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At least 289 records · Page 16

Compilation and Evaluation of Beta-Delayed Neutron Emission Probabilities and Half-Lives for Z > 28 Precursors

We present a compilation and evaluation of experimental β-delayed neutron emission probabilities (P n ) and half-lives (T 1/2 ) for known or potential β-delayed neutron precursors with atomic number Z >28 ( 73 Cu – 233 Fr). This article includes the recommended values of both of these quantities, together with a compilation of experimental measurements when available. Some notable cases, as well as proposed standards forβ-delayed neutron measurements are also discussed. Evaluated data has also been compared to systematics using three different approaches.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Beta-delayed gamma spectra compilation and analysis following the thermal-neutron induced fission of 235 U, 239,241 Pu

The integral gamma and electron spectra emitted by fission products, also known as delayed gamma and electron spectra, were measured at Oak Ridge National Laboratory in the 1970s for the thermal-neutron induced fission of 235 U and 239,241 Pu. Scintillator detectors were used to measure these spectra, data used later on to obtain decay heat values - that is, the spectra mean values per unit time as function of time - work that was published in the Nuclear Science and Technology journal; the spectral data, however, was only published in laboratory reports. Here, in this work, we analyze the gamma spectra data using modern methods and nuclear databases to reveal the signature of individual fission products as well as to gauge the performance of the ENDF/B-VIII.0 decay data sub-library, concluding about possible future enhancements in predictive capabilities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Vascular endothelial growth factor receptor-1 (FLT1) interactions with amyloid-beta in Alzheimer’s disease: A putative biomarker of amyloid-induced vascular damage

We have identified FLT1 as a protein that changes during Alzheimer's disease (AD) whereby higher brain protein levels are associated with more amyloid, more tau, and faster longitudinal cognitive decline. Given FLT1's role in angiogenesis and immune activation, we hypothesized that FLT1 is upregulated in response to amyloid pathology, driving a vascular-immune cascade resulting in neurodegeneration and cognitive decline. We sought to determine (1) if in vivo FLT1 levels (CSF and plasma) associate with biomarkers of AD neuropathology or differ between diagnostic staging in an aged cohort enriched for early disease, and (2) whether FLT1 expression interacts with amyloid on downstream outcomes, such as phosphorylated tau levels and cognitive performance. Additionally, we sought to replicate FLT1 interactions in the brain. The results showed that higher levels of FLT1 in CSF and post-mortem brain tissue related to increased tau, particularly among amyloid positive individuals. These analyses help clarify the potential utility of FLT1 as a biomarker among individuals with evidence of brain amyloidosis.

60 APPLIED LIFE SCIENCES↗

Electropolishing parameters study for surface smoothening of low-$\beta$650 MHz five-cell niobium superconducting radio frequency cavity

Electropolishing (EP) is applied to niobium (Nb) superconducting radio frequency (SRF) cavities, which are used in particle accelerators for their surface treatment. The EP process for 1.3 GHz cavities has been extensively studied earlier. In this work, a parametric study on EP of low-β (0.61) 650 MHz Nb SRF cavities (LB650), which will be used in pre-production cryomodule for proton improvement plan-II (PIP-II) linear accelerator, was conducted to determine adequate EP conditions for attaining a smooth surface of the cavities. EP performed with the standard parameters and an initial cathode (cathode-I) having a cathode surface area of ~5% of the cavity surface area yielded a rough equator surface of the cavity. The grain step height on the equator weld position was measured to be ~ 32 μm. The rough surface was attributed to preferential grain etching confirmed by a polarization curve showing a linear relationship between the EP current and voltage and the absence of the current plateau region. The cathode was modified to make its surface area twice that of cathode-I. The modified cathode (cathode-M) provided a current plateau region in the corresponding I-V curves measured at different cavity temperatures. The onset voltage for the plateau was found to be higher at higher cavity temperatures. Here this study revealed that even with cathode-M, the standard 18 V was low for EP of such large-sized cavities when the cavity temperature was 18 °C. EP performed at a higher voltage of 22–24.5 V with cathode-M yielded a smooth surface with a grain step height of only 0.6 μm. The applied EP conditions also improved removal uniformity along the cavity length. In contrast to the cavity treated with cathode-I, the cavities treated with cathode-M achieved a significantly higher accelerating gradient (E acc ) in vertical tests conducted in a cryostat at 2 K. The modified EP was found efficient to produce the cavities that achieved E acc of 22.4 MV/m, required by PIP II project in the baseline RF tests, to qualify for further surface processing used to enhance their quality factors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Integration of high confinement, high poloidal beta plasma with dual radiated power and detachment controls for divertor protection and ELM suppression

Divertor detachment without serious core confinement quality loss in DIII-D’s high poloidal β scenario has been combined with impurity-induced ELM mitigation without disruption. Use of Ne previously granted access to a detached, non-ELMing regime that retained high confinement quality due to stimulation of Internal Transport Barrier (ITB) growth, but suffered from on-going core fuel dilution and high disruptivity. Excess Ne accumulation in the core plasma has now been avoided by feeding back core radiated power ($P_{rad}$) measurements to control Ne seeding, rather than using attachment fraction ($A_{frac}$) control with Ne; this also reduces disruptivity. At the same time, N 2 seeding is used in a feedback loop with $A_{frac}$ measurements, which previously posed low disruption risk. In this way, the effect of Ne in the core is managed while avoiding excess seeding, and N 2 acts to correct for any excess heat exhaust that might interfere with detachment. The average Ne flow rate was 38% of what was used in pure Ne $A_{frac}$ control, plus average N 2 flow that was 43% of pure N 2 $A_{frac}$ control, even while meeting an even deeper detachment target. Meanwhile, a steep pressure gradient in the core plasma reduces sensitivity to impurity-induced degradation of the pedestal and reasonable confinement quality was maintained despite operational challenges that blocked formation of an ITB in these experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Beta decay of the axially asymmetric ground state of 192 Re

The β decay of 192 75 Re 117 , which lies near the boundary between the regions of predicted prolate and oblate deformations, has been investigated using the KEK Isotope Separation System (KISS) in RIKEN Nishina Center. This is the first case in which a low-energy beam of rhenium isotope has been successfully extracted from an argon gas-stopping cell using a laser-ionization technique, following production via multi-nucleon transfer between heavy ions. The ground state of 192 Re has been assigned J π = (0⁻) based on the observed β feedings and deduced logft values towards the 0⁺ and 2⁺ states in 192 Os, which is known as a typical γ-soft nucleus. Furthermore, the shape transition from axial symmetry to axial asymmetry in the Re isotopes is discussed from the viewpoint of single-particle structure using the nuclear Skyrme-Hartree-Fock model.

192Re↗

Insights on keto-hydroperoxide formation from O 2 addition to the beta-tetrahydrofuran radical

Cyclic ethers provide an interesting case study of low-temperature oxidation chemistry, especially in relevance to biofuels. A recent experimental study revealed new questions regarding the low-temperature oxidation mechanism of tetrahydrofuran (THF) concerning the formation of keto-hydroperoxides. In particular, keto-hydroperoxides originating from the THF-β radical were not captured accurately by current literature models, motivating this work to calculate the energetics of the first and second O 2 -addition pathways for THF radicals. Electronic structure calculations at the CCSD(T)/cc-pV∞Z//M06-2X/cc-pVTZ level of theory were used to generate potential energy surfaces for the α-C and β-C THF radicals and subsequent pathways to the formation of the keto-hydroperoxide isomers. These are the first theoretical calculations of the second O 2 -addition radical pathways for the THF-β radical. Results from the theorical work provided further insight into the low-temperature oxidation of THF. This included identifying the pathways most likely to form the keto-hydroperoxide isomers observed in prior experimental work; and detecting that the shortcomings in prior models are likely due to uncertainties in R + THF abstraction reaction rates. Here, these conclusions will motivate future work for accurate THF kinetic model development.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗