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At least 307 records · Page 17

Solar gamma rays

Calculations are presented for the production of gamma-ray lines and continuum emission in solar flares. The interaction models used in the calculations are described, neutron-producing reactions are identified, and formation of the 2.2-MeV line is analyzed. The most important prompt gamma-ray lines that can be observed during solar flares are determined, and the production of gamma-ray continuum emission by electron-proton bremsstrahlung is examined. The results are compared with data on the solar flare of August 4, 1972, to deduce the number and spectrum of accelerated particles at the sun as well as the energy deposited by them in the solar atmosphere. Problems concerning the formation of the 0.51-MeV line by positron annihilation are investigated, and estimates are made for the high-energy gamma-ray and neutron fluxes (at earth) produced by the August 4 flare. The main findings for that flare are: (1) the strongest line, at 2.2 MeV, was due to neutron capture by protons in the photosphere; (2) the intensity of that line depended on the photospheric He-3 abundance; (3) the neutrons were produced mainly in proton-alpha reactions by accelerated particles with energies in excess of 30 MeV/nucleon; and (4) the strongest prompt lines were due to deexcitation of excited states in C-12, O-16, and N-15.

Ramaty, R.↗

IER-620 CED-3b: Experiment Execution Summary for the Pulsed-Neutron Die-Away Experiments (PNDA) with Propylene Glycol and Mobilmet 423

There is a strong need for new benchmarks to validate neutron thermal scattering laws (TSLs). Lawrence Livermore National Laboratory (LLNL) has designed a Pulsed-Neutron Die Away (PNDA) testbed for this purpose. The experiment has a deuterium-tritium (D-T) neutron generator that impinges a 10 -4 s, mono-energetic pulse of 14.1 MeV neutrons on a target sample. After the pulse, the neutron population moderates and establishes a thermal equilibrium within the sample, with a fundamental spatial mode and characteristic decay-time eigenvalue, ⍺. The ⍺ eigenvalue can be extracted from the experimental measurements of the time-dependent neutron flux coming off the surface of the sample and can then be used as an integral parameter (similar to k eff ) to validate nuclear data involved with neutron migration, thermalization, and absorption. For moderating materials and geometric configurations, the ⍺ eigenvalue is heavily dependent on thermal neutron scattering of the target material. For that reason, a PNDA experiment can have a higher sensitivity to TSLs than is commonly available with the k eff parameter in critical experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Technical Documents for Gateway for Accelerated Innovation in Nuclear (GAIN)

The Gateway for Accelerated Innovation in Nuclear (GAIN) provides the nuclear energy community with access to the technical, regulatory, and financial support necessary to move new or advanced nuclear reactor designs toward commercialization. GAIN provides the nuclear community with a single point of access to the broad range of capabilities (i.e., people, facilities, materials, and data) across the U.S. Department of Energy (DOE) complex and its National Lab capabilities. The Fast Flux Test Facility (FFTF) is the most recent liquid metal reactor (LMR) to be designed, constructed, and operated by DOE. The 400-MWt sodium-cooled, fast-neutron flux reactor plant was designed for irradiation testing of nuclear reactor fuels and materials for liquid metal fast breeder reactors. Following the demise of the breeder reactor program in the United States, FFTF continued to play a key role in providing a test bed for demonstrating performance of advanced fuel designs and demonstrating operation, maintenance, and safety of advanced liquid metal reactors. The FFTF Program provides valuable information for potential follow-on reactor projects in the areas of plant system and component design, component fabrication, fuel design and performance, reactor control, prototype testing, and site construction. This report provides documents related to three important aspects of FFTF design and operation: 1) irradiation behavior of structural alloys and absorber materials, 2) thermohydraulics of rod bundles (i.e., coolant mixing), and 3) natural circulation heat transfer in the areas of modeling and validation. These technical documents are believed to be of interest to the nuclear industry and in particular to designers of new liquid metal reactors.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Assessment of the Impact of Realistic Sensor Physics and the Integration of Ex-Core Sensors on Reactor Power Synthesis

In the work documented in this report, a weighting function–based core power synthesis method was applied to multiple Monte Carlo N-Particle (MCNP) reactor models, which are informed based on simulated self-powered neutron detector (SPND) responses. The weighting function method used has been coined the point-based iterative (PBI) method. The goal of this application is to assess the impact of considering realistic sensor physics in the generation of the simulated SPND outputs as well as to consider how the synthesis is impacted based on the inclusion of ex-core detectors in the model. The NuScale small modular reactor (SMR) and Westinghouse AP1000 pressurized water reactor (PWR) are the models that served as the testbeds for the assessment of realistic sensor physics; this was achieved by using Geant4 SPND models in comparison with analytical models, such that the effect of electron transport in realistic SPND geometries in the Geant4 model can be understood in terms of synthesis error and convergence time. The comparison was considered for fuel burnup–induced perturbations, for a range of sensor string densities and synthesized power distribution axial fidelities. The Texas A&M Testing, Research, Isotopes, General Atomics Reactor (TAMU TRIGA) reactor MCNP model was used to assess the impact of ex-core sensors; this was done by performing synthesis with and without the ex-core detectors and by quantifying the synthesis error and number of iterations associated with Gaussian-type perturbations in many locations in the core. The TAMU TRIGA model was particularly pertinent for this study because of the interest in future experimental tests with SPNDs in this reactor, as well as the ease of modifying the MCNP model to include ex-core detectors with heterogeneously described response functions. Results from the comparison between the Geant4 and analytical SPND models indicate that similar average and maximum synthesis errors were obtained for burnup-induced perturbations in both the NuScale SMR and the AP1000. This was true for a range of sensor string densities and axial fidelities. However, there were marked differences between both the Geant4 and analytically informed models in terms of the iterations required to converge on the synthesized power distribution. Namely, the Geant4-informed models tended to lead to fewer iterations, except for a few sensor–core configurations that had particularly numerous iterations. Results from the ex-core sensor assessment with the TAMU TRIGA model indicate that the inclusion of ex-core sensors drastically reduces the synthesis error of Gaussian-type perturbations close to the edge of the core, and it slightly reduces synthesis errors for perturbations closer to the center of the core. This was achieved with a minimal increase in computational cost—that is, the number of iterations required for convergence. The errors were identified to be in the same location as the perturbation in the core, indicating that the methodology remains robust for unperturbed regions of the core. A secondary result from this study with the TAMU TRIGA was yielded by analysis of the neutron flux levels in the in-core and ex-core sensor locations of the core; these flux levels indicate that SPNDs could be used as both in-core and ex-core sensors, so long as the emitter material is sensitive to thermal neutrons. The results from these studies provide a quantitative understanding of the importance of considering realistic sensor physics and including ex-core sensors to perform accurate and timely power distribution synthesis of a reactor core.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

MPACT 4.4 Theory Manual

MPACT is a three-dimensional (3D) full-core neutron transport code capable of calculating subpin power distributions. Calculations are based on the Boltzmann transport equation for neutron fluxes for problems in which the detailed geometrical configuration of fuel components such as the pellet and cladding are explicitly retained. The cross-section data needed for the neutron transport calculation are obtained directly from a multigroup cross section library, which has traditionally been used by lattice physics codes to generate few-group homogenized cross sections for nodal core simulators. Hence, MPACT assumes neither a priori homogenization nor group condensation for the full core spatial solution. The 3D MPACT transport solution can be obtained using the method of characteristics (MOC), which employs discrete ray tracing within each fuel pin. However, for practical reactor applications, the direct application of MOC to 3D core configurations requires an excessive amount of memory and computing time due to the very large number of rays. For practical 3D full-core calculations, MPACT commonly uses an approximate “2D/1D” method that treats the radial (x and y) variables differently from the axial (z) variable. In particular, the radial dependence of the solution is calculated using transport theory, and the axial dependence is calculated using diffusion or P 3 theory. The 2D/1D method requires the core to be divided into a vertical stack of axial slices with a thickness of Δ z ≈ 5–10 cm. Each axial slice is divided radially into coarse spatial cells with boundaries that usually constitute the pin cell boundaries, for which Δ x = Δ y ≈ 1.5 cm. Then, each coarse radial cell (pin cell) is divided into 50–100 fine radial cells, which resolve the angular flux in the fuel, cladding, and moderator regions.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Evidence for the Sequestration of Hydrogen-Bearing Volatiles Towards the Moons Southern Pole-Facing Slopes

The Lunar Exploration Neutron Detector (LEND) onboard the Lunar Reconnaissance Orbiter (LRO) detects a widespread suppression of the epithermal neutron leakage flux that is coincident with the pole-facing slopes (PFS) of the Moon's southern hemisphere. Suppression of the epithermal neutron flux is consistent with an interpretation of enhanced concentrations of hydrogen-bearing volatiles within the upper meter of the regolith. Localized flux suppression in PFS suggests that the reduced solar irradiation and lowered temperature on PFS constrains volatility to a greater extent than in surrounding regions. Epithermal neutron flux mapped with LEND's Collimated Sensor for Epithermal Neutrons (CSETN) was analyzed as a function of slope geomorphology derived from the Lunar Orbiting Laser Altimeter (LOLA) and the results compared to co-registered maps of diurnally averaged temperature from the Diviner Lunar Radiometer Experiment and an averaged illumination map derived from LOLA. The suppression in the average south polar epithermal neutron flux on equator-facing slopes (EFS) and PFS (85-90 deg S) is 3.3 +/- 0.04% and 4.3 +/- 0.05% respectively (one-sigma-uncertainties), relative to the average count-rate in the latitude band 45-90 deg S. The discrepancy of 1.0 +/- 0.06% between EFS and PFS neutron flux corresponds to an average of approximately 23 parts-per-million-by-weight (ppmw) more hydrogen on PFS than on EFS. Results show that the detection of hydrogen concentrations on PFS is dependent on their spatial scale. Epithermal flux suppression on large scale PFS was found to be enhanced to 5.2 +/- 0.13%, a discrepancy of approximately 45 ppmw hydrogen relative to equivalent EFS. Enhanced poleward hydration of PFS begins between 50 deg S and 60 deg S latitude. Polar regolith temperature contrasts do not explain the suppression of epithermal neutrons on pole-facing slopes. The Supplemental on-line materials include supporting results derived from the uncollimated Lunar Prospector Neutron Spectrometer and the LEND Sensor for Epithermal Neutrons.

Ices↗

Long-Length SiC/SiC Tube Irradiation Experiment at LWR Temperatures Inserted into HFIR

This report describes the pre-irradiation characterization and successful assembly of a High Flux Isotope Reactor (HFIR) irradiation experiment designed to assess radiation-induced lateral bowing of silicon carbide fiber–reinforced, silicon carbide matrix composite (SiC/SiC) components under a radial fast neutron flux gradient at representative light-water reactor (LWR) temperatures of approximately 300 °C. The over-arching goal of this work is to validate thermomechanical models of SiC/SiC composite fuel assembly distortion used to predict the extent of lateral bowing and dose at which bowing reaches a maximum value. Ultimately, these models are used to ensure that fuel assembly distortion does not block coolant channels, interfere with control rod/blade movements, and/or impact local reactivity. The experiment contains six cladding tube specimens that are approximately 558.5 mm long with representative pressurized water reactor (PWR) outer and inner diameters of 9.5 mm and 7.5 mm, respectively. The specimens were thoroughly characterized prior to irradiation using traditional dimensional inspection and surface profilometry so that these measurements can later be compared with similar measurements that will be made post-irradiation to determine radiation-induced deformations. Furthermore, fine engraving markers were inscribed along the outer surfaces of the specimen and mapped using analytic photography and a three-dimensional stage. This technique allowed for accurate measurements of the marker spacings, which can be compared with similar measurements that will be made post-irradiation to provide local radiation-induced strain mapping. A light curtain optical micrometer was also employed to measure the pre-irradiation bowing of each specimen. The experiment was successfully assembled and inserted into position VXF-19 for HFIR cycle 516, which began May 12, 2026. The experiment will be removed after cycle 519, which is currently scheduled to end in December 2026.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Yield and PDV Measurements of the Godiva-IV Critical Assembly

A high dynamic range, scinillator based detector, the MHD-240, was used to measure the gamma and neutron flux of several prompt critical bursts of the Godiva-IV assembly. The measurements provided the alpha and FWHM for several different burst temperatures. Calibrations of the MHD240 gamma and neutron sensitivity along with MCNP based simulation of the Godiva-IV assembly allowed us to also determine the total fission yield of the burst integrated over approximately 5 ms. In addition a Photo Doppler Velocimetry measurement was conducted to determine the surface motion vibrational frequency of Godiva-IV assembly during the bursts. The combined data were collected to be used as input to multi-physics simulation of the Godiva-IV assembly. This is a preliminary report, there is an ongoing effort to update the MCNP simulations used in the analysis and develop a correction for the room return component of the measured signal.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Yield and PDV Measurements of the Godiva-IV Critical Assembly (Preliminary Report)

A high dynamic range, scinillator based detector, the MHD-240, was used to measure the gamma and neutron flux of several prompt critical bursts of the Godiva-IV assembly. The measurements provided the alpha and FWHM for several different burst temperatures. Calibrations of the MHD240 gamma and neutron sensitivity along with MCNP based simulation of the Godiva-IV assembly will allow us to also determine the total fission yield of the burst integrated over approximately 5 ms. Work is ongoing to check the calibrations of the MHD-240, and improve the MCNP simulations. This is a preliminary report, and the fission yields reported here are not final and are likely inaccurate. The measured alpha and FWHM are not impacted by the calibration issues and are considered final.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Calculated angular distributions of energetic atmospheric neutrons

Calculated angular distributions of atmospheric leakage neutron fluxes from 19 MeV to 1 GeV are presented. Comparisons with the balloon measurements of Preszler et al. and Kanbach et al. are made and show substantial agreement, strengthening the belief in the importance of the CRAND (cosmic-ray albedo-neutron decay) contribution to the high-energy protons in the earth's inner radiation belt. The calculation is presented as a means for investigating features of atmospheric flux distributions.

Merker, M.↗

The Random Ray Method Versus Multigroup Monte Carlo: The Method of Characteristics in OpenMC and SCONE

The Random Ray Method (TRRM) is a recently developed approach to solving neutral particle transport problems based on the Method of Characteristics. While the method previously has been implemented only in closed-source or limited-functionality codes, this work describes its implementation in two open-source Monte Carlo codes: OpenMC and SCONE. The random ray implementations required small modifications to the existing Multigroup Monte Carlo (MGMC) solvers, offering a rare venue for redundant, fine-grained, "apples-to-apples" speed and accuracy comparisons between transport methods. To this end, TRRM and MGMC solvers are evaluated against each other using each code's native capabilities on reactor eigenvalue problems with different degrees of energy discretization. On the C5G7 benchmark (featuring only seven energy groups), TRRM achieves a maximum pin power error comparable to or lower than that of MGMC for a given run time. On a problem with 69 energy groups, MGMC is found to scale more efficiently, obtaining a lower pin power error for a given run time. However, the defining difference between the two transport methods is found to be their vastly different uncertainty distributions. Specifically, TRRM is found to maintain similar levels of accuracy and uncertainty throughout the simulation domain whereas MGMC can exhibit orders-of-magnitude greater errors in areas of the problem that feature low neutron flux. For instance, TRRM provided an up to 373 times speed advantage compared with MGMC for computing the flux in low-flux regions in the moderator surrounding the C5G7 core.

42 ENGINEERING↗

Neutron capture effects in lunar gadolinium and the irradiation histories of some lunar rocks.

The Gd isotopic composition in 19 lunar rock and soil samples from three Apollo sites is reported. The analytical techniques and the high precision mass spectrometric measurements are discussed. Enrichments in the Gd-158 oxide to G-157 oxide ratio due to neutron capture range up to 0.75%. Integrated 'thermal' neutron fluxes derived from the isotopic anomalies of Gd are compared with spallation Kr data from aliquot samples to construct a model which gives both average cosmic-ray irradiation depths and effective neutron exposure ages for some rocks. Rock 14310 is the first lunar sample where Kr anomalies due to resonance neutron capture in Br are observed. A Kr-81/Kr exposure age of 262 (plus or minus 7)m.y. is calculated for this rock.

Lugmair, G. W.↗

Aircraft Radiation Shield Experiments--Preflight Laboratory Testing

In the past, measurements onboard a research Boeing 57F (RB57-F) aircraft have demonstrated that the neutron environment within the aircraft structure is greater than that in the local external environment. Recent studies onboard Boeing 737 commercial flights have demonstrated cabin variations in radiation exposure up to 30 percent. These prior results were the basis of the present study to quantify the potential effects of aircraft construction materials on the internal exposures of the crew and passengers. The present study constitutes preflight measurements using an unmoderated Cf-252 fission neutron source to quantify the effects of three current and potential aircraft materials (aluminum, titanium, and graphite-epoxy composite) on the fast neutron flux. Conclusions about the effectiveness of the three selected materials for radiation shielding must wait until testing in the atmosphere is complete; however, it is clear that for shielding low-energy neutrons, the composite material is an improved shielding material over aluminum or titanium.

Singleterry, Robert C., Jr.↗

Report on Evolution of Inconel 718 Following HFIR Irradiation

The report presents the microstructure and mechanical properties of 3D printed Inconel 718 after irradiation in the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL) to assess its potential use as a structural material. The structural components near the outlets of several proposed reactor cores will experience significant neutron fluxes and outlet coolant temperatures ranging from the hot standby temperature of 300 °C to nearly 550 °C at the center of the part. These components must support the core in appropriate loading conditions and require structural analysis at relevant temperatures. In FY21, three heat treatments were designed and conducted to simplify the microstructure and to determine how each precipitating phase contributed to the overall strength. In FY21, baseline mechanical properties were measured from uniaxial tensile tests on subsize SS-J2 specimens at room temperature and at elevated temperatures of 300, 450, and 600 °C to serve a comparison to the irradiated properties. Four capsules containing 3D printed Inconel 718 were inserted into HFIR in FY21 for a matrix of two temperatures and two doses. The lower of the two doses was available for characterization in FY22. Multiple heat treatments of Inconel 718 irradiated to nominal conditions of 2 displacements per atom (dpa) at either 300 or 600 °C were strained with uniaxial tensile tests at the Irradiated Material Examination and Testing (IMET) Facility to discern the mechanical properties. Transmission electron microscopy was performed to correlate the observed mechanical properties with nanoscale features. The initially homogenous AM718-HM increased in strength at both irradiation temperatures based on a high density of nanometer-scale radiation-induced cavities at lower temperature and nucleation and growth of γ" precipitates at higher temperatures. The precipitate-hardened AM718-HT2 showed very small differences in strength before and after irradiation: the contribution to strength from γ" precipitates was replaced with dislocation loops. Because the radioactivity of the nickel superalloys from neutron activation limited the scope of the analysis, a feasibility study examined the possibility of an ultra-miniature specimen geometry, colloquially SS-Tiny (SS-T), for mechanical property determination using the nonirradiated Inconel 718. This study found an overestimation of ductility from the SS-T geometry with yield strength and ultimate tensile strength slightly above the SS-J2 geometry: this could be contributed to a reduction in specimen thickness.

36 MATERIALS SCIENCE↗

Measurement of the 73 As ⁢(𝑛,𝛾) cross section at thermal neutron energies

A measurement of the thermal neutron capture cross section of 73 As (t 1/2 = 80.3 d) was performed utilizing the University of Missouri Research Reactor. Two sealed quartz tubes containing 73 As were prepared and characterized before being irradiated for ≈1 week. The resulting production of 74 As was quantified with γ-ray spectroscopy. Monitor foils of Fe, Zr, and Mo were irradiated alongside the 73 As samples to assess the thermal and resonance region neutron fluxes. In conclusion, the thermal 73 As ⁢(𝑛,𝛾) cross section was determined to be 56.1 ± 8.9 b based on the average of the two 73 As samples and represents the first neutron-induced reaction cross section measured on 73 As.

and nuclear chemistry↗

FFTF Acceptance and Startup Testing for GAIN

The Fast Flux Test Facility (FFTF) is the most recent liquid metal reactor (LMR) to be designed, constructed, and operated by the U.S. Department of Energy (DOE). The 400-MWt sodium-cooled, fast-neutron flux reactor plant was designed for irradiation testing of nuclear reactor fuels and materials for liquid metal fast breeder reactors. Following the demise of the breeder reactor program in the United States, FFTF continued to play a key role in providing a test bed for demonstrating performance of advanced fuel designs and demonstrating operation, maintenance, and safety of advanced liquid metal reactors. FFTF operations ceased in April 1992 after a determination by DOE that no combination of proposed missions was financially feasible over a ten-year period. The reactor is currently deactivated and in a long-term surveillance and maintenance (S&M) mode. This report provides information on the extensive and rigorous process that was used to conduct turnover from construction followed by acceptance and startup testing of the FFTF. This paper is in support of the Gateway for Accelerated Innovation in Nuclear (GAIN), which provides the nuclear energy community with access to the technical, regulatory, and financial support necessary to move new or advanced nuclear reactor designs toward commercialization while ensuring the continued safe, reliable, and economic operation of the existing nuclear fleet. The information obtained from the design, startup, and operation of the FFTF provides valuable insight for follow-on reactor projects, such as the Versatile Test Reactor (VTR), in the areas of plant system and component design, component fabrication, fuel design and performance, prototype testing, site construction, reactor startup and operations, and reactor deactivation and decommissioning (D&D). The focus of this report is on the process used to startup the FFTF and to ensure that operations could be conducted efficiently and safely. A reference section is provided of documents detailing the successful turnover and testing process implemented for startup of the reactor and its supporting systems. The documents listed can be retrieved upon request and are believed useful for future reactor startup endeavors.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Micro cavity fission chamber radiation detection system

A radiation detector to monitor the neutron flux of a nuclear reactor or other high-radiation environment, that can withstand the high temperatures and radiation fields of such environment, is provided. A small dielectric substrate with a low neutron-activation cross section is provided. The substrate is coated with a neutron conversion material, such as uranium oxide or thorium oxide. One or more substrates form a micro-sized detection cavity that is filled with a detection gas. A voltage is provided across anode and cathode wires in the detection cavity. A neutron absorbed in the conversion material may release reaction products into the gas, causing ionization of the gas which then produces a current or voltage signal. The small detector volume minimizes energy deposition into the detection gas by competing particles such as gamma rays, fast electrons, and beta particles, and therefore minimizes false counts while retaining large signals from neutron interactions.

McGregor, Douglas S.↗

Physics-Informed Neural Network Solution of Point Kinetics Equations for a Nuclear Reactor Digital Twin

A digital twin (DT) for nuclear reactor monitoring can be implemented using either a differential equations-based physics model or a data-driven machine learning model. The challenge of a physics-model-based DT consists of achieving sufficient model fidelity to represent a complex experimental system, whereas the challenge of a data-driven DT consists of extensive training requirements and a potential lack of predictive ability. We investigate the performance of a hybrid approach, which is based on physics-informed neural networks (PINNs) that encode fundamental physical laws into the loss function of the neural network. We develop a PINN model to solve the point kinetic equations (PKEs), which are time-dependent, stiff, nonlinear, ordinary differential equations that constitute a nuclear reactor reduced-order model under the approximation of ignoring spatial dependence of the neutron flux. The PINN model solution of PKEs is developed to monitor the start-up transient of Purdue University Reactor Number One (PUR-1) using experimental parameters for the reactivity feedback schedule and the neutron source. The results demonstrate strong agreement between the PINN solution and finite difference numerical solution of PKEs. We investigate PINNs performance in both data interpolation and extrapolation. For the test cases considered, the extrapolation errors are comparable to those of interpolation predictions. Extrapolation accuracy decreases with increasing time interval.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗