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DOE OSTI2025

X-ray absorption spectroscopy measurements of radiatively ionized argon gas

X-ray absorption spectroscopy is a diagnostic tool that can characterize the temperature and ionization state of a plasma. This technique requires experiments to characterize the platform, careful data calibration, and comparison with atomic models to understand the plasma parameters. We performed ionizing radiation wave experiments at the OMEGA Laser Facility that used an ∼ 80 eV X-ray source to heat an Argon (Ar) gas cell at fill pressures of 3 atm. To diagnose the Ar plasma, we used a capsule backlighter offset 10 mm from the gas cell, to produce X-rays that were absorbed by the ionized Ar gas. The absorption analysis was calibrated using the significant line structure in the backlighter spectrum, which served as independent energy fiducials enabling definitive measurements of a 50-eV shift in the energy of the Ar K-edge due to ionization. We compare the measured absorption spectra to two independent atomic models, PrismSPECT and SCRAM, and show that the observed K-edge shift in the heated gas is consistent with ionization up to Ar 4+ and temperatures of 10 eV.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2015

FIRST INVESTIGATION OF THE COMBINED IMPACT OF IONIZING RADIATION AND MOMENTUM WINDS FROM A MASSIVE STAR ON A SELF-GRAVITATING CORE

Massive stars shape the surrounding interstellar matter (ISM) by emitting ionizing photons and ejecting material through stellar winds. To study the impact of the momentum from the wind of a massive star on the surrounding neutral or ionized material, we implemented a new HEALPix-based momentum-conserving wind scheme in the smoothed particle hydrodynamics (SPH) code SEREN. A qualitative study of the impact of the feedback from an O7.5-like star on a self-gravitating sphere shows that on its own, the transfer of momentum from a wind onto cold surrounding gas has both a compressing and dispersing effect. It mostly affects gas at low and intermediate densities. When combined with a stellar source's ionizing ultraviolet (UV) radiation, we find the momentum-driven wind to have little direct effect on the gas. We conclude that during a massive star's main sequence, the UV ionizing radiation is the main feedback mechanism shaping and compressing the cold gas. Overall, the wind's effects on the dense gas dynamics and on the triggering of star formation are very modest. The structures formed in the ionization-only simulation and in the combined feedback simulation are remarkably similar. However, in the combined feedback case, different SPH particles end up being compressed. This indicates that the microphysics of gas mixing differ between the two feedback simulations and that the winds can contribute to the localized redistribution and reshuffling of gas.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2019

Electron-impact ionization of the Si atom

Electron-impact ionization cross sections are calculated for the ground configuration of the Si atom for application in erosion diagnostics of plasma facing components in magnetically confined fusion experiments. The single ionization cross sections include contributions from outer subshell direct ionization and excitation-autoionization. The dominant direct ionization cross sections are calculated using a non-perturbative time-dependent close-coupling method. A significant reduction in the direct ionization cross section is found when compared to perturbative distorted-wave results. The theoretical cross sections are compared with available crossed-beams measurements.

Loch, S. D.↗

DOE OSTI2025

Effects of non-equilibrium ionization and excitation on radiation absorption in plasma plumes induced by ablation of metal targets with nanosecond laser pulses

Ionization and radiation absorption in nanosecond laser-induced plasma plumes are routinely modeled using the Saha–Boltzmann equilibrium ionization model (EQM). However, the equilibrium assumption can be inaccurate during the laser pulse when non-equilibrium effects significantly impact radiation absorption. In the present work, the EQM and non-equilibrium collisional-radiative model (CRM) are compared to reveal the effect of plasma non-equilibrium on radiation absorption in non-homogeneous plumes and degree of plasma shielding. Simulations of plume expansion induced by irradiation of a copper target in 1 atm argon background gas with a 10 ns Gaussian pulse at a fluence from 8 Jcm −2 to 14 Jcm −2 are performed with a hybrid computational model that couples a lumped particle direct simulation Monte Carlo method with either CRM or EQM. The simulations show that the EQM strongly underestimates the effects of ionization and radiation absorption compared to CRM and, contrary to the CRM, predict strong ionization of the background gas. The differences between the models are explained by the qualitatively different coupling between plume expansion and dynamics of ionization and exitation processes in the CRM and EQM under conditions when the characteristic times for most radiation- and electron-induced processes are longer than the pulse duration. The CRM-based predictions are also found to agree much better with available experimental data. In conclusion, these results indicate that the model of Saha–Boltzmann equilibrium cannot be used for reliable prediction of the degree of plasma shielding in plumes induced by nanosecond laser pulses or for processing results of spectroscopic measurements at early stages of expansion of such plumes.

Physics - Plasma physics↗

DOE OSTI2020

Multiphase outflows in post-starburst E+A galaxies - II. A direct connection between the neutral and ionized outflow phases

ABSTRACT Post-starburst E+A galaxies are systems that hosted a powerful starburst that was quenched abruptly. Simulations suggest that these systems provide the missing link between major merger ULIRGs and red and dead ellipticals, where AGN feedback is responsible for the expulsion or destruction of the molecular gas. However, many details remain unresolved and little is known about AGN-driven winds in this short-lived phase. We present spatially resolved IFU spectroscopy with MUSE/VLT of SDSS J124754.95-033738.6, a post-starburst E+A galaxy with a recent starburst that started 70 Myr ago and ended 30 Myr ago, with a peak SFR of $\sim 150\, \mathrm{M_{\odot }\,yr^{ -1}}$. We detect disturbed gas throughout the entire field of view, suggesting triggering by a minor merger. We detect fast-moving multiphased gas clouds, embedded in a double-cone face-on outflow, which are traced by ionized emission lines and neutral NaID emission and absorption lines. We find remarkable similarities between the kinematics, spatial extents, and line luminosities of the ionized and neutral gas phases, and propose a model in which they are part of the same outflowing clouds, which are exposed to both stellar and AGN radiation. Our photoionization model provides consistent ionized line ratios, NaID absorption optical depths and EWs, and dust reddening. Using the model, we estimate, for the first time, the neutral-to-ionized gas mass ratio (about 20), the sodium neutral fraction, and the size of the outflowing clouds. This is one of the best ever observed direct connections between the neutral and ionized outflow phases in AGN.

Baron, Dalya↗

DOE OSTI2019

On the iron ionization balance of cool stars

Abstract High-resolution spectroscopic studies of solar-type stars have revealed higher iron abundances derived from singly ionized species compared to neutral, violating the ionization equilibrium under the assumption of local thermodynamic equilibrium. In this work, we investigate the overabundances of Fe ii lines reported in our previous work for a sample of 451 solar-type HARPS stars in the solar neighborhood. The spectroscopic surface gravities of this sample, which emerge from the ionization balance, appear underestimated for the K-type stars. In order to understand this behaviour, we search our Fe ii line list for unresolved blends and outliers. First, we use the Vienna Atomic Line Database to identify possible unresolved blends around our lines and calculate which ones are strong enough to cause overestimations in the equivalent width measurements. Second, for our sample we use reference parameters (effective temperature and metallicity) and the Gaia DR2 parallaxes to derive surface gravities (trigonometric gravities) and calculate the Fe i and Fe ii abundances from different line lists. We exclude the Fe ii lines which produce overabundances above 0.10 dex. The derived surface gravities from the clean line list are now in agreement with the trigonometric. Moreover, the difference between Fe i and Fe ii abundance does not show now a correlation with the effective temperature. Finally, we show that the ionization balance of Ti can provide better estimates of surface gravities than iron. With this analysis, we provide a solution to the ionization balance problem observed in the atmospheres of cool dwarfs.

Tsantaki, M.↗

DOE OSTI2026

Probing Excited-State Dynamics of Transmon Ionization

The fidelity and quantum nondemolition character of the dispersive readout in circuit QED are limited by unwanted transitions to highly excited states at specific photon numbers in the readout resonator. This observation can be explained by multiphoton resonances between computational states and highly excited states in strongly driven nonlinear systems, analogous to multiphoton ionization in atoms and molecules. In this work, we utilize the multilevel nature of high-𝐸 𝐽 /𝐸 𝐶 transmons to probe the excited-state dynamics induced by strong drives during readout. With up to ten resolvable states, we quantify the critical photon number of ionization, the resulting state after ionization, and the fraction of the population transferred to highly excited states. Moreover, using pulse shaping to control the photon number in the readout resonator in the high-power regime, we tune the adiabaticity of the transition and verify that transmon ionization is a Landau-Zener-type transition. We further extend these methods to a typical transmon with 𝐸 𝐽 /𝐸 𝐶 ≈ 55 and probe the offset-charge dependence of ionization dynamics in a timed-resolved manner. Our experimental results agree well with the theoretical prediction from a semiclassical driven transmon model and may guide future exploration of strongly driven nonlinear oscillators.

cavity quantum electrodynamics↗

DOE OSTI2015

Field ionization of Rydberg atoms in a single-cycle pulse

Here, we study the ionization of Rydberg atoms in a single-cycle-pulse electric field based on both classical and quantum calculations. The ionization-probability curve exhibits a “ripple” structure as a function of the pulse duration and the field amplitude. These ripple structures are found to be dependent on the angular distribution of the initial state. A large electron-emission asymmetry is observed, and the ionized electron is almost completely emitted to one side of the atom except when the pulse length is roughly one Rydberg period. In both the long-pulse and the short-pulse regimes, larger electron energy can be expected from the ionization of lower-lying Rydberg states, matching the observation in a recent experiment [S. Li and R. R. Jones, Phys. Rev. Lett. 112, 143006 (2014)]. This trend is closely related to the electron-emission asymmetry associated with the field-direction change in a single-cycle pulse. The possible implications of the different energy transfer in a single-cycle pulse from that in a multicycle pulse are also discussed briefly for the strong-field ionization of the ground atomic state.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2015

Evidence for unnatural-parity contributions to electron-impact ionization of laser-aligned atoms

Recent measurements have examined the electron-impact ionization of excited-state laser-aligned Mg atoms. In this paper we show that the ionization cross section arising from the geometry where the aligned atom is perpendicular to the scattering plane directly probes the unnatural parity contributions to the ionization amplitude. The contributions from natural parity partial waves cancel exactly in this geometry. Our calculations resolve the discrepancy between the nonzero measured cross sections in this plane and the zero cross section predicted by distorted-wave approaches. Finally, we demonstrate that this is a general feature of ionization from p-state targets by additional studies of ionization from excited Ca and Na atoms.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2015

Two-photon double ionization of atomic beryllium with ultrashort laser pulses

Here, we investigate the two-photon double ionization of beryllium atom induced by ultrashort pulses. We use a time-dependent formalism to evaluate the ionization amplitudes and generalized cross sections for the ejection of the 2s 2 valence shell electrons in the presence of a fully occupied 1s 2 frozen core shell. The relative contributions of the two-photon direct and sequential process are systematically explored by varying both pulse duration and central frequency. The energy and angular differential ionization yields reveal the signatures of both mechanisms, as well as the role of electron correlation in both the single and double ionization continua. In contrast with previous results on the helium atom, the presence of an electronic core strongly affects the final state leading to back-to-back electron emission even in the a priori less correlated two-photon sequential mechanism. In particular, a dominant pathway via excitation ionization through the Be + (2p) determines the profiles and pulse-duration dependencies of the energy and angle differential yields.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2019

Phase-dependent ionization of Rydberg atoms in static fields

Using a laser intensity modulated synchronously with a 15.9 GHz microwave field we have examined laser excitation of Li atoms to the vicinity of the ionization limit in the presence of the microwave field and a parallel static field. The static field breaks the symmetry of ionization in the two microwave half cycles, and as the intensity modulated laser beam is delayed relative to the microwave field, maxima in the ionization are observed every microwave field cycle, not every half cycle, as in the absence of the static field. Here, when the laser is tuned below the ionization limit there is an unexpected phase reversal of the modulation in the ionization, the origin of which is clarified by a classical model.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2024

Single-shot ionization-based monitor for pulsed electron beams

In this work, we present an experimental demonstration of a single-shot, nondestructive electron beam diagnostic based on the ionization of a low-density pulsed gas jet. In our study, 7 MeV electron bunches from a radio-frequency photoinjector, carrying up to 100 pC of charge, traversed a localized distribution of nitrogen gas (N 2 ). The interaction of the electron bunches with the N 2 gas generated a correlated signature in the ionized particle distribution, which was spatially magnified using a series of electrostatic lenses and recorded with a microchannel-plate detector. Various modalities, including point-to-point imaging and velocity mapping, are investigated. A temporal trace of the detector current enabled the identification of single- and double-ionization events. The characteristics of the ionization distribution, dependence on gas density, total bunch charge, and other parameters, are described. Approaches to scaling to higher electron bunch density and energy are suggested. Additionally, the instrument proves useful for comprehensive studies of the ionization process itself.

47 OTHER INSTRUMENTATION↗

DOE OSTI2019

Kinetic Simulations of Magnetic Reconnection in Partially Ionized Plasmas

Fast magnetic reconnection occurs in nearly all natural and laboratory plasmas and rapidly releases stored magnetic energy. Although commonly studied in fully ionized plasmas, if and when fast reconnection can occur in partially ionized plasmas, such as the interstellar medium or solar chromosphere, is not well understood. Here, this Letter presents the first fully kinetic particle-in-cell simulations of partially ionized reconnection and demonstrates that fast reconnection can occur in partially ionized systems. In the simulations, the transition to fast reconnection occurs when the current sheet width thins below the ion-inertial length in contrast to previous analytic predictions. The peak reconnection rate is ≥ 0.08 when normalized to the bulk Alfvén speed (including both ion and neutral mass), consistent with previous experimental results. However, when the bulk Alfvén speed falls below the neutral sound speed, the rate becomes system size dependent. The normalized inflow velocity is ionization fraction dependent, which is shown to be a result of neutral momentum transport. A model for the inflow is developed which agrees well with the simulation results.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2016

Ionizing Energy Depositions After Fast Neutron Interactions in Silicon

In our study we present the ionizing energy depositions in a 300 μm thick silicon layer after fast neutron impact. With the Time-of-Flight (ToF) technique, the ionizing energy deposition spectra of recoil silicons and secondary charged particles were assigned to (quasi-)monoenergetic neutron energies in the range from 180 keV to hundreds of MeV. We also show and interpret representative measured energy spectra. By separating the ionizing energy losses of the recoil silicon from energy depositions by products of nuclear reactions, the competition of ionizing (IEL) and non-ionizing energy losses (NIEL) of a recoil silicon within the silicon lattice was investigated. Furthermore, the data give supplementary information to the results of a previous measurement and are compared with different theoretical predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2022

Cross-polarized common-path temporal interferometry for high-sensitivity strong-field ionization measurements

Absolute density measurements of low-ionization-degree or low-density plasmas ionized by lasers are very important for understanding strong-field physics, atmospheric propagation of intense laser pulses, Lidar etc. A cross-polarized common-path temporal interferometer using balanced detection was developed for measuring plasma density with a sensitivity of ∼0.6 mrad, equivalent to a plasma density-length product of ∼2.6 × 10 13 cm −2 if using an 800 nm probe laser. By using this interferometer, we have investigated strong-field ionization yield versus intensity for various noble gases (Ar, Kr, and Xe) using 800 nm, 55 fs laser pulses with both linear (LP) and circular (CP) polarization. The experimental results were compared to the theoretical models of Ammosov-Delone-Krainov (ADK) and Perelomov-Popov-Terent’ev (PPT). We find that the measured phase change induced by plasma formation can be explained by the ADK theory in the adiabatic tunneling ionization regime, while PPT model can be applied to all different regimes. We have also measured the photoionization and fractional photodissociation of molecular (MO) hydrogen. By comparing our experimental results with PPT and MO-PPT models, we have determined the likely ionization pathways when using three different pump laser wavelengths of 800 nm, 400 nm, and 267 nm.

47 OTHER INSTRUMENTATION↗

DOE OSTI2018

A Novel Non-Parametric Density Estimation Approach to Measuring Muon Ionization Cooling and Reverse Emittance Exchange in the MICE Experiment

The Muon Ionization Cooling Experiment (MICE) located at Rutherford Ap- pleton Laboratory in the U.K. has demonstrated muon ionization beam cooling for the rst time. A beam of muons in MICE is produced from high-energy proton beam collision with a xed target, generating pions which in turn decay into muons. Pion-decay muons, thus, are tertiary particles and, as a result, occupy a large vol- ume in position{momentum phase space. To t the muon beam into smaller and more cost-eective accelerating devices, muon beam phase{space volume needs to be reduced (beam cooling). Ionization beam cooling, which before MICE has never been demonstrated experimentally for muons, is the only technique fast enough to be used for muons within their short lifetime. Ionization cooling occurs when muons traverse an absorbing material and lose momentum through ionization energy loss. The cooling eect in MICE is measured using two scintillating-ber tracking detec- tors. These trackers, one upstream and one downstream of the absorber, reconstruct and measure the position and momentum coordinates of each muon. Given the pre- cision MICE needed to demonstrate beam cooling, it is necessary to develop analysis tools that can account for any eects that may lead to inaccurate measurement of cooling, such as non{linear eects in beam optics. Non{parametric density estima- tion techniques, such as kernel density estimation (KDE), provide a basis for creating analysis tools that are robust against these eects, directly calculating the muon beam phase-space density and volume for demonstrating beam cooling. This thesis focuses on the application of KDE to the measurement of beam cooling in MICE. The KDE technique is validated using known distributions and is applied to sim- ulated and experimental MICE data corresponding to the various magnet, optics, and absorber congurations. Using the KDE technique, muon beam cooling in the four{dimensional transverse phase space, as well as reverse emittance exchange using MICE data have been demonstrated.

43 PARTICLE ACCELERATORS↗

DOE OSTI2019

The impacts of ionization chemistry on hydrocarbon detonation [Thesis]

As carbon emissions are negatively impacting ecosystems across the globe, researchers are in a race against time to provide cleaner and more efficient power. Detonation engines can help meet the increasing demands for cleaner and more efficient power generation by providing an alternative means to use oxy-fuel combustion for carbon sequestration. By pairing a detonation engine with a magnetohydrodynamic (MHD) generator, power can be directly extracted from the ionized gases behind the detonation front via the Lorentz force. This eliminates the moving components found in gas turbine engines, which are unable to withstand high temperatures encountered in oxy-fuel combustion. The electrical conductivity of the ionized gas behind the detonation front can be increased by several orders of magnitude with the addition of readily ionizing seed particles such as potassium, increasing the power generation of the engine. However, this increase has a limit as dilution studies have shown decreases in detonation speeds with increasing diluent. To better understand the interaction of seed particles with the detonation front and the electrical conductivity of the mixed gas, a detailed hydrocarbon kinetic model has been created in conjunction with a detonation solver. This model is, to my knowledge, the first detailed hydrocarbon model to be used in detonation simulations. I used this model to study the parasitic interaction arising from using potassium seed material. I found that the ionization of the seed particles negatively impacted detonation velocities up to 8% and power production up to 15%, pointing to the need for further research development into detonation kinetic models and ionization fields.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

DOE OSTI2021

Identifying Candidate Biomarkers of Ionizing Radiation in Human Pulmonary Microvascular Lumens Using Microfluidics—A Pilot Study

The microvasculature system is critical for the delivery and removal of key nutrients and waste products and is significantly damaged by ionizing radiation. Single-cell capillaries and microvasculature structures are the primary cause of circulatory dysfunction, one that results in morbidities leading to progressive tissue and organ failure and premature death. Identifying tissue-specific biomarkers that are predictive of the extent of tissue and organ damage will aid in developing medical countermeasures for treating individuals exposed to ionizing radiation. In this pilot study, we developed and tested a 17 µL human-derived microvascular microfluidic lumen for identifying candidate biomarkers of ionizing radiation exposure. Through mass-spectrometry-based proteomics, we detected 35 proteins that may be candidate early biomarkers of ionizing radiation exposure. This pilot study demonstrates the feasibility of using humanized microfluidic and organ-on-a-chip systems for biomarker discovery studies. A more elaborate study of sufficient statistical power is needed to identify candidate biomarkers and test medical countermeasures of ionizing radiation.

59 BASIC BIOLOGICAL SCIENCES↗