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The Jupiter High-240 Experiment

The Jupiter High-240 experiment was performed in May of 2019 by researchers from Los Alamos National Laboratory (LANL) at the National Criticality Experiments Research Center (NCERC) in the Device Assembly Facility (DAF) located at the Nevada National Security Site (NNSS). This experiment has previously been mentioned briefly in prior publication related to a collaborative effort with the Japan Atomic Energy Agency (JAEA) to assess lead void coefficients of reactivity in uranium- and plutonium-fueled systems with lead. This series of experiments supports JAEA’s research into the development of an accelerator driven transmutation system for spent nuclear fuel. The Jupiter High-240 experiment built upon the previous Jupiter experiment by incorporating plutonium fuel plates with higher 240 Pu content. Efforts to formally benchmark the original Jupiter experiment have continued for inclusion in the benchmark handbook of the International Criticality Safety Benchmark Evaluation Project (ICSBEP). Whereas there is much similarity between the two Jupiter experiments, there is a desire to also evaluate and benchmark this second experiment to further contribute towards the availability of lead-sensitive benchmarks. The components utilized in these two experiments have also been used to perform other subcritical and Rossi-α measurements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

First NCSP Sponsored Experiment at LANSCE

Uranium-233 has played an important role in solution critical experiments going back to the 50's and 60's, including experiments from the Falstaff Program. More recently, management of legacy 233 U material across the DOE complex has led to a requirement for improved nuclear cross sections.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Developing a New Criticality Safety Hands-On Training Utilizing ZPPR Plates

Nuclear criticality safety is an extremely important part of the work at Los Alamos National Laboratory (LANL). As part of the work LANL performs to continue to keep criticality safety a top priority, LANL has developed and regularly teaches nuclear criticality safety training classes for both the United States Department of Energy Nuclear Criticality Safety Program as well as internal trainings for LANL employees. A portion of the training classes is comprised of hands-on demonstrations, where students get the opportunity to handle special nuclear material at the National Criticality Experiments Research Center (NCERC). One hands-on demonstration uses the “Class foils,” thin HEU foils which are stacked with lucite moderator plates. A hand-stack is performed until the multiplication reaches the “three-quarters rule,” where the demonstration is continued remotely on a vertical lift assembly up until the system is critical. This hands-on demonstration eventually achieves a critical configuration and follows the ANS-1 guidelines on an approach to critical. Another hands-on demonstration involves handling clad plutonium and neptunium spheres, and follows procedures using criticality safety evaluations to ensure that the hands-on demonstrations remain subcritical.This hands-on demonstration also involves the use of polyethylene shells around the plutonium sphere to demonstrate how additional reflector increases the criticality of a system. This paper is focused on developing a new hands-on demonstration using Zero Power Physics Reactor (ZPPR) plates. This new hands-on demonstration will follow the ANS-8 standards as it is not desired to achieve criticality with the ZPPR plates during the hands-on demonstration. A hands-on demonstration using multiple plutonium parts will likely be more applicable to personnel who handle plutonium on a daily basis, such as LANL glovebox operators.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Preliminary Chlorine Worth Study Benchmark Evaluation

The Chlorine Worth Studies (CWS) experiments with polyvinyl chloride (PVC with chemical formula (C 2 H 3 Cl) n ), chlorinated polyvinyl chloride (CPVC with chemical formula (C 9 H 11 Cl 7 ) n ), and high density polyethylene (HDPE with chemical formula (CH 2 ) n ) were a series of measurements performed at the National Criticality Experiments Research Center (NCERC). The purpose of the CWS experiments was to perform integral experiments that were highly sensitive to the thermal 35 Cl(n,γ) reaction and matched the sensitivities of aqueous chloride operations at the plutonium facility at Los Alamos National Laboratory (LANL). The CWS experiments were performed on the Planet critical assembly machine at NCERC and utilized weapons grade plutonium (WGPu) plates as fuel. The design process and design of the CWS experiment were discussed previously. This paper discusses the benchmark evaluation of the experiment, intended for the International Criticality Safety Benchmark Evaluation Project (ICSBEP). Criticality calculations were performed with MCNP version 6.3. Results presented here are preliminary, as the benchmark has not yet been submitted to the ICSBEP.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

International Intercomparison for Nuclear Accident Dosimetry Using Godiva-IV

During the week of August 22, 2022, Integral Experiment Request (IER) 538, an international blind intercomparison for nuclear accident dosimetry (NAD) exercise, was completed using the Godiva-IV critical assembly at the National Criticality Experiments Research Center (NCERC) located in the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS). This exercise builds upon a series of experiments that include the characterization the radiation fields around Godiva (IER-147) and Flattop (IER-252) and follow up intercomparisons of dosimetry around both Godiva IV and Flattop (IER-148 and IER-253, respectively). The participants consisted of seven Department of Energy laboratories and one laboratory each from the US Navy, United Kingdom, and France. The participants of the exercise were Lawrence Livermore National Laboratory (LLNL); Los Alamos National Laboratory (LANL); Sandia National Laboratory (SNL); Savannah River Site (SRS); Hanford Site, Missions Support and Test Services (MSTS); Y-12 National Security Complex (Y-12); Naval Dosimetry Center (NDC); Atomic Weapons Establishment (AWE); and Institut de Radioprotection et de Sûreté Nucléaire (IRSN). MSTS dosimeters were included in the irradiations but not reported for evaluation. This report primarily discusses the performance of the 24 hour results submitted by participants, though available final results are briefly discussed. Information for each irradiation performed is provided for participating laboratories to produce their own final report which will be incorporated into the CED-4a report.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutron Noise Analysis of the Neptunium Subcritical Observation (NESO) Experiment

The Neptunium Subcritical Observation (NeSO) experiment was a subcritical integral benchmark experiment. This experiment was designed in 2017-2018 and was performed at the National Criticality Experiments Research Center (NCERC) in 2019. Eight different subcritical configurations were measured with varying Nickel reflector thickness. For all configurations, a 3 He detection system was used to record neutron events. The focus of this work is to share neutron noise results of the measured data.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Assessment of Existing Transportation Packages for Use with HALEU

Commercial light water reactor operators and fuel vendors in the United States are pursuing changes to fuel that include increased 235 U enrichment. Economic studies generally anticipate maximum near-term fuel assembly designs with up to 8 wt.% 235 U. Many next-generation nuclear reactor designs require high-assay low-enriched uranium (HALEU) (19.75 wt.% > 235 U > 5 wt.%) fuel. One necessary element for the commercial-scale use of HALEU is the ability to safely transport large quantities of enriched fuel material in multiple forms. However, there is uncertainty as to whether subcriticality requirements can be satisfied with existing package designs and whether existing critical benchmark experiment data are sufficient to support criticality safety code validation for HALEU transportation applications. This study assesses the potential to use currently licensed transportation packages for the transportation of increased enrichment unirradiated U fuel forms. The assessment uses selected package designs that represent the five categories of fuel form-boiling water reactor pins and assemblies, pressurized water reactor pins and assemblies, UF 6 , U-metal and tristructural isotropic (TRISO) particles, and UO 2 pellets or powder-and focuses on demonstrating subcriticality and identifying benchmark critical experiments appropriate for use in criticality computer code validation. Key quantities of interest that relate to subcriticality are limiting conditions (e.g., optimum moderation), package or package array k eff , package capacity, and package transportation array size. The SCALE TSUNAMI-3D and TSUNAMI Indices and Parameters codes are used for sensitivity and uncertainty calculations and for identification of candidate critical benchmark experiments for code validation. The primary metric for identifying candidate benchmarks is the similarity coefficient, c k . For each fuel form category, a representative package is evaluated. Results provided for each package evaluation include enrichment and packaging limits (e.g., maximum transportation array size as a function of enrichment) and benchmark critical experiment similarity coefficients. Results indicate that there are viable means for increasing enrichments into the HALEU range across the spectrum of fuel forms with differing increase amounts available for different packages. Sources of subcriticality margin to offset increased enrichment reactivity include reduced transportation array size, reduced fissile mass, burnable absorber credit, and safety analysis margin harvesting. For all packages except the DN-30, numerous critical benchmark experiment candidates for validation were identified.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Which nuclear data can be validated with LLNL pulsed-sphere experiments?

It is shown here that 14-MeV D+T LLNL pulsed-sphere experiments bring complementary information into the process of validating nuclear data compared to experiments that are traditionally used for this purpose—such as critical assemblies. To be more specific, the 14-MeV D+T LLNL pulsed-sphere neutron-leakage spectra enable to validate scattering and fission nuclear data up to 15 MeV (compared to approximately up to 5 MeV when using criticality experiments) and employ to this end simple compound targets containing only few isotopes. In this work, sensitivity profiles of the spectra to nuclear data are calculated in order to understand in detail which isotopes, observables, and energy ranges of nuclear data contribute significantly to their simulation. These profiles are presented for a few selected spheres containing 16 O, 12 C, 56 Fe, and 239 Pu. It is shown that the neutron-leakage spectra of spheres containing light elements are mostly sensitive to elastic- and inelastic-scattering cross sections on discrete levels and corresponding angular distributions. Spheres of structural materials are sensitive to elastic- and inelastic-scattering cross sections, including scattering on discrete levels and the continuum, and double-differential cross sections. Actinide spheres are also strongly sensitive to the fission observables, in particular to the total-fission neutron spectrum. Thin spheres (in which neutrons experience on average less than one scatter) are mostly sensitive to data near the elastic peak, in the energy range from 12–15 MeV, while thicker ones can be sensitive to data at lower incident-neutron energies due to multiple-scattering effects. This information is brought together with simulations of 71 pulsed-sphere neutron-leakage spectra using the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear-data libraries. This analysis highlights ENDF/B-VIII.0 data that could be further investigated for potential shortcomings ( 6 Li, 12 C, 16 O, 24-26 Mg, 27 Al, 48 Ti, 56 Fe, and 208 Pb) or are likely reliable ( 1,2 H, 7 Li, 9 Be, 14 N, 235,238 U, and 239 Pu) as indicated by validating with LLNL pulsed-sphere experiments.

14-MeV D+T LLNL pulsed-sphere neutron-leakage spec↗

Horizontal Split Table Conceptual Design for Advanced Reactor Validation

Oak Ridge National Laboratory and Lawrence Livermore National Laboratory are collaborating to develop a conceptual design for a horizontal split table for use in performing critical experiments. The goal of this design effort is to provide nuclear data testing and validation capabilities for advanced reactors such as pebble-bed high-temperature gas-cooled reactors, molten salt reactors, and heat pipe microreactor, but it could also be used for the current generation of reactors. The first concept being explored for the horizontal split table, a pebble-bed design based on the HTR-10 reactor, is described in this paper. A critical configuration corresponding to a footprint of about 4.5 m 2 was determined with SCALE/KENO-VI to fit the planned dimensions of the horizontal split table. The similarity of the pebble-bed design and the HTR-10 reactor application was assessed using SCALE/TSUNAMI, and a similarity coefficient $c_k$ of 0.9982 was obtained, proving that the concept will be useful for nuclear data validation and assimilation of pebble-bed type advanced reactors. In the proposed design, the materials with the highest $k_{eff}$ sensitivity are graphite and uranium, demonstrating that particular care must be given to carbon-related cross-section data. The effect of mechanical uncertainties between the fixed and moving tables was also assessed by calculating the reactivity change caused by vertical and horizontal gaps, as well as angular and torsion offsets between the two sides of the horizontal split table concept. The highest relative changes on the concept’s reactivity were caused by angular perturbations. The same analysis process is currently being used to create a molten salt advanced reactor type horizontal split table concept based on the Molten Salt Reactor Experiment (MSRE).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Molten Chloride Reactor Experiment

MCRE will be the first fast spectrum, molten chloride reactor in operation. Small critical experiment to provide data for future reactors. - Collaboration between Southern Company Services, TerraPower, and Idaho National Laboratory (INL), as well as other partners. - Expected to be built and operated at the LOTUS testbed (ZPPR). - Authorized by the U.S. Department of Energy. - Technology development of salt synthesis.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

The Neutron Pulse 1st Quarter 2026 Edition

Things have been busy at National Criticality Experiments Research Center (NCERC) since the start of the year. This quarter NCERC hosted three weeks of criticality safety courses allowing students hands-on experience with fissionable material. They also performed an experiment funded by the DOE-NRC Collaboration (DNCSH) in support of data for TerraPower. Additionally, this quarter included staging, measurement, and repacking operations to prepare for future experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Godiva-IV Dosimetry Exercise 2022 (IER-538 CED4A Report)

This report presents the final results of IER 538, The International Nuclear Accident Dosimeter (NAD) Intercomparison Exercise with Godiva-IV. The purpose of the exercise, held in August of 2022, was to test participants’ NADs and dosimetry personnel to the dose estimation requirements established by ANSI/HPS-N13.3 Dosimetry for Criticality Accidents and DOE-STD-1098-2017, Radiological Control. Two prompt critical bursts of the Godiva critical assembly were used to simulate criticality accidents, and NADs from participating laboratories were placed at known locations around Godiva, mounted on either BOttle Manikin ABsorptions (BOMABs) phantoms (to simulate doses received by people) or plates (to simulate doses in free air). Similar exercises have been held in 2016 and 2018 using National Criticality Experiments Research Center’s (NCERC’s) Flattop and Godiva assemblies.

61 RADIATION PROTECTION AND DOSIMETRY↗

Integral Experiment Execution of Thermal or Epithermal eXperiments using Plutonium with Polyethylene and Iron, IER 519, TEX-Hanford (-Iron), CED-3b

This report documents the execution of experiments and measurements for IER 519, Thermal/Epithermal eXperiments (TEX) for Hanford applications, using plutonium Zero Power Physics Reactor (ZPPR) plates moderated by interstitial polyethylene and iron (Fe) absorber plates. Initial hand stack, mass, and dimensional measurements were performed in July 2025. The experiments were completed over three weeks from December 2025 to January 2026 at the National Criticality Experiments Research Center (NCERC) at the Nevada National Security Sites (NNSS). All photos and critical data were provided by NCERC and experimenters in LANL’s NEN-2.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron Noise Analysis of the Neptunium Subcritical Observation (NESO) Experiment

The Neptunium Subcritical Observation (NeSO) experiment was a subcritical integral benchmark experiment. This experiment was designed in 2017-2018 and was performed at the National Criticality Experiments Research Center (NCERC) in 2019. Eight different subcritical configurations were measured with varying Nickel reflector thickness. For all configurations, a 3 He detection system was used to record neutron events. The focus of this work is to share neutron noise results of the measured data.

3-Helium↗

TEX-Hf: Integral Experiment Execution of Thermal/Epithermal eXperiments using Highly Enriched Uranium with Polyethylene and Hafnium (IER-532 CED-3b Report)

This report documents the experimental configurations and measurements for IER-532, Thermal/Epithermal eXperiments (TEX) with highly enriched uranium (HEU) fuel and interstitial hafnium (Hf), moderated and reflected by polyethylene. TEX-Hf is a variation of and based on the TEX-HEU (IER-297) design, with the inclusion of hafnium. These configurations provide integral experiments for validation of hafnium in the thermal, intermediate, and fast neutron energy regimes by maximizing the sensitivity in k eff to the hafnium isotope cross sections. The experiment campaign was completed over seven weeks during the end of FY22 and beginning of FY23 at the National Critical Experiments Research Center at the Nevada National Security Site. The campaign produced seven experimental configurations, four reproducibility measurements, and many additional dimensional measurements that will be of use to the future benchmark evaluation of this experiment and other experiments using the same HEU fuel. Table 1 summarizes the TEX-Hf experimental configurations, including their physical parameters, calculated fission fractions, and estimated excess reactivities.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The Case for and Against a Gadolinium Bias in SCALE: Round 2

The “Opening Arguments” for and against a gadolinium bias in SCALE were presented at the American Nuclear Society Annual Meeting in Philadelphia, Pennsylvania, in June, 2018. Some critical experiments included in the Oak Ridge National Laboratory Verified, Archived Library of Inputs and Data (VALID) indicate a significant bias as a function of gadolinium concentration. Other experiments indicate that no significant bias exists. The work presented here develops a larger suite of gadolinium-bearing benchmark models to further examine code, data, and benchmark performance. The new benchmark models have been reviewed for accuracy, but documentation and review for addition to the VALID library have not been completed. The problematic benchmarks included in VALID are HEU-SOL-THERM-014 and -016. These are two evaluations from a series of experiments from the Institute for Physics and Power Engineering (IPPE), Russia, documented in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. The entire set of evaluations also includes HEU-SOL-THERM-015, -017, -018, -019, and -025. Each evaluation contains a different uranium concentration, and different configurations within each evaluation include different gadolinium concentrations. These 7 evaluations contain a total of 52 configurations and form the largest subset of experiments considered, and they allow for a more complete assessment of the performance of these benchmarks than has historically been possible using just the HEU-SOL-THERM-014 and -016 results. Additional solution experiments are considered, including MIX-SOL-THERM-006 and -007 and PU-SOL-THERM-034. MIX-SOL-THERM-007 is in the VALID library, whereas MIX-SOL-THERM-006 and PU-SOL-THERM-034 are not. The results for MIX-SOL THERM-007 have not shown a gadolinium trend. These mixed- and plutonium-fueled solutions include 28 configurations. Some experiments including solid fuel and solid gadolinium are also included. These experiments include highly enriched uranium (HEU) foils moderated with polyethylene in HEU-MET-THERM-010, -016, and -034, and low enriched uranium (LEU) pin arrays with gadolinia absorber rods in LEU-COMP THERM-036 and -043. A total 32 cases with solid fuel are included. The IPPE solution benchmarks show a fairly high degree of variability, but no clear trend as a function of gadolinium concentration can be observed. The mixed- and plutonium-fueled solutions show less variability than the HEU solutions and also no trend relative to gadolinium concentration. The solid-fueled experiments also show no trend as a function of gadolinium content. The entire set of benchmarks shows no clear trend on gadolinium content or the energy of the average neutron lethargy causing fission.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NCERC-CL TREAT Free Field Characterization Foil Reaction Rate Results

This report summarizes the analysis and preliminary MCNP reaction rate modeling of free field characterization measurements performed in the Transient Reaction Test Facility (TREAT) at Idaho National Laboratory (INL) between 12/18/2023 and 2/22/2024. A series of seven irradiations were performed using the Big-BUSTER (Broad Use Specimen Transient Experiment Rig) core configuration. Foil sets including 19.5% LEU-Zr alloy wire, S, Au, Fe, Ni, Co, Ti, and Zr were deployed in each irradiation. Identical foil sets were supplied to Los Alamos National Laboratory (LANL), Lawrence Livermore National Laboratory (LLNL), and INL. All foils were supplied by INL. Additional details on the experiment can be found in [2]. The foil sets were shipped to the National Criticality Experiments Research Center Counting Laboratory (NCERC-CL) branch at LANL (NCERC-CL NISC) and were received on 3/25/2024. Additional details on receipt and counting are reported in [3]. All reactor dosimetry measurements were performed in adherence to the ASTM standards applicable to reactor dosimetry. Measured reaction rates from Au, Co, Fe, Ni, and Ti are reported. Select reaction rate ratios and simulated reaction rates and ratios are discussed. Reaction rates for all measured reaction products were modeled with MCNP 6.3.1 and a TREAT input deck supplied by Edward Lum. Neutron emission estimates calculated using the measured and simulated reaction rates show excellent agreement between the three fast-threshold n-p reactions with the percent differences being < 9% between the three reactions. The capture reactions had poorer, but still reasonable, agreement with < 20% percent differences between the neutron emission estimates of the three capture reactions. The percent difference between the fast-threshold and capture reactions is ∼ 100% for each reaction. This supports the TREAT model is not accurately modeling the neutron spectrum and additional measurements are required to characterize TREAT and match measurements to simulation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗