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At least 307 records · Page 17

Dynamical evolution of viscous disks around be stars. II. Polarimetry

Be stars exhibit variability for a great number of observables. Putting the pieces of the disk dynamics together is not an easy task and requires arduous modeling before achieving a good fit to the observational data. In order to guide the modeling process and make it more efficient, it is very instructive to investigate reference dynamical cases. This paper focuses on continuum polarimetric quantities and is the second of a series that aims to demonstrate the capacity of deriving the dynamical history and fundamental parameters of a classical Be star through follow-up of various observables. After a detailed study of the different opacities at play in the formation of polarized spectra, we investigate predictions of polarimetric observables in the continuum for different dynamical scenarios. Our models are based on a coupling of a hydrodynamic viscous decretion simulations in a disk and a three-dimensional non-LTE radiative transfer code. Through introduction of the polarization color diagram (PCD), we show that certain combinations of polarimetric observables exhibit features that are characteristic of a mass-loss history. This diagram also enables estimates of fundamental parameters such as the inclination angle, disk density scale, and the α viscous diffusion parameter. We present the PCD as a powerful diagnosis tool to track the dynamical phases of a Be star, such as disk build-up, dissipation, periodic, and episodic outbursts. Finally, we confront our models with observations of four Be stars that exhibited long-term polarimetric activity.

79 ASTRONOMY AND ASTROPHYSICS↗

La 0.6 Sr 0.4 CoO 3−δ Films Under Deoxygenation: Magnetic And Electronic Transitions Are Apart from The Structural Phase Transition

Abstract Topotactic phase transitions induced by changes in the oxygen vacancy concentration can largely alter the physical properties of complex oxides, including electronic and magnetic phases, while maintaining the structural integrity of the crystal lattice. An oxygen‐vacancy‐induced topotactic phase transition from perovskite (PV) to brownmillerite (BM) is achieved in epitaxial La 0.6 Sr 0.4 CoO 3−δ (LSCO) thin films. Two novel intermediate states with different oxygen content are identified by X‐ray diffraction, which involves a single‐phase reduced PV state and a mixed state of co‐existing PV and BM. The combination of depth‐sensitive polarized neutron reflectometry (PNR) and Rutherford backscattering (RBS) allows a quantitative determination of magnetization and the mean oxygen content in all states, revealing a continuous transition from La 0.6 Sr 0.4 CoO 2.97 to La 0.6 Sr 0.4 CoO 2.5 . BM formation is observed for an LSCO layer with an oxygen content of 2.67, while the magnetic and electronic transition already occurs for a layer with a higher oxygen content of 2.77 (and above) and in the absence of a BM signature. These results demonstrate that the physics of electronic metal‐to‐insulator transition (MIT), magnetic ferromagnet‐to‐non‐ferromagnet transition (FM‐to‐non‐FM), and structural PV‐to‐BM phase transition should be considered within the framework of separate but interrelated processes.

36 MATERIALS SCIENCE↗

An Experimental Study on Low Pressure Frost Formation for Lunar Polar Water Capture

In-situ resource utilization (ISRU) is a vital component of NASA’s mission to the Moon and beyond, as the extraction of resources from the environment can reduce payload weight and the frequency of resupply missions. Since the discovery of water in the regolith of the permanently shadowed regions (PSR) of the Moon, its extraction and transport has become an area of increasing interest for NASA. One proposed method is heating icy regolith to free the water before de-sublimating and transporting it as ice in a tanker. However, little is known regarding the dynamics of frost growth at low pressures, and an understanding of the heat transfer process is required to properly size the heat exchanger for the tanker. To investigate this phenomenon, a cold plate was placed in a vacuum chamber with water vapor directed at its surface. The chamber pressure (300 and 500 Pa) and cold plate temperature (–18 to –5 °C) were kept below the triple point and varied throughout the experiment to examine their impact on frost layer heat transfer. As water flowed into the chamber and deposited on the cold plate surface, the heat flux and temperature were measured along with the frost layer thickness and/or mass. Density calculated at the conclusion of each test suggests the frost layer is denser than that of frost grown at atmospheric pressure. The results demonstrate unexpected density and heat transfer characteristics and require development of a new model of frost growth for lunar conditions

Lunar polar↗

Double layers and plasma-wave resistivity in extragalactic jets - Cavity formation and radio-wave emission

Current driven electrostatic-wave- and electromagnetic-wave-produced resistivities do not occur in extragalactic jets for estimated values of the carried currents. Strong plasma double layers, however, may exist within self-maintained density cavities. The relativistic double-layer-emitted electron and ion beams drive plasma-wave resistivities in the low- and high-potential plasma adjacent to the double layers. The double-layer-emitted electron beams may also emit polarized radio waves via a collective bremsstrahlung process mediated by electrostatic two-stream instabilities.

Borovsky, Joseph E.↗

A Resolved Near-Infrared Image of the Inner Cavity in the GM Aur Transitional Disk

We present high-contrast H-band polarized intensity (PI) images of the transitional disk around the young solar like star GM Aur. The near-infrared direct imaging of the disk was derived by polarimetric differential imaging using the Subaru 8.2 m Telescope and HiCIAO. An angular resolution and an inner working angle of 0 07 and radius approximately 0 05, respectively, were obtained. We clearly resolved a large inner cavity, with a measured radius of 18+/ 2 au, which is smaller than that of a submillimeter interferometric image (28 au). This discrepancy in the cavity radii at near-infrared and submillimeter wavelengths may be caused by a 34M(sub Jup) planet about 20 au away from the star, near the edge of the cavity. The presence of a near-infrared inner cavity is a strong constraint on hypotheses for inner cavity formation in a transitional disk. A dust filtration mechanism has been proposed to explain the large cavity in the submillimeter image, but our results suggest that this mechanism must be combined with an additional process. We found that the PI slope of the outer disk is significantly different from the intensity slope obtained from HSTNICMOS, and this difference may indicate the grain growth process in the disk.

high-contrast H-band polarized intensity (PI)↗

Meso-Scale Electrodynamic Coupling of the Earth Magnetosphere-Ionosphere System

Within the fully integrated magnetosphere-ionosphere system, many electrodynamic processes interact with each other. We review recent advances in understanding three major meso-scale coupling processes within the system: the transient field-aligned currents (FACs), mid-latitude plasma convection, and auroral particle precipitation. (1) Transient FACs arise due to disturbances from either dayside or nightside magnetosphere. As the interplanetary shocks suddenly compress the dayside magnetosphere, short-lived FACs are induced at high latitudes with their polarity successively changing. Magnetotail dynamics, such as substorm injections, can also disturb the current structures, leading to the formation of substorm current wedges and ring current disruption. (2) The mid-latitude plasma convection is closely associated with electric fields in the system. Recent studies have unraveled some important features and mechanisms of subauroral fast flows. (3) Charged particles, while drifting around the Earth, often experience precipitating loss down to the upper atmosphere, enhancing the auroral conductivity. Recent studies have been devoted to developing more self-consistent geospace circulation models by including a better representation of the auroral conductance. It is expected that including these new advances in geospace circulation models could promisingly strengthen their forecasting capability in space weather applications. The remaining challenges especially in the global modeling of the circulation system are also discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

The Strength and Characteristics of VPPA Welded 2219-T87 Aluminum Alloy

A study of the variable polarity plasma arc (VPPA) welding process and those factors that control the structure and properties of VPPA welded aluminum alloy 2219-T87 was conducted. The importance of joint preparation, alignment of parts and welding process variables are already established. Internal weld defects have been eliminated. However, a variation of properties was found to be due to the size variation of interdendritic particles in the fusion zone. These particles contribute to the void formation process, which controls the ultimate tensile strength of the welded alloy. A variation of 150 microns in particle size correlated with a 10 ksi variation of ultimate tensile strength. It was found that all fracture surfaces were of the dimple rupture type, with fracture initiating within the fusion zone.

Jemian, W. A.↗

Quantification of waste morphology in Martian fretted terrain

Qualitative and quantitative analyses are performed on the northern fretted terrain of the Martian Isnenius Lacus quadrangle to determine the formation processes. The fretted terrain lies between 35-50 deg N latitude and 305-350 deg W longitude and was mapped with Viking orbiter instrumentation. The dominant landforms are a sequence of heavily cratered terrain, scattered flat-floored, fretted valleys, linear waste-covered valleys between flat-topped mesas, circum-mesa debris areas, a transition from mesas to knobby terrain, fewer upland forms, and low-relief, mantled, polar plains. The features spread out from a cratered terrain boundary in a succession of shapes. A principal components analysis characterizes definable spatial variations in the surface morphology and suggests that the features are youngest in the southwest direction. Relationships are also found between neighboring features. The principal components analysis technique is concluded to be a valuable tool for explaining the geomorphic evolution of the Martian surface.

Kochel, R. C.↗

Pattern formation in a coupled membrane-bulk reaction-diffusion model for intracellular polarization and oscillations

Reaction-diffusion systems have been widely used to study spatio-temporal phenomena in cell biology, such as cell polarization. Coupled bulk-surface models naturally include compartmentalization of cytosolic and membrane-bound polarity molecules. Here we study the distribution of the polarity protein Cdc42 in a mass-conserved membrane-bulk model, and explore the effects of diffusion and spatial dimensionality on spatio-temporal pattern formation. We first analyze a one-dimensional (1-D) model for Cdc42 oscillations in fission yeast, consisting of two diffusion equations in the bulk domain coupled to nonlinear ODEs for binding kinetics at each end of the cell. In 1-D, our analysis reveals the existence of symmetric and asymmetric steady states, as well as anti-phase relaxation oscillations typical of slow-fast systems. We then extend our analysis to a two-dimensional (2-D) model with circular bulk geometry, for which species can either diffuse inside the cell or become bound to the membrane and undergo a nonlinear reaction-diffusion process. We also consider a nonlocal system of PDEs approximating the dynamics of the 2-D membrane-bulk model in the limit of fast bulk diffusion. In all three model variants we find that mass conservation selects perturbations of spatial modes that simply redistribute mass. In 1-D, only anti-phase oscillations between the two ends of the cell can occur, and in-phase oscillations are excluded. In higher dimensions, no radially symmetric oscillations are observed. Instead, the only instabilities are symmetry-breaking, either corresponding to stationary Turing instabilities, leading to the formation of stationary patterns, or to oscillatory Turing instabilities, leading to traveling and standing waves. Codimension-two Bogdanov—Takens bifurcations occur when the two distinct instabilities coincide, causing traveling waves to slow down and to eventually become stationary patterns. Our work clarifies the effect of geometry and dimensionality on behaviors observed in ma.ss-conserved cell polarity models.

97 MATHEMATICS AND COMPUTING↗

Double layers and plasma-wave resistivity in extragalactic jets: Cavity formation and radio-wave emission

For estimated values of the currents carried by extragalactic jets, current-driven electrostatic-wave- and electromagnetic-wave-produced resistivities do not occur. Strong plasma double layers, however, may exist within self-maintained density cavities, the relativistic double-layer-emitted electron, and ion beams driving plasma-wave resistivities in the low- and high-potential plasma adjacent to the double layers. The double-layer-emitted electron beams may also emit polarized radio waves via a collective bremsstrahlung process mediated by electrostatic two-stream instabilities.

Borovsky, Joseph E.↗

Direct-drive inertial confinement fusion: A review

In this study, the direct-drive, laser-based approach to inertial confinement fusion (ICF) is reviewed from its inception following the demonstration of the first laser to its implementation on the present generation of high-power lasers. The review focuses on the evolution of scientific understanding gained from target-physics experiments in many areas, identifying problems that were demonstrated and the solutions implemented. The review starts with the basic understanding of laser–plasma interactions that was obtained before the declassification of laser-induced compression in the early 1970s and continues with the compression experiments using infrared lasers in the late 1970s that produced thermonuclear neutrons. The problem of suprathermal electrons and the target preheat that they caused, associated with the infrared laser wavelength, led to lasers being built after 1980 to operate at shorter wavelengths, especially 0.35 um—the third harmonic of the Nd:glass laser—and 0.248 um (the KrF gas laser). The main physics areas relevant to direct drive are reviewed. The primary absorption mechanism at short wavelengths is classical inverse bremsstrahlung. Nonuniformities imprinted on the target by laser irradiation have been addressed by the development of a number of beam-smoothing techniques and imprint-mitigation strategies. The effects of hydrodynamic instabilities are mitigated by a combination of imprint reduction and target designs that minimize the instability growth rates. Several coronal plasma physics processes are reviewed. The two-plasmon–decay instability, stimulated Brillouin scattering (together with cross-beam energy transfer), and (possibly) stimulated Raman scattering are identified as potential concerns, placing constraints on the laser intensities used in target designs, while other processes (self-focusing and filamentation, the parametric decay instability, and magnetic fields), once considered important, are now of lesser concern for mainline direct-drive target concepts. Filamentation is largely suppressed by beam smoothing. Thermal transport modeling, important to the interpretation of experiments and to target design, has been found to be non-local in nature. Advances in shock timing and equation-of-state measurements relevant to direct-drive ICF are reported. Room-temperature implosions have provided an increased understanding of the importance of stability and uniformity. The evolution of cryogenic implosion capabilities, leading to an extensive series carried out on the 60-beam OMEGA laser [T. R. Boehly et al., Opt. Commun. 133, 495 (1997)], is reviewed together with major advances in cryogenic target formation. A polar-drive concept has been developed that will enable direct-drive–ignition experiments to be performed on the National Ignition Facility [C. A. Haynam et al., Appl. Opt. 46 (16), 3276 (2007)]. The advantages offered by the alternative approaches of fast ignition and shock ignition and the issues associated with these concepts are described. The lessons learned from target-physics and implosion experiments are taken into account in ignition and high-gain target designs for laser wavelengths of 1/3 μm and 1/4 μm. Substantial advances in direct-drive inertial fusion reactor concepts are reviewed. Overall, the progress in scientific understanding over the past five decades has been enormous, to the point that inertial fusion energy using direct drive shows significant promise as a future environmentally attractive energy source.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Interface effects and relaxation processes in nanocomposites based on CdSe/ZnS semiconductor quantum dots and porphyrin molecules

Controllable self-assembly and properties of nanocomposites based on CdSe/ZnS semiconductor quantum dots (QDs) and tetrapyridylporphyrin molecules (H{sub 2}P) as well as the dynamics of relaxation processes in these systems were studied for solutions and single nanoobjects in the temperature range of 77–295 K. It was proved that the formation of surface states of different nature is crucial to nonradiative relaxation of exciton excitation in QDs. The efficiency of QD→Н{sub 2}Р energy transfer was shown to be at most 10–15%. Regularities of photoluminescence (PL) quenching for QDs in nanocomposites in solutions of different polarity correlate with the dependences of PL blinking for single QDs. A scheme was proposed of excited states and main relaxation channels of exciton excitation energy in semiconductor QDs and QD–Н{sub 2}Р nanocomposites.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

The magnetic field of Mercury, part 1

An updated analysis and interpretation is presented of the magnetic field observations obtained during the Mariner 10 encounter with the planet Mercury. The combination of data relating to position of the detached bow shock wave and magnetopause, and the geometry and magnitude of the magnetic field within the magnetosphere-like region surrounding Mercury, lead to the conclusion that an internal planetary field exists with dipole moment approximately 5.1 x 10 the 22nd power Gauss sq cm. The dipole axis has a polarity sense similar to earth's and is tilted 7 deg from the normal to Mercury's orbital plane. The magnetic field observations reveal a significant distortion of the modest Hermean field (350 Gamma at the equator) by the solar wind flow and the formation of a magnetic tail and neutral sheet which begins close to the planet on the night side. The composite data is not consistent with a complex induction process driven by the solar wind flow.

Ness, N. F.↗

Lyotropic Liquid Crystalline Phase Behavior of Boron Nitride Nanotube Aqueous Dispersions

Boron nitride nanotubes (BNNTs) are gaining significant interest due to their outstanding mechanical and thermal properties, as well as their potential to serve as a model nanorod system. Processing BNNT liquid crystalline (LC) dispersions enables precise control over BNNT orientation in macroscopic assemblies, while their low absorption in the visible spectrum facilitates studying LCs at exceptionally high concentrations. Here, we investigate the behavior of BNNTs in aqueous solutions stabilized by the surfactant sodium deoxycholate (SDC), examining the effect of BNNT purity and BNNT−SDC concentrations on lyotropic LC formation. We disperse up to 15wt% BNNT in SDC solutions and use polarized light microscopy to detail the transition from an isotropic state to a biphasic regime, where isotropic and nematic domains coexist due to phase separation, to a single fully nematic phase. Cryogenic electron microscopy provides direct evidence of BNNT alignment within nematic domains. Our results show that enhanced depletion-induced attractions, driven by increased surfactant concentration, lower the threshold concentration of BNNT required to form nematic domains. In contrast, low surfactant concentrations relative to BNNT result in insufficiently coated nanotube surfaces, leading to poor dispersions and BNNT aggregation. Additionally, we fabricate well-aligned BNNT films from aqueous LC dispersions. Our findings advance the understanding of BNNT LCs, offering insight into controlling their orientation and highlighting their potential for high-performance materials.

Joe Khoury↗

Ab initio kinetics and thermal decomposition mechanism of mononitrobiuret and 1,5-dinitrobiuret

Mononitrobiuret (MNB) and 1,5-dinitrobiuret (DNB) are tetrazole-free, nitrogen-rich, energetic compounds. For the first time, a comprehensive ab initio kinetics study on the thermal decomposition mechanisms of MNB and DNB is reported here. In particular, the intramolecular interactions of amine H-atom with electronegative nitro O-atom and carbonyl O-atom have been analyzed for biuret, MNB, and DNB at the M06-2X/aug-cc-pVTZ level of theory. The results show that the MNB and DNB molecules are stabilized through six-member-ring moieties via intramolecular H-bonding with interatomic distances between 1.8 and 2.0 Å, due to electrostatic as well as polarization and dispersion interactions. Furthermore, it was found that the stable molecules in the solid state have the smallest dipole moment amongst all the conformers in the nitrobiuret series of compounds, thus revealing a simple way for evaluating reactivity of fuel conformers. The potential energy surface for thermal decomposition of MNB was characterized by spin restricted coupled cluster theory at the RCCSD(T)/cc-pV∞ Z//M06-2X/aug-cc-pVTZ level. It was found that the thermal decomposition of MNB is initiated by the elimination of HNCO and HNN(O)OH intermediates. Intramolecular transfer of a H-atom, respectively, from the terminal NH{sub 2} group to the adjacent carbonyl O-atom via a six-member-ring transition state eliminates HNCO with an energy barrier of 35 kcal/mol and from the central NH group to the adjacent nitro O-atom eliminates HNN(O)OH with an energy barrier of 34 kcal/mol. Elimination of HNN(O)OH is also the primary process involved in the thermal decomposition of DNB, which processes C{sub 2v} symmetry. The rate coefficients for the primary decomposition channels for MNB and DNB were quantified as functions of temperature and pressure. In addition, the thermal decomposition of HNN(O)OH was analyzed via Rice–Ramsperger–Kassel–Marcus/multi-well master equation simulations, the results of which reveal the formation of (NO{sub 2} + H{sub 2}O) to be the major decomposition path. Furthermore, we provide fundamental interpretations for the experimental results of Klapötke et al. [Combust. Flame 139, 358–366 (2004)] regarding the thermal stability of MNB and DNB, and their decomposition products. Notably, a fundamental understanding of fuel stability, decomposition mechanism, and key reactions leading to ignition is essential in the design and manipulation of molecular systems for the development of new energetic materials for advanced propulsion applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Systems for Transducing Entanglement Between Photons and Electron Spins

The transfer of quantum properties and entanglement between photons and matter (transduction) is a major challenge in QIS, especially with regard to networking quantum information processing. In order to overcome this challenge, it is important to know how non-classical light (single or entangled photons) interacts with matter. This project specifically addresses fundamental questions about the interaction of single and entangled photons with molecules and nanostructures to produce electrons with prescribed spin polarizations and pairs of electrons with entangled spins, thus resulting in transduction by addressing two major objectives: (2) In Objective 1, we will investigate the formation of polarization-encoded radical (spin qubit) pairs and molecular triplet states photoexcited by single quantum emitter light sources. (2) In Objective 2, we will demonstrate the use of two entangled photons, generated by spontaneous parametric down conversion (SPDC) or by the coherent biexcitonic states of perovskite NPLs, to produce two entangled radical (spin qubit) pairs or molecular triplet states.

74 ATOMIC AND MOLECULAR PHYSICS↗

A Model for Energy Buildup and Eruption Onset in Coronal Mass Ejections

Coronal mass ejections (CMEs) and eruptive flares (EFs) are the most energetic explosions in the solar system. Their underlying origin is the free energy that builds up slowly in the sheared magnetic field of a filament channel. We report the first end-to-end numerical simulation of a CME/EF, from zero-free-energy initial state through filament channel formation to violent eruption, driven solely by the magnetic-helicity condensation process. Helicity is the topological measure of linkages between magnetic flux systems, and is conserved in the corona, building up inexorably until it is ejected into interplanetary space. Numerous investigations have demonstrated that helicity injected by small-scale vortical motions, such as those observed in the photosphere, undergoes an inverse cascade from small scales to large, “condensing” at magnetic-polarity boundaries. Our new results verify that this process forms a filament channel within a compact bipolar region embedded in a background dipole field, and show for the first time that a fast CME eventually occurs via the magnetic-breakout mechanism. We further show that the trigger for explosive eruption is reconnection onset in the flare current sheet that develops above the polarity inversion line: this reconnection forms flare loops below the sheet and a CME flux rope above, and initiates high-speed outward flow of the CME. Our findings have important implications for magnetic self organization and explosive behavior in solar and other astrophysical plasmas, as well as for understanding and predicting explosive solar activity.

filaments↗

Scan‐Path‐ and Initial‐State‐Dependent Superdomain Switching in (111)‐Oriented PZT

Polarization switching in ferroelectric materials arises from the collective evolution of complex domain hierarchies, yet deterministic control over these processes remains challenging. Here, we investigate scan-path- and initial-state-dependent switching in epitaxial (111)-oriented PbZr 0.2 Ti 0.8 O 3 thin films using automated AFM-based writing combined with quantitative 3D piezoresponse force microscopy. We show that the scan trajectory acts as an experimentally accessible control parameter for superdomain formation. Box-in-box raster scans reproducibly stabilize ordered stripe superdomains with a reduced subset of symmetry-allowed variants, whereas spiral trajectories generate frustrated mixed-variant states with a broader distribution of final microstructures. Automated pulsing experiments further show that the local superdomain configuration at the nucleation site strongly influences the final written morphology. Phase-field modeling qualitatively reproduces the contrast between representative initial-state geometries and supports the role of compatibility constraints among competing ferroelastic pathways. These findings establish scan-path and initial-state engineering as practical handles to program ferroic order in hierarchical ferroelectric domain structures.

Vasudevan, Rama K. [Oak Ridge National Laboratory ↗