Theoretical investigation - The scattering of light by a planetary atmosphere Interim report, 22 Sep. - 22 Dec. 1965
Light scattering and polarization in planetary atmosphere
PLANETARY ATMOSPHERE↗
SEARCH · Engineering Papers
Results for “Optical Polarization”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Polarization - A key to an airborne optical system for the detection of oil on water.
Skylight polarization, which varies with the position of the sun in the sky, influences the contrast of oil on water. Good contrast is most consistently obtained by viewing in azimuth directions toward or away from the sun. Contrast is enhanced by imaging selected polarization components and by taking the difference between orthogonal polarization components.
Millard, J. P.↗
Polarizing 3 He via metastability exchange optical pumping using a 1.2 mbar sealed cell at magnetic fields up to 5 T
Here, we report high nuclear polarization of 1.2 mbar 3 He gas in a sealed cell in magnetic fields up to 5 T using Metastability Exchange Optical Pumping (MEOP). The creation of a highly polarized 3 He gas target for use in the 5 T field of Jefferson Lab’s CLAS12 spectrometer would enable new studies of spin-dependent asymmetries on the neutron. We describe a systematic study which was conducted for the first time up to the full 5 T field required for the final target design to evaluate the effects of discharge intensity, pump laser power, and optical pumping transition schemes on nuclear polarization and pumping rates. Steady-state polarizations up to 86% in magnetic fields between 2 and 5 T were achieved, with a discharge-on relaxation time of 898 s at 5 T. These results underscore the potential of MEOP for high-field applications in nuclear physics experiments.
3He polarization↗
Dark Exciton in 2D Hybrid Halide Perovskite Films Revealed by Magneto-Photoluminescence at High Magnetic Field
Here, a comprehensive study of the exciton fine structure (EFS) is presented in 2D-phenethylammonium lead iodide films using magnetic field-induced polarization of photoluminescence (PL) in both Faraday and Voigt configurations at fields up to 25 Tesla. Three exciton bands are identified in the PL spectrum associated with bound, dark, and bright excitons, respectively. Under a high magnetic field in Faraday/Voigt configuration, large field-induced circular/linear polarization is observed in the PL band related to the dark exciton, which is magnetically activated. Furthermore, it is found that the dark exciton has an anomalous field-induced circular polarization, which cannot be explained by the classical Boltzmann distribution of spin-polarized species. These findings are well explained by an effective mass model that includes exchange terms unique to the monoclinic symmetry as a perturbation of the EFS in the approximate tetragonal symmetry. It is also confirmed that the field-induced linear polarization is sensitive to the monoclinic exchange term, whereas the field-induced circular polarization is immune to such term.
14 SOLAR ENERGY↗
Wavelength dependence of polarization by small graphite flakes.
Wavelength dependence of polarization by small graphite flakes with anisotropic dielectric constant
OPTICAL POLARIZATION↗
Characteristics of optical emissions and particle precipitation in polar cap arcs
Auroral emission features at high geomagnetic latitudes are identified and characterized using simultaneous optical and particle data from the ISIS-2 satellite. Polar cap arcs are identified from two-dimensional geomagnetic transforms of the optical data along with precipitating electron data for the time at which the satellite is on the field line intersecting the arc. No precipitating protons were detected for any of the arc crossings. The precipitations particle characteristics include: (1) an electron energy spectrum with a peak in the range 350-750 eV superposed on a soft spectrum like that observed in polar rain; (2) a normally isotropic pitch angle dependence, with the exception that field-aligned fluxes are observed in association with an inverted 'v' event; and (3) an energy flux range of approximately 0.8-3 erg/(sq cm s). A possible explanation of the observed precipitating particle characteristics is that parallel electric fields are accelerating polar rain type spectra at an altitude of several thousand km.
Murphree, J. S.↗
Nonlinear optical response of metal-barrier-metal junctions
The optical response of metal-barrier-metal (MBM) junctions is discussed, with emphasis on the nonlinearity of response associated with reversal of polarity as optical intensity is increased. This nonlinear behavior can be used to measure correlation functions of optical pulses or to generate ultrashort electrical pulses. Expressions for the current flowing through the insulating barrier (junction), and for the rectification current, are given. Pulse signal and polarity of the electrical pulse evolves as the junction bias is varied about the null-signal bias. The apparatus used to obtain rectification pulse signals is described; the calculated evolution of the rectified pulse shape is found to correspond to that of pulse signals obtained experimentally. The generation of pulses six orders of magnitude smaller than a previously-obtained instrument-limited 1.6 nanosecond pulse has been observed.
Fan, B.↗
Simultaneous type-I and type-II phase matching for second-order nonlinearity in integrated lithium niobate waveguide
Second-order optical nonlinearity is widely used for both classical and quantum photonic applications. Due to material dispersion and phase matching requirements, the polarization of optical fields is pre-defined during the fabrication. Only one type of phase matching condition is normally satisfied, and this limits the device flexibility. Here, we demonstrate that phase matching for both type-I and type-II second-order optical nonlinearity can be realized simultaneously in the same waveguide fabricated from thin-film lithium niobate. This is achieved by engineering the geometry dispersion to compensate for the material dispersion and birefringence. The simultaneous realization of both phase matching conditions is verified by the polarization dependence of second-harmonic generation. Correlated photons are also generated through parametric down conversion from the same device. This work provides a novel approach to realize versatile photonic functions with flexible devices.
Briggs, Ian↗
Ultraviolet spectropolarimetry of high redshift quasars with the Hubble Space Telescope
Ultraviolet spectropolarimetry of three bright high-redshift low polarization quasars (LPQ's) was obtained with the Faint Object Spectrograph of the Hubble Space Telescope. Two of the quasars, PG 1634+706 and PG 2302+029, had polarizations of rho is approximately equal to 0.5-1.0 percent throughout the ultraviolet, and showed no significant variation of polarization amplitude or position angle with wavelength. PG 2302+029 was also marginally (2.4 sigma) circularly polarized in the optical continuum. For the highest redshift quasar, PG 1222+228 (Ton 1530), the polarization was measured down to rest wavelengths below 800 A. Although the continuum of PG 1222+228 was weakened by Lyman limit absorption from an intergalactic gas cloud, the polarization increased sharply from 1 percent to about 4.5 percent, a change of 4 sigma significance. This abrupt rise in polarization does not appear attributable to any known instrumental artifact. These UV polarizations were only slightly less than those previously observed for these same objects in the optical. The polarization spectra were flat with a typical slope of the polarized flux pF(sub upsilon) varies as upsilon(exp -0.8 plus or minus 0.5). Unlike the polarization spectra of several high luminosity Seyfert 1 nuclei studied previously, such a flat wavelength dependence of polarization cannot be explained by scattering from dust grains. The hypotheses that the polarization in these quasars is produced by transmission through aligned interstellar grains (in the Milky Way or the host galaxy), or by a synchrotron power law component, also appear to be ruled out. These observed spectra are consistent with a wavelength-independent polarization proportional to the total nonstellar light or, possibly, to the contribution of the blue thermal component.
Impey, Chris D.↗
Ultraviolet spectropolarimetry of high-redshift quasars with the Hubble Space Telescope
Ultraviolet spectropolarimetry of three bright high-redshift low-polarization quasars (LPQs) was obtained with the Faint Object Spectrograph of the Hubble Space Telescope (HST). Two of the quasars, PG 1634+706 and PG 2302+029, had polarizations p approximately = 0.5%-1.0% throughout the ultraviolet, and showed no significant variation of polarization amplitude or position angle with wavelength. PG 2302+029 was also marginally (2.4 sigma) circularly polarized in the optical continuum. For the highest redshift quasar, PG 1222+228 (Ton 1530), the polarization was measured down to rest wavelengths below 800 A. Although the continuum of PG 1222+228 was weakened by Lyman limit absorption from an intergalactic gas cloud, the polarization increased sharply from 1% to about 4.5%, a change of 4 sigma significance. This abrupt rise in polarization does not appear attributable to any known instrumental artifact. These UV polarizations were only slightly less than those previously observed for these same objects in the optical. The polarization spectra were flat with a typical slope of the polarized flux pF(sub nu) proportional to nu(exp -0.8 +/- 0.5). Unlike the case of several high luminosity Seyfert 1 nuclei studied previously, polarization caused by scattering from dust grains does not provide the best fit to the polarization spectra of these luminous quasars. These observed spectra are consistent with a wavelength-independent polarization proportional to the total nonstellar light or, possibly, to the contribution of the blue thermal component. The polarization spectra have insufficient signal-to-noise to locate the scatterers with respect to the continuum source and the much larger broad line region. A decrease in amplitude and rotation of the position angle of the polarization vector at the shortest wavelengths, which could result from general relativistic effects near a spinning black hole, was not observed. In fact, in PG 1222+228, the polarization was observed to increase at the shortest wavelengths. The rise in polarization with frequency is so sharp that it cannot be due to any wavelength-independent polarizing mechanism at any radius in an accretion disk. Such a rise could be attributable, for example, to a relative increase in scattering opacity over absorption at higher frequencies.
Impey, C. D.↗
Constitutive Modeling of the Mechanical Properties of Optical Fibers
Micromechanical modeling of the composite mechanical properties of optical fibers was conducted. Good agreement was obtained between the values of Young's modulus obtained by micromechanics modeling and those determined experimentally for a single mode optical fiber where the wave guide and the jacket are physically coupled. The modeling was also attempted on a polarization-maintaining optical fiber (PANDA) where the wave guide and the jacket are physically decoupled, and found not to applicable since the modeling required perfect bonding at the interface. The modeling utilized constituent physical properties such as the Young's modulus, Poisson's ratio, and shear modulus to establish bounds on the macroscopic behavior of the fiber.
Moeti, L.↗
Valley-selective optical Stark effect of exciton-polaritons in a monolayer semiconductor
Selective breaking of degenerate energy levels is a well-known tool for coherent manipulation of spin states. Though most simply achieved with magnetic fields, polarization-sensitive optical methods provide high-speed alternatives. Exploiting the optical selection rules of transition metal dichalcogenide monolayers, the optical Stark effect allows for ultrafast manipulation of valley-coherent excitons. Compared to excitons in these materials, microcavity exciton-polaritons offer a promising alternative for valley manipulation, with longer lifetimes, enhanced valley coherence, and operation across wider temperature ranges. Here, we show valley-selective control of polariton energies in WS 2 using the optical Stark effect, extending coherent valley manipulation to the hybrid light-matter regime. Ultrafast pump-probe measurements reveal polariton spectra with strong polarization contrast originating from valley-selective energy shifts. This demonstration of valley degeneracy breaking at picosecond timescales establishes a method for coherent control of valley phenomena in exciton-polaritons.
36 MATERIALS SCIENCE↗
A Methodology for Surface Soil Moisture and Vegetation Optical Depth Retrieval Using the Microwave Polarization Difference Index
A methodology for retrieving surface soil moisture and vegetation optical depth from satellite microwave radiometer data is presented. The procedure is tested with historical 6.6 GHz brightness temperature observations from the Scanning Multichannel Microwave Radiometer over several test sites in Illinois. Results using only nighttime data are presented at this time, due to the greater stability of nighttime surface temperature estimation. The methodology uses a radiative transfer model to solve for surface soil moisture and vegetation optical depth simultaneously using a non-linear iterative optimization procedure. It assumes known constant values for the scattering albedo and roughness. Surface temperature is derived by a procedure using high frequency vertically polarized brightness temperatures. The methodology does not require any field observations of soil moisture or canopy biophysical properties for calibration purposes and is totally independent of wavelength. Results compare well with field observations of soil moisture and satellite-derived vegetation index data from optical sensors.
Owe, Manfred↗
The Far-Infrared Polarization Spectrum: First Results and Analysis
We present data on the polarization of the thermal emission from Galactic Clouds at 60 micrometers, 100 micrometers, and 350 micrometers. There are examples of rising polarization spectra in dense cloud cores [P(350 micrometers/P(100 micrometers) approximately equal to 2], and falling spectra in cloud envelopes [P(350)/P(100 micrometers) approximately equal to 0.6]. We also present data showing that the relationship, P(tau), between polarization and optical depth in cloud cores is different from that in cloud envelopes. We review the principles governing the far-infrared polarization spectrum and discuss applications to the data on P(lambda) and P(tau). We conclude that the cloud envelopes we have observed must contain two populations of grains that differ in their polarization efficiencies and in their emission spectra. We propose a model for cloud envelopes in which the contrasting populations reside in domains of different mean temperatures where the warmer domains contain the aligned grains.
Hildebrand, R. H.↗
Thin film processing of photorefractive BaTiO3
During the period covered by this report, October 11, 1991 through October 10, 1992, the research has progressed in a number of different areas. The sol-gel technique was initially studied and experimentally evaluated for depositing films of BaTiO3. The difficulties with the precursors and the poor quality of the films deposited lead to the investigation of pulsed laser deposition as an alternative approach. The development of the pulsed laser deposition technique has resulted in continuous improvements to the quality of deposited films of BaTiO3. The initial depositions of BaTiO3 resulted in amorphous films, however, as the pulsed laser deposition technique continued to evolve, films were deposited in the polycrystalline state, then the textured polycrystalline state, and most recently heteroepitaxial films have also been successfully deposited on cubic (100) oriented SrTiO3 substrates. A technique for poling samples at room temperature and in air is also undergoing development with some very preliminary but positive results. The analytical techniques, which include x-ray diffraction, ferroelectric analysis, UV-Vis spectrophotometry, scanning electron microscopy with x-ray compositional analysis, optical and polarized light microscopy, and surface profilometry have been enhanced to allow for more detailed evaluation of the samples. In the area of optical characterization, a pulsed Nd:YAG laser has been incorporated into the experimental configuration. Now data can also be acquired within various temporal domains resulting in more detailed information on the optical response of the samples and on their photorefractive sensitivity. The recent establishment of collaborative efforts with two departments at Johns Hopkins University and the Army Research Lab at Fort Belvoir has also produced preliminary results using the metallo-organic decomposition technique as an alternative method for thin film processing of BaTiO3. RF and DC sputtering is another film deposition approach that should be initiated in the near future. Other techniques for optical characterization, which may even allow for intragrannular (within single grains) investigations, are also being considered.
Schuster, Paul R.↗
Multifunctional Cu 2 TSiS 4 (T = Mn and Fe): Polar Semiconducting Antiferromagnets with Nonlinear Optical Properties
In this work, Cu 2 TSiS 4 (T = Mn and Fe) polycrystalline and single-crystal materials were prepared with high-temperature solid-state and chemical vapor transport methods, respectively. The polar crystal structure (space group Pmn2 1 ) consists of chains of corner-sharing and distorted CuS 4 , Mn/FeS 4 , and SiS 4 tetrahedra, which is confirmed by Rietveld refinement using neutron powder diffraction data, X-ray single-crystal refinement, electron diffraction, energy-dispersive X-ray spectroscopy, and second harmonic generation (SHG) techniques. Magnetic measurements indicate that both compounds order antiferromagnetically at 8 and 14 K, respectively, which is supported by the temperature-dependent (100–2 K) neutron powder diffraction data. Additional magnetic reflections observed at 2 K can be modeled by magnetic propagation vectors k = (1/2,0,1/2) and k = (1/2,1/2,1/2) for Cu 2 MnSiS 4 and Cu 2 FeSiS 4 , respectively. The refined antiferromagnetic structure reveals that the Mn/Fe spins are canted away from the ac plane by about 14°, with the total magnetic moments of Mn and Fe being 4.1(1) and 2.9(1) μ B , respectively. Both compounds exhibit an SHG response with relatively modest second-order nonlinear susceptibilities. Density functional theory calculations are used to describe the electronic band structures.
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
Multi-Frequency Observations of Gamma-Ray Blazar 1633 plus 382
We perform monthly monitoring of the quasar 1633+382 (4C+38.41) within a sample of gamma-ray blazars with the VLBA at 43 GHz along with optical photometric and polarimetric observations. We construct the gamma-ray light curve of 1633+382 using data obtained by the Fermi LAT. We find that a high gamma-ray state of the quasar starting in 2009 September is simultaneous with an increase of the flux in the mm-wave VLBI core. We resolve a superluminal feature on the VLBA images that appears to be responsible for the mm-wave flux increase. We find a strong correlation between optical and gamma-ray light curves with a delay of gamma-ray variations of 5+/-3 days, as well as a strong correlation between optical flux and degree of polarization during the high gamma-ray state. Comparison between the optical polarization position angle and that in the VLBI core supports the idea that in the quasar 1633+382 a high gamma-ray state is connected with processes originating near the mm-VLBI core.
Jorstad, S. G.↗
The infrared polarization of the infrared star in Cygnus.
Wavelength dependence of polarization of IR star in Cygnus measured by far IR lead sulfide photopolarimeter
POLARIMETRY↗