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At least 289 records · Page 16

Constraining the properties of gaseous halos via cross-correlations of upcoming galaxy surveys and thermal Sunyaev-Zel’dovich maps

The thermal Sunyaev-Zel’dovich (tSZ) effect induces a Compton-$\mathit{y}$ distortion in cosmic microwave background (CMB) temperature maps that is sensitive to a line-of-sight integral of the ionized gas pressure. By correlating the positions of galaxies with maps of the Compton-$\mathit{y}$ distortion, one can probe baryonic feedback processes and study the thermodynamic properties of a significant fraction of the gas in the Universe. Using a model fitting approach, we forecast how well future galaxy and CMB surveys will be able to measure these correlations, and show that powerful constraints on halo pressure profiles can be obtained. In this work, our forecasts are focused on correlations between galaxies and halos identified by the upcoming Dark Energy Spectroscopic Instrument survey and tSZ maps from the Simons Observatory and CMB-S4 experiments, but have general applicability to other surveys, such as the Large Synoptic Survey Telescope. We include prescriptions for observational systematics, such as halo miscentering and halo mass bias, demonstrating several important degeneracies with pressure profile parameters. Assuming modest priors on these systematics, we find that measurements of halo-$\mathit{y}$ and galaxy-$\mathit{y}$ correlations with future surveys yield tight constraints on the pressure profiles of group-scale dark matter halos, and enable current feedback models to either be confirmed or ruled out.

79 ASTRONOMY AND ASTROPHYSICS↗

Anthropogenic influences on the African easterly jet–African easterly wave system

The African easterly jet (AEJ) and African easterly waves (AEWs) can have both local and far-reaching impacts on weather. It is therefore crucial to understand how the AEJ and AEWs will respond to future climate change. In this study, we examine anthropogenic influences on the AEJ–AEW system using the Weather Research and Forecasting (WRF) model configured as a tropical channel model (TCM). Hindcast simulations for the years 2001–2010 were performed using the WRF TCM, and ten additional years of simulations were performed using the pseudo-global warming method with the initial and boundary conditions of the model modified as if it were the late twenty-first century. A comparison of the simulations from the two climate scenarios indicates robust changes to both the AEJ and AEWs. For the AEJ, the jet is weaker and shifted northwards and upwards in the future climate, in association with an increase in precipitation over the Sahel and a strengthening of the meridional temperature gradient. For the AEWs, there is an increase in the number and strength of the waves in the future climate, in association with an increase in the baroclinic and barotropic energy conversions. Here, the barotropic energy conversion in particular has a larger contribution in the future climate, which manifests in the southern AEW track experiencing greater future strengthening than the northern track.

54 ENVIRONMENTAL SCIENCES↗

WRF-Comfort: simulating microscale variability in outdoor heat stress at the city scale with a mesoscale model

Abstract. Urban overheating and its ongoing exacerbation due to global warming and urban development lead to increased exposure to urban heat and increased thermal discomfort and heat stress. To quantify thermal stress, specific indices have been proposed that depend on air temperature, mean radiant temperature (MRT), wind speed, and relative humidity. While temperature and humidity vary on scales of hundreds of meters, MRT and wind speed are strongly affected by individual buildings and trees and vary on the meter scale. Therefore, most numerical thermal comfort studies apply microscale models to limited spatial domains (commonly representing urban neighborhoods with building blocks) with resolutions on the order of 1 m and a few hours of simulation. This prevents the analysis of the impact of city-scale adaptation and/or mitigation strategies on thermal stress and comfort. To solve this problem, we develop a methodology to estimate thermal stress indicators and their subgrid variability in mesoscale models – here applied to the multilayer urban canopy parameterization BEP-BEM within the Weather Research and Forecasting (WRF) model. The new scheme (consisting of three main steps) can readily assess intra-neighborhood-scale heat stress distributions across whole cities and for timescales of minutes to years. The first key component of the approach is the estimation of MRT in several locations within streets for different street orientations. Second, mean wind speed and its subgrid variability are downscaled as a function of the local urban morphology based on relations derived from a set of microscale LES and RANS simulations across a wide range of realistic and idealized urban morphologies. Lastly, we compute the distributions of two thermal stress indices for each grid square, combining all the subgrid values of MRT, wind speed, air temperature, and absolute humidity. From these distributions, we quantify the high and low tails of the heat stress distribution in each grid square across the city, representing the thermal diversity experienced in street canyons. In this contribution, we present the core methodology as well as simulation results for Madrid (Spain), which illustrate strong differences between heat stress indices and common heat metrics like air or surface temperature both across the city and over the diurnal cycle.

Geology↗

Impact of Meteorological Factors on the Mesoscale Morphology of Cloud Streets during a Cold-Air Outbreak over the Western North Atlantic

We report postfrontal clouds (PFC) are ubiquitous in the marine boundary layer, and their morphology is essential to estimating the radiation budget in weather and climate models. Here we examine the roles of sea surface temperature (SST) and meteorological factors in controlling the mesoscale morphology and evolution of shallow clouds associated with a cold-air outbreak that occurred on 1 March 2020 during phase I of the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE). Our results show that the simulated PFC structure and ambient conditions by the Weather Research and Forecasting (WRF) Model are generally consistent with observations from GOES-16 and dropsonde measurements. We also examine the thermodynamical and dynamical influences in the cloud mesoscale morphology using WRF sensitivity experiments driven by two meteorological forcing datasets with different domain-mean SST and spatial gradients, which lead to dissimilar values of hydrometeor water path and cloud core fraction. The SST from ERA5 leads to weaker stability and higher inversion height than the SST from FNL does. In addition, the use of large-scale meteorological forcings from ERA5 yields a distinctive time evolution of wind direction shear in the inner domain, which favors the formation and persistence of longer cloud rolls. Both factors contribute to a change in the time evolution of domain-mean water path and cloud core fraction of cloud streets. Our study takes advantage of the simulation driven by the differences between two large-scale forcing datasets to illustrate the importance of SST and wind direction shear in the cloud street morphology in a realistic scenario.

54 ENVIRONMENTAL SCIENCES↗

Evaluating downscaled products with expected hydroclimatic co-variances

Abstract. There has been widespread adoption of downscaled products amongst practitioners and stakeholders to ascertain risk from climate hazards at the local scale (e.g., ∼ 5 km resolution). Such products must nevertheless be consistent with physical laws to be credible and of value to users. Here we evaluate statistically and dynamically downscaled products by examining local co-evolution of downscaled temperature and precipitation during convective and frontal precipitation events (two mechanisms testable with just temperature and precipitation). We find that two widely used statistical downscaling techniques (Localized Constructed Analogs version 2, LOCA2, and Seasonal Trends and Analysis of Residuals Empirical Statistical Downscaling Model, STAR-ESDM) generally preserve expected co-variances during convective precipitation events over the historical and future projected intervals as compared to European Centre for Medium-Range Weather Forecasts Reanalysis v5 (ERA5) and two observation-based data products (Livneh and nClimGrid-Daily). However, both techniques dampen future intensification of frontal precipitation that is otherwise robustly captured in global climate models (i.e., prior to downscaling) and with process-based dynamical downscaling across five different regional climate models. In the case of LOCA2, this leads to appreciable underestimation of future frontal precipitation event intensity. This study is one of the first to quantify a likely ramification of the stationarity assumption underlying statistical downscaling methods and identify a phenomenon where projections of future change diverge depending on data production method employed. Finally, our work proposes expected co-variances during convective and frontal precipitation as useful evaluation diagnostics that can be universally applied to a wide range of statistically downscaled products.

54 ENVIRONMENTAL SCIENCES↗

Severe Convective Storms in Limited Instability Organized by Pattern and Distribution

Abstract Severe convection occurring in high-shear, low-CAPE (HSLC) environments is a common cool-season threat in the southeastern United States. Previous studies of HSLC convection document the increased operational challenges that these environments present compared to their high-CAPE counterparts, corresponding to higher false-alarm ratios and lower probability of detection for severe watches and warnings. These environments can exhibit rapid destabilization in the hours prior to convection, sometimes associated with the release of potential instability. Here, we use self-organizing maps (SOMs) to objectively identify environmental patterns accompanying HSLC cool-season severe events and associate them with variations in severe weather frequency and distribution. Large-scale patterns exhibit modest variation within the HSLC subclass, featuring strong surface cyclones accompanied by vigorous upper-tropospheric troughs and northward-extending regions of instability, consistent with prior studies. In most patterns, severe weather occurs immediately ahead of a cold front. Other convective ingredients, such as lower-tropospheric vertical wind shear, near-surface equivalent potential temperature (θ e ) advection, and the release of potential instability, varied more significantly across patterns. No single variable used to train SOMs consistently demonstrated differences in the distribution of severe weather occurrence across patterns. Comparison of SOMs based on upper and lower quartiles of severe occurrence demonstrated that the release of potential instability was most consistently associated with higher-impact events in comparison to other convective ingredients. Overall, we find that previously developed HSLC composite parameters reasonably identify high-impact HSLC events. Significance Statement Even when atmospheric instability is not optimal for severe convective storms, in some situations they can still occur, presenting increased challenges to forecasters. These marginal environments may occur at night or during the cool season, when people are less attuned to severe weather threats. Here, we use a sorting algorithm to classify different weather patterns accompanying such storms, and we distinguish which specific patterns and weather system features are most strongly associated with severe storms. Our goals are to increase situational awareness for forecasters and to improve understanding of the processes leading to severe convection in marginal environments.

Meteorology & Atmospheric Sciences↗

Development of Short-Term Forecasting Models Using Plant Asset Data and Feature Selection

Nuclear power plants collect and store large volumes of heterogeneous data from various components and systems. With recent advances in machine learning (ML) techniques, these data can be leveraged to develop diagnostic and short-term forecasting models to better predict future equipment condition. Maintenance operations can then be planned in advance whenever degraded performance is predicted, thus resulting in fewer unplanned outages and the optimization of maintenance activities. This enables lower maintenance costs and improves the overall economics of nuclear power. This paper focuses on developing a short-term forecasting process that leverages a feature selection process to distill large volumes of heterogeneous data and predict specific equipment parameters. A variety of feature selection methods, including Shapley Additive Explanations (SHAP) and variance inflation factor (VIF), were used to select the optimal features as inputs for three ML methods: long short-term memory (LSTM) networks, support vector regression (SVR), and random forest (RF). Each combination of model and input features was used to predict a pump bearing temperature both 1 and 24 hours in advance, based on actual plant system data. The optimal inputs for the LSTM and SVR were selected using the SHAP values, while the optimal input for the RF consisted solely of the response variable itself. Each model produced similar 1-hour-ahead predictions, with root mean square errors (RMSEs) of roughly 0.006. For the 24-hour-ahead predictions, differences could be seen between LSTM, SVR, and RF, as reflected by model performances of 0.036 +- 0.014, 0.0026 +- 0, and 0.063 +- 0.004 RMSE, respectively. As big data and continuous online monitoring become more widely available, the proposed feature selection process can be used for many applications beyond the prediction of process parameters within nuclear infrastructure.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A 30-yr high-resolution weather research and forecasting model downscaling data over California and Nevada

This dataset presents a 30-year high resolution meteorological dataset obtained using the WRF model (Advanced version Research WRF version 4.4). We used WRF and European Centre for Medium-Range Weather Forecasts Reanalysis v5 as initial and boundary conditions to generate gridded meteorological variables. A large number of surface weather stations was used for model validation. A multi-physics analysis was first developed to identify a good physics suite extended from 6 November 00 UTC to 10 November 23 UTC, 2018, which included the Camp Fire in northern California. Based on the best physics suite, the downscaling dataset extends from 1 December to 28 February, 1990–2021 and the horizontal domain has 1.5 km grid spacing covering the entire states of California and Nevada in the United States. Comparisons between hourly surface observations and WRF simulations of air temperature, relative humidity and wind speeds show mean absolute errors on the order of (1.6-2.0 C), (10 %) and 1.2–1.5 m s -1 , respectively.

54 ENVIRONMENTAL SCIENCES↗

Measurements and Model Improvement: Insight into NWP Model Error Using Doppler Lidar and Other WFIP2 Measurement Systems

Abstract Doppler-lidar wind-profile measurements at three sites were used to evaluate NWP model errors from two versions of NOAA’s 3-km-grid HRRR model, to see whether updates in the latest version 4 reduced errors when compared against the original version 1. Nested (750-m grid) versions of each were also tested to see how grid spacing affected forecast skill. The measurements were part of the field phase of the Second Wind Forecasting Improvement Project (WFIP2), an 18-month deployment into central Oregon–Washington, a major wind-energy-producing region. This study focuses on errors in simulating marine intrusions, a summertime, 600–800-m-deep, regional sea-breeze flow found to generate large errors. HRRR errors proved to be complex and site dependent. The most prominent error resulted from a premature drop in modeled marine-intrusion wind speeds after local midnight, when lidar-measured winds of greater than 8 m s −1 persisted through the next morning. These large negative errors were offset at low levels by positive errors due to excessive mixing, complicating the interpretation of model “improvement,” such that the updates to the full-scale versions produced mixed results, sometimes enhancing but sometimes degrading model skill. Nesting consistently improved model performance, with version 1’s nest producing the smallest errors overall. HRRR’s ability to represent the stages of sea-breeze forcing was evaluated using radiation budget, surface-energy balance, and near-surface temperature measurements available during WFIP2. The significant site-to-site differences in model error and the complex nature of these errors mean that field-measurement campaigns having dense arrays of profiling sensors are necessary to properly diagnose and characterize model errors, as part of a systematic approach to NWP model improvement. Significance Statement Dramatic increases in NWP model skill will be required over the coming decades. This paper describes the role of major deployments of accurate profiling sensors in achieving that goal and presents an example from the Second Wind Forecast Improvement Program (WFIP2). Wind-profile data from scanning Doppler lidars were used to evaluate two versions of HRRR, the original and an updated version, and nested versions of each. This study focuses on the ability of updated HRRR versions to improve upon predicting a regional sea-breeze flow, which was found to generate large errors by the original HRRR. Updates to the full-scale HRRR versions produced mixed results, but the finer-mesh versions consistently reduced model errors.

Meteorology & Atmospheric Sciences↗

Geostationary Satellite Retrievals with Irradiances and Cloud Properties / Processed Data

The Geostationary Operational Environmental Satellite (GOES) records sky brightness temperatures and irradiances at several wavelengths. From these the cloud microphysical and optical properties can be routinely retrieved. These properties are derived using the technique proposed by Minnis et al. 2020, and is similar to the technique used for deriving cloud properties from Moderate Resolution Imaging Spectroradiometer (MODIS) data. The derived GOES properties for the duration of the second Wind Forecasting Improvement Project (WFIP2) within the domain are reported here. Nominally the retrieved dataset has a 30- minute temporal and a 9 km spatial resolution.

17 WIND ENERGY↗

The Tropical Basin Interaction Model Intercomparison Project (TBIMIP)

Abstract. Large-scale interaction between the three tropical ocean basins is an area of intense research that is often conducted through experimentation with numerical models. A common problem is that modeling groups use different experimental setups, which makes it difficult to compare results and delineate the role of model biases from differences in experimental setups. To address this issue, an experimental protocol for examining interaction between the tropical basins is introduced. The Tropical Basin Interaction Model Intercomparison Project (TBIMIP) consists of experiments in which sea surface temperatures (SSTs) are prescribed to follow observed values in selected basins. There are two types of experiments. One type, called standard pacemaker, consists of simulations in which SSTs are restored to observations in selected basins during a historical simulation. The other type, called pacemaker hindcast, consists of seasonal hindcast simulations in which SSTs are restored to observations during 12-month forecast periods. TBIMIP is coordinated by the Climate and Ocean – Variability, Predictability, and Change (CLIVAR) Research Focus on Tropical Basin Interaction. The datasets from the model simulations will be made available to the community to facilitate and stimulate research on tropical basin interaction and its role in seasonal-to-decadal variability and climate change.

Richter, Ingo↗

A Privacy Preserving Model-Free Optimization and Control Framework for Demand Response from Residential Thermal Loads

We consider the problem of optimizing the cost of procuring electricity for a large collection of homes managed by a load serving entity, by pre-cooling or pre-heating the thermal inertial loads in the homes to avoid procuring power during periods of peak electricity pricing. We would like to accomplish this objective in a completely privacy-preserving and model-free manner, that is, without direct access to the state variables (temperatures or power consumption) or the dynamical models (thermal characteristics) of individual homes, while guaranteeing personal comfort constraints of the consumers. We propose a two-stage optimization and control framework to address this problem. In the first stage, we use a long short-term memory (LSTM) network to predict hourly electricity prices, based on historical pricing data and weather forecasts. Given the hourly price forecast and thermal models of the homes, the problem of designing an optimal power consumption trajectory that minimizes the total electricity procurement cost for the collection of thermal loads can be formulated as a large-scale integer program (with millions of variables) due to the on-off cyclical dynamics of such loads. We provide a simple heuristic relaxation to make this large-scale optimization problem model-free and computationally tractable. In the second stage, we translate the results of this optimization problem into distributed open-loop control laws that can be implemented at individual homes without measuring or estimating their state variables, while simultaneously ensuring consumer comfort constraints. We demonstrate the performance of this approach on a large-scale test case comprising of 500 homes in the Houston area and benchmark its performance against a direct model-based optimization and control solution.

Sivaranjani, S.↗

PERSIANN Dynamic Infrared–Rain Rate Model (PDIR) for High-Resolution, Real-Time Satellite Precipitation Estimation

Precipitation measurements with high spatiotemporal resolution are a vital input for hydrometeorological and water resources studies; decision-making in disaster management; and weather, climate, and hydrological forecasting. Moreover, real-time precipitation estimation with high precision is pivotal for the monitoring and managing of catastrophic hydroclimate disasters such as flash floods, which frequently transpire after extreme rainfall. While algorithms that exclusively use satellite infrared data as input are attractive owing to their rich spatiotemporal resolution and near-instantaneous availability, their sole reliance on cloud-top brightness temperature (T b ) readings causes underestimates in wet regions and overestimates in dry regions—this is especially evident over the western contiguous United States (CONUS). We introduce an algorithm, the Precipitation Estimations from Remotely Sensed Information Using Artificial Neural Networks (PERSIANN) Dynamic Infrared–Rain rate model (PDIR), which utilizes climatological data to construct a dynamic (i.e., laterally shifting) T b –rain rate relationship that has several notable advantages over other quantitative precipitation-estimation algorithms and noteworthy skill over the western CONUS. Validation of PDIR over the western CONUS shows a promising degree of skill, notably at the annual scale, where it performs well in comparison to other satellite-based products. Analysis of two extreme landfalling atmospheric rivers show that solely IR-based PDIR performs reasonably well compared to other IR- and PMW-based satellite rainfall products, marking its potential to be effective in real-time monitoring of extreme storms. This research suggests that IR-based algorithms that contain the spatiotemporal richness and near-instantaneous availability needed for rapid natural hazards response may soon contain the skill needed for hydrologic and water resource applications.

54 ENVIRONMENTAL SCIENCES↗

Predicting Frigid Mixed-Phase Clouds for Pristine Coastal Antarctica

Supercooled water is common in the clouds near coastal Antarctica and occasionally occurs at temperatures at or below -30°C. Yet the ice physics in most regional and global numerical models will glaciate out these clouds. This presents a challenge for the simulation of highly supercooled clouds that were observed at McMurdo, Antarctica during the Atmospheric Radiation Measurement (ARM) West Antarctic Radiation Experiment (AWARE) project during 2015–2017. The polar optimized version of the Weather Research and Forecasting model (Polar WRF) with the recently developed two-moment P3 microphysics scheme was used to simulate observed supercooled liquid water cases during March and November 2016. Nudging of the simulations to observed rawinsonde profiles and Antarctic automatic weather station observations provided increased realism and much greater cloud water amounts. Furthermore, sensitivity tests that adjust the ice physics for extremely low ice nucleating particle (INP) concentrations decrease cloud ice and increases the cloud liquid water closer to observed amounts. In these tests, a liquid layer near cloud top is simulated, in agreement with observations. Accurate representation of INP concentrations appears to be critical for the simulation of coastal Antarctic clouds.

54 ENVIRONMENTAL SCIENCES↗

Alaska Meteorology, Energy, and Transmission (MET) Toolkit

The Alaska MET (Meteorology, Energy, and Transmission) Toolkit is the National Laboratory of the Rockies' (NLR) new flagship atmospheric dataset, designed to support comprehensive long-term planning and operations across the entire power sector. Serving as the regional counterpart to CONUS-wide HRRR MET Toolkit, this dataset provides a comprehensive, high-fidelity meteorological record covering Alaska.The Alaska MET Toolkit is delivered at an hourly resolution on a standardized 2-km horizontal grid. This dataset is repackaged from the National Oceanic and Atmospheric Administration's (NOAA) operational High-Resolution Rapid Refresh for Alaska (HRRR-AK) forecasts. Spanning from 2019 to 2025, it overcomes the technical barriers of native weather models by providing spatial regridding from the native 3-km HRRR-AK horizontal resolution to a 2-km grid, temporal gap-filling, and vertical interpolation at key energy-relevant heights. By delivering highly accurate, validation-backed data across a comprehensive suite of atmospheric variables - including temperature, pressure, humidity, and wind characteristics - the Alaska MET Toolkit provides a highly accessible and strictly standardized foundation for modern power system modeling.

17 WIND ENERGY↗

Microphysical Piggybacking in the Weather Research and Forecasting Model

Abstract This paper presents incorporation of the microphysical piggybacking into the Weather Research and Forecasting (WRF) model. Microphysical piggybacking is to run a single simulation applying two microphysical schemes, the first scheme driving the simulation and the second piggybacking this simulated flow. “Driving the simulation” means that the simulated microphysical processes, affect the cloud buoyancy and thus force the simulated flow. In contrast, the piggybacking variables are advected by the simulated flow and undergo microphysical transformation, but they do not affect the simulated flow (like in prescribed flow—kinematic—simulations). The two sets of variables (driver and piggybacker) include temperature, water vapor mixing ratio, and all microphysical variables. We provide details of implementing piggybacking into the WRF model, illustrate its applications, and demonstrate the benefits of this methodology in two idealized three‐dimensional cases: (a) a squall line case applying two microphysics schemes, the Thompson bulk microphysics scheme and the University of Pécs/NCAR bin (UPNB) scheme. The piggybacking simulations revealed that the microphysics‐dynamics interaction plays a more important role than the pure microphysical size sorting effect in the transition zone formation. (b) A case of daytime shallow‐to‐deep convective development over land. This case uses the UPNB scheme and contrasts convection developing in environments with either pristine or polluted cloud condensation nuclei (CCN). The piggybacking results indicated that the increase of cloud cover and decrease of supersaturation are mainly associated with the microphysical effect of increasing CCN while the change of precipitation on the ground is also influenced by microphysics‐dynamics interactions.

54 ENVIRONMENTAL SCIENCES↗

Cross-Scale Land-Atmosphere Experiment (CSLAEX) (Final Report)

It is now well recognized that land-atmosphere interactions play an important role in both weather and climate. These interactions take place over a wide range of spatial and temporal scales. Most of the current formulations of the momentum, heat and moisture transport laws are informed by observations with a limited temporal or spatial scale, and hence may have limited applicability. The objective of this work is to improve the multi-scale representation of the near-surface heat transfer in the ground and in the atmosphere using a combination of modeling and field observations. Our knowledge and predictive capacity in land-atmosphere coupling is limited by our capacity to observe the full-scale spectrum at play. In order to bridge this fundamental gap in our observation capacity I will work to: create the first long-term Integrated Cross-Scale land-Atmosphere Experiment (CSLAEX) since I will work to: measure the components of the surface energy balance at a spatial scale relevant to remote sensing and meteorological applications (5km), along with observations of the nested subscale processes with Distributed Temperature Sensors (DTS). This proposal aims to fill the gaps in modeling and observing land-atmosphere interactions across scales via a novel Cross-Scale Land-Atmosphere Experiment (CSLAEX) to be implemented as part of the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site near Lamont, Oklahoma. The proposed research effort aims at exploring land-atmosphere processes across multiple spatial scales and to investigate the effect of landscape heterogeneity using Distributed Temperature Sensor measurements. The novel instrumentation of the Surface Energy Balance and simultaneous observations of the atmospheric state (boundary layer, cloud, convection) available at the DOE ARM SGP site will be used to create CSLAEX. This dataset will be used to frame and evaluate new transport laws and parameterizations for the boundary layer and the land surface, which can be implemented into the Weather and Research Forecasting (WRF) model and Community Atmospheric Model (CAM). The result of this study should impact multiple fields: meteorology, climate, and hydrology.

54 ENVIRONMENTAL SCIENCES↗

Modeling the Sources and Transport Processes During Extreme Ammonia Episodes in the U.S. Corn Belt

Abstract Atmospheric ammonia (NH 3 ) is the primary form of reactive nitrogen (N r ) and a precursor of ammonium (NH 4 + ) aerosols. Ammonia has been linked to adverse impacts on human health, the loss of ecosystem biodiversity, and plays a key role in aerosol radiative forcing. The midwestern United States is the major NH 3 source in North America because of dense livestock operations and the high use of synthetic nitrogen fertilizers. Here, we combine tall‐tower (100 m) observations in Minnesota and Weather Research and Forecasting model coupled with Chemistry (WRF‐Chem) modeling to investigate high and low NH 3 emission episodes within the U.S. Corn Belt to improve our understanding of the distribution of emission sources and transport processes. We examined observations and performed model simulations for cases in February through November of 2017 and 2018. The results showed the following: (1) Peak emissions in November 2017 were enhanced by above‐normal air temperatures, implying a Q 10 (i.e., the change in NH 3 emissions for a temperature increase of 10°C) of 2.5 for emissions. (2) The intensive livestock emissions rom northern Iowa, approximately 400 km away from the tall tower, accounted for 17.6% of the abundance in tall‐tower NH 3 mixing ratios. (3) Ammonia mixing ratios in the innermost domain 3 frequently (i.e., 336 hr, 48% of November 2017) exceeded 5.3 ppb, an important air quality health standard. (4) In November 2017, simulated NH 3 net ecosystem exchange (the difference between NH 3 emissions and dry deposition) accounted for 60–65% of gross NH 3 emissions for agricultural areas and was 2.8–3.1 times the emissions of forested areas. (5) We estimated a mean annual NH 3 net ecosystem exchange of 1.60 ± 0.06 nmol · m −2 · s −1 for agricultural lands and −0.07 ± 0.02 nmol · m −2 · s −1 for forested lands. These results imply that future warmer fall temperatures will enhance agricultural NH 3 emissions, increase the frequency of dangerous NH 3 episodes, and enhance dry NH 3 deposition in adjacent forested lands.

Hu, Cheng↗