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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Biaxially strained PtPb/Pt core/shell nanoplate boosts oxygen reduction catalysis

Compressive surface strains have been necessary to boost oxygen reduction reaction (ORR) activity in core/shell M/Pt catalysts (where M can be Ni, Co, Fe). We report a class of PtPb/Pt core/shell nanoplate catalysts that exhibit large biaxial tensile strains. The stable Pt (110) facets of the nanoplates have high ORR specific and mass activities that reach 7.8 milliampere per centimeter square and 4.3 ampere per milligram of platinum at 0.9 volts versus the reversible hydrogen electrode (RHE), respectively. Density functional theory calculations revealed that the edge-­Pt and top (bottom)-Pt (110) facets undergo large tensile strains that help optimize the Pt-­O bond strength. The intermetallic core and uniform 4 layers of Pt shell of the PtPb/Pt nanoplates appear to underlie the high endurance of these catalysts, which can undergo 50,000 voltage cycles with negligible activity decay and no apparent structure and composition changes.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗
DOE OSTI2025

Halide segregation to boost all-solid-state lithium-chalcogen batteries

Mixing electroactive materials, solid-state electrolytes, and conductive carbon to fabricate composite electrodes is the most practiced but least understood process in all-solid-state batteries, which strongly dictates interfacial stability and charge transport. Here, we report on universal halide segregation at interfaces across various halogen-containing solid-state electrolytes and a family of high-energy chalcogen cathodes enabled by mechanochemical reaction during ultrahigh-speed mixing. Bulk and interface characterizations by multimodal synchrotron x-ray probes and cryo–transmission electron microscopy show that the in situ segregated lithium halide interfacial layers substantially boost effective ion transport and suppress the volume change of bulk chalcogen cathodes. Various all-solid-state lithium-chalcogen cells demonstrate utilization close to 100% and extraordinary cycling stability at commercial-level areal capacities.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Nonextensive hydrodynamics of boost-invariant plasmas

We use quasiparticle anisotropic hydrodynamics to study the non-conformal and non-extensive dynamics of a system undergoing boost-invariant Bjorken expansion. To introduce nonextensivity, we use an underlying Tsallis distribution with a time-dependent nonextensivity parameter q. By taking moments of the quasiparticle Boltzmann equation in the relaxation-time approximation, we obtain dynamical equations which allow us to determine the time evolution of all microscopic parameters including q. We compare numerical solutions for bulk observables obtained using the nonextensive evolution with results obtained using quasiparticle anisotropic hydrodynamics with a Boltzmann distribution function (q → 1). We show that the evolution of the temperature, pressure ratio, and scaled energy density, are quite insensitive to which distribution function is assumed. However, we find significant differences in the early-time evolution of the bulk pressure which are observed for even small deviations from the Boltzmann distribution function. Finally, we discuss the existence of non-conformal hydrodynamic attractors for the longitudinal and transverse pressures, the bulk and shear viscous corrections, and the nonextensivity parameter q.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Measurement of the differential $\hbox {t}\overline{\hbox {t}}$ production cross section as a function of the jet mass and extraction of the top quark mass in hadronic decays of boosted top quarks

A measurement of the jet mass distribution in hadronic decays of Lorentz-boosted top quarks is presented. The measurement is performed in the lepton + jets channel of top quark pair production ($\hbox {t}\overline{\hbox {t}}$) events, where the lepton is an electron or muon. The products of the hadronic top quark decay are reconstructed using a single large-radius jet with transverse momentum greater than 400 GeV. The data were collected with the CMS detector at the LHC in proton-proton collisions and correspond to an integrated luminosity of 138 fb -1 . The differential $\hbox {t}\overline{\hbox {t}}$ production cross section as a function of the jet mass is unfolded to the particle level and is used to extract the top quark mass. The jet mass scale is calibrated using the hadronic W boson decay within the large-radius jet. The uncertainties in the modelling of the final state radiation are reduced by studying angular correlations in the jet substructure. These developments lead to a significant increase in precision, and a top quark mass of 173.06 ± 0.84 GeV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

CFD modeling of pre-spark heat release in a boosted direct-injection spark-ignition engine

Accurate predictions of low-temperature heat release (LTHR) are critical for modeling auto-ignition processes in internal combustion engines. While LTHR is typically obscured by deflagration, extremely late ignition phasing can lead to LTHR prior to the spark, a behavior known as pre-spark heat release (PSHR). In this research, PSHR in a boosted direct-injection spark-ignition engine was studied using 3-D computational fluid dynamics (CFD) and detailed chemical kinetics. The turbulent combustion was modeled via a hybrid approach that incorporates the G-equation model for tracking the turbulent flame front, and the well-stirred reactor model with detailed chemistry for assessing the low-temperature reactions in unburnt gas. Simulations were conducted using Co-Optima alkylate and E30 fuels at operating conditions characterized by different PSHR intensities. The predicted in-cylinder pressure and heat release rate were found to agree well with experiments. It was found the estimate of previous-cycle trapped residuals is of utmost importance for capturing PSHR correctly. A simulation best practice was developed which keeps the detailed chemistry solver active throughout the entire simulation, allowing to track the evolution of intermediate species from one cycle to the next. Following the validation, the dynamics of PSHR were analyzed in detail employing the pressure-temperature (P-T) trajectory framework. It was shown that PSHR correlated with the first-stage ignition delay of the fuel, hence showing close relation to the in-cylinder P-T trajectory and the chemical kinetics. Besides, it was indicated that LTHR is a self-limiting process that has the effect of attenuating the thermal stratification in the combustion chamber. Furthermore, it was observed the occurrence of PSHR caused the P-T trajectory of end-gas to overlap with the negative temperature coefficient region of the fuel’s ignition-delay maps. This effect was more significant in the fuel-rich regions where engine knock tendency would be generally higher, with potential implications on knock control and mitigation.

42 ENGINEERING↗
DOE OSTI2019

Redefining Eligibility by Analyzing Canceled Intraoperative Radiotherapy as a Boost for Patients Undergoing Breast-Conserving Treatment

Background: Intraoperative radiotherapy (IORT) with a 50-kV x-ray is used for a tumor bed boost during breast-conserving surgery. This study evaluated the anatomicosurgical factors associated with cancellation of planned IORT. Methods: Patient eligibility for the study included age of 20 years or older, compatibility for lumpectomy, and ductal carcinoma in situ or stages 1–3 invasive carcinoma. All the patients underwent magnetic resonance imaging (MRI) and multidisciplinary team evaluations. Resection margins were assessed by frozen pathology. Pre- and intraoperative variables were compared between the IORT and IORT-cancellation groups. Results: A total of 434 patients underwent surgeries for IORT between August 2014 and December 2017. For 90 of these patients, IORT was canceled because of repeated positive margins leading to a large cavity or total mastectomy (n = 27), insufficient cavity-skin distance (n = 14), satellite lesions leading to a large cavity or total mastectomy (n = 12), MRI findings of a large primary tumor or uncertain margins leading to a large cavity (n = 6), cavity geometry unsuitable for IORT (n = 6), subareolar tumor extension (n = 6), tumor abutting the pectoralis muscle (n = 3), patient refusal (n = 5), intraoperative confirmation of bilateral breast cancer (n = 3) or benign pathology (n = 3), device malfunction (n = 3), or scheduling difficulty (n = 2). A tumor larger than 2 cm (P = 0.014) and the presence of satellite lesions (P = 0.014) were independent predictors of IORT cancellation. Conclusions: Surgical procedures resulting in large cavities were the leading cause of IORT cancellation. Multidisciplinary evaluations using MRI were critical for completion of IORT procedures.

62 RADIOLOGY AND NUCLEAR MEDICINE↗
DOE OSTI2021

Engineering well-expressed, V2-immunofocusing HIV-1 envelope glycoprotein membrane trimers for use in heterologous prime-boost vaccine regimens

HIV-1 vaccine immunofocusing strategies may be able to induce broadly-reactive neutralizing antibodies (NAbs). Here, we engineered a panel of diverse, membrane-resident native HIV-1 trimers vulnerable to two broad targets—the V2 apex and fusion peptide (FP). Selection criteria included i) high expression and ii) infectious function, so that trimer neutralization sensitivity can be profiled in pseudovirus (PV) assays. Initially, we boosted the expression of 17 candidate trimers by truncating gp41 and introducing a gp120-gp41 SOS disulfide to prevent gp120 shedding. "Repairs" were made to fill glycan holes and eliminate other strain-specific aberrations. A new neutralization assay allowed PV infection when our standard assay was insufficient. Trimers with exposed V3 loops, a target of non-NAbs, were discarded. To try to increase V2-sensitivity, we removed clashing glycans and modified the C-strand. Notably, a D167N mutation improved V2-sensitivity in several cases. Glycopeptide analysis of JR-FL trimers revealed near complete sequon occupation and that filling the N197 glycan hole was well-tolerated. In contrast, sequon optimization and inserting/removing glycans at other positions frequently had global "ripple" effects on glycan maturation and sequon occupation throughout the gp120 outer domain and gp41. V2 MAb CH01 selectively bound to trimers with small high mannose glycans near the base of the V1 loop, thereby avoiding clashes. Knocking in a rare N49 glycan was found to perturb gp41 glycans, increasing FP NAb sensitivity—and sometimes improving expression. Finally, a biophysical analysis of VLPs revealed that i) ~25% of particles bear Env spikes, ii) spontaneous particle budding is high and only increases 4-fold upon Gag transfection, and iii) Env+ particles express ~30–40 spikes. Taken together, we identified 7 diverse trimers with a range of sensitivities to two targets to allow rigorous testing of immunofocusing vaccine concepts.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2017

Boosting the Search for New Physics at the Frontiers

This is the final report for the DOE grant "Boosting the Search for New Physics at the Frontiers" from Prof. Jesse Thaler at MIT. During the grant period, Thaler’s research group made substantial contributions to research in theoretical high energy physics. The three categories of research proposed and funded by this DOE grant are: Jet Substructure, Novel Dark Matter Dynamics, and Supersymmetry Breaking. Descriptions of the research carried out during the 8.5 month funding period are provided below. The present affiliations of Thaler’s collaborators are provided in the research descriptions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Corrosion Potential of Selected Bio-blendstock Fuel Candidates for Boosted Spark Ignited Engines

Eight bio-blendstock fuel candidates for boosted spark ignited engines were evaluated for their susceptibility to corrode infrastructure metals. These candidates included five alcohols (methanol, ethanol, isobutanol, n-propanol, and isopropanol), diisobutylene, mixed furans, and aromatics. Methanol was also added to the list for comparison. These molecules are not corrosive to metals since they cannot dissociate into ions and anions. However, the addition of contaminants and a separate water phase may facilitate corrosion due to phenomena associated with the formation of ions and anions (from key contaminants), differential aeration cell (due to dissolved oxygen), and microbial-induced corrosion. A literature review was conducted to determine the influence of these phenomena on corrosion for the nine fuel candidates. In addition, the oxygen solubility of each fuel type was determined to ascertain their relative influence on forming and enhancing a differential aeration cell. Of the fuel candidates, only the alcohols are water soluble, and therefore have an opportunity to cause corrosion. However, differential aeration cells, by themselves have not been shown to contribute to corrosion. Other factors, such as galvanic coupling and/or crevice regions are necessary to promote corrosion in laboratory conditions. However, differential aeration as a corrosion mechanism has not been established in the field. Likewise, microbial-induced corrosion is another known corrosion pathway that has yet to be positively identified for blends of the fuel candidates with gasoline. In summary, corrosion is not anticipated with any of the bio-blendstock candidates with infrastructure metals.

09 BIOMASS FUELS↗
DOE OSTI2018

Gathering and boosting acid gas removal (AGR)

Acid gas removal (AGR) at natural gas gathering and boosting facilities. To access the model referenced in the report, please visit https://www.netl.doe.gov/energy-analysis/details?id=EDAE31FF-B0EB-4F7E-82D8-D8692E16B733

03 NATURAL GAS↗
DOE OSTI2018

Gathering and boosting centrifugal compression venting

Gathering and boosting centrifugal compression venting (not including venting from compressor driver). To access the model referenced in the report, please visit https://www.netl.doe.gov/energy-analysis/details?id=6610B516-DDE9-4BC7-945C-5FDD22B0FB26

42 ENGINEERING↗
DOE OSTI2018

Gathering and boosting flaring

Flaring of natural gas at natural gas gathering and boosting facilities. To access the model referenced in the report, please visit https://www.netl.doe.gov/energy-analysis/details?id=C525676C-5246-4B1F-B693-4395051858E5

03 NATURAL GAS↗
DOE OSTI2021

Renewable Octane Hyper boosting Blendstock for High-Efficiency (CRADA 494)

The goal of this project is to scale up the chemistry developed by Visolis to produce a high energy-density fuel blend stock mixture from fermentation derived intermediate. Fuel property measurements will be conducted on the initial mixture to guide process refinement to produce a blend stock mixture that has the optimum composition and combustion properties to boost the octane rating of the finished fuels.

09 BIOMASS FUELS↗
DOE OSTI2024

Next Gen High Efficiency Boosted Engine Development

This work represents an advanced engineering research project partially funded by the U.S. Department of Energy (DOE). Ford Motor Company, FEV North America, and Oak Ridge National Laboratory collaborated to develop a next generation boosted spark ignited engine concept. The project goals, specified by the DOE, were 23% improved fuel economy and 15% reduced weight relative to a 2015 or newer light-duty vehicle. The fuel economy goal was achieved by designing an engine incorporating high geometric compression ratio, high dilution tolerance, low pumping work, and low friction. The increased tendency for knock with high compression ratio was addressed using early intake valve closing (EIVC), cooled exhaust gas recirculation (EGR), an active pre-chamber ignition system, and careful management of the fresh charge temperature. Engine weight reduction measures were implemented throughout the engine system making use of composite materials, advanced manufacturing techniques, and architectural choices. This report outlines the analytical, design, fabrication, and test work conducted for the duration of the project. The combustion system stability, EGR tolerance, and knock resistance were validated on a single cylinder engine. An inline six-cylinder engine was then designed targeting application in the Ford F150. Multi-cylinder engines were produced and tested achieving the target vehicle fuel economy improvement of 23% assessed using measured engine fuel consumption combined with a vehicle drive cycle simulation. Actions were identified and designs were demonstrated to achieve the 15% weight reduction target. This project included items covering a range of technology readiness levels. Some of the technologies explored are production ready, while others were investigated to understand the limitations for what can be achieved in a stoichiometric, gasoline-fueled, spark-ignited internal combustion engine.

42 ENGINEERING↗
DOE OSTI2026

Boosting CO2R Performance of Ag Electrocatalysts by Sulfur-Doped Carbon Support

We find that S-doped carbon support can boost the CO2 reduction (CO2R) performance of Ag electrocatalysts. Firstly, surface science enabled electrocatalysis showed that Ag supported on S-doped highly oriented pyrolytic graphite (HOPG), a model electrocatalyst, demonstrated 100% higher CO turnover frequency (TOFCO = 3.6 ± 0.2 CO/atomAg/s) than that supported on S-free HOPG (TOFCO = 1.8 ± 0.2 CO/atomAg/s). Computational modeling based on density functional theory (DFT) revealed a more stabilized *COOH intermediate on Ag supported on S-doped carbon and thus a more favorable energetic pathway of CO2-to-CO, consistent with experimental results from the model electrocatalysts studies. Finally, this proof of concept was translated to the synthesis of powder electrocatalyst with 2 wt% Ag supported on S-doped carbon black, demonstrating > 40-fold high CO mass activity than a commercial Ag cathode with steady FECO ~ 96% at 100 mA/cm2 for 50 hours of continuous operation in a gas diffusion electrode (GDE) electrolyzer. For comparison, 2 wt% Ag supported on carbon black without S- doping showed a maximum FECO ~ 70% at 100 mA/cm2. This work demonstrates a successful bottom-up design of CO2R electrocatalysts guided by surface science enabled electrocatalysis.

CO2 conversion↗
DOE OSTI2026

Search for New Physics via EFT in collisions containing a top quark and a boosted Z or Higgs boson

We present a generator-level sensitivity study of physics beyond the Standard Model within the framework of Effective Field Theory (EFT). The targeted signal processes are single top quark production in association with a Lorentz-boosted Higgs or Z boson (tHq and tZq) in proton-proton collisions at a center-of-mass energy of 13.6 TeV. Event selection requires one electron or muon, a high-transverse-momentum, large-radius (AK8) jet reconstructing hadronic H → b̄b or Z → b̄b decays, at least two distinct, non-overlapping small-radius (AK4) jets with one originating from a b quark, and a missing transverse energy greater than 30 GeV. Signal and background samples are generated via Monte Carlo simulation using MadGraph with MadJax to perform EFT matrix-element calculations. Deviations from the Standard Model are parametrized through dimension-six EFT operators that probe modified top quark interactions. This generator-level study identifies kinematic observables with enhanced sensitivity to EFT operators and motivates future reconstruction-level analyses of tHq and tZq channels.

Meshramkar, Daniel [Baylor U., Waco]↗
DOE OSTI2026

Search for New Physics via EFT in collisions containing a top quark and a boosted Z or Higgs boson

We present a generator-level sensitivity study of physics beyond the Standard Model within the framework of Effective Field Theory (EFT). The targeted signal processes are single top quark production in association with a Lorentz-boosted Higgs or Z boson (tHq and tZq) in proton-proton collisions at a center-of-mass energy of 13.6 TeV. Event selection requires one electron or muon, a high-transverse-momentum, large-radius (AK8) jet reconstructing hadronic H → b̄b or Z → b̄b decays, at least two distinct, non-overlapping small-radius (AK4) jets with one originating from a b quark, and a missing transverse energy greater than 30 GeV. Signal and background samples are generated via Monte Carlo simulation using MadGraph with MadJax to perform EFT matrix-element calculations. Deviations from the Standard Model are parametrized through dimension-six EFT operators that probe modified top quark interactions. This generator-level study identifies kinematic observables with enhanced sensitivity to EFT operators and motivates future reconstruction-level analyses of tHq and tZq channels.

Meshramkar, Daniel [Baylor U., Waco]↗