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NASA NTRS2005

Assimilation of MLS and OMI Ozone Data

Ozone data from Aura Microwave Limb Sounder (MLS) and Ozone Monitoring Instrument (OMI) were assimilated into the ozone model at NASA's Global Modeling and Assimilation Office (GMAO). This assimilation produces ozone fields that are superior to those from the operational GMAO assimilation of Solar Backscatter Ultraviolet (SBUV/2) instrument data. Assimilation of Aura data improves the representation of the "ozone hole" and the agreement with independent Stratospheric Aerosol and Gas Experiment (SAGE) III and ozone sonde data. Ozone in the lower stratosphere is captured better: mean state, vertical gradients, spatial and temporal variability are all improved. Inclusion of OMI and MLS data together, or separately, in the assimilation system provides a way of checking how consistent OMI and MLS data are with each other, and with the ozone model. We found that differences between OMI total ozone column data and model forecasts decrease after MLS data are assimilated. This indicates that MLS stratospheric ozone profiles are consistent with OMI total ozone columns. The evaluation of error characteristics of OMI and MLS ozone will continue as data from newer versions of retrievals becomes available. We report on the initial step in obtaining global assimilated ozone fields that combine measurements from different Aura instruments, the ozone model at the GMAO, and their respective error characteristics. We plan to use assimilated ozone fields in estimation of tropospheric ozone. We also plan to investigate impacts of assimilated ozone fields on numerical weather prediction through their use in radiative models and in the assimilation of infrared nadir radiance data from NASA's Advanced Infrared Sounder (AIRS).

Stajner, I.↗
NASA NTRS2005

Assimilation of ozone profiles from the Improved Limb Atmospheric Spectrometer: Study on Antarctic Ozone - 2

Ozone data from the Improved Limb Atmospheric Spectrometer-II (ILAS-II) were included in addition to other satellite observations in the ozone assimilation system at the Global Modeling and Assimilation Office (GMAO) of NASA/Goddard. The control run assimilated data from NOAA 16 Solar Backscatter Ultraviolet/2 (SBUV/2) and Polar Ozone and Aerosol Measurement III (POAM III) instruments. Persistent impacts over Antarctica and transient impacts over northern middle and high latitudes are seen from April to October 2003, when ILAS-II provided good coverage. The largest improvements with respect to independent ozone sonde data are seen over the South Pole station. Ozone analyses and forecasts from the assimilation of SBUV/2, POAM III and ILAS-II data b e used to investigate the transport of ozone to southern middle latitudes following the breakup of the Antarctic vortex. The quality of analyses and forecasts is evaluated by comparison with independent Stratospheric Aerosol and Gas Experiment III (SAGE III) ozone data near 46degs. Anomaly correlations between SAGE III data and forecasts'exceed 0.6 for up to five to seven days at 30,50, and 70 ma. The loss of skill with advancing forecast length is related to dynamical errors due to an excessively persistent vortex in longer forecasts, which hampers the transport of low ozone air into middle latitudes.

Stajner, Ivanka↗
NASA NTRS2005

Convective lofting links Indian Ocean air pollution to paradoxical South Atlantic ozone maxima

We describe a broad resolution of the Atlantic Parado concerning the seasonal and geographic distribution, of tropical tropospheric ozone. We highlight periods of significant maximum tropospheric O3 for Jan.- April, 1999, exploiting satellite estimates and SHADOZ (Southern Hemisphere Additional Ozonesondes). Trajectory analyses connecting sondes and Total Tropospheric Ozone (TTO) maps suggest a complex influence from the Indian Ocean: beginning with mixed combustion sources, then low level transport, cumulonimbus venting, possible stratospheric input, and finally high-level transport to the west, with possible mixing over Africa. For the Jan.-March highest column-O3 periods in the Atlantic, distinct sounding peaks trace to specific NO sources, especially lightning, while in the same episodes, recurring every 20-50 days, more diffuse buildups of Indian-to-Atlantic pollution make important contributions.

Chatfield, R. B.↗
NASA NTRS2006

SAGE III solar ozone measurements: Initial results

Results from two retrieval algorithms, o3-aer and o3-mlr , used for SAGE III solar occultation ozone measurements in the stratosphere and upper troposphere are compared. The main differences between these two retrieved (version 3.0) ozone are found at altitudes above 40 km and below 15 km. Compared to correlative measurements, the SAGE II type ozone retrievals (o3-aer) provide better precisions above 40 km and do not induce artificial hemispheric differences in upper stratospheric ozone. The multiple linear regression technique (o3_mlr), however, can yield slightly more accurate ozone (by a few percent) in the lower stratosphere and upper troposphere. By using SAGE III (version 3.0) ozone from both algorithms and in their preferred regions, the agreement between SAGE III and correlative measurements is shown to be approx.5% down to 17 km. Below 17 km SAGE III ozone values are systematically higher, by 10% at 13 km, and a small hemispheric difference (a few percent) appears. Compared to SAGE III and HALOE, SAGE II ozone has the best accuracy in the lowest few kilometers of the stratosphere. Estimated precision in SAGE III ozone is about 5% or better between 20 and 40 km and approx.10% at 50 km. The precision below 20 km is difficult to evaluate because of limited coincidences between SAGE III and sondes. SAGE III ozone values are systematically slightly larger (2-3%) than those from SAGE II but the profile shapes are remarkably similar for altitudes above 15 km. There is no evidence of any relative drift or time dependent differences between these two instruments for altitudes above 15-20 km.

Wang, Hsiang-Jui↗
NASA NTRS2006

Tropospheric and stratospheric ozone from assimilation of Aura data

Ozone is an atmospheric trace gas with multiple impacts on the environment. Global ozone fields are needed for air quality predictions, estimation of the ultraviolet radiation reaching the surface, climate-radiation studies, and may also have an impact on longer-term weather predictions. We estimate global ozone fields in the stratosphere and troposphere by combining the data from EOS Aura satellite with an ozone model using data assimilation. Ozone exhibits a large temporal variability in the lower stratosphere. Our previous work showed that assimilation of satellite data from limb-sounding geometry helps constrain ozone profiles in that region. We assimilated ozone data from the Aura Microwave Limb Sounder (MLS) and the Ozone Monitoring Instrument (OMI) into the ozone system at NASA's Global Modeling and Assimilation Office (GMAO). Ozone is transported within a general circulation model (GCM) which includes parameterizations for stratospheric photochemistry, tropospheric chemistry, and a simple scheme for heterogeneous ozone loss. The focus of this study is on the representation of ozone in the lower stratosphere and tropospheric ozone columns. We plan to extend studies of tropospheric ozone distribution through assimilation of ozone data from the Tropospheric Emission Spectrometer (TES). Comparisons with ozone sondes and occultation data show that assimilation of Aura data reproduces ozone gradients and variability in the lower stratosphere well. We proceed by separating the contributions to temporal changes in the ozone field into those that are due to the model and those that are due to the assimilation of Aura data. The impacts of Aura data are illustrated and their role in the representation of ozone variability in the lower stratosphere and troposphere is shown.

Stajner, I.↗
NASA NTRS2006

Tropospheric Ozone from Assimilation of Aura Data using Different Definitions of the Tropopause

Ozone data from Aura OMI and MLS instruments were assimilated into the general circulation model (GCM) constrained by assimilated meteorological fields from the Global Modeling and Assimilation Office at NASA Goddard. Properties of tropospheric ozone and their sensitivity to the definition of the tropopause are investigated. Three definitions of the tropopause are considered: (1) dynamical (using potential vorticity and potential temperature), (2) using temperature lapse rate, and (3) using a fixed ozone value. Comparisons of the tropospheric ozone columns using these tropopause definitions will be presented and evaluated against coincident profiles from ozone sondes. Assimilated ozone profiles are used to identify possible tropopause folding events, which are important for stratosphere-troposphere exchange. Each profile is searched for multiple levels at which ozone attains the value typical of the troposphere-stratosphere transition in order to identify possible tropopause folds. Constrained by the dynamics from a global model and by assimilation of Aura ozone data every 3-hours, this data set provides an opportunity to study ozone evolution in the upper troposphere and lower stratosphere with high temporal resolution.

Stajner, Ivanka↗
NASA NTRS2007

An Ozone Increase in the Antarctic Summer Stratosphere: A Dynamical Response to the Ozone Hole

Profiles of ozone concentration retrieved from the SBUV series of satellites show an increase between 1979 and 1997 in the summertime Antarctic middle stratosphere (approx. 25-10 hPa). Data over the South Pole from ozone sondes confirm the increase. A similar ozone increase is produced in a chemistry climate model that allows feedback between constituent changes and the stratospheric circulation through radiative heating. A simulation that excludes the radiative coupling between predicted ozone and the circulation does not capture this ozone increase. We show that the ozone increase in our model simulations is caused by a dynamical feedback in response to the changes in the stratospheric wind fields forced by the radiative perturbation associated with the Antarctic ozone hole.

Stolarski, R. S.↗
NASA NTRS2008

Progress on the Use of Combined Analog and Photon Counting Detection for Raman Lidar

The Atmospheric Radiation Measurement (ARM) program Raman Lidar (CARL) was upgraded in 2004 with a new data system that provides simultaneous measurements of both the photomultiplier analog output voltage and photon counts. The so-called merge value added procedure (VAP) was developed to combine the analog and count-rate signals into a single signal with improved dynamic range. Earlier versions of this VAP tended to cause unacceptably large biases in the water vapor mixing ratio during the daytime as a result of improper matching between the analog and count-rate signals in the presence of elevated solar background levels. We recently identified several problems and tested a modified version of the merge VAP by comparing profiles of water vapor mixing ratio derived from CARL with simultaneous sonde data over a six month period. We show that the modified merge VAP significantly reduces the daytime bias, and results in mean differences that are within approximately 1% for both nighttime and daytime measurements.

Newsom, Rob↗
NASA NTRS2008

EAQUATE: An International Experiment for Hyper-Spectral Atmospheric Sounding Validation

The international experiment called EAQUATE (European AQUA Thermodynamic Experiment) was held in September 2004 in Italy and the United Kingdom to demonstrate certain ground-based and airborne systems useful for validating hyperspectral satellite sounding observations. A range of flights over land and marine surfaces were conducted to coincide with overpasses of the AIRS instrument on the EOS Aqua platform. Direct radiance evaluation of AIRS using NAST-I and SHIS has shown excellent agreement. Comparisons of level 2 retrievals of temperature and water vapor from AIRS and NAST-I validated against high quality lidar and drop sonde data show that the 1K/1km and 10%/1km requirements for temperature and water vapor (respectively) are generally being met. The EAQUATE campaign has proven the need for synergistic measurements from a range of observing systems for satellite cal/val and has paved the way for future cal/val activities in support of IASI on the European Metop platform and CrIS on the US NPP/NPOESS platform.

Taylor, J. P.↗
NASA NTRS2008

Evaluation of Near-Tropopause Ozone Distributions in the Global Modeling Initiative Combined Stratosphere/Troposphere Model with Ozonesonde Data

The NASA Global Modeling Initiative has developed a combined stratosphere/troposphere chemistry and transport model which fully represents the processes governing atmospheric composition near the tropopause. We evaluate model ozone distributions near the tropopause, using two high vertical resolution monthly mean ozone profile climatologies constructed with ozonesonde data, one by averaging on pressure levels and the other relative to the thermal tropopause. Model ozone is high biased at the SH tropical and NH midlatitude tropopause by approx. 45% in a 4 deg. latitude x 5 deg. longitude model simulation. Increasing the resolution to 2 deg. x 2.5 deg. increases the NH tropopause high bias to approx. 60%, but decreases the tropical tropopause bias to approx. 30%, an effect of a better-resolved residual circulation. The tropopause ozone biases appear not to be due to an overly vigorous residual circulation or excessive stratosphere/troposphere exchange, but are more likely due to insufficient vertical resolution or excessive vertical diffusion near the tropopause. In the upper troposphere and lower stratosphere, model/measurement intercomparisons are strongly affected by the averaging technique. NH and tropical mean model lower stratospheric biases are less than 20%. In the upper troposphere, the 2 deg. x 2.5 deg. simulation exhibits mean high biases of approx. 20% and approx. 35% during April in the tropics and NH midlatitudes, respectively, compared to the pressure averaged climatology. However, relative-to-tropopause averaging produces upper troposphere high biases of approx. 30% and 70% in the tropics and NH midlatitudes. This is because relative-to-tropopause averaging better preserves large cross-tropopause O3 gradients, which are seen in the daily sonde data, but not in daily model profiles. The relative annual cycle of ozone near the tropopause is reproduced very well in the model Northern Hemisphere midlatitudes. In the tropics, the model amplitude of the near tropopause annual cycle is weak. This is likely due to the annual amplitude of mean vertical upwelling near the tropopause, which analysis suggests is approx. 30% weaker than in the real atmosphere.

Considine, David B.↗
NASA NTRS2008

OMI Validation from the SAUNA and ARCTAS Campaigns

Initial results are presented on Ozone Monitoring Instrumnet (OMI) validation from the Sodankyla Total Column Ozone Intercomparison (SAUNA) and from the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) campaign. SAUNA was held in Sodankyla, Finland in March-April 2006 and February-March 2007 in support of Aura validation. The purpose of SAUNA was to assess the comparative performance of the ground-based instruments and algorithms when measuring total column ozone at large solar zenith angles and high total column ozone amounts. Results showed that the ozone profiles from the satellite instruments (MLS on Aura and SBUV/2 on NOAA 16) generally agreed with profiles from the ground-based instruments (lidar and sondes) within 10%. The ARCTAS spring campaign was flown out of Fairbanks, Alaska, from, April 1 - April 19, 2008. The purpose of ARCTAS was to study arctic haze and pollution sources in the arctic, but also to provide validation of CALIPSO and Aura. The differences between the OMI OMTO3 ozone retrieval and the DOAS ozone are examined.

McPeters, R. D.↗
NASA NTRS2008

Impact of Surface Emissions to the Zonal Variability of Tropical Tropospheric Ozone and Carbon Monoxide for November 2004

The chemical and dynamical processes governing the zonal variability of tropical tropospheric ozone and carbon monoxide are investigated for November 2004 using satellite observations, in-situ measurements, and chemical transport models in conjunction with inverse-estimated surface emissions. Vertical ozone profile estimates from the Tropospheric Emission Spectrometer (TES) and ozone sonde measurements from the Southern Hemisphere Additional Ozonesondes (SHADOZ) network show the so called zonal 'wave-one' pattern, which is characterized by peak ozone concentrations (70-80 ppb) centered over the Atlantic, as well as elevated concentrations of ozone over Indonesia and Australia (60-70 ppb) in the lower troposphere. Observational evidence from TES CO vertical profiles and Ozone Monitoring Instrument (OMI) NO2 columns point to regional surface emissions as an important contributor to the elevated ozone over Indonesia. This contribution is investigated with the GEOS-Chem chemistry and transport model using surface emission estimates derived from an optimal inverse model, which was constrained by TES and Measurements Of Pollution In The Troposphere (MOPITT) CO profiles (Jones et al., 2007). These a posteriori estimates, which were over a factor of 2 greater than climatological emissions, reduced differences between GEOS-Chem and TES ozone observations by 30-40% and led to changes in GEOS-Chem upper tropospheric ozone of up to 40% over Indonesia. The remaining residual differences can be explained in part by upper tropospheric ozone produced from lightning NOx in the South Atlantic. Furthermore, model simulations from GEOS-Chem indicate that ozone over Indonesian/Australian is more sensitive to changes in surface emissions of NOx than ozone over the tropical Atlantic.

tropical tropospheric ozone↗
NASA NTRS2007

Mechanisms for the Intraseasonal Variability of Tropospheric Ozone over the Indian Ocean during the Winter Monsoon

We synthesize daily sonde (vertical) information and daily satellite (horizontal) information to provide an empirical description of ozone origins over the northern Indian Ocean during the INDOEX (Indian Ocean Experiment) field campaign (February-March 1999). This area is shown to be a significant portion of the "high-ozone tropics". East-west O3 features and their flow are identified, and ozone origins are compared to other tropical regions, using water vapor as a second tracer. In the study period, multiple processes contribute to O3 column enhancements, their importance varying strongly by latitude: (1) Low-altitude O3 pollution over the northern Indian Ocean mainly originates from the Indian subcontinent and is traceable to high emission areas. Convective activity south of Sri Lanka helps direct ozone outflow from the northern Indian subcontinent. (2) Middle tropospheric O3 maxima over the northern Indian Ocean originate from various sources, often transitioning within a few hours. Convective venting of Asian pollutants can add 20-30 ppbv to the middle troposphere at 5degN-10degN, alternating with stratospheric influence. (3) A number of cases suggest that strong mixing-in of stratospheric air along the subtropical jet raised tropospheric O3 in early March by approx.40-50 ppbv, especially poleward of approx. 10degN. (4) Influences of lightning and large-scale biomass burning were not strong during this period, in contrast to the situation in Africa and the South Atlantic or locally in Southeast Asia. This work illustrates successes and limitations in approaches to synthesizing disparate information on trace-gas distributions taken from satellite retrieval products and ozonesondes.

Chatfield, R. b.↗
NASA NTRS2006

Controlling Herds of Cooperative Robots

A document poses, and suggests a program of research for answering, questions of how to achieve autonomous operation of herds of cooperative robots to be used in exploration and/or colonization of remote planets. In a typical scenario, a flock of mobile sensory robots would be deployed in a previously unexplored region, one of the robots would be designated the leader, and the leader would issue commands to move the robots to different locations or aim sensors at different targets to maximize scientific return. It would be necessary to provide for this hierarchical, cooperative behavior even in the face of such unpredictable factors as terrain obstacles. A potential-fields approach is proposed as a theoretical basis for developing methods of autonomous command and guidance of a herd. A survival-of-the-fittest approach is suggested as a theoretical basis for selection, mutation, and adaptation of a description of (1) the body, joints, sensors, actuators, and control computer of each robot, and (2) the connectivity of each robot with the rest of the herd, such that the herd could be regarded as consisting of a set of artificial creatures that evolve to adapt to a previously unknown environment. A distributed simulation environment has been developed to test the proposed approaches in the Titan environment. One blimp guides three surface sondes via a potential field approach. The results of the simulation demonstrate that the method used for control is feasible, even if significant uncertainty exists in the dynamics and environmental models, and that the control architecture provides the autonomy needed to enable surface science data collection.

Quadrelli, Marco B.↗
NASA NTRS2010

STROZ Lidar Results at the MOHAVE III Campaign, October, 2009, Table Mountain, CA

During October, 2009 the GSFC STROZ Lidar participated in a campaign at the JPL Table Mountain Facility (Wrightwood, CA, 2285 m Elevation) to measure vertical profiles of water vapor from near the ground to the lower stratosphere. On eleven nights, water vapor, aerosol, temperature and ozone profiles were measured by the STROZ lidar, two other similar lidars, frost-point hygrometer sondes, and ground-based microwave instruments made measurements. Results from these measurements and an evaluation of the performance of the STROZ lidar during the campaign will be presented in this paper. The STROZ lidar was able to measure water vapor up to 13-14 km ASL during the campaign. We will present results from all the STROZ data products and comparisons with other instruments made. Implications for instrumental changes will be discussed.

McGee, T. J.↗
NASA NTRS2010

Far-IR Measurements at Cerro Toco, Chile: FIRST, REFIR, and AERI

In mid-2009, the Radiative Heating in the Underexplored Bands Campaign II (RHUBC-II) was conducted from Cerro Toco, Chile, a high, dry, remote mountain plateau, 23degS , 67.8degW at 5.4km, in the Atacama Desert of Northern Chile. From this site, dominant IR water vapor absorption bands and continuum, saturated when viewed from the surface at lower altitudes, or in less dry locales, were investigated in detail, elucidating IR absorption and emission in the atmosphere. Three FTIR instruments were at the site, the Far-Infrared Spectroscopy of the Troposphere (FIRST), the Radiation Explorer in the Far Infrared (REFIR), and the Atmospheric Emitted Radiance Interferometer (AERI). In a side-by-side comparison, these measured atmospheric downwelling radiation, with overlapping spectral coverage from 5 to100um (2000 to 100/cm), and instrument spectral resolutions from 0.5 to 0.64/cm, unapodized. In addition to the FTIR and other ground-based IR and microwave instrumentation, pressure/temperature/relative humidity measuring sondes, for atmospheric profiles to 18km, were launched from the site several times a day. The derived water vapor profiles, determined at times matching the FTIR measurement times, were used to model atmospheric radiative transfer. Comparison of instrument data, all at the same spectral resolution, and model calculations, are presented along with a technique for determining adjustments to line-by-line calculation continuum models. This was a major objective of the campaign.

Cageao, Richard P.↗
NASA NTRS2011

The Observed Relationship Between Water Vapor and Ozone in the Tropical Tropopause Saturation Layer and the Influence of Meridional Transport

We examine balloonsonde observations of water vapor and ozone from three Ticosonde campaigns over San Jose, Costa Rica [10 N, 84 W] during northern summer and a fourth during northern winter. The data from the summer campaigns show that the uppermost portion of the tropical tropopause layer between 360 and 380 K, which we term the tropopause saturation layer or TSL, is characterized by water vapor mixing ratios from proximately 3 to 15 ppmv and ozone from approximately 50 ppbv to 250 ppbv. In contrast, the atmospheric water vapor tape recorder at 380 K and above displays a more restricted 4-7 ppmv range in water vapor mixing ratio. From this perspective, most of the parcels in the TSL fall into two classes - those that need only additional radiative heating to rise into the tape recorder and those requiring some combination of additional dehydration and mixing with drier air. A substantial fraction of the latter class have ozone mixing ratios greater than 150 ppbv, and with water vapor greater than 7 ppmv this air may well have been transported into the tropics from the middle latitudes in conjunction with high-amplitude equatorial waves. We examine this possibility with both trajectory analysis and transport diagnostics based on HIRDLS ozone data. We apply the same approach to study the winter season. Here a very different regime obtains as the ozone-water vapor scatter diagram of the sonde data shows the stratosphere and troposphere to be clearly demarcated with little evidence of mixing in of middle latitude air parcels.

Selkirk, Henry B.↗