plasma effects. This initial study suggests that the inclusion of impurities in single crystal silicon significantly improved its microwave absorption (loss factor) to a point where heating silicon wafers directly can be accomplished in minimal time. Bonding of these substrates, however, occurs only at points of intimate surface to surface contact. The inclusion of a thin metallic layer on the surfaces enhances the bonding process.

Budraa, N. K.↗
DOE OSTI2025

Screening of Coulombic Interactions To Achieve a Higher Power Factor in Conjugated Polymers

Thermoelectric properties of conducting polymers typically suffer from molecular chain disordering, as charge transport is predominantly controlled by morphology. This is especially more problematic when counterions are introduced to tune the carrier concentration for optimal thermoelectric performance, which disturbs the morphology further. Here, in this work, we introduce a new avenue for enhancing thermoelectric properties without needing to regulate the morphology, namely, by controlling the coulombic interaction between polarons and counterions. We perform in situ de-doping thermoelectric experiments over 3 orders of magnitude change in electrical conductivity of three distinct thermoelectric polymers, namely, poly(3-hexylthiophene-2,5-diyl) (P3HT), poly[2,5-bis(3-dodecylthiophen-2-yl)thieno[3,2-b]thiophene] (PBTTT-C 12 ), and poly[2,5-(2-octyldodecyl)-3,6-diketopyrrolopyrrole-alt-5,5-(2,5-di(thien-2-yl)thieno[3,2-b]thiophene)] (OD-PDPP2T-TT) conjugated polymers, followed by grazing-incidence wide-angle X-ray scattering (GIWAXS) to study their respective morphologies. We demonstrate a 9-fold enhancement in the thermoelectric power factor in OD-PDPP2T-TT compared to PBTTT-C 12 and link it to the coulombic screening of charge carriers, including in the optimally doped regime. We support this hypothesis using Boltzmann transport equations and show that, in both P3HT and PBTTT-C 12 , as the polymer is doped, impurity scattering remains the dominant scattering mechanism, while in OD-PDPP2T-TT, the scattering mechanism changes from impurity to acoustic phonon limited, resulting in more effective screening of ionized counterions. Our results provide an additional knob to enhance the fundamental understanding of thermoelectric physics of conducting polymers and provide a pathway to achieve higher performance in the field of organic thermoelectrics.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Enhanced helium exhaust during edge-localized mode suppression by resonant magnetic perturbations at DIII-D

Effective helium confinement time, τ p * ,He , and its ratio with energy confinement time, τ p * ,He / τ E , are key metrics quantifying the suitability of fusion plasmas for a continuous burn. Comparisons in the DIII-D tokamak of discharges with suppression of edge localized modes (ELMs) by resonant magnetic field perturbations (RMPs) to the corresponding unperturbed ELMy discharges found that both of these metrics were strongly reduced, by a factor of approximately 2, after application of the RMPs. This reduction in τ p * ,He during RMP ELM suppression was observed in the plasma core, edge, and pumping plenum, where higher neutral helium concentration during RMPs was also measured. In conclusion, these findings provide evidence that future devices employing RMP ELM suppression may meet or even exceed the helium exhaust provided by the ELMs themselves, reducing helium ash, and thus maintaining high fusion gain.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Characterizing the Variation and Covariation of Cloud Microphysical Properties and Implications for Simulation of Subgrid-scale Warm-Rain Processes in Earth System Models (Final DOE-ASR Report)

Warm marine boundary layer (MBL) clouds constitute an important component in the global climate system, and precipitation plays a central role in controlling the water budget, radiative effects, and lifetime of these MBL clouds. Unfortunately, because of the relatively coarse effective grid resolution of the current generation of Earth system models (ESMs), the variety of cloud microphysical processes occurring inside an ESM grid cell are often oversimplified or unconstrained by observations. For example, the warm rain processes (e.g., autoconversion and accretion) are usually parameterized as nonlinear functions of grid-mean cloud properties. Because of the nonlinear nature of these functions, neglecting variability within the ESM grid volume can lead to substantial biases in precipitation production, cloud cover, and surface radiative fluxes. In state-of-the art ESMs, the influence of subgrid-scale variability is represented as an enhancement factor (EF) coefficient to the autoconversion, and accretion rates calculated from the model variables. However, EF is typically taken to be a constant or even used as a knob to tune model cloud properties to match observations, an ad hoc approach that may yield a desired cloud outcome yet introduce compensating errors. In this project, we used the combination of in situ cloud microphysics measurements from the ACE-ENA field campaign and large-eddy simulations (LES) to characterize and understand subgrid-scale variations and co-variations of cloud microphysical properties and use the results to evaluate and improve the representation of subgrid warm-rain processes in ESMs, in particular the EF used to tune the autoconversion and accretion processes. In this final report, we summarize our research activities and main findings in Section 2, provide a list of publications (Section 3) and presentations (Section 4) resulted from our research, and briefly discuss the student activities supported by this project.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1973

Composition and physics of the lunar atmosphere.

The existence in the lunar atmosphere of helium, neon, argon, and possibly molecular hydrogen has been confirmed by the Apollo 17 mass spectrometer. The observed helium concentrations and distribution agree closely with model predictions for a non-condensable gas based on a solar wind source, thermal escape and a Monte Carlo random walk calculated longitudinal distribution. Heavier gases are lost by photoionization and subsequent sweeping away by the solar wind electric field. The observed nighttime neon concentration of 80,000 molecules per cu cm is consistent with expected amounts. Argon, however, is adsorbed on the lunar surface late at night when the surface temperature is lowest. It shows the expected predawn enhancement exhibited by condensable gases released into the atmosphere at the sunrise terminator. Hydrogen appears to exist in the molecular rather than atomic state. Its observed concentration is less than a factor of 3 higher than that predicted by a model similar to that used for helium.

Hoffman, J. H.↗
NASA NTRS1994

Heating of the nighttime D region by very low frequency transmitters

VLF signals propagating in the Earth-ionosphere waveguide are used to probe the heated nighttime D region over three U.S. Navy very low frequency (VLF,3-30 kHz) transmitters. Ionospheric cooling and heating are observed when a transmitter turns off and on in the course of normal operations. Heating by the 24.0-kHz NAA transmitter in Cutler, Maine, (1000 kW radiated power) was observed by this method in 41 of 52 off/on episodes during December 1992, increasing the amplitude and retarding the phase of the 21.4-kHz NSS probe wave propagating from Annapolis, Maryland, to Gander, Newfoundland, by as much as 0.84 dB and 5.3 deg, respectively. In 6 of these 41 episodes, the amplitude of the 28.5-kHz NAU probe wave propagating from Puerto Rico to Gander was also perturbed by as much as 0.29 dB. The latter observations were unexpected due to the greater than 770 km distance between NAA and the NAU-Gander great circle path. Heating by the NSS (21.4 kHz, 265 kW) and NLK (24.8 kHz, 850 kW) transmitters was observed serendipitously in data from earlier measurements of the amplitudes of VLF signals propagating in the Earth-ionosphere waveguide. A three-dimensional model of wave absorption and electron heating in a magnetized, weakly ionized plasma is used to calculate the extent nad shape of the collision frequency (i.e., electron temperature) enhancement above a VLF transmitter. The enhancements are annular, with a geomagnetic north-south asymmetry and a radius at the outer half-maximum of the collision frequency enhancement of about 150 km. Heating by the NAA transmitter is predicted to increase the nighttime D region electron temperature by as much as a factor of 3. The calculated changes in the D region conductivity are used in a three-dimensional model of propagation in the Earth-ionosphere wavelength to predict the effect of the heated patch on a subionospheric VLF probe wave. The range of predicted scattered field amplitudes is in general consistent with the observed signal perturbations. Discrepanices in the predictions are attributed to lack of knowledge of the D region electron density profile along the probe wave great circle paths.

Rodriguez, Juan V.↗
NASA NTRS2022

Tentative Evidence for Water Vapor in the Atmosphere of the Neptune-sized Exoplanet HD106315c

We present a transmission spectrum for the Neptune-sized exoplanet HD 106315c from optical to infrared wavelengths based on transit observations from the Hubble Space Telescope/Wide Field Camera 3, K2, and Spitzer. The spectrum shows tentative evidence for a water absorption feature in the 1.1–1.7 μm wavelength range with a small amplitude of 30 ppm (corresponding to just 0.8 ± 0.04 atmospheric scale heights). Based on an atmospheric retrieval analysis, the presence of water vapor is tentatively favored with a Bayes factor of 1.7–2.6 (depending on prior assumptions). The spectrum is most consistent with either an enhanced metallicity or high-altitude condensates, or both. Cloud-free solar composition atmospheres are ruled out at >5σ confidence. We compare the spectrum to grids of cloudy and hazy forward models and find that the spectrum is fit well by models with moderate cloud lofting or haze formation efficiency over a wide range of metallicities (1–100× solar). We combine the constraints on the envelope composition with an interior structure model and estimate that the core mass fraction is ≳0.3. With a bulk composition reminiscent of that of Neptune and an orbital distance of 0.15 au, HD 106315c hints that planets may form out of broadly similar material and arrive at vastly different orbits later in their evolution.

Exoplanet atmospheres↗