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At least 307 records · Page 17

Compilation of Experimental Yield Data for Spontaneous Fission of 252 Cf

We present a comprehensive compilation and curation of experimental fission yield (FY) data for the spontaneous fission of 252 Cf, extracted from the EXFOR database. The compilation follows a structured methodology developed for prior compilations of neutron-induced fission yields, and incorporates both independent (IFY) and cumulative (CFY) yields. A total of 62 datasets were reviewed, with entries spanning from 1955 to 2021. A significant portion of the literature reports pre-neutron emission yields, which were excluded from the present compilation due to limitations in format compatibility. Each accepted dataset was processed into a standardized JSON format, including metadata, uncertainties, and bibliographic references. Where available, decay radiation information was used to update the FY data using the latest ENSDF evaluations; 237 data points were corrected accordingly. These corrections are fully traceable and preserve original values. The result is a curated dataset suitable for use in nuclear data evaluations. This work is part of an ongoing effort to modernize the handling of FY data and provide evaluators with high-quality, machine-readable experimental inputs

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

On the emission mechanism in high current hollow cathode arcs

Large hollow cathodes have been operated in a magnetoplasmadynamic arc over wide ranges of current and mass flow, with orifice current densities and mass fluxes encompassing those encountered in low current steady state hollow cathode arcs. Detailed cathode interior measurements of current and potential distributions show that maximum current penetration into the cathode is about one diameter axially upstream from the tip, with peak inner surface current attachment up to one cathode diameter upstream of the tip. The spontaneous attachment of peak current upstream of the cathode tip is suggested as a criterion for characteristic hollow cathode operation. This empirical criterion was verified by experiment.

Krishnan, M.↗

Van der Waals Nanowires with Continuously Variable Interlayer Twist and Twist Homojunctions

Abstract Moiré patterns at van der Waals interfaces between twisted 2D crystals give rise to distinct optoelectronic excitations, as well as, narrowly dispersive bands responsible for correlated electron phenomena. Contrasting with the conventional, mechanically stacked planar twist moirés, recent work shows twisted van der Waals interfaces spontaneously formed in nanowires of layered crystals, where Eshelby twist due to axial screw dislocations stabilizes a chiral structure with small interlayer rotation. Here, the realization of tunable twist in germanium(II) sulfide (GeS) van der Waals nanowires is reported. Tapered nanowires host continuously variable interlayer twist. Homojunctions between dislocated (chiral) and defect‐free (achiral) segments are obtained by triggering the emission of axial dislocations during growth. Measurements across such junctions, implemented here using local absorption and luminescence spectroscopy, provide a convenient tool for detecting twist effects. The results identify a versatile system for 3D twistronics, probing moiré physics, and for realizing moiré architectures without equivalent in planar systems.

Sutter, Peter↗

Instrumentation for correlated prompt n – γ emission studies in coincidence with fission fragments

Recent theoretical and experimental results have brought renewed interest and focus on the topic of fission fragment angular momentum. Measurements of neutrons and rays in coincidence with fission fragments remain the most valuable tool in the exploration of fission physics. To achieve these scientific goals, we have developed a system that combines a state-of-the-art fission fragment detector and n – γ radiation detectors. A new twin Frisch-gridded ionization chamber has been designed and constructed for use with a spontaneous fission source and an array of forty trans-stilbene organic scintillators (FS-3) at Argonne National Laboratory. The new ionization chamber design we present in this work aims at minimizing particle attenuation in the chamber walls, and provides a compact apparatus that can be fit inside existing experimental systems. The ionization chamber is capable of measuring fission fragment masses and kinetic energies, whereas the FS-3 provides neutron and γ-ray multiplicities and spectra. Here, the details of both detector assemblies are presented along with the first experimental results of this setup. Planned event-by-event analysis and future experiments are briefly discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Cosmological constraints on pseudo-Nambu-Goldstone bosons

Particle physics models with pseudo-Nambu-Goldstone bosons (PNGBs) are characterized by two mass scales: a global spontaneous symmetry breaking scale, f, and a soft (explicit) symmetry breaking scale, Lambda. General model insensitive constraints were studied on this 2-D parameter space arising from the cosmological and astrophysical effects of PNGBs. In particular, constraints were studied arising from vacuum misalignment and thermal production of PNGBs, topological defects, and the cosmological effects of PNGB decay products, as well as astrophysical constraints from stellar PNGB emission. Bounds on the Peccei-Quinn axion scale, 10(exp 10) GeV approx. = or less than f sub pq approx. = or less than 10(exp 10) to 10(exp 12) GeV, emerge as a special case, where the soft breaking scale is fixed at Lambda sub QCD approx. = 100 MeV.

Frieman, Joshua A.↗

Solutions to Droop and the Green Gap by Novel Carrier Injection

Long-wavelength (green, yellow, red) visible light-emitting diodes (LEDs) have historically been inefficient compared to blue light-emitters in the III-nitrides. This is due to many factors, including poor material quality due to the low growth temperatures required for high Incomposition InGaN quantum wells (QWs), and the polar nature of the III-nitride crystal structure. Spontaneous and piezoelectric polarization in the III-nitrides causes enhanced quantum-confined Stark effect (QCSE), which spatially separates electrons and holes and reduces radiative recombination (ie: light output) from the devices. Polarization in the crystal also induces additional potential barriers that electrons and holes must cross over before entering the QWs where they can recombine to emit light. Both of these polarization effects worsen as emission wavelength increases, making blue III-nitride LEDs are the most efficient and red III-nitride LEDs the least efficient. The focus of this project has been solving the latter polarization-related issue through the implementation of V-defects in long wavelength LEDs. V-defects are morphological defects which are commonly observed in c-plane III-nitrides. They are observed as hexagonal pyramid-shaped depressions on the c-plane surface, with six semipolar sidewalls. They typically form at the apex of threading dislocations (TDs) under conditions of kinetically-limited growth and low growth-temperature. They were initially thought to be detrimental to LED performance and much early work focused on eliminating them entirely from III-nitride devices. However, over the past decade work has emerged that indicate that they can improve LED performance by allowing electrons and holes to bypass the polarization-induced barriers present in the c-plane and directly enter the QWs of an LED. This is due to the semipolar nature of the V-defect sidewall: these sidewalls are thin and lack the polarization-induced barriers which prevent carriers easily moving between layers. V-defects have since been determined to be an efficient avenue by which to inject electrons and holes into the c-plane QWs where they can recombine to emit light. Throughout this project we have explored lateral injection through a variety of methods: simulation (Task 2), epitaxial growth of V-defect and non-V-defect LEDs (Tasks 1, 3, 4, 5, 6), and advanced characterization methods (Task 7). All tasks have been completed. A description of each task completed follows from this section.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Nanoflares and the solar X-ray corona

Observations of the sun with high time and spatial resolution in UV and X-rays show that the emission from small isolated magnetic bipoles is intermittent and impulsive, while the steadier emission from larger bipoles appears as the sum of many individual impulses. We refer to the basic unit of impulsive energy release as a nanoflare. The observations suggest, then, that the active X-ray corona of the sun is to be understood as a swarm of nanoflares. This interpretation suggests that the X-ray corona is created by the dissipation at the many tangential discontinuities arising spontaneously in the bipolar fields of the active regions of the sun as a consequence of random continuous motion of the footpoints of the field in the photospheric convection. The quantitative characteristics of the process are inferred from the observed coronal heat input.

Parker, E. N.↗

Dielectronic recombination rates, ionization equilibrium, and radiative emission rates for Mn ions in low-density high-temperature plasmas

The analysis of optically-thin far-ultraviolet and X-ray emission lines of multiply-charged ions is one of the basic methods for determining the temperatures and densities of laboratory and astrophysical plasmas. In addition, the energy balance in these plasmas can be significantly influenced by the emission of radiation from relatively low concentrations of multiple-charged atomic ions. Because the populations of the excited levels are expected to depart substantially from their local thermodynamic equilibrium values a detailed treatment of the elementary collisional and radiative processes must be employed in order to predict the emission line intensities. In this investigation the authors present the results of calculations based on a corona equilibrium model in which a detailed evaluation is made of the dielectronic recombination rate coefficients. The ionization and autoionization following inner-shell electron excitation from each ground state are balanced by direct radiative and dielectronic recombination. The spectral line intensities emitted by the low-lying excited states, which are assumed to undergo spontaneous radiative decay in times that are short compared with the collision time, are evaluated in terms of the corona ionization equilibrium distributions of the ground states and their electron-impact excitation states.

Jacobs, V. L.↗

NASA Numerical and Experimental Evaluation of UTRC Low Emissions Injector

Computational and experimental analyses of a PICS-Pilot-In-Can-Swirler technology injector, developed by United Technologies Research Center (UTRC) are presented. NASA has defined technology targets for near term (called "N+1", circa 2015), midterm ("N+2", circa 2020) and far term ("N+3", circa 2030) that specify realistic emissions and fuel efficiency goals for commercial aircraft. This injector has potential for application in an engine to meet the Pratt & Whitney N+3 supersonic cycle goals, or the subsonic N+2 engine cycle goals. Experimental methods were employed to investigate supersonic cruise points as well as select points of the subsonic cycle engine; cruise, approach, and idle with a slightly elevated inlet pressure. Experiments at NASA employed gas analysis and a suite of laser-based measurement techniques to characterize the combustor flow downstream from the PICS dump plane. Optical diagnostics employed for this work included Planar Laser-Induced Fluorescence of fuel for injector spray pattern and Spontaneous Raman Spectroscopy for relative species concentration of fuel and CO2. The work reported here used unheated (liquid) Jet-A fuel for all fuel circuits and cycle conditions. The initial tests performed by UTRC used vaporized Jet-A to simulate the expected supersonic cruise condition, which anticipated using fuel as a heat sink. Using the National Combustion Code a PICS-based combustor was modeled with liquid fuel at the supersonic cruise condition. All CFD models used a cubic non-linear k-epsilon turbulence wall functions model, and a semi-detailed Jet-A kinetic mechanism based on a surrogate fuel mixture. Two initial spray droplet size distribution and spray cone conditions were used: (1) an initial condition (Lefebvre) with an assumed Rosin-Rammler distribution, and 7 degree Solid Spray Cone; and (2) the Boundary Layer Stripping (BLS) primary atomization model giving the spray size distribution and directional properties. Contour and line plots are shown in comparison with experimental data (where this data is available) for flow velocities, fuel, and temperature distribution. The CFD results are consistent with experimental observations for fuel distribution and vaporization. Analysis of gas sample results, using a previously-developed NASA NOx correlation, indicates that for sea-level takeoff, the PICS configuration is predicted to deliver an EINOx value of about three for the targeted supersonic aircraft. Emissions results at supersonic cruise conditions show potential for meeting the NASA goals with liquid fuel.

Hicks, Yolanda R.↗

NASA Numerical and Experimental Evaluation of UTRC Low Emissions Injector

Computational and experimental analyses of a PICS-Pilot-In-Can-Swirler technology injector, developed by United Technologies Research Center (UTRC) are presented. NASA has defined technology targets for near term (called "N+1", circa 2015), midterm ("N+2", circa 2020) and far term ("N+3", circa 2030) that specify realistic emissions and fuel efficiency goals for commercial aircraft. This injector has potential for application in an engine to meet the Pratt & Whitney N+3 supersonic cycle goals, or the subsonic N+2 engine cycle goals. Experimental methods were employed to investigate supersonic cruise points as well as select points of the subsonic cycle engine; cruise, approach, and idle with a slightly elevated inlet pressure. Experiments at NASA employed gas analysis and a suite of laser-based measurement techniques to characterize the combustor flow downstream from the PICS dump plane. Optical diagnostics employed for this work included Planar Laser-Induced Fluorescence of fuel for injector spray pattern and Spontaneous Raman Spectroscopy for relative species concentration of fuel and CO2. The work reported here used unheated (liquid) Jet-A fuel for all fuel circuits and cycle conditions. The initial tests performed by UTRC used vaporized Jet-A to simulate the expected supersonic cruise condition, which anticipated using fuel as a heat sink. Using the National Combustion Code a PICS-based combustor was modeled with liquid fuel at the supersonic cruise condition. All CFD models used a cubic non-linear k-epsilon turbulence wall functions model, and a semi-detailed Jet-A kinetic mechanism based on a surrogate fuel mixture. Two initial spray droplet size distribution and spray cone conditions were used: 1) an initial condition (Lefebvre) with an assumed Rosin-Rammler distribution, and 7 degree Solid Spray Cone; and 2) the Boundary Layer Stripping (BLS) primary atomization model giving the spray size distribution and directional properties. Contour and line plots are shown in comparison with experimental data (where this data is available) for flow velocities, fuel, and temperature distribution. The CFD results are consistent with experimental observations for fuel distribution and vaporization. Analysis of gas sample results, using a previously-developed NASA NOx correlation, indicates that for sea-level takeoff, the PICS configuration is predicted to deliver an EINOx value of about 3 for the targeted supersonic aircraft. Emissions results at supersonic cruise conditions show potential for meeting the NASA goals with liquid fuel.

Hicks, Yolanda R.↗

Spectral characterization of an SPDC source with a fast broadband spectrometer

Knowing the properties of single photons produced in a Spontaneous Parametric Down-Conversion (SPDC) source can be crucial for specific applications and uses. In particular, the spectral properties are of key relevance. Here, we investigate a commercial SPDC source using our fast broadband spectrometer. Our analysis is a valid method for other SPDC sources, as well as other single-photon generation techniques, thus providing a good example of how to use this spectrometer design. We calibrate the spectrometer using known lines of the argon emission spectrum. We show that the two down-converted photons from the SPDC source have different spectral properties depending on the pump power, and under which condition we measured spectrally similar down-converted photons. Finally, we were able to reconstruct and investigate the spectral information for the pump photon.

79 ASTRONOMY AND ASTROPHYSICS↗

Advanced Optical Diagnostic Methods for Describing Fuel Injection and Combustion Flowfield Phenomena

Over the past decade advanced optical diagnostic techniques have evolved and matured to a point where they are now widely applied in the interrogation of high pressure combusting flows. At NASA Glenn Research Center (GRC), imaging techniques have been used successfully in on-going work to develop the next generation of commercial aircraft gas turbine combustors. This work has centered on providing a means by which researchers and designers can obtain direct visual observation and measurements of the fuel injection/mixing/combustion processes and combustor flowfield in two- and three-dimensional views at actual operational conditions. Obtaining a thorough understanding of the chemical and physical processes at the extreme operating conditions of the next generation of combustors is critical to reducing emissions and increasing fuel efficiency. To accomplish this and other tasks, the diagnostic team at GRC has designed and constructed optically accessible, high pressurer high temperature flame tubes and sectar rigs capable of optically probing the 20-60 atm flowfields of these aero-combustors. Among the techniques employed at GRC are planar laser-induced fluorescence (PLIF) for imaging molecular species as well as liquid and gaseous fuel; planar light scattering (PLS) for imaging fuel sprays and droplets; and spontaneous Raman scattering for species and temperature measurement. Using these techniques, optical measurements never before possible have been made in the actual environments of liquid fueled gas turbines. 2-D mapping of such parameters as species (e.g. OH-, NO and kerosene-based jet fuel) distribution, injector spray angle, and fuel/air distribution are just some of the measurements that are now routinely made. Optical imaging has also provided prompt feedback to researchers regarding the effects of changes in the fuel injector configuration on both combustor performance and flowfield character. Several injector design modifications and improvements have resulted from this feedback. Alternate diagnostic methods are constantly being evaluated as to their suitability as a diagnostic tool in these environments. A new method currently under examination is background oriented Schlieren (BOS) for examining the fuel/air mixing processes. While ratioing the Stokes and anti-Stokes nitrogen lines obtained from spontaneous Raman is being refined for temperature measurement. While the primary focus of the GRC diagnostic work remains optical species measurement and flow stream characterization, an increased emphasis has been placed on our involvement in flame code validation efforts. A functional combustor code should shorten and streamline future combustor design. Quantitative measurements of flow parameters such as temperature, species concentration, drop size and velocity using such methods as Raman and phase Doppler anemometry will provide data necessary in this effort.

Locke, Randy J.↗

Theoretical studies of Resonance Enhance Stimulated Raman Scattering (RESRS) of frequency doubled Alexandrite laser wavelengths in cesium vapor

It is well known that the presence of a real atomic level which is nearly resonant with the pump field can greatly enhance the Raman emission cross section. In order to accurately calculate the Raman gain in systems where resonance enhancement plays a dominant role, expressions for the pump and signal susceptibilities must be derived. These expressions should be valid for arbitrary field strengths in order to allow for pump and signal saturation. In addition, the theory should allow for arbitrary longitudinal and transverse relaxation rates. This latter point is extremely vital for three level atomic systems such as the alkali earth metals since they do not have population reservoirs and can have widely varying spontaneous lifetimes on the three pertinent transitions. Moreover, the dephasing rates are strong functions of electron states and are therefore also different for the three coupled pairs of levels. These considerations are not as important when molecular systems are concerned since the large reservoir of rotational states serve to produce essentially equal longitudinal recovery rates for the population of the three levels. The three level system with three arbitrary longitudinal and transverse relaxation rates was solved. There is no need for setting either pair of rates equal and the expressions are valid for arbitrarily strong fields.

Lawandy, N. M.↗

Optimal filtering and generation of entangled photons for quantum applications in the presence of noise

Filtering is commonly used in quantum optics to reject noise photons, and also to enable interference between independent photons. However, filtering the joint spectrum of photon pairs can reduce the inherent coincidence probability or loss-independent heralding efficiency. Here we investigate filtering for multiphoton applications based on entanglement and interference (e.g., quantum teleportation). We multiplex C-band entangled photons and C-band classical communications into the same long-distance fibers, which enables scalable low-loss quantum networking but requires filtering of spontaneous Raman scattering noise from classical light. Using tunable-bandwidth filters, low-jitter detectors, and polarization filters, we distribute wavelength-degenerate time-bin entangled photons in the C band (1536.5 nm) over 25 km/25 km standard fibers (50 km) each carrying 10 Gbit/s C-band classical data signals. Narrow filtering enables milliwatt-level C-band power, which exceeds the power achieved by comparable studies by roughly an order of magnitude and could feasibly support terabit per second classical rates. We evaluate how performance depends on pump and filter bandwidths, multipair emission, filter shapes, loss, phase matching, and how quantum information is measured. We find a trade-off between reducing noise impact and increasing single-mode purity, and discuss mitigation methods toward optimal multiphoton applications. Importantly, these results apply to noise in free space and in quantum devices (sources, frequency converters, switches, detectors, etc.) and provide insight into filter-induced degradation of single-photon purity and rates even in noise-free environments.

Thomas, Jordan M. [Fermilab; Northwestern U.]↗

The 630 nm dayglow

The daytime thermospheric emission at 630 nm from the (3P-1D) transition of atomic oxygen is examined using data from the Atmosphere Explorer C and E spacecraft. Observed altitude distributions of the emission rate measured using the Visible Airglow Experiment are compared with those calculated from in situ measurements of ion and neutral densities and temperatures, and from a model of the photon and photoelectron flux. Good agreement is obtained for most orbits with photoelectron impact on O, photodissociation of O2, and dissociative recombination of O2(+) providing most of the production. Implications for some of the controversial points of O(1D) chemistry, such as the solar EUV and Schumann-Runge continuum flux, the yield of O(1D) from the reaction of N(2D) with O2, the value of spontaneous transition coefficients, and the rate of quenching by O(3P) are discussed.

Solomon, Stanley C.↗

The X ray corona, the coronal hole, and the heliosphere

The question of why the sun heats the corona in active regions with an energy input of 10 exp 7 erg sq cm/s is addressed. It is argued that the trapped gas is heated by the intermittent dissipation of magnetic energy (nanoflares) at the current sheets that arise spontaneously in any magnetic field subject to continuous deformation. Most of the heat input is close to the sun, in the first 1-2 RS, raising the gas slowly out through the gravitational field and gradually accelerating it through the speed of sound at a distance of about 3-5 RS. The only source for the principle heat input close to the sun appears to be the network activity; thus the mass loss and the formation of the heliosphere are primarily a consequence of the smallest-scale activity supplemented by occasional flares and coronal mass ejections. The X-ray emission is largely a consequence of the smallest flares, the nanoflares, supplemented by occasional X-ray bursts from large flares.

Parker, E. N.↗

Spatial decay of electromagnetic waves from hypervelocity impact plasmas

Due to the high kinetic energy of impactors in space, hypervelocity impacts on spacecraft can ablate spacecraft material and produce plasmas. These plasmas have been observed in ground-based experiments to produce electromagnetic pulses (EMPs) and are suspected to be a cause of spacecraft anomalies. The initial EMP that is produced after plasma formation is replicated using a 2D electromagnetic plasma simulation, consisting of a discontinuous Galerkin, particle-in-cell (DG-PIC) framework. The spontaneous formation of EMPs from an initial quasineutral plasma is consistent with previous works and show behavior similar to that of waves emitted by antennas. The EMP emits from the plasma with a frequency less than the plasma frequency associated with the point of maximum density, showing the importance of the density gradient, and the far-field region of the “plasma antenna” is estimated. From the proportionality between plasma frequency and EMP frequency, there is a direct correlation between plasma density and radiation. Finally, as the plasma density decreases, the EMP frequency decreases, which suggests that several observable phenomena, such as optical flashes, radio frequency emission, and microwave emission, all result from the same plasma-related mechanism within a single hypervelocity impact.

42 ENGINEERING↗

Backscatter-Immune Injection-Locked Brillouin Laser in Silicon

As self-sustained oscillators, lasers possess the unusual ability to spontaneously synchronize. These nonlinear dynamics are the basis for a simple yet powerful stabilization technique known as injection locking, in which a laser’s frequency and phase can be controlled by an injected signal. Because of its inherent simplicity and favorable noise characteristics, injection locking has become a workhorse for coherent amplification and high-fidelity signal synthesis in applications ranging from precision atomic spectroscopy to distributed sensing. Within integrated photonics, however, these injection-locking dynamics remain relatively untapped—despite significant potential for technological and scientific impact. In this work, we demonstrate injection locking in a silicon photonic Brillouin laser. Injection locking of this monolithic device is remarkably robust, allowing us to tune the laser emission by a significant fraction of the Brillouin gain bandwidth. Harnessing these dynamics, we demonstrate amplification of small signals by more than 23 dB. Moreover, we demonstrate that the injection-locking dynamics of this system are inherently nonreciprocal, yielding unidirectional control and backscatter immunity in an all-silicon system. This device physics opens the door to strategies for phase-noise reduction, low-noise amplification, and backscatter immunity in silicon photonics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗