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At least 289 records · Page 16
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Benzimidazoles as Metal-Free and Recyclable Hydrides for CO 2 Reduction to Formate

We report a novel metal-free chemical reduction of CO 2 by a recyclable benzimidazole-based organo-hydride, whose choice was guided by quantum chemical calculations. Notably, benzimidazole-based hydride donors rival the hydride-donating abilities of noble-metal-based hydrides such as [Ru(tpy)(bpy)H] + and [Pt(depe) 2 H] + . Chemical CO 2 reduction to the formate anion (HCOO–) was carried out in the absence of biological enzymes, a sacrificial Lewis acid, or a base to activate the substrate or reductant. 13 CO 2 experiments confirmed the formation of H 13 COO – by CO 2 reduction with the formate product characterized by 1H NMR and 13C NMR spectroscopy and ESI-MS. The highest formate yield of 66% was obtained in the presence of potassium tetrafluoroborate under mild conditions. The likely role of exogenous salt additives in this reaction is to stabilize and shift the equilibrium toward the ionic products. After CO 2 reduction, the benzimidazole-based hydride donor was quantitatively oxidized to its aromatic benzimidazolium cation, establishing its recyclability. In addition, we electrochemically reduced the benzimidazolium cation to its organo-hydride form in quantitative yield, demonstrating its potential for electrocatalytic CO 2 reduction. These results serve as a proof of concept for the electrocatalytic reduction of CO 2 by sustainable, recyclable, and metal-free organo-hydrides.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Mass measurements show slowdown of rapid proton capture process at waiting-point nucleus 64Ge

Abstract X-ray bursts are among the brightest stellar objects frequently observed in the sky by space-based telescopes. A type-I X-ray burst is understood as a violent thermonuclear explosion on the surface of a neutron star, accreting matter from a companion star in a binary system. The bursts are powered by a nuclear reaction sequence known as the rapid proton capture process (rp process), which involves hundreds of exotic neutron-deficient nuclides. At so-called waiting-point nuclides, the process stalls until a slower β + decay enables a bypass. One of the handful of rp process waiting-point nuclides is 64 Ge, which plays a decisive role in matter flow and therefore the produced X-ray flux. Here we report precision measurements of the masses of 63 Ge, 64,65 As and 66,67 Se—the relevant nuclear masses around the waiting-point 64 Ge—and use them as inputs for X-ray burst model calculations. We obtain the X-ray burst light curve to constrain the neutron-star compactness, and suggest that the distance to the X-ray burster GS 1826–24 needs to be increased by about 6.5% to match astronomical observations. The nucleosynthesis results affect the thermal structure of accreting neutron stars, which will subsequently modify the calculations of associated observables.

Physics↗
DOE OSTI2015

Multidiagnostic analysis of ion dynamics in ultrafast laser ablation of metals over a large fluence range

The dynamics of ions in ultrafast laser ablation of metals is studied over fluences ranging from the ablation threshold up to ≈75 J/cm{sup 2} by means of three well-established diagnostic techniques. Langmuir probe, Faraday cup, and spectrally resolved intensified charge coupled device imaging simultaneously monitored the ions produced during ultrafast laser ablation of a pure copper target with 800 nm, ≈50 fs, Ti: Sapphire laser pulses. The fluence dependence of ion yield is analyzed, resulting in the observance of three different regimes. The specific ion yield shows a maximum at about 4–5 J/cm{sup 2}, followed by a gradual reduction and a transition to a high-fluence regime above ≈50 J/cm{sup 2}. The fluence dependence of the copper ions angular distribution is also analyzed, observing a gradual increase in forward-peaking of Cu ions for fluences up to ≈10 J/cm{sup 2}. A broader ion component is observed at larger angles for fluences larger than ≈10 J/cm{sup 2}. Finally, an experimental characterization of the ionic angular distribution for several metallic targets (Mg, Al, Cr, Fe, Cu, and W) is carried out at a relatively high fluence of ≈66 J/cm{sup 2}. Interestingly, the ion emission from the volatile metals shows a narrow, forward-peaked distribution, and a high peak ion yield compared to the refractory metals. Moreover, the width of ionic angular distributions presents a striking correlation with the peak ion yield.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Beam hardening and smoothing correction effects on performance of micro-ct SkyScan 1173 for imaging low contrast density materials

We have designed and fabricated phantom mimicking breast cancer composition known as a region that has low contrast density. The used compositions are a microcalcifications, fatty tissues and tumor mass by using Al{sub 2}O{sub 3}, C{sub 27}H{sub 46}O, and hard nylon materials. Besides, phantom also has a part to calculate low cost criteria /CNR (Contrast to Noise Ratio). Uniformity will be measured at water distillation medium located in a part of phantom scale contrast. Phantom will be imaged by using micro ct-sky scan 1173 high energy type, and then also can be quantified CT number to examine SkyScan 1173 performance in imaging low contrast density materials. Evaluation of CT number is done at technique configuration parameter using voltage of 30 kV, exposure 0.160 mAs, and camera resolution 560x560 pixel, the effect of image quality to reconstruction process is evaluated by varying image processing parameters in the form of beam hardening corrections with amount of 25%, 66% and100% with each smoothing level S10,S2 and S7. To obtain the better high quality image, the adjustment of beam hardening correction should be 66% and smoothing level reach maximal value at level 10.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

High-density carbon ablator ignition path with low-density gas-filled rugby hohlraum

A recent low gas-fill density (0.6 mg/cc 4 He) cylindrical hohlraum experiment on the National Ignition Facility has shown high laser-coupling efficiency (>96%), reduced phenomenological laser drive corrections, and improved high-density carbon capsule implosion symmetry [Jones et al., Bull. Am. Phys. Soc. 59(15), 66 (2014)]. In this Letter, an ignition design using a large rugby-shaped hohlraum [Amendt et al., Phys. Plasmas 21, 112703 (2014)] for high energetics efficiency and symmetry control with the same low gas-fill density (0.6 mg/cc 4 He) is developed as a potentially robust platform for demonstrating thermonuclear burn. The companion high-density carbon capsule for this hohlraum design is driven by an adiabat-shaped [Betti et al., Phys. Plasmas 9, 2277 (2002)] 4-shock drive profile for robust high gain (>10) 1-D ignition performance and large margin to 2-D perturbation growth.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

High energy X-ray pinhole imaging at the Z facility

A new high photon energy (hν > 15 keV) time-integrated pinhole camera (TIPC) has been developed as a diagnostic instrument at the Z facility. This camera employs five pinholes in a linear array for recording five images at once onto an image plate detector. Each pinhole may be independently filtered to yield five different spectral responses. The pinhole array is fabricated from a 1-cm thick tungsten block and is available with either straight pinholes or conical pinholes. Each pinhole within the array block is 250 μm in diameter. The five pinholes are splayed with respect to each other such that they point to the same location in space, and hence present the same view of the radiation source at the Z facility. The fielding distance from the radiation source is 66 cm and the nominal image magnification is 0.374. Initial experimental results from TIPC are shown to illustrate the performance of the camera.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Femtosecond diffraction studies of the sodium chloride phase diagram under laser shock compression

The phase diagram of sodium chloride (NaCl) under laser shock compression has been studied at Linac Coherent Light Source (LCLS) at the x-ray free-electron laser facility. Both solid–solid (B1 → B2) and solid–liquid (B2 → liquid) transitions have been observed along the Hugoniot over nanosecond time scales. By combining structural measurements through in situ x-ray diffraction, pressure determination through velocimetry, and a thermal equation-of-state, the shock-compressed data are used to constrain the phase diagram of NaCl. Transformation into the B2 phase is found to occur at 28(2) GPa, and B2–liquid coexistence is observed between 54(4) and 66(6) GPa, with near full melt at 66(6) GPa. Late-time pressure release from an initial shocked B2-state results in a B2 → B1 back transformation. Our results show agreement with previous static compression data, suggesting that the time scale for melting is very rapid and that equilibrium states in NaCl are being accessed over nanosecond time scales. Finally, a multiphase equation-of-state description of NaCl incorporated into a one-dimensional hydrocode is used to interpret pressure and temperature evolution over these rapid time scales.

36 MATERIALS SCIENCE↗
DOE OSTI2012

ABRUPT CHANGES OF THE PHOTOSPHERIC MAGNETIC FIELD IN ACTIVE REGIONS AND THE IMPULSIVE PHASE OF SOLAR FLARES

We compared time profiles of changes of the unsigned photospheric magnetic flux in active regions with those of their associated soft X-ray (SXR) bursts for a sample of 75 {>=} M5 flares well observed by Global Oscillation Network Group longitudinal magnetographs. Sixty-six of these events had stepwise changes in the spatially integrated unsigned flux during the SXR flares. In superposed epoch plots for these 66 events, there is a sharp increase in the unsigned magnetic flux coincident with the onset of the flare impulsive phase while the end of the stepwise change corresponds to the time of peak SXR emission. We substantiated this result with a histogram-based comparison of the timing of flux steps (onset, midpoint of step, and end) for representative points in the flaring regions with their associated SXR event time markers (flare onset, onset of impulsive phase, time of peak logarithmic derivative, maximum). On an individual event basis, the principal part of the stepwise magnetic flux change occurred during the main rise phase of the SXR burst (impulsive phase onset to SXR peak) for {approx}60% of the 66 cases. We find a close timing agreement between magnetic flux steps and >100 keV emission for the three largest hard X-ray (>100 keV) bursts in our sample. These results identify the abrupt changes in photospheric magnetic fields as an impulsive phase phenomenon and indicate that the coronal magnetic field changes that drive flares are rapidly transmitted to the photosphere.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

PALM-3000: EXOPLANET ADAPTIVE OPTICS FOR THE 5 m HALE TELESCOPE

We describe and report first results from PALM-3000, the second-generation astronomical adaptive optics (AO) facility for the 5.1 m Hale telescope at Palomar Observatory. PALM-3000 has been engineered for high-contrast imaging and emission spectroscopy of brown dwarfs and large planetary mass bodies at near-infrared wavelengths around bright stars, but also supports general natural guide star use to V ≈ 17. Using its unique 66 × 66 actuator deformable mirror, PALM-3000 has thus far demonstrated residual wavefront errors of 141 nm rms under ∼1'' seeing conditions. PALM-3000 can provide phase conjugation correction over a 6.''4 × 6.''4 working region at λ = 2.2 μm, or full electric field (amplitude and phase) correction over approximately one-half of this field. With optimized back-end instrumentation, PALM-3000 is designed to enable 10{sup –7} contrast at 1'' angular separation, including post-observation speckle suppression processing. While continued optimization of the AO system is ongoing, we have already successfully commissioned five back-end instruments and begun a major exoplanet characterization survey, Project 1640.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

A SPATIALLY RESOLVED STUDY OF THE SYNCHROTRON EMISSION AND TITANIUM IN TYCHO’S SUPERNOVA REMNANT USING NuSTAR

We report results from deep observations (∼750 ks) of Tycho's supernova remnant (SNR) with NuSTAR. Using these data, we produce narrow-band images over several energy bands to identify the regions producing the hardest X-rays and to search for radioactive decay line emission from {sup 44}Ti. We find that the hardest (>10 keV) X-rays are concentrated in the southwest of Tycho, where recent Chandra observations have revealed high emissivity “stripes” associated with particles accelerated to the knee of the cosmic-ray spectrum. We do not find evidence of {sup 44}Ti, and we set limits on its presence and distribution within the SNR. These limits correspond to an upper-limit {sup 44}Ti mass of M{sub 44} < 2.4 × 10{sup −4} M{sub ⊙} for a distance of 2.3 kpc. We perform a spatially resolved spectroscopic analysis of 66 regions across Tycho. We map the best-fit rolloff frequency of the hard X-ray spectra, and we compare these results to measurements of the shock expansion and ambient density. We find that the highest energy electrons are accelerated at the lowest densities and in the fastest shocks, with a steep dependence of the rolloff frequency with shock velocity. Such a dependence is predicted by models where the maximum energy of accelerated electrons is limited by the age of the SNR rather than by synchrotron losses, but this scenario requires far lower magnetic field strengths than those derived from observations in Tycho. One way to reconcile these discrepant findings is through shock obliquity effects, and future observational work is necessary to explore the role of obliquity in the particle acceleration process.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

FERMI GAMMA-RAY SPACE TELESCOPE OBSERVATIONS OF THE GAMMA-RAY OUTBURST FROM 3C454.3 IN NOVEMBER 2010

The flat-spectrum radio quasar 3C454.3 underwent an extraordinary 5 day {gamma}-ray outburst in 2010 November when the daily flux measured with the Fermi Large Area Telescope (LAT) at photon energies E > 100 MeV reached (66 {+-} 2) x 10{sup -6} photons cm{sup -2} s{sup -1}. This is a factor of three higher than its previous maximum flux recorded in 2009 December and {approx}> 5 times brighter than the Vela pulsar, which is normally the brightest source in the {gamma}-ray sky. The 3 hr peak flux was (85 {+-} 5)x10{sup -6} photons cm{sup -2} s{sup -1}, corresponding to an apparent isotropic luminosity of (2.1 {+-} 0.2)x10{sup 50} erg s{sup -1}, the highest ever recorded for a blazar. In this Letter, we investigate the features of this exceptional event in the {gamma}-ray band of the Fermi-LAT. In contrast to previous flares of the same source observed with the Fermi-LAT, clear spectral changes are observed during the flare.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

Atomic Fermi gas in the unitary limit by quantum Monte Carlo methods: Effects of the interaction range

We calculate the ground-state properties of an unpolarized two-component Fermi gas with the aid of the diffusion quantum Monte Carlo (DMC) methods. Using an extrapolation to the zero effective range of the attractive two-particle interaction, we find E/E{sub free} in the unitary limit to be 0.212(2), 0.407(2), 0.409(3), and 0.398(3) for 4, 14, 38, and 66 atoms, respectively. Our calculations indicate that the dependence of the total energy on the effective range of the interaction R{sub eff} is sizable and the extrapolation to R{sub eff}=0 is therefore important for reaching the true unitary limit. To test the quality of nodal surfaces and to estimate the impact of the fixed-node approximation, we perform released-node DMC calculations for 4 and 14 atoms. Analysis of the released-node and the fixed-node results suggests that the main sources of the fixed-node errors are long-range correlations, which are difficult to sample in the released-node approaches due to the fast growth of the bosonic noise. Besides energies, we evaluate the two-body density matrix and the condensate fraction. We find that the condensate fraction for the 66-atom system converges to 0.56(1) after the extrapolation to the zero interaction range.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Superconductivity and phase diagrams of CaK(Fe 1- x Mn x ) 4 As 4 single crystals

In order to study the effects of Mn substitution on the superconducting and magnetic ground state of CaKFe 4 As 4 (T c = 35 K), members of the CaK (Fe 1–x Mn x ) 4 As 4 series have been synthesized by high-temperature solution growth in single-crystalline form and characterized by elemental analysis, thermodynamic, and transport measurements. These measurements show that the superconducting transition temperature decreases monotonically and is finally suppressed below 1.8 K as x is increased from 0 to 0.036. For x values greater than 0.016, signatures of a magnetic transition can be detected in both thermodynamic and transport measurements in which kinklike features allow for the determination of the transition temperature T* that increases as Mn substitution increases. Here, a temperature-composition (T–x) phase diagram is constructed, revealing a half-dome of superconductivity with the magnetic transition temperature T* appearing near 26 K for x ~ 0.017 and rising slowly up to 33 K for x ~ 0.036. In addition to the creation of the T–x phase diagram for CaK(Fe 1–x Mn x ) 4 As 4 , specific-heat data are used to track the jump in specific heat at T c ; the CaK(Fe 1–x Mn x ) 4 As 4 data do not follow the scaling of ΔC p with $T$$^{3}_{c}$ as many of the other Fe-based superconducting systems do. These data suggest that, as magnetic pair breaking is present, the jump in C p for a given T c is reduced. Elastoresistivity coefficients 2m 66 and m 11 – m 12 as a function of temperature are also measured. 2m 66 and m 11 – m 12 are qualitatively similar to CaK(Fe 1–x Ni x ) 4 As 4 . This may indicate that the magnetic order in Mn-substituted system may be still the same as CaK(Fe 1–x Mn x ) 4 As 4 . Superconductivity of CaK(Fe 1–x Mn x ) 4 As 4 is also studied as a function of magnetic field. A clear change in H' c2 (T)/T c , where H' c2 (T) is dH' c2 (T)/dT, at x ~ 0.015 is observed and probably is related to change of the Fermi surface due to magnetic order. Coherence lengths and the London penetration depths are also calculated based on H c1 and H c2 data. Coherence lengths as the function of x also show the changes near x = 0.015, again consistent with Fermi-surface changes associated with the magnetic ordering seen for higher-x values.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Femtosecond tracking of carrier relaxation in germanium with extreme ultraviolet transient reflectivity

Extreme ultraviolet (XUV) transient reflectivity around the germanium M 4,5 edge (3d core-level to valence transition) at 30 eV is advanced to obtain the transient dielectric function of crystalline germanium [100] on femtosecond to picosecond time scales following photoexcitation by broadband visible-to-infrared (VIS/NIR) pulses. By fitting the transient dielectric function, carrier-phonon induced relaxations are extracted for the excited carrier distribution. The measurements reveal a hot electron relaxation rate of 3.2±0.2ps attributed to the X-L intervalley scattering and a hot hole relaxation rate of 600±300fs ascribed to intravalley scattering within the heavy hole (HH) band, both in good agreement with previous work. An overall energy shift of the XUV dielectric function is assigned to a thermally induced band gap shrinkage by formation of acoustic phonons, which is observed to be on a timescale of 4-5 ps, in agreement with previously measured optical phonon lifetimes. The results reveal that the transient reflectivity signal at an angle of 66° with respect to the surface normal is dominated by changes to the real part of the dielectric function, due to the near critical angle of incidence of the experiment (66°-70° for the range of XUV energies used. Finally, this work provides a methodology for interpreting XUV transient reflectivity near core-level transitions, and it demonstrates the power of the XUV spectral region for measuring ultrafast excitation dynamics in solids.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2020

Primary $\gamma$-ray intensities and $\gamma$-strength functions from discrete two-step $\gamma$-ray cascades in radiative proton-capture experiments

Background: Reaction rates of radiative capture reactions can play a crucial role in the nucleosynthesis of heavy nuclei in explosive stellar environments. These reaction rates depend strongly on $\gamma$-ray decay widths in the reaction products, which are, for nonresonant capture reactions at high excitation energies, derived from the $\gamma$-ray strength function and the nuclear level density. Recently, the ratio method was applied to primary $\gamma$ rays observed from ($\textit{d, p}$) reactions and nuclear resonance fluorescence measurements to extract the dipole strength in atomic nuclei and to test the generalized Brink-Axel hypothesis. Purpose: The purpose of this work is to apply the ratio method to primary $\gamma$-ray intensities of the 63,65 Cu($\textit{p},\gamma$) reactions to extract $\gamma$-ray strength information on the nuclei 64,66 Zn. Here, the impact of spin distribution, total $\gamma$-ray decay widths, level densities, and width fluctuations on the application of the ratio method will be discussed. Additionally, by comparing the relative $\gamma$-ray strength at different excitation energies, conclusions on the validity of the generalized Brink-Axel hypothesis can be made. Method: The radiative proton capture reaction measurements have been performed at the HORUS $\gamma$-ray spectrometer of the University of Cologne at one excitation energy for each reaction. Primary $\gamma$-ray intensities have been determined by normalizing secondary $\gamma$-ray transitions in two-step cascades using their absolute branching ratio. The ratio method was applied to the measured primary $\gamma$-ray intensities as well as to previous measurements by Erlandsson et al. at different excitation energies. Results: The relative strength function curve for 64 Zn from our measurement shows no significant deviation from the previous measurement at a different excitation energy. The same is true for 66 Zn where both measurements were at almost the same excitation energy. Absolute $\gamma$-strength function values have been obtained by normalizing the relative curves to quasiparticle random phase approximation calculations because of the absence of experimental data in the respective energy region. Conclusion: The generalized Brink-Axel hypothesis, i.e., the independence of the strength function on the excitation energy, seems to hold in the studied energy region and nuclei. The method to obtain primary $\gamma$-ray intensities from two-step cascade spectra was shown to be a valuable and sensitive tool although its uncertainties are connected to the knowledge of the low-energy level scheme of the investigated nucleus. The scaling in the ratio method should be taken with care, because the relative strength is not a simple sum of $f_{E1}$ and $f_{M1}$ but a somewhat complex linear combination dependent on the excitation energy of the nucleus.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

94 {beta}-Decay Half-Lives of Neutron-Rich 55Cs to 67Ho: Experimental Feedback and Evaluation of the r-Process Rare-Earth Peak Formation

The β-decay half-lives of 94 neutron-rich nuclei 144$-$151 Cs, 146$-$154 Ba, 148$-$156 La, 150$-$158 Ce, 153$-$160 Pr, 156$-$162 Nd, 159$-$163 Pm, 160$-$166 Sm, 161$-$168 Eu, 165$-$170 Gd, 166$-$172 Tb, 169$-$173 Dy, 172$-$175 Ho, and two isomeric states 174m Er, 172m Dy were measured at the Radioactive Isotope Beam Factory, providing a new experimental basis to test theoretical models. Strikingly large drops of β-decay half-lives are observed at neutron-number N = 97 for 58 Ce, 59 Pr, 60 Nd, and 62 Sm, and N = 105 for 63 Eu, 64 Gd, 65 Tb, and 66 Dy. Lastly, features in the data mirror the interplay between pairing effects and microscopic structure. r-process network calculations performed for a range of mass models and astrophysical conditions show that the 57 half-lives measured for the first time play an important role in shaping the abundance pattern of rare-earth elements in the solar system

Wu, J.↗
DOE OSTI2016

Seasonal responses of terrestrial ecosystem water‐use efficiency to climate change

Abstract Ecosystem water‐use efficiency ( EWUE ) is an indicator of carbon–water interactions and is defined as the ratio of carbon assimilation ( GPP ) to evapotranspiration ( ET ). Previous research suggests an increasing long‐term trend in annual EWUE over many regions and is largely attributed to the physiological effects of rising CO 2 . The seasonal trends in EWUE , however, have not yet been analyzed. In this study, we investigate seasonal EWUE trends and responses to various drivers during 1982–2008. The seasonal cycle for two variants of EWUE , water‐use efficiency ( WUE , GPP / ET ), and transpiration‐based WUE ( WUE t , the ratio of GPP and transpiration), is analyzed from 0.5° gridded fields from four process‐based models and satellite‐based products, as well as a network of 63 local flux tower observations. WUE derived from flux tower observations shows moderate seasonal variation for most latitude bands, which is in agreement with satellite‐based products. In contrast, the seasonal EWUE trends are not well captured by the same satellite‐based products. Trend analysis, based on process‐model factorial simulations separating effects of climate, CO 2 , and nitrogen deposition ( NDEP ), further suggests that the seasonal EWUE trends are mainly associated with seasonal trends of climate, whereas CO 2 and NDEP do not show obvious seasonal difference in EWUE trends. About 66% grid cells show positive annual WUE trends, mainly over mid‐ and high northern latitudes. In these regions, spring climate change has amplified the effect of CO 2 in increasing WUE by more than 0.005 gC m −2 mm −1 yr −1 for 41% pixels. Multiple regression analysis further shows that the increase in springtime WUE in the northern hemisphere is the result of GPP increasing faster than ET because of the higher temperature sensitivity of GPP relative to ET . The partitioning of annual EWUE to seasonal components provides new insight into the relative sensitivities of GPP and ET to climate, CO 2, and NDEP .

Huang, Mengtian↗
DOE OSTI2016

An integrated assessment of the potential of agricultural and forestry residues for energy production in China

Biomass has been widely recognized as an important energy source with high potential to reduce greenhouse gas emissions while minimizing environmental pollution. In this study, we employ the Global Change Assessment Model to estimate the potential of agricultural and forestry residue biomass for energy production in China. Potential availability of residue biomass as an energy source was analyzed for the 21st century under different climate policy scenarios. Currently, the amount of total annual residue biomass, averaged over 2003-2007, is around 15519PJ in China, consisting of 10818PJ from agriculture residues (70%) and 4701PJ forestry residues (30%). We estimate that 12693PJ of the total biomass is available for energy production, with 66% derived from agricultural residue and 34% from forestry residue. Most of the available residue is from south central China (3347PJ), east China (2862PJ) and south-west China (2229PJ), which combined exceeds 66% of the total national biomass. Under the reference scenario without carbon tax, the potential availability of residue biomass for energy production is projected to be 3380PJ by 2050 and 4108PJ by 2095, respectively. When carbon tax is imposed, biomass availability increases substantially. For the CCS 450ppm scenario, availability of biomass increases to 9002PJ (2050) and 11524PJ (2095), respectively. For the 450ppm scenario without CCS, 9183 (2050) and 11150PJ (2095) residue biomass, respectively, is projected to be available. Moreover, the implementation of CCS will have a little impact on the supply of residue biomass after 2035. Our results suggest that residue biomass has the potential to be an important component in China's sustainable energy production portfolio. As a low carbon emission energy source, climate change policies that involve carbon tariff and CCS technology promote the use of residue biomass for energy production in a low carbon-constrained world.

bioenergy↗