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All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Understanding Changes in Cloud Simulations from E3SM Version 1 to Version 2

This study documents clouds simulated by the Energy Exascale Earth System Model (E3SM) version 2 (E3SMv2) and attempts to understand what causes the model behavior change in clouds relative to E3SMv1. This is done by analyzing the last 30-year (1985–2014) data from the 165-year historical simulations using E3SMv1 and v2 and four sensitivity tests to isolate the impact of changes in model parameter choices in its turbulence, shallow convection, and cloud macrophysics parameterization (CLUBB), microphysical parameterization (MG2), and deep convection scheme (ZM), as well as model physics changes in convective triggering. It is shown that E3SMv2 significantly improves the simulation of subtropical coastal stratocumulus clouds (Sc) and clouds with optical depth larger than 3.6 over the stratocumulus to cumulus transition regimes, where Shortwave Cloud Radiative Effect (SWCRE) is also improved, and the Southern Ocean (SO) while seeing an overall slight degradation in low clouds over other tropical and subtropical oceans. The better performance in E3SMv1 over those regions is partially due to error compensation between its simulated optically thin and intermediate low clouds for which E3SMv2 actually improves simulation of optically intermediate low clouds. Sensitivity tests indicate that the changes in low clouds are primarily due to the tuning made in CLUBB. The impact of the ZM tuning is mainly on optically intermediate and thick high clouds, contributing to improved SWCRE and Longwave Cloud Radiative Effect (LWCRE). The impact of the MG2 tuning and the new convective trigger is primarily on the high latitudes and the Southern Ocean (SO). They have a relatively smaller impact on clouds than do the CLUBB and ZM tunings. This study offers additional insights about clouds simulated in E3SMv2 by utilizing multiple data sets and the COSP diagnostic tool as well as through sensitivity tests. The improved understanding will benefit the future E3SM developments.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Understanding changes in cloud simulations from E3SM version 1 to version 2

Abstract. This study documents clouds simulated by the Energy Exascale Earth System Model (E3SM) version 2 (E3SMv2) and attempts to understand what causes the model behavior change in clouds relative to E3SMv1. This is done by analyzing the last 30-year (1985–2014) data from the 165-year historical simulations using E3SMv1 and v2 and four sensitivity tests to isolate the impact of changes in model parameter choices in its turbulence, shallow convection, and cloud macrophysics parameterization (Cloud Layers Unified By Binormals, CLUBB); microphysical parameterization (MG2); and deep-convection scheme (ZM), as well as model physics changes in convective triggering. It is shown that E3SMv2 significantly improves the simulation of subtropical coastal stratocumulus clouds and clouds with optical depth larger than 3.6 over the stratocumulus-to-cumulus transition regimes, where the shortwave cloud radiative effect (SWCRE) is also improved, and the Southern Ocean (SO) while seeing an overall slight degradation in low clouds over other tropical and subtropical oceans. The better performance in E3SMv1 over those regions is partially due to error compensation between its simulated optically thin and intermediate low clouds for which E3SMv2 actually improves simulation of optically intermediate low clouds. Sensitivity tests indicate that the changes in low clouds are primarily due to the tuning done in CLUBB. The impact of the ZM tuning is mainly on optically intermediate and thick high clouds, contributing to an improved SWCRE and longwave cloud radiative effect (LWCRE). The impact of the MG2 tuning and the new convective trigger is primarily on the high latitudes and the SO. They have a relatively smaller impact on clouds than CLUBB tuning and ZM tuning do. This study offers additional insights into clouds simulated in E3SMv2 by utilizing multiple data sets and the Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP) diagnostic tool as well as sensitivity tests. The improved understanding will benefit future E3SM developments.

58 GEOSCIENCES↗
NASA NTRS1983

Observation of El Chichon volcanic aerosols by the solar backscattered ultraviolet (SBUV) experiment

The Solar Backscatter Ultraviolet Experiment (SBUV) aboard the Nimbus-7 satellite identified large amounts of SO2 in the tropical stratosphere on April 15, 1982, 11 days after major eruption of the El Chichon volcano in southern Mexico. It is shown in the present study that the backscattered ultraviolet radiances measured by the SBUV experiment have been strongly affected by the presence of stratospheric volcanic cloud from the El Chichon eruptions. Both SO2 and aerosol amounts present in the volcanic cloud have been mapped on the basis of an analysis of the radiances measured by the SBUV and TOMS (Total Ozone Mapping Spectrometer) experiments. It is estimated that a volcanic cloud of optical depths as small as 0.03 can be detected using SBUV, provided the cloud reaches the middle atmosphere. Lower-altitude clouds have progressively smaller effects on the radiances as well as on the ozone profile derived from them and are therefore harder to detect.

Bhartia, P. K.↗
NASA NTRS1989

Studies of radiative effects for polar stratospheric clouds

Data from the Antarctic Ozone Experiment of 1987 are used to model the radiative effects of polar stratospheric clouds. Heating and cooling rates are examined, showing that the heating and/or cooling rates within a polar stratospheric cloud depend on particle size, composition, optical depth of the cloud, solar angle, and temperature profile. The rates for an optically thin Type I cloud are too small to drive vertical motions in the stratosphere, while optically thin Type II clouds cause a stratospheric cooling.

Kinne, S.↗
NASA NTRS2018

Retrievals of Cloud Droplet Size from the Research Scanning Polarimeter Data: Validation Using In Situ Measurements

We present comparisons of cloud droplet size distributions (DSDs) retrieved from the research scanning polarimeter (RSP) data with correlative in situ measurements made during the North Atlantic Aerosols and Marine Ecosystems Study (NAAMES). The airborne portion of this field experiment was based out of St. John's airport, Newfoundland, Canada with the focus of this paper being on the deployment in May - June 2016. RSP was onboard the NASA C-130 aircraft together with an array of in situ and other remote sensing instrumentation. The RSP is an along-track scanner measuring the polarized and total reflectance in 9 spectral channels. Its uniquely high angular resolution allows for characterization of liquid water droplet sizes using the rainbow structure observed in the polarized reflectance over the scattering angle range from 135 to 165.degrees The rainbow is dominated by single scattering of light by cloud droplets, so its structure is characteristic specifically of the droplet sizes at cloud top (within unit optical depth into the cloud, equivalent to approximately 50m). A parametric fitting algorithm applied to the polarized reflectance provides retrievals of the droplet effective radius and variance assuming a prescribed size distribution shape (gamma distribution). In addition to this, we use a non-parametric method, the Rainbow Fourier Transform (RFT), which allows us to retrieve the droplet size distribution itself. The latter is important in the case of clouds with complex microphysical structure, or multiple layers of cloud, which result in multi-modal DSDs. During NAAMES the aircraft performed a number of flight patterns specifically designed for comparisons between remote sensing retrievals and in situ measurements. These patterns consisted of two flight segments above the same straight ground track. One of these segments was flown above clouds allowing for remote sensing measurements, while the other was near the cloud top where cloud droplets were sampled. We compare the DSDs retrieved from the RSP data with in situ measurements made by the Cloud Droplet Probe (CDP). The comparisons generally show good agreement (better than 1 micron for effective radius and in most cases better than 0.02 for effective variance) with deviations explainable by the position of the aircraft within the cloud, or by the presence of additional cloud layers between the cloud being sampled by the in situ instrumentation and the altitude of the remote sensing segment. In the latter case, the multi-modal DSDs retrieved from the RSP data were consistent with the multi-layer cloud structures observed in the correlative High Spectral Resolution Lidar (HSRL) profiles. The results of these comparisons provide a rare validation of polarimetric droplet size retrieval techniques, demonstrating their accuracy and robustness and the potential of satellite data of this kind on a global scale.

Remote Sensing↗
NASA NTRS1993

A regional analysis of cloudy mean spherical albedo over the marine stratocumulus region and the tropical Atlantic Ocean

Since clouds are the largest variable in Earth's radiation budget, it is critical to determine both the spatial and temporal characteristics of their radiative properties. The relationships between cloud properties and cloud fraction are studied in order to supplement grid scale parameterizations. The satellite data used is from three hourly ISCCP (International Satellite Cloud Climatology Project) and monthly ERBE (Earth Radiation Budget Experiment) data on a 2.5 deg x 2.5 deg latitude-longitude grid. Mean cloud spherical albedo, the mean optical depth distribution, and cloud fraction are examined and compared off the coast of California and the mid-tropical Atlantic for July 1987 and 1988. Individual grid boxes and spatial averages over several grid boxes are correlated to Coakley's theory of reflection for uniform and broken layered cloud and to Kedem, et al.'s findings that rainfall volume and fractional area of rain in convective systems is linear. Kedem's hypothesis can be expressed in terms of cloud properties. That is, the total volume of liquid in a box is a linear function of cloud fraction. Results for the marine stratocumulus regime indicate that albedo is often invariant for cloud fractions of 20% to 80%. Coakley's satellite model of small and large clouds with cores (1 km) and edges (100 m) is consistent with this observation. The cores maintain high liquid water concentrations and large droplets while the edges contain low liquid water concentrations and small droplets. Large clouds are just a collection of cores. The mean optical depth (TAU) distributions support the above observation with TAU values of 3.55 to 9.38 favored across all cloud fractions. From these results, a method based upon Kedem, et al's theory is proposed to separate the cloud fraction and liquid water path (LWP) calculations in a general circulation model (GCM). In terms of spatial averaging, a linear relationship between albedo and cloud fraction is observed. For tropical locations outside the Intertropical Convergence Zone (ITCZ), results of cloud fraction and albedo spatial averaging followed that of the stratus boxes containing few overcast scenes. Both the ideas of Coakley and Kedem, et al. apply. Within the ITCZ, the grid boxes tended to have the same statistical properties as stratus boxes containing many overcast scenes. Because different dynamical forcing mechanisms are present, it is difficult to devise a method for determining subgrid scale variations. Neither of the theories proposed by Kedem, et al. or Coakley works well for the boxes with numerous overcast scenes.

Ginger, Kathryn M.↗
NASA NTRS1993

A Regional Analysis of Cloudy Mean Spherical Albedo over the Marine Stratocumulus Region and the Tropical Atlantic Ocean

Since clouds are the largest variable in Earth's radiation budget, it is critical to determine both the spatial and temporal characteristics of their radiative properties. This study examines the relationships between cloud properties and cloud fraction in order to supplement grid scale parameterizations. The satellite data used in this study is from three hourly ISCCP (International Satellite Cloud Climatology Project) and monthly ERBE (Earth Radiation Budget Experiment) data on a 2.50 x 2.50 latitude-longitude grid. Mean cloud spherical albedo, the mean optical depth distribution and cloud fraction are examined and compared off the coast of California and the mid-tropical Atlantic for July 1987 and 1988. Individual grid boxes and spatial averages over several grid boxes are correlated to Coakleys (1991) theory of reflection for uniform and broken layered cloud and to Kedem, et al.(1990) findings that rainfall volume and fractional area of rain in convective systems is linear. Kedem's hypothesis can be expressed in terms of cloud properties. That is, the total volume of liquid in a box is a linear function of cloud fraction. Results for the marine stratocumulus regime indicate that albedo is often invariant for cloud fractions of 20% to 80%. Coakley's satellite model of small and large clouds with cores (1 km) and edges (100 in) is consistent with this observation. The cores maintain high liquid water concentrations and large droplets while the edges contain low liquid water concentrations and small droplets. Large clouds are just a collection of cores. The mean optical depth (TAU) distributions support the above observation with TAU values of 3.55 to 9.38 favored across all cloud fractions. From these results, a method based upon Kedem, et al. theory is proposed to separate the cloud fraction and liquid water path (LWP) calculations in a general circulation model (GCM). In terms of spatial averaging, a linear relationship between albedo and cloud fraction is observed. For tropical locations outside the Intertropical Convergence Zone (ITCZ), results of cloud fraction and albedo spatial averaging followed that of the stratus boxes containing few overcast scenes. Both the ideas of Coakley and Kedem, et al. apply. Within the ITCZ, the grid boxes tended to have the same statistical properties as stratus boxes containing many overcast scenes. Because different dynamical forcing mechanisms are present, it is difficult to devise a method for determining subgrid scale variations. Neither of the theories proposed by Kedem, et al. or Coakley works well for the boxes with numerous overcast scenes.

Ginger, Kathryn M.↗
NASA NTRS1987

Thermodynamic constraint on the cloud liquid water feedback in climate models

The cloud liquid water feedback in climate models consists of the increase (decrease) in optical depth of clouds resulting from higher (lower) liquid water contents that might accompany tropospheric warming (cooling). The change in cloud liquid water with temperature is shown to depend on the rate of change of the slope of the moist adiabat with respect to temperature, and it is a strong function of temperature. The value of this rate of change in the tropics is about half that in mid and high latitudes and is much less than the value obtained by assuming that liquid water scales with the saturation mixing ratio.

Betts, Alan K.↗
NASA NTRS1995

Considerations for modeling thin cirrus effects via brightness temperature differences

Brightness temperature difference (BTD) values are calculated for selected Geostationary Operational Environmental Satellite (GOES-6) channels (3.9, 12.7 micrometer) and Advanced Very High Resolution Radiometer channels (3.7, 12.0 micrometer). Daytime and nighttime discrimination of particle size information is possible given the infrared cloud extinction optical depth and the BTD value. BTD values are presented and compared for cirrus clouds composed of equivalent ice spheres (volume, surface area) versus randomly oriented hexagonal ice crystals. The effect of the hexagonal ice crystals is to increase the magnitude of the BTD values calculated relative to equivalent ice sphere (volume, surface area) BTDs. Equivalent spheres (volume or surface area) do not do a very good job of modeling hexagonal ice crystal effects on BTDs; however, the use of composite spheres improves the simulation and offers interesting prospects. Careful consideration of the number of Legendre polynomial coefficients used to fit the scattering phase functions is crucial to realistic modeling of cirrus BTDs. Surface and view-angle effects are incorporated to provide more realistic simulation.

Schmidt, E. O.↗
DOE OSTI2015

Sunphotometer (00)

The Cimel sunphotometer (CSPHOT) is a multi-channel, automatic sun-and-sky scanning radiometer that measures the direct solar irradiance and sky radiance at the Earth’s surface. It takes measurements at predetermined discrete wavelengths in the visible and near-infrared parts of the spectrum to determine atmospheric transmission and scattering properties. The CSPHOT only operates during daylight (sun above horizon).

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2008

An Observational Study of the Relationship between Cloud, Aerosol and Meteorology in Broken Low-Level Cloud Conditions

Global satellite analyses showing strong correlations between aerosol optical depth and 3 cloud cover have stirred much debate recently. While it is tempting to interpret the results as evidence of aerosol enhancement of cloud cover, other factors such as the influence of meteorology on both the aerosol and cloud distributions can also play a role, as both aerosols and clouds depend upon local meteorology. This study uses satellite observations to examine aerosol-cloud relationships for broken low-level cloud regions off the coast of Africa. The analysis approach minimizes the influence of large-scale meteorology by restricting the spatial and temporal domains in which the aerosol and cloud properties are compared. While distributions of several meteorological variables within 5deg 5deg latitude-longitude regions are nearly identical under low and high aerosol optical depth, the corresponding distributions of single-layer low cloud properties and top-of-atmosphere radiative fluxes differ markedly, consistent with earlier studies showing increased cloud cover with aerosol optical depth. Furthermore, fine-mode fraction and Angstrom Exponent are also larger in conditions of higher aerosol optical depth, even though no evidence of systematic latitudinal or longitudinal gradients between the low and high aerosol optical depth populations are observed. When the analysis is repeated for all 5deg 5deg latitude-longitude regions over the global oceans (after removing cases in which significant meteorological differences are found between the low and high aerosol populations), results are qualitatively similar to those off the coast of Africa.

Loeb, Norman G.↗
DOE OSTI2015

Cold and warm atomic gas around the Perseus molecular cloud. II. The impact of high optical depth on the HI column density distribution and its implication for the HI-TO-H{sub 2} transition

We investigate the impact of high optical depth on the HI saturation observed in the Perseus molecular cloud by using Arecibo HI emission and absorption measurements toward 26 radio continuum sources. The spin temperature and optical depth of individual HI components are derived along each line of sight, enabling us to estimate the correction for high optical depth. We examine two different methods for the correction, Gaussian decomposition and isothermal methods, and find that they are consistent (maximum correction factor ∼1.2), likely due to the relatively low optical depth and insignificant contribution from the diffuse radio continuum emission for Perseus. We apply the correction to the optically thin HI column density on a pixel-by-pixel basis and find that the total HI mass increases by ∼10%. Using the corrected HI column density image and far-infrared data from the IRIS Survey, we then derive the H{sub 2} column density on ∼0.4 pc scales. For five dark and star-forming sub-regions, the HI surface density is uniform with Σ{sub HI} ∼ 7–9 M{sub ⊙} pc{sup −2}, in agreement with the minimum HI surface density required for shielding H{sub 2} against photodissociation. As a result, Σ{sub H{sub 2}}/Σ{sub HI} and Σ{sub HI}+Σ{sub H{sub 2}} show a tight relation. Our results are consistent with predictions for H{sub 2} formation in steady state and chemical equilibrium and suggest that H{sub 2} formation is mainly responsible for the Σ{sub HI} saturation in Perseus. We also compare the optically thick HI with the observed “CO-dark” gas and find that the optically thick HI only accounts for ∼20% of the “CO-dark” gas in Perseus.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2001

Cloud Overlapping Detection Algorithm Using Solar and IR Wavelengths With GOSE Data Over ARM/SGP Site

One of the most perplexing problems in satellite cloud remote sensing is the overlapping of cloud layers. Although most techniques assume a 1-layer cloud system in a given retrieval of cloud properties, many observations are affected by radiation from more than one cloud layer. As such, cloud overlap can cause errors in the retrieval of many properties including cloud height, optical depth, phase, and particle size. A variety of methods have been developed to identify overlapped clouds in a given satellite imager pixel. Baum el al. (1995) used CO2 slicing and a spatial coherence method to demonstrate a possible analysis method for nighttime detection of multilayered clouds. Jin and Rossow (1997) also used a multispectral CO2 slicing technique for a global analysis of overlapped cloud amount. Lin et al. (1999) used a combination infrared, visible, and microwave data to detect overlapped clouds over water. Recently, Baum and Spinhirne (2000) proposed 1.6 and 11 microns. bispectral threshold method. While all of these methods have made progress in solving this stubborn problem, none have yet proven satisfactory for continuous and consistent monitoring of multilayer cloud systems. It is clear that detection of overlapping clouds from passive instruments such as satellite radiometers is in an immature stage of development and requires additional research. Overlapped cloud systems also affect the retrievals of cloud properties over the ARM domains (e.g., Minnis et al 1998) and hence should identified as accurately as possible. To reach this goal, it is necessary to determine which information can be exploited for detecting multilayered clouds from operational meteorological satellite data used by ARM. This paper examines the potential information available in spectral data available on the Geostationary Operational Environmental Satellite (GOES) imager and the NOAA Advanced Very High Resolution Radiometer (AVHRR) used over the ARM SGP and NSA sites to study the capability of detecting overlapping clouds

Kawamoto, Kazuaki↗
NASA NTRS2001

Cloud Overlapping Detection Algorithm Using Solar and IR Wavelengths with GOES Data Over ARM/SGP Site

One of the most perplexing problems in satellite cloud remote sensing is the overlapping of cloud layers. Although most techniques assume a one layer cloud system in a given retrieval of cloud properties, many observations are affected by radiation from more than one cloud layer. As such, cloud overlap can cause errors in the retrieval of many properties including cloud height, optical depth, phase, and particle size. A variety of methods have been developed to identify overlapped clouds in a given satellite imager pixel. Baum et al used CO2 slicing and a spatial coherence method to demonstrate a possible analysis method for nighttime detection of multilayered clouds. Jin and Rossow also used a multispectral CO2 slicing technique for a global analysis of overlapped cloud amount. Lin et al. used a combination infrared (IR), visible (VIS), and microwave data to detect overlapped clouds over water. Recently, Baum and Spinhirne proposed a 1.6 and 11 micron bispectral threshold method. While all of these methods have made progress in solving this stubborn problem none have yet proven satisfactory for continuous and consistent monitoring of multilayer cloud systems. It is clear that detection of overlapping clouds from passive instruments such as satellite radiometers is in an immature stage of development and requires additional research. Overlapped cloud systems also affect the retrievals of cloud properties over the Atmospheric Radiation Measurement (ARM) domains and hence should be identified as accurately as possible. To reach this goal, it is necessary to determine which information can be exploited for detecting multilayered clouds from operational meteorological satellite data used by ARM. This paper examines the potential information available in spectral data available on the Geostationary Operational Environmental Satellite (GOES) imager and the National Oceanic Atmospheric Administration (NOAA) Advanced Very High Resolution Radiometer (AVHRR) used over the ARM Program's Southern Great Plains (SGP), and North Slope of Alaska (NSA) sites to study the capability of detecting overlapping clouds.

Kawamoto, K.↗
NASA NTRS1978

Properties of the clouds of Venus, as inferred from airborne observations of its near-infrared reflectivity spectrum

The shape and absolute value of Venus' reflectivity spectrum is measured in the 1.2- to 4.0 micrometer spectral region with a circular variable filter wheel spectrometer having a spectral resolution of 1.5%. Comparing these spectra with synthetic spectra generated with a multiple-scattering computer code, a number of properties of the Venus clouds are inferred. Evidence is obtained indicating that the clouds are made of a water solution of sulfuric acid in their top unit optical depth, and that the clouds are made of this material down to an optical depth of at least 25. In addition, the acid concentration is 84 plus or minus 2% H2SO4 by weight in the top unit optical depth, the total optical depth of the clouds is 37.5 plus or minus 12.5, and the cross-sectional weighted mean particle radius lies between 0.5 and 1.4 micrometers in the top unit optical depth of the clouds. It is found that the average volume mixing ratio of H2SO4 and H2O contained in the cloud material both equal approximately 2 x 10 to the -6. Employing vapor pressure arguments, the acid concentration is shown to equal 84 plus or minus 6% at the cloud bottom and the water vapor mixing ratio beneath the clouds lies between 6 x 10 to the -4 and 10 to the -2.

Pollack, J. B.↗
NASA NTRSDate not supplied

Ice-Over-Water Cloud Identification in an Artificial Neural Network Approach

An artificial neural network (ANN) algorithm, employing several Aqua MODIS channels, the retrieved cloud phase and total cloud visible optical depth, and temperature and humidity vertical profiles is trained to detect multilayer (ML) ice-over-water cloud systems identified by matched 2008 CloudSat and CALIPSO (CC) data. The trained MLANN was applied to 2009 MODIS data resulting in combined ML and single layer detection accuracies of 87% (89%) and 86% (89%) for snow-free (snow-covered) regions during the day and night, respectively. When corrected for the viewing-zenith-angle dependence of each parameter, the ML fraction detected is relatively invariant across the swath. Compared to the CC ML variability, the MLANN is robust seasonally and interannually, and produces similar distribution patterns over the globe, except in the polar regions. Additional research is needed to conclusively evaluate the VZA dependence and further improve the MLANN accuracy. This approach should greatly improve the monitoring of cloud vertical structure using operational passive sensors.

MODIS↗
NASA NTRS1986

UV albedo of clouds from TOMS data

The Pilot Climate Data System (PCDS) was found to be useful in examining a subset of data from the Nimbus-7 Total Ozone Mapping Spectrometer (TOMS). The TOMS instrument scans with six channels between .3 and .4 micrometers. It was suggested that by analyzing albedo values from the longer wavelength channels of the TOMS, the effects of increasing optical depth could be determined. It is spectral relationship of albedo-to-optical depth that is investigated here. The question can be stated: Is there spectral differentiation in albedo with changes in the optical depth of clouds? Nimbus-7 TOMS data were obtained through the PCDS for an area and time period for which correlative NOAA AVHRR data were available. The AVHRR data were important in determining the existing cloud patterns. As expected, no spectral differentiation was observed at very high albedos (associated with high optical depths). However, at lower optical depths, evidence of spectral dependence on albedo was observed. Mapping the results geographically was deemed highly desirable but was not possible through the PCDS at the time. The PCDS can be viewed as an effective research tool to access selected portions of data. Without being intimately familiar with a data set, a PCDS user can successfully manipulate data in a scientific study.

Short, D.↗
DOE OSTI2019

Radiative cooling resource maps for the contiguous United States

Passive cooling devices take advantage of the partially transparent properties of the atmosphere in the longwave spectral band from 8 to 13 μ m (the so-called “atmospheric window”) to reject radiation to outer space. Spectrally designed thermophotonic devices have raised substantial attention recently for their potential to provide passive and carbon-free alternatives to air conditioning. However, the level of transparency of the atmospheric window depends on the local content of water vapor in the atmosphere and on the optical depth of clouds in the local sky. Thus, the radiative cooling capacity of solar reflectors not only depends on the optical properties of their surfaces but also on local meteorological conditions. In this work, detailed radiative cooling resource maps for the contiguous United States are presented with the goal of determining the best climates for large-scale deployment of passive radiative cooling technologies. The passive cooling potential is estimated based on ideal optical properties, i.e., zero shortwave absorptance (maximum reflectance) and blackbody longwave emittance. Both annual and season-averaged maps are presented. Daytime and nighttime cooling potential are also computed and compared. The annual average cooling potential over the contiguous United States is 50.5 m -2 . The southwestern United States has the highest annual averaged cooling potential, over 70 W m -2 , due to its dry and mostly clear sky meteorological conditions. The southeastern United States has the lowest potential, around 30 W m -2 , due to frequent humid and/or overcast weather conditions. In the spring and fall months, the Arizona and New Mexico climates provide the highest passive cooling potential, while in the summer months, Nevada and Utah exhibit higher potentials. Passive radiative cooling is primarily effective in the western United States, while it is mostly ineffective in humid and overcast climates elsewhere.

Thermo optic effects↗