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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 307 records · Page 17
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Life Cycle of Major Sudden Stratospheric Warmings in the Southern Hemisphere from a Multimillennial GCM Simulation

Abstract Sudden stratospheric warmings (SSWs) are rare in the Southern Hemisphere (SH), making it difficult to study possible precursors or subsequent impacts. Using a multimillennial coupled climate model simulation producing 161 SSWs in the SH, we present a detailed study of their life cycle. We show that SH SSWs are predominantly displacement events forced by wave-1 planetary waves, and that a surface signature similar to the negative phase of the Southern Annular Mode (SAM) is detectable up to two months before the onset date, but there is a tendency for a transition from wave 1 before to zonally symmetric anomalies after onset. We identify a strong weakening of the Amundsen Sea low as one of the most prominent precursors, which weakens the climatological wave-2 and wave-3 stationary waves and strengthens wave-1 forcing. Compared to their northern counterparts, SH SSWs generally have a longer time scale, and while there is evidence of pre-onset forcing related to tropical sea surface temperatures, the Indian Ocean dipole is more important than El Niño–Southern Oscillation. Significance Statement Sudden stratospheric warmings (SSWs) are extreme events where the winter polar stratosphere warms within a few days to temperatures usually only experienced in summer. These events are rare in the Southern Hemisphere. Therefore, both the observational record and standard climate model simulations are not enough to understand how SSWs develop, or how they might change surface weather. Here we use very long global climate simulations that produce a large number of SSWs in the Southern Hemisphere to study the development and impact of these events. This includes possible precursors as well as the influence they have on surface weather after they occur.

Meteorology & Atmospheric Sciences↗
NASA NTRS1983

The low-lying 2-sigma-minus states of OH

The configuration-interaction method is used to determine the electronic wave functions of the two lowest 2-sigma-minus states of OH using four different atomic orbital basis sets. Potential energy curves, transition moments, oscillator strengths, and photodissociation cross sections are obtained. Electronic transition dipole moments connecting the excited 1 2-sigma-minus and 2(D)2-sigma-minus states with each other and with the ground chi-2-pi state are presented as functions of internuclear distance. The theoretical absorption oscillator strengths for the D-2-sigma-minus(v prime = 0) from chi-2-pi(v double prime = 0) transition are in good agreement with the empirical value derived from astronomical measurement. The photodissociation cross sections for absorption from the v prime = 0, 1, and 2 levels of the ground state into the continuum of the 1 2-sigma-minus state are calculated, and the interstellar and cometary photodissociation rates are derived.

Van Dishoeck, E. F.↗
NASA NTRS1983

The apparent spectral broadening of VLF transmitter signals during transionospheric propagation

ISIS 1 and 2 and ISEE 1 VLF/ELF electric field wave data indicate the existence of a novel phenomenon, in which initially narrow band upgoing signals from ground-based VLF transmitters undergo a significant spectral broadening as they propagate through the ionosphere and protonosphere, up to altitudes in the 600-3800 km range. For transmitter signals in the 10-20 kHz range, the spectral broadening can be as high as 10 percent of the input signal's nominal frequency. In many cases, the bandwidth of the spectrally broadened signals is a strong function of the electric dipole antenna orientation with respect to the local direction of the earth's magnetic field. The unusual dispersion in the components of the spectrally broadened pulses suggests that the spectral broadening may be due to a Doppler shift effect in which the initial signals scatter from irregularities in the F region and couple into quasi-electrostatic modes of short wave length.

Bell, T. F.↗
NASA NTRS1990

Linear and non-linear studies of Alfven waves in space. Stationary and dynamic processes in magnetospheric plasmas

The Final Technical Report on linear and non-linear studies of Alfven waves in space is presented. Areas of research included relaxation of magnetotail plasmas with field-aligned currents; the equilibrium dayside magnetosphere; macroscale particle simulation of kinetic Alfven wave physics; ballooning stability of plasmas with sheared equilibrium flows; theory of the drift-mirror instability; collisionless tearing instability in magnetotail plasmas; and nonadiabatic behavior of the magnetic moment of a charged particle in a dipole magnetic field and the development of stochastic webs.

Bhattacharjee, A.↗
NASA NTRS1976

Preliminary results on the apparent size of the sources of type III bursts observed at low frequencies

We present preliminary results on the apparent angular size of the sources of four type III bursts observed between 3500 and 50 kHz from the IMP-6 spacecraft. The observations were made with a dipole rotating in the plane of the ecliptic where the sources are assumed to be. The apparent angular sizes obtained are unexpectedly large. We discuss different explanations for the results. It seems that the scattering of radio waves by electron density inhomogeneities is the most likely cause. We report a temporal increase of the apparent angular size of the source during the burst lifetime for some bursts. From its characteristics it appears to be a real effect.

Alvarez, H.↗
NASA NTRS1987

Inhomogeneous cosmology. III - Primordial gravitational waves and dust

In this paper, the properties of a special class of inhomogeneous cosmological models and the interaction of the inhomogeneities with the evolution of the background geometry and matter are studied. The cosmological model is chosen so that the initial inhomogeneities evolve into 'plane' gravitational waves propagating through a smooth Bianchi I dust background. It is shown how the inhomogeneities interact with matter, 3 K radiation, and the background geometry, causing the expansion to slow down in some regions and speed up in others. It is also shown how the gravitational waves can produce a 'dragging of the inertial frame' which will affect the observed distribution of matter and 3 K radiation. In particular, this frame-dragging effect can account for a major fraction of the obsserved dipole component between the 3 K background radiation and the rest frame of global matter, an effect usually assumed to have been produced by large-scale local motion.

Adams, P. J.↗
DOE OSTI2025

Mitigation of ICRF—edge plasma interaction in Alcator C-Mod

The parasitic interaction between ion cyclotron range of frequencies (ICRF) waves and the edge plasma has long limited high-power ICRF utilization in magnetically confined fusion plasmas. In this paper, we report on the successful mitigation of this interaction by power tapering a four-strap field-aligned (FA) antenna in the Alcator C-Mod tokamak. With the antenna operated in dipole phasing ($0\pi0\pi$), the ratio of the power coupled by the central two straps ($P_\mathrm {cent}$) to the power coupled by the outer two straps was varied at fixed total coupled ICRF power ($P_\mathrm {tot}$). With $P_\mathrm {cent}$/$P_\mathrm {tot} \approx 0.8-0.9$, no enhancement of the plasma potential was measured despite 1 MW of coupled ICRF power. When the antenna is powered, energy deposition increases on its four corners and on neighboring limiter tiles magnetically connected to some of those corners. The energy deposited on the antenna and limiter is minimized together with near-field plasma potentials. Additionally, we show that deviation from $P_\mathrm {cent}$/$P_\mathrm {tot} \approx 0.8$ enhances wave-plasma interactions in places not magnetically connected to the antenna. These far-field effects are correlated with changes in the antenna spectrum. Hence, on C-Mod, near-field and far-field interactions were minimized for about the same range of $P_\mathrm {cent}$/$P_\mathrm {tot}$. Optimal power tapering was also found to improve ICRF heating efficiency and facilitate H-mode access. Finally, we show that the heat flux pattern on the toroidally aligned antennas reverses with the direction of the RF-induced E×B flow in front of the antenna, a correlation not observed for the FA antenna. We argue that the RF-induced E×B flow, which carries high-density plasma from the near-SOL, is aligned with the FA antenna and does not intercept its corners, where the plasma potential is large. This could explain the previously reported smaller impurity generation by the FA antenna (Wukitch et al 2013 Phys. Plasmas 20 056117).

Alcator C-Mod↗
DOE OSTI2024

Broadband Rotational Spectroscopy in Uniform Supersonic Flows: Chirped Pulse/Uniform Flow for Reaction Dynamics and Low Temperature Kinetics

ConspectusThe study of gas-phase chemical reactions at very low temperatures first became possible with the development and implementation of the CRESU (French acronym for Reaction Kinetics in Uniform Supersonic Flows) technique. CRESU relies on a uniform supersonic flow produced by expansion of a gas through a Laval (convergent-divergent) nozzle to produce a wall-less reactor at temperatures from 10 to 200 K and densities of 1016-1018 cm-3 for the study of low temperature kinetics, with particular application to astrochemistry. In recent years, we have combined uniform flows with revolutionary advances in broadband rotational spectroscopy to yield an instrument that affords near-universal detection for novel applications in photodissociation, reaction dynamics, and kinetics. This combination of uniform supersonic flows with chirped-pulse Fourier-transform microwave spectroscopy (Chirped-Pulse/Uniform Flow, CPUF) permits detection of any species with a modest dipole moment, thermalized to the uniform temperature of the gas flow, with isomer, conformer, and vibrational state specificity. In addition, the use of broadband, high-resolution, and time-dependent (microsecond time scale) micro- and mm-wave spectroscopy makes it an ideal tool for characterizing both transient and stable molecules, as well as studying their spectroscopy and dynamics.In this Account, we review recent advances made using the CPUF technique, including studies of photodissociation, radical-radical reaction dynamics, and low temperature kinetics. These studies highlight both the strength of universal and multiplexed detection and the challenges of coupling it to a high-density collisional environment. Product branching and product evolution as a function of time have been measured for astrochemically relevant systems, relying on the detailed characterization of these flow conditions via experiments and fluid dynamics simulations. In the photodissociation of isoxazole, an unusual heterocyclic molecule with a very low-energy conical intersection, we have identified 7 products in 5 reaction channels and determined the product branching, pointing to both direct and indirect pathways. We have also approached the same system from separated NO and C3H3 reactants to explore a broader range of the potential energy surface, demonstrating the power of multichannel branching measurements for complex radical-radical reactions. We determined the product branching in the C3H2 isomers in the photodissociation of the propargyl radical and identified the importance of a hydrogen atom catalyzed isomerization to the lowest energy cyclic form. This then motivated a study of direct D-H exchange reaction in radicals, in which we demonstrate that it is an important and overlooked pathway for deuterium fractionation in astrochemical environments. Recently, we have shown the measurement of low temperature kinetics inside an extended Laval nozzle, after which a shock-free secondary expansion to low temperature and density affords an ideal environment for detection by rotational spectroscopy. These results highlight the power and potential of the CPUF approach, and future prospects will also be discussed in light of these developments.

Dias, Nureshan↗
NASA NTRS1990

Intraseasonal oscillations in the extratropics - Hopf bifurcation and topographic instabilities

A potential vorticity model in a beta-channel is used to analyze the resonant response of equivalent-barotropic flow to topography in the presence of a forced zonal jet with arbitrary meridional structure. The nonlinear dynamics near different resonances is studied considering both wave-wave and wave-zonal flow interactions. It is shown that Hopf bifurcations from stationary to periodic flows are possible due to the nonlinear instability of nonzonal, topographically forced flow. Low-frequency, finite-amplitude oscillations arise due to a combination of two factors: (1) nonlinear wave-wave interactions, which tend to reduce the Rossby wave frequency; and (2) wave-zonal flow interactions, which reflect the importance of wave momentum transport in shifting the westerly jet and of the topographic form drag. The physical mechanism of atmospherically realistic Hopf bifurcations depends crucially on the meridional profile of the mean zonal flow giving rise to a dipole-shaped resonance.

Jin, F.-F.↗
NASA NTRS1998

Radio Emissions Observed by Galileo near Io

The Galileo spacecraft observed spin modulation of radio wave emissions near Io in the frequency range from about 600 kHz to about 1.2 MHz. Assuming transverse EM radiation, we have used the modulation of the high-frequency sweep-frequency receiver signals of the electric dipole antenna over many spins to estimate the plane through the source. The emission has a range of frequencies close to the local upper hybrid frequency of the plasma near Io. We conclude that the emission may be associated with either the plasma torus or magnetic flux tubes in the wake of Io (the Alfven current system). We postulate this emission may be associated with a free-energy source such as density gradients, energetic plasma beams and/or an electron distribution with a temperature anisotropy. All of these free-energy sources are observed or expected in the torus near Io. The observations are the first in the hectometric frequency range that have a source associated with Io or in the Io torus.

Menietti, J. D.↗
DOE OSTI2023

Quantum beats in two-color photoionization to the spin-orbit split continuum of Ar

We report a study of the quantum beats in two-color photoionization of argon. An attosecond extreme ultraviolet pulse train prepares an electronic wave packet of definite odd parity, with total angular momentum J = 1, targeting the states between 14.0 and 14.5 eV from the ground state. Two-photon ionization of this wave packet with a tunable infrared probe pulse makes the constituent states interfere in both continuum channels, corresponding to the core angular momenta j c = 1/2 and 3/2, respectively. We analyze photoelectron spectrograms as a function of the time delay of the probe pulse and identify oscillations due to several pairs of states through Fourier decomposition. We observe phase differences between the corresponding beat signals in the two spin-orbit split continua. Comparison of theoretical simulations with the experimental measurements allows us to interpret the amplitudes and phases of ionization signals. Furthermore, we express the observed phase differences in terms of the off-diagonal elements of the short-range scattering matrix and the dipole matrix elements to the continuum eigenchannels.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2026

Eikonal spin-dependent odderon and gluon Sivers function of a proton and its small-𝑥 evolution

The matrix element in the proton of the eikonal Odderon operator, with a helicity flip, has been shown to correspond to the dipole gluon Sivers function. We employ a three quark light-front model of the proton to determine the Sivers function at moderately small 𝑥 0 ∼ 0.1 and transverse momentum 𝑘 ⊥ ≲ 1 GeV. The model light-cone (LC) wave function predicts the properties of 𝑥⁢𝑓$^{⊥⁢𝑔}_{1⁢𝑇⁡}$(𝑥,𝑘 ⊥ ) such as its overall magnitude, the position of its peak in 𝑘 ⊥ , and its behavior at small 𝑘 ⊥ . We then compute numerically the Balitsky-Fadin-Kuraev-Lipatov anomalous dimension characterizing the power-law tail at 𝑘 ⊥ ≳ 1.5 GeV of the gluon Sivers function at small (but preasymptotic) LC momentum fractions 𝑥 ∼ 𝑥 0 ⁢𝑒 −1/𝛼 𝑠 : 𝑥⁢𝑓$^{⊥⁢𝑔}_{1⁢𝑇⁡}$⁡(𝑥,𝑘 ⊥ ) ∼ 𝑘$^{−3.3}_{⊥}$.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1986

A modified coupled pair functional approach

A modified coupled pair functional (CPF) method is presented for the configuration interaction problem that dramatically improves properties for cases where the Hartree-Fock reference configuration is not a good zeroth-order wave function description. It is shown that the tendency for CPF to overestimate the effect of higher excitations arises from the choice of the geometric mean for the partial normalization denominator. The modified method is demonstrated for ground state dipole moment calculations of the NiH, CuH, and ZnH transition metal hydrides, and compared to singles-plus-doubles configuration interaction and the Ahlrichs et al. (1984) CPF method.

Chong, D. P.↗
DOE OSTI2021

Observation of Scale Invariance in Two-Dimensional Matter-Wave Townes Solitons

We report near-deterministic generation of two-dimensional (2D) matter-wave Townes solitons, and a precision test on scale invariance in attractive 2D Boses gases. We induce a shape-controlled modulational instability in an elongated 2D matter-wave to create an array of isolated solitary waves of various sizes and peak densities. We confirm scale invariance by observing the collapse of solitary-wave density profiles onto a single curve in a dimensionless coordinate rescaled according to their peak densities, and observe that the scale-invariant profiles measured at different coupling constants can further collapse onto the universal profile of Townes solitons. The reported scaling behavior is tested with a nearly 60-fold difference in soliton interaction energies, and allows us to discuss the impact of a non-negligible magnetic dipole-dipole interaction (MDDI) on 2D scale invariance. Here, we confirm that the effect of MDDI in our alkali cesium quasi-2D samples effectively conforms to the same scaling law governed by a contact interaction to well within our experiment uncertainty.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1980

Parity-violating electric-dipole transitions in helium

The paper examines parity-violating electric-dipole transitions in He in order to gain insight into the reliability of approximate calculations which are carried out for transitions in many-electron atoms. The contributions of the nearest-lying states are computed with a variety of wave functions, including very simple product wave functions, Hartree-Fock functions and Hylleraas-type wave functions with up to 84 parameters. It is found that values of the matrix elements of the parity-violating interaction can differ considerably from the values obtained from the good wave functions, even when these simple wave functions give accurate values for the matrix elements in question

Hiller, J.↗
DOE OSTI2021

Spin–Orbit Natural Transition Orbitals and Spin-Forbidden Transitions

Natural transition orbitals (NTOs) are in widespread use for visualizing and analyzing electronic transitions. Here, the present work introduces the analysis of formally spin-forbidden transitions with the help of complex-valued spin-orbit (SO) NTOs. The analysis specifically focuses on the components in such transitions that cause their intensity to be non-zero because of SO coupling. Transition properties such as transition dipole moments are partitioned into SO-NTO hole-particle pairs, such that contributions to the intensity from specific occupied and unoccupied orbitals are obtained. The method has been implemented within the restricted active space (RAS) self-consistent field wave function theory framework, with SO coupling treated by RAS state interaction. SO-NTOs have a broad range of potential applications, which is illustrated by the T 2 -S 1 state mixing in pyrazine, spin-forbidden vs. spin-allowed 4f–5d transitions in the Tb 3+ ion, and the phosphorescence of tris(2-phenylpyridine) iridium [Ir(ppy) 3 ].

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗