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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18
All sourcesNASA NTRSDOE OSTI
NASA NTRS1995

Application of non-coherent Doppler data types for deep space navigation

Recent improvements in computational capability and Deep Space Network technology have renewed interest in examining the possibility of using one-way Doppler data alone to navigate interplanetary spacecraft. The one-way data can be formulated as the standard differenced-count Doppler or as phase measurements, and the data can be received at a single station or differenced if obtained simultaneously at two stations. A covariance analysis is performed which analyzes the accuracy obtainable by combinations of one-way Doppler data and compared with similar results using standard two-way Doppler and range. The sample interplanetary trajectory used was that of the Mars Pathfinder mission to Mars. It is shown that differenced one-way data is capable of determining the angular position of the spacecraft to fairly high accuracy, but has relatively poor sensitivity to the range. When combined with single station data, the position dispersions are roughly an order of magnitude larger in range and comparable in angular position as compared to dispersions obtained with standard data two-way types. It was also found that the phase formulation is less sensitive to data weight variations and data coverage than the differenced-count Doppler formulation.

Bhaskaran, Shyam↗
NASA NTRS1995

Application of Non-Coherent Doppler Data Types for Deep Space Navigation

improvements in computational capability and DSN technology have renewed interest in examining the possibility of using one-way Doppler data alone to navigate interplanetary spacecraft. The one-way data can be formulated as the standard difference-count Doppler or as phase measurements, and the data can be received at a single station or differenced if obtained simultaneously at two stations. A covariance analysis is performed which analyzes the accuracy obtainable by combinations of one-way Doppler data and compared with similar results using standard tow-way Doppler and range. The sample interplanetary trajectory used was that of the Mars Pathfinder mission to Mars. It is shown that differenced one-way data is capable of determining the angular position of the spacecraft to fairly high accuracy, but has relatively poor sensitivity to the range. When combined with single station data, the position dispersions are roughly an order of magnitude larger in range and comparable in angular position as compared to dispersions obtained with standard data two-way types. It was also found that the phase formulation is less sensitive to data weight variations and data coverage than the differenced-count Doppler formulation.

Deep↗
NASA NTRS1995

The application of noncoherent Doppler data types for Deep Space Navigation

Recent improvements in computational capability and DSN technology have renewed interest in examining the possibility of using one-way Doppler data alone to navigate interplanetary spacecraft. The one-way data can be formulated as the standard differenced-count Doppler or as phase measurements, and the data can be received at a single station or differenced if obtained simultaneously at two stations. A covariance analysis, which analyzes the accuracy obtainable by combinations of one-way Doppler data, is performed and compared with similar results using standard two-way Doppler and range. The sample interplanetary trajectory used was that of the Mars Pathfinder mission to Mars. It is shown that differenced one-way data are capable of determining the angular position of the spacecraft to fairly high accuracy, but have relatively poor sensitivity to the range. When combined with single-station data, the position dispersions are roughly an order of magnitude larger in range and comparable in angular position as compared to dispersions obtained with standard two-way data types. It was also found that the phase formulation is less sensitive to data weight variations and data coverage than the differenced-count Doppler formulation.

Bhaskaran, S.↗
DOE OSTI2021

Modeling impurity concentrations in liquid argon detectors

Impurities in noble liquid detectors used for neutrino and dark matter experiments can significantly impact the quality of data. We present an experimentally verified model for describing the dynamics of impurity distributions in liquid argon (LAr) detectors. The model considers sources, sinks, and transport of impurities within and between the gas and liquid argon phases. Measurements of oxygen concentrations in a 20-L LAr multi-purpose test stand are compared to calculations made with this model to show that an accurate description of the concentrations under various operational conditions can be obtained. A result of this analysis is a determination of Henry’s coefficient for oxygen in LAr. Additionally, these calculations also show that some processes have small effects on the impurity dynamics and excluding them yields a solution as a sum of two exponential terms. This solution provides a simple way to extract Henry’s coefficient with negligible approximation error. It is applied to the data and the Henry’s coefficient for oxygen in LAr is obtained as 0.84 +0.09 -0.05 , consistent with literature results. Finally, based on the analysis of the data with the model, we further suggest that, for a large liquid argon detector, barriers to flow (“baffles”) installed in the gas phase to restrict flow can help reduce the ultimate impurity concentration in the LAr.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1992

A Gaussian measure of quantum phase noise

We study the width of the semiclassical phase distribution of a quantum state in its dependence on the average number of photons (m) in this state. As a measure of phase noise, we choose the width, delta phi, of the best Gaussian approximation to the dominant peak of this probability curve. For a coherent state, this width decreases with the square root of (m), whereas for a truncated phase state it decreases linearly with increasing (m). For an optimal phase state, delta phi decreases exponentially but so does the area caught underneath the peak: all the probability is stored in the broad wings of the distribution.

Schleich, Wolfgang P.↗
NASA NTRSDate not supplied

Autonomous Navigation of a Lunar Relay Using GNSS and Other Measurements

Many of the highest priority destinations at the Moon lack a continuous view of Earth, such as the lunar poles or lunar far side. Exploration of these sites will require spacecraft in cislunar space to relay communications and provide position, navigation, and timing (PNT) services. Accurate knowledge of relay position, velocity, and time is essential to these services. This paper describes a concept for a PNT Instrument being developed for the Lunar Communications Relay and Navigation Systems (LCRNS) Project. The instrument is intended as a payload that would enable autonomous, on-board, real-time navigation and timing using Global Navigation Satellite System (GNSS), optical navigation, and one-way measurements from Earth-based ground stations. Hardware-in-the-loop simulations using flight software are used to realistically characterize performance on hardware platforms with a path to flight. These results provide preliminary validation of the proposed PNT Instrument, demonstrate the benefits of augmenting GNSS with other measurements, and serve as an insightful reference for the design of future lunar missions, including those that will operate within the LunaNet framework of standards. This instrument concept relies on several technologies developed at NASA Goddard Space Flight Center (GSFC). For GNSS observables, the instrument relies on the high-altitude NavCube 3 mini (NC3m) GNSS receiver specifically designed for cislunar applications. The autoNGC system, which consists of flight software and a hardware platform, is responsible for fusing the observables using its extended Kalman filter, the Goddard Enhanced Onboard Navigation System (GEONS). Optical navigation observables are processed within autoNGC (“autonomous Navigation, Guidance, and Control”) using the Goddard Image Analysis & Navigation Tool (GIANT) which is also responsible for simulating high-fidelity images for test and analysis. In addition to describing the PNT Instrument and its components, the paper will present predicted performance based on simulation results. As a baseline, it will present GNSS-only hardware-in-the loop results using a NC3m test unit to process Spirent-simulated GPS signals in a potential lunar relay trajectory: a 12-hour elliptical frozen lunar orbit (ELFO). GEONS then processes the GPS pseudorange and time differenced carrier phase measurements to estimate and propagate the relay state (position, velocity, and time). These results extend previously published work that showed preliminary ELFO performance. Previous work has shown the importance of other measurement types, so additional simulations are performed which augment GNSS with ground station observables and several methods of optical navigation, including celestial navigation, limb-finding (e.g., observations of the lunar horizon), and terrain relative navigation (TRN). TRN involves correlating simulated predicted images of the lunar surface with actual imagery; misalignments of landmarks identified in each image are translated into relay state updates. TRN is valuable as a measurement of the relay’s state relative to the Moon, especially during GNSS outages or after maneuvers. One-way Pseudorange and Doppler measurements from Earth-based ground stations are also simulated. The full set of observables is processed using autoNGC. These simulations make use of autoNGC and NC3m test units, a lab atomic clock, and a pulse-per-second (PPS) generation and distribution system. This combination of subsystems, and the hardware platforms used in this analysis, represents a PNT Instrument that could be flown on a lunar relay. Results from the hardware-in-the-loop simulations presented in this paper provide a preliminary assessment of the achievable navigation performance of this instrument concept. PNT Instrument performance is compared to the GPS-only performance, and a discussion is provided on the apparent merits and challenges of each measurement type.

Ben Ashman↗
DOE OSTI2022

Single-shot measurement of longitudinal phase space beam profile in an electron storage ring

A novel scheme to measure the longitudinal emittance and phase space profile in an electron storage ring by using correlations between time and the vertical coordinate, and between energy and the horizontal coordinate, is proposed. This longitudinal profile measurement scheme will help to demonstrate recent results of advanced studies for manipulating the longitudinal beam profile and for investigating beam instability in an electron storage ring.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1987

Analysis of counting errors in the phase/Doppler particle analyzer

NASA is investigating the application of the Phase Doppler measurement technique to provide improved drop sizing and liquid water content measurements in icing research. The magnitude of counting errors were analyzed because these errors contribute to inaccurate liquid water content measurements. The Phase Doppler Particle Analyzer counting errors due to data transfer losses and coincidence losses were analyzed for data input rates from 10 samples/sec to 70,000 samples/sec. Coincidence losses were calculated by determining the Poisson probability of having more than one event occurring during the droplet signal time. The magnitude of the coincidence loss can be determined, and for less than a 15 percent loss, corrections can be made. The data transfer losses were estimated for representative data transfer rates. With direct memory access enabled, data transfer losses are less than 5 percent for input rates below 2000 samples/sec. With direct memory access disabled losses exceeded 20 percent at a rate of 50 samples/sec preventing accurate number density or mass flux measurements. The data transfer losses of a new signal processor were analyzed and found to be less than 1 percent for rates under 65,000 samples/sec.

Oldenburg, John R.↗
DOE OSTI2023

2023 American Society for Mass Spectrometry (ASMS) 71st Annual Conference on Mass Spectrometry and Allied Topics

Introduction (120 words max) Understanding metal-cluster chemistry occuring at solvent boundaries in the aqueous and organic phases has applications in environments from cellular processes to nuclear fuel reprocessing. Transport of metal ions at the boundaries from aqueous to organic phases involves forming a metal-ligand complex, and wherever the initial metal coordination environment is significantly different from the final one, the metal transitions through a series of transient species in passing from one phase to another. Here an investigation of the role of coordination in the chemistry of the transient species using gas-phase measurements that are free of solvent effects to better understand the binding of complexes of metals with triphenylphosphine chalcogenide ligands, examining metal-ligand homo- and hetero-dimers to better understand transient species. Methods (120 word max) Mass spectrometry and collision induced dissociation (CID) experiments were performed with a Bruker (Billerica, MA, USA) micrOTOF-Q II quadrupole time-of-flight mass spectrometer (QTOF) and Bruker amaZon speed ETD (ion trap). High resolution/high mass accuracy spectra were generated using the QTOF. External calibration was performed with Agilent (Santa Clara, CA, USA) ESI-L Low Concentration tuning mix. Both mass spectrometers were equipped with either the electrospray ionization source or nanospray sources. Metal samples were prepared between 40 – 60 uM of the metal-ligand complex in 25% water and 75% acetonitrile. Metal-ion clusters were isolated and subjected to collision induced dissociation. Density functional theory calculations were performed. Preliminary Data or Plenary Speakers Abstract (300 words max) Metal ion clusters with triphenylphosphine chalcogenide ligands were observed for group I metals with triphenylphosphine chalcogenide samples in the mass spectrum upon electrospray ionization. For each metal ligand complex of interest, the parent ion was isolated and collision induced dissociation fragmentation spectra were acquired. We observed clusters of group I metal with triphenylphosphine oxide, triphenyl phosphine sulfide, and triphenylphosphine selenide, with homodimers and heterodimer formation. In samples where the ligands were mixed, we observed mixed sodium ligand clusters at varying amounts. These mixed ligand clusters were fragmented. Metal clusters of mixed ligand dimers containing triphenylphosphine oxide showed preferential loss of the other ligand, either triphenylphosphine sulfide or triphenyl selenide. In samples with mixed triphenylphosphine sulfide and triphenylphosphine selenium ligands, sodium bound similarly between the ligands, and losses were more evenly split, showing loss ratio upon CID with losses of triphenylphosphine sulfide:triphenylphosphine selenide 43:57 ratio observed on CID. These results suggest that the oxide binds significantly more strongly than either the selenium or sulfur triphenylphosphine ligand, and the sulfur and selenium ligands are more evenly bound. Calculations were performed using density functional theory to calculate likely structures and bond energies between the group I metal and the ligands. Novel Aspect Novel analysis of sodium bound dimers with chalcogenide triphenylphosphine ligands were investigated using mass spectrometry and theoretical calculations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

The Effects of Silicon and Niobium Concentration on the Solidification Behavior and Microstructure of Cast Monel Alloys

Cast Monel alloys are used in applications requiring a combination of good mechanical properties and excellent resistance to corrosion. Despite prevalent industrial use, relatively few studies have been conducted to investigate the relationships between composition, solidification behavior, and microstructure. Given that these alloys are used in the cast and welded conditions, these factors have a significant influence over the material properties. Here, in this work, microstructural characterization, electron probe microanalysis, X-ray diffraction, and differential scanning calorimetry were used to study how changes in Si and Nb concentrations affected the solidification path and microstructure of Monel alloys. It was found that increasing Nb concentration stabilized higher amounts of MC carbides and suppressed graphite formation during solidification. It was also found that the high nominal concentration and segregation of Si to the liquid led to the formation of Ni 31 Si 12 and other silicides via terminal eutectic reactions at the end of solidification. A pseudo-binary solidification diagram was constructed using experimental data and was applied to predict the mass fraction of solidified eutectic as a function of composition. The modeled microstructures were found to be in good agreement with experimentally measured phase fractions.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Wave and Particle Analysis of Z-Mode and O-Mode Emission in the Jovian Inner Magnetosphere

We report some of the most intense Z-mode and O-mode observations obtained by the Juno spacecraft while in orbit about Jupiter in a low to mid-latitude region near the inner edge of the Io torus. We have been able to estimate the density of the plasma in this region based on the lower frequency cutoff of the observed Z-mode emission. The results are compatible with the electron density measurements of the Jovian Auroral Distributions Experiment (JADE), on board the Juno spacecraft, if we account for unmeasured cold plasma. Direction-finding measurements indicate that the Z- and O-mode emission have distinct source regions. We have also used the measured phase space density of the JADE and the Jupiter energetic particle detector instruments to calculate estimated local growth rates of the observed O-mode and Z-mode emission assuming a loss cone instability and quasilinear analysis. The results suggest the emissions were observed near, but not within, a source region, and the free energy source is consistent with a loss cone. We have thus carried out the quasilinear wave analysis of the assumed remote Z- and O-mode wave growths. It is shown that the remotely generated waves, propagated through an inhomogeneous medium to the satellite location, may account for the observed wave characteristics. The importance of Z-mode in accelerating electrons in the inner Jovian magnetosphere makes these new wave mode confirmations at Jupiter of particular interest.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Water flipping and the oxygen evolution reaction on Fe 2 O 3 nanolayers

Hematite photoanodes are promising for the oxygen evolution reaction, however, their high overpotential (0.5-0.6 V) for water oxidation and limited photocurrent make them economically unviable at present. The work needed to orient dipoles at an electrode surface may be an overlooked contribution to the overpotential, especially regarding dipoles of water, the electron source in the oxygen evolution reaction (OER). Here, we employ second harmonic amplitude and phase measurements to quantify the number of net-aligned Stern layer water molecules and the work associated with water flipping, on hematite, an earth abundant OER semiconductor associated with a high overpotential. At zero applied bias, the pH-dependent potentials for Stern layer water molecule flipping exhibit Nernstian behavior. At positive applied potentials and pH 13, approximately one to two monolayers of water molecules points the oxygen atoms towards the electrode, favorable for the OER. The work associated with water flipping matches the cohesive energy of liquid water (44 kJ mol -1 ) and the OER current density is highest. This current is negligible at pH 5, where the work approaches 100 kJ mol -1 . Our findings suggest a causal relationship between the need for Stern layer water flipping and the OER overpotential, which may lead to developing strategies for decreasing the latter.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Sulfate reduction accelerates groundwater arsenic contamination even in aquifers with abundant iron oxides

Groundwater contamination by geogenic arsenic is a global problem affecting nearly 200 million people. In South and Southeast Asia, a cost-effective mitigation strategy is to use oxidized low-arsenic aquifers rather than reduced high-arsenic aquifers. Aquifers with abundant oxidized iron minerals are presumably safeguarded against immediate arsenic contamination, due to strong sorption of arsenic onto iron minerals. However, preferential pumping of low-arsenic aquifers can destabilize the boundaries between these aquifers, pulling high-arsenic water into low-arsenic aquifers. We investigate this scenario in a hybrid field-column experiment in Bangladesh where naturally high-arsenic groundwater is pumped through sediment cores from a low-arsenic aquifer, and detailed aqueous and solid-phase measurements are used to constrain reactive transport modelling. Here we show that elevated groundwater arsenic concentrations are induced by sulfate reduction and the predicted formation of highly mobile, poorly sorbing thioarsenic species. Furthermore, this process suggests that contamination of currently pristine aquifers with arsenic can occur up to over 1.5 times faster than previously thought, leading to a deterioration of urgently needed water resources.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Entangled-photon interferometry for plasmas

Subpicosecond coincidence timing from nonlocal intensity interference of entangled photons allows quantum interferometry for plasmas. Using a warm plasma dispersion relation, we correlate phase measurement sensitivity with different plasma properties or physics mechanisms over six orders of magnitude. Due to Nα (α≤−1/2) scaling with the photon number N, quantum interferometry using entangled light can probe small signals in plasmas not previously accessible. As an example, it is predicted that plasmas will induce shifts to a Gaussian dip, a well-known quantum optics phenomenon that is yet to be demonstrated for plasmas.

Wang, Zhehui (ORCID:0000000178264063)↗
DOE OSTI2020

Mechanistic aspects of plasma-enhanced catalytic methane decomposition by time-resolved operando diffuse reflectance infrared Fourier transform spectroscopy

To study mechanistic aspects of plasma-enhanced catalysis, methane is decomposed by a supported Ni catalyst assisted by an Ar/O 2 atmospheric pressure plasma jet (APPJ). Here, the time-resolved surface response of the Ni catalyst is investigated by operando diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) using various experimental settings. Catalyst temperatures of room temperature (RT) and 500 °C and nozzle-catalyst surface distances of 3, 5 and 8 mm were examined, and the amount of O 2 of the Ar/O 2 gas mixture flowing through the APPJ was either 0 or 0.5%. A synergistic effect of surface bonded C-O was observed during the exposure of the Ni catalyst to the APPJ for low oxygen operating conditions (pure Ar jet). Surface bonded C-O formed only when there was plasma present and the C-O signal was enhanced for higher catalyst temperature. When the supported Ni catalyst was subjected to the plasma-generated particle fluxes using highly oxidizing conditions, the presence of surface bonded C-O was suppressed. The plasma-catalytic CO and CO 2 production in the gas phase measured downstream mirrored the surface behavior of C-O bonds when the plasma source operating condition was changed from a low oxygen portion to a high oxygen portion at high catalyst temperature (500 °C). CH n (n =1, 2, ) species on the catalyst surface were also studied by DRIFTS, and CHn destruction was found to correlate with C-O formation. In particular, the time-resolved CH n response showed a possible conversion process of CH n to C-O when the Ni catalyst was exposed to the plasma source. This finding may indicate a plasma-mediated regeneration of the catalyst by plasma-catalyst surface interactions.

42 ENGINEERING↗
DOE OSTI2024

Variable-spectrum mode control of high poloidal beta discharges

DIII-D experiments demonstrate that high pressure, broad current profile equilibria can be accessed in the high poloidal beta regime by optimizing the MHD mode control poloidal spectrum. A novel, variable spectrum (VS) magnetic feedback scheme implemented using the DIII-D internal non-axisymmetric coils (I-coils) facilitated access to reduced internal inductance $l$ i operation above the no-wall beta limit compared with both no feedback and fixed spectrum feedback. In addition, the VS feedback helped avoid beta collapses caused by marginally unstable resistive wall mode activity. The lower and upper I-coil rows were configured in two independent feedback loops, allowing the feedback field's poloidal spectrum to vary and track changes in the plasma mode structure as the edge safety factor q 95 varied from 11 to 6 during the discharges. The q 95 dependence of the measured phase difference between the lower and upper I-coil rows during VS feedback is qualitatively compatible with ideal MHD simulations of the least-stable plasma kink mode and with plasma response simulations that included kinetic modifications to ideal MHD. The VS feedback approach is a straightforward way to improve resilience to variations in mode structure that occur as plasma parameters change. The demonstrated expansion of the operating space to lower $l$ i is expected to improve the coupling of the plasma kink mode to external fields and beneficial wall eddy currents, and is compatible with high bootstrap fraction operation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Operation modes of the KATRIN experiment Tritium Loop System using 83m Kr

The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to search for the effective electron antineutrino mass with a sensitivity of 0.2 eV (90 % C.L.). In order to achieve this goal, KATRIN measurement phases focusing on the neutrino mass search are alternated with phases of investigations of systematic effects. During these phases, metastable 83m Kr is used as a calibration source. The monoenergetic conversion electrons emitted accompanying the decay of 83m Kr allow a direct access to the starting conditions of β-electrons produced inside the windowless gaseous tritium source (WGTS) of KATRIN. To make use of 83m Kr in the WGTS, the Tritium Loop System, which provides a stable flow of tritium to the WGTS, needs to be operated in special modes. This paper focuses on the technical implementation of these modes and their performance with regard to the achievable 83m Kr-rates, gas densities, and gas compositions inside the WGTS.

47 OTHER INSTRUMENTATION↗
DOE OSTI2023

Dust from evolved stars: a pilot analysis of the AGB to PN transition

ABSTRACT We present a novel approach to address dust production by low- and intermediate-mass stars. We study the asymptotic giant branch (AGB) phase, during which the formation of dust takes place, from the perspective of post-AGB and planetary nebula (PN) evolutionary stage. Using results from stellar evolution and dust formation modelling, we interpret the spectral energy distribution of carbon-dust-rich sources currently evolving through different evolutionary phases, believed to descend from progenitors of similar mass and chemical composition. Comparing the results of different stages along the AGB to PNe transition, we can provide distinct insights on the amount of dust and gas released during the very late AGB phases. While the post-AGB traces the history of dust production back to the tip of the AGB phase, investigating the PNe is important to reconstruct the mass-loss process experienced after the last thermal pulse. The dust surrounding the post-AGB was formed soon after the tip of the AGB. The PNe dust-to-gas ratio is ∼10−3, 2.5 times smaller than what expected for the same initial mass star during the last AGB interpulse, possibly suggesting that dust might be destroyed during the PN phase. Measuring the amount of dust present in the nebula can constrain the capacity of the dust to survive the central star heating.

Dell’Agli, F. (ORCID:0000000324426981)↗