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Atmospheric pressure ionisation - mass spectrometry for argon online monitoring in ASTRID

Safety, operability, waste transmutation and mastered investment costs are key issues for the development of generation IV reactors, especially sodium cooled fast reactors. To achieve a development scheduled around 2040, the nuclear energy division of CEA, France, is studying a prototype called ASTRID (Advanced Sodium Technological Reactor for Industrial Demonstration) which is in its conceptual design phase. To achieve a high level of maturity, In Service Inspection and Repair is very important, in particular fuel cladding failure detection. If such a failure occurs, fission products Xenon and Krypton are released. Their fast and sensitive detection is a challenge. The use of a commercial API-MS is evaluated in this work. Detection limits below 10 ppt have been measured for Kr 84 and for Xe 132. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Thick Films acoustic sensors devoted to MTR environment measurements. Thick Films acoustic sensors devoted to Material Testing Reactor environment measurements

The development of advanced instrumentation for in-pile experiments in Material Testing Reactor constitutes a main goal for the improvement of the nuclear fuel behavior knowledge. An acoustic method for fission gas release detection was tested with success during a first experiment called REMORA 3 in 2010 and 2011, and the results were used to differentiate helium and fission gas release kinetics under transient operating conditions. This experiment was lead at OSIRIS reactor (CEA Saclay, France). The maximal temperature on the sensor during the irradiation was about 150 deg. C. In this paper we present a thick film transducer produce by screen printing process. The screen printing of piezoelectric offers a wide range of possible applications for the development of acoustic sensors and piezoelectric structure for measurements in high temperature environment. We firstly produced a Lead Zirconate Titanate (PZT) based paste composed of Pz27 powder from Ferroperm, CF7575 glass, and organic solvent ESL 400. Likewise a Bismuth Titanate based paste synthesized in our laboratory was produced. With these inks we produced thick film up to 130 μm by screen printing process. Material properties characterizations of these thick-film resonators are essential for device design and applications. The piezoelectric coefficients d33 and pyro-electric P(T) coefficient are investigated. The highest P(T) and d33 are respectively 80 μC.m{sup -2}.K{sup -1} and 130 μC.N{sup -1} for the PZT transducer -which validates the fabrication process-. In view of the development of this transducer oriented for high temperature and irradiation environment, we investigated the electrical properties of the transducers for different ranges of frequencies and temperature - from 20 Hz up to 40 MHz between 30 and 400 deg. C. We highlight the evolution of the impedance response and piezoelectric parameters of screen printed piezoelectric structures on alumina. Shortly an irradiation will be realized in order to investigate their reliability towards neutron fluence. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Education and training in the field of nuclear instrumentation and measurement: CEA/INSTN (National Institute for Nuclear Sciences and Technologies) strategy to improve and develop new pedagogical tools and methods

Part of the French Alternative Energies and Atomic Energy Commission (CEA), the National Institute for Nuclear Science and Technology (INSTN) is a higher education institution whose mission is to provide students and professionals a high level of scientific and technological qualification in all disciplines related to nuclear energy applications. In this frame, INSTN carries out education and training (E and T) programs in nuclear instrumentation and radioprotection. Its strategy has always been to complete theoretical courses by training courses and laboratory works carried out on an extensive range of training tools that includes a large panel of nuclear instrumentation as well as software applications. Since its creation in 1956, the INSTN has conducted both education and vocational programs on ionizing radiation detection. An extensive range of techniques have commonly been used during practical works with students and employees of companies who need to get the knowledge and specialization in this field. Today, the INSTN is mainly equipped with usual detectors and electronics in large numbers in order to be able to accommodate up to 48 trainees at the same time in two classrooms, with only two trainees for one workstation in order to optimize their learning. In the field of the neutron detection systems, the INSTN has strongly developed its offer taking advantage of the use of research reactors, such as ISIS reactor (700 kW) at Saclay. The implementation of neutron detection systems specific to the courses offers a unique way of observing and analysing the signal coming from neutron detectors, as well as learning how to set the parameters of the detection system in real conditions. Providing the trainees with an extensive overview of each part of the neutron monitoring instrumentation apply to a nuclear reactor, hands-on measurements on the ISIS reactor play a major role in ensuring a practical and comprehensive understanding of the neutron detection system and their integration in the safety system of nuclear reactors. It also gives a solid background for the follow up and the development of the neutron detection systems. Another field of activity of the INSTN is the development of new teaching tools using software applications. We describe hereafter two applications that have recently been developed by the institute, O.S.I.R.I.S and DOSIMEX. The INSTN and the company OREKA have developed an innovative teaching tool named O.S.I.R.I.S. The tool is built on a virtual 3D environment in which users operate in a totally free way. The action is located in a pressurised water reactor in the environment of a steam generator building. The users are students or professionals who want to learn and train on concrete situations on how to protect the workers against radiation. Through the use of this serious game, users must: establish a predictive dose evaluation, implement the principles of radiation protection, perform the dose result of the operation, analyse the gap between the predictive collective dose and the collective dose achieved, and decide about the lessons to provide feedback. Taking into account the increasing constraints related to radiation protection, it is essential to use computer codes to evaluate the dose rates generated by sources of ionizing radiation. Many powerful codes exist but are often relatively complex to implement and are dedicated to experts. In addition, these codes are often 'black boxes' that does not allow the user to understand the underlying physics. The objective of DOSIMEX codes developed by the INSTN is to give, by the means of a VBA code with a simple interface, the ability to easily conduct a wide range of radiological exposure situations: calculation of gamma, beta, neutron equivalent dose rate, calculation of internal contamination and atmospheric transfer.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Upgrade of High-Energy X-Ray real-time radioscopy for KROTOS experiment

As part of its R and D programs on severe accidents, in particular on understanding of corium-water interaction, CEA is commissioning an update of the KROTOS experiment at Cadarache. The Xray imaging setup (high energy real-time radioscopy) is upgraded to provide the best performances for the new experimental program. In order to fit the performance needs (faster acquisition, smaller detection limit and higher field of view), two radioscopy setups, with two linear accelerators (linacs 9 MV and 6 MV), are placed in the irradiation cell. Having discussed the expected performances in terms of frequency, detection limit and field-of-view, this article details each stage of both radioscopy chains: principles and technical characteristics. Then, linacs and cameras synchronization (at few hundred Hertz), data flows and storage setups are detailed. Finally, experimental characterizations and performance validations on phantom are presented. (authors)

43 PARTICLE ACCELERATORS↗

JHR Project: a future Material Testing Reactor working as an International user Facility: The key-role of instrumentation in support to the development of modern experimental capacity

Research and development on fuel and material behaviour under irradiation is a key issue for sustainable nuclear energy in order to meet specific needs by keeping the best level of safety. These needs mainly deal with a constant improvement of performances and safety in order to optimize the fuel cycle and hence to reach nuclear energy sustainable objectives. A sustainable nuclear energy requires a high level of performances in order to meet specific needs such as: - Pursuing improvement of the performances and safety of present and coming water cooled reactor technologies. This will require a continuous R and D support following a long-term trend driven by the plant life management, safety demonstration, flexibility and economics improvement. Experimental irradiations of structure materials are necessary to anticipate these material behaviours and will contribute to their optimisation. - Upgrading continuously nuclear fuel technology in present and future nuclear power plants to achieve better performances and to optimise the fuel cycle keeping the best level of safety. Fuel evolution for generation II, III and III+ is a key stake requiring developments, qualification tests and safety experiments to ensure the competitiveness and safety: experimental tests exploring the full range of fuel behaviour determine fuel stability limits and safety margins, as a major input for the fuel reliability analysis. To perform such accurate and innovative progress and developments, specific and ad hoc instrumentation, irradiation devices, measurement methods are necessary to be set up inside or beside the material testing reactor (MTR) core. These experiments require beforehand in situ and on line sophisticated measurements to accurately determine different key parameters such as thermal and fast neutron fluxes and nuclear heating in order to precisely monitor and control the conducted assays. The new Material Testing Reactor JHR (Jules Horowitz Reactor) currently under construction at CEA Cadarache research centre in the south of France will represent a major Research Infrastructure for scientific studies regarding material and fuel behavior under irradiation. It will also be devoted to medical isotopes production. Hence JHR will offer a real opportunity to perform R and D programs regarding needs above and hence will crucially contribute to the selection, optimization and qualification of these innovative materials and fuels. The JHR reactor objectives, principles and main characteristics associated to specific experimental devices associated to measurement techniques and methodology, their performances, their limitations and field of applications will be presented and discussed. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Status of the MeLoDIE experiment, an advanced device for the study of the irradiation creep of LWR cladding with full online capabilities

As a prototype of future instrumented material experiments in the Jules Horowitz Reactor (JHR), the MELODIE project was launched in 2009 by the CEA in collaboration with VTT. Being designed as a biaxial creep experiment with online capability, MELODIE is able to apply an online-controlled biaxial loading on a LWR clad sample up to 120 MPa and to perform an online measurement of its biaxial deformation. An important experimental challenge was to perform reliably accurate measurements under the high nuclear heat load of in-core locations while keeping within their tight space. For that purpose, specific sensors were co-designed with and built by IFE Halden. Manufacturing of the MELODIE components was completed one year ago. The complexity of its in-pile section and of the pressurization system requested a step-by-step tuning of the setup. The toughest part of this process dealt with the Diameter gauge which required a partial redesign to take into account unexpected and unwanted electromagnetic interactions with the hosting device. Final cold performance tests of the on-board instrumentation will be presented. The MELODIE device is now ready and irradiation should start in OSIRIS reactor this spring. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Methodology comparison for gamma-heating calculations in material-testing reactors

The Jules Horowitz Reactor (JHR) is a Material-Testing Reactor (MTR) under construction in the south of France at CEA Cadarache (French Alternative Energies and Atomic Energy Commission). It will typically host about 20 simultaneous irradiation experiments in the core and in the beryllium reflector. These experiments will help us better understand the complex phenomena occurring during the accelerated ageing of materials and the irradiation of nuclear fuels. Gamma heating, i.e. photon energy deposition, is mainly responsible for temperature rise in non-fuelled zones of nuclear reactors, including JHR internal structures and irradiation devices. As temperature is a key parameter for physical models describing the behavior of material, accurate control of temperature, and hence gamma heating, is required in irradiation devices and samples in order to perform an advanced suitable analysis of future experimental results. From a broader point of view, JHR global attractiveness as a MTR depends on its ability to monitor experimental parameters with high accuracy, including gamma heating. Strict control of temperature levels is also necessary in terms of safety. As JHR structures are warmed up by gamma heating, they must be appropriately cooled down to prevent creep deformation or melting. Cooling-power sizing is based on calculated levels of gamma heating in the JHR. Due to these safety concerns, accurate calculation of gamma heating with well-controlled bias and associated uncertainty as low as possible is all the more important. There are two main kinds of calculation bias: bias coming from nuclear data on the one hand and bias coming from physical approximations assumed by computer codes and by general calculation route on the other hand. The former must be determined by comparison between calculation and experimental data; the latter by calculation comparisons between codes and between methodologies. In this presentation, we focus on this latter kind of bias. Nuclear heating is represented by the physical quantity called absorbed dose (energy deposition induced by particle-matter interactions, divided by mass). Its calculation with Monte Carlo codes is possible but computationally expensive as it requires transport simulation of charged particles, along with neutrons and photons. For that reason, the calculation of another physical quantity, called KERMA, is often preferred, as KERMA calculation with Monte Carlo codes only requires transport of neutral particles. However, KERMA is only an estimator of the absorbed dose and many conditions must be fulfilled for KERMA to be equal to absorbed dose, including so-called condition of electronic equilibrium. Also, Monte Carlo computations of absorbed dose still present some physical approximations, even though there is only a limited number of them. Some of these approximations are linked to the way how Monte Carlo codes apprehend the transport simulation of charged particles and the productive and destructive interactions between photons, electrons and positrons. There exists a huge variety of electromagnetic shower models which tackle this topic. Differences in the implementation of these models can lead to discrepancies in calculated values of absorbed dose between different Monte Carlo codes. The magnitude of order of such potential discrepancies should be quantified for JHR gamma-heating calculations. We consequently present a two-pronged plan. In a first phase, we intend to perform compared absorbed dose / KERMA Monte Carlo calculations in the JHR. This way, we will study the presence or absence of electronic equilibrium in the different JHR structures and experimental devices and we will give recommendations for the choice of KERMA or absorbed dose when calculating gamma heating in the JHR. In a second phase, we intend to perform compared TRIPOLI4 / MCNP absorbed dose calculations in a simplified JHR-representative geometry. For this comparison, we will use the same nuclear data library for both codes (the European library JEFF3.1.1 and photon library EPDL97) so as to isolate the effects from electromagnetic shower models on absorbed dose calculation. This way, we hope to get insightful feedback on these models and their implementation in Monte Carlo codes. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Monte-Carlo Simulations of the Nuclear Energy Deposition Inside the CARMEN-1P Differential Calorimeter Irradiated into OSIRIS Reactor

The nuclear heating measurements in Material Testing Reactors (MTRs) are crucial for the study of nuclear materials and fuels under irradiation. The reference measurements of this nuclear heating are especially performed by a differential calorimeter including a graphite sample material. These measurements are then used for other experimental conditions in order to predict the nuclear heating and thermal conditions induced in the irradiation devices. Nuclear heating is a great deal of interest at the moment as the measurement of such heating is an important issue for MTRs reactors. This need is especially generated by the new Jules Horowitz Reactor (JHR), under construction at CEA/Cadarache 'French Alternative Energies and Atomic Energy Commission'. This new reactor, that will be operational in late 2019, is a new facility for the nuclear research on materials and fuels. Indeed the expected nuclear heating rate is about 20 W/g for nominal capacity of 100 MW. The present Monte Carlo calculation works belong to the IN-CORE (Instrumentation for Nuclear radiation and Calorimetry On line in Reactor): a joint research program between the CEA and Aix- Marseille University in 2009. One scientific aim of this program is to design and develop a multi-sensors device, called CARMEN, dedicated to the measurements of main physical parameters simultaneously encountered inside JHR's experimental channels (core and reflector) such as neutron fluxes, photon fluxes, temperature, and nuclear heating. A first prototype was already developed. This prototype includes two mock-ups dedicated respectively to neutronic measurements (CARMEN-1N) and to photonic measurements (CARMEN-1P) with in particular a specific differential calorimeter. Two irradiation campaigns were performed successfully in the periphery of OSIRIS reactor (a MTR located at Saclay, France) in 2012 for nuclear heating levels up to 2 W/g. First Monte Carlo calculations reduced to the graphite sample of the calorimeter were carried out. A preliminary analysis shows that the numerical results overestimate the measurements by about 20 %. A new approach has been developed in order to estimate the nuclear heating by two methods (energy deposition or KERMA) by considering the whole complete geometry of the sensor. This new approach will contribute to the interpretation of the irradiation campaign and will be useful to improve the out-of-pile calibration procedure of the sensor and its thermal response during irradiations. The aim of this paper is to present simulations made by using MCNP5 Monte-Carlo transport code (using ENDF/B-VI nuclear data library) for the nuclear heating inside the different parts of the calorimeter (head, rod and base). Calculations into two steps will be realized. We will use as an input source in the model new spectra (neutrons, prompt-photons and delayed-photons) calculated with the Monte Carlo code TRIPOLI-4{sup R} inside different experimental channels (water) located into the OSIRIS periphery and used during the CARMEN-1P irradiation campaign. We will consider Neutrons- Photons-Electrons and Photons-Electrons modes. We will begin by a brief description of the differential-calorimeter device geometry. Then the MCNP5 model used for the calculations of nuclear heating inside the calorimeter elements will be introduced. The energy deposition due to the prompt-gamma, delayed-gamma and neutrons, the neutron-activation of the device will be considered. The different components of the nuclear heating inside the different parts of the calorimeter will be detailed. Moreover, a comparison between KERMA and nuclear energy deposition estimations will be given. Finally, a comparison between this total nuclear heating Calculation and Experiment in graphite sample will be determined. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

HPGe detector shielding optimization with MCNPX for the MEDINA PGNAA cell

Radioactive waste repositories must guarantee the non-toxicity of the waste in the long term, not only regarding radioactivity but also regarding other environmental contamination such as toxic chemicals. Analytical methods already exist for chemical characterization (ICP-MS, ICP-AES...) but they are based on test sampling. A possible alternative, for waste packages with an appropriate gamma radiation level, is to use Prompt Gamma Neutron Activation Analysis (PGNAA), a non-destructive measurement technique sensitive to several toxic chemicals. In view of the characterization of radioactive wastes in Germany and France, collaboration between the CEA Cadarache (France) and the Forschungszentrum Juelich (Germany) was initiated a few years ago. FZJ holds a PGNAA graphite cell called MEDINA (Multi Element Detection based on Instrumental Neutron Activation), allowing the characterization of 225 L drums. Fast neutrons are emitted from a D-T pulsed 14 MeV neutron generator and thermalized in graphite to induced radiative captures in the waste materials. Prompt capture gamma rays are detected using a 104% relative efficiency n-type HPGe. However, HPGe crystal is sensitive to fast neutron damage and to thermal neutron activation. A thermal neutron shield made of lithium fluorine and lithium carbonate is already used around the detector. In order to further decrease the current of fast and thermal neutrons coming into the crystal without penalizing MEDINA sensitivity (by decreasing the thermal neutron flux and neutron die away time of the cell, the gamma detection efficiency, or increasing the gamma background), some configurations based on easy-to-implement modifications of MEDINA have been simulated with MCNPX with a model of the cell already validated by experiments. Results show that fast and thermal neutron incoming current in the HPGe could easily be reduced by about a factor of 2 by additional quantities of graphite and by replacing lithium carbonate by lithium fluorine with a higher {sup 6}Li concentration. In addition, these modifications slightly increase the thermal neutron flux in the cell without deteriorating the neutron die away time, and reduce the gamma background about a factor of 2 during the neutron pulse but 5 times less after it. More important changes have also been tested, such as the addition of polyethylene and lead between the neutron generator and the HPGe detector, which is more effective regarding neutron shielding but decreases the neutron die away time, partly compensated by a larger initial thermal neutron flux. Concerning gamma background, hydrogen capture gamma ray (2.23 MeV) is increased due to the presence of polyethylene but lead around the HPGe decreases the total gamma background. In conclusion, simple modifications are possible to improve detector shielding and life time before thermal annealing of the crystal, without reducing MEDINA cell performances. Some of these modifications will be tested in the coming months. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Impact Study on the Methodology used for Photon- Heating Determination in Material-Testing Reactors

Determination of photon heating by calculation is an important issue for the Jules Horowitz Reactor (JHR), the next international Material-Testing Reactor (MTR) under construction at CEA Cadarache research center in the south of France. Accurate knowledge of photon heating in structure materials and irradiation devices is necessary for JHR design and safety studies. In this paper, we quantify the impact of different photon-heating calculation routes by comparing absorbed dose and KERMA calculations (Kinetic Energy Released per Mass) from two different Monte Carlo codes, TRIPOLI-4.9{sup R} and MCNP (Monte Carlo N-Particle transport code). These calculations are carried out in JHR-representative geometries with the nuclear-data library JEFF3.1.1 and the photon-data library EPDL97. Discrepancies amounting to up to 18% between absorbed dose and KERMA are found in JHR irradiation devices and are linked to charged-particle transport effects taking place in heterogeneous materials of small dimensions. In a JHR assembly cell, discrepancies of about 1% on photon KERMA and of about 3% on absorbed dose are highlighted between the two Monte Carlo codes. These latter discrepancies are small compared to typical sources of uncertainty for Monte Carlo calculation (for instance, nuclear data uncertainty) and are supposed to be due to differences in the processing of gamma-production data by neutron interactions and to differences in electromagnetic-shower models and implementation between the two codes. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

MEXIICO: a new equipment to study the pressure impact on the irradiated fuel behavior

The new MEXIICO experimental loop has recently been started in the LECA-STAR hot-cell facility of the CEA Cadarache. It is dedicated to the understanding of the basic mechanisms occurring in nuclear fuels during nuclear reactor power transients and accidental situations. Under such conditions the nuclear fuels are submitted to thermo-mechanical stresses. These stresses play a major role on fission product release and fuel fragmentation. Evaluating such fuel behavior represents a key issue for reactor safety analyses. In the first part of the paper, we describe the complete MEXIICO device, which main component is a hot isostatic press allowing to perform analytical experiments in the [20 -1600 C. degrees / 10 MPa - 160 MPa] region. As shown by simulations (ALCYONE fuel performance code), the upper value of the pressure (160 MPa) is consistent with the one experienced by fuels under nuclear power transients. We also present the experimental loop starting from the argon pressurized feed-line, the furnace and its associated instrumentation and the exhaust line equipped with specific valves and flowmeters controlling the pressure and flowrate. We then focus on the gamma spectrometry measurement which allows recording the fission gas release kinetics. In the second part of the paper, we detail the capability of the MEXIICO device to provide new experimental data regarding the influence of pressure on the fission gas release and fuel fragmentation, and to determine a pressure threshold above which fission gas release and fuel fragmentation may be inhibited. This device also allows investigating the impact of pressure on the microstructure evolution, coupling it with post-test microanalysis examinations: this procedure will allow characterizing the effect of temperature and pressure on the bubble evolution and interconnection. Evolutions of the fuel modeling, needed to simulate correctly these new experimental data, will be also presented. In the last section of the paper, we present the commissioning tests of the MEXIICO device showing the good reproducibility of the tests performed first in conventional laboratory and then in hot-cell laboratory. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Updated Radiological Inventory of G1 Reactor Thanks to a Strengthened Data Processing - 17271

The radiological inventory of G1 reactor is under refinement and consolidation. This reactor, located at the CEA Marcoule center in France, presents an issue for Chlorine-36 as graphite was used as moderator. The improvement of the 3D physical description and a better understanding of historical events enable the computation of activation levels thanks to a numerical model. These results are compared to old samples and more recent ones to quantify nuclide activity levels as well as their spatial distributions. In particular a spatial and statistical correction of sample bias leads to an update of the radiological inventory with an expected reduction of average activity levels. Another part of the work consists in identifying missing pieces of information and still uncertain parts of the reactor (sample analysis of activated concrete for instance) to reinforce the radiological inventory of G1 reactor. This will be the basis of future investigation works. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Disposing of waste package with respect to physico-chemical characteristics - 15041

The waste inventory to be taken into account for the design of the Cigeo project is defined in the industrial program for waste management established in cooperation between nuclear operators (EDF, AREVA, CEA) and Andra. This waste inventory has been constituted with a list of different families of radioactive waste packages from High Level Waste (HLW) to Intermediate Level Long-lived Waste (IL-LLW). IL-LLW include a large variety of items such as structural elements from fuel assemblies (cladding from the fuel rods called 'hulls', end pieces called 'end caps' and assembly spacer grids, etc.), sludge from effluent treatment or miscellaneous equipment (filters, pumps, etc.). Most ILLW (except solidified sludges) are basically metallic but organic and inorganic components such as plastics (cellulose, PVC...) and salts may also be included. The rules used for designing Cigeo are based on the separation of waste having different physico-chemical characteristics in different cells. However it could be possible to dispose of waste packages with different physico-chemical characteristics in the same cell if we can demonstrate that a type of waste does not generate significant physico-chemical perturbations on other co-stored families. The first step of our analysis has been the identification of categories of materials present in waste likely to interact with each other. The second step consisted in analysing qualitatively the physico-chemical interactions between these materials. In the third step, we defined criteria allowing evaluation of the consequences of these interactions on (i) gas production (mainly H{sub 2}), (ii) radionuclide release and transfer and (iii) degradation of concrete components of the disposal cell. We built then a table allowing qualitative comparison of the consequences of the interactions between the materials types defined in the first step. The conclusion of this study shows that it is necessary to pay a very careful attention before disposing of waste packages containing organic components nearby waste packages containing actinides radionuclides. The geochemical phenomena coupling must also be quantitatively evaluated so as to analyse possible interaction processes between the released organic compounds and the cementitious components of the cells, the near-field clay-stone and the radionuclides migration. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Remotely controlled manipulators using tele-robotic software provide enhanced efficiency and ergonomy for work in hot cells - 15101

Computer aid and electrical assistance have been applied to remote manipulation inside hostile environments. A heavy duty master/slave manipulator system, the MT200, has been updated with the addition of an electronic bay with specialized software, a motion module and a poly-articulated master arm. This is the result of an ambitious 20-year continuous improvement program undertaken by the French nuclear institutions, CEA LIST Interactive Robotics Unit and AREVA in order to improve ergonomics, safety and efficiency at the AREVA La Hague nuclear plant. The new manipulator system, named MT200 TAO, uses tele-robotics to improve ergonomics by literally lightening the workload transmitted to operators. The link between the master and slave arms is electrical rather than mechanical. The poly-articulated master arm uses haptic (force feedback) technology, so the operator effort is multiplied by a homothetic coefficient in the slave arm. Simplification of the offset function, now integrated into the master arm, means that the operator can be correctly positioned for each task. Some repetitive tasks can be carried out with great precision in playback (robotic mode). In addition, this technology contributes to better efficiency, higher availability rate, lower maintenance costs with increased MTBF (Mean Time Between Failures), reduced waste, improved performance and safer use (remote workstations are feasible). (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Measurement of the plutonium hold-up in glove box before dismantling - 15111

The French Bruyeres-Le-Chatel CEA (Commissariat a l'Energie Atomique et aux Energies Alternatives - French Alternatives Energies and Atomic Energy Commission) research center is going through a period of cleaning and dismantling of theses old treatment facilities on fissile materials and others associated nuclides. Some very large glove boxes contained some machines like melting furnace which can't be moved and are dismantled in situ. We need to evaluate the quantity of fissile materials to prevent criticality risk, to bring the evidence to the safety authority, to manage for the best the radioprotection of the workers and to manage waste production. A melting furnace in a glove box was dismantled. Measurements by gamma spectrometry with an HPGe detector (High Purity Germanium) and passive neutron counting (coincidence counting with shift register) are done in situ (furnace in the glove box). In order to refine the measurements, some data acquisitions by sector of glove box were carried out. In view of the geometries to characterize, some modelings have been created, in order to correct the different attenuations and to determine the plutonium masses content in the glove box, including the use of infinite energy technique. For the measurement by passive neutron counting (coincidence counting with shift register), we have used two slabs in high density polythene including nine He3 counters in each slab. This measurement technique is complementary to gamma spectrometry, and allows quantizing the fissile material which would be included in interstice of high Z material. The 100-L and 200-L drums produced during the dismantling were also measured. Based on simplified assumptions to analyze in situ measurements, plutonium weight could be evaluated. This approach of measurement in amount, during and after dismantling, has allowed to quantize the fissile material mass present in the glove box and didn't produce waste package which wouldn't respected the technical specifications of storage outlets. The results show good agreement between in situ and waste measurements. (authors)

07 ISOTOPE AND RADIATION SOURCES↗

Mobile platform for radiological characterization of sites under or after decommissioning - 15139

Nowadays, nuclear industry is facing a crucial need in establishing radiological characterization for the assessment and the monitoring of any remediation work. Regarding its experience in this domain, the French Commission for Atomic Energy and Alternative Energies (CEA) of Fontenay-aux-Roses, established an important feedback and developed a sound methodology for radiological characterization. A clean-up project is managed from the initial surface characterization to the final one, once volumes of contaminated soil have been removed. Samples are collected via recognized methods and data is gathered by real-time acquisition with different conveyance such as all-in-vehicles, cart, walking, helicopter or drone. Accurate radiological analyses are performed on site thanks to the mobile laboratories cluster, called SMaRT. It enables to realize long-time gamma spectroscopy, chemical preparation for alpha spectroscopy or beta liquid scintillation counting. Data is processed with geo-statistics via the software Kartotrak, 2D or 3D mapping are created with the associated uncertainty and probability map. Drilling profiles with geological data (layers composition, particles size, etc.) are studied in order to understand the behavior of the contamination in depth. Source term, contaminated volumes and sanitary impact are calculated in order to determine the optimum excavation depth. Finally, data is stored in an online site that insures the traceability of the whole process. This just-in-time production model allows a fast response and control of costs and avoids the disadvantages of radioactive material transport. This whole innovative process, developed inside the mobile platform, requires all these tools that have been used in France and continuously evolving for more than 10 years thanks to a learning organization. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

EDF industrial strategy for the management of radioactive waste - 15204

In France, EDF is in charge of electronuclear power operation since the sixties and consequently has to manage radioactive waste. Radioactive waste management is based on the control of each industrial step, taking into account the classification by activity level and radioactive half life. The main steps are to limit waste quantities at the generation stage, sort out non-rad and recoverable items from the waste, recycle, treat and package the radioactive waste as soon as it is generated, limit the use of interim storage, prepare and achieve as soon as reasonably practicable conditioning and disposal. EDF aims to empower operators in charge of NPP operating and of decommissioning and to centralize interfaces with the stakeholders in order to pool management routes and to guarantee the consistency of our industrial policy. The French regulatory framework for the management of radioactive waste and material is set by the French 2006 planning Act, in line with the European Directive. The legal framework structures interactions between EDF and the regulatory bodies (Nuclear Safety Authority, General Directorate for Energy and Climate), the French National Radioactive Waste Management Agency (ANDRA) and other waste producer (mainly AREVA Company and CEA). Regarding short lived waste, management routes are in current operation for the large majority of this waste generated both by power plants in service and during decommissioning. EDF is working on new management route for metallic materials knowing the future evolution of deposits is the field of large refit and decommissioning activities. Regarding long lived waste, disposal development represents a major stake for EDF. EDF contributes to design studies of the geological disposal center and collaborates with ANDRA for the acceptance of future national waste disposal. (authors)

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Chooz-A steam generators characterization - 15205

EDF nuclear waste management requires a deep understanding of characterization, classification and waste sorting operations. In fact, French nuclear waste management defines several classes with specific management, treatment and storage facilities. Based on particular criteria, the more the radiological risk of the nuclear waste is important, the more its management will be complex and expensive. During the dismantling of the first French pressurized reactor Chooz-A, decontamination of the primary water circuits (not including the reactor vessel), the steam generators and the pressurizer have been carried out in order to reduce their activity levels. Thanks to these decontamination operations, and a specific characterization methodology, EDF was able to de-classify the 4 steam generators and store them in one piece at the ANDRA Very Low Level Activity disposal facilities instead of the Low and Intermediate Level activity one. This de-classification allowed EDF to avoid important cutting and packaging processes. Therefore, significant dose reductions for the operators and financial gain have been made. To characterize and declare Chooz-A SG activity, EDF-CIDEN uses a methodology defined by the French institute of atomic energy, CEA. The method is based on external gamma spectrometry measurements performed with NaI collimated detectors, associated with MERCURAD simulations providing the transfer functions for the detectors and activity sources. Internal measurements are carried out with a CZT (CdZnTe) probe inside the SG tubes to refine the 3D model. In fact, the primary side represents the main source of activity, and understanding its contamination distribution is important to reduce the model and calculation uncertainties. Measurements eventually provide SG {sup 60}Co global activity, from which the activities of other radionuclides of the spectrum are determined using scaling factors. The final activity declaration takes into account the standard deviation of the measurements in order to cover the uncertainties of the methodology. Thereby, the declaration is 'slightly over-estimative', enough to meet the waste storage facility acceptance criteria. (authors)

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