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At least 289 records · Page 16

Opportunities for gas-phase science at short-wavelength free-electron lasers with undulator-based polarization control

Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin-orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology, and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines. Published by the American Physical Society 2025

Ilchen, Markus↗

Beyond single tetrahedron physics of the breathing pyrochlore compound Ba 3 ⁢Yb 2 ⁢Zn 5 ⁢O 11

Recently, a new class of quantum magnets, the so-called breathing pyrochlore spin systems, have attracted much attention due to their potential to host exotic emergent phenomena. Here, we present magnetometry, heat capacity, thermal conductivity, muon-spin relaxation, and polarized inelastic neutron scattering measurements performed on high-quality single crystal samples of the breathing pyrochlore compound Ba 3 ⁢Yb 2 ⁢Zn 5 ⁢O 11 . We interpret these results using a simplified toy model and provide insight into the low-energy physics of this system beyond the single tetrahedron physics proposed previously.

36 MATERIALS SCIENCE↗

Ethylene line emission from the North Pole of Jupiter

A significant enhancement in infrared emission from hydrocarbon constituents of Jupiter's stratosphere was observed at a north polar hot spot (60 degrees latitude, 180 degrees longitude). A unique probe of this phenomena is ethylene (C2H4), which has not been observed previously from the ground. The profile of the emission line from ethylene at 951.742 cm-1, measured near the north pole of Jupiter, was analyzed to determine the morphology of the enhancement, the increase in C2H4 abundance and local temperature, as well as possible information on the altitude (pressure regions) where the increased emission is formed. Measurements were made using infrared heterodyne spectroscopy at the NASA Infrared Telescope Facility on Mauna Kea, Hawaii in December 1989. At 181 degrees longitude a very strong emission line was seen, which corresponds to a 13-fold increase in C2H4 abundance or a 115K increase in temperature in the upper stratosphere, compared to values outside the hot spot. The hot spot was found to be localized to approx. 10 degrees in longitude; the line shape (width) implied that the enhanced emission originated very high in the stratosphere.

Kostiuk, Theodor↗

Using OSSEs to Evaluate the Impacts of Geostationary Infrared Sounders

An observing system simulation experiment (OSSE) was performed to assess the impact of assimilating hyperspectral infrared (IR) radiances from geostationary orbit on numerical weather prediction, with a focus on the proposed sounder on board the Geostationary Extended Observations (GeoXO) program’s central satellite. Infrared sounders on a geostationary platform would fill several gaps left by IR sounders on polar-orbiting satellites, and the increased temporal resolution would allow the observation of weather phenomena evolution. The framework for this OSSE was the Global Modeling and Assimilation Office (GMAO) OSSE system, which includes a full suite of meteorological observations. The experiment additionally assimilated four identical IR sounders from geostationary orbit to create a “ring” of vertical profiling observations. Based on the experimentation, assimilation of the IR sounders provided a beneficial impact on the analyzed mass and wind fields, particularly in the tropics, and produced an error reduction in the initial 24–48 h of the subsequent forecasts. Specific attention was paid to the impact of the GeoXO Sounder (GXS) over the contiguous United States (CONUS) as this is a region that is well-observed and as such difficult to improve. The forecast sensitivity to observation impact (FSOI) metric, computed across all four synoptic times over the CONUS, reveals that the GXS had the largest impact on the 24-h forecast error of the assimilated hyperspectral infrared satellite radiances as measured using a moist energy error norm. Based on this analysis, the proposed GXS has the potential to improve numerical weather prediction globally and over the CONUS.

OSSE↗

Strong electron-phonon coupling driven pseudogap modulation and density-wave fluctuations in a correlated polar metal

Abstract There is tremendous interest in employing collective excitations of the lattice, spin, charge, and orbitals to tune strongly correlated electronic phenomena. We report such an effect in a ruthenate, Ca 3 Ru 2 O 7 , where two phonons with strong electron-phonon coupling modulate the electronic pseudogap as well as mediate charge and spin density wave fluctuations. Combining temperature-dependent Raman spectroscopy with density functional theory reveals two phonons, B 2 P and B 2 M , that are strongly coupled to electrons and whose scattering intensities respectively dominate in the pseudogap versus the metallic phases. The B 2 P squeezes the octahedra along the out of plane c -axis, while the B 2 M elongates it, thus modulating the Ru 4d orbital splitting and the bandwidth of the in-plane electron hopping; Thus, B 2 P opens the pseudogap, while B 2 M closes it. Moreover, the B 2 phonons mediate incoherent charge and spin density wave fluctuations, as evidenced by changes in the background electronic Raman scattering that exhibit unique symmetry signatures. The polar order breaks inversion symmetry, enabling infrared activity of these phonons, paving the way for coherent light-driven control of electronic transport.

36 MATERIALS SCIENCE↗

Large-scale negative polarity magnetic fields on the sun and particle-emitting flares

Some observational facts about the large-scale patterns formed by solar negative polarity magnetic fields during the 19th and 20th cycles of solar activity are presented. The close relation of the position of occurrence of very large flares accompanied by cosmic ray and PCA events as well as other phenomena of solar activity during the declining part of the 19th cycle of the regularities in the internal structure of large scale negative polarity features are demonstrated.

Bumba, V.↗

Remote sensing of plasma injection and acceleration phenomena

Dynamics Explorer-1 High Altitude Plasma Instrument data have been used to investigate the injection of magnetosheath plasma into the polar cusp, the injection of auroral ion beams into the magnetosphere, and the acceleration of electrons transverse to the magnetic field direction, and the results are discussed. In the case of polar cusp plasmas, it is found that injection occurs at the high-latitude magnetopause, at geocentric distances near eight earth radii. In the case of auroral ion beams it is determined that ion bands are not produced by equatorial injection from the plasma sheet, but by the upward acceleration of ions from auroral acceleration regions. Finally, conical electron distributions are found to be consistent with transverse acceleration at altitudes of a thousand or more km, within or below the magnetic-field-aligned potential drops of the auroral acceleration regions.

Burch, J. L.↗

Observed relationships between electric fields and auroral particle precipitation

Simultaneous electric field and plasma observations with the low altitude, polar orbiting satellite Injun (Hawkeye) 5 provided a comprehensive survey of convection electric fields and their association with magnetospheric plasma phenomena. The most prominent features of the convection electric fields are reversals located at high magnetic latitudes, with generally anti sunward convection poleward convection equatorward of the electric field reversal location. The electric field reversal is interpreted as the boundary between open and closed magnetic field lines. To investigate the electric field and plasma interrelationships during a polar magnetic substorm, a series of passes obtained prior to and during a substrom is presented. Large, anti sunward convection velocities were detected over the polar cap several tens of minutes before the onset of the expansive phase of the substrom. These convection velocities gradually decreased during the decay phase of the substrom. Measurements of enhanced anti sunward flow over the polar cap region are generally consistent with concepts of the origin of substroms.

Gurnett, D. A.↗

Environmental and Polarization Characterizations of E-Beam Plasma-Based AlF 3 -Passivated Aluminum Mirrors for Astronomical Telescopes

Astronomical space telescopes to study astrophysical phenomena from the far ultraviolet (FUV) to the near infrared (NIR) will require mirror coatings with high reflectance over this entire spectral region. While coatings for the optical and NIR part of the spectrum are fairly well developed with proven performance, the FUV range has presented significant challenges, particularly below 120nm. Recent developments in electron-beam (e-Beam) generated plasma treatment in a SF 6 environments has enabled the effective passivation of aluminum (Al) coatings for applications in the FUV, by native oxide removal and the formation of a AlF 3 passivation layer which could be tuned to any desired AlF 3 thickness. These results have been produced through a collaboration between the Goddard Space Flight Center (GSFC) and the Naval Research Laboratory (NRL). The passivation experiments have been carried out using the Large Area Plasma Processing System (LAPPS) at NRL using bare aluminum samples and provided by the coating group at GSFC. This novel procedure has demonstrated improved Al mirrors with state-of-the-art FUV reflectivity (e.g. R=91% at 121.6nm). In this paper, we will be reporting on environmental testing, micro-roughness, as well as polarization studies of these E-beam treated samples. These characterizations are being done in order to advance the Technology Readiness Level (TRL) for these Al+AlF 3 mirror coatings produced at LAPPS. The ultimate goal is to demonstrate the promise of using this coating technology to deliver reflectance performance plus stability and uniformity over a large area for a future IR/O/UV space telescope observatory.

FUV reflectance↗

Evidence from the limb infrared monitor of the stratosphere for nonlocal thermodynamic equilibrium in the nu2 mode of mesospheric water vapour and the nu3 mode of stratospheric nitrogen dioxide

Data from the 6.9-micron H2O channel and the 6.2-micron NO2 channel of the Nimbus 7 Limb Infrared Monitor of the Stratosphere (LIMS) have been used to investigate the daytime enhancement to H2O; the high concentration of H2O sometimes observed in the polar night mesosphere; and the high ratio of daytime to nighttime NO2 in the upper stratosphere. These three phenomena deviate noticeably from the predictions of photochemical theory. The 20 to 30 percent diurnal variation in stratospheric H2O apparent in LIMS data cannot be reconciled with a photochemical lifetime in excess of four months. This is attributed to departure from local thermodynamic equilibrium of daytime emission which had not been accounted for in retrievals. Speculative possibilities of NLTE emission from the H2O nu2 and NO2 nu3 hot bands are discussed. It is found that the nonthermal emission from NO2 significantly affects retrieval of H2O in the polar nighttime and NO2 in the daytime stratosphere at low latitudes.

Kerridge, Brian J.↗

Chirality, vorticity and spin polarization — Experimental overview

In this paper, we provide an exploration of the interrelated topics of chirality, vorticity, and spin polarization in relativistic heavy ion collisions. Our discussion delves into the intricate relationships among these phenomena, examining the recent measurements conducted at both RHIC and LHC. We review the challenges faced, the progress made, and the current state of understanding regarding hot QCD matter under rotation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dilute magnetic impurity-induced effective phonon magnetic moment in Fe-doped monolayer MoS 2

Realization of large effective phonon magnetic moment in monolayer MoS 2 has established an important route for exploring intriguing magnetic phenomena in a nonmagnetic material. The sizable coupling between the orbital transition and the circularly polarized phonon results in the large effective phonon magnetic moment. In this work, using magneto-Raman spectroscopy, we investigate substitutional doping of magnetic atoms as a tuning knob of the electronic and phononic properties of MoS 2 . We show that Fe-doping polarizes the spin of the conduction bands and introduces a localized Fe band underneath the conduction band. As a result, an additional orbital transition between the Mo 4d and Fe 3d states emerges, producing an orbital-phonon hybridized mode at 283 cm −1 . Our magnetic field dependent measurements demonstrate that this new mode carries 2.8 $\mu_{\mathrm{B}}$ effective phonon magnetic moment, which is comparable to that of the undoped MoS 2 . Moreover, even though a long-range magnetic order is absent in Fe-doped MoS 2 , the local magnetic moment of Fe modifies the nature of the spin fluctuation, producing monotonically increasing quasielastic scattering spectral weight as temperature decreases. Our results highlight two-dimensional dilute magnetic semiconductors synthesized by substitutional doping as a promising material platform to manipulate the phonon magnetic moment through orbital-phonon coupling.

36 MATERIALS SCIENCE↗

Grad E x B effects on heavy ions in the magnetosphere

Following a theory briefing on the currents in a plasma of mixed species caused by the motion of charged particles, the paper presents a report on the observations of regions of the magnetosphere in which significant values of grad E (E being the electric field) can be inferred from measurements of E made on board the IMP 6 satellite using two pairs of long (91.5 m and 45.7 m) unfurlable antenna sensors. Electric fields were measured by applying double floating probe techniques to the antenna sensors, and grad E values of up to 1.4/1000 emu were inferred from the fluctuations in E along the orbit. The critical values of grad E for various ions, in a range of magnetic fields are compared, and the difference in the behavior of Ba+ ions which cause Ba+ currents in the subcritical and supercritical regions is discussed. The results show that the electric currents flowing in the E x B direction may cause secondary polarization fields on the barium cloud. The possible significance of these effects to natural geophysical phenomena is also pointed out.

Cole, K. D.↗

The ISPM unified radio and plasma wave experiment

Hardware for the International Solar Polar Mission (ISPM) Unified Radio and Plasma (URAP) wave experiment is presented. The URAP determines direction and polarization of distant radio sources for remote sensing of the heliosphere, and studies local wave phenomena which determine the transport coefficients of the ambient plasma. Electric and magnetic field antennas and preamplifiers; the electromagnetic compatibility plan and grounding; radio astronomy and plasma frequency receivers; a fast Fourier transformation data processing unit waveform analyzer; dc voltage measurements; a fast envelope sampler for the solar wind, and plasmas near Jupiter; a sounder; and a power converter are described.

Stone, R. G.↗

Very large array observations of Jupiter's nonthermal radiation

The VLA has been used at 18 and 20 cm to obtain observational data on Jupiter at all rotational aspects in all four Stokes parameters, yielding maps of the total, linearly polarized and circularly polarized intensity with a resolution of 0.25 Jupiter radii. These maps reveal such previously undetected phenomena as an emission feature close to the planetary surface north and south of each of the two main radiation peaks. The emission from 1.8 to about 3 Jupiter radii from the planet's center is sharply confined to the magnetic equator.

De Pater, I.↗

Book Review: Encyclopedia of Astronomy and Astrophysics

This massive reference work (hereafter EAA) summarizes a great deal of what we knew in the astronomical sciences at the most recent Millennium. An associated website may keep much of it up-to-date for years to come. The contents are extensive indeed: the index alone consists of 76 pages, each with three columns of fine-type listings, and there are 'nearly 700 main articles'. The main articles are what make EAA worthwhile. They are generally by experts, who took much care in their preparation. The degree to which the articles are illustrated and referenced, however, seems to depend on the inclination of the individual author. On the other hand, articles on Saturn's rings and on its satellites are heavily illustrated, but with just two or three citations in each. The coverage of solar physics is especially thorough in EAA. There are numerous articles on major topics, notably in the physics and phenomena of the corona and the chromosphere, and some on more specialized areas, such as 'Polar Plumes' and 'Coronal Cavities.'

Maran, Stephen Paul↗

Permutable SOS (symmetry operational similarity)

Abstract Based on symmetry consideration, quasi-one-dimensional (1D) objects, relevant to numerous observables or phenomena, can be classified into eight different types. We provide various examples of each 1D type and discuss their symmetry operational similarity (SOS) relationships, which are often permutable. A number of recent experimental observations, including current-induced magnetization in polar or chiral conductors, non-linear Hall effect in polar conductors, spin-polarization of tunneling current to chiral conductors, and ferro-rotational domain imaging with linear gyration are discussed in terms of (permutable) SOS. In addition, based on (permutable) SOS, we predict a large number of new phenomena in low symmetry materials that can be experimentally verified in the future.

Materials Science↗

Observed relationships between electric fields and auroral particle precipitation.

Simultaneous electric field and plasma observations with the low-altitude polar-orbiting satellite Injun 5 have provided a comprehensive survey of convection electric fields and their association with magnetospheric plasma phenomena. The most prominent features of the convection electric fields are reversals located at high magnetic latitudes, with generally antisunward convection poleward and sunward convection equatorward of the electric field reversal location. The electric field reversal is interpreted as the boundary between open and closed magnetic field lines. During local day the electric field reversal is observed to coincide with the equatorward boundary of the polar cusp. The plasma flow in the dayside polar cusp region is dominantly E-W, away from the stagnation point, the convection velocities typically being about 1 km/sec. At local evening, 'inverted V' electron precipitation bands are observed near or at the position of the electric field reversal. In the local late-evening sector the electric field reversal becomes less distinct, and often no single well-defined electric field reversal can be identified. In all cases the inverted V electron precipitation events are closely associated with large, typically greater than 30 mV/m, irregular electric field fluctuations with time scales of a few seconds or less.

Gurnett, D. A.↗