Polyethylene glycol as a robust, biocompatible encapsulant for two-stage treatment of food and beverage wastewater
Polyethylene glycol beads encapsulating anaerobic microbes developed for on-site food and beverage wastewater treatment.
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Polyethylene glycol beads encapsulating anaerobic microbes developed for on-site food and beverage wastewater treatment.
Genome-wide association studies (GWAS) at biobank scale are computationally intensive, especially for admixed populations requiring robust statistical models. SAIGE is a widely used method for generalized linear mixed-model GWAS but is limited by its CPU-based implementation, making phenome-wide association studies impractical for many research groups. We developed SAIGE-GPU, a GPU-accelerated version of SAIGE that replaces CPU-intensive matrix operations with GPU-optimized kernels. The core innovation is distributing genetic relationship matrix calculations across GPUs and communication layers. Applied to 2068 phenotypes from 635 969 participants in the Million Veteran Program, including diverse and admixed populations, SAIGE-GPU achieved a 5-fold speedup in mixed model fitting on supercomputing infrastructure and cloud platforms. We further optimized the variant association testing step through multi-core and multi-trait parallelization. Deployed on Google Cloud Platform and Azure, the method provided substantial cost and time savings. Source code and binaries are available for download at https://github.com/saigegit/SAIGE/tree/SAIGE-GPU-1.3.3. A code snapshot is archived at Zenodo for reproducibility (DOI: [10.5281/zenodo.17642591]). SAIGE-GPU is available in a containerized format for use across HPC and cloud environments and is implemented in R/C++ and runs on Linux systems.
This study investigated the effects of increasing concentrations of minor components on simulated Hanford low-activity waste (LAW) glass properties to allow for LAW glass composition envelope expansion. A test matrix of ten glasses was generated by spiking three previously studied simulated Hanford LAW glass compositions with increasing concentrations of minor component mixes up to a total concentration of 2 wt%. In this study, the ten glasses were fabricated, and key properties were measured including crystal formation after canister centerline cooling (CCC), crystallinity as a function of temperature, density, viscosity, electrical conductivity, glass durability using the Vapor Hydration Test (VHT), product consistency using the Product Consistency Test (PCT), and sulfur solubility. The data from these tests are presented in this report.
The project used a multi-disciplinary approach to test test if 2° materials, added to traditional cermet components, enhanced SOFC mechanical strength, anode resilience and durability when subjected to electrochemical and environmental redox cycling. Findings from fracture testing, electrochemical studies and operando Raman spectroscopy measurements demonstrated that aluminum titanate (Al 2 TiO 5 or ALT) mechanically mixed with NiO-YSZ cermets confers superior mechanical strength and slower degradation rates under polarization. No deleterious effects from ALT in conversion efficiency were observed. Specific accomplishments included the following: (1) Refined methods used to fabricate ALT enhanced anodes into bi-layer anode supports to achieve high power densities; (2) Compared the effects of adding ALT mechanically to Ni-YSZ powders prior to anode fabrication with adding ALT through infiltration and co-infiltration of YSZ scaffolds; (3) Tested the resilience of these novel materials to electrochemical and environmental redox cycling and thermal stresses commonly encountered in functioning SOFCs; and (4) Characterized the ability of ALT to improve the carbon tolerance of Ni-YSZ anodes operating with dry methane.
Tensile specimens with irradiation doses ranging from approximately 0.7 to 7.6 displacements per atom (dpa) were fabricated from 316L samples removed from Spallation Neutron Source (SNS) target vessels after service. Tensile tests were performed in conjunction with digital image correlation (DIC) characterization, which permitted detailed analysis of the strain distribution and deformation behavior of the specimen gauge sections during testing. The results show, while considerable hardening (500–700 MPa increase in yield strength) occurred in the 316L SNS target material with increasing dose, appreciable ductility (19–23% total elongation) remained in the material after irradiation to 7.6 dpa in the mixed neutron/proton environment of the SNS target region. The DIC data showed the strain distribution and deformation behavior of all irradiated specimens were nonuniform during testing. Strain localization in the form of deformation bands or “hotspots” was observed during testing, and in some specimens, the bands propagated as deformation waves along the gauge section. The “traveling wave” deformation behavior affected the amount of elongation each specimen achieved, and the scatter in the elongation data was attributed to the large variation in deformation behavior observed among different specimens. Bands of localized strain, or deformation bands, oriented at specific angles were observed in two-dimensional plots of the strain distribution in the gauge sections of some specimens. Overall, this paper describes the experimental procedures, results, and deformation behavior of tensile specimens from SNS targets after service and illustrates the value of DIC characterization during tensile testing of irradiated materials.
Experiments on the National Ignition Facility (NIF) have provided clear evidence of ablator material mixing into the Hot-Spot, leading to degraded performance. However, inferring the amount of mix and Hot-Spot conditions from typical experimental observations (e.g. x-ray spectra and images) is highly challenging. Here, we have developed an analysis method that utilizes machine learning assisted Bayesian inference to find the probability distributions of the Hot-Spot and mix conditions. This approach uses a neural network, trained on an idealized 2-dimensional representation of the Hot-Spot and mix distribution, and Bayesian inference to find the statistical distributions of Hot-Spot conditions that provide a match with observations. We have tested this method with synthetic data from simulations.
A two-truck platoon based on a prototype cooperative adaptive cruise control (CACC) system was tested on a closed test track in a variety of realistic traffic and transient operating scenarios - conditions that truck platoons are likely to face on real highways. The fuel consumption for both trucks in the platoon was measured using the SAE J1321 gravimetric procedure as well as calibrated J1939 instantaneous fuel rate, serving as proxies to evaluate the impact of aerodynamic drag reduction under constant-speed conditions. These measurements demonstrate the effects of: the presence of a multiple-passenger-vehicle pattern ahead of and adjacent to the platoon, cut-in and cut-out manoeuvres by other vehicles, transient traffic, the use of mismatched platooned vehicles (van trailer mixed with flatbed trailer), and the platoon following another truck with adaptive cruise control (ACC). These scenarios are intended to address the possibility of “background aerodynamic platooning” impacting realized savings on public roads. Using calibrated J1939 fuel rate analysis, fuel savings for curved track sections versus straight track sections were also evaluated for these scenarios, highlighting differences in the implementation of the CACC control strategies compared to a stock ACC implementation. The use of different trailer types and the presence of passenger-vehicle traffic patterns showed a measurable impact on platoon performance in some conditions, but the basic fuel savings trends were retained.
The primary objective of this project was to develop and demonstrate an integrated pilot-scale circuitry for recovering high-value rare earth elements (REEs) from coal and coal byproducts. The target performance was to produce a mixed REE product with content of at least two percent by weight on a dry mass basis in a cost-effective and environmentally benign manner. During the first nine months of the project period (Phase 2 Budget Period 2), pilot plant construction was completed including all field site startup activities such as permitting, engineering design, procurement/bidding, unit fabrication, site construction, equipment installation, module assembly, safety training, and circuit shakedown. During the remaining 21 months of project period (Phase 2 Budget Period 3), detailed field-testing activities were performed including feedstock sample collection and preparation, exploratory testing, circuit modification, detailed parametric study, and performance optimization. A detailed techno-economic analysis was performed based on the pilot plant testing findings which provided various scenarios for REE production. The project successfully accomplished the proposed target performance by producing mixed rare earth oxide (REO) with greater than 90% purity by weight in a continuous pilot scale operation from two distinctly different coarse refuse materials (i.e., West Kentucky No. 13 and Fire Clay coal seams), and at least three secondary sources (i.e., heap leach process and naturally formed acid mine drainage system). Project partners included the University of Kentucky, Virginia Tech, West Virginia University, Alliance Coal, Blackhawk Mining, Mineral Refining Company, and Mineral Separation Technologies. The pilot scale test facility was constructed at a former mining complex owned by Alliance Natural Resource Partners (Alliance Coal). The site was rehabilitated to accommodate the equipment installation, construction and fabrication, electrical power requirement, water line management and containment. The process units constructed and installed included X-ray sorting unit, crushing and grinding unit, physical separation unit, acid leaching unit, solvent extraction unit, and wastewater management unit. A rare earth mineral concentration unit was constructed as a standalone unit for flexible operation. A detailed environmental assessment and control plan was carried out to identify and quantify any potential impacts of the pilot-scale processing circuitry on the human and eco-system health and well-being. Corresponding mitigation strategies and control measures were provided. A conceptual flowsheet was developed to effectively remove thorium and uranium from high purity rare earth oxide mix or any potential radionuclide enriched stream. The two distinct feedstock materials were secured from the Blackhawk Mining Complex in eastern Kentucky where the Fire Clay (Hazard No. 4) seam is processed. The West Kentucky No. 13 (Baker) coarse refuse material was collected from an active process stream at an Alliance coal preparation plant located in western Kentucky. Characterization analysis indicated that both of feed materials generated from the two sources contained >300 ppm of TREEs on a dry whole mass basis which met the requirements for a qualified feed stock. The two feedstocks were further upgraded using a dual x-ray sorter to prepare the feed material for hydrometallurgical circuit. Thermal treatment on feed material prior to leaching was found to: 1) improve the leaching recovery of REEs, 2) increase the leaching kinetics, and 3) allow the leaching reaction to occur at lower acidity. Roasting at 600°C was selected as the pre-treatment condition for both West Kentucky No. 13 and Fire Clay coarse refuse material. Over 40% of leaching recovery was achieved by roasting West Kentucky No. 13 material having a top particle size of 3 mm in the pilot scale operation using 1.2M sulfuric acid leaching at 75OC. Initial pilot scale testing involved continuous operation of the pilot plant for 94 hours. The leaching unit was operated at solid-to-liquid ratio of 1 to 10 (w/v) using 0.5M sulfuric acid solution at a temperature of 75°C. The continuous solvent extraction circuit utilized rougher and cleaner units with DEHPA and TBP as the extractants. An innovative stripping circuit was developed to accumulate the REE concentration in the stripping solution to a level above 600 ppm. A bleed stream from the recycled strip solution was treated using oxalic acid precipitation which produced a high grade rare earth oxalate. The oxalate product was roasted to remove the oxalate which produced a rare earth oxide product having a purity greater 90%. Due to high concentrations of contaminant ions in the pregnant leach solution (PLS), a modified flowsheet was developed that involved pre-concentration of the REEs using multiple stages of precipitation and redissolution. The advantage of this process was improved removal of contamination before the downstream purification process and a significant cost reduction relative to the circuit that utilized the solvent extraction process. The modified circuitry included processes involving leaching, multistage precipitation, redissolution, and oxalate precipitation followed by roasting of the oxalate product. The circuit produced a mixed REO that was 92.96% pure from the initial test. A detailed parametric test plan was carried out which involved varying key parameters including solids feed rate, acid flowrate, acid concentration, multistage precipitation pH, redissolution pH, oxalate precipitation dosage and pH. The response variables included REE recovery, contaminant recovery, REO product grade and overall chemical consumption. Test results indicated that the acid-to-solid ratio is the key parameter to leaching efficiency as performance deteriorated with an increase in solids concentration. The optimal pH determined for REE precipitation and redissolution was 6.5 and 2.5, respectively. Additional tests were conducted to further improve the flowsheet. Recirculating a portion of the PLS to the feed of the leach tanks improved the leaching performance by lowering the pH of the leaching system and reducing the contamination recovery by shortening the residence time. Moreover, the removal of Al prior to REE precipitation significantly reduced the oxalic acid consumption in the oxalate precipitation circuit. The modified circuit produced over 90% grade REO by weight from both West Kentucky No. 13 and Fire Clay coarse refuse material in pilot scale continuous test programs. A case analysis model was developed to project the REE and major contaminants concentration in each PLS stream based on the leaching condition, pH cut point, and oxalic acid dosage. A correlation was established using empirical and semi-empirical models. Using the models, chemical consumption required for each stage was predicted based on the projected performance of the hydrometallurgy circuit. After identifying the optimum conditions, validation tests were carried out for the treatment of both West Kentucky No. 13 and Fire Clay coarse refuse materials in the pilot plant. The actual circuit performance and chemical consumptions were very close to the model predictions. Other than the two coarse refuse sources, several secondary feedstocks were also tested in the pilot plant facility. A “heap leach” system was constructed using the coarse refuse material generated from cleaning the West Kentucky No. 13 seam coal. Using the two stage SX rougher and cleaner circuit, a concentrate with a grade >90% REO was produced while recovering >97% of the REEs from the heap leach PLS. Naturally generated acid mine drainage (AMD) from West Kentucky No.13 mine was processed using the multistage precipitation circuit in the pilot plant in a test conducted for a period of 32 hours. The final grade of the mix RE oxide produced from the AMD was 90.84% with an overall circuit recovery of 64%. The primary source of REE was the selective precipitation steps involving iron and aluminum rejection. The hydrophobic-hydrophilic separation (HHS) process was proven to effectively recover coal from fine waste materials. For REM recovery, the HHS process was able to produce concentrates at grades of approximately 1.8% REE on an ash basis; however, recovery values were typically low, <10%, under the optimal conditions determined in the laboratory-scale testing. Staged testing of the pilot-scale HHS process for coal recovery and semi-continuous laboratory testing for REM testing showed that a total concentration ratio of more than 15x was observed for the REM recovery process. A circuit simulation package was developed for REE extraction and purification using a spreadsheet-based platform (Microsoft Excel). The REESim circuit simulation package is configured to track the mass and volume flows of components passing through a series of unit operations specified and configured by the user. The mass rates can then be utilized by the user to determine important performance indicators such as product mass yields, concentrate purity levels, element-by-element recoveries, and so forth. The techno-economic analysis showed that the roasting and leaching operations were the most expensive capital items, each contributing approximately 30% to the total capital cost. One notable contributor to the high production costs was the low REE recovery observed in the pilot scale trials. The product basket price was shown to have a strong influence on the economic viability of the scenarios, with the scandium price being the most significant influencer. Operating cost was shown to be extremely sensitive to REE recovery, REE feed grade, and leaching acid consumption. An analysis of ten different scenarios for a 500 t/h commercial operation revealed that three were economically favorable, producing internal rates of return varying from 27.7% to 33.1% and payback periods of 4 to 5 years. The project successfully developed and demonstrated a process to recover REEs from coal and coal byproducts in a pilot-plant operation which consistently produced over 90% grade REO mix from varies types of feedstocks. Commercialization analysis showed that the technology readiness level successfully achieved TRL 6 at the end of the project and demonstrated the need and the potential for scaling the process to further advance the technologies toward the goal of providing a domestic supply of REEs at a commercial scale.
Groundwater in the Lost Lake Aquifer Zone (LLAZ) in the Southern Sector of the M-Area Hazardous Waste management Facility (HWMF) is contaminated with chlorinated ethenes, including trichloroethylene (TCE) and tetrachloroethylene (PCE). Treatment of contaminated groundwater with humic acid is being evaluated as a potential corrective action for these volatile organic compounds (VOCs) in the LLAZ in Southern Sector (SRNS, 2019). Pilot scale injections of Huma-K brand humic acid for groundwater treatment were previously performed in M-Area between 2017 and 2020 (Amidon, 2023). Groundwater was extracted from the Lost Lake Aquifer Zone (LLAZ), then a solution of humate was mixed with recovered groundwater and subsequently re-injected into the same aquifer unit. Operations of the historical humate pilot testing were discontinued in 2020 due to COVID-19 restrictions, low injection rates, and recirculation fluid spillage. No further field scale or laboratory research to investigate humate amended groundwater injection was performed at the SRS until 2024. At the request of Area Completion Projects (ACP), the Savannah River National Laboratory (SRNL) performed supplementary testing to help determine the viability of further injection of humate as a remedial option for VOCs within the LLAZ in the Southern Sector of the M-Area HWMF.
We investigate the phenomenology of a dark QCD sector interacting with the Standard Model (SM) via the electroweak (EW) portals. The portal interactions allow SM bosons, such as Z and h, or additional bosons that mix with them, to decay into dark quarks, producing dark showers. The light dark mesons are expected to be long-lived particles (LLPs), as their decays back to the SM states through the EW-portal interactions typically have macroscopic decay lengths. We focus on dark shower events initiated by various bosons at the Large Hadron Collider (LHC). The most prominent signal is the displaced decay of GeV-scale dark pions as LLPs. Current limits on dark shower signals at LHC detectors are recast from public data to provide simplified limits insensitive to UV physics details. Future limits in the high-luminosity phase and proposed auxiliary detectors are also projected. Additionally, we study the flavor-changing neutral current (FCNC) B decays into dark pions, obtaining both current and projected constraints at the LHC and other facilities. These constraints can be combined for specific models, which are illustrated in two EW-portal benchmarks: one with the heavy doublet fermion mediation and another with the Z′ mediator including a mass mixing. The collider reach shows significant potential to probe the parameter space unconstrained by EW precision tests, highlighting the necessity of dedicated LLP search strategies and facilities.
ABSTRACT Knowing the redshift of galaxies is one of the first requirements of many cosmological experiments, and as it is impossible to perform spectroscopy for every galaxy being observed, photometric redshift (photo-z) estimations are still of particular interest. Here, we investigate different deep learning methods for obtaining photo-z estimates directly from images, comparing these with ‘traditional’ machine learning algorithms which make use of magnitudes retrieved through photometry. As well as testing a convolutional neural network (CNN) and inception-module CNN, we introduce a novel mixed-input model that allows for both images and magnitude data to be used in the same model as a way of further improving the estimated redshifts. We also perform benchmarking as a way of demonstrating the performance and scalability of the different algorithms. The data used in the study comes entirely from the Sloan Digital Sky Survey (SDSS) from which 1 million galaxies were used, each having 5-filtre (ugriz) images with complete photometry and a spectroscopic redshift which was taken as the ground truth. The mixed-input inception CNN achieved a mean squared error (MSE) =0.009, which was a significant improvement ($30{{\ \rm per\ cent}}$) over the traditional random forest (RF), and the model performed even better at lower redshifts achieving a MSE = 0.0007 (a $50{{\ \rm per\ cent}}$ improvement over the RF) in the range of z < 0.3. This method could be hugely beneficial to upcoming surveys, such as Euclid and the Vera C. Rubin Observatory’s Legacy Survey of Space and Time (LSST), which will require vast numbers of photo-z estimates produced as quickly and accurately as possible.
Mixing controlled combustion of alcohol fuels has been identified as a promising technology based on their low propensity for particulate and NOx production, but the higher heats of vaporization and auto-ignition temperatures of these fuels make their direct use in diesel engine architectures a challenge. To realize the potential of alcohol-fueled combustion, a computational fluid dynamics (CFD) modeling framework is developed, validated, and exercised to identify designs that maximize engine thermal efficiency. To evaluate the use of thermal barrier coatings (TBCs), a simplified one-dimensional (1D) conjugate heat transfer (CHT) modeling framework is employed. The addition of the 1D CHT model only increases the computational expense by 15% relative to traditional approaches, yet offers more accurate heat transfer predictions over constant temperature boundary conditions. The validated model is then used to explore a range of injector orientations and piston bowl geometries. Using a design of experiments (DoE) approach, several designs were identified that improved fuel-air mixing, shortened the combustion duration, and increased thermal efficiency. The most promising design was fabricated and tested in a Caterpillar 1Y3700 single-cylinder oil test engine (SCOTE). Engine testing confirmed the findings from the CFD simulations and found that the co-optimized injector and piston bowl design yielded over 2-percentage point increase in thermal efficiency at the same equivalence ratio (0.96) and over 6-percentage point increase at the same engine load (10.1 bar indicated mean effective pressure (IMEP)), while satisfying design constraints for peak pressure and maximum pressure rise rate.
The United States Department of Energy and the European Atomic Energy Community (EURATOM) collaborate to test, evaluate, and improve the performance of the FRAM 6.1 code with various nuclear materials, especially mixed oxide (MOX) containing an isotopic blend of uranium and very high burnup plutonium. This joint effort is intended to promote effective implementation of the FRAM 6.1 code into nuclear material verification methods.
The $η$ and $η^{\prime}$ mesons are nearly unique in the particle universe since they are nearly Goldstone bosons, and their decay dynamics are strongly constrained. While earlier experiments collected samples of order $\sim 10^{9}η$, the proposed REDTOP (Rare Eta Decays To Observe Physics Beyond the Standard Model) facility targets $\mathcal{O}(10^{14})η$ and $\mathcal{O}(10^{12})η^\prime$, enabling broad searches for physics beyond the Standard Model. In this work, we present studies evaluating REDTOP sensitivity to processes that couple the Standard Model to New Physics through four portals: the Vector (dark photon), the Scalar (Higgs-mixing), the Axion-like, and the Heavy Lepton. In parallel, the proposed statistics allow precise tests of $CP$ and $T$ invariance and lepton universality and improve determinations of the $η/η'$ transition form factors, which are crucial inputs to the hadronic light-by-light contribution to the muon anomalous magnetic moment $(g-2)_μ$.
A two-truck platoon based on a prototype cooperative adaptive cruise control (CACC) system was tested on a closed test track in a variety of realistic traffic and transient operating scenarios - conditions that truck platoons are likely to face on real highways. The fuel consumption for both trucks in the platoon was measured using the SAE J1321 gravimetric procedure as well as calibrated J1939 instantaneous fuel rate, serving as proxies to evaluate the impact of aerodynamic drag reduction under constant-speed conditions. These measurements demonstrate the effects of: the presence of a multiple-passenger-vehicle pattern ahead of and adjacent to the platoon, cut-in and cut-out manoeuvres by other vehicles, transient traffic, the use of mismatched platooned vehicles (van trailer mixed with flatbed trailer), and the platoon following another truck with adaptive cruise control (ACC). These scenarios are intended to address the possibility of “background aerodynamic platooning” impacting realized savings on public roads. Using calibrated J1939 fuel rate analysis, fuel savings for curved track sections versus straight track sections were also evaluated for these scenarios, highlighting differences in the implementation of the CACC control strategies compared to a stock ACC implementation. The use of different trailer types and the presence of passenger-vehicle traffic patterns showed a measurable impact on platoon performance in some conditions, but the basic fuel savings trends were retained.
Dual-Mode Excitation, also referred to as mode-mixing, is a superposition of two fundamental pi modes in an SRF cavity. In 9-cell TESLA cavities used for the LCLSII-HE project, the two modes that are commonly excited are the pi mode (1300.2 MHz), and the 7/9 pi mode (1297.8 MHz). During vertical cavity qualification testing, only the pi mode is driven by the RF system. However, at high gradients, emitted power at the frequency of the 7/9 pi mode grows despite the RF system only powering the pi mode. When this happens, the RF power measurement system is unable to differentiate between the superimposed modes, and any data taken is invalid. The previous method of dealing with mode-mixing was to turn off power to the cavity, let both modes decay fully, then restore power. Because of the time-sensitive nature of this testing, this leads to underestimates of Q0 or any radiant field emission present in the cavity. The novel RF control solution prevents the 7/9 pi mode from being excited while not interfering with measurements of the fundamental pi mode. A second RF control system is connected to the cavity which drives the 7/9 pi mode. The loop phase for driving the 7/9 pi mode in self excited loop mode is determined then shifted by 180 degrees, thus providing a negative feedback to the undesired mode. Because this off-resonance power can be very small, on the order of milliwatts, it does not interfere with the high-power measurements of the fundamental pi mode. At Jefferson Lab, we are now able to test a cavity for the LCLSII-HE project with no problems from mode-mixing, which allows for CW processing of high-gradient multipacting and field emission.
Current operational models for nuclear cloud rise over land were developed and validated using observations from shallow-buried or surface detonations, where lofted soil quickly mixed with fission products from the detonation. These models poorly predict fallout from elevated detonations near the fallout-free height of burst (FFHOB), where interactions with the ground are limited and the mixing of fission products and lofted soil is incomplete. Fallout-free is a misnomer at this HOB, as fallout was observed in these cases, but was below the levels of concern, especially off-grounds of the nuclear test site. To correctly characterize and model fallout from detonations near the FFHOB, models must be developed which can capture the stratified nature of the particle and activity-size distributions within the cloud. Previously, it was shown that the Weather Research and Forecasting (WRF) model can accurately simulate nuclear cloud rise for airbursts with little to no ground interactions (Arthur et al., 2021). That work is expanded here by (1) using a radiation-hydrodynamics code to improve the fireball initialization in WRF, (2) further developing an aerosol package from WRF-Chem to simulate lofted soil, and (3) combining the WRF cloud rise simulations with the operational models used at the National Atmospheric Release Advisory Center (NARAC) for fallout modeling. Using this combination of codes, the Upshot-Knothole Grable detonation, which was just below the FFHOB, is simulated from seconds after detonation through cloud rise and fallout, and results are compared to historical test data. Here, the results show improved prediction of dose rate and highlight the need to correctly characterize the entrainment of material into the cloud and the subsequent mixing of fission products with entrained material.
Nucleosynthetic isotope anomalies show that the first few million years of solar system history were characterized by two distinct cosmochemical reservoirs, CC (carbonaceous chondrites and related differentiated meteorites) and NC (the terrestrial planets and all other groups of chondrites and differentiated meteorites), widely interpreted to correspond to the outer and inner solar system, respectively. At some point, however, bulk CC and NC materials became mixed, and several dynamical models offer explanations for how and when this occurred. We use xenoliths of CC materials in polymict ureilite (NC) breccias to test the applicability of such models. Polymict ureilites represent regolith on ureilitic asteroids but contain carbonaceous chondrite-like xenoliths. We present the first 54 Cr isotope data for such clasts, which, combined with oxygen and hydrogen isotopes, show that they are unique CC materials that became mixed with NC materials in these breccias. It has been suggested that such xenoliths were implanted into ureilites by outer solar system bodies migrating into the inner solar system during the gaseous disk phase ~3–5 Myr after CAI, as in the "Grand Tack" model. However, combined textural, petrologic, and spectroscopic observations suggest that they were added to ureilitic regolith at ~50–60 Myr after CAI, along with ordinary, enstatite, and Rumuruti-type chondrites, as a result of the breakup of multiple parent bodies in the asteroid belt at this time. This is consistent with models for an early instability of the giant planets. The C-type asteroids from which the xenoliths were derived were already present in inner solar system orbits.