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At least 289 records · Page 16

Relaxed Bell inequalities with arbitrary measurement dependence for each observer

Bell's inequality was originally derived under the assumption that experimenters are free to select detector settings independently of any local “hidden variables” that might affect the outcomes of measurements on entangled particles. This assumption has come to be known as “measurement independence” (also referred to as “freedom of choice” or “settings independence”). For a two-setting, two-outcome Bell test, we derive modified Bell inequalities that relax measurement independence, for either or both observers, while remaining locally causal. We describe the loss of measurement independence for each observer using the parameters M 1 and M 2 , as defined by Hall in 2010, and also by a more complete description that adds two new parameters, which we call M 1 ^ and M 2 ^ , deriving a modified Bell inequality for each description. These “relaxed” inequalities subsume those considered in previous work as special cases, and quantify how much the assumption of measurement independence needs to be relaxed in order for a locally causal model to produce a given violation of the standard Bell-Clauser-Horne-Shimony-Holt (Bell-CHSH) inequality. We demonstrate that both relaxed Bell inequalities are tight bounds on the CHSH parameter by constructing locally causal models that saturate them. For any given Bell inequality violation, the new two-parameter and four-parameter models each require significantly less mutual information between the hidden variables and measurement settings than previous models. We conjecture that the new models, with optimal parameters, require the minimum possible mutual information for a given Bell violation. We also argue that, contrary to various claims in the literature, relaxing freedom of choice need not imply superdeterminism.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Quantum algorithm for simulating the wave equation

We present a quantum algorithm for simulating the wave equation under Dirichlet and Neumann boundary conditions. The algorithm uses Hamiltonian simulation and quantum linear system algorithms as subroutines. It relies on factorizations of discretized Laplacian operators to allow for polynomially improved scaling in truncation errors and improved scaling for state preparation relative to general purpose quantum algorithms for solving linear differential equations. Relative to classical algorithms for simulating the D-dimensional wave equation, our quantum algorithm achieves exponential space savings and achieves a speedup which is polynomial for fixed D and exponential in D. Furthermore, we also consider using Hamiltonian simulation for Klein-Gordon equations and Maxwell's equations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Strong dependence of photoionization time delay on energy and angle in the neighborhood of Fano resonances

In this work, we uncover dramatic variations of the Wigner photoemission time delay with energy and angle in the vicinity of a Fano resonance with the time delay taking opposite signs at different angles at the same energy as well as at the opposite sides of the resonance at the same angle. These variations are illustrated by choosing the Ne 2s → 3p autoionizing state as a case study. Moreover, we demonstrate the existence of strikingly significant changes in time delay due to relativistic effects despite Ne being a low-Z atom. This finding shows the possibility for utilizing time delay chronoscopy as a route towards experimental probing of relativistic interactions and the phases of individual transition matrix elements upon atomic photoionization of low-Z atoms. Finally, we develop a practical parametrization to model and explain the angle and energy variation of the autoionizing resonance time delay in the nonrelativistic limit.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Controlling error orientation to improve quantum algorithm success rates

The success probability of a quantum algorithm constructed from noisy quantum gates cannot be accurately predicted from single-parameter metrics that compare noisy and ideal gates. We illustrate this concept by examining a system with coherent errors and comparing algorithm success rates for different choices of two-qubit gates that are constructed from composite pulse sequences, where the residual gate errors are related by a unitary transformation. As a result, all of the sequences have the same error relative to the ideal gate under any distance measure that is invariant under unitary transformations. However, the circuit success can vary dramatically by choosing error orientations that do not affect the final outcome and error orientations that cancel between conjugate controlled-nots, as demonstrated here with Clifford circuits, compiled Toffoli gates, and quantum simulation algorithms. Furthermore, the results point to the utility of both minimizing the error and optimizing the error direction and also to the advantages of using multiple control sequences for the same gate type within a single algorithm.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Ionization from Rydberg atoms and wave packets by scaled terahertz single-cycle pulses

The strong-field ionization behavior when a Rydberg atom is exposed to a terahertz single-cycle pulse is studied. Fully three-dimensional time-dependent Schrödinger equations and classical trajectory Monte Carlo calculations are performed. Results from stationary eigenstates and Rydberg wave packets are presented, and it is found that the ionization properties can be different for the two cases. All of the pulse parameters and physical quantities are scaled versus the principal quantum number n. The ionized electron's scaled radial, energy, and angular distributions are investigated for different n, and the quantum results are interpreted using a semiclassical method. Furthermore, the scaling relations of quantum interference amplitudes are discussed.

74 ATOMIC AND MOLECULAR PHYSICS↗

Practical and reliable error bars for quantum process tomography

Current techniques in quantum process tomography typically return a single point estimate of an unknown process based on a finite albeit large amount of measurement data. Due to statistical fluctuations, however, other processes close to the point estimate can also produce the observed data with near certainty. Unless appropriate error bars can be constructed, the point estimate does not carry any sound operational interpretation. Here, we provide a solution to this problem by constructing a confidence region estimator for quantum processes. Our method enables reliable estimation of essentially any figure of merit for quantum processes on few qubits, including the diamond distance to a specific noise model, the entanglement fidelity, and the worst-case entanglement fidelity, by identifying error regions which contain the true state with high probability. We also provide a software package, QPtomographer, implementing our estimator for the diamond norm and the worst-case entanglement fidelity. We illustrate its usage and performance with several simulated examples. Furthermore, our tools can be used to reliably certify the performance of, e.g., error correction codes, implementations of unitary gates, or more generally any noise process affecting a quantum system.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Digitization of scalar fields for quantum computing

Qubit, operator, and gate resources required for the digitization of lattice λΦ 4 scalar field theories onto quantum computers are considered, building upon the foundational work by Jordan et al. [Quantum Inf. Comput. 14, 1014 (2014); Science 336, 1130 (2012)], with a focus towards noisy intermediate-scale quantum devices. The Nyquist-Shannon sampling theorem, introduced in this context by Macridin et al. [Phys. Rev. A 98, 042312 (2018)] building on the work of Somma [Quantum Inf. Comput. 16, 1125 (2016)], provides a guide with which to evaluate the efficacy of two field-space bases, the eigenstates of the field operator, as used by Jordan et al., and eigenstates of a harmonic oscillator, to describe ( 0 + 1 )- and ( d + 1 )-dimensional scalar field theory. We show how techniques associated with improved actions, which are heavily utilized in lattice QCD calculations to systematically reduce lattice-spacing artifacts, can be used to reduce the impact of the field digitization in λΦ 4 , but are found to be inferior to a complete digitization improvement of the Hamiltonian using a quantum Fourier transform. When the Nyquist-Shannon sampling theorem is satisfied, digitization errors scale as | log | log | ε dig | | | ~ n Q (number of qubits describing the field at a given spatial site) for the low-lying states, leaving the familiar power-law lattice-spacing and finite-volume effects that scale as | log | ε latt | | ~ N Q (total number of qubits in the simulation). For localized (delocalized) field-space wave functions, it is found that n Q ~ 4 ( 7 ) qubits per spatial lattice site are sufficient to reduce theoretical digitization errors below error contributions associated with approximation of the time-evolution operator and noisy implementation on near-term quantum devices. Only classical computing resources have been used to obtain the results presented in this work.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Dominance of correlation and relativistic effects on photodetachment time delay well above threshold

In this work, Wigner time delay in photodetachment from the 3 p 3 / 2 and 3 p 1 / 2 subshells of Cl - has been studied in the vicinity of the 2 p 3 / 2 and 2 p 1 / 2 thresholds, using the relativistic random phase approximation (RRPA). The results show time delay spectra dominated by many-body correlations along with very complicated dependence on the energy over a broad spectral range. In addition, the time delay spectra of the two spin-orbit split 3 p subshells differ significantly from one another, thereby revealing the importance of relativistic effects even in the case of a low- Z system.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Real-Space Imaging of the Tailored Plasmons in Twisted Bilayer Graphene

Here, we report a systematic plasmonic study of twisted bilayer graphene (TBLG)—two graphene layers stacked with a twist angle. Through real-space nanoimaging of TBLG single crystals with a wide distribution of twist angles, we find that TBLG supports confined infrared plasmons that are sensitively dependent on the twist angle. At small twist angles, TBLG has a plasmon wavelength comparable to that of single-layer graphene. At larger twist angles, the plasmon wavelength of TBLG increases significantly with apparently lower damping. Further analysis and modeling indicate that the observed twist-angle dependence of TBLG plasmons in the Dirac linear regime is mainly due to the Fermi-velocity renormalization, a direct consequence of interlayer electronic coupling. Our work unveils the tailored plasmonic characteristics of TBLG and deepens our understanding of the intriguing nano-optical physics in novel van der Waals coupled two-dimensional materials.

36 MATERIALS SCIENCE↗

Simulations of coherent scattering experiments at storage ring synchrotron radiation sources in the hard x-ray range

Detailed simulations of experiments carried out at modern light sources are directly related to the most efficient and productive use of these facilities for research in multiple branches of science and technology. The “Synchrotron Radiation Workshop” computer code with its Python interface, and Sirepo web-browser-based graphical user interface, currently supports physical optics simulations of coherent X-ray scattering and imaging experiments on user-defined virtual samples. We present examples of simulations of coherent scattering experiments that are typically performed at the Coherent Hard X-ray beamline at Brookhaven National Laboratory’s (BNL) National Synchrotron Light Source II. We also present several comparisons of the simulations with the results of actual coherent X-ray scattering experiments with nano-fabricated test samples produced at BNL’s Center for Functional Nanomaterials.

36 MATERIALS SCIENCE↗

SU-E-T-445: Lateral Optical Density Variation in Flatbed Scanners in Combination with Gafchromic Film

Purpose This study investigates the origin of lateral optical density (OD) variation for Gafchromic film (EBT and EBT2) scanned in transmission mode with Epson flatbed scanners (1680 Expression Pro and 10000XL). Effects investigated are: cross talk, optical path length and polarization. Methods Cross talk has been examined with triangular shaped light-transmission sheets with OD ranging from 0 to opaque. Optical path length has been studied with absorptive and reflective OD-filters (OD range 0.2 to 2.0). Dependency on light-polarization on the scanner read out has been investigated using linear polarizer sheets. All experiments have been performed at centre scanner position (norm point) and at several lateral scan positions, without and with (un)irradiated EBT-film. Dose values used ranged between 0.2 to 9 Gy, yielding an OD-range between 0.25 to 1.1. Results The lateral OD variation is dose dependent and increases up to 14% at most lateral position for dose up to 9 Gy. Cross talk effect contributes to 0.5% in clinical used OD ranges but equals 2% for extreme high dose gradients. Film induced optical path length will effect the lateral OD variation up to 3% at most lateral points. Light polarization is inherent present in these scanners due to multiple reflection on mirrors. In addition film induced polarization is the most important effect generating the observed lateral OD variation. Both Gafchromic film base and sensitive layer have polarizing capabilities; for the sensitive layer its influence is dose dependent. Conclusions Lateral OD variation origins from optical physics (i.e. polarization and reflection) related to scanner and film construction. Cross talk can be ignored in film dosimetry for clinical used dose values and gradients. Therefore it is recommended to determine the lateral OD variation per film type and scanner.

60 APPLIED LIFE SCIENCES↗

Simple method for determining fullerene negative ion formation

A robust potential wherein is embedded the crucial core-polarization interaction is used in the Regge-pole methodology to calculate low-energy electron elastic scattering total cross section for the C 60 fullerene in the electron impact energy range 0.02 ≤ E ≤ 10.0 eV. The energy position of the characteristic dramatically sharp resonance appearing at the second Ramsauer–Townsend minimum of the total cross section representing stable C 60 - fullerene negative ion formation agrees excellently with the measured electron affinity of C 60 [Huang et al., J. Chem. Phys. 140, 224315 (2014)]. The benchmarked potential and the Regge-pole methodology are then used to calculate electron elastic scattering total cross sections for selected fullerenes, from C 54 through C 240 . The total cross sections are found to be characterized generally by Ramsauer–Townsend minima, shape resonances and dramatically sharp resonances representing long-lived states of fullerene negative ion formation. For the total cross sections of C 70 , C 76 , C 78 , and C 84 the agreement between the energy positions of the very sharp resonances and the measured electron affinities is outstanding. Additionally, we compare our extracted energy positions of the resultant fullerene anions from our calculated total cross sections of the C 86 , C 90 and C 92 fullerenes with the estimated electron affinities ≥3.0 eV by the experiment [Boltalina et al., Rapid Commun. Mass Spectrom. 7, 1009 (1993)]. Resonance energy positions of other fullerenes, including C 180 and C 240 are also obtained. Most of the total cross sections presented in this paper are the first and only; our novel approach is general and should be applicable to other fullerenes as well and complex heavy atoms, such as the lanthanide atoms. We conclude with a remark on the catalytic properties of the fullerenes through their negative ions.

74 ATOMIC AND MOLECULAR PHYSICS↗

Qubit noise deconvolution

We present a noise deconvolution technique to remove a wide class of noises when performing arbitrary measurements on qubit systems. In particular, we derive the inverse map of the most common single qubit noisy channels, and exploit it at the data processing step to obtain noise-free estimates of observables evaluated on a qubit system subject to known noise. We illustrate a self-consistency check to ensure that the noise characterization is accurate providing simulation results for the deconvolution of a generic Pauli channel, as well as experimental evidence of the deconvolution of decoherence noise occurring on Rigetti quantum hardware.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Bimolecular Chemistry in the Ultracold Regime

Advances in atomic, molecular, and optical physics techniques allowed the cooling of simple molecules down to the ultracold regime ([Formula: see text]1 mK) and opened opportunities to study chemical reactions with unprecedented levels of control. This review covers recent developments in studying bimolecular chemistry at ultralow temperatures. We begin with a brief overview of methods for producing, manipulating, and detecting ultracold molecules. We then survey experimental works that exploit the controllability of ultracold molecules to probe and modify their long-range interactions. Further combining the use of physical chemistry techniques such as mass spectrometry and ion imaging significantly improved the detection of ultracold reactions and enabled explorations of their dynamics in the short range. We discuss a series of studies on the reaction KRb + KRb → K 2 + Rb 2 initiated below 1 μK, including the direct observation of a long-lived complex, the demonstration of product rotational state control via conserved nuclear spins, and a test of the statistical model using the complete quantum state distribution of the products.

Chemistry↗

36 Hz integral linewidth laser based on a photonic integrated 4.0 m coil resonator

Laser stabilization sits at the heart of many precision scientific experiments and applications, including quantum information science, metrology, and atomic timekeeping. Many of these systems narrow the laser linewidth and stabilize the carrier by use of Pound–Drever–Hall (PDH) locking to a table-scale, ultrahigh quality factor (Q), vacuum spaced Fabry–Perot reference cavity. Integrating these cavities to bring characteristics of PDH stabilization to the chip scale is critical to reducing their size, cost, and weight, and enabling a wide range of portable and system-on-chip applications. We report a significant advance in integrated laser linewidth narrowing, stabilization, and noise reduction by use of a photonic integrated 4.0 m long coil resonator to stabilize a semiconductor laser. We achieve a 36 Hz 1 / π <#comment/> -integral linewidth, Allan deviation of 1.8 × <#comment/> 10 − <#comment/> 13 at 10 ms measurement time, and a 2.3 kHz/s drift—to the best of our knowledge, the lowest integral linewidth and highest stability demonstrated for an integrated waveguide reference cavity. This performance represents over an order of magnitude improvement in integral linewidth and frequency noise over previous integrated waveguide PDH stabilized reference cavities and bulk-optic and integrated injection locked approaches, and over two orders of magnitude improvement in frequency and phase noise than integrated injection locked approaches. Two different wavelength coil designs are demonstrated, stabilizing lasers at 1550 nm and 1319 nm. The resonator is bus-coupled to a 4.0 m long coil, with a 49 MHz free spectral range, mode volume of 1.0 × <#comment/> 10 10 µ <#comment/> m 3 , and 142 million intrinsic Q , fabricated in a CMOS compatible, ultralow loss silicon nitride waveguide platform. Our measurements and simulations show that the thermorefractive noise floor for this particular cavity is reached for frequencies down to 20 Hz in an ambient environment with simple passive vibration isolation and without vacuum or thermal isolation. The thermorefractive noise limited performance is estimated to yield an 8 Hz 1 / π <#comment/> -integral linewidth and Allan deviation of 5 × <#comment/> 10 − <#comment/> 14 at 10 ms, opening a stability regime that heretofore has been available only in fundamentally non-integrated systems. These results demonstrate the potential to bring the characteristics of laboratory-scale stabilized lasers to the integrated, wafer-scale compatible chip scale, and are of interest for a number of applications in quantum technologies and atomic, molecular, and optical physics, and with further developments below 10 Hz linewidth, can be highly relevant to ultralow noise microwave generation.

Liu, Kaikai (ORCID:0000000213609646)↗

Optoacoustic Microscopy for Investigation of Material Nanostructures-Embracing the Ultrasmall, Ultrafast, and the Invisible

The goal of this grant was the development of a new type of scanning acoustic microscope for nanometer resolution ultrasound imaging, based on ultrafast optoacoustics (>GHz). In the microscope, subpicosecond laser pulses was used to generate and detect very high frequency ultrasound with nanometer wavelengths. We report here on the outcome of the 3-year DOE/BES grant which involved the design, multifaceted construction, and proof-of-concept demonstration of an instrument that can be used for quantitative imaging of nanoscale material features – including features that may be buried so as to be inaccessible to conventional lightwave or electron microscopies. The research program has produced a prototype scanning optoacoustic microscope which, in combination with advanced computational modeling, is a system-level new technology (two patents issues) which offer novel means for precision metrology of material nanostructures, particularly those that are of contemporary interest to the frontline micro- and optoelectronics device industry. For accomplishing the ambitious technical goals, the research roadmap was designed and implemented in two phases. In Phase I, we constructed a “non-focusing” optoacoustic microscope instrument (“POAM”), with nanometer vertical (z-) resolution, while limited to approximately 10 micrometer scale lateral recolution. The Phase I version of the instrument which was guided by extensive acoustic and optical numerical modeling of the basic underlying acoustic and optical physics, featured nanometer scale close loop positioning between the optoacoustic transducer element and a nanostructured material sample under investigation. In phase II, we implemented and demonstrated a scanning version of the instrument (“SOAM”) where incident acoustic energy is focused, and scanned on lateral (x-y) spatial scale in the 100 nm range as per the goals of the project. In so doing we developed advanced numerical simulations to provide computational models of the focusing of multi-GHz acoustic waves to the nanometer scale and innovated a series fabrication approaches for a new type of broadband high-frequency acoustic focusing microscope objective by applying methods on nanoimprinting and focused-ion beam techniques. In the following, the Phase I and Phase II instrument development is reported as Section II. The first segment of this section describes the POAM instrument and its development, while including much of the underlying ultrafast acoustic physics which is common to all of our work for this grant. Then, the science and engineering of the SOAM instrument is described, including the methods of fabricating new types of acoustic microlenses. The results section is followed by reports on publications (Section III), Participants (Section IV), and statement of full use of the allocated grant funds (Section V).

36 MATERIALS SCIENCE↗

Atoms and Ions Interacting with Particles and Fields: Final Report

This grant supported research in basic atomic, molecular and optical physics related to the interactions of atoms with particles and fields. The duration of the grant was the 10 year period from 8/2003 to 8/2013. All of the support from the grant was used to pay salaries of the PI, postdocs, graduate students, and undergraduates and travel to conferences and meetings. The results were in the form of publications in peer reviewed journals. There were 65 peer reviewed publications over these 10 years with 8 of the publications in Physical Review Letters; all of the other articles were in respected peer reviewed journals (Physical Review A, New Journal of Physics, Journal of Physics B, ...). I will disuss the results for the periods of time relevant for each grant period.

74 ATOMIC AND MOLECULAR PHYSICS↗

Imaging Multi-Particle Atomic and Molecular Dynamics

Final Report for Grant Number: DE- FG02-10ER16146 This grant supported research in basic atomic, molecular and optical physics related to the interactions of atoms and molecules with photons and electrons. The duration of the grant was the 5 year period from 4/1/2010 – 10/31/2015. All of the support from the grant was used to pay salaries of the PI, graduate students, and undergraduates and travel to conferences and meetings. The results were in the form of publications in peer reviewed journals. There were 20 peer reviewed publications over these 5 years with 2 of the publications in Physical Review Letters and 1 in Nature; all of the other articles were in respected peer reviewed journals (Physical Review A, New Journal of Physics, Journal of Physics B ...).

74 ATOMIC AND MOLECULAR PHYSICS↗