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NASA NTRS1983

Solar variability and quasi-stationary planetary wave behavior

A steady state analysis of winter winds shows that the speed of the upper atmospheric polar vortex approaches and occasionally exceeds the value required to reflect externally forced planetary wave 1 energy back towards the surface of the earth. Historical observations suggest that solar UV variability and geomagnetic disturbances are two primary forces which modulate the planetary wave trapping mechanism. Through the solar-terrestrial process described, small changes in the sun's behavior can be physically linked to both shortand long-term changes in tropospheric weather patterns.

Springer, B. D.↗

NASA NTRS1983

Transport and the seasonal variation of ozone

The transport mechanisms responsible for the seasonal behavior of total ozone are deduced from the comparison of model results to stratospheric data. The seasonal transport is dominated by a combination of the diabatic circulation and transient planetary wave activity acting on a diffusively and photochemically determined background state. The seasonal variation is not correctly modeled as a diffusive process. The buildup of total ozone at high latitudes during winter is dependent upon transient planetary wave activity of sufficient strength to cause the breakdown of the polar vortex. While midwinter warmings are responsible for enhanced ozone transport to high latitudes, the final warming marking the transition from zonal mean westerlies to zonal mean easterlies is the most important event leading to the spring maximum. The final warming is not followed by reacceleration of the mean flow; so that the ozone transport associated with this event is more pronounced than that associated with midwinter warmings.

Rood, R. B.↗

NASA NTRS1985

Characteristics of polar stratospheric clouds as observed by SAM II, SAGE, and lidar

Satellite and lidar data sets developed over several years of observations are analyzed to detail the macroscopic and microphysical characteristics of polar stratospheric clouds (PSCs). Mappings were made of the sizes, locations, probabilities of occurrence and temperature dependence of the PSCs, and indicated that PSCs are correlated with an extended stratospheric cloud bank in the cold polar vortex region. The bank is bounded by a 188 K isotherm, and the probability of occurrence drops to 50 percent at the 193 K isotherm. Values of 6.3 particles/cu cm and radii averaging 0.0725 micron/particle are calculated, along with an estimated downward velocity of 0.01 m/sec.

Mccormick, M. P.↗

NASA NTRS1985

Mean Winds of the Mesosphere (60-80 Km), as Measured by MF Radars

Winds data obtained from medium frequency (MF) radars for heights of 60 to 80 km are discussed: locations are Saskatoon (52 N, 107 W), Christchurch (44 S, 173 W), Adelside (35 S, 183 E) and Townsville (20 S, 147 E). Whereas well defined summer easterly jets centered near 70 km develop in summer, no regular buildups and decays are observed in winter at midlatitudes. Part of this variability can be associated with stratospheric warmings, which develop into breakdown of the polar vortex in the Northern Hemisphere. Amplitude and phase profiles of the annual and semiannual oscillations are also presented. The radar winds from Saskatoon are compared and combined with rocket derived winds up to 60 km from Primrose Lake (54 N, 110 W) to give consistent cross sections from 20 to 110 km. The SH radar winds are compared with a model based on rocket winds which extends up to 80 km. The latter evidence considerable smoothing, as no winter variability is evident. The other consistent difference is that heights of the summer easterly maxima for the model are 5 to 10 km lower than the radar winds at all latitudes.

Manson, A. H.↗

NASA NTRS1985

On the use of potential vorticity for the diagnosis of stratospheric synoptics

According to quasi-geostrophic approximation, regions of strong cross flow gradient of geopotential vortivity support Rossby wave propagation. Using potential vorticity as a dynamical tracer, the polar vortex can be considered as a material entity. In addition to synoptic charts of geopotential heights and temperatures, maps of potential vorticity are used to describe some distinct features of the circulation of the winter stratosphere.

Rose, K.↗

NASA NTRS1985

Transport processes as manifested in satellite and lidar aerosol measurements

A large increase in stratospheric aerosol data has become available recently from the SAM II and SAGE satellite sensors and the impetus from increased volcanic perturbations. Six years of SAM II and nearly 3 years of SAGE measurements have been accumulated. The increase in large volcanic eruptions since 1979 has caused an acceleration of new data sets from worldwide lidars and airborne lidar campaigns and from various airborne in situ measurements. The SAM II and SAGE data sets show the tropical stratosphere as a source for background stratospheric aerosols, and midlatitudes as a possible sink. Analyses of SAM II data show that the aerosol within the northern wintertime polar vortex becomes isolated from the outside. Subsidence occurs within the vortex, changing the vertical aerosol distribution over the winter period. SAM II and SAGE data show that the aerosol is transported in the stratosphere from low to high latitudes in wintertime. Entry regions of tropospheric air in the Tropics are also evident in the SAGE data as shown by stratospheric cirrus clouds being formed well above the local tropopause. Nature has provided over the past 5 years a number of large volcanic eruptions which spewed tons of new aerosol into the stratosphere. These eruptions have occurred at various latitudes which allow transport differences to be studied. Satellite and lidar aerosol data will be used to describe the stratospheric motions of aerosols produced after these violet volcanic eruptions.

Mccormick, M. P.↗

NASA NTRS1987

Gravity waves

Gravity waves contributed to the establishment of the thermal structure, small scale (80 to 100 km) fluctuations in velocity (50 to 80 m/sec) and density (20 to 30%, 0 to peak). Dominant gravity wave spectrum in the middle atmosphere: x-scale, less than 100 km; z-scale, greater than 10 km; t-scale, less than 2 hr. Theorists are beginning to understand middle atmosphere motions. There are two classes: Planetary waves and equatorial motions, gravity waves and tidal motions. The former give rise to variability at large scales, which may alter apparent mean structure. Effects include density and velocity fluctuations, induced mean motions, and stratospheric warmings which lead to the breakup of the polar vortex and cooling of the mesosphere. On this scale are also equatorial quasi-biennial and semi-annual oscillations. Gravity wave and tidal motions produce large rms fluctuations in density and velocity. The magnitude of the density fluctuations compared to the mean density is of the order of the vertical wavelength, which grows with height. Relative density fluctuations are less than, or of the order of 30% below the mesopause. Such motions may cause significant and variable convection, and wind shear. There is a strong seasonal variation in gravity wave amplitude. Additional observations are needed to address and quantify mean and fluctuation statistics of both density and mean velocity, variability of the mean and fluctuations, and to identify dominant gravity wave scales and sources as well as causes of variability, both temporal and geographic.

Fritts, David↗

NASA NTRS1986

Antarctic springtime measurements of ozone, nitrogen dioxide, and aerosol extinction by SAM II, SAGE, and SAGE II

Simultaneous vertical profiles of O3, NO2, and aerosol extinction obtained with the Stratospheric Aerosol Measurement II, Stratospheric Aerosol and Gas Experiment (SAGE), and SAGE II satellite instruments across the southern polar vortex show that significant differences exist at all altitudes. Both gaseous species display lower concentrations within the vortex over measurement altitudes ranging from the tropopause to 60 km and 20 to 40 km for O3 and NO2, respectively. Aerosol extinction above 15-18 km and total aerosol stratospheric column are also lower inside the vortex than outside. Total column amounts of O3 and NO2 are found to be strongly coupled to spatial location within the vortex, with minimum total values located around the vortex center. Vertical profiles selected to emphasize the observed difference across the circumpolar vortex are presented for October 13, 1981, and October 13, 1985, near 70 and 68 deg S latitude, respectively.

Mccormick, M. P.↗

NASA NTRS1986

Characteristics of Arctic polar stratospheric clouds and as measured by airborne lidar

Airborne lidar measurements of backscattering from polar stratospheric clouds (PSCs) obtained in January 1984 are examined. The flights, principal characteristics of the lidar system, and the meteorological conditions during the flights are described. The characteristics and conditions for the formation of PSCs and the optical characteristics of the clouds are discussed. The properties of the North Polar vortex and El Chichon stratospheric aerosol are studied. Variations in the aerosol optical properties with temperature and water vapor concentrations are analyzed and modeled using a model based on volcanic aerosols and water vapor concentration. The modeled and experimental backscattering-temperature relationship are compared and good correlation is observed at pressure levels of 100 and 70 mb.

Kent, G. S.↗

NASA NTRS1987

Infrared measurements of several nitrogen species above the South Pole in December 1980 and November-December 1986

This paper reports the results of the determinations of total column amounts of HNO3 for December 1980 and November 1986, and NO and NO2 for November-December 1986, deduced from ground-based high-resolution IR solar absorption spectra recorded from the Amundsen-Scott South Pole Station. The measurements were obtained shortly after the austral spring ozone minimum and define, for the first time, the ambient levels of these nitrogen species immediately following the break up of the polar vortex.

Murcray, F. J.↗

NASA NTRS1988

Measurements of several atmospheric gases above the South Pole in December 1986 from high-resolution 3- to 4-micron solar spectra

This paper reports the quantitative analysis of absorption features of a number of atmospheric gases in 0.02/cm resolution 3- to 4-micron solar spectra recorded at the Amundsen-Scott South Pole Station. The measurements were obtained shortly after the austral spring ozone minimum and define, for the first time, the ambient levels of the species immediately following the breakup of the polar vortex. The retrieved total vertical column amounts in molecules per sq cm are: 2.4 + or - 0.4 x 10 to the 21st for H2(O-16), 4.5 + or - 0.5 x 10 to the 18th for H2(O-18), 3.9 + or - 0.4 x 10 to the 17th for HDO, 2.1 + or - 0.2 x 10 to the 19th for CH4, 5.1 + or - 0.5 x 10 to the 21st for CO2, 3.9 + or - 0.4 x 10 to the 18th for N2O, and 3.7 + or - 0.5 x 10 to the 15th for C2H6. Identification of (C-12)H3D absorption features and a search for H2CO absorption in the spectral data are also described.

Goldman, Aaron↗

NASA NTRS1988

Antarctic measurements of ozone by SAGE II in the spring of 1985, 1986, and 1987

This paper presents a three-year (1985, 1986, and 1987) comparison of ozone profiles within the southern polar vortex for September and October, using data obtained by the Stratospheric Aerosol and Gas Experiment II. It was found that, by the first half of October 1986, daily minima in total ozone showed a moderate recovery of 5-7 percent relative to 1985, whereas in 1987, a significant drop of 15 percent from the 1985 minima was observed. The interannual variability of total ozone, temperature, and temperature area or vortex size were found to display a quasi-biennial oscillation (QBO) signal similar to that established by Garcia and Solomon (1987) for Antarctica. Since the 1985 and 1987 years displayed the same QBO phase (westerly) and the 1987 depletion was greater than that of 1985, it is concluded that the long-term secular ozone trend continues to be downward.

Mccormick, M. P.↗

NASA NTRS1988

Comparison of in situ aerosol measurements with SAGE 2 and SAM 2 aerosol measurements during the airborne Antarctic ozone experiment

Models indicate that stratospheric aerosols play a major role in the destruction of ozone during the Austral winter. Although many in situ measurements of stratospheric aerosols were made during the Airborne Antarctic Ozone Experiment, changes of aerosol concentration and size distributions across the polar vortex are important to understanding changes of chemical species taking place during this time. Therefore comparing the in situ measurements with measurements made by satellites scanning wider areas will give a clearer picture of the possible role played by aerosols during this period. The wire impactor size distributions are compared to those from the aerosol spectrometers and a best fit size distribution determined. Aerosol extinctions are calculated from the in situ measurements and compared to the extinctions measured by the satellites. Five comparisons are made with SAGE 2 and four with SAM 2. Extinctions agree as close as a factor of two.

Ferry, G. V.↗

NASA NTRS1988

Filter measurements of chemical composition during the airborne Antarctic ozone experiment

During the Airborne Antarctic Ozone Experiment campaign, a filter sampler was flown to measure the bulk composition of aerosol and gas phases. The background sulfate aerosol was measured in regions inside and outside of the chemically perturbed region (CPR) of the polar vortex. The mass ratio of sulfate outside to inside was 2.8. This is indicative of a cleansing mechanism effecting the CPR or of a different air mass inside versus outside. The absolute value of the sulfate mixing ratio shows that the background aerosol has not been influenced by recent volcanic eruptions. The sulfate measured on the ferry flight returning to NASA Ames shows a decrease towards the equator with increasing concentrations in the northern hemisphere. Nitrate in the aerosol phase was observed on two flights. The largest amount of nitrate measured in the aerosol was 44 percent of the total amount of nitrate observed. Other samples on the same flights show no nitrate in the aerosol phase. The presence of nitrate in the aerosol is correlated with the coldest temperatures observed on a given flight. Total nitrate (aerosol plus acidic vapor nitrate) concentrations were observed to increase at flight altitude with increasing latitude north and south of the equator. Total nitrate was lower inside the CPR than outside. Chloride and flouride were not detected in the aerosol phase. From the concentrations of acidic chloride vapor, the ratio of acidic vapor Cl to acidic vapor F and a summing of the individual chloride containing species to yield a total chloride concentration, there is a suggestion that some of the air sampled was dechlorinated. Acidic vapor phase fluoride was observed to increase at flight altitude with increasing latitude both north and south of the equator. The acidic vapor phase fluoride was the only compound measured with the filter technique that exhibited larger concentrations inside the CPR than outside.

Grandrud, B. W.↗

NASA NTRS1988

Extinction and backscatter measurements of Antarctic PSC's, 1987: Implications for particle and vapor removal

The temperature dependence is examined of optical properties measured in the Antarctic during 1987 at the 70 mb level (near 18 km), a level chosen to correlate the results with in situ measurements made from the NASA-Ames ER-2 aircraft during the 1987 Airborne Antarctic Ozone Experiment (AAOE). The data set consists of extinction measurements by Sam 2 inside the Antarctic polar vortex from May to October 1987; and backscatter measurements by the UV-DIAL (Ultraviolet Differential Absorption Lidar) system aboard the Ames DC-8 aircraft during selected AAOE flights. Observed trends are compared with results from a revised version of Pole and McCormick's model to classify the PSC observations by Type (1 or 2) and infer the temporal behavior of the ambient aerosol and ambient vapor mixing ratios. The sample figures show monthly ensembles of the 70-mb Sam 2 extinction ratio (the ratio of aerosol or PSC extinction to molecule extinction) as a function of NMC temperature at the beginning (June) and (October) of the 1987 Antarctic winter. Both ensembles show two rather distinct clusters of points: one oriented in the near vertical direction which depicts the change with temperature of the ambient aerosol extinction ratio; and a second cluster oriented in the near horizontal direction whose position on the vertical scale marks a change in particle phase (i.e., PSC formation) and whose length (the extinction enhancement related to that of the ambient aerosol) is an indicator of PSC type.

Poole, L. R.↗

NASA NTRS1988

Stratospheric column NO2 measurements from three Antarctic sites

The significance of stratospheric odd-nitrogen compounds in Antarctic ozone depletion studies has prompted an increase in Antarctic activities. Although several species are being studied, work has concentrated on the acquisition of NO2 data. Ground-based measurements of stratospheric column NO2 have been made at Arrival Heights, Antarctica, since spring 1982, with some gaps in the data base. Additional data has been acquired since February 1986 at Pole Station and Halley Bay, thus providing a chain of stations across the continent. The technique used is that of absorption spectroscopy in several wavelength regions, although here only those measurements are reported in the 430 to 450 nm region where strongly structured absorption been determined experimentally. However, theory features due to NO2 are identified in scattered sunlight in the zenith sky. Operation of a moon-tracking system at Arrival Heights has provided some additional data during the polar night. Previous analyses have shown that the NO2 column observed from the ground is strongly influenced by the season, and by the location of the site with respect to that of the polar vortex. The column amount correlates strongly with stratospheric temperature at about 70 mbar. The present data set further illustrates these features, and demonstrates both the strengths and qualifications apparent in the technique.

Keys, J. G.↗

NASA NTRS1988

Near UV atmospheric absorption measurements from the DC-8 aircraft during the 1987 airborne Antarctic ozone experiment

During the Airborne Antarctic Ozone Experiment from 28 August to 30 September 1987 near UV zenith scattered sky measurements were made over Antarctic from the NASA DC-8 aircraft using a one third m spectrograph equipped with a diode-array detector. Scattered sky light data in the wavelength range 348 nm to 388 nm was spectrally analyzed for O3, NO2, OClO, and BrO column abundances. Slant column abudances of O3, NO2, OClO and BrO were determined, using a computer algorithm of non-linear and linear least square correlation of Antarctic scattered sky spectra to laboratory absorption cross section data. Using measured vertical electrochemical sonde ozone profiles from Palmer, Halley Bay, and the South Pole Stations the slant columns of O3 were converted into vertical column abundances. The vertical column amounts of NO2, OClO, and BrO were derived using vertical profiles calculated by a chemical model appropriate for Antarctica. NO2 vertical column abundances show steep latitudinal decrease with increasing latitude for all 13 flights carried out during the mission. In the regions where NO2 abudances are low, OClO and BrO were observed. The spatial and temporal vertical column abundances of these species are discussed in the context of the chemistry and dynamics in the antarctic polar vortex during the austral spring.

Wahner, A.↗

NASA NTRS1988

Infrared aircraft measurements of stratospheric composition over Antarctica during September 1987

The JPL Mark IV interferometer recorded high resolution, infared solar spectra from the NASA DC-8 aircraft during flights over Antarctica in September 1987. The atmospheric absorption features in these spectra were analyzed to determine the overburdens of O3, NO, NO2, HNO3, ClONO2, HCl, HF, CH4, N2O, CO, H2O and CFC-12. The spectra were obtained at latitudes which ranged between 64 degrees S and 86 degrees S, allowing the composition in the interior of the polar vortex to be compared with that at the edge. The latitude dependence observed for NO, HO2, HNO3, ClONO2, HCl and HF are summerized. The values at 30 deg S were observed on the ferry flight from New Zealand to Hawaii. The dashed lines connecting the two were interpolated across the region for which there are no measurements. The chemically perturbed region is seen to consist of a collar of high HNO3 and ClONO2 surrounding a core in which the overburdens of these and of HCl and NO2 are very low. Clear increases in the overburdens of HF and HNO3 were observed during the course of September in the vortex core. HCl and NO2 exhibited smaller, less significant increases. The overburdens of the tropospheric source gases, N2O, CH4, CF2Cl2, and H2O were observed to much smaller over Antarctica than at mid-latitudes. This, together with the fact that HF over Antarctica was more that double its mid-latitude value, suggests that downwelling has occurred.

Toon, Goeff C.↗