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At least 271 records · Page 15

Overview/Recap of the 2020 Accelerated Irradiation of Reactor Structural Materials Workshop

The workshop provided a snapshot look at current international, in-reactor testing and irradiation capabilities. Gaps were identified where possible, and discussions focused on potential mitigation strategies and recommended paths forward. As new material innovations are being developed for in-reactor applications for reactor life extension long-term operation, and advanced reactor technologies, there is an increased need for materials qualification and assessment programs. In-reactor testing capabilities are vital to the on-going success of these DOE-NE programs and initiatives. In recent years, multiple international research reactors have been placed in a permanent shut-down state and have begun full decommissioning. These activities have created new risks in the delivery of on-going and/or expected research programs. Beyond performing simple irradiations in test reactors, few facilities exist internationally which can perform instrumented, in-situ irradiations on structural materials, and with the recent shut down of facilities hosted at Halden and NRU (example: instrumented fatigue loop, and in-situ creep), there are further gaps in the industry left un-filled. A new focus is being placed on the use of accelerator- based technologies to fill in some of these gaps, but these must be viewed as supplemental, and not surrogates to in-reactor capabilities

36 - MATERIALS SCIENCE↗

Assessment of Near-Term Fuel Screening and Qualification Needs for Nuclear Thermal Propulsion Systems

Nuclear thermal propulsion (NTP) is an in-space propulsion technology capable of both high specific impulse (850–1000 s) and thrust (44–1112 kN), which can help reduce trip times for crewed missions beyond low Earth orbit. NTP technology has been demonstrated during historic programs. Over 20 ground test reactor experiments were performed, which demonstrated the prototypic reactor operations, during the Nuclear Engine for Rocket Vehicle Application (NERVA)/Rover program (1955–1972). Although historical programs have shown that NTP is a viable in-space propulsion technology, developing NTP in modern programs is contingent on the development and qualification of ultrahigh-temperature nuclear fuel technologies that can withstand engine operating conditions. In historical NTP development programs such as NERVA/Rover, prototypic reactor/engine schemes were ground tested to assess the overall system feasibility and to qualify the reactor fuel forms for eventual flight systems. Although this approach is effective to verify fuel performance under prototypic conditions, relying solely on full-scale NTP reactor tests as the pathway for verifying or qualifying fuel is inefficient and cost prohibitive today. Additionally, modern nuclear licensing requirements state that before test reactor approval, reactor components and fuel elements should be qualified via non-nuclear (out-of-pile) and nuclear (in-pile) testing under representative operating conditions. Using this methodology, fuel matures as production scale fabrication methods are established, and as produced fuel performance is demonstrated. Here, this paper provides an overview of historical approaches to NTP fuel performance maturation, including fuel screening and qualification needs, and provides insight for establishing an efficient testing paradigm that can be implemented to rapidly and affordably develop NTP fuel forms for eventual qualification.

42 ENGINEERING↗

Irradiation performance of nonfertile (Pu-MA-Zr) fast reactor metal fuels

This work was part of a program begun in 2001 to develop advanced nuclear fuels, originally as carriers for plutonium and minor actinides (neptunium, curium, and americium) taken from spent commercial light-water reactors (LWR) so that the plutonium and minor actinides could be ‘burned’ or transmuted in an accelerator or a fast nuclear reactor. A central part of these experiment programs has been the development of advanced fast reactor fuels, because a fast reactor was considered the most efficient vehicle to transmute the actinide waste products, and metallic fuels is a central focus of these tests. An experiment design was developed in which a thermal test reactor, the Advanced Test Reactor (ATR), was used to test small fuel pin prototypes, by creating areas in the core shielded by cadmium filters to produce a largely epithermal and fast neutron spectrum environment in which the pins could be irradiated. The results of non-fertile metallic fuel (no uranium) tests are presented here. Pu-Am-Np-Zr fuels were irradiated to fission densities up to 33 × 10 20 fission/cm 3 and Pu-239 depletions of up to 39%. The depletions were created by roughly 2/3 by fission and 1/3 by transmutation neutron capture. Up to five fuel ‘rodlets’ were irradiated in three sealed capsules stacked axially in the core, and the peak cladding temperatures ranged from 300°C to 500°C, depending on axial location as those near the core centerline are operating hotter and to higher fission densities. Several post-irradiation examinations (precision gamma scanning and fission gas release) were similar to other historical metal fuel experiments in fast reactors. However, optical metallography indicated that two of the rodlets had breached. The exact reasons are unclear. Due to the design of this irradiation experiment a rodlet breach could have increased the temperature in others in the same capsule by contaminating the thermal gap helium with heavier and less conductive fission product gases. Finally, some of those rodlets showed high amounts of fuel/cladding chemical interaction (FCCI).

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Progress Towards Developing Neutron Tolerant Magnetostrictive and Piezoelectric Transducers

Current generation light water reactors (LWRs), sodium cooled fast reactors (SFRs), small modular reactors (SMRs), and next generation nuclear plants (NGNPs) produce harsh environments in and near the reactor core that can severely tax material performance and limit component operational life. To address this issue, several Department of Energy Office of Nuclear Energy (DOE-NE) research programs are evaluating the long duration irradiation performance of fuel and structural materials used in existing and new reactors. In order to maximize the amount of information obtained from Material Testing Reactor (MTR) irradiations, DOE is also funding development of enhanced instrumentation that will be able to obtain in-situ, real-time data on key material characteristics and properties, with unprecedented accuracy and resolution. Such data are required to validate new multi-scale, multi-physics modeling tools under development as part of a science-based, engineering driven approach to reactor development. It is not feasible to obtain high resolution/microscale data with the current state of instrumentation technology. However, ultrasound-based sensors offer the ability to obtain such data if it is demonstrated that these sensors and their associated transducers are resistant to high neutron flux, high gamma radiation, and high temperature. To address this need, the Advanced Test Reactor National Scientific User Facility (ATR-NSUF) is funding an irradiation, led by PSU, at the Massachusetts Institute of Technology Research Reactor to test the survivability of ultrasound transducers. As part of this effort, PSU and collaborators have designed, fabricated, and provided piezoelectric and magnetostrictive transducers that are optimized to perform in harsh, high flux, environments. Four piezoelectric transducers were fabricated with either aluminum nitride, zinc oxide, or bismuth titanate as the active element that were coupled to either Kovar or aluminum waveguides and two magnetostrictive transducers were fabricated with Remendur or Galfenol as the active elements. Pulse-echo ultrasonic measurements of these transducers are made in-situ. This paper will present an overview of the test design including selection criteria for candidate materials and optimization of test assembly parameters, data obtained from both out-of-pile and in-pile testing at elevated temperatures, and an assessment based on initial data of the expected performance of ultrasonic devices in irradiation conditions

Reinhardt1, Brian↗

Critical response to M. Worrall et al. Published in Annals of Nuclear Energy 207 (2024) 110731

M. Worrall et al. recently published a manuscript titled “Fast neutron irradiation capability in existing thermal test reactors” (Worrall, 2024) that summarizes an irradiation vehicle design that would boost the fast neutron flux in the Advanced Test Reactor (ATR) for testing of nonfuel materials in a neutron flux energy spectrum that is more representative of fast reactors. Here, the authors compare their design with a separate vehicle design that they conceived of that would be implemented within the High Flux Isotope Reactor (HFIR). They analyzed both designs and drew conclusions on the most realistic near-term options for shielded nonfuel material irradiations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

A User Guide to PARET/ANL

PARET was originally created in 1969 at what is now Idaho National Laboratory (INL), to analyze reactivity insertion events in research and test reactor cores cooled by light or heavy water, with fuel composed of either plates or pins. The use of PARET is also appropriate for fuel assemblies with curved fuel plates when their radii of curvatures are large with respect to the fuel plate thickness. The PARET/ANL version of the code has been developed at Argonne National Laboratory (ANL) under the sponsorship of the U.S. Department of Energy/NNSA since the inception of the Reactor Conversion Program. Since Reduced Enrichment for Research and Test Reactors (RERTR) began in 1978, PARET/ANL has been benchmarked to experimental data including SPERT testing, and used to determine the expected transient behavior of many reactors both inside and outside the Reactor Conversion Program. This document provides the pertinent information for the use of PARET/ANL Version 7.6.

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PARET/ANL v7.7 User Guide

PARET was originally created in 1969 at what is now Idaho National Laboratory (INL), to analyze reactivity insertion events in research and test reactor cores cooled by light or heavy water, with fuel composed of either plates or pins. The use of PARET is also appropriate for fuel assemblies with curved fuel plates when their radii of curvatures are large with respect to the fuel plate thickness. The PARET/ANL version of the code has been developed at Argonne National Laboratory (ANL) under the sponsorship of the U.S. Department of Energy/NNSA since the inception of the Reactor Conversion Program. Since Reduced Enrichment for Research and Test Reactors (RERTR) began in 1978, PARET/ANL has been benchmarked to experimental data including SPERT testing, and used to determine the expected transient behavior of many reactors both inside and outside the Reactor Conversion Program. This document provides the pertinent information for the use of PARET/ANL v7.7.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

A User Guide to PARET/ANL

PARET was originally created in 1969 at what is now Idaho National Laboratory (INL), to analyze reactivity insertion events in research and test reactor cores cooled by light or heavy water, with fuel composed of either plates or pins. The use of PARET is also appropriate for fuel assemblies with curved fuel plates when their radii of curvatures are large with respect to the fuel plate thickness. The PARET/ANL version of the code has been developed at Argonne National Laboratory (ANL) under the sponsorship of the U.S. Department of Energy/NNSA since the inception of the Reactor Conversion Program. Since Reduced Enrichment for Research and Test Reactors (RERTR) began in 1978, PARET/ANL has been benchmarked to experimental data including SPERT testing, and used to determine the expected transient behavior of a large number of reactors regardless of enrichment both inside and outside the Reactor Conversion Program. This document provides the pertinent information for the use of PARET/ANL Version 7.6. PARET/ANL models the various fueled regions of a reactor core as channels. Each of these channels consists of a single flat fuel plate/pin (including cladding and, optionally, a gap) with water coolant on each side. In slab geometry the coolant channels for a given fuel plate are of identical dimensions (mirror symmetry), but they can be of different thickness in each channel. There can be many channels, but each channel is independent and coupled only through reactivity feedback effects to the whole core. The time-dependent differential equations that represent the system are replaced by an equivalent set of finite-difference equations in space and time, which are integrated numerically. PARET/ANL uses fundamentally the same numerical scheme as RELAP5 for the time-integration of the point-kinetics equations. The one-dimensional thermal-hydraulic model includes temperature-dependent thermal properties of the solid materials, such as heat capacity and thermal conductivity, as well as the transient heat production and heat transfer from the fuel meat to the coolant. Temperature- and pressure-dependent thermal properties of the coolant such as enthalpy, density, thermal conductivity, and viscosity are also used in determining parameters such as friction factors and heat transfer coefficients. The code first determines the steady-state solution for the initial state. Then the solution of the transient is obtained by integration in time and space. Multiple heat transfer, DNB and flow instability correlations are available. The code was originally developed to model reactors cooled by an open loop, which was adequate for rapid transients in pool-type cores. An external loop model appropriate for Miniature Neutron Source Reactors (MNSR’s) was also added to PARET/ANL to model natural circulation within the vessel, heat transfer from the vessel to pool and heat loss by evaporation from the pool. PARET/ANL also contains models for decay heat after shutdown, control rod reactivity versus time or position, time-dependent pump flow, and loss-of-flow event with flow reversal as well as logic for trips on period, power, and flow. Feedback reactivity effects from coolant density changes and temperature changes are represented by tables. Feedback reactivity from fuel heat-up (Doppler Effect) is represented by a four-term polynomial in powers of fuel temperature. Photo-neutrons produced in beryllium or in heavy water may be included in the point-kinetics equations by using additional delayed neutron groups.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Challenges and Solutions for Fast Neutron Irradiation of Bulk Material Specimens

Reactor developers continue to recognize opportunities for further enhancing fast spectrum reactor designs with advanced core materials, but all the material test reactors currently available to the United States are thermal spectrum designs. Fortunately, the Advanced Test Reactor and High Flux Isotope Reactor are versatile high flux facilities where spectral modification strategies can be used to reduce undesirable thermal neutron capture transmutation damage and augment fast flux delivered to specimens. New opportunities to leverage high flux regions and specially designed fast flux boosting experiment configurations can be used to achieve meaningful fast fluences on large specimens in ATR. New optimization potentials can be employed to achieve even higher fluences, albeit for smaller specimens, using thermal neutron filters in HFIR test positions. These capabilities, while not true fast reactors, can provide highly relevant environments for researchers needing to study the effects of fast neutron damage in bulk material specimens.

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High-temperature irradiation-resistant thermocouple instability model for in-pile reactor use

This article presents an instability model for the high-temperature irradiation-resistant thermocouple (HTIR-TC). Here the term instability defines the superposition of both drift and inhomogeneity of TC thermoelements occurring simultaneously. The HTIR-TC is an advanced thermocouple (TC) that uses the refractory metals niobium and molybdenum as sensing thermoelements for generating electromotive force (EMF) in a field of neutrons and at temperatures upward of 1,600°C. In the Advanced Gas Reactor (AGR) 5/6/7 tests conducted at Idaho National Laboratory’s Advanced Test Reactor (ATR), the HTIR-TCs showed low to moderate instability throughout the life of the test. The instability model reveals that HTIR-TCs can, when the operating temperature of the reactor fuel is normal, maintain performance throughout an 18-month refueling cycle typical of nuclear power plants, reflecting an instability of less than ±1%. The HTIR-TC is also qualified for incorporation into a test fixture during the testing of new fuels.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Irradiations for Advanced Reactors

The presentation is for a public seminar explaining test reactor capabilities for testing advanced reactor fuels and materials

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Bridging microscale to macroscale mechanical property measurements and predication of performance limitation for FeCrAl alloys under extreme reactor applications

Microscale mechanical testing has greatly benefited nuclear materials studies in at least two aspects: one is its feasibility to integrate with SEM and TEM microscopes for in situ atomic scale or microscale structural characterization to reveal fundamental details, and the other is its significance in development of accelerator-based ion irradiation technique as a surrogate method to simulate neutron damage. Ion irradiation is able to reach damage creation at a level at least three orders of magnitudes higher than test reactors. However, limited ion penetration depths, which are about a few microns for MeVs heavy ions and 10s microns for MeV light ions, make microscale mechanical tests a necessity. But, there is a great challenge to bridge microscale tests to macroscale tests because a bulk specimen of irradiated nuclear materials for high dose applications cannot be obtained in laboratory.

36 MATERIALS SCIENCE↗

Bridging microscale to macroscale mechanical property measurements and predication of performance limitation for FeCrAl alloys under extreme reactor applications

Microscale mechanical testing has greatly benefited nuclear materials studies in at least two aspects: one is its feasibility to integrate with SEM and TEM microscopes for in situ atomic scale or microscale structural characterization to reveal fundamental details, and the other is its significance in development of accelerator-based ion irradiation technique as a surrogate method to simulate neutron damage. Ion irradiation is able to reach damage creation at a level at least three orders of magnitudes higher than test reactors. However, limited ion penetration depths, which are about a few microns for MeVs heavy ions and 10s microns for MeV light ions, make microscale mechanical tests a necessity. But, there is a great challenge to bridge microscale tests to macroscale tests because a bulk specimen of irradiated nuclear materials for high dose applications cannot be obtained in laboratory.

36 MATERIALS SCIENCE↗

Testing and Simulation of an Updated Cartridge Loop Vehicle

The Versatile Test Reactor (VTR) is a sodium-cooled, fast-spectrum test reactor that is being developed in the United States and will support a variety of irradiation test vehicle configurations, including cartridge loops. This work includes out-of-pile experimental results from a single-phase, natural circulation cartridge loop vehicle with geometry relevant to VTR irradiation sites, as well as comparisons between the experimental results and results predicted using the TRAC/RELAP Advanced Computational Engine (TRACE) modeling tool. The experiments were conducted in the thermosyphon test loop (TSTL) facility at Oak Ridge National Laboratory. Comparisons are also made between the current experimental data and results from natural circulation experiments previously conducted in the TSTL in a cartridge vehicle that is similar in design but has smaller flow areas. This cartridge vehicle and the experimental program were developed to add to the single-phase, natural circulation data collected in the previous iteration of the cartridge loop design, which supports future irradiation experiments and adds to a database that is useful for validating computer models. Comparisons of experimental results to TRACE model predictions is a pertinent step in validating the computational tool for supporting future irradiation experiment design and safety calculations, and comparisons to previous cartridge loop results highlight the impact of the design changes made to the test vehicle. The experiments conducted include several steady state tests and transients, including power ramp, loss of offsite power, and loss of external flow scenarios. This work shows that TRACE can accurately predict temperatures and flow conditions in the cartridge loop and the updated vehicle design achieves higher mass flow rates at the same steady state power levels.

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COR-0011 Rev 6 MARVEL Project Code of Record

This Code of Record identifies the codes, standards, and procedures necessary to design, develop, construct, and startup the Microreactor Applications Research Validation and Evaluation (MARVEL) Project at the Materials and Fuel Complex (MFC) Transient Reactor Test (TREAT) Facility and the Idaho National Laboratory (INL). The MARVEL Project is an INL test microreactor funded by the United States Department of Energy (DOE) via the Microreactor Program (MRP). The goal of the project is to establish an operational nuclear applications test bed that can generate combined heat and power to enable integration and R&D with end-user technologies, as well as allow microreactor technologists to test next-generation control systems. The microreactor is a thermal reactor utilizing Uranium Zirconium Hydride (UZrH) fuel with review and authorization by the Department of Energy Idaho Operations Office (DOE-ID) for National Environmental Policy Act (NEPA) compliance, safety review, and supplemental readiness assessments for startup and operation. To enable rapid deployment, the MARVEL reactor will reside in the Transient Reactor Test (TREAT) Facility and utilize the existing operating Category B reactor facility, approved facility safety basis, operating crews, and recent re-start experience.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Establishing Maximal Core Excess Reactivity Envelope for TREAT Test Vehicle Insertion

The Transient Reactor Test (TREAT) Facility is an air-cooled reactor composed of graphite-urania fuel encapsulated in zirconium alloy canisters and surrounded by ~2 ft (~61 cm) of nuclear grade graphite. The primary role of TREAT is to provide in-pile nuclear-heated safety research via transient testing [1]. The following work represents further analyses building upon previously reported work to support larger volume test vehicles within TREAT [2]. The Broad Use Specimen Transient Experiment Rig (BUSTER) provides ample versatility for numerous transient test concepts. However, future testing and experiment needs will require testing environments of different in-core footprints. The versatility of TREAT allows for the development of variegated core layouts with key limitations emplaced as operational safety temperature restrictions and available core reactivity. The focus of this current effort is to gauge core arrangements for TREAT core loadings to support centralized experimental testing of varying dimensional capacity. The total core excess reactivity (ER) was computed for different arrangements to establish comparison tables that enable ready assessment of core ER available for future experiment concepts. Test vehicle worths would then be necessary to establish available ER to support transient testing requirements and to perform reactor performance and safety calculations [3,4].

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Developing Separate Effects Transient Test Experiments Using an Out-of-Pile Flowing Water Loop

In 2017 the Transient Reactor Test Facility was restarted after being placed in a standby state since 1994. This Test Reactor’s restart has since enabled the progressive development of new nuclear technologies within the U.S. that were previously required to outsource to other countries. While the reactor’s restart was a large feat worthy of recognition, the experimental use of its characteristics has required the further development of in-pile experimental infrastructure sufficient to support programmatic needs. This hardware have taken the form of capsule designs (compact and elongated) as well as loop concepts representing the phenomena of interest for a subset of separate effects tests desire for each respective testing campaign. The Transient Testing Program has a large-integrated effort that aligns with the U.S. Department of Energy’s current needs. This study compliments those programmatic elements by developing, fabricating and demonstrating a full-scale flowing water loop in an out-of-pile environment. The goal of this effort is to develop a pragmatic understanding of the engineering capabilities and limitations associated with geometric form-factors, metering technology, and controls logic under representative thermal hydraulic conditions that would be experienced within the TREAT reactor during an in-pile reactivity initiated accident test. The outcomes of this study result in an evaluation of the conceptual design of a comprehensive flowing water loop including objective figures of merit (FoMs) for comparing unique instrumentation and the basis for their selection during operations. These efforts directly contribute to and are required for the further advancement of transient testing capabilities within the U.S.

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