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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Integrated edge-to-exascale workflow for real-time steering in neutron scattering experiments

We introduce a computational framework that integrates artificial intelligence (AI), machine learning, and high-performance computing to enable real-time steering of neutron scattering experiments using an edge-to-exascale workflow. Focusing on time-of-flight neutron event data at the Spallation Neutron Source, our approach combines temporal processing of four-dimensional neutron event data with predictive modeling for multidimensional crystallography. At the core of this workflow is the Temporal Fusion Transformer model, which provides voxel-level precision in predicting 3D neutron scattering patterns. The system incorporates edge computing for rapid data preprocessing and exascale computing via the Frontier supercomputer for large-scale AI model training, enabling adaptive, data-driven decisions during experiments. This framework optimizes neutron beam time, improves experimental accuracy, and lays the foundation for automation in neutron scattering. Although real-time experiment steering is still in the proof-of-concept stage, the demonstrated potential of this system offers a substantial reduction in data processing time from hours to minutes via distributed training, and significant improvements in model accuracy, setting the stage for widespread adoption across neutron scattering facilities and more efficient exploration of complex material systems.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2022

Monitoring the SNS basement neutron background with the MARS detector

Here, we present the analysis and results of the first dataset collected with the MARS neutron detector deployed at the Oak Ridge National Laboratory Spallation Neutron Source (SNS) for the purpose of monitoring and characterizing the beam-related neutron (BRN) background for the COHERENT collaboration. MARS was positioned next to the COH-CsI coherent elastic neutrino-nucleus scattering detector in the SNS basement corridor. This is the basement location of closest proximity to the SNS target and thus, of highest neutrino flux, but it is also well shielded from the BRN flux by infill concrete and gravel. Furthermore, these data show the detector registered roughly one BRN per day. Using MARS' measured detection efficiency, the incoming BRN flux is estimated to be 1.20 ± 0.56 neutrons/m 2 /MWh for neutron energies above ~3.5 MeV and up to a few tens of MeV. We compare our results with previous BRN measurements in the SNS basement corridor reported by other neutron detectors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

SOURCES4D

SOURCES is a code for computing neutron source rates and spectra from spontaneous fission (including delayed neutrons) and (alpha,n) reactions in homogeneous materials and (alpha,n) reactions in single-interface and two-interface geometries. SOURCES is a Los Alamos National Laboratory (LANL) code that is written in FORTRAN and distributed through the Radiation Safety Information Computation Center (RSICC). LANL’s last release of SOURCES to RSICC was SOURCES4C in 2002. This disclosure covers the latest version of SOURCES, SOURCES4D. This version adds sensitivity capabilities for (alpha,n) sources in homogeneous materials. Specifically, SOURCES4D writes new output that can be used to calculate, in post-processing, first and second derivatives of the (alpha,n) source rate density and spectrum with respect to nuclide densities in a homogeneous material and first derivatives of the (alpha,n) source rate density and spectrum with respect to nuclide stopping powers and (alpha,n) cross sections (nuclear data). These derivatives are useful for uncertainty quantification, predictive modeling, and other applications in neutron transport problems.

Favorite, Jeffrey A.↗
DOE OSTI2024

10 Boron-film-based gas detectors at ESS

The development of detectors for the European Spallation Source is an important parallel element to the effort put into the design and construction of the neutron source and instruments. The 10Boron-film-based detector developments that started over a decade ago as basic detector concepts have now reached technical maturity after intense prototyping work and numerous testing campaigns. Several of the ESS beamlines that will soon enter the commissioning phase started welcoming the detector systems built with the 10 B-film converter technology. The real-size demonstrators evolved in the last 2–3 years into a diverse suite of gas proportional counters for use in diffraction, reflectometry and small-angle scattering studies in spite of the operational complexity posed by the requirements for large-area coverage, low material budget and robustness for operation in the high-flux and high-radiation environment of ESS. The detectors are now being shipped to ESS or undergoing the last performance and calibration tests before being handed over to the instrument teams for installation in the host beamlines. A common feature of these detector systems is the very large number of readout channels that they are instrumented with in order to fulfill the demanding requirements for sensitivity, spatial resolution and count-rate capability. Across all of the detector types that will operate at ESS, the integration, testing and commissioning of the read-out technologies and software tools for data reduction, calibration and analysis are the focus of the detector and integration teams. These will yield a wealth of knowledge about their operation as well as initial results on the in-situ performance, a very important asset to ensure rapid commissioning of the detectors when neutrons from the ESS source become available. In this paper we will give an overview of the 10 B-film-based detector technologies included in the ESS detector suite that are currently facing the transition from the production phase to installation and integration with the other beamline components, which comes with its own specific challenges of both organizational and technical nature.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Dual particle imaging using time-of-flight neutron classification

Fast-neutron imaging technology is well-suited for passive nuclear material monitoring, secondary inspection of flagged cargo, and wide-area search for lost neutron sources. However, imaging systems that use pulse shape discrimination for event classification require complex pulse waveform analysis. In this work, we evaluate time-of-flight (TOF) based particle classification as an alternative solution for fast-neutron imaging by classifying all events with a TOF above a maximum threshold as neutrons. We measured a Cf-252 source next to Cs-137 using a 12-bar organic-glass scintillator array. By varying the TOF thresholds for neutron identification, we demonstrate a clear trade-off between event yield and backprojection image fidelity, with stricter thresholds improving precision at the cost of statistics, TOF thresholded data generated an image that predicted the neutron source direction with 20% reduced mean central angle prediction error compared to a traditional pulse shape discrimination (PSD) method with comparable event count. Time-of-flight particle classification shows promise as an alternative to pulse shape discrimination systems for fast neutron imaging systems looking to minimize costs and size of electronics with comparable imaging quality. The sources used demonstrate that the method is effective in classifying measured neutrons in a measurement environment with 150 μCi Cs-137 and 1.6 × 10 6 n/s Cf-252 sources positioned at distances of 66 cm and 81 cm from the detector. Additionally, the method classifies low-energy neutron events that pulse shape discrimination removes, so a combination of both methods would result in a higher overall neutron event efficiency.

Heriot, William [Univ. of Michigan, Ann Arbor, MI ↗
DOE OSTI2023

Lineshape response of plastic scintillator to pair production of 4.44 MeV γ’s

We measure the distribution of energy deposited in a 40 × 88 mm plastic scintillator by e + e – pair production of 4.44 MeV γ-rays. He, we observe the double-escape peak of 3.42 MeV from pair production by tagging 511 keV annihilation radiation in two high-Z scintillators. The source is a standard commercial neutron source using α-emitting 241 Am encapsulated with 9 Be, which has a reaction branch feeding the first I π = 2 + state of 12 C making the 4.44 MeV γ-rays. We demonstrate the extraction of the double-escape peak from the large neutron-produced backgound, and explore some of the features and difficulties of this technique with our apparatus.

Beta calibration↗
DOE OSTI2023

Demonstration of INCC6 for advanced list-mode data acquisition and analysis using ALMM

The International Neutron Coincidence Counting (INCC) software plays an important role in nuclear safeguards and nuclear material control and accounting (NMC&A) measurements. While the current version, INCC5, represents the traditional standard utilized by inspectorates as well as facilities and practitioners alongside shift register hardware, LANL has recently developed an upgraded version of the software, INCC6. INCC6 offers the same analysis tools as INCC5 while adding new capabilities including acquisition and analysis of list-mode data, recording and storage of list-mode data files, and an expanded set of advanced analysis tools that make use of the additional information available from list-mode data. Here, this paper presents the first demonstration of data acquisition and analysis using INCC6 and the Advanced List Mode Multiplicity Module (ALMM). The capability of INCC6 to perform live list-mode data acquisition and analysis is demonstrated for a variety of neutron sources with a range of neutron emission rates relevant for practical applications and validated against the results obtained with INCC5 and traditional shift register hardware. Advanced list-mode analysis tools introduced by INCC6, such as time-interval and coincidence matrix analysis, are also demonstrated. Finally, the capability of INCC6 to analyze list-mode data files is tested and validated against traditional shift register results using INCC5.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

γ-ray measurements in fast-neutron-induced reactions on 203 Tl

Fast-neutron-induced reactions can be used to characterize reaction mechanisms, investigate nuclear structure, and impose constraints on nuclear models. Because of the difficulty in predicting such effects, experimental data are important to constrain models. Thallium isotopes located close to the doubly magic Pb 208 nucleus are important for comparison with shell-model calculations. Study the population of excited states in Tl 203 and lighter isotopes in such reactions. Our methods are as follows. γ -ray cross sections were measured. The data were taken by using the Germanium Array for Neutron-Induced Excitations spectrometer. The pulsed neutron source of the Los Alamos Neutron Science Center's Weapons Neutron Research facility provided neutrons in the energy range from 1 to 300 MeV. The time-of-flight technique was used to determine the incident neutron energies. Cross sections for emission of several γ rays in 20 reaction channels were determined. Candidates for the intruder 9 / 2 - state in Tl 203 , from the odd proton in the h 9 / 2 orbital, and the first 5 + states in Tl 202 , 204 , from admixture of configurations, were identified. The excitation energy of the candidate 9 / 2 - , π h 9 / 2 state is in good agreement with the theoretical prediction from a semi-empirical weak-coupling model and its half-life is in the range of tens of nanoseconds. The feeding of a previously known isomer in Tl 202 exhibits similarities with the feeding of other isomers in this mass region.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Nonstatistical fluctuations in the 35 Cl(n,p) 35 S reaction cross section at fast-neutron energies from 0.6 to 6 MeV

The lack of experimental data on the 35 Cl(n,p) 35 S reaction above 100 keV has led to nuclear data evaluations that are relatively unconstrained at fast neutron energies. As a result, efforts to explore, develop, and potentially certify next generation reactor designs that incorporate chloride salts as a coolant material have been hindered. Here, we report partial cross section data for the 35 Cl(n,p) 35 S and 35 Cl(n,α) 32 P reactions at incident neutron energies between 0.6 MeV and 6 MeV. The measurement was performed using the pulsed beam of neutrons at the unmoderated WNR spallation neutron source at the Los Alamos Neutron Science Center, with the outgoing charged particles detected by the LENZ experimental setup, consisting of annular silicon detectors. Nonstatistical fluctuations in the 35 Cl(n,p 0 ) cross section were observed up to around 3 MeV, and the magnitude of the cross section was systematically lower than all available data evaluations at energies above 1 MeV. Modifications to the ENDF/B-VIII.0 data evaluation are suggested to better reproduce the energy averaged experimental data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Low-energy measurement of the 25 Mg ⁢(𝛼,𝑛)⁢ 28 Si reaction via neutron spectroscopy

During core helium and carbon burning in massive stars, neutrons are produced mainly by the 22 Ne⁢ (𝛼,𝑛) ⁢25 Mg reaction. Some of these released neutrons are captured by heavy seed nuclei from previous nucleosynthesis events, resulting in the slow production of many of the elements between masses 60 ≤ 𝐴 ≤ 90 via the weak 𝑠 process. Determining the overall neutron flux available in this environment is one of the main challenges in modeling its contributions to heavy element production. Not only must the reaction rate be well defined for the primary neutron source, but the rates of neutron poison and recycling reactions must also be well determined. One critical reaction in the simulation network is 25 Mg ⁢(𝛼,𝑛) ⁢ 28 Si. This reaction, together with 25 Mg ⁢(𝑛,𝛾)⁢ 26 Mg and 25 Mg⁢ (𝛼,𝛾) ⁢ 29 Si, determine how 25 Mg nuclei affect the available neutron flux. Past attempts to measure the 25 Mg ⁢(𝛼,𝑛)⁢ 28 Si cross section using neutron moderator counters have been greatly hindered by lower-𝑍 background reactions. Here, in the present work, neutron spectroscopy with deuterated liquid scintillator detectors has been used. The experimental spectra have been analyzed by applying spectrum unfolding techniques to achieve improved background discrimination for the 25 Mg⁢ (𝛼,𝑛)⁢ 28 Si reaction at low energies, down to 𝐸 𝛼 = 1.75 MeV. The separation of the different background contributions gives further insight into the results of previous moderator counter measurements and the measurements lead to a revised and more reliable determination of the reaction rate.

hydrostatic stellar nucleosynthesis↗
DOE OSTI2020

Epithermal Neutron Resonance Analysis Using a Compact D-T Generator

Nuclear material identification and isotopic composition analysis are important capabilities for safeguards and the verification of nuclear arms control and nonproliferation treaties. Epithermal neutron resonance imaging has been proposed for spent fuel assay measurements, and the development of a mobile neutron imaging system could provide such a tool for on-site applications. This technique is highly sensitive to isotopes of interest for safeguards applications (e.g. 235,238 U, 238,239,240 Pu) and yields unique transmission spectra for a target containing actinides and some mid- and high-Z elements. Paired with a position-sensitive neutron detector, such a system could provide spatial information of the target isotopic composition. Recent progress in the development of high intensity neutron sources could make mobile epithermal neutron imaging designs increasingly feasible to serve as a tool for nuclear inspectors. In this work, Monte Carlo (MC) simulations were performed to further optimize a previous design for an epithermal neutron resonance-based analysis apparatus using a D-T portable neutron generator. Additionally, experimental work is being performed to test the feasibility of this method. The MC simulations of moderation time distributions for different moderator compositions and thicknesses were measured to provide a multi-group correction for neutron time-of-flight energy reconstruction.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Photoneutron Production Using an Electron Linear Accelerator for Applications in Neutron Imaging

Photoneutron production is possible using an electron linear accelerator and a target capable of generating photonuclear reactions. A short pulse neutron source can be useful for neutron imaging dynamic experiments. This study is aimed at the feasibility of photoneutron production using a 20 MeV electron linear accelerator and tungsten and depleted uranium targets of various thicknesses. MCNP6 (Monte Carlo N-Particle) code will be used to develop a computational model to estimate total neutron yield, and this will be verified at the Idaho State University’s Accelerator Center. After verification of the neutron yield and energy spectra, an additional MCNP6 model will be developed to analyze the neutron imaging processes. This study will potentially prove it is possible to conduct multi-mode imaging experiments on the anticipated Scorpius electron linear accelerator at the Nevada National Security Sites.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Recent H - ion source research and development at the Oak Ridge National Laboratory

The U.S. Spallation Neutron Source (SNS) is a state-of-the-art neutron scattering facility delivering the world's most intense pulsed neutron beams to a wide array of instruments which are used to conduct investigations in many fields of science and engineering. Neutrons are produced from spallation of liquid Hg by bombardment of short (~1 μs), intense (~35 A) pulses of protons delivered at 60 Hz by a storage ring which is fed by a high-intensity, ~1 GeV H - LINAC. This facility has operated almost continuously since 2006, with ion source performance increasing over those years, and currently providing 50–60 mA of H - ions with a duty-factor of 6% for maintenance-free runs of several months with near 100% availability. Ion source research and development at ORNL has played a key role in enabling and supporting this success: this report provides an update on some of the ongoing ion source research and development efforts which have been undertaken since the previous Negative Ion Beams and Sources (NIBS) conference in 2020. These include significant improvements to H - beam current by extraction from a larger source outlet aperture and improvements to the electron dumping system which should eliminate the gradual loss of electrode voltage over the course of a run which has occasionally impacted SNS operations. Improvement and simplification of the plasma ignition system for the external antenna ion source, a long-standing problem, was also realized. Lastly, RF coupling efficiency was measured for both the SNS internal and external antenna ion sources.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Magnetic Designs of New First Target Beamline Magnets for the ORNL SNS Upgrade

The Spallation Neutron Source (SNS) at ORNL currently is being upgraded from 1.0 GeV to 1.3 GeV. Several water-cooled magnets should be upgraded to transport 30% of higher beam energy. New chicane, injection/extraction septum, and Lambertson magnets were designed. Designing the magnets was a challenging task because the new magnets required good combined integrated field quality and needed to occupy the old magnets space but with about 20% greater integrated magnetic field. Additional strong requirements applied to the magnets fringe field do not disturb the circulating beam. The special field profiles had to be provided in foil areas between magnets. The analysis described here was based on OPERA3D simulations. A special technique was used for analyzing the integrated field harmonics. Initially, the particle track was simulated, and integrated field components were calculated along this track for the reference radius, which were used for the harmonics analysis. In addition, 3D field maps were provided for beam optics simulations. The final beamline analysis confirmed good beam transmission and low losses.

3d field maps↗
DOE OSTI2021

Experimental validation of an integrated modelling approach to neutron emission studies at JET

An integrated modelling methodology for the calculation of realistic plasma neutron sources for the JET tokamak has been developed. The computational chain comprises TRANSP plasma transport and DRESS neutron spectrum calculations, and their coupling to the MCNP neutron transport code, bridging plasma physics and neutronics. Here, we apply the developed methodology to the analysis of neutron emission properties of deuterium and helium plasmas at JET, and validate individual modelling steps against neutron diagnostic measurements. Two types of JET discharges are modelled—baseline-like and three-ion radio-frequency scenarios—due to their diversity in plasma heating, characteristics of the induced fast ion population, and the imprint of these on neutron emission properties. The neutron emission modelling results are quantitatively compared to the total neutron yield from fission chambers, neutron emissivity profiles from the neutron camera, neutron spectra from the time-of-flight spectrometer, and neutron activation measurements. The agreement between measured and calculated quantities is found to be satisfactory for all four diagnostic systems within the estimated experimental and computational uncertainties. Additionally, the effect of neutrons not originating from the dominating D(D, n) 3 He reactions is studied through modelling of triton burnup DT neutrons, and, in mixed D- 3 He plasmas, neutrons produced in the 9 Be(D, nγ) 10 B reaction on impurities. It is found that these reactions can contribute up to several percent to the total neutron yield and dominate the neutron activation of samples. Finally, the effect of MeV-range fast ions on the neutron activation of 115 In and 27 Al samples is measured and computationally validated.

integrated modelling↗
DOE OSTI2021

Recent performance of the SNS H - ion source with a record long run

The Spallation Neutron Source (SNS) accelerator system includes a 65 keV H - injector, a 2.5 MeV radio frequency quadrupole (RFQ), a 1 GeV linac chain (DTL-CCL-SCL) and an accumulator ring. The H - injector consists of an RF-driven, Cs-enhanced, multi-cusp H - ion source and a compact, two-lens electrostatic low energy beam transport (LEBT). In 2018, a new RFQ was installed in place of the original RFQ along with upgraded ion source support infrastructure. This paper presents the operational performance and some highlights of beam studies with the SNS ion source since the new RFQ was put into operation. SNS routinely operates at 1.4 MW average beam power for three run cycles per year. During the most recently finished run, FY20B, we operated a single source for the entire run spanning ~4 months with a >99.5% availability. A single dose of cesiation was conducted during the ion source startup which yielded ≥54 mA current for the entire run with just few minor adjustments of parameters.

Han, Baoxi↗
DOE OSTI2026

Performance assessment of PHITS simulations for the inverse-kinematic p( 7 Li,n) 7 Be reaction based on fast-neutron measurements with a diamond detector

The inverse-kinematics p( 7 Li,n) 7 Be reaction produces forward-focused neutron emission, offering enhanced usable flux and reduced shielding requirements. Reliable simulation of such neutron fields is essential for the development of compact accelerator-based neutron sources. In this study, a PHITS-based simulation framework for the reaction was experimentally assessed using fast-neutron measurements. Forward-directed neutrons were measured with a diamond neutron detector and quantitatively compared with simulations with newly prepared IK-Frag cross-section file based on the proton-induced reaction data in ENDF/B-VIII.1, TENDL-2023, and JENDL-4.0/HE. Measurements and simulations were performed for incident 7 Li 3+ energies ranging from 15.0 to 25.0 MeV using a 50 μm-thick polypropylene target. For all conditions, the PHITS-based simulation framework reproduced the deposited energy spectra at the correct order of magnitude. The comparison of deposited energy spectra in the diamond detector showed high correlation coefficients across all investigated energies, indicating reasonable agreement in spectral shape between simulations and measurements. This work represents an initial step toward establishing a benchmark for PHITS simulations of the inverse kinematic reaction between an incident lithium-ion and a proton target.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Measurement of AmLi Sources for Active Well Coincidence Counter

To support the use of the Oak Ridge National Laboratory (ORNL) large-volume active well coincidence counter (LV-AWCC) in material control and accountancy (MC&A) measurements, a set of AmLi neutron sources was acquired from Savannah River National Laboratory (SRNL). These sources were measured to verify their suitability for use in the ORNL LV-AWCC. The sources produce neutrons at a rate that is within 4% of the rate for one set of AmLi sources already in use and 40% higher than the rate for the other set. These measurements indicate that the SRNL sources are suitable for use in the LV-AWCC because their sensitivity and measurement precision will be similar to those of the sets already in use. However, the SRNL sources still need to be evaluated for MC&A use.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗