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At least 289 records · Page 16

Geometry dependence of optical pulse broadening in multiple scattering media

A Monte Carlo simulation method has been used to evaluate the temporal response at a variety of receivers to an instantaneous laser pulse input to a turbid medium. The results are compared to the description of the ensemble of all transmitted photons for which a diffusion theory was developed. It was shown that the arrival times for all photons transmitted through the cloud are exponentially distributed with a mean time that varies as the product of the cloud thickness and the momentum transfer optical depth. For large optical depths the mean time delay associated with all reflected photons was found to depend only on the cloud thickness. The impulse response function for receivers on the beam axis varied with field of view and for small fields of view it was dominated by single scattering even for optically thick clouds. In these cases, the mean time delay could be up to 10 to the 6th times shorter than that associated with all transmitted photons with a related increase in the maximum modulation frequency.

Thomas, R. W. L.↗

Raman Lidar Measurements of Water Vapor and Cirrus Clouds During The Passage of Hurricane Bonnie

The NASA/GSFC Scanning Raman Lidar (SRL) was stationed on Andros Island in the Bahamas during August - September, 1998 as a part of the third Convection and Moisture Experiment (CAMEX-3) which focussed on hurricane development and tracking. During the period August 21 - 24, hurricane Bonnie passed near Andros Island and influenced the water vapor and cirrus cloud measurements acquired by the SRL. Two drying signatures related to the hurricane were recorded by the SRL and other sensors. Cirrus cloud optical depths (at 351 nm) were also measured during this period. Optical depth values ranged from less than 0.01 to 1.5. The influence of multiple scattering on these optical depth measurements was studied. A correction technique is presented which minimizes the influences of multiple scattering and derives information about cirrus cloud optical and physical properties. The UV/IR cirrus cloud optical depth ratio was estimated based on a comparison of lidar and GOES measurements. Simple radiative transfer model calculations compared with GOES satellite brightness temperatures indicate that satellite radiances are significantly affected by the presence of cirrus clouds if IR optical depths are approximately 0.005 or greater. Using the ISCCP detection threshold for cirrus clouds on the GOES data presented here, a high bias of up to 40% in the GOES precipitable water retrieval was found.

Whiteman, D. N.↗

IRAS low-resolution spectral observations of the 10 and 18 micron silicate emission feature

The IRAS LRS Atlas contains 8-23 micron spectra of 1816 stars with silicate emission features. In order to study the shapes of the silicate dust features, the 117 stars whose emission features appear to be optically thin and which have the best signal-to-noise ratio at the longest wavelengths were analyzed. Simple spherical dust shell models were calculated in both the optically thin and the slightly optical thick approximations. From the comparison of the predicted spectra of the dust and stellar continuum, the emissivity function Kappa(lambda) was derived. In the different stars, the shape of the 10-micron feature is either narrow or broad and it is peaked either at about 9.7 microns or at 10 microns. Either particle size effects (particles above 0.75 microns in radius) or optical depth effects (central optical depth about 1) could broaden the 10-micron feature. Chemical composition differences no doubt are also important, particularly as regards the position of the peak of the 10-micron feature. The stars with the peak at 10 microns are more closely confined to the Galactic plane than the stars with the peak at 9.7 microns. The shape of the 18-micron feature is essentially the same in all stars, and can be used to extend the interstellar extinction curve past 13 to 22 microns.

Simpson, Janet P.↗

Sources, Transport, and Climate Impacts of Biomass Burning Aerosols

In this presentation, I will first talk about fundamentals of modeling of biomass burning emissions of aerosols, then show the results of GOCART model simulated biomass burning aerosols. I will compare the model results with observations of satellite and ground-based network in terms of total aerosol optical depth, aerosol absorption optical depth, and vertical distributions. Finally the long-range transport of biomass burning aerosols and the climate effects will be addressed. I will also discuss the uncertainties associated with modeling and observations of biomass burning aerosols

Chin, Mian↗

A Unified Picture of Pinatubo Aerosol Global-to Micro-Scale Evolution, From Space, Air, and Ground Measurements

We combine a variety of measurements to develop a composite picture of the post-Pinatubo aerosol and assess the consistency and uncertainties of the measurement and retrieval techniques. Satellite infrared spectroscopy, particle morphology, and evaporation temperature measurements are in accord with theoretical calculations in showing a dominant particle composition of H2SO4-H2O mixture, with H2SO4 weight fraction of 65-80% for most stratospheric temperatures and humidities. Important exceptions are: (1) the presence of volcanic ash at all altitudes initially and in a layer just above the tropopause until at least March 1992, and (2) much smaller H2SO4 weight fractions at the low temperatures attained in high latitude winters and at the tropical tropopause, Laboratory spectroscopy and theoretical calculations yield wavelength- and temperature-dependent refractive indices for the dominant H2SO4-H2O droplets. These in turn permit derivation of particle size spectra from measured optical depth spectra, for comparison to direct measurements by impactors and optical counters. All three techniques paint a generally consistent picture of the evolution of R(sub eff), the effective, or area-weighted, particle radius. In the first month after the eruption, although particle numbers increased by orders of magnitude, R(sub eff) was similar to the preemption value of 0.1 to 0.2 microns, because both small (r less than 0.2 microns) and large (r greater than 0.6 micron particles increased in number. Over the next 3-6 months, R(sub eff) increased to about 0.5 microns reflecting particle growth through condensation and coagulation. In general, R(sub eff) continued to increase for about a year after the eruption. Extinction spectra computed from in situ size distribution measurements are consistent with optical depth measurements, which show spectra with maxima initially at wavelengths of 0.42 microns or less, and thereafter progressively increasing to between 0.78 and 1 micron. Not until 1993 do optical depth spectra begin to show a clear return to the preemption signature of maximizing at the shortest visible wavelengths or in the near UV. This coupled evolution in particle size distribution and optical depth spectra helps explain the relationship between the global maps of 0.5- 1.0- micron optical depth derived from the AVHRR and SAGE satellite measurements.

Russell, Philip B.↗

Pinatubo Aerosol Global-to-Micro-Scale Evolution: A Unified Picture From Space, Air, and Ground Measurements

We combine a variety of measurements to develop a composite picture of the post-Pinatubo aerosol and assess the consistency and uncertainties of the measurement and retrieval techniques Satellite infrared spectroscopy, particle morphology, and evaporation temperature measurements are in accord with theoretical calculations In showing a dominant particle composition of H2SO4-H2O mature with H2SO4 weight traction of 65-80% for most stratospheric temperatures and humidities. Important exceptions are: (1) the presence of volcanic ash at all attitudes initially and in a layer just above the tropopause until at least March 1992, and (2) much smaller H2SO4 weight fractions at the low temperatures attained In high latitude winters and at the tropical tropopause. Laboratory spectroscopy and theoretical calculations yield wavelength- and temperature-dependent refractive indices for the dominant H2SO4-H2O droplets. These in turn permit derivation of particle size spectra from measured optical depth spectra for comparison to direct measurements by impactors and optical counters, All three techniques paint a generally consistent picture of the evolution of R(sub eff) the effective, or area-weighted, particle radius. In the first month after the eruption, although particle numbers increased by orders of magnitude, R(sub eff) was similar to the pre-eruption value of 0.1 to 0.2 microns because both small (r less than 0.2 microns) and large (r greater than 0.6 microns) particles increased in number. Over the next 3-6 months, R(sub eff) increased to about 0.5 microns, reflecting particle growth through condensation and coagulation. In general, R(sub eff) continued to increase for about a year after the eruption. Extinction spectra computed from in situ size distribution measurements are consistent with optical depth measurements, which show spectra with maxima initially at wavelengths of 0.42 microns or less, and thereafter progressively increasing to between 0.78 and 1 micron. Not until 1993 does optical depth spectra begin to show a clear return to the preeruption signature of maximizing at the shortest visible wavelengths or in the near UV. This coupled evolution in particle size distribution and optical depth spectra helps explain the relationship between the global maps of 0.5- and 1.0-kilometer optical depth derived from the AVHRR and SAGE satellite measurements. It also sets a context for evaluating remaining uncertainties in each of these satellite data products. We also show how the effects of wavelength-dependent refractive index on backscatter spectra can influence particle sizes retrieved from multiwavelength lidar measurements.

Russell, Philip B.↗

The 27-28 October 1986 FIRE IFO cirrus case study: Cirrus parameter relationships derived from satellite and lidar data

Cirrus cloud radiative and physical characteristics are determined using a combination of ground-based, aircraft, and satellite measurements taken as part of the First ISCCP Regional Experiment (FIRE) Cirrus Intensive Field Observations (IFO) during October and November 1986. Lidar backscatter data are used to define cloud base, center, and top heights and the corresponding temperatures. Coincident GOES 4 km visible (0.65 microns) and 8 km infrared window (11.5 microns) radiances are analyzed to determine cloud emittances and reflectances. Infrared optical depth is computed from the emittance results. Visible optical depth is derived from reflectance using a theoretical ice crystal scattering model and an empirical bidirectional reflectance mode. No clouds with visible optical depths greater than 5 or infrared optical depths less than 0.1 were used in the analysis. Average cloud thickness ranged from 0.5 km to 8 km for the 71 scenes. An average visible scattering efficiency of 2.1 was found for this data set. The results reveal a significant dependence of scattering efficiency on cloud temperature.

Minnis, Patrick↗

The 27-28 October 1986 FIRE IFO cirrus case study - Cirrus parameter relationships derived from satellite and lidar data

Cirrus cloud radiative and physical characteristics are determined using a combination of ground-based, aircraft, and satellite measurements taken as part of the First ISCCP Regional Experiment (FIRE) Cirrus Intensive Field Observations (IFO) during October and November 1986. Lidar backscatter data are used to define cloud base, center, and top heights and the corresponding temperatures. Coincident GOES 4 km visible (0.65 microns) and 8 km infrared window (11.5 microns) radiances are analyzed to determine cloud emittances and reflectances. Infrared optical depth is computed from the emittance results. Visible optical depth is derived from reflectance using a theoretical ice crystal scattering model and an empirical bidirectional reflectance mode. No clouds with visible optical depths greater than 5 or infrared optical depths less than 0.1 were used in the analysis. Average cloud thickness ranged from 0.5 km to 8 km for the 71 scenes. An average visible scattering efficiency of 2.1 was found for this data set. The results reveal a significant dependence of scattering efficiency on cloud temperature.

Minnis, Patrick↗

UV albedo of clouds from TOMS data

The Pilot Climate Data System (PCDS) was found to be useful in examining a subset of data from the Nimbus-7 Total Ozone Mapping Spectrometer (TOMS). The TOMS instrument scans with six channels between .3 and .4 micrometers. It was suggested that by analyzing albedo values from the longer wavelength channels of the TOMS, the effects of increasing optical depth could be determined. It is spectral relationship of albedo-to-optical depth that is investigated here. The question can be stated: Is there spectral differentiation in albedo with changes in the optical depth of clouds? Nimbus-7 TOMS data were obtained through the PCDS for an area and time period for which correlative NOAA AVHRR data were available. The AVHRR data were important in determining the existing cloud patterns. As expected, no spectral differentiation was observed at very high albedos (associated with high optical depths). However, at lower optical depths, evidence of spectral dependence on albedo was observed. Mapping the results geographically was deemed highly desirable but was not possible through the PCDS at the time. The PCDS can be viewed as an effective research tool to access selected portions of data. Without being intimately familiar with a data set, a PCDS user can successfully manipulate data in a scientific study.

Short, D.↗

Investigations of atmospheric extinction using direct solar radiation measurements made with a multiple wavelength radiometer.

A multiple wavelength solar radiometer designed for the purpose of measuring atmospheric optical depth at discrete wavelengths through the visible region is described. Experimental techniques, including sample observations, are presented for obtaining atmospheric optical depth from radiometer measurements. These techniques apply for conditions where the optical depth is either temporally variant or invariant during the course of a day. The influence of the aerosol size distribution on optical depth is investigated. Theoretical calculations of the wavelength dependency of the aerosol optical depth contribution are presented for several representative aerosol size distributions. Methods are also presented for estimating the aerosol size distribution and aerosol mass loading from multiwavelength optical depth measurements.

Shaw, G. E.↗

Inferring Cloud Properties from Passive Solar Sensors

The most common approach for retrieving cloud optical depth from ground-based observations uses downwelling fluxes measured by pyranometers and Multi-Filter Rotating Shadowband Radiometers (MFRSR). The key element in both retrieval techniques is the one-to-one mapping of the "observed" fluxes into cloud optical depth through plane-parallel radiative transfer. Both methods are expected to work well only for completely overcast clouds giving an effective optical depth for the whole sky. To infer cloud optical depth locally one can assume to use a narrow-field-of view radiometer that measures radiances instead of fluxes. However, lack of one-to-one relationships between radiance and cloud optical depth, prevents the direct use of radiances either. Here we discuss a new method for retrieving cloud optical depth from ground-based measurements of zenith radiance in the RED and near infrared (NIR) spectral regions. In addition to an algebraic combinations of spectral radiances such as Normalized Difference Cloud Index (NDCI) that largely removes nonuniqueness and the radiative effects of cloud inhomogeneity but can result in poor retrievals due to its insensitivity to cloud fraction, both RED and NIR radiances as points on the "RED vs. NIR" plane are proposed to be used for retrieval. The proposed retrieval method is applied to a multi- channel sunphotometer (as a part of AERONET) measurements at the ARM site in Oklahoma. The results of retrieval are compared with the ones from Microwave Radiometer (MWR) and MFRSR. In addition to cloud optical depth, the new retrieval method also infers a "radiatively effective" cloud fraction.

Marshak, A.↗

Cloud Radiative Forcing at the ARM Climate Research Facility: Technique, Validation, and Comparison to Satellite-derived Diagnostic Quantities - Part 1

It has been hypothesized that continuous ground-based remote sensing measurements from active and passive remote sensors combined with regular soundings of the atmospheric thermodynamic structure can be combined to describe the effects of clouds on the clear sky radiation fluxes. We critically test that hypothesis in this paper and a companion paper (Part II). Using data collected at the Southern Great Plains (SGP) Atmospheric Radiation Measurement (ARM) site sponsored by the U.S. Department of Energy, we explore an analysis methodology that results in the characterization of the physical state of the atmospheric profile at time resolutions of five minutes and vertical resolutions of 90 m. The description includes thermodynamics and water vapor profile information derived by merging radiosonde soundings with ground-based data, and continues through specification of the cloud layer occurrence and microphysical and radiative properties derived from retrieval algorithms and parameterizations. The description of the atmospheric physical state includes a calculation of the infrared and clear and cloudy sky solar flux profiles. Validation of the methodology is provided by comparing the calculated fluxes with top of atmosphere (TOA) and surface flux measurements and by comparing the total column optical depths to independently derived estimates. We find over a 1-year period of comparison in overcast uniform skies, that the calculations are strongly correlated to measurements with biases in the flux quantities at the surface and TOA of less than 10% and median fractional errors ranging from 20% to as low as 2%. In the optical depth comparison for uniform overcast skies during the year 2000 where the optical depth varies over 3 orders of magnitude we find a mean positive bias of 46% with a median bias of less than 10% and a 0.89 correlation coefficient. The slope of the linear regression line for the optical depth comparison is 0.86 with a normal deviation of 20% about this line. In addition to a case study where we examine the cloud radiative effects at the TOA, surface and atmosphere by a middle latitude synoptic-scale cyclone, we examine the cloud top pressure and optical depth retrievals of ISCCP and LBTM over a period of 1 year. Using overcast period from the year 2000, we find that the satellite algorithms tend to bias cloud tops into the middle troposphere and underestimate optical depth in high optical depth events (greater than 100) by as much as a factor of 2.

Mace, Gerald G.↗

Aerosol Climate Effects: Local Radiative Forcing and Column Closure Experiments

In an effort to reduce uncertainties in climate change predictions, experiments are being planned and conducted to measure anthropogenic aerosol properties and effects, including effects on radiative fields. The global average, direct anthropogenic aerosol effect on upwelling shortwave fluxes is estimated to be about +1/2 W/sq m, whereas errors in flux changes measured with airborne and spaceborne radiometers are 2 to 8 W/sq m or larger. This poses the question of whether flux changes expected in field experiments will be large enough to measure accurately. This paper obtains a new expression for the aerosol-induced change in upwelling flux, compares it to two-stream and adding-doubling (AD) results, and uses all three methods to estimate expected flux changes. The new expression accounts for the solar zenith angle dependences of aerosol transmission and reflection, as well as of surface albedo, all of which can have a strong effect in determining flux changes measured in field experiments. Despite its relative simplicity, the new expression gives results similar to previous two-stream results. Relative to AD results, it agrees within a few watts per square meter for the intermediate solar elevation angles where the flux changes peak (roughly 10 to 30 degrees), but it has negative errors for higher Sun and positive errors for lower Sun. All three techniques yield aerosol-induced changes in upwelling flux of +8 to +50 W/sq m for aerosol midvisible optical depths of 0.1 to 0.5. Because such aerosol optical depths occur frequently off the U.S. and European Atlantic coasts in summer, the flux changes they induce should be measurable by airborne, and possibly by spaceborne, radiometers, provided sufficient care is taken in experiment design (including measurements to separate aerosol radiative effects from those of absorbing gases). The expected flux changes are about 15 to 100 times larger than the global average flux change expected for the global average anthropogenic sulfate optical depth of 0.04. Reasons for the larger flux changes include the larger optical depths considered here (factor 2.5 to 12), plus restricting the measurements to cloud-free, daytime conditions over the ocean (factor 5 to 9).

Russell, P. B.↗

SAM 2 measurements of the polar stratospheric aerosol. Volume 9: October 1982 - April 1983

The Stratospheric Aerosol Measurement (SAM) II sensor aboard Nimbus 7 is providing 1.0 micron extinction measurements of Antarctic and Arctic stratospheric aerosols with a vertical resolution of 1 km. Representative examples and weekly averages including corresponding temperature profiles provided by NOAA for the time and place of each SAM II measurement are presented. Contours of aerosol extinction as a function of altitude and longitude or time are plotted, and aerosol optical depths are calculated for each week. Typical values of aerosol extinction and stratospheric optical depth in the Arctic are unusually large due to the presence of material from the El Chichon volcano eruption in the Spring of 1982. For example, the optical depth peaked at 0.068, more than 50 times background values. Typical values of aerosol extinction and stratospheric optical depth in the Antarctic varied considerably during this period due to the transport and arrival of the material from the El Chichon eruption. For example, the stratospheric optical depth varied from 0.002 in October 1982, to 0.021 in January 1983. Polar stratospheric clouds were observed during the Arctic winter, as expected. A representative sample is provided of the ninth 6-month period of data to be used in atmospheric and climatic studies.

Mcmaster, L. R.↗

Cloud Physics Lidar Measurements During the SAFARI-2000 Field Campaign

A new remote sensing instrument, the Cloud Physics Lidar (CPL) has been built for use on the ER-2 aircraft. The first deployment for CPL was the SAFARI-2000 field campaign during August-September 2000. The CPL is a three-wavelength lidar designed for studies of cirrus, subvisual cirrus, and boundary layer aerosols. The CPL utilizes a high repetition rate, low pulse energy laser with photon counting detectors. A brief description of the CPL instrument will be given, followed by examples of CPL data products. In particular, examples of aerosol backscatter, including boundary layer smoke and cirrus clouds will be shown. Resulting optical depth estimates derived from the aerosol measurements will be shown. Comparisons of the CPL optical depth and optical depth derived from microPulse Lidar and the AATS-14 sunphotomer will be shown.

McGill, Matthew↗

Estimates of the Spectral Aerosol Single Sea Scattering Albedo and Aerosol Radiative Effects during SAFARI 2000

Using measurements of the spectral solar radiative flux and optical depth for 2 days (24 August and 6 September 2000) during the SAFARI 2000 intensive field experiment and a detailed radiative transfer model, we estimate the spectral single scattering albedo of the aerosol layer. The single scattering albedo is similar on the 2 days even though the optical depth for the aerosol layer was quite different. The aerosol single scattering albedo was between 0.85 and 0.90 at 350 nm, decreasing to 0.6 in the near infrared. The magnitude and decrease with wavelength of the single scattering albedo are consistent with the absorption properties of small black carbon particles. We estimate the uncertainty in the single scattering albedo due to the uncertainty in the measured fractional absorption and optical depths. The uncertainty in the single scattering albedo is significantly less on the high-optical-depth day (6 September) than on the low-optical-depth day (24 August). On the high-optical-depth day, the uncertainty in the single scattering albedo is 0.02 in the midvisible whereas on the low-optical-depth day the uncertainty is 0.08 in the midvisible. On both days, the uncertainty becomes larger in the near infrared. We compute the radiative effect of the aerosol by comparing calculations with and without the aerosol. The effect at the top of the atmosphere (TOA) is to cool the atmosphere by 13 W/sq m on 24 August and 17 W/sq m on 6 September. The effect on the downward flux at the surface is a reduction of 57 W/sq m on 24 August and 200 W/sq m on 6 September. The aerosol effect on the downward flux at the surface is in good agreement with the results reported from the Indian Ocean Experiment (INDOEX).

Bergstrom, Robert W.↗

An analysis of haze effects on LANDSAT multispectral scanner data

Early season changes in optical depth change brightness, primarily along the soil line; and during crop development, changes in optical depth change both greenness and brightness. Thus, the existence of haze in the imagery could cause an unsuspecting analyst to interpret the spectral appearance as indicating an episodal event when, in fact, haze was present. The techniques for converting LANDSAT-3 data to simulate LANDSAT-2 data are in error. The yellowness and none such computations are affected primarily. Yellowness appears well correlated to optical depth. Experimental evidence with variable background and variable optical depth is needed, however. The variance of picture elements within a spring wheat field is related to its equivalent in optical depth changes caused by haze. This establishes the sensitivity of channel 1 (greenness) pixels to changes in haze levels. The between field picture element means and variances were determined for the spring wheat fields. This shows the variability of channel data on two specific dates, emphasizing that crop development can be influenced by many factors. The atmospheric correction program ATCOR reduces segment data from LANDSAT acquisitions to a common haze level and improves the results of analysis.

Johnson, W. R.↗

Distribution and Radiative Forcing of Tropical Thin Cirrus Clouds

To understand the radiative impact of tropical thin cirrus clouds, the frequency of occurrence and optical depths of these clouds have been derived. Thin cirrus clouds are defined here as being those that are not detected by the operational Moderate Resolution Imaging Spectroradiometer (MODIS) cloud mask, corresponding to an optical depth value of approximately 0.3 or smaller, but that are detectable in terms of the cirrus reflectance product based on the MODIS 1.375-micron channel. With such a definition, thin cirrus clouds were present in more than 40% of the pixels flagged as clear sky by the operational MODIS cloud mask algorithm. It is shown that these thin cirrus clouds are frequently observed in deep convective regions in the western Pacific. Thin cirrus optical depths were derived from the cirrus reflectance product. Regions of significant cloud fraction and large optical depths were observed in the Northern Hemisphere during the boreal spring and summer and moved southward during the boreal autumn and winter. The radiative effects of tropical thin cirrus clouds were studied on the basis of the retrieved cirrus optical depths, the atmospheric profiles derived from the Atmospheric Infrared Sounder (AIRS) observations, and a radiative transfer model in conjunction with a parameterization of ice cloud spectral optical properties. To understand how these clouds regulate the radiation field in the atmosphere, the instantaneous net fluxes at the top of the atmosphere (TOA) and at the surface were calculated. The present study shows positive and negative net forcings at the TOA and at the surface, respectively. The positive (negative) net forcing at the TOA (surface) is due to the dominance of longwave (shortwave) forcing. Both the TOA and surface forcings are in a range of 0-20 W/sq m, depending on the optical depths of thin cirrus clouds.

THIN CIRRUS CLOUDS↗