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At least 289 records · Page 16

Atomic oxygen-metal surface studies as applied to mass spectrometer measurements of upper planetary atmospheres

The problem of atomic oxygen loss in mass spectrometer ion sources can be reduced to an understanding of the possible surface interactions between oxygen atoms and the metal surface of the ion source. Results are presented for an experimental study in which an atomic oxygen beam apparatus and a mass spectrometer were used to measure the oxygen atom reflection, recombination, general surface reaction, and occlusion probabilities on six different engineering surfaces as a function of atomic oxygen exposure. The materials studied are gold, Nichrome V, aluminum, titanium, silver, and platinum. The variation in measured reflection probability seems to occur with metals that form oxides, Nichrome V being stable in terms of reflection stability. Recombination is observed an all surfaces except aluminum and platinum. Variation in the complete set of measurements in a single experiment is the result of varying surface conditions.

Sjolander, G. W.↗

The open-source neutral-mass spectrometer on Atmosphere Explorer-C, -D, and -E.

The open-source mass spectrometer will be used to obtain the number densities of the neutral atmospheric gases in the mass range 1 to 48 amu at the satellite location. The ion source has been designed to allow gas particles to enter the ionizing region with the minimum practicable number of prior collisions with surfaces. This design minimizes the loss of atomic oxygen and other reactive species due to reactions with the walls of the ion source. The principal features of the open-source spectrometer and the laboratory calibration system are discussed.

Nier, A. O.↗

Gas Pressure Gauge Based on Alpha-Particle Induced Ion Currents

The use of ionization currents for measuring pressure was first demonstrated in the late 1940's. The early gauges operated at high voltages and used rather large ion sources. The ionization gauge is actually a densitometer that is sensitive to the temperature and pressure of the gas in the chamber. This report describes the use of low voltages and small ion sources in the development of a prototype.

transducers gas pressure gauge alpha particles ion↗

The Origin of the Near-Earth Plasma Population During a Substorm on November 24, 1996

We investigate the origins and the transport of ions observed in the near-Earth plasma sheet during the growth and expansion phases of a magnetospheric substorm that occurred on November 24, 1996. Ions observed at Geotail were traced backward in time in time-dependent magnetic and electric fields to determine their origins and the acceleration mechanisms responsible for their energization. Results from this investigation indicate that, during the growth phase of the substorm, most of the ions reaching Geotail had origins in the low latitude boundary layer (LLBL) and had already entered the magnetosphere when the growth phase began. Late in the growth phase and in the expansion phase a higher proportion of the ions reaching Geotail had their origin in the plasma mantle. Indeed, during the expansion phase more than 90% of the ions seen by Geotail were from the mantle. The ions were accelerated enroute to the spacecraft; however, most of the ions' energy gain was achieved by non-adiabatic acceleration while crossing the equatorial current sheet just prior to their detection by Geotail. In general, the plasma mantle from both southern and northern hemispheres supplied non-adiabatic ions to Geotail, whereas the LLBL supplied mostly adiabatic ions to the distributions measured by the spacecraft. Distribution functions computed at the ion sources indicate that ionospheric ions reaching Geotail during the expansion phase were significantly heated. Plasma mantle source distributions indicated the presence of a high-latitude reconnection region that allowed ion entry into the magnetosphere when the IMF was northward. These ions reached Geotail during the expansion phase. Ions from the traditional plasma mantle had access to the spacecraft throughout the substorm.

Ashour-Abdalla, M.↗

Mass spectrometric determination of the composition of the Venus clouds

The design of a mass spectrometer, based on the results of the Venera and Mariner probes, with sensitivity high enough to detect the HCl in the Venus atmosphere is discussed. One way to analyze the clouds is by the introduction of the atmosphere with cloud particles through a molecular leak into the mass spectrometer. The analysis can be performed in regular Nier-type ion sources with the electrodes of materials which are completely free of Cl and F. The problem of preventing the blockage of the capillaries to the Nier type ion source is also considered.

Source record↗

Characterization and automated optimization of laser-driven proton beams from converging liquid sheet jet targets

Compact, stable, and versatile laser-driven ion sources hold great promise for applications ranging from medicine to materials science and fundamental physics. While single-shot sources have demonstrated favorable beam properties, including the peak fluxes necessary for several applications, high-repetition-rate operation will be necessary to generate and sustain the high average flux needed for many of the most exciting applications of laser-driven ion sources. Further, to navigate through the high-dimensional space of laser and target parameters toward experimental optima, it is essential to develop ion acceleration platforms compatible with machine learning techniques and capable of autonomous real-time optimization. Here, we present a multi-Hz ion acceleration platform employing a liquid sheet jet target. We characterize the laser-plasma interaction and the laser-driven proton beam across a variety of key parameters governing the interaction using an extensive suite of online diagnostics. We also demonstrate real-time, closed-loop optimization of the ion beam maximum energy by tuning the laser wave front using a Bayesian optimization scheme. This approach increased the maximum proton energy by 11% compared to a manually optimized wave front by enhancing the energy concentration within the laser focal spot, demonstrating the potential for closed-loop optimization schemes to tune future ion accelerators for robust high-repetition-rate operation.

Glenn, G. D. [SLAC National Accelerator Laboratory↗

A new mass spectrometer system for investigating laser-induced vaporization phenomena

A laser has been combined with a mass spectrometer in a new configuration developed for studies of high-temperature materials. A vacuum-lock, solid-sample inlet is mounted at one end of a cylindrical, high-vacuum chamber one meter in length with a nude ion-source, time-of-flight mass spectrometer at the opposite end. The samples are positioned along the axis of the chamber at distances up to one meter from the ion source, and their surfaces are vaporized by a pulsed laser beam entering via windows on one side of the chamber. The instrumentation along with its capabilities is described, and results from laser-induced vaporization of several graphites are presented.

Lincoln, K. A.↗

Operating Characteristics of a 15-cm dia. Ion Engine for Small Planetary Spacecraft

A 15-cm diameter, scaled-down version of the NASA light-weight 30-cm ion engine has been developed for potential application to very small planetary spacecraft. Integration of the 15-cm ion source into 4x15-cm segmented engine configuration results in a 30-cm equivalent engine which can be throttled over a 7-to-1 input power variation with a constant beam current in each of the four segments. Throttling the segmented engine by turning off individual segments can result in a significant decrease in the required service life (and qualification requirements) of the ion source components.

grids segmented ion engine↗

Sputter sample preparation for ion beam delivery of radium-223 at ATLAS

A radium-223 ion beam was delivered to an experiment from the electron cyclotron resonance ion source, ECR2, at the Argonne Tandem Linac Accelerator System (ATLAS). Here, the radium-223 material was in a nitrate salt form within a vial, prior to being converted to a usable sputter sample. The sputter sample was produced using a new sample preparation method, where the radium nitrate was dissolved into a solution and pipetted onto pressed aluminum powder. This sample was then allowed to dry, distributing the radium-223 material throughout the sputter sample. Ion source operation using the radium sputter sample is described with the operating parameters listed. The intensity and energy requirements for this ion beam were 1 × 10 6 particles/s and 1.07 GeV, respectively. Because the intensity is relatively low compared to most experiments at ATLAS, previously developed accelerator mass spectrometry methods were used Scott et al. to avoid the need for tuning of the low-intensity beam of interest. Handling of the radium material, as well as loading and unloading of the sputter sample from ECR2, required collaboration with Health Physics. Procedures were used and dry runs were carried out before, during, and after the experiment to ensure the safety of the workers. The processes used and lessons learned are described within.

07 ISOTOPE AND RADIATION SOURCES↗

Experiments with a prototype titanium hot cavity surface ionization source intended for electromagnetic separation of radioactive samarium and other lanthanide elements

This paper reports experimental results of a prototype titanium surface ionization source. For the first time, a lanthanide ion beam has been produced with a surface ionizer composed completely of titanium metal. Titanium does not readily activate with neutron irradiation. This offers the potential for inserting an ion source made of titanium directly into a reactor with a pre-loaded non-radioactive lanthanide target. This seamlessly integrates target irradiation with isotope separation, eliminating post irradiation sample manipulation. Samarium ion beam currents up to 960 nA have been produced in an off-line test bench equipped with rudimentary beam optics. This is a crucial step toward the development of an ionization source adopted for the electromagnetic isotope separator (EMIS) facility, which has been designed for high throughput separations of radioactive 153 Sm and other lanthanides of interest in the field of nuclear medicine. The ion current and important factors affecting the performance of the ion source, such as the ionizer temperature and thermal gradient, are discussed. Lastly, the experimental results are presented together with a discussion of future modifications to optimize the overall surface ionization source performance.

07 ISOTOPE AND RADIATION SOURCES↗

Atomic and molecular oxygen densities in the lower thermosphere

The Atmospheric Explorer-C satellite used a neutral mass spectrometer containing a quasi-open ion source operating either in normal mode or in one that utilizes the satellite velocity to distinguish between incoming ambient particles and ambient particles which have struck instrument surfaces and become accommodated. An analysis was made of data from the mass spectrometer for those orbits when the open ion source operated either partially or entirely in the fly-through mode. A comparison of N2 density, total O density and O2/N2 density values at 200 km was made. The average N2 and O2 density values agree well with previous rocket soundings and other studies. It is believed that the individual absolute number densities obtained in the normal mode of operation are accurate to within 20% while those deduced from fly-through data may be accurate to only 30%.

Nier, A. O.↗

In situ Detection of Plasma Induced Surface Interaction based on Deep Learning based Visual Diagnostics (Technical Report)

It is characteristic for many plasma devices to undergo plasma-material interaction leading to surface erosion. These processes, often not easily detectable, lead to changes in device performance and lifespan. State-of-the-art lifetime tests and wear experiments require over 1000s hours. A self-consistent model for accurately predicting the erosion's effects is not available. In situ detection of these processes is not a trivial task since the surface variations at the early stages have a micron scale. Such limitations not only restrict testing and prediction capabilities but also slow the development of new thrusters and limit mission duration. To address these challenges, an in-situ diagnostic for real-time erosion assessment has been developed, aiming to expedite lifetime testing and broaden experimental campaigns. Several works were dedicated to real-time and in situ monitoring of material erosion during plasma exposure using laser holography, microscopy, and with telemicroscopes. However, the applicability of these approaches is limited due to complexity, cost and less flexibility as they often require placing diagnostic equipment inside the vacuum chamber. In collaboration with Princeton Collaborative Research Facility (PCRF), Princeton Plasma Physics Laboratory (PPPL), a new diagnostic approach is developed, where geometry modifications to the ceramic channel walls were introduced that would result in accelerated channel erosion. We employed Long-distance microscope (LDM) imagery, combined with Deep-Learning based Shape from focus or depth from focus (DFF or SFF) approach, that provides an accessible and cost-effective solution. LDM employs focus variation techniques to continuously capture multiple images of the target object at distinct focal planes. DFF, an optical focus variation method, generates a 3D topographical surface depth map from a sequence of variably focused images. Combined with the developed diagnostic, this approach offers a controllable means to study erosion under accelerated conditions. In this work, we develop Neural Network-based DFF algorithm applicable for LDM data to quantitatively evaluate plasma induced surface modification from LDM data. Next, we develop Deep Learning-based super-resolution depth map image reconstruction technique to increase the resolution of depth maps obtained from DFF algorithm to improve the accuracy of erosion measurements. Thirdly, we develop several image processing techniques to remove noise and improve the quality of depth map image. Here we report the results of initial tests for this approach. An experimental setup designed and built in PPPL was employed that consists of a 3-cm gridded ion source that produces a neutralized argon beam with energies up to 600 eV. A hexagonal boron nitride (h-BN) ceramic target, designed based on computational predictions, was used. Tests were conducted to reconstruct the complex geometry of the target under the lighting conditions of the operated ion source.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Low-energy H- beam injectors for particle accelerators: upgrade requirements, challenges and future plans [Slides]

High brightness, negative hydrogen ion sources are used extensively in large, accelerator-based, user facilities operating worldwide. Negative hydrogen beams have become the preferred means of filling circular accelerators and storage rings as well as enabling efficient extraction from cyclotrons. Much larger beams of H- ions are also utilized for neutral beams injection into fusion machines and will be discussed in a separate companion presentation. Some of the accelerator facilities include the US Spallation Neutron Source (SNS), Japan Proton Accelerator Research Complex (J-PARC), Rutherford Appleton Laboratory (RAL-ISIS), Los Alamos Neutron Science Center (LANSCE), Fermi National Accelerator Laboratory (FNAL), Brookhaven National Laboratory (BNL), the CERN LHC injector, the Chinese Spallation Neutron Source (CSNS) as well as numerous installations of D-Pace (licenced by TRIUMF) ion sources used mainly with cyclotrons. Many facilities are currently working on various improvement / upgrade projects, both in the near and long term, which are driving further development of their ion source and LEBT (Low Energy Beam Transport) and, in some cases, their overall front end injector system. This report will first provide a simple description of each facilities existing ion source and LEBT and summarize the operational parameters which are currently being routinely injected into their accelerators. Next, the parametric goals of each of the facilities upgrade projects are specified as well as development efforts currently underway to meet these requirement and improvement goals. It is hoped that that this work will not only capture the current state-of-the-art of worldwide H- beam injectors and clarify the research goals and efforts of the community in general but will also encourage further inter laboratory collaborations.

43 PARTICLE ACCELERATORS↗

MAVEN Observation of an Obliquely Propagating Low-Frequency Wave Upstream of Mars

We report Mars Atmosphere and Volatile EvolutioN (MAVEN) mission observations of a large amplitude low-frequency plasma wave that propagated oblique to the ambient magnetic field upstream of Mars along with a non-solar-wind plasma component that had a flow velocity perpendicular to the magnetic field. We consider nine possibilities for this wave that include various combinations of its propagation direction, polarization in the solar wind frame, and ion source responsible for its generation. Using the observed wave parameters and the measured plasma parameters as constraints, we uniquely identify the wave by systematically discarding these possibilities. We determine that the wave is a right-hand polarized wave that propagated upstream in the solar wind frame. We find two possibilities for the ion source that can be responsible for this wave generation. They are either newly born pickup protons or reflected solar wind protons from the bow shock.We determine that the observed non-solar-wind component is not responsible for the wave generation, and it is likely that the non-solar-wind component was merely perturbed by the passage of the wave.

low frequency wave↗

Isotope-ratio-monitoring gas chromatography-mass spectrometry: methods for isotopic calibration

In trial analyses of a series of n-alkanes, precise determinations of 13C contents were based on isotopic standards introduced by five different techniques and results were compared. Specifically, organic-compound standards were coinjected with the analytes and carried through chromatography and combustion with them; or CO2 was supplied from a conventional inlet and mixed with the analyte in the ion source, or CO2 was supplied from an auxiliary mixing volume and transmitted to the source without interruption of the analyte stream. Additionally, two techniques were investigated in which the analyte stream was diverted and CO2 standards were placed on a near-zero background. All methods provided accurate results. Where applicable, methods not involving interruption of the analyte stream provided the highest performance (sigma = 0.00006 at.% 13C or 0.06% for 250 pmol C as CO2 reaching the ion source), but great care was required. Techniques involving diversion of the analyte stream were immune to interference from coeluting sample components and still provided high precision (0.0001 < or = sigma < or = 0.0002 at.% or 0.1 < or = sigma < or = 0.2%).

NASA Discipline Exobiology↗

Data acquisition techniques for exploiting the uniqueness of the time-of-flight mass spectrometer: Application to sampling pulsed gas systems

Mass spectra are produced in most mass spectrometers by sweeping some parameter within the instrument as the sampled gases flow into the ion source. It is evident that any fluctuation in the gas during the sweep (mass scan) of the instrument causes the output spectrum to be skewed in its mass peak intensities. The time of flight mass spectrometer (TOFMS) with its fast, repetitive mode of operation produces spectra without skewing or varying instrument parameters and because all ion species are ejected from the ion source simultaneously, the spectra are inherently not skewed despite rapidly changing gas pressure or composition in the source. Methods of exploiting this feature by utilizing fast digital data acquisition systems, such as transient recorders and signal averagers which are commercially available are described. Applications of this technique are presented including TOFMS sampling of vapors produced by both pulsed and continuous laser heating of materials.

Lincoln, K. A.↗

Mass spectrometer beam system for applications in the stratosphere

A special gas inlet system is required for reduction of high ambient pressures to ion source operating pressures for mass spectrometer investigations in the stratosphere for the determination of the abundance of minor constituents. A system has been designed which combines a mass spectrometer and a gas inlet system reducing pressure by differential pumping using high-speed liquid helium pumps and small orifices. The gas particles are formed into a neutral beam with a flag mechanism proceeding into the mass spectrometer ion source where they are ionized for subsequent mass separation. A laboratory model has been tested under conditions simulating stratospheric pressures. It was shown that the process is able to identify gases with abundances below 10 to the -8th. Some of the problems associated with gas analysis of trace constituents have been alleviated, and other applications of the system have been identified, such as pollution control and medicine.

Mauersberger, K.↗

Laser power density dependence on charge state distribution of Ta ion laser plasma

Laser power density per pulse, which is commonly expressed with the unit of “W/cm2,” is an important parameter to characterize ablation plasma. To match a design charge state of heavy ion beam induced by a laser ion source, a laser power density must be carefully chosen. Above around 108 W/cm2 of laser power density, laser ablation plasma is emitted from the surface of solid material. Then, up to 109 W/cm2, the most abundant charge state is 1+. Because the ionization energy increases with higher charge states, increasing the laser intensity leads to the charge state distribution shifting higher. Increasing the density to increase charge states also results in lower time of flight due to higher velocities. The maximum laser power density is obtained by the smallest available laser spot size on the target material which is determined by the quality of the laser beam. For many accelerator applications, higher charge state beams are preferred. In particular cases, singly charge ion beams are demanded. Therefore, production of intermediate charge state beams has not been investigated well. In this study, we selected Ta4+ as an example demanded beam and tried to clarify how the transition of charge state distribution depends on laser power density. Conclusively, the possible specification of a laser ion source for Ta4+ delivery was elucidated.

Okamura, Masahiro (ORCID:0000000255521706)↗