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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Bolometer tomography on Wendelstein 7-X for study of radiation asymmetry

The algorithm for bolometer tomography at Wendelstein 7-X (W7-X) has been recently improved using a novel regularization functional, based on relative gradient smoothing (RGS) of the sought radiation profile. It has been validated using radiation patterns provided by 3D modeling under real plasma conditions as phantoms and then applied to bolometer measurements performed during the first divertor operation phase of W7-X. The following results are presented: 1) edge-localized 2D radiation patterns with clearly resolved magnetic island radiation structures, 2) an up-down asymmetry in the impurity radiation that is not captured by the 3D edge plasma transport modeling, 3) reversal of the asymmetry with reversed magnetic field direction. Further analysis reveals a poloidal variation of the emissivity in the outer confined plasma region with a field-direction dependent asymmetry, also supported by the soft X-ray measurements. This asymmetry is considered to be related to asymmetric impurity distributions, driven by the pronounced ion-impurity friction force at the plasma edge where the collisionality of the W7-X plasma is sufficiently high to develop impurity asymmetry as predicted by neoclassical theory of parallel impurity transport.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Loss of energetic particles due to resistive wall mode instability in ITER

Effects of an unstable n = 1 (n is the toroidal mode number) resistive wall mode (RWM) on the energetic particle (EP) confinement and loss are numerically investigated, for an ITER steady state scenario with 10 MA plasma current and 5.3 T toroidal field. The eigenfunction of the RWM is computed, with the associated three-dimensional magnetic field perturbation superposed with the 2D equilibrium field for tracing the EP drift orbits. Considered are mono-energetic EPs at 0.5 MeV and 1 MeV for deuterium ions, and 3.5 MeV for fusion-born alphas, with a range of distribution in the particle pitch angle. Modeling finds that less than 20% of EPs can be lost to the limiting surface in ITER assuming a source distribution uniform in minor radius, due to an unstable RWM that produces 100 Gauss poloidal field perturbation at the outboard mid-plane just inside the (effective) resistive wall surface. On top of the initial prompt drift orbit loss for counter-current EPs, the RWM induced particle loss occurs on a one second time scale, which is comparable to the RWM growth time in ITER. The 'wetted' area, due to the lost EPs striking the limiting surface, is generally found to be large due to the RWM. This is a favorable prediction for ITER. Here, the loss distribution in the poloidal angle is more uniform for co-current EPs. Counter-current EPs experience outward orbit drift when launched from the low-field side, and tend to more often hit the bottom region of the limiting surface.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Synthesis, disorder and Ising anisotropy in a new spin liquid candidate PrMgAl 11 O 19

Here we report the successful synthesis of large single crystals of triangular frustrated PrMgAl 11 O 19 using the optical floating zone technique. Single crystal x-ray diffraction (XRD) measurements unveiled the presence of quenched disorder within the mirror plane, specifically ~7% of Pr ions deviating from the ideal 2d site towards the 6h site. Magnetic susceptibility measurements revealed an Ising anisotropy with the c-axis being the easy axis. Despite a large spin–spin interaction that develops below ~10 K and considerable site disorder, the spins do not order or freeze down to at least 50 mK. The availability of large single crystals offers a distinct opportunity to investigate the exotic magnetic state on a triangular lattice with an easy axis out of the plane.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Hydroxycinnamaldehyde-derived benzofuran components in lignins

Abstract Lignin is an abundant polymer in plant secondary cell walls. Prototypical lignins derive from the polymerization of monolignols (hydroxycinnamyl alcohols), mainly coniferyl and sinapyl alcohol, via combinatorial radical coupling reactions and primarily via the endwise coupling of a monomer with the phenolic end of the growing polymer. Hydroxycinnamaldehyde units have long been recognized as minor components of lignins. In plants deficient in cinnamyl alcohol dehydrogenase, the last enzyme in the monolignol biosynthesis pathway that reduces hydroxycinnamaldehydes to monolignols, chain-incorporated aldehyde unit levels are elevated. The nature and relative levels of aldehyde components in lignins can be determined from their distinct and dispersed correlations in 2D 1H–13C-correlated nuclear magnetic resonance (NMR) spectra. We recently became aware of aldehyde NMR peaks, well resolved from others, that had been overlooked. NMR of isolated low-molecular-weight oligomers from biomimetic radical coupling reactions involving coniferaldehyde revealed that the correlation peaks belonged to hydroxycinnamaldehyde-derived benzofuran moieties. Coniferaldehyde 8-5-coupling initially produces the expected phenylcoumaran structures, but the derived phenolic radicals undergo preferential disproportionation rather than radical coupling to extend the growing polymer. As a result, the hydroxycinnamaldehyde-derived phenylcoumaran units are difficult to detect in lignins, but the benzofurans are now readily observed by their distinct and dispersed correlations in the aldehyde region of NMR spectra from any lignin or monolignol dehydrogenation polymer. Hydroxycinnamaldehydes that are coupled to coniferaldehyde can be distinguished from those coupled with a generic guaiacyl end-unit. These benzofuran peaks may now be annotated and reported and their structural ramifications further studied.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2026

Charge correlations and magnetoelastic coupling in intercalated transition metal dichalcogenides

The large van der Waals gap in transition metal dichalcogenides (TMDs) offers an avenue to tune the ground state of 2D materials through the intercalation of magnetic atoms. Here, we investigate the charge correlations in Fe 1/3 ⁢TaS 2 , Co 1/3 ⁢TaS 2 , and Fe 0.35 ⁢NbS 2 by combining angle-resolved photoemission spectroscopy (ARPES), x-ray scattering, magnetometry, and density functional theory (DFT). We find that, while short-range charge fluctuations develop in Ta-based compounds, Fe 0.35 ⁢NbS 2 exhibits long-range charge order which is strongly coupled with magnetic order and tunable by external magnetic field. Our electronic structure analysis reveals that intercalation reconstructs the Fermi surface via charge transfer and band renormalization, yet does not generate the nesting conditions compatible with the observed ordering vectors. Complementary phonon calculations further exclude a conventional electron-phonon origin of charge order. Together, these results establish magnetoelastic coupling as the dominant mechanism behind charge ordering in Fe 0.35 ⁢NbS 2 and highlight the contrasting role of Nb and Ta hosts in stabilizing correlated ground states in intercalated TMDs.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Holographic Quantum Simulation of Strongly Correlated Electron Systems

The project aimed to demonstrate a new holographic quantum simulation approach and co‐ designed quantum hardware to tackle three specific problems that fall within the broad umbrella of unraveling the physics of strongly correlated electron systems (SCES). These tasks were: (1) holographic preparation of ground‐ and thermal‐ states of correlated magnetic and electronic systems including quasi‐2d frustrated‐spin, Fermi‐Hubbard, and fractional quantum Hall (FQH) systems, (2) holographic‐simulation of long‐time out‐of‐equilibrium dynamics and (3) holographic analogs of embedding methods such as dynamical mean‐ field theory (DMFT) and density‐matrix embedding theory (DMET) to solve systems with complex structure or long‐range interactions. These tasks are prototypes for the kinds of material simulation problems of interest to BES, such as the simulation of multiferroic materials, perovskite photovoltaics and high‐temperature superconductors, that tax the capabilities of the most powerful classical supercomputers.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2026

Statistical Study of Energy Dissipation in Magnetic Structures During Turbulent Reconnection in the Earth's Magnetotail

Magnetic reconnection is a ubiquitous plasma phenomenon that plays a critical role in particle heating and energization. During reconnection, the topology of magnetic field rearranges, depositing energy into the surrounding plasma through bulk flow, thermal heating, or non-thermal particle acceleration. While the pathways of this transformation from magnetic energy into kinetic have been studied extensively in recent years through theoretical or case-by-case observations, comprehensive statistical studies remain limited. In this paper, we present a statistical investigation using data from the Magnetospheric Multiscale (MMS) mission, and detail the particle energization mechanisms in magnetic structures found near reconnecting regions in turbulent Earth's magnetotail. We find that electrons with motion perpendicular to the magnetic field dominate $\vec{j}$ ⋅ $\vec{E}$ dissipation. In contrast to the conventional picture of unidirectional energy transfer to particles by laminar two-dimensional (2D) reconnection, we find that energy exchange within magnetic structures during turbulent reconnection tends to be bidirectional with only a small positive bias from electromagnetic fields to particles. Specific electron energization mechanisms are quantified, including those due to parallel electric field, Fermi energization from curvature drift, betatron heating from magnetic field inhomogeneity, and polarization drift.

Wang, Rachel [Princeton University, NJ (United Sta↗
DOE OSTI2022

Particle Acceleration in Magnetic Reconnection with Ad Hoc Pitch-angle Scattering

Particle acceleration during magnetic reconnection is a long-standing topic in space, solar, and astrophysical plasmas. Recent 3D particle-in-cell simulations of magnetic reconnection show that particles can leave flux ropes due to 3D field-line chaos, allowing particles to access additional acceleration sites, gain more energy through Fermi acceleration, and develop a power-law energy distribution. This 3D effect does not exist in traditional 2D simulations, where particles are artificially confined to magnetic islands due to their restricted motions across field lines. Full 3D simulations, however, are prohibitively expensive for most studies. Here, we attempt to reproduce 3D results in 2D simulations by introducing ad hoc pitch-angle scattering to a small fraction of the particles. We show that scattered particles are able to transport out of 2D islands and achieve more efficient Fermi acceleration, leading to a significant increase of energetic particle flux. We also study how the scattering frequency influences the nonthermal particle spectra. This study helps achieve a complete picture of particle acceleration in magnetic reconnection.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Dimensional crossover in spin Hall oscillators

Auto-oscillations of magnetization driven by direct spin current have been previously observed in multiple quasi-zero-dimensional (0D) ferromagnetic systems such as nanomagnets and nanocontacts. Recently, it was shown that pure spin Hall current can excite coherent auto-oscillatory dynamics in quasi-one-dimensional (1D) ferromagnetic nanowires but not in quasi-two-dimensional (2D) ferromagnetic films. Here we study the 1D to 2D dimensional crossover of current-driven magnetization dynamics in wire-based Pt/Ni 80 Fe 20 bilayer spin Hall oscillators via varying the wire width. We find that increasing the wire width results in an increase of the number of excited auto-oscillatory modes accompanied by a decrease of the amplitude and coherence of each mode. We also observe a crossover from a hard to a soft onset of the auto-oscillations with increasing wire width. The amplitude of auto-oscillations rapidly decreases with increasing temperature suggesting that interactions of the phase-coherent auto-oscillatory modes with incoherent thermal magnons play an important role in suppression of the auto-oscillatory dynamics. Our measurements in this work set the upper limit on the dimensions of an individual spin Hall oscillator and elucidate the mechanisms leading to suppression of coherent auto-oscillations with increasing oscillator size.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Exchange Bias Between van der Waals Materials: Tilted Magnetic States and Field-Free Spin–Orbit-Torque Switching

Magnetic van der Waals heterostructures provide a unique platform to study magnetism and spintronics device concepts in the 2D limit. Here, studies of exchange bias from the van der Waals antiferromagnet CrSBr acting on the van der Waals ferromagnet Fe3GeTe2 (FGT) are reported. Additionally, the orientation of the exchange bias is along the in-plane easy axis of CrSBr, perpendicular to the out-of-plane anisotropy of the FGT, inducing a strongly tilted magnetic configuration in the FGT. Furthermore, the in-plane exchange bias provides sufficient symmetry breaking to allow deterministic spin–orbit torque switching of the FGT in CrSBr/FGT/Pt samples at zero applied magnetic field. A minimum thickness of the CrSBr of >10 nm is needed to provide a non-zero exchange bias at 30 K.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Thermal and Quantum Melting Phase Diagrams for a Magnetic-Field-Induced Wigner Solid

A sufficiently large perpendicular magnetic field quenches the kinetic (Fermi) energy of an interacting two-dimensional (2D) system of fermions, making them susceptible to the formation of a Wigner solid (WS) phase in which the charged carriers organize themselves in a periodic array in order to minimize their Coulomb repulsion energy. In low-disorder 2D electron systems confined to modulation-doped GaAs heterostructures, signatures of a magnetic-field-induced WS appear at low temperatures and very small Landau level filling factors ($\textit{ν}$ ≃ 1/5). In dilute GaAs 2D hole systems, on the other hand, thanks to the larger hole effective mass and the ensuing Landau level mixing, the WS forms at relatively higher fillings ($\textit{ν}$ ≃ 1/3). Here we report our measurements of the fundamental temperature vs filling phase diagram for the 2D holes’ WS-liquid thermal melting. Moreover, via changing the 2D hole density, we also probe their Landau level mixing vs filling WS-liquid quantum melting phase diagram. In this work, we find our data to be in good agreement with the results of very recent calculations, although intriguing subtleties remain.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Electron and Proton Energization in 3D Reconnecting Current Sheets in Semirelativistic Plasma with Guide Magnetic Field

Abstract Using 3D particle-in-cell simulation, we characterize energy conversion, as a function of guide magnetic field, in a thin current sheet in semirelativistic plasma, with relativistic electrons and subrelativistic protons. There, magnetic reconnection, the drift-kink instability (DKI), and the flux-rope kink instability all compete and interact in their nonlinear stages to convert magnetic energy to plasma energy. We compare fully 3D simulations with 2D in two different planes to isolate reconnection and DKI effects. In zero guide field, these processes yield distinct energy conversion signatures: ions gain more energy than electrons in 2Dxy(reconnection), while the opposite is true in 2Dyz(DKI), and the 3D result falls in between. The flux-rope instability, which occurs only in 3D, allows more magnetic energy to be released than in 2D, but the rate of energy conversion in 3D tends to be lower. Increasing the guide magnetic field strongly suppresses DKI, and in all cases slows and reduces the overall amount of energy conversion; it also favors electron energization through a process by which energy is first stored in the motional electric field of flux ropes before energizing particles. Understanding the evolution of the energy partition thus provides insight into the role of various plasma processes, and is important for modeling radiation from astrophysical sources such as accreting black holes and their jets.

Astronomy & Astrophysics↗
DOE OSTI2020

Quantum Criticality in the 2D Quasiperiodic Potts Model

Quantum critical points in quasiperiodic magnets can realize new universality classes, with critical properties distinct from those of clean or disordered systems. Here, we study quantum phase transitions separating ferromagnetic and paramagnetic phases in the quasiperiodic q-state Potts model in 2+1D. Using a controlled real-space renormalization group approach, we find that the critical behavior is largely independent of q, and is controlled by an infinite-quasiperiodicity fixed point. In conclusion, the correlation length exponent is found to be ν = 1, saturating a modified version of the Harris-Luck criterion.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Distinguishing surface and bulk electromagnetism via their dynamics in an intrinsic magnetic topological insulator

The indirect exchange interaction between local magnetic moments via surface electrons has been long predicted to bolster the surface ferromagnetism in magnetic topological insulators (MTIs), which facilitates the quantum anomalous Hall effect. This unconventional effect is critical to determining the operating temperatures of future topotronic devices. However, the experimental confirmation of this mechanism remains elusive, especially in intrinsic MTIs. Here, we combine time-resolved photoemission spectroscopy with time-resolved magneto-optical Kerr effect measurements to elucidate the unique electromagnetism at the surface of an intrinsic MTI MnBi 2 Te 4 . Theoretical modeling based on 2D Ruderman-Kittel-Kasuya-Yosida interactions captures the initial quenching of a surface-rooted exchange gap within a factor of two but overestimates the bulk demagnetization by one order of magnitude. This mechanism directly explains the sizable gap in the quasi-2D electronic state and the nonzero residual magnetization in even-layer MnBi 2 Te 4 . Furthermore, it leads to efficient light-induced demagnetization comparable to state-of-the-art magnetophotonic crystals, promising an effective manipulation of magnetism and topological orders for future topotronics.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2025

Nonlinear Scaling of Water–Ion Interactions and Dynamics in Alkaline Solutions

Water-ion interactions govern many solvent properties critical to solution-phase chemistry and the behavior of liquid water. The water-ion interactions in alkaline conditions were probed using two-dimensional infrared spectroscopy (2D IR), small-angle x-ray scattering (SAXS), and nuclear magnetic resonance spectroscopy (NMR). Energy transfer between the donor molecule KSeCN, used as a 2D IR probe, and the acceptor molecule NaOD was used to track the average separation distance of ions in a D 2 O solution, while SAXS measurements showed effects in the bulk D 2 O solvent. Here, we observe consistent nonlinear scaling in the SeCN - and OD - average separation distance as a function of NaOD concentration while bulk solution D 2 O-to-D 2 O average separation distance remained highly linear. Ultrafast measurements of solution dynamics via 2D IR and polarization-selective pump-probe spectroscopy show consistent scaling in correlation times as a function of concentration. These results suggests that the SeCN - and OD - anions participate in a water-ion network that significantly reduces the degrees of freedom for the distribution of ions in solution below the standard stochastic for ion distribution.

2D IR Spectroscopy↗
DOE OSTI2020

Thermal Hall conductance and a relative topological invariant of gapped two-dimensional systems

We derive a Kubo-like formula for the thermal Hall conductance of a 2d lattice systems which is free from ambiguities associated with the definition of energy magnetization. We use it to define a relative topological invariant of gapped 2d lattice systems at zero temperature. Up to a numerical factor, it can be identified with the difference of chiral central charges for the corresponding edge modes. This establishes the bulk-boundary correspondence for the chiral central charge. Here, we also show that for any local commuting projector Hamiltonian, the relative chiral central charge vanishes, while for free fermionic systems, it is related to the zero-temperature electric Hall conductance via the Wiedemann-Franz law.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Observation of Scale Invariance in Two-Dimensional Matter-Wave Townes Solitons

We report near-deterministic generation of two-dimensional (2D) matter-wave Townes solitons, and a precision test on scale invariance in attractive 2D Boses gases. We induce a shape-controlled modulational instability in an elongated 2D matter-wave to create an array of isolated solitary waves of various sizes and peak densities. We confirm scale invariance by observing the collapse of solitary-wave density profiles onto a single curve in a dimensionless coordinate rescaled according to their peak densities, and observe that the scale-invariant profiles measured at different coupling constants can further collapse onto the universal profile of Townes solitons. The reported scaling behavior is tested with a nearly 60-fold difference in soliton interaction energies, and allows us to discuss the impact of a non-negligible magnetic dipole-dipole interaction (MDDI) on 2D scale invariance. Here, we confirm that the effect of MDDI in our alkali cesium quasi-2D samples effectively conforms to the same scaling law governed by a contact interaction to well within our experiment uncertainty.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗