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All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Effective radiative forcing of anthropogenic aerosols in E3SMv1: historical changes, causality, decomposition, and parameterization sensitivities

The effective radiative forcing of anthropogenic aerosols (ERF aer ) is an important measure of the anthropogenic aerosol effects simulated by a global climate model. Here we analyze ERF aer simulated by the E3SMv1 atmosphere model using both century-long free-running atmosphere-land simulations and short nudged simulations. We relate the simulated ERF aer to characteristics of the aerosol composition and optical properties, and evaluate the relationships between key aerosol and cloud properties. In terms of historical changes from the year 1870 to 2014, our results show that the global mean anthropogenic aerosol burden and optical depth increase during the simulation period as expected, but the regional averages show large differences in the temporal evolution. The largest regional differences are found in the emission-induced evolution of the burden and optical depth of the sulfate aerosol: a strong decreasing trend is seen in the Northern Hemisphere high-latitude region after around 1970, while a continued increase is simulated in the tropics. Consequently, although the global mean anthropogenic aerosol burden and optical depth increase from 1870 to 2014, the ERF aer magnitude does not increase after around year 1970. The relationships between key aerosol and cloud properties (relative changes between preindustrial and present-day conditions) also show evident changes after 1970, diverging from the linear relationships exhibited for the period from 1870 to 2014. The ERF aer in E3SMv1 is relatively large compared to the recently published multi-model estimates; the primary reason is the large indirect aerosol effect (i.e., through aerosol-cloud interactions). Compared to other models, E3SMv1 features a stronger sensitivity of the cloud droplet effective radius to changes in the cloud droplet number concentration. Large sensitivity is also seen in the liquid cloud optical depth, which is determined by changes in both the effective radius and liquid water path. Aerosol-induced changes in liquid and ice cloud properties in E3SMv1 are found to have a strong correlation, as the evolution of anthropogenic sulfate aerosols affects both the liquid cloud formation and the homogeneous ice nucleation in cirrus clouds. The ERF aer estimates in E3SMv1 for the shortwave and longwave components are sensitive to the parameterization changes in both liquid and ice cloud processes. When the parameterization of ice cloud processes is modified, the top-of-atmosphere forcing changes in the shortwave and longwave components largely offset each other, so the net effect is negligible. This suggests that, to reduce the magnitude of the net ERF aer , it would be more effective to reduce the anthropogenic aerosol effect through liquid or mixed-phase clouds.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Southern Great Plains (SGP) Three-Dimensional Observations of Fair-Weather Cumuli Field Campaign Report

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility Southern Great Plains (SGP) Three-Dimensional (3D) Observations of Fair-Weather Cumuli (SGP3DOBS) experiment employed scanning Doppler lidar and the recently installed stereo camera ring to conduct a one-month intensive operational period (IOP) of fair-weather cumuli in a 3D domain at the ARM SGP Central Facility (CF). The SGP3DOBS is part of the Climate Model Development and Validation (CMDV) “Coupling Mechanistically the Convective Motions and Cloud Macrophysics in a Climate Model” (CM4) project and provides advanced observational analyses for improving physical understanding of shallow cumulus and supporting model parameterization evaluation. For the CM4 project, cloud macroscale and dynamical properties are determined using vertically pointing active remote-sensing measurements (e.g., lidar and radar), which provide a 2D view of fair-weather cumuli (FWC). It is critical to evaluate how well the 2D observations represent 3D cloud fields. The objectives of SGP3DOBS include: 1) evaluate the 3D gridded cloud field from stereo photogrammetry with scanning Doppler lidar measurements; 2) retrieve sub-cloud-layer turbulence (vertical velocity and mass flux) in a 3D domain; 3) estimate shallow cumulus lateral entrainment rate and its relation to environment conditions. The SGP3DOBS IOP was held at the SGP Central Facility from August 31 to September 30, 2017, as the fair-weather nonprecipitating shallow cumuli are prevalent during summertime over land (Lamer and Kollias, 2015). A weather forecast team conducted a short-range forecast of weather conditions in the early morning each day to determine whether it was favorable for FWC. For each IOP day, the Doppler lidar at the SGP Central Facility ran under the range height indicator (RHI) scanning mode in the cross-wind direction. Occasionally, plan position indicator (PPI) scanning mode was run for updated wind directions. During each RHI scanning, the Doppler lidar run continuously between 30- and 150-degree elevation angles. The scanning rate was approximately 10 degree/s, corresponding to a transverse resolution of 111 m at 2 km of a typical FWC height. The newly established three pairs of stereo cameras ran concurrently during the IOP.

Southern Great Plains, Doppler lidar, fair-weather↗
DOE OSTI2018

Macquarie Island Cloud and Radiation Experiment (MICRE) Ice Nucleating Particle Measurements Field Campaign Report

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility Macquarie Island Cloud and Radiation Experiment (MICRE) Ice Nucleating Particle Measurements campaign was aligned as a supplemental activity with the second year of the overall MICRE campaign. The purpose of the supplemental campaign was to provide a first-ever annual cycle of ice nucleating particle (INP) measurements at a Southern Ocean (SO) site, toward the investigation/characterization of sources of INPs in the marine boundary layer as being from the production or primary sea spray aerosol (SSA) emissions versus other long-range transport influences. Furthermore, measuring the variability in INPs seasonally in this region, as this may relate to meteorology and ocean biological processes, is expected to help constrain (via parameterizations) numerical model simulations of cloud phase and regional climate. In concert with other SO studies during the time frame of the campaign (March 2017 to March 2018), MICRE sought to evaluate the hypotheses that SSA INPs represent the major INP source in the SO and, due to their generally less efficient INP activation properties compared to terrestrial sources, that they may directly influence the persistence of supercooled clouds in a unique manner for this climatic region. These measurements supplemented the original deployment of primarily radiation measurements provided in the ARM MICRE request and the associated Australian Antarctic Division (AAD) Antarctic Clouds and Radiation Experiment (ACRE). Assistance and collaboration was obtained from the AAD, the Commonwealth Scientific and Industrial Research Organization (CSIRO) and the Australian Bureau of Meteorology (BOM). Follow-up plans will include investigations with their additional aerosol, cloud, and radiative transfer measurements. AAD also saw to the transport to Australia and storage of filters at the end of the campaign. The added effort involved an average of twice-weekly collections (a 48-hour and a 72-hour collection) of pre-sterilized, open-faced, polycarbonate filter samples for post-processing of INP number concentrations and tests to analyze the nature of INP sources. Collections were made by AAD technician Emry Thaggard Crocker after online training from our team. Images of the filter sampler and site are shown in Figure 1. Sampling occurred from an approximate elevation of 4m MSL. Filters were returned frozen to Colorado State University (CSU) at the end of the campaign. Initial processing to obtain INP temperature spectra (0 to -28°C) of the concentrations of INPs active via the immersion freezing mechanism were conducted using the CSU ice spectrometer (IS) instrument systems (Hiranuma et al. 2015; McCluskey et al. 2018). In this method, particles are first removed from filters using ultrapure water while under mechanical agitation. Arrays of the particle suspensions from a portion of filter rinses are then cooled to obtain immersion freezing data per volume of water, and finally are related to sampling volumes to obtain numbers per volume of air following the analysis methods of Vali (1971). A total of 103 filters were collected, including blanks at selected intervals throughout the project. For archival and completion of tasks under this ARM proposal, nearly half of the filter collections (46) were processed for basic temperature spectra, and half of these (23) were also tested for microbial/proteinaceous contributions toward INPs via 95°C pre-treatment of portions of the original suspensions.

Southern Ocean, aerosols, marine clouds, MARCUS ca↗
DOE OSTI2019

The double ITCZ syndrome in GCMs: A coupled feedback problem among convection, clouds, atmospheric and ocean circulations

The appearance of a spurious double ITCZ south of the equator in coupled general circulation models has been a stubborn problem ever since the beginning of coupled model development. This article reviews the past research in this area, with a focus on three possible major contributors to the double ITCZ biases: 1) the southeastern Pacific marine stratus clouds and associated warm sea surface temperature (SST) biases; 2) the extratropical shortwave absorption biases over Southern Ocean; and 3) convective parameterization. The negative biases in marine boundary layer clouds in the southeastern Pacific lead to warm SST biases. Through coupled atmosphere-ocean interactions, it contributes to the double ITCZ bias. Positive shortwave absorption biases over Southern Ocean is believed to be an extratropical contributor to the double ITCZ biases in models. Since the heat from excess shortwave absorption must be transported to the northern hemisphere by the Hadley circulation, the position of the ITCZ must shift southward. However, later research finds that reducing the extratropical shortwave absorption has little effect on the ITCZ position. One possibility is that some feedback mechanism involving subtropical low-level clouds as intermediary is missing. For convective parameterization, changes in various elements in convection schemes can have large impacts on the ITCZ simulation. It involves a complex chain of interactions among convection, large-scale atmospheric circulation, SST, and upper ocean circulation. In one scheme, changes in the scheme lead to the elimination of double ITCZ in all seasons, giving hope that we can finally take on the double ITCZ problem.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

The Implementation of Framework for Improvement by Vertical Enhancement Into Energy Exascale Earth System Model

Abstract The low cloud bias in global climate models (GCMs) remains an unsolved problem. Coarse vertical resolution in GCMs has been suggested to be a significant cause of low cloud bias because planetary boundary layer parameterizations cannot resolve sharp temperature and moisture gradients often found at the top of subtropical stratocumulus layers. This work aims to ameliorate the low cloud problem by implementing a new computational method, the Framework for Improvement by Vertical Enhancement (FIVE), into the Energy Exascale Earth System Model (E3SM). Three physics schemes representing microphysics, radiation, and turbulence as well as vertical advection are interfaced to vertically enhanced physics (VEP), which allows for these processes to be computed on a higher vertical resolution grid compared to the rest of the E3SM model. We demonstrate the better representation of subtropical boundary layer clouds with FIVE while limiting additional computational cost from the increased number of levels. When the vertical resolution approaches the large eddy simulation‐like vertical resolution in VEP, the climatological low cloud amount shows a significant increase of more than 30% in the southeastern Pacific Ocean. Using FIVE to improve the representation of low‐level clouds does not come with any negative side effects associated with the simulation of mid‐ and high‐level cloud and precipitation, that can occur when running the full model at higher vertical resolution.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Cloud-atmosphere impacts on the central Arctic surface energy budget (Final Report)

This project investigated how clouds and atmosphere-sea ice interactions shape the central Arctic surface energy budget using observations from the MOSAiC expedition and coordinated model experiments. Analyses focused on three themes. First, a new method applied to thermistor string data revealed that snow thermal conductivity is systematically higher than assumed in most models, strongly influencing conductive heat flux and sea ice growth, especially under clear skies. Second, a full annual cycle of surface energy budget observations, combined with detailed cloud microphysical retrievals, demonstrated how cloud regimes regulate radiative, turbulent, and conductive fluxes, driving seasonal contrasts in sea ice energy balance: in winter, radiative forcing elicits strong turbulent and conductive responses, while in summer excess energy is primarily partitioned into surface melt. Third, these observations were used to evaluate and improve regional and global forecast models. While some models captured key Arctic cloud-radiation states, most exhibited persistent deficiencies in representing liquid-containing clouds, snow-on-sea-ice processes, and flux responses to radiative forcing. Together, these results provide unprecedented benchmarks for understanding coupled Arctic processes, improve parameterizations of snow, sea ice, and cloud interactions, and highlight critical pathways by which atmospheric variability drives sea ice change in a rapidly evolving Arctic system. Lastly, the project was a resounding success, resulting in 38 peer-reviewed publications and dozens of presentations, while also supporting an early career scientist.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Improving Predictability of Mixed-Phase Clouds and Aerosol Interactions in the Community Earth System Model (CESM) with ARM Measurements

The objective of this project is to improve the simulation and predictability of mixed-phase clouds and aerosol interactions in the Community Earth System Model (CESM) through comparisons with the DOE ARM observations. There are four major goals of the proposed study: (1) Improve the representation of ice microphysical processes in mixed-phase clouds; (2) Develop a long-term multi-sensor mixed-phase cloud dataset; (3) Test the performance of improved ice microphysics in CESM-CAM5 with the ARM data; and (4) Examine mixed-phase cloud microphysics-aerosol-dynamics-radiation interactions in CESM-CAM5. In this project, we have (1) Improved the representation of ice microphysical processes in mixed-phase clouds that include ice nucleation, ice depositional growth through the Wegener–Bergeron–Findeisen (WBF) process, feedbacks between cloud microphysics, dynamics and radiation, and provides links to aerosol properties in the Community Earth System Model (CESM)-Community Atmosphere Model version 5 (CAM5); (2) Developed a long-term multi-sensor mixed-phase cloud dataset. The mixed-phase cloud retrieval algorithms are improved by refining the phase determinations and ice number concentration retrievals. A multi-year mixed-phase cloud observation dataset (1999-2004; October 2013-February 2017) is regenerated at the ARM Barrow site with the improved algorithms. The dataset has been used in the global model evaluation to improve the model parameterizations; (3) Tested the performance of improved ice microphysics in CESM-CAM5 with the ARM data. CESM-CAM5 is run in the DOE Cloud-Associated Parameterizations Testbed (CAPT) and in the single-column model (SCM) mode to facilitate comparison with ARM observations. Multi-year CAPT simulations of seasonal variations of cloud microphysical properties, cloud liquid water path (LWP) and ice water path (IWP), cloud longwave and shortwave forcings, cloud occurrence frequency are evaluated against the ARM multi-sensor mixed-phase cloud retrievals; and (4) Examined mixed-phase cloud microphysics-aerosol-dynamics-radiation interactions in CESM-CAM5 that include the impacts of different ice nucleation mechanisms, sensitivity to dust IN concentration, treatment of the WBF process on mixed-phase cloud properties. Aerosol effect on mixed-phase clouds through the liquid phase (droplet activation) and ice phase processes (e.g., the glaciation indirect effect) is investigated.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Processing of Ice Cloud In Situ Data Collected by Bulk Water, Scattering, and Imaging Probes: Fundamentals, Uncertainties, and Efforts toward Consistency

Abstract In situ observations of cloud properties made by airborne probes play a critical role in ice cloud research through their role in process studies, parameterization development, and evaluation of simulations and remote sensing retrievals. To determine how cloud properties vary with environmental conditions, in situ data collected during different field projects processed by different groups must be used. However, because of the diverse algorithms and codes that are used to process measurements, it can be challenging to compare the results. Therefore it is vital to understand both the limitations of specific probes and uncertainties introduced by processing algorithms. Since there is currently no universally accepted framework regarding how in situ measurements should be processed, there is a need for a general reference that describes the most commonly applied algorithms along with their strengths and weaknesses. Methods used to process data from bulk water probes, single-particle light-scattering spectrometers and cloud-imaging probes are reviewed herein, with emphasis on measurements of the ice phase. Particular attention is paid to how uncertainties, caveats, and assumptions in processing algorithms affect derived products since there is currently no consensus on the optimal way of analyzing data. Recommendations for improving the analysis and interpretation of in situ data include the following: establishment of a common reference library of individual processing algorithms, better documentation of assumptions used in these algorithms, development and maintenance of sustainable community software for processing in situ observations, and more studies that compare different algorithms with the same benchmark datasets.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Estimating Drizzle Parameters by Aircraft Sampling

In-cloud supersaturation is calculated from aircraft derived measurements of the in-cloud vertical gradient of liquid water content, vertical velocity, the pt and 3 rd cloud droplet radius moments and a parameter related to the heat and mass transport during condensation and evaporation of cloud droplets. The aircraft data where taken during the VOCALS 2008 study in marine stratocumulus clouds off the coast of Chile. Approximately 16000 discrete samples, 2.5 meter in length, were used in the present analysis of in-cloud supersaturation and its variability, both of which are indicative of turbulent processes within the cloud and their significant impact on drizzle formation. Two additional drizzle parameters, the eddy persistence time and the variance of fluctuations in in-cloud droplet growth rate were also estimated from this data set. These results will help to constrain parameterizations of underlying turbulent microphysical processes of clouds and thereby advance the future development of warm cloud and precipitation models for climate simulation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

A new parameterization of ice heterogeneous nucleation coupled to aerosol chemistry in WRF-Chem model version 3.5.1: evaluation through ISDAC measurements

In the Arctic, during polar night and early spring, ice clouds are separated into two leading types of ice clouds (TICs): (1) TIC1 clouds characterized by a large concentration of very small crystals and TIC2 clouds characterized by a low concentration of large ice crystals. Using a suitable parameterization of heterogeneous ice nucleation is essential for properly representing ice clouds in meteorological and climate models and subsequently understanding their interactions with aerosols and radiation. Here, we describe a new parameterization for ice crystal formation by heterogeneous nucleation in water-subsaturated conditions coupled to aerosol chemistry in the Weather Research and Forecasting model coupled with chemistry (WRF-Chem). The parameterization is implemented in the Milbrandt and Yau (2005a, b) two-moment cloud microphysics scheme, and we assess how the WRF-Chem model responds to the run-time interaction between chemistry and the new parameterization. Well-documented reference cases provided us with in situ data from the spring 2008 Indirect and Semi-Direct Aerosol Campaign (ISDAC) over Alaska. Our analysis reveals that the new parameterization clearly improves the representation of the ice water content (IWC) in polluted or unpolluted air masses and shows the poor performance of the reference parameterization in representing ice clouds with low IWC. The new parameterization is able to represent TIC1 and TIC2 microphysical characteristics at the top of the clouds, where heterogenous ice nucleation is most likely occurring, even with the known bias of simulated aerosols by WRF-Chem over the Arctic.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Prescribing the aerosol effective radiative forcing in the Simple Cloud-Resolving E3SM Atmosphere Model v1

Aerosol effective radiative forcing critically influences climate projections but remains poorly constrained. Using the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM) v1 configuration, we assess the sensitivity of the radiative forcing due to anthropogenic aerosol changes using a simplified prescribed aerosol scheme (SPA) derived from E3SM v3. Nudged simulations at 3 and 12 km horizontal grid spacings reveal a more negative aerosol forcing than the reference 100 km E3SM v3 whence the SPA properties are derived. The resulting globally averaged aerosol forcing signal is largely due to aerosol–cloud interactions and exhibits little overall resolution sensitivity, while hints of resolution sensitivity appear regionally between the 3 and 12 km runs. While the default SPA scheme overestimates cloud droplet dependence on aerosols, parameterization adjustments in the activation process reconcile forcing estimates with the reference model. Our results demonstrate the ability to use a prescribed aerosol scheme to hold aerosol forcing to a desired strength across resolutions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

The importance of considering sub-grid cloud variability when using satellite observations to evaluate the cloud and precipitation simulations in climate models

Abstract. Satellite cloud observations have become an indispensable tool for evaluating general circulation models (GCMs). To facilitate the satellite and GCM comparisons, the CFMIP (Cloud Feedback Model Inter-comparison Project) Observation Simulator Package (COSP) has been developed and is now increasingly used in GCM evaluations. Real-world clouds and precipitation can have significant sub-grid variations, which, however, are often ignored or oversimplified in the COSP simulation. In this study, we use COSP cloud simulations from the Super-Parameterized Community Atmosphere Model (SPCAM5) and satellite observations from the Moderate Resolution Imaging Spectroradiometer (MODIS) and CloudSat to demonstrate the importance of considering the sub-grid variability of cloud and precipitation when using the COSP to evaluate GCM simulations. We carry out two sensitivity tests: SPCAM5 COSP and SPCAM5-Homogeneous COSP. In the SPCAM5 COSP run, the sub-grid cloud and precipitation properties from the embedded cloud-resolving model (CRM) of SPCAM5 are used to drive the COSP simulation, while in the SPCAM5-Homogeneous COSP run only grid-mean cloud and precipitation properties (i.e., no sub-grid variations) are given to the COSP. We find that the warm rain signatures in the SPCAM5 COSP run agree with the MODIS and CloudSat observations quite well. In contrast, the SPCAM5-Homogeneous COSP run which ignores the sub-grid cloud variations substantially overestimates the radar reflectivity and probability of precipitation compared to the satellite observations, as well as the results from the SPCAM5 COSP run. The significant differences between the two COSP runs demonstrate that it is important to take into account the sub-grid variations of cloud and precipitation when using COSP to evaluate the GCM to avoid confusing and misleading results.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

The Single Column Atmosphere Model Version 6 (SCAM6): Not a Scam but a Tool for Model Evaluation and Development

The Single Column Atmosphere Model (SCAM) is a single column model version of the Community Atmosphere Model (CAM). Here we describe the functionality and features of SCAM6, available as part of CAM6 in the Community Earth System Model, version 2 (CESM2). SCAM6 features a wide selection of standard cases, as well as the ability to easily configure a case specified by the user based on a particular point in a CAM 3-D simulation. This work illustrates how SCAM6 reproduces CAM6 results for physical parameterizations, mostly of moisture and clouds. We demonstrate how SCAM6 can be used for model development through different physics selections, as well as with parameter sweep experiments to highlight the sensitivity of cloud properties to the specification of the vapor deposition process in the cloud microphysics. Furthermore, we use SCAM6 to illustrate the sensitivity of CAM6 cloud radiative properties and precipitation to variable drop number (cloud microphysics properties). Finally, we illustrate how SCAM6 can be used to explore critical emergent processes such as cloud feedbacks and show that CAM6 cloud responses to surface warming in stratus and stratocumulus regimes are similar to those in CAM5. CAM6 has a larger response in the shallow cumulus regime than CAM5. CAM6 cloud feedbacks in the shallow cumulus regime are sensitive to turbulence parameters. SCAM6 is thus a valuable tool for model development, evaluation, and scientific analy sis and an important part of the model hierarchy in Community Earth System Model, version 2.

58 GEOSCIENCES↗
DOE OSTI2016

Site Scientist for the North Slope of Alaska Site

Under this grant our team contributed scientific support to the Department of Energy Atmospheric Radiation Program’s (DOE-ARM) Infrastructure team to maintain high quality research data at the DOE-ARM North Slope of Alaska with special emphasis on the radars. Under our guidance two major field campaigns focusing on mixed-phase Arctic clouds were conducted that greatly increased the community’s understanding of the many processes working together to control the evolution of single-layer cloud mixed-phase clouds. A series of modeling and observational studies revealed that the longevity of the radiatively important liquid phase is strongly dependent on how the ice phase develops in mixed-phase clouds. A new ice microphysics parameterization was developed to capture better the natural evolution of ice particle growth in evolving environments. An ice particle scattering database was developed for all ARM radar frequencies. This database was used in a radar simulator (Doppler spectrum and polarimetric variables) to aid in the interpretation of the advanced ARM radars. At the conclusion of this project our team was poised to develop a complete radar simulator consistent with the new microphysical parameterization, taking advantage of parameterization’s advanced characterization of the ice shape and ice density.

47 OTHER INSTRUMENTATION↗
DOE OSTI2018

Deep Convection: Onset, Diurnal Cycle, and Role in Climate Variability and Sensitivity (Final Report)

The ASR SGP testbed for continuous modeling offers new opportunities to improve GCM parameterizations. We conducted an ASR investigation of convective and cloud microphysical processes that used existing ARM data as a testing ground for meaningful approaches to model evaluation and set the stage for later strategic use of the testbed to improve cumulus parameterizations and better understand deep convective cloud feedback. Our research consisted of the following tasks: Diurnal cycle of continental convection Deep convection at the SGP occurs in two forms: Organized mesoscale convection that originates upstream and produces peak precipitation at night; and local shallow convection that develops into deep convection that peaks in late afternoon. Local transitions are a logical next step from the shallow convection that will be the early focus of the testbed. This transition constrains entrainment and cold pools, since GCMs produce a continental rain peak near noon. We studied ARSCL-observed transition cases using the WRF, determined the sources of SCM diurnal cycle errors and made parameterization changes as appropriate. Factors controlling convective detrainment and anvil evolution Convective detrainment is a major source of high cloud ice water content and cloud forcing. The GISS GCM diagnoses a convective updraft speed profile, assumes a particle size distribution (PSD), and uses size-fallspeed relations to determine the fraction of condensate carried upward vs. precipitating. We used SCM case studies for TWP-ICE and MC3E for which vertical velocity has been retrieved to test whether entrainment improvements produce realistic updraft speeds and then improved the updraft microphysics parameterization. We compared detrained ice water contents and fall speeds to ARM and other field experiment data to refine the GCM’s fall speed and PSD assumptions. Role of convective cloud radiative processes in the Madden-Julian Oscillation (MJO) Changes in entrainment and rain evaporation and a cold pool parameterization have produced an MJO in the GISS GCM for the first time and allowed us to reproduce the KAZR dependence of convection depth on humidity during AMIE-Gan. We determined whether recent model changes including cold pools improve or degrade the MJO and made adjustments accordingly.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Contribution of feldspar and marine organic aerosols to global ice nucleating particle concentrations

Ice-nucleating particles (INPs) are known to affect the amount of ice in mixed-phase clouds, thereby influencing many of their properties. The atmospheric INP concentration changes by orders of magnitude from terrestrial to marine environments, which typically contain much lower concentrations. Many modelling studies use parameterizations for heterogeneous ice nucleation and cloud ice processes that do not account for this difference because they were developed based on INP measurements made predominantly in terrestrial environments without considering the aerosol composition. Errors in the assumed INP concentration will influence the simulated amount of ice in mixed-phase clouds, leading to errors in top-of-atmosphere radiative flux and ultimately the climate sensitivity of the model. Here we develop a global model of INP concentrations relevant for mixed-phase clouds based on laboratory and field measurements of ice nucleation by K-feldspar (an ice-active component of desert dust) and marine organic aerosols (from sea spray). The simulated global distribution of INP concentrations based on these two species agrees much better with currently available ambient measurements than when INP concentrations are assumed to depend only on temperature or particle size. Underestimation of INP concentrations in some terrestrial locations may be due to the neglect of INPs from other terrestrial sources. Our model indicates that, on a monthly average basis, desert dusts dominate the contribution to the INP population over much of the world, but marine organics become increasingly important over remote oceans and they dominate over the Southern Ocean. However, day-to-day variability is important. Because desert dust aerosol tends to be sporadic, marine organic aerosols dominate the INP population on many days per month over much of the mid- and high-latitude Northern Hemisphere. This study advances our understanding of which aerosol species need to be included in order to adequately describe the global and regional distribution of INPs in models, which will guide ice nucleation researchers on where to focus future laboratory and field work.

Vergara-Temprado, Jesús (ORCID:0000000231050946)↗
DOE OSTI2021

Mixed‐Phase Clouds Over the Southern Ocean as Observed From Satellite and Surface Based Lidar and Radar

Abstract This study investigates the occurrence of mixed‐phase clouds (MPC, i.e., cloud layers containing both liquid and ice water at sub‐freezing temperatures) over the Southern Ocean (SO) using space‐ and surface‐based lidar and radar observations. The occurrence of supercooled clouds is dominated by geometrically thin (<1 km) layers that rarely contain ice. We diagnose layers that are geometrically thicker than 1 km to contain ice ~65% and ~4% of the time from below by surface remote sensors and from above by orbiting remote sensors, respectively. We examine the discrepancy in MPC occurrence statistics as diagnosed from below and above the cloud layer. From above, we find that MPC occurrence has a gradient associated with the Antarctic Polar Front near 55°S with a rare occurrence of satellite‐derived MPC south of that latitude. In contrast, surface sensors find ice in 33% of supercooled liquid water layers. We infer using observing system simulation experiments and data analysis that space‐based lidar cannot identify the occurrence of MPC except when secondary ice‐forming processes operate in convection that is, sufficiently strong to loft ice crystals to cloud tops. We conclude that the CALIPSO phase statistics of MPC have a severe low bias in MPC occurrence. Based on surface‐based statistics in the SO, we present a parameterization of the frequency of MPC as a function of cloud top temperature that differs substantially from that used in recent climate model simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Final DOE-ASR Report for the Project “Advancing our Understanding and the Remote Sensing of Ice Clouds”

This project has evolved during its execution, and what follows are the key project findings. This project has arguably provided the first global view of how cirrus cloud (defined as having cloud base temperature T < 235 K) nucleation physics (evaluated through satellite retrievals of ice particle number concentration Ni, effective diameter De and ice water content IWC) evolves with the seasons for a given temperature, latitude zone and surface type (e.g. ocean vs. land), based on a new satellite remote sensing method developed for this project. The retrieval method is unique in that it is very sensitive to the small ice crystals that govern the number concentration Ni, allowing Ni to be retrieved. The method currently samples single-layer cirrus clouds having visible optical depth ranging from about 0.3 to 3.0, using co-located observations from the Infrared Imaging Radiometer (IIR) and from the CALIOP (Cloud and Aerosol Lidar with Orthogonal Polarization) lidar aboard the CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) polar orbiting satellite, employing IIR channels at 10.6 μm and 12.05 μm. Retrievals of Ni are primarily used to estimate the cirrus cloud formation mechanism; that is, either homo- or heterogeneous ice nucleation (henceforth hom and het). This is possible since, in general, hom produces more than an order of magnitude more ice crystals than does het. Thus the retrievals provide insight on how these mechanisms change with the seasons for a given latitude zone or region, based on the years 2008 and 2013. Using a conservative criterion for hom cirrus, on average, the sampled cirrus clouds formed through hom occur about 43% of the time in the Arctic and 50% of the time in the Antarctic, and during winter at mid-latitudes in the Northern Hemisphere, hom cirrus occur 37% of the time. Elsewhere (and during other seasons in the Northern Hemisphere mid-latitudes), this hom cirrus fraction is lower, and it is lowest in the tropics. Thus, the microphysical properties of cirrus clouds in the Polar Regions are much different than they are in the tropics; something unknown prior to this study. Moreover, the frequency of cirrus cloud occurrence in the Polar Regions varies strongly with season, peaking during winter in the Arctic and during spring in the Antarctic. Considering these seasonal changes in microphysics and inferred cloud coverage, this leads us to speculate that the buildup of Arctic cirrus during winter may significantly contribute to tropospheric heating in that region, possibly affecting winter jet-stream dynamics and mid-latitude weather patterns through the thermal-wind balance relationship. This cirrus cloud research provides essential guidance for realistically representing cirrus clouds in climate models; guidance previously unavailable. For example, mid-latitude hom cirrus were widespread during winter over or nearby mountainous terrain, evidently due to mountain-induced waves that produce strong updrafts at cirrus cloud levels. The treatment of turbulent mountain stress and gravity waves will likely need to be improved in climate models in order to adequately represent cirrus clouds outside the tropics. Another goal of this project was to develop a ground-based 94-GHz radar retrieval for winter snowstorms, based on (1) an improved analytical framework describing the interaction of radiation from radar with snowfall and (2) the development of a steady-state snow growth model that predicts the height-evolution of the ice particle size distribution through ice particle growth by vapor diffusion, aggregation and riming (i.e. the growth of snow through collisions with supercooled cloud droplets). Although activities (1) and (2) were completed, there was insufficient time to test and finalize the radar retrieval scheme. However, activity (2) provided a new method for relating ice particle mass “m” and projected area “A” to the ice particle maximum dimension “D”. The ice cloud microphysical processes (which determine ice cloud radiative properties) in climate models are parameterized in terms of these m-D and A-D relationships. By improving these relationships, the ice cloud radiative properties in Community Atmosphere Model version 5, or CAM5 (an atmosphere global climate model, or GCM) were improved. Student funding from the University of Nevada, Reno, was combined with funds from this project to conduct some basic research on the mechanism of the North American monsoon, or NAM. Federal research on the NAM has dwindled since 2006, but atmospheric soundings taken during research vessel cruises in the Gulf of California (GC) during the North American Monsoon Experiment (NAME) were used to reveal a likely mechanism that explains the relationship between an intrusion of tropical warm water into the GC during late spring-early summer and the onset of relatively heavy NAM rainfall in northwest Mexico and the southwestern United States. These soundings, combined with reanalysis data, satellite sea surface temperatures and satellite measurements of outgoing longwave radiation were used to develop and provide evidence for a planetary-scale NAM mechanism. As far as we know, no other physical explanation has been offered for the spring-summer evolution of the NAM system.

54 ENVIRONMENTAL SCIENCES↗