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At least 307 records · Page 17

Constraints on PSC Particle Microphysics Derived From Lidar Observations

Based on extensive T-matrix computations of light scattering by polydispersions of randomly oriented, rotationally symmetric nonspherical particles, we analyze existing lidar observations of polar stratospheric clouds (PSCs) and derive several constraints on PSC particle microphysical properties. We show that sharp-edged nonspherical particles (finite circular cylinders) exhibit less variability of lidar backscattering characteristics with particle size and aspect ratio than particles with smooth surfaces (spheroids). For PSC particles significantly smaller than the wavelength, the backscatter color index Alpha and the depolarization color index Beta are essentially shape-independent. Observations for type Ia PSCs can be reproduced by spheroids with aspect ratios larger than 1.2, oblate cylinders with diameter-to-length ratios greater than 1.6, and prolate cylinders with length-to-diameter ratios greater than 1.4. The effective equal-volume-sphere radius for type la PSCs is about 0.8 microns or larger. Type Ib PSCs are likely to be composed of spheres or nearly spherical particles with effective radii smaller than 0.8 microns. Observations for type II PSCs are consistent with large ice crystals (effective radius greater than 1 micron modeled as cylinders or prolate spheroids.

Liu, Li↗

Do Solar Coronal Holes Affect the Properties of Solar Energetic Particle Events?

The intensities and timescales of gradual solar energetic particle (SEP) events at 1 AU may depend not only on the characteristics of shocks driven by coronal mass ejections (CMEs), but also on large-scale coronal and interplanetary structures. It has long been suspected that the presence of coronal holes (CHs) near the CMEs or near the 1-AU magnetic footpoints may be an important factor in SEP events. We used a group of 41 E (is) approx. 20 MeV SEP events with origins near the solar central meridian to search for such effects. First we investigated whether the presence of a CH directly between the sources of the CME and of the magnetic connection at 1 AU is an important factor. Then we searched for variations of the SEP events among different solar wind (SW) stream types: slow, fast, and transient. Finally, we considered the separations between CME sources and CH footpoint connections from 1 AU determined from four-day forecast maps based on Mount Wilson Observatory and the National Solar Observatory synoptic magnetic-field maps and the Wang-Sheeley-Arge model of SW propagation. The observed in-situ magnetic-field polarities and SW speeds at SEP event onsets tested the forecast accuracies employed to select the best SEP/CH connection events for that analysis. Within our limited sample and the three analytical treatments, we found no statistical evidence for an effect of CHs on SEP event peak intensities, onset times, or rise times. The only exception is a possible enhancement of SEP peak intensities in magnetic clouds.

Coronal mass ejections - low coronal signatures↗

Spectro-Microscopy Studies of Atmospheric Particles

Our project investigated composition and physical properties of individual atmospheric particles collected in field campaigns organized by the DOE Atmospheric Systems Research and Atmospheric Radiation Measurement (ASR/ARM) programs, such as the Green Ocean Amazon (GoAmazon, 2014/5), the Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE, 2016/7), the Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA, 2017/8), the Aerosol–Ice Formation Closure Pilot Study (AEROICESTUDY, 2019) and in additional small-scale supporting field experiments focused on the investigation of the light-absorbing (aka brown carbon) atmospheric particles. In these studies, we investigated the contribution of natural and anthropogenic sources to populations of atmospheric particles during representative atmospheric conditions; characterized particle composition and evaluated their hygroscopic properties and propensity to act as cloud condensation nuclei (CCN) and ice nuclei (IN); correlated typical particle-type and mixing state characteristics with real-time measurements in the areas of studies. We used multi-modal spectro-microscopy techniques to examine elemental and molecular composition, mixing state, size, and higher order morphology for individual particles. Specifically, we used computer-controlled scanning electron microscopy and X-ray microanalysis for quantitative analysis of particle elemental composition, and we used transmission electron microscopy to provide additional information on the distribution of different components within individual particles (particle heterogeneity). We used synchrotron-based scanning transmission X-ray microscopy for quantitative description of the mixing state and molecular bonding of carbon in particles. The particle composition, mixing state, and morphology from analyzed periods was then combined with the real-time ARM measurements of aerosol size distribution, CCN concentration, hygroscopicity, and aerosol bulk composition. Combined together, results of our studies allowed us to assess the major particle sources (biogenic vs. anthropogenic, primary vs secondary) and gain insight into the atmospheric processing of aerosol particles resulting from condensation, coagulation, oxidative aging, and cloud processing. In collaboration with other scientists involved in field campaigns, we carried out statistical analysis of particle properties and their source-specific contributions to regional aerosol loading under representative air mass, meteorological, and cloud conditions.

scanning transmission X-ray microscopy↗

Source apportionment of soot particles and aqueous-phase processing of black carbon coatings in an urban environment

Abstract. The impacts of soot particles on climate and human health depend on the concentration of black carbon (BC) as well as the thickness and composition of the coating material, i.e., organic and inorganic compounds internally mixed with BC. In this study, the size-resolved chemical composition of BC-containing aerosol was measured using a high-resolution soot particle aerosol mass spectrometer (SP-AMS) during wintertime in Fresno, California, a location influenced by abundant combustion emissions and frequent fog events. Concurrently, particle optical properties were measured to investigate the BC absorption enhancement. Positive matrix factorization (PMF) analysis was performed on the SP-AMS mass spectral measurements to explore the sources of soot particles and the atmospheric processes affecting the properties of BC coatings. The analysis revealed that residential woodburning and traffic are the dominant sources of soot particles. Alongside primary soot particles originating from biomass burning (BBOABC) and vehicles (HOABC) two distinct types of processed BC-containing aerosol were identified: fog-related oxidized organic aerosol (FOOABC) and winter-background OOABC (WOOABC). Both types of OOABC showed evidence of having undergone aqueous processing, albeit with differences. The concentration of FOOABC was substantially elevated during fog events, indicating the formation of aqueous secondary organic aerosol (aqSOA) within fog droplets. On the other hand, WOOABC was present at a relatively consistent concentration throughout the winter and was likely related to the formation of secondary organic aerosol (SOA) in both the gas phase and aerosol liquid water. By comparing the chemical properties and temporal variations in FOOABC and WOOABC, we gain insights into the key aging processes of BC aerosol. It was found that aqueous-phase reactions facilitated by fog droplets had a significant impact on the thickness and chemical composition of BC coatings, thereby affecting the light absorption and hygroscopic properties of soot particles. These findings underscore the important role of chemical reactions occurring within clouds and fogs and influencing the climate forcing of BC aerosol in the atmosphere.

54 ENVIRONMENTAL SCIENCES↗

Dynamical and photometric investigation of cometary type 2 tails

The absolute calibration of the photometric profile of the antitail of Comet Kohoutek 1973 XII on plates taken with the Curtis Schmidt telescope of the University of Michigan at the Cerro Tololo Inter-American Observatory is described in detail. The formula for the determination of the air mass, and the correction for atmospheric absorption and for the loss of light due to vignetting are included. The calibration stars were used to derive the coefficients converting the relative intensity scale to the absolute surface-brightness units. The extensive results of the study of the orbital evolution of vaporizing dust particles are listed in a tabular form. Gradual evaporation from the surface of a particle results typically in its expulsion from the solar system. The properties of the particle and the elements of its orbit at expulsion are given as functions of the particle's properties and orbit before appreciable evaporation commenced. Also given are circumstances at an encounter of an expelled particle with the earth as a function of the particle's properties. A few specific cases are represented graphically.

Sekanina, Z.↗

Optical and transport properties of plasma mixtures from ab initio molecular dynamics

Predicting the charged particle transport properties of warm dense matter/hot dense plasma mixtures is a challenge for analytical models. High accuracy ab initio methods are more computationally expensive, but can provide critical insight by explicitly simulating mixtures. In this work, we investigate the transport properties and optical response of warm dense carbon–hydrogen mixtures at varying concentrations under either conserved electronic pressure or mass density at a constant temperature. We compare options for mixing the calculated pure species properties to estimate the results of the mixtures. We find that a combination of the Drude model with the Matthiessen's rule works well for DC electron transport and low-frequency optical response. This breaks down at higher frequencies, where a volumetric mix of pure-species AC conductivities works better.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Particle Scattering in the Resonance Regime: Full-Wave Solution for Axisymmetric Particles with Large Aspect Ratios

Reliable descriptions of the optical properties of clouds and aerosols are essential for studies of radiative transfer in planetary atmospheres. The scattering algorithms provide accurate estimates of these properties for spherical particles with a wide range of sizes and refractive indices, but these methods are not valid for non-spherical particles (e.g., ice crystals, mineral dust, and smoke). Even though a host of methods exist for deriving the optical properties of nonspherical particles that are very small or very large compared with the wavelength, only a few methods are valid in the resonance regime, where the particle dimensions are comparable with the wavelength. Most such methods are not ideal for particles with sharp edges or large axial ratios. We explore the utility of an integral equation approach for deriving the single-scattering optical properties of axisymmetric particles with large axial ratios. The accuracy of this technique is shown for spheres of increasing size parameters and an ensemble of randomly oriented prolate spheroids of size parameter equal to 10.079368. In this last case our results are compared with published results obtained with the T-matrix approach. Next we derive cross sections, single-scattering albedos, and phase functions for cylinders, disks, and spheroids of ice with dimensions extending from the Rayleigh to the geometric optics regime. Compared with those for a standard surface integral equation method, the storage requirement and the computer time needed by this method are reduced, thus making it attractive for generating databases to be used in multiple-scattering calculations. Our results show that water ice disks and cylinders are more strongly absorbing than equivalent volume spheres at most infrared wavelengths. The geometry of these particles also affects the angular dependence of the scattering. Disks and columns with maximum linear dimensions larger than the wavelength scatter much more radiation in the forward and backward directions and much less radiation at intermediate phase angles than equivalent volume spheres.

Zuffada, Cinzia↗

Assessment of Global Cloud Datasets from Satellites: Project and Database Initiated by the GEWEX Radiation Panel

Clouds cover about 70% of the Earth's surface and play a dominant role in the energy and water cycle of our planet. Only satellite observations provide a continuous survey of the state of the atmosphere over the whole globe and across the wide range of spatial and temporal scales that comprise weather and climate variability. Satellite cloud data records now exceed more than 25 years in length. However, climatologies compiled from different satellite datasets can exhibit systematic biases. Questions therefore arise as to the accuracy and limitations of the various sensors. The Global Energy and Water cycle Experiment (GEWEX) Cloud Assessment, initiated in 2005 by the GEWEX Radiation Panel, provided the first coordinated intercomparison of publically available, standard global cloud products (gridded, monthly statistics) retrieved from measurements of multi-spectral imagers (some with multiangle view and polarization capabilities), IR sounders and lidar. Cloud properties under study include cloud amount, cloud height (in terms of pressure, temperature or altitude), cloud radiative properties (optical depth or emissivity), cloud thermodynamic phase and bulk microphysical properties (effective particle size and water path). Differences in average cloud properties, especially in the amount of high-level clouds, are mostly explained by the inherent instrument measurement capability for detecting and/or identifying optically thin cirrus, especially when overlying low-level clouds. The study of long-term variations with these datasets requires consideration of many factors. A monthly, gridded database, in common format, facilitates further assessments, climate studies and the evaluation of climate models.

Stubenrauch, C. J.↗

New quantum physics, solving puzzles of Wheeler’s delayed choice and a particle’s passing N slits simultaneously and quantum oscillator in experiments

Abstract This paper discovers new quantum physics, and gives solutions to puzzles of Wheeler’s delayed choice and a particle’s passing many slits simultaneously by exact quantum physics expressions. We further show new quantum control, new quantum oscillation, new quantum control experiments and new quantum oscillator being able to be installed in quantum communication network etc. We discover that the ability of a photon to hit electrons out in photoelectric effect is complementarily equivalent to the ability of wave of a photon to simultaneously pass through many slits in wave-particle duality. Objective criterion for distinguishing classical and quantum particles is found, and this paper gives applicable realm of quantum theories and new quantum physics expressions of wave-particle duality. All these studies above should be classified as classical and quantum particles, then classical particle and quantum particle wave cannot and can pass many slits, respectively. This paper discovers wave-particle duality’s origin of displaying both wave property from plane wave part of the general Fourier expansion and particle property from the general Fourier expansion coefficients with the particle’s global property and spins etc. We give the superposition state representation of wave-particle duality, further find the collapse of the duality superposition state to wave or particle state. The collapsed wave or particle state is related to the measure of wave or particle property. Then, we explain why sometimes it's a wave or a particle. Our achieved results are truly tested, and we discover new measured attractive state and quantum wave collapse velocity expression.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Investigation of resistive magnetic field generation by intense proton beams in dense plasmas

Current and future applications of intense proton sources abound, including radiography, cancer therapy, warm dense matter generation, and inertial confinement fusion. With increasingly efficient acceleration and focusing mechanisms, proton current densities may soon approach and exceed 10 10 A/cm 2 , e.g., via intense laser drivers. Simulations have previously shown that in this current density regime, beam-induced field generation plays a significant role in beam transport through dense plasmas. Here, we present a theoretical model for the generation of resistive magnetic fields by intense proton beam transport through solid density plasmas. The theoretical evolution of the magnetic field profile is calculated using an analytic model for aluminum resistivity, heat capacity, and stopping power, applicable from cold matter to hot plasma. The effects of various beam and material parameters on the field are investigated and explained for both monoenergetic and Maxwellian proton beams. For a proton beam with Maxwellian temperature 5 MeV and total energy 10 J, the model calculates resistive magnetic fields up to 150 T in aluminum. In conclusion, the calculated field profiles from several beam cases are compared with 2D hybrid particle-in-cell simulations, with good agreement found in magnitude and time scale.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Particle Size Effects on Flow Properties of PS304 Plasma Spray Feedstock Powder Blend

The effects of BaF2-CaF2 particle size and size distribution on PS304 feedstock powder flowability have been investigated. Angular BaF2-CaF2 eutectic powders were produced by comminution and classified by screening to obtain 38 to 45 microns 45 to 106 microns, 63 to 106 microns, 45 to 53 microns, 63 to 75 microns, and 90 to 106 microns particle size distributions. The fluorides were added incrementally from 0 to 10 wt% to the other powder constituents of the PS304 feedstock: nichrome, chromia, and silver powders. The flow rate of the powder blends decreased linearly with increasing concentration of the fluorides. Flow was degraded with decreasing BaF2-CaF2 particle size and with increasing BaF2-CaF2 particle size distribution. A semiempirical relationship is offered to describe the PS304 powder blend flow behavior. The Hausner Ratio confirmed the funnel flow test results, but was slightly less sensitive to differences in BaF2-CaF2 particle size and size distribution. These findings may have applicability to other powders that do not flow easily, such as ceramic powders.

Stanford, Malcolm K.↗

A precise electron EDM constraint on CP-odd heavy-quark Yukawas

CP-odd Higgs couplings to bottom and charm quarks arise in many extensions of the standard model and are of potential interest for electroweak baryogenesis. These couplings induce a contribution to the electron EDM. The experimental limit on the latter then leads to a strong bound on the CP-odd Higgs couplings. We point out that this bound receives large QCD corrections, even though it arises from a leptonic observable. We calculate the contribution of CP-odd Higgs couplings to the bottom and charm quarks in renormalisation-group improved perturbation theory at next-to-leading order in the strong interaction, thereby reducing the uncertainty to a few percent.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Impact of the cosmic neutrino background on long-range force searches

Light bosons can mediate long-range forces. We show that light bosonic mediators interacting with a background medium, in particular, with the cosmic neutrino background (CνB), may induce medium-dependent masses which could effectively screen long-range forces from detection. This leads to profound implications for long-range force searches in e.g. the Eöt-Wash, MICROSCOPE, and lunar laser-ranging (LLR) experiments. For instance, we find that when the coupling of the mediator to neutrinos is above 3 × 10 −10 or 5 × 10 −13 , bounds from LLR and experiments employing the Sun as an attractor, respectively, would be entirely eliminated. Larger values of the coupling can also substantially alleviate bounds from searches conducted at shorter distances.

79 ASTRONOMY AND ASTROPHYSICS↗

Optical-Microphysical Cirrus Model

A model is presented that permits the simulation of the optical properties of cirrus clouds as measured with depolarization Raman lidars. It comprises a one-dimensional cirrus model with explicit microphysics and an optical module that transforms the microphysical model output to cloud and particle optical properties. The optical model takes into account scattering by randomly oriented or horizontally aligned planar and columnar monocrystals and polycrystals. Key cloud properties such as the fraction of plate-like particles and the number of basic crystals per polycrystal are parameterized in terms of the ambient temperature, the nucleation temperature, or the mass of the particles. The optical-microphysical model is used to simulate the lidar measurement of a synoptically forced cirrostratus in a first case study. It turns out that a cirrus cloud consisting of only monocrystals in random orientation is too simple a model scenario to explain the observations. However, good agreement between simulation and observation is reached when the formation of polycrystals or the horizontal alignment of monocrystals is permitted. Moreover, the model results show that plate fraction and morphological complexity are best parameterized in terms of particle mass, or ambient temperature which indicates that the ambient conditions affect cirrus optical properties more than those during particle formation. Furthermore, the modeled profiles of particle shape and size are in excellent agreement with in situ and laboratory studies, i.e., (partly oriented) polycrystalline particles with mainly planar basic crystals in the cloud bottom layer, and monocrystals above, with the fraction of columns increasing and the shape and size of the particles changing from large thin plates and long columns to small, more isometric crystals from cloud center to top. The findings of this case study corroborate the microphysical interpretation of cirrus measurements with lidar as suggested previously.

Reichardt, J.↗

Properties and effects of dust particles suspended in the Martian atmosphere

Direct measurements of the optical depth above the two Viking landers are presented for a period covering the summer, fall, and winter seasons in the Northern Hemisphere, a time period during which two global dust storms occurred. The data are used to define the properties of suspended dust particles in the Martian atmosphere and to assess their role in a number of meteorological and geological processes. Major conclusions are that (1) both the radiative effects of dust particles and the thermodynamical effects of large-scale atmospheric motions have a significant impact on the vertical temperature structure; (2) Pertinent feedback effects play an important part in the generation of some local dust storms, in the expansion of local dust storms to global proportions, and in the subsequent decay of global dust storms; (3) An important mechanism for the removal of dust particles from the atmosphere is the CO2 condensation-sedimentation process; and (4) that the polar laminae are constructed from atmospheric dust and water ice is hypothesized.

Pollack, J. B.↗