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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18

The Mu2e Experiment at Fermilab: A Search for Lepton Flavor Violation

The Mu2e experiment at Fermilab will search for the charged lepton flavor violating process of neutrino-less μ → e coherent conversion in the field of an aluminum nucleus. About 7⋅1017 muons, provided by a dedicated muon beam line in construction at Fermilab, will be stopped in 3 years in the aluminum target. The corresponding single event sensitivity will be 2.5⋅10−17. In this presentation, a brief overview of the physics explored by the μ → e conversion will be given, followed by a description of the Mu2e experimental apparatus and the expected detector performance.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

A (S)TEM Gas Cell Holder with Localized Laser Heating for In Situ Experiments

The advent of aberration correction for transmission electron microscopy has transformed atomic resolution imaging into a nearly routine technique for structural analysis. Now an emerging frontier in electron microscopy is the development of in situ capabilities to observe reactions at atomic resolution in real time and within realistic environments. Here we present a new in situ gas cell holder that is designed for compatibility with a wide variety of sample type (i.e., dimpled 3-mm discs, standard mesh grids, various types of focused ion beam lamellae attached to half grids). Its capabilities include localized heating and precise control of the gas pressure and composition while simultaneously allowing atomic resolution imaging at ambient pressure. The results show that 0.25-nm lattice fringes are directly visible for nanoparticles imaged at ambient pressure with gas path lengths up to 20 μm. Additionally, we quantitatively demonstrate that while the attainable contrast and resolution decrease with increasing pressure and gas path length, resolutions better than 0.2 nm should be accessible at ambient pressure with gas path lengths less than the 15 μm utilized for these experiments.

aberration correction↗

Closing the Gap Between Modeling and Experiments in the Self-assembly of Biomolecules at Interfaces and in Solution

Molecular self-assembly is a powerful tool in materials design, wherein non-covalent interactions like electrostatic, hydrophobic, hydrogen bonding, and van der Waals can be exploited to produce supramolecular nanostructures that are functional and highly tunable. Biomolecules are attractive building blocks, as they are biocompatible, biodegradable and adopt a wide array of higher order structures. Moreover, naturally occurring protein systems display a manifold of structures and interactions that can be replicated in synthetic biomolecules. In this perspective, we highlight advances in multiscale simulation techniques across broad spatiotemporal scales that can aid in characterizing self-assembly of hybrid and hierarchical bionanomaterial systems, with an emphasis on physics-based simulation approaches currently employed to study biomolecules at mineral interfaces. The power of these approaches is highlighted across a few recent areas where molecular simulations have advanced our understanding of self-assembly spanning peptides to protein self-assembly. Looking forward, we discuss how in the near future emerging methods in statistical and machine learning will advance this research field in all areas from expanding the capabilities of physics-based simulation methods to enabling new analyses of high throughput experiments. These advances will pave the way for understanding the molecular recognition patterns in systems that are dictated by self-assembly - biomineralizing peptides, hierarchical peptoids, and large protein assemblies, and will aid in the development of a new synthesis science for achieving precise molecular control in materials design

Sampath, Janani↗

Modeling Pb(II) Adsorption on Mineral Surfaces: Bridging Density Functional Theory and Experiment with Thermodynamic Insights

Despite decades of work on aqueous lead (Pb) adsorption on a-Fe2O3 (hematite) and a-Al2O3 (alumina), gaps between measurements and modeling obscure molecular-level understanding. Achieving well-matched geometries between theory and experimental for mineral-water interfaces is a hurdle, as surface functional group type and distribution must be accounted for in determining mechanisms. Additionally, computational methods that can describe the substrate are often not appropriate to capture aqueous effects. Progress requires focusing on well-studied and relevant systems, such as key facets (001),(012), and (110) of hematite and alumina, and ubiquitous contaminants such as aqueous Pb. In the past, bulk-parametrized bond-valence principles were used to rationalize Pb(II) adsorption trends. These approaches can break down at surfaces, where flexible bonding environments and adsorption-induced surface relaxations play a critical role. Here, we adapt and apply a density functional theory (DFT) and thermodynamics framework, integrating DFT-calculated energies with experimental data and electrochemical principles, to predict Pb(II) adsorption. Our model results capture trends across the full set of surfaces and predict that inner-sphere Pb(II) sorption on (001) alumina varies from unfavorable to weakly favorable across a range of pH conditions. This aligns with experiment insights that Pb(II) interacts at that surface through outer-sphere interactions. Extending to Fe(II) adsorption, we demonstrate a coverage-dependent site preference, potentially explaining disorder in overlayers grown by the oxidative adsorption of Fe(II) on hematite (001).

lead contamination↗

Uptake of Uranium from Seawater by Amidoxime-Based Polymeric Adsorbent: Field Experiments, Modeling, and Updated Economic Assessment

Uranium recovery from seawater has been investigated for several decades for the purpose of securing nuclear fuel for energy production. In this study, field column experiments have been performed at the Marine Sciences Laboratory of the Pacific Northwest National Laboratory (PNNL) using a laboratory-proven, amidoxime-based polymeric adsorbent developed at the Oak Ridge National Laboratory (ORNL). The adsorbent was packed either in in-line filters or in flow-through columns. The maximum amount of uranium uptake from seawater was 3.3 mg of U/g of adsorbent after 8 weeks of contact between the adsorbent and seawater. This uranium adsorption amount was about 3 times higher than the maximum amount achieved in this study by a leading adsorbent developed at the Japan Atomic Energy Agency (JAEA).

Kim, Jungseung↗

Atmospheric River Detection Under Changing Seasonality and Mean-State Climate: ARTMIP Tier 2 Paleoclimate Experiments

Atmospheric rivers (ARs) are filamentary structures within the atmosphere that account for a substantial portion of poleward moisture transport and play an important role in Earth's hydroclimate. However, there is no one quantitative definition for what constitutes an atmospheric river, leading to uncertainty in quantifying how these systems respond to global change. This study seeks to better understand how different AR detection tools (ARDTs) respond to changes in climate states utilizing single-forcing climate model experiments under the aegis of the Atmospheric River Tracking Method Intercomparison Project (ARTMIP). We compare a simulation with an early Holocene orbital configuration and another with CO2 levels of the Last Glacial Maximum to a preindustrial control simulation to test how the ARDTs respond to changes in seasonality and mean climate state, respectively. We find good agreement among the algorithms in the AR response to the changing orbital configuration, with a poleward shift in AR frequency that tracks seasonal poleward shifts in atmospheric water vapor and zonal winds. In the low CO2 simulation, the algorithms generally agree on the sign of AR changes, but there is substantial spread in their magnitude, indicating that mean-state changes lead to larger uncertainty. This disagreement likely arises primarily from differences between algorithms in their thresholds for water vapor and its transport used for identifying ARs. These findings warrant caution in ARDT selection for paleoclimate and climate change studies in which there is a change to the mean climate state, as ARDT selection contributes substantial uncertainty in such cases.

Atmospheric river, paleoclimate↗

In-situ Experiments to Capture the Evolution of Microstructure During Phase Transformation of Titanium Under Dynamic Loading

Under sufficient stresses, such as during dynamic loading, titanium experiences a phase transformation from hcp alpha phase to hexagonal omega phase. Omega phase is often retained in the microstructure after unloading, and has a strong influence on subsequent mechanical properties. Simulations suggest there are multiple pathways and underlying mechanisms for this transformation. Due to the incredibly short timescales involved, experimental measurements for model validation have been difficult. However, new capabilities at the Advanced Photon Source have enabled diffraction measurements during plate impact experiments to study the evolution of titanium during transformation. These high-rate data allow us to probe the mechanism and kinetics of phase transformations in new ways. Recent results will be presented and compared to post-mortem characterization of soft-recovered shocked specimens. Comparisons are then made with previous tests where material was shock-loaded and soft recovered for microstructural analysis. Together these techniques create a consistent picture of material behavior during the shock-induced α–ω phase transformation in titanium.

36 MATERIALS SCIENCE↗

A Freon-Filled Bubble Chamber for Neutron Detection in Inertial Confinement Fusion Experiments

Neutron imaging is one of the main methods used in inertial confinement fusion experiments to measure the core symmetry of target implosions. Previous studies have shown that bubble chambers have the potential to obtain higher resolution images of the targets for a shorter source-to-target distance than typical scintillator arrays. A bubble chamber for neutron imaging with Freon 115 as the active medium was designed and built for the OMEGA laser system. Bubbles resulting from spontaneous nucleation were recorded. Bubbles resulting from neutron–Freon interactions were observed at neutron yields of 1013 emitted from deuterium–tritium target implosions on OMEGA. The measured column bubble density was too low for neutron imaging on OMEGA but agreed with the model of bubble formation. The recorded data suggest that neutron bubble detectors are a promising technology for the higher neutron yields expected at National Ignition Facility.

Ghilea, M C↗

Forward Drift Chamber for the GlueX Experiment at the 12 GeV CEBAF Machine

The GlueX experiment will search for exotic mesons produced by 9 GeV linearly polarized photons from the upgraded CEBAF machine. It is critical to detect and measure the four-momenta of all the charged particles and photons resulting from the decays of the mesons. The solenoid-based detector system includes tracking detectors and calorimeters. The Forward Drift Chamber, FDC, consists of 24 circular planar drift chambers of 1m diameter. Additional cathode readout is required to achieve efficient pattern recognition. The detection of photons by the electromagnetic calorimeters imposes constraints on the amount of material used in the FDC. The specific features of the detector and the readout electronics will be described. Results from the tests of the full scale prototype will be presented, as well.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Recent N* results from photoproduction experiments at CLAS

The recent breakthroughs in the technology of polarised targets have enabled a new generation of meson photo-production experiments to be carried out. A measurement of a full set of polarisation observables off both polarised proton and neutron targets and in a large number of meson-production channels has come within sight. Such a measurement would very significantly reduce model-dependence in the analysis of the data and thus has the potential to resolve long-standing issues, such as the 'missing resonance' problem, and shed new light on the nucleon excitation spectrum. This has formed the motivation for the recent N* experimental programme of CLAS.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Simulation of microtearing turbulence in national spherical torus experiment

Thermal energy confinement times in National Spherical Torus Experiment (NSTX) dimensionless parameter scans increase with decreasing collisionality. While ion thermal transport is neoclassical, the source of anomalous electron thermal transport in these discharges remains unclear, leading to considerable uncertainty when extrapolating to future spherical tokamak (ST) devices at much lower collisionality. Linear gyrokinetic simulations find microtearing modes to be unstable in high collisionality discharges. First non-linear gyrokinetic simulations of microtearing turbulence in NSTX show they can yield experimental levels of transport. Magnetic flutter is responsible for almost all the transport ({approx}98%), perturbed field line trajectories are globally stochastic, and a test particle stochastic transport model agrees to within 25% of the simulated transport. Most significantly, microtearing transport is predicted to increase with electron collisionality, consistent with the observed NSTX confinement scaling. While this suggests microtearing modes may be the source of electron thermal transport, the predictions are also very sensitive to electron temperature gradient, indicating the scaling of the instability threshold is important. In addition, microtearing turbulence is susceptible to suppression via sheared E Multiplication-Sign B flows as experimental values of E Multiplication-Sign B shear (comparable to the linear growth rates) dramatically reduce the transport below experimental values. Refinements in numerical resolution and physics model assumptions are expected to minimize the apparent discrepancy. In cases where the predicted transport is strong, calculations suggest that a proposed polarimetry diagnostic may be sensitive to the magnetic perturbations associated with the unique structure of microtearing turbulence.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

X-ray conversion efficiency in vacuum hohlraum experiments at the National Ignition Facility

X-ray fluxes measured in the first 96 and 192 beam vacuum hohlraum experiments at the National Ignition Facility (NIF) were significantly higher than predicted by computational simulations employing XSN average atom atomic physics and highly flux-limited electron heat conduction. For agreement with experimental data, it was found that the coronal plasma emissivity must be simulated with a detailed configuration accounting model that accounts for x-ray emission involving all of the significant ionization states. It was also found that an electron heat conduction flux limit of f= 0.05 is too restrictive, and that a flux limit of f= 0.15 results in a much better match with the NIF vacuum hohlraum experimental data. The combination of increased plasma emissivity and increased electron heat conduction in this new high flux hohlraum model results in a reduction in coronal plasma energy and, hence, an explanation for the high ({approx}85%-90%) x-ray conversion efficiencies observed in the 235 < T{sub r} < 345 eV NIF vacuum hohlraum experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Suppressing electron turbulence and triggering internal transport barriers with reversed magnetic shear in the National Spherical Torus Experiment

The National Spherical Torus Experiment (NSTX) [M. Ono et al., Nucl. Fusion 40, 557 (2000)] can achieve high electron plasma confinement regimes that are super-critically unstable to the electron temperature gradient driven (ETG) instability. These plasmas, dubbed electron internal transport barriers (e-ITBs), occur when the magnetic shear becomes strongly negative. Using the gyrokinetic code GYRO [J. Candy and R. E. Waltz, J. Comput. Phys. 186, 545 (2003)], the first nonlinear ETG simulations of NSTX e-ITB plasmas reinforce this observation. Local simulations identify a strongly upshifted nonlinear critical gradient for thermal transport that depends on magnetic shear. Global simulations show e-ITB formation can occur when the magnetic shear becomes strongly negative. Finally, while the ETG-driven thermal flux at the outer edge of the barrier is large enough to be experimentally relevant, the turbulence cannot propagate past the barrier into the plasma interior.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A novel approach for x-ray scattering experiments in magnetic fields utilizing trapped flux in type-II superconductors

We introduce a novel approach to x-ray scattering studies in applied magnetic fields by exploiting vortices in superconductors. This method is based on trapping magnetic flux in a small disk-shaped superconductor (known as a trapped field magnet, TFM) with a single-crystal sample mounted on or at close proximity to its surface. This opens an unrestricted optical access to the sample and allows magnetic fields to be applied precisely along the x-ray momentum transfer, facilitating polarization-sensitive experiments that have been impractical or impossible to perform to date. The TFMs used in our study remain stable and provide practically uniform magnetic fields for days, which are sufficient for comprehensive x-ray diffraction experiments, specifically x-ray resonance exchange scattering (XRES) to study field-induced phenomena at a modern synchrotron source. The TFM instrument has been used in a “proof-of-principle” XRES study of a meta-magnetic phase in a rare-earth compound, TbNi2Ge2, in order to demonstrate its potential.

36 MATERIALS SCIENCE↗

Spherical shock-ignition experiments with the 40 + 20-beam configuration on OMEGA

Spherical shock-ignition experiments on OMEGA used a novel beam configuration that separates low-intensity compression beams and high-intensity spike beams. Significant improvements in the performance of plastic-shell, D 2 implosions were observed with repointed beams. The analysis of the coupling of the high-intensity spike beam energy into the imploding capsule indicates that absorbed hot-electron energy contributes to the coupling. The backscattering of laser energy was measured to reach up to 36% at single-beam intensities of ~ 8 x 10 15 W/cm/ 2 . Hard x-ray measurements revealed a relatively low hot-electron temperature of ~30 keV independent of intensity and timing. At the highest intensity, stimulated Brillouin scattering occurs near and above the quarter-critical density and the two-plasmon-decay instability is suppressed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Copper K-shell emission cross sections for laser–solid experiments

Published measurements and models of the cross section for electrons causing K-shell emission from copper are reviewed to find a suitable expression to use when analyzing K{sub α}-emission measurements in laser–solid experiments at peak intensities above 10{sup 18} W/cm{sup 2}. Few measurements exist in the 0.1- to 10-MeV electron energy range currently of interest, leaving a number of possible suitable models that are summarized here with a number of typing errors corrected. Two different limiting forms for the cross section at relativistic energies are used, and existing measurements do not give a clear indication as to which is correct. Comparison with the limiting form of electron stopping power indicates an alternative relativistic form and also that the density-effect correction will be important in copper above 10 MeV. For data analysis relying on relative K{sub α} emission caused by electrons with energy much greater than the K-shell binding energy, the existing uncertainty in cross sections is unimportant, but it will be a source of uncertainty when using absolute values and for electron energies up to ∼6× the binding energy. K-shell emission caused by photons and protons is also briefly reviewed.

74 ATOMIC AND MOLECULAR PHYSICS↗

Heavy photon search experiment at JLAB

The Heavy Photon Search (HPS) experiment in Hall-B at Jefferson Lab will search for new heavy vector boson(s), aka 'heavy photons', in the mass range of 20 MeV/c{sup 2} to 1000 MeV/c{sup 2} using the scattering of high energy, high intensity electron beams off a high Z target. The proposed measurements will cover the region of parameter space favored by the muon g-2 anomaly, and will explore a significant region of parameter space, not only at large couplings (α′/α > 10{sup −7}), but also in the regions of small couplings, down to α′/α∼10{sup −10}. The excellent vertexing capability of the Si-tracker uniquely enables HPS to cover the small coupling region. Also, HPS will search for heavy photons in an alternative to the e{sup +}e{sup −} decay mode, in the heavy photon's decay to μ{sup +}μ−.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗