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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Dimensional crossover of electron weak localization in ZnO/TiO{sub x} stacked layers grown by atomic layer deposition

We report on the dimensional crossover of electron weak localization in ZnO/TiO{sub x} stacked layers having well-defined and spatially-localized Ti dopant profiles along film thickness. These films were grown by in situ incorporation of sub-monolayer TiO{sub x} on the growing ZnO film surface and subsequent overgrowth of thin conducting ZnO spacer layer using atomic layer deposition. Film thickness was varied in the range of ∼6–65 nm by vertically stacking different numbers (n = 1–7) of ZnO/TiO{sub x} layers of nearly identical dopant-profiles. The evolution of zero-field sheet resistance (R{sub ◻}) versus temperature with decreasing film thickness showed a metal to insulator transition. On the metallic side of the metal-insulator transition, R{sub ◻}(T) and magnetoresistance data were found to be well corroborated with the theoretical framework of electron weak localization in the diffusive transport regime. The temperature dependence of both R{sub ◻} and inelastic scattering length provided strong evidence for a smooth crossover from 2D to 3D weak localization behaviour. Results of this study provide deeper insight into the electron transport in low-dimensional n-type ZnO/TiO{sub x} stacked layers which have potential applications in the field of transparent oxide electronics.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

A spatial light modulator that uses scattering in a cholesteric liquid crystal

When a cholesteric liquid crystal (helical pitch: 5 μm) was sandwiched between two glass plates with no alignment coating (gap: 20 μm), a random-domain texture appeared and a strong light scattering took place. This translucent texture turned to a transparent homeotropic phase when an electric voltage of 20 V was applied to the liquid crystal layer. This phase transition was used for constructing a spatial light modulator that needed no polarizers. Indium-tin-oxide electrodes (0.8 mm square) were arranged on a glass substrate to create a 20 × 20 pixel array (20 mm square). The liquid crystal was injected into a gap (20 μm thickness) between this substrate and another glass plate with a uniform electrode (ground). The transmittance of the pixels was originally below 10% and decreased to 0% by 7 V application because of increase in the scattering loss. As the voltage was raised, the transmittance increased gradually in the 7–17 V range and then rapidly in the 17–20 V range, attaining 40% at 27 V. Various transmittance distributions or gray-scale images were attainable by applying a suitable voltage (7–27 V) to each pixel. The transmission range of this spatial light modulator extended from ultraviolet (350 nm) to infrared wavelengths (>800 nm). Owing to this wide transmission range as well as capability of the polarizer-free operation, this spatial light modulator is useful to control a lamp spectrum in spectroscopic measurements.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2015

Alternative Binding Modes Identified for Growth and Differentiation Factor-associated Serum Protein (GASP) Family Antagonism of Myostatin

Myostatin, a member of the TGF-β family of ligands, is a strong negative regulator of muscle growth. As such, it is a prime therapeutic target for muscle wasting disorders. Similar to other TGF-β family ligands, myostatin is neutralized by binding one of a number of structurally diverse antagonists. Included are the antagonists GASP-1 and GASP-2, which are unique in that they specifically antagonize myostatin. However, little is known from a structural standpoint describing the interactions of GASP antagonists with myostatin. In this paper, we present the First low resolution solution structure of myostatin-free and myostatin-bound states of GASP-1 and GASP-2. Our studies have revealed GASP-1, which is 100 times more potent than GASP-2, preferentially binds myostatin in an asymmetrical 1:1 complex, whereas GASP-2 binds in a symmetrical 2:1 complex. Additionally, C-terminal truncations of GASP-1 result in less potent myostatin inhibitors that form a 2:1 complex, suggesting that the C-terminal domains of GASP-1 are the primary mediators for asymmetric complex formation. Overall, this study provides a new perspective on TGF-β antagonism, where closely related antagonists can utilize different ligand-binding strategies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2016

Electric dipole polarizability from first principles calculations

The electric dipole polarizability quantifies the low-energy behavior of the dipole strength and is related to critical observables such as the radii of the proton and neutron distributions. Its computation is challenging because most of the dipole strength lies in the scattering continuum. In our paper we combine integral transforms with the coupled-cluster method and compute the dipole polarizability using bound-state techniques. Furthermore, employing different interactions from chiral effective field theory, we confirm the strong correlation between the dipole polarizability and the charge radius, and study its dependence on three-nucleon forces. Finally, we find good agreement with data for the 4 He, 40 Ca, and 16 O nuclei, and predict the dipole polarizability for the rare nucleus 22 O.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Nonreciprocal Frequency Domain Beam Splitter

The canonical beam splitter—a fundamental building block of quantum optical systems—is a reciprocal element. It operates on forward- and backward-propagating modes in the same way, regardless of direction. The concept of nonreciprocal quantum photonic operations, by contrast, could be used to transform quantum states in a momentum- and direction-selective fashion. In this study, we demonstrate the basis for such a nonreciprocal transformation in the frequency domain through intermodal Bragg scattering four-wave mixing (BSFWM). Since the total number of idler and signal photons is conserved, the process can preserve coherence of quantum optical states, functioning as a nonreciprocal frequency beam splitter. We explore the origin of this nonreciprocity and find that the phase-matching requirements of intermodal BSFWM produce an enormous asymmetry ( 76 × ) in the conversion bandwidths for forward and backward configurations, yielding ~ 25 dB of nonreciprocal contrast over several hundred GHz. We also outline how the demonstrated efficiencies ( ~ 10 – 4 ) may be scaled to near-unity values with readily accessible powers and pumping configurations for applications in integrated quantum photonics.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1981

Wave direction measured by four different systems

A March 1977 wave direction measurement experiment is reported in which four systems were used to provide offshore wave-direction information: (1) synthetic aperture radar (SAR), (2) a coastal imaging radar, (3) an offshore pressure-gage array, and (4) aerial photography. From the coastal radar images and aerial photographs, the direction and length of the principal wavetrains were measured by a manual analysis. The SAR images were processed using fast Fourier transform to give two-dimensional wave spectra. Scatter diagrams are presented which intercompare the measurements of all four systems, and show good agreement among all imaging systems. It is concluded that aerial photography and SAR will prove more useful when wave measurements are needed over a large area or when there are rapidly changing wave characteristics.

Mattie, M. G.↗
NASA NTRS1981

Limiting cases of the small-angle scattering approximation solutions for the propagation of laser beams in anisotropic scattering media

The propagation of photons in a medium with strongly anisotropic scattering is a problem with a considerable history. Like the propagation of electrons in metal foils, it may be solved in the small-angle scattering approximation by the use of Fourier-transform techniques. In certain limiting cases, one may even obtain analytic expressions. This paper presents some of these results in a model-independent form and also illustrates them by the use of four different phase-function models. Sample calculations are provided for comparison purposes

Box, M. A.↗
NASA NTRS1986

Large reflector antenna study

In some applications, the wires used to construct the grids are plated over with highly conducting materials such as gold or silver. In those cases, depending on the frequency of operation, the coating may not be thick enough to prevent currents from flowing in the substrate. The conjugate gradient method, in conjunction with the fast Fourier transform is employed to solve the problem of scattering from such rectangular grids. An internal impedance is utilized to account for the effects of the substrate conductivity on the induced current densities. Calculated values of the reflection coefficient and induced currents from different coating thicknesses, angles of incidence and polarizations are presented and discussed.

Christodoulou, C. G.↗
NASA NTRS2012

Rainbow Fourier Transform

We present a novel technique for remote sensing of cloud droplet size distributions. Polarized reflectances in the scattering angle range between 135deg and 165deg exhibit a sharply defined rainbow structure, the shape of which is determined mostly by single scattering properties of cloud particles, and therefore, can be modeled using the Mie theory. Fitting the observed rainbow with such a model (computed for a parameterized family of particle size distributions) has been used for cloud droplet size retrievals. We discovered that the relationship between the rainbow structures and the corresponding particle size distributions is deeper than it had been commonly understood. In fact, the Mie theory-derived polarized reflectance as a function of reduced scattering angle (in the rainbow angular range) and the (monodisperse) particle radius appears to be a proxy to a kernel of an integral transform (similar to the sine Fourier transform on the positive semi-axis). This approach, called the rainbow Fourier transform (RFT), allows us to accurately retrieve the shape of the droplet size distribution by the application of the corresponding inverse transform to the observed polarized rainbow. While the basis functions of the proxy-transform are not exactly orthogonal in the finite angular range, this procedure needs to be complemented by a simple regression technique, which removes the retrieval artifacts. This non-parametric approach does not require any a priori knowledge of the droplet size distribution functional shape and is computationally fast (no look-up tables, no fitting, computations are the same as for the forward modeling).

Alexandrov, Mikhail D.↗
DOE OSTI2022

MENUS—Materials engineering by neutron scattering

Materials engineering by neutron scattering (MENUS) at the second target station will be a transformational high-flux, versatile, multiscale materials engineering diffraction beamline with unprecedented new capabilities for the study of complex materials and structures. It will support both fundamental and applied materials research in a broad range of fields. MENUS will combine unprecedented long-wavelength neutron flux and unique detector coverage to enable real-time studies of complex structural and functional materials under external stimuli. The incorporated small angle neutron scattering and transmission/imaging capabilities will extend its sensitivity to larger length scales and higher spatial resolution. Multimodal MENUS will provide crystallographic and microstructure data to the materials science and engineering community to understand lattice strain/phase transition/microstructure/texture evolution in three orthogonal directions in complex material systems under combined extreme applied conditions. Finally, the capabilities of MENUS will open new scientific opportunities and meet the research needs for science challenges to enable studies of a range of phenomena and answer the key questions in material design/exploration, advanced material processing, transformative manufacturing, and material operations of national impacts in our daily life.

47 OTHER INSTRUMENTATION↗
NASA NTRS2022

Characterization of Aerogel Scattering Filters for Astronomical Telescopes

We have developed a suite of novel infrared-blocking filters made by embedding scattering particles in a polymer aerogel substrate. Our developments allow us to tune the spectral performance of the filters based on both the composition of the base aerogel material and the properties of the scattering particles. Our filters are targeted for use in a variety of applications, from ground-based CMB experiments to planetary science probes. We summarize the formulations we have fabricated and tested to date, including several polyimide base aerogel formulations incorporating a range of size distributions of diamond scattering particles. We also describe the spectral characterization techniques used to measure the filters’ optical properties, including the development o fa mm-wave Fourier transform spectrometer testbed.

aerogel, filter, blocking, scattering, Fourier Tra↗
DOE OSTI2019

Pressure-Induced Transformations of Three-Component Heterostructural Nanocrystals with CdS–Au 2 S Janus Nanoparticles as Hosts and Small Au Nanoparticles as Satellites

Heterostructural nanocrystals (HNCs) have drawn enormous attention because of the combined and synergistic properties inherited from their individual components and interactions. In this paper, we design a three-component CdS-Au 2 S-Au Janus-satellite HNC to study the pressure process of HNC superlattices (HNC-SLs). In situ small/wide-angle X-ray scattering shows that the HNC-SLs can undergo structural transformations at both atomic and meso scales. At the same time, CdS-Au 2 S-Au Janus-satellite HNCs can morphologically transform into CdS-Au 2 S-Au heterotrimer HNCs through intraparticle migration and coalescence of Au satellites. Our results demonstrate that pressure can be employed as a clean and efficient way to fabricate complex heterostructural nanomaterials suitable for potential applications in photocatalysis and theranostics.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2024

Massive twistor worldline in electromagnetic fields

We study the (ambi-)twistor model for spinning particles interacting via electromagnetic field, as a toy model for studying classical dynamics of gravitating bodies including effects of both spins to all orders. We compute the momentum kick and spin kick up to one-loop order and show precisely how they are encoded in the classical eikonal. The all-orders-in-spin effects are encoded as a dynamical implementation of the Newman-Janis shift, and we find that the expansion in both spins can be resummed to simple expressions in special kinematic configurations, at least up to one-loop order. We confirm that the classical eikonal can be understood as the generator of canonical transformations that map the in-states of a scattering process to the out-states. We also remark that cut contributions for converting worldline propagators from time-symmetric to retarded amount to the iterated action of the leading eikonal at one-loop order.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2014

Complementary study of molecular dynamics and domain sizes in heterogenous nanocomposites PBT/DA-C{sub 60} and PBT/TCNEO-C{sub 60}

A comprehensive study of molecular dynamics and structure in new heterogenous nanocomposites based on poly(butylene terephthalate) and nanoparticles C{sub 60} modified by n-decylamine or tetracyanoethylene oxide has been performed. The domain structure of new nanocomposites has been investigated by Fourier transform infrared spectroscopy, wide-angle X-ray scattering, and differential scanning calorimetry techniques. Solid-state {sup 1}H NMR techniques were used to study molecular dynamics and domain sizes in new nanocomposites. Information about the electronic properties of these nanocomposites was obtained by means of electron paramagnetic resonance method. It was shown that the structure and molecular dynamics of new nanocomposites were strongly dependent on the properties and concentration of fullerene derivates.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2014

Phase transformations in multiferroic Bi{sub 1−x}La{sub x}Fe{sub 1−y}Ti{sub y}O{sub 3} ceramics probed by temperature dependent Raman scattering

Optical phonons and phase transitions of Bi{sub 1−x}La{sub x}Fe{sub 1−y}Ti{sub y}O{sub 3} (BLFTO, 0.02 ≤ x ≤ 0.12, 0.01 ≤ y ≤ 0.08) ceramics have been investigated by Raman scattering in the temperature range from 80 to 680 K. Four phase transitions around 140, 205, 570, and 640 K can be observed. The Raman modes are sensitive to the spin reorientation around 140 and 205 K, owing to the strong magnon-phonon coupling. The transformation around 570 K is a structural transition from rhombohedral to orthorhombic phase due to an external pressure induced by the chemical substitution. The anomalies of the phonon frequencies near Néel temperature T{sub N} have been discussed in the light of the multiferroicity. Moreover, it was found that the structural transition temperature and T{sub N} of BLFTO ceramics decrease towards room temperature with increasing doping composition as a result of size mismatch between substitution and host cations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Dissipative time-dependent quantum transport theory: Quantum interference and phonon induced decoherence dynamics

A time-dependent inelastic electron transport theory for strong electron-phonon interaction is established via the equations of motion method combined with the small polaron transformation. In this work, the dissipation via electron-phonon coupling is taken into account in the strong coupling regime, which validates the small polaron transformation. The corresponding equations of motion are developed, which are used to study the quantum interference effect and phonon-induced decoherence dynamics in molecular junctions. Numerical studies show clearly quantum interference effect of the transport electrons through two quasi-degenerate states with different couplings to the leads. We also found that the quantum interference can be suppressed by the electron-phonon interaction where the phase coherence is destroyed by phonon scattering. This indicates the importance of electron-phonon interaction in systems with prominent quantum interference effect.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

X-ray scattering signatures of early-time accelerations in iodine dissociation

Ultrafast time-resolved x-ray scattering (TRXS) from a photoexcited molecular ensemble measures a distribution $S(Q, τ)$ of the x-ray momentum transfer Q and pump-probe delay τ in which all modes of motion induced by the excitation overlap. Frequency-resolved x-ray scattering (FRXS) based on $\tilde {S}\left(Q,\omega \right)$ separates each oscillation and dissociation channel in the TRXS data, enabling measurements of vibrational frequencies and phases, and dissociation velocities and time shifts. In this work, we extend FRXS analysis to study early-time accelerations as well. We show how these appear as diffuse scattering patterns with characteristic phase evolution in FXRS and we develop a set of transformations that isolate individual channels to measure the early-time accelerated motion. This procedure is used to analyze diatomic iodine x-ray scattering data with multiple dissociations, and the ability of this technique to characterize early-time accelerations of one dissociation channel even in the presence of another dissociation is demonstrated.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2015

From Bessel beam to complex-source-point cylindrical wave-function

This investigation shows that a scalar Bessel beam can be transformed into the non-paraxial complex-source-point cylindrical wave (CSPCW). High-order CSPCW solutions, termed here high-order quasi-Gaussian cylindrical beams, which exactly satisfy the Helmholtz equation, are derived analytically. Moreover, partial-derivatives of the high-order CSPCW solutions satisfy the Helmholtz equation. In addition, the CSPCW solutions satisfy the nonrelativistic Schrödinger equation within standard quantum mechanics, thus, the results can be used in the description of elementary particle/matter motion and related applications in quantum scattering theory. Furthermore, the analysis is extended to the case of vector beams in which the components of the electromagnetic (EM) field are obtained based on different polarizations of the magnetic and electric vector potentials, which exactly satisfy Maxwell’s vectorial equations and Lorenz’ gauge condition. An attractive feature of the high-order solutions is the rigorous description of strongly focused (or strongly divergent) cylindrical wave-fields without any approximations, nor the need for numerical methods. Possible applications are in beam-forming design using high-aperture or collimated cylindrical laser/electron quasi-Gaussian beams in imaging microscopy, particle manipulation, optical tweezers, and the study of the scattering, and radiation forces on objects. - Highlights: • Bessel beam is transformed into the non-paraxial cylindrical complex-source-point. • Exact high-order tightly focused solutions are derived without any approximations. • The exact solutions also satisfy the nonrelativistic Schrödinger equation. • Electromagnetic beams are obtained as solutions of Maxwell’s vectorial equations. • Applications are in laser/electron beam imaging, tweezers, and radiation force.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗