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At least 307 records · Page 17
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Non-local Thermodynamic Equilibrium Abundance Analyses of the Extreme Helium Stars V652 Her and HD 144941

Optical high-resolution spectra of V652 Her and HD 144941, the two extreme helium stars with exceptionally low C/He ratios, have been subjected to a non-LTE abundance analysis using the tools TLUSTY and SYNSPEC. Defining atmospheric parameters were obtained from a grid of non-LTE atmospheres and a variety of spectroscopic indicators including He i and He ii line profiles, and the ionization equilibrium of ion pairs such as C ii/C iii and N ii/N iii. The various indicators provide a consistent set of atmospheric parameters: T {sub eff} = 25,000 ± 300 K, log g = 3.10 ± 0.12(cgs), and ξ = 13 ± 2 km s{sup −1} are provided for V652 Her, and T {sub eff} = 22,000 ± 600 K, log g = 3.45 ± 0.15 (cgs), and ξ = 10 km s{sup −1} are provided for HD 144941. In contrast to the non-LTE analyses, the LTE analyses—LTE atmospheres and an LTE line analysis—with the available indicators do not provide a consistent set of atmospheric parameters. The principal non-LTE effect on the elemental abundances is on the neon abundance. It is generally considered that these extreme helium stars with their very low C/He ratio result from the merger of two helium white dwarfs. Indeed, the derived composition of V652 Her is in excellent agreement with predictions by Zhang and Jeffery, who model the slow merger of helium white dwarfs; a slow merger results in the merged star having the composition of the accreted white dwarf. In the case of HD 144941, which appears to have evolved from metal-poor stars, a slow merger is incompatible with the observed composition but variations of the merger rate may account for the observed composition. More detailed theoretical studies of the merger of a pair of helium white dwarfs are to be encouraged.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

ROLE OF THE CORONAL ALFVÉN SPEED IN MODULATING THE SOLAR-WIND HELIUM ABUNDANCE

The helium abundance He/H in the solar wind is relatively constant at ∼0.04 in high-speed streams, but varies in phase with the sunspot number in slow wind, from ∼0.01 at solar minimum to ∼0.04 at maximum. Suggested mechanisms for helium fractionation have included frictional coupling to protons and resonant interactions with high-frequency Alfvénic fluctuations. We compare He/H measurements during 1995–2015 with coronal parameters derived from source-surface extrapolations of photospheric field maps. We find that the near-Earth helium abundance is an increasing function of the magnetic field strength and Alfvén speed v {sub A} in the outer corona, while being only weakly correlated with the proton flux density. Throughout the solar cycle, fast wind is associated with short-term increases in v {sub A} near the source surface; resonance with Alfvén waves, with v {sub A} and the relative speed of α -particles and protons decreasing with increasing heliocentric distance, may then lead to enhanced He/H at 1 au. The modulation of helium in slow wind reflects the tendency for the associated coronal Alfvén speeds to rise steeply from sunspot minimum, when this wind is concentrated around the source-surface neutral line, to sunspot maximum, when the source-surface field attains its peak strengths. The helium abundance near the source surface may represent a balance between collisional decoupling from protons and Alfvén wave acceleration.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Room temperature thermal conductivity measurements of neat MOF-5 compacts with high pressure hydrogen and helium

Metal-organic frameworks (MOFs) are a highly porous crystalline material with potential in various applications including on-board vehicle hydrogen storage for fuel cell vehicles. The thermal conductivity of MOFs is an important parameter in the design and ultimate performance of an on-board hydrogen storage system. However, in-situ thermal conductivity measurements have not been previously reported. The present study reports room temperature thermal conductivity and thermal diffusivity measurements performed on neat MOF-5 cylindrical compacts (ρ = 0.4 g/mL) as a function of pressure (0.27–90 bar) and gas type (hydrogen and helium). The transient plane source technique was used to measure both the non-directional thermal properties (isotropic method) and the directional thermal properties (anisotropic method). High pressure measurements were made using our in-house built low-temperature, high pressure thermal conductivity sample cell. The intrinsic thermal properties of neat MOF-5 measured under vacuum were—Isotropic: k isotropic = 0.1319 W/m K, α isotropic = 0.4165 mm 2 /s; Anisotropic: k axial = 0.1477 W/m K, k radial = 0.1218 W/m K, α axial = 0.5096 mm 2 /s, and α radial = 0.4232 mm 2 /s. The apparent thermal properties of neat MOF-5 increased with increasing hydrogen and helium pressure, with the largest increase occurring in the narrow pressure range of 0–10 bar and then monotonically asymptoting with increasing pressures up to around 90 bar. On average, a greater than two-fold enhancement in the apparent thermal properties was observed with neat MOF-5 in the presence of helium and hydrogen compared to the intrinsic values of neat MOF-5 measured under vacuum. The apparent thermal properties of neat MOF-5 measured with hydrogen were higher than those measured with helium, which were directly related to the gas-specific thermal properties of helium and hydrogen. Neat MOF-5 exhibited a small degree of anisotropy under all conditions measured with thermal conductivities and diffusivities in the axial direction being higher than those in the radial direction. As a result, the low temperature specific heat capacities of neat MOF-5 were also measured and reported for the temperature range of 93–313 K (–180–40 °C).

36 MATERIALS SCIENCE↗
DOE OSTI2021

Effects of helium on irradiation response of reduced-activation ferritic-martensitic steels: Using nickel isotopes to simulate fusion neutron response

Understanding the effects of helium on microstructures and mechanical properties of reduced-activation ferritic-martensitic steels is important to use of these steels in fusion reactor structures. The 9Cr-2WVTa steels were doped with 58Ni and 60Ni isotopes at 2 weight percent to control the rate of transmutation helium generation. The samples were irradiated in the High Flux Isotope Reactor to ~24 displacements per atom at nominal temperatures of 300, 400, and 500°C, producing 228 and 7 atomic parts-per-million helium in the 58 Ni- and 60 Ni-doped samples, respectively. Transmission electron microscopy revealed a variety of precipitates and the radiation-induced dislocation loops and cavities (voids or helium bubbles). Tensile tests of the irradiated samples at the irradiation temperatures showed radiation-induced hardening at 300°C and radiation-induced softening at 400°C. Analysis indicates that the hardening primarily originated from the loops and cavities. The 58 Ni-doped samples had greater strengthening contributions from loops and cavities, leading to higher hardening with lower ductility than the 60 Ni-doped samples. The greater helium production of 58 Ni did not show pronounced reductions in ductility of the samples.

36 MATERIALS SCIENCE↗
DOE OSTI2014

Effects of helium implantation on the tensile properties and microstructure of Ni₇₃P₂₇ metallic glass nanostructures

We report fabrication and nanomechanical tension experiments on as-fabricated and helium-implanted ~130 nm diameter Ni₇₃P₂₇ metallic glass nano-cylinders. The nano-cylinders were fabricated by a templated electroplating process and implanted with He⁺ at energies of 50, 100, 150, and 200 keV to create a uniform helium concentration of ~3 at. % throughout the nano-cylinders. Transmission electron microscopy (TEM) imaging and through-focus analysis reveal that the specimens contained ~2 nm helium bubbles distributed uniformly throughout the nano-cylinder volume. In-situ tensile experiments indicate that helium-implanted specimens exhibit enhanced ductility as evidenced by a 2-fold increase in plastic strain over as-fabricated specimens, with no sacrifice in yield and ultimate tensile strengths. This improvement in mechanical properties suggests that metallic glasses may actually exhibit a favorable response to high levels of helium implantation.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Coupling a single electron on superfluid helium to a superconducting resonator

Abstract Electrons on helium form a unique two-dimensional system on the interface of liquid helium and vacuum. A small number of trapped electrons on helium exhibits strong interactions in the absence of disorder, and can be used as a qubit. Trapped electrons typically have orbital frequencies in the microwave regime and can therefore be integrated with circuit quantum electrodynamics (cQED), which studies light–matter interactions using microwave photons. Here, we experimentally realize a cQED platform with the orbitals of single electrons on helium. We deterministically trap one to four electrons in a dot integrated with a microwave resonator, allowing us to study the electrons’ response to microwaves. Furthermore, we find a single-electron-photon coupling strength of $$g/2\pi =4.8\pm 0.3$$ g ∕ 2 π = 4.8 ± 0.3 MHz, greatly exceeding the resonator linewidth $$\kappa /2\pi =0.5$$ κ ∕ 2 π = 0.5 MHz. These results pave the way towards microwave studies of Wigner molecules and coherent control of the orbital and spin state of a single electron on helium.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Simulating the absorption spectra of helium clusters (N = 70, 150, 231, 300) using a charge transfer correction to superposition of fragment single excitations

Simulations of the n = 2 absorption spectra of HeN(N = 70, 150, 231, 300) clusters are reported, with nuclear configurations sampled by path integral molecular dynamics. The electronic structure is treated by a new approach, ALMO-CIS+CT, which is a formulation of configuration interaction singles (CIS) based on absolutely localized molecular orbitals (ALMOs). The method generalizes the previously reported ALMO-CIS model [K. D. Closser et al. J. Chem. Theory Comput. 11, 5791 (2015)] to include spatially localized charge transfer (CT) effects. It is designed to recover large numbers of excited states in atomic and molecular clusters, such as the entire n = 2 Rydberg band in helium clusters. ALMO-CIS+CT is shown to recover most of the error caused by neglecting charge transfer in ALMO-CIS and has comparable accuracy to standard CIS for helium clusters. For the n = 2 band, CT stabilizes states towards the blue edge by up to 0.5 eV. ALMO-CIS+CT retains the formal cubic scaling of ALMO-CIS with respect to system size. With improvements to the implementation over that originally reported for ALMO-CIS, ALMO-CIS+CT is able to treat helium clusters with hundreds of atoms using modest computing resources. Here, a detailed simulation of the absorption spectra associated with the 2s and 2p bands of helium clusters up to 300 atoms is reported, using path integral molecular dynamics with a spherical boundary condition to generate atomic configurations at 3 K. The main features of experimentally reported fluorescence excitation spectra for helium clusters are reproduced.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Improving helium abundance determinations with Leo P as a case study

Currently, the primordial helium abundance is best estimated through spectroscopic observations of H II regions in metal-poor galaxies. However these determinations are limited by several systematic uncertainties which ultimately limit our ability to accurately ascertain the primordial abundance. In this study, we improve the methodologies for solving for the reddening, the emission contributions from collisional excitation of the H I atoms, the effects underlying absorption in the H I and He I emission lines, and the treatment of the blended H I and He I emission at λ3889 with the aim of lowering the systematic uncertainties in helium abundance determinations. To apply these methods, we have obtained observations of the He I λ10830 emission line in the brightest H II region in the extremely metal-poor (3% Z ⊙ ) galaxy Leo P with the LUCI1 instrument on the LBT. We combine this measurement with previous MODS/LBT observations to derive an improved helium abundance. In doing so, our present analysis results in a decrease in the uncertainty in the helium abundance of Leo P by approximately 70%. Furthermore, this result is combined with data from other observations to estimate the primordial helium mass fraction, Yp= 0.2453 ± 0.0034.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Electron drift and longitudinal diffusion in high pressure xenon-helium gas mixtures

We report new measurements of the drift velocity and longitudinal diffusion coefficients of electrons in pure xenon gas and in xenon-helium gas mixtures at 1-9 bar and electric field strengths of 50-300 V/cm. In pure xenon we find excellent agreement with world data at all E/P, for both drift velocity and diffusion coefficients. However, a larger value of the longitudinal diffusion coefficient than theoretical predictions is found at low E/P in pure xenon, below the range of reduced fields usually probed by TPC experiments. A similar effect is observed in xenon-helium gas mixtures at somewhat larger E/P. Drift velocities in xenon-helium mixtures are found to be theoretically well predicted. Although longitudinal diffusion in xenon-helium mixtures is found to be larger than anticipated, extrapolation based on the measured longitudinal diffusion coefficients suggest that the use of helium additives to reduce transverse diffusion in xenon gas remains a promising prospect.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Modeling Helium Segregation to the Surfaces of Plasma-Exposed Tungsten as a Function of Temperature and Surface Orientation

We provide a description of the dependence on surface crystallographic orientation and temperature of the segregation of helium implanted with energies consistent with low-energy plasma exposure to tungsten surfaces. Here, we describe multiscale modeling results based on a hierarchical approach to scale bridging that incorporates atomistic studies based on a reliable interatomic potential to parameterize a spatially dependent drift-diffusion-reaction cluster-dynamics code. An extensive set of molecular dynamics (MD) simulations has been performed at 933 K and/or 1200 K to determine the probabilities of desorption and modified trap mutation that occurs as small, mobile Hen (1 ≤ n ≤ 7) clusters diffuse from the near-surface region toward surfaces of varying crystallographic orientation due to an elastic interaction force that provides the thermodynamic driving force for surface segregation. These near-surface cluster dynamics have significant effects on the surface morphology, the near-surface defect structures, and the amount of helium retained in the material upon plasma exposure, for which we have developed an extensive MD database of cumulative evolution during high-flux helium implantation at 933 K, which we compare to our properly parameterized cluster-dynamics model. This validated model is then used to evaluate the effects of temperature on helium retention and subsurface helium clustering.

Blondel, Sophie↗
DOE OSTI2018

Uncertainty quantification for incident helium flux in plasma-exposed tungsten

In this work, the surface response of a tungsten plasma-facing component was simulated by a cluster-dynamics code, Xolotl, with a focus on quantifying the impact of uncertainty in one of the input parameters to Xolotl, namely, the incident helium flux. The simulated conditions involve a tungsten surface exposed to 100 eV helium ion implantations with a flux of either 4 × 10 22 or 4 × 10 25 He m -2 s -1 . Furthermore, two sources were used to describe the implanted helium depth distribution in tungsten, either molecular dynamics (MD) or a binary collision approximation code, the stopping and range of ions in matter (SRIM). The aim of this work is to evaluate and examine uncertain predictions on the helium retention based on these two different modeling methodologies that either neglect electronic energy loss or the crystalline structure of the solid, respectively. An embedded model-form error approach was pursued here in order to arrive at predictions that account for variability due to the two different data sources, and the impact of this model-form uncertainty in incident helium flux on Xolotl output was presented for the two implantation fluxes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2018

Resistively Heated Target Tests Using Helium Flow Loop

A helium flow and heat transfer experiment has been conducted using the helium flow loop facility at the Los Alamos National Laboratory. In order to replicate the helium cooled Mo-100 plant design disks during beam heating, an array of resistive heaters were placed within the helium flow loop, and cooled via helium. The resistively heated test piece is comprised of seven ceramic electric heaters with embedded thermocouples allowing temperature measurements of each heater.Computation fluid dynamic (CFD) simulations and analysis from theory are compared to the experiment results in order to have predictable capabilities for future experiments.

42 ENGINEERING↗
DOE OSTI2023

Testing of Helium Cooled Metal Molybdenum Disk Target System

NorthStar Medical Radioisotopes LLC is planning to produce the important medical radioisotope molybdenum-99 (Mo-99) through a photonuclear reaction on molybdenum-100 (Mo-100). In this approach, multiple thin disks of enriched molybdenum metal will be bombarded with a 40-MeV electron beam. Because enriched Mo-100 is expensive, we intend to use as much beam power as possible to achieve maximum production yield and minimize the size of the target. This requirement leads to very high beam power density (heat deposition in the target), which sets challenging requirements for cooling. Together with scientists at Los Alamos National Laboratory, a team at Argonne National Laboratory has developed and demonstrated a cooling approach using pressurized helium, which allows for efficient heat removal. One of the challenges in this approach is the management of the heat load on the target window. The target window separates the high-pressure helium atmosphere inside the target from the vacuum in the beamline, so it is constantly under stress from differential pressure. Also, the window is cooled only by the helium gas flow from one side, making the window design challenging. High heat deposition in the target disks also imposes a strict requirement on performance of the helium cooling system and thickness of the target disks. The target disks are produced from metal powder via a press-and-sinter process. The resulting disks do not possess as high a tensile strength as solid molybdenum and might not survive the vibration from the high-velocity helium coolant and the high thermal stress from beam heating.

42 ENGINEERING↗
DOE OSTI2024

Testing of Helium-Cooled Metal Molybdenum Disk Target

NorthStar Medical Radioisotopes LLC is planning to produce an important medical radioisotope, molybdenum-99 (Mo-99), through photonuclear reaction on molybdenum-100 (Mo-100). In this approach, molybdenum metal will be bombarded with a 40-MeV electron beam. Because enriched Mo-100 is expensive, it is desired to use as much beam power as possible to achieve maximum production yield and minimize target mass. This objective leads to very high beam power density (heat deposition in the target), which sets challenging requirements for cooling. Together with scientists at Los Alamos National Laboratory, a team at Argonne National Laboratory has developed and demonstrated a cooling approach using pressurized helium, which allows for efficient heat removal. One of the main challenges in this approach is the management of the heat load on the target window. The target window separates the high-pressure helium inside the target from the vacuum in the beamline, so it is constantly under stress from differential pressure. Also, the window is cooled only by the helium gas flowing on one side, making the window cooling even more challenging. High heat deposition in the target disks also imposes a strict requirement on performance of the helium cooling system and thickness of the target disks. The target disks are produced from metal powder via a press-and-sinter process. The resulting disks do not possess tensile strength as high as solid molybdenum and might not survive the vibration from the high-velocity helium coolant and high thermal stress from beam heating. An Argonne team of scientists performed a series of tests at Argonne’s Low Energy Accelerator Facility (LEAF) [3-7]. This report describes two series of tests for scale down production target designs that utilize full-scale 29 millimeters diameter, 0.75 mm thick press-and-sintered disks. We performed two thermal tests with different beam parameters and configurations of the disk laminations. We compared the results of the window temperature measurements and cooling system parameters obtained in the experiments with those predicted by analytical calculations and Computation Flow Dynamic (CFD) simulations. Results of the experiments and calculations are presented below.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Where do $AMS-02$ anti-helium events come from?

We discuss the origin of the anti-helium-3 and -4 events possibly detected by AMS-02. Using up-to-date semi-analytical tools, we show that spallation from primary hydrogen and helium nuclei onto the ISM predicts a anti-helium-3 flux typically one to two orders of magnitude below the sensitivity of AMS-02 after 5 years, and a anti-helium-4 flux roughly 5 orders of magnitude below the AMS-02 sensitivity. We argue that dark matter annihilations face similar difficulties in explaining this event. We then entertain the possibility that these events originate from anti-matter-dominated regions in the form of anti-clouds or anti-stars. In the case of anti-clouds, we show how the isotopic ratio of anti-helium nuclei might suggest that BBN has happened in an inhomogeneous manner, resulting in anti-regions with a anti-baryon-to-photon ratio of one in a thousand of the baryon-to-photon ratio. We discuss properties of these regions, as well as relevant constraints on the presence of anti-clouds in our Galaxy. We present constraints from the survival of anti-clouds in the Milky-Way and in the early Universe, as well as from gamma-ray observations. In particular, these require the anti-clouds to be almost free of normal matter. We also discuss an alternative where anti-domains are dominated by surviving anti-stars. We suggest that part of the unindentified sources in the 3FGL catalog can originate from anti-clouds or anti-stars. AMS-02 and GAPS data could further probe this scenario.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

New helium recapture and reliquefier system for Dynamic Nuclear Polarization at UNH.

A new helium recapture and reliquefaction system, consisting of a gas bag, recapture manifold, cooling chiller, cryogenic purifier and, a gas storage cylinder banks, has been installed in the dynamic nuclear polarized target lab at the University of New Hampshire. This new system has the capability to improve the efficiency of our capacity to do target polarization runs by recycling our cryogenic helium which would otherwise be lost during polarization operations. Our helium liquefier is rated upto 40 L/Day under normal full-capacity operations, and is rated for a capacity of 500 liquid liters of helium. I explain the initial installation process followed by a discussion of the challenges with installation, including issues of impurities which appeared during the initial operation of the system. Then I discuss how we overcame these difficulties. Finally, I discuss the function of the system during normal operation and the present situation of the helium recapture and reliquefaction processing in the UNH Lab.

Lama, Chhetra [Univ. of New Hampshire, Durham, NH ↗
NASA NTRS1972

Solar flares and solar wind helium enrichments - July 1965-July 1967.

It has previously been suggested that the very high relative abundances of helium occasionally observed in the solar wind mark the plasma accelerated by major solar flares. To confirm this hypothesis, we have studied the 43 spectra with He/H greater than 15% that were observed among 10,300 spectra collected by Vela 3 between July 1965-July 1967. Six new flare-enhancement events are discussed in this paper. It is concluded that the association of helium enhancements with major flares is real, nonrandom, and very strong. With this study, there are 12 cases of reliable associations between helium enhancements and flares reported in the literature. The general characteristics of these events are discussed. It is found that the flares are typically large and bright (2B or 3B), often they produce cosmic ray protons, and they are widely distributed in solar longitude. A qualitative discussion of some of the possibilities for the source of helium enhanced plasma is presented. It is suggested that the helium enriched plasma may be the piston producing the shock causing the Type II radio emission.

Hirshberg, J.↗
NASA NTRS1973

Helium abundance of the sun.

Critical review of the four methods that have been used to estimate the ratio of helium to hydrogen in the sun - the solar neutrino flux, spectral intensity of helium lines in prominences and the chromosphere, elemental abundance of solar cosmic rays, and variations of solar wind He/H. At present the measured value for the neutrino flux cannot be explained by any of the theoretical models of the sun, and thus the neutrino measurements cannot yield an estimate of He/H. Helium line intensity measurements give the most accurate values for He/H now available - i.e., 5 to 8% helium by number. However, these results refer to the chromosphere and prominences only, and questions of spatial and temporal variations of the observed quantities and of the inferred helium abundances have not yet been dealt with adequately.

Hirshberg, J.↗