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NASA NTRS2014

Revised (Mixed-Effects) Estimation for Forest Burning Emissions of Gases and Smoke, Fire/Emission Factor Typology, and Potential Remote Sensing Classification of Types for Ozone and Black-Carbon Simulation

We summarize recent progress (a) in correcting biomass burning emissions factors deduced from airborne sampling of forest fire plumes, (b) in understanding the variability in reactivity of the fresh plumes sampled in ARCTAS (2008), DC3 (2012), and SEAC4RS (2013) airborne missions, and (c) in a consequent search for remotely sensed quantities that help classify forest-fire plumes. Particle properties, chemical speciation, and smoke radiative properties are related and mutually informative, as pictures below suggest (slopes of lines of same color are similar). (a) Mixed-effects (random-effects) statistical modeling provides estimates of both emission factors and a reasonable description of carbon-burned simultaneously. Different fire plumes will have very different contributions to volatile organic carbon reactivity; this may help explain differences of free NOx(both gas- and particle-phase), and also of ozone production, that have been noted for forest-fire plumes in California. Our evaluations check or correct emission factors based on sequential measurements (e.g., the Normalized Ratio Enhancement and similar methods). We stress the dangers of methods relying on emission-ratios to CO. (b) This work confirms and extends many reports of great situational variability in emissions factors. VOCs vary in OH reactivity and NOx-binding. Reasons for variability are not only fuel composition, fuel condition, etc., but are confused somewhat by rapid transformation and mixing of emissions. We use "unmixing" (distinct from mixed-effects) statistics and compare briefly to approaches like neural nets. We focus on one particularly intense fire the notorious Yosemite Rim Fire of 2013. In some samples, NOx activity was not so suppressed by binding into nitrates as in other fires. While our fire-typing is evolving and subject to debate, the carbon-burned delta(CO2+CO) estimates that arise from mixed effects models, free of confusion by background-CO2 variation, should provide a solid base for discussion. (c) We report progress using promising links we find between emissions-related "fire types" and promising features deducible from remote observations of plumes, e.g., single scatter albedo, Angstrom exponent of scattering, Angstrom exponent of absorption, (CO column density)/(aerosol optical depth).

Remote sensing↗

NASA NTRS1998

Validation of POLDER/ADEOS data using a ground-based lidar network: Preliminary results for semi-transparent and cirrus clouds

At mid and tropical latitudes, cirrus clouds are present more than 50% of the time in satellites observations. Due to their large spatial and temporal coverage, and associated low temperatures, cirrus clouds have a major influence on the Earth-Ocean-Atmosphere energy balance through their effects on the incoming solar radiation and outgoing infrared radiation. At present the impact of cirrus clouds on climate is well recognized but remains to be asserted more precisely, for their optical and radiative properties are not very well known. In order to understand the effects of cirrus clouds on climate, their optical and radiative characteristics of these clouds need to be determined accurately at different scales in different locations i.e. latitude. Lidars are well suited to observe cirrus clouds, they can detect very thin and semi-transparent layers, and retrieve the clouds geometrical properties i.e. altitude and multilayers, as well as radiative properties i.e. optical depth, backscattering phase functions of ice crystals. Moreover the linear depolarization ratio can give information on the ice crystal shape. In addition, the data collected with an airborne version of POLDER (POLarization and Directionality of Earth Reflectances) instrument have shown that bidirectional polarized measurements can provide information on cirrus cloud microphysical properties (crystal shapes, preferred orientation in space). The spaceborne version of POLDER-1 has been flown on ADEOS-1 platform during 8 months (October 96 - June 97), and the next POLDER-2 instrument will be launched in 2000 on ADEOS-2. The POLDER-1 cloud inversion algorithms are currently under validation. For cirrus clouds, a validation based on comparisons between cloud properties retrieved from POLDER-1 data and cloud properties inferred from a ground-based lidar network is currently under consideration. We present the first results of the validation.

Chepfer, H.↗

NASA NTRS2021

Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) Science Plan

Coastal cities provide the opportunity to characterize marine clouds and the substantial effects of manmade particles on cloud properties and processes. La Jolla lies to the north of San Diego, California, but it is often about a day directly downwind of the major pollution sources located in the ports of Los Angeles and Long Beach. The large dynamic range of aerosol particle concentrations combined with the multi-hour to multi-day persistence of stratocumulus cloud layers makes the site ideal for investigating the seasonal changes in cloud and aerosol properties as well as the quantitative relationships between cloud and aerosol properties. The focus of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) is to characterize the extent, radiative properties, aerosol interactions, and precipitation characteristics of stratocumulus clouds in the Eastern Pacific across all four seasons at a coastal location, the Scripps Pier and the Scripps Mt. Soledad sites in La Jolla. An important enhancement to this study will be the collection of simultaneous in-cloud aerosol and droplet measurements to investigate the differences in these cloud properties during regional polluted and clean marine conditions. The combined observations will provide an unprecedented set of constraints for the following questions: 1. Cloud and Aerosol Climatology: What are the seasonal and diurnal cycles of marine stratocumulus cloud and aerosol properties on the northeastern Pacific coast? 2. Cloud Radiative Fluxes: How do cloud properties, including the ratio of direct-to-diffuse radiation, change as coastal clouds are advected inland? 3. Aerosol-Cloud Interactions: Will retrieved cloud properties reflect the regional signatures of aerosol?

Eastern Pacific Cloud Aerosol Precipitation Experi↗

NASA NTRS1969

Theoretical evaluation of the simulation of radiative heating of planetary entry vehicles.

Shock layer properties, radiative and convective heat transfer about two hypersonic blunt bodies at zero angle of attack in assumed Martian atmosphere

Dohner, C. V.↗

DOE OSTI2022

Thermal radiation analysis of a pressurized oxy-coal combustor with discrete ordinate model

Concerns over climate change have led to numerous efforts in developing low-carbon energy technologies. Pressurized oxy-combustion (POC) is a promising candidate to reduce carbon emissions in power generation. Pressure strongly impacts thermal radiation, leading to a substantial difference in heat transfer between POC and conventional atmospheric pressure combustion. A good understanding of thermal radiation in POC is needed to aid new combustor development. The present work is a step in this direction, initiating a systematic analysis of thermal radiation and heat transfer in a pilot-scale POC combustor, which has been developed at Washington University in St. Louis (WUSTL). In a POC process, pulverized coal is burned under elevated pressure and O2-CO2 environment. Few researchers have investigated the thermal radiation of pressurized oxy-combustion. This work adopted the discrete ordinate model to simulate the radiation of a 1-D cylinder with predetermined conditions (temperature, pressure, gas compositions) to predict the influence of radiative properties of flue gas on the radiation in the combustor.

Li, Lei↗

NASA NTRS2004

Small-Scale Variability of Large Cloud Drops

Cloud droplet size distribution is one of the most fundamental subjects in cloud physics. Understanding of spatial distribution and small-scale fluctuations of cloud droplets is essential for both cloud physics and atmospheric radiation. For cloud physics, it relates to the coalescence growth of raindrops while for radiation, it has a strong impact on a cloud's radiative properties. Most of the existing cloud radiation and precipitation formation models assume that the mean number of drops with a given radius varies proportionally to volume. The analysis of microphysical data on liquid water drop sizes shows that, for sufficiently small volumes, the number is proportional to the drop size dependent power of the volume. For abundant small drops present, the exponent is 1 as assumed in the conventional approach. However, for rarer large drops, the exponents fall below unity. At small scales, therefore, the mean number of large drops decreases with volume at a slower rate than the conventional approach assumes, suggesting more large drops at these scales than conventional models account for; their impact is consequently underestimated. Size dependent models of spatial distribution of cloud drops that simulate the observed power laws show strong drop clustering, the more so the larger the drops. The degree of clustering is determined by the observed exponents. The strong clustering of large drops arises naturally from the observed power-law statistics. Current theories of photon-cloud interaction and warm rain formation will need radical revision in order to produce these statistics; their underlying equations are unable to yield the observed power law.

Marshak, Alexander↗

NASA NTRS2004

Contrail Coverage Over the USA Derived from NOAA and EOS Satellite Data

Contrails, like natural cirrus clouds, can cause a warming of the Earth-atmospheric system by absorbing longwave radiation from the surface and lower troposphere and radiating additional radiation back to the surface. They can also produce some cooling of the surface during the daytime by reflecting some sunlight back to space. Recently, Minnis et al. (2004) determined from surface observations of cirrus cloud cover that the overall impact appears to be a warming that is consistent with theoretical calculations, at least over the United States of America (USA) and surrounding areas. This finding highlights the need to better understand the formation and persistence of contrails and their radiative properties. To better assess the climatic impact of contrails, it is essential to determine the variability of the contrail microphysical properties, their impact on the atmospheric radiation budget, and their relationship to the atmospheric state. To that end, this paper continues the analyses of Advanced Very High Resolution Radiometer (AVHRR) data from the NOAA-15 (N15), NOAA-16 (N16), and NOAA-17 (N17) satellites, Moderate Resolution Imaging Spectroradiometer (MODIS) data from the Terra and Aqua satellites. The combination of these satellites provides a relatively comprehensive coverage of the daily cycle of air traffic. Thus, it should be possible to use these data to help understand the impact of air traffic on the upper tropospheric humidity during the day as well as determine the local-time variability of contrail coverage. The results will be valuable for developing models of contrail effects and methods for mitigating the impact of aviation on climate.

Palikonda, Rabindra↗

NASA NTRS1997

Characterization of Aircraft Produced Soot and Contrails Near the Tropopause

Participation in the SUCCESS project primarily involved development and deployment of specific instruments for characterizing jet aircraft exhaust emissions as particulates and their subsequent evolution as contrail particles, either liquid or solid, as cirrus. Observations can be conveniently considered in two categories - close or distant from the aircraft. Thus close to the aircraft the exhaust is mixing through the engine turbulence with a much drier and colder environment and developing water/ ice supersaturation along the trail depending on circumstances (near field), whereas distant from the aircraft (far field) the exhaust has cooled essentially to ambient temperature, the turbulence has decayed and any particle growth or evaporation is controlled by the prevailing ambient conditions. Intermediate between these two regions the main aircraft vortices form (one on each side of the aircraft) which tend to inhibit mixing under some conditions, a region extending from a few aircraft lengths to sometimes a hundred times this distance. Our approach to the problem lay in experience gained in characterizing the smoke from hydrocarbon combustion in terms of its cloud forming properties and its potential influence on the radiation properties of the smoke and subsequent cloud from the viewpoint of reduction (absorbtion and scattering ) of solar radiation flux leading to significant global cooling (Hudson et al 1991; Hallett and Hudson 1991). Engine exhaust contains a much smaller proportion of the fuel carbon than is sometimes present in ordinary combustion (less than 0.01% compared with 10%) and influences condensation in quite different ways, to be characterized by the Cloud Condensation Nucleus, CCN - supersaturation spectrum. The transition to ice is to be related to the dilution of solution droplets to freeze by homogeneous nucleation at temperatures somewhat below -40C (Pueschel et al 1998). The subsequent growth of ice particles depends critically on temperature, supersaturation and to some extent pressure, as is demonstrated in an NSF funded project being carried out in parallel with the work reported here. As will be discussed below, nucleation processes themselves and also exhaust impurities also influence the growth of ice particles and may control some aspects of growth of ice in contrails. Instrumentation was designed to give insight into these questions and to be flown on the NASA DC- 8 as a platform. In addition a modest program was undertaken to investigate the properties of laboratory produced smoke produced under controlled conditions from the viewpoint of forming both CCN and CN. The composition of the smoke could inferred from a thermal characterization technique; larger particles were captured by formvar replicator for detailed analysis; ice particles were captured and evaporated in flight on a new instrument, the cloudscope, to give their mass, density and impurity content.

Hallett, John↗

NASA NTRS1968

Measurements report - Thermal property measurements of Manned Spacecraft Center spacesuit materials

Thermal radiation properties of Lexan and other space suit materials

Turnbow, F. J.↗

NASA NTRS1970

Instrumentation for measuring flow properties in an explosively driven shock tube

Flow and radiative properties of air in high explosive shock tube

Borucki, W. J.↗

NASA NTRSDate not supplied

Coupling of Dust Mineralogy to Radiation in NASA GISS ModelE: Impact Upon Dust Optical Properties and Direct Radiative Effect

Estimates of dust direct radiative effect (DRE) are still largely uncertain mainly due to the poor constraining of regional variations of dust absorption, whose known connection with mineral composition is still largely neglected by most Earth System Models. The inaccurate knowledge of soil mineralogy and insufficient measurements of dust physical and optical properties still present the main challenges for a proper representation of the dust-radiation interaction in climate models. We recently upgraded the coupling of dust minerals to shortwave radiation in the NASA GISS ModelE. In particular, we extended the interaction to online-calculated minerals and implemented two different mixing configurations: i) external mixing of three main mineral components and ii) internal mixing of all minerals, allowing a dynamic fraction of iron oxides. We used a semi-empirical approach for the optical calculations, mostly based on aerosol chamber measurements from natural soils, aiming to reduce the influence of uncertain assumptions on the optical properties and mixing state of individual minerals. In this contribution, we present the results of our first calculations of dust optical properties and DREs based on different mixing configurations of interactive minerals. We show the changes to dust optical depth and single scattering albedo, with respect to the control case using homogeneous dust composition, and the consequent global and regional variations in dust DREs at the top of atmosphere and at surface. We also compare the model optical properties with AERONET data, filtered to identify dust scenes. We find that accounting for the diverse properties of dust minerals modifies the pattern of regional dust absorption and therefore its impact upon climate. We also show that the mineralogy effect is sensitive to the assumed mixing state of minerals.

dust direct radiative effect↗

NASA NTRSDate not supplied

Cloud Climate Data Records from Geostationary Satellites to Support CERES: Challenges and Recent Progress

clouds↗

NASA NTRSDate not supplied

Development of a Consistent GEOsat Cloud Property Dataset for the CERES Climate Data Record

Cloud properties are critical for understanding the Earth’s radiation budget and cloud feedbacks. At NASA Langley Research Center, the Satellite ClOud and Radiative Property retrieval System (SatCORPS) provides real-time and historical analyses of clouds derived from Geostationary satellite (GEOsat) data for weather and climate applications. For the Clouds and the Earth’s Radiant Energy System (CERES) program, the global constellation of GEOsats has been analyzed since 2000 to help characterize and account for the diurnal cycle of clouds and their radiative impacts in the CERES climate data record. Obtaining consistent cloud properties over the GEOsat data record during the CERES era is a major objective but a significant challenge considering the diversity of imaging capabilities deployed during that time. The GEOsat data analysis approach for the current CERES Edition-4 (Ed4) data products was focused on accuracy and consistency with MODIS by employing as much spectral information as possible from each satellite. However, the inconsistent use of spectral information across GEOsats led to marked discontinuities in the spatial and temporal record of cloud properties that had to be accounted for post facto in downstream CERES processing. This paper reports progress in developing a new GEOsat analysis system for the next CERES edition (Ed5) that has potential to improve cross-platform consistency and continuity. In this approach, the spectral channel complement is limited to just 3-channels during daytime, ~0.65 µm (VIS), ~3.9 µm (NIR), and ~10.8 µm (IR), common to nearly all of the satellites in the record. At night, a 2-channel approach is taken with the NIR and IR, and ~6.7 µm bands that includes a machine learning approach for optically thick cloud properties. A tradeoff is the potential for reduced accuracy particularly using data from the more advanced satellites that have more spectral channels (e.g. SEVIRI, AHI and ABI) that are known to help improve thin cirrus detection, cloud-aerosol discrimination and estimates in other difficult conditions that challenge cloud remote sensing. The new continuity approach is applied to one month of global GEOSat data for each year of the CERES record since 2000 and compared with the Ed4 GEO and MODIS cloud property time series in order to evaluate the level of improved consistency in the GEOsat record and to assess the accuracy impacts. Cloud fraction will also be assessed with CALIPSO data. Outstanding issues and challenges will be discussed. The results are expected to guide future work needed to develop a more robust GEOsat cloud data record for CERES.

CERES CDR↗

DOE OSTI2025

Contact Freezing of Water Droplets by Crystalline Organic Acids

The ability of water to freeze into ice crystals in mixed-phase clouds affects physical properties, including particle size, precipitation rates, and radiative properties. The presence of an insoluble particle at the surface of water droplets can promote ice nucleation at temperatures higher than that of pure water, even in the absence of a collision. However, contact freezing remains an underexplored mode of ice nucleation. Here, we present a study of atmospherically relevant organic acids and their role as effective ice-nucleating particles (INP) in contact mode using a Raman-microscope-equipped environmental chamber. We determined contact freezing temperatures induced by solid crystals of docosanol, adipic acid, cis-pinonic acid, fumaric acid, 4-hydroxybenzoic acid, palmitic acid, phthalic acid, sebacic acid, stearic acid, terephthalic acid, and vanillic acid. All solids except fumaric acid promoted contact freezing of water droplets at significantly higher temperatures than pure water in the chamber (−15.0 to −18.5 °C vs −21.3 °C). Physical and chemical properties were identified which correlate with greater effectiveness of INPs in the contact mode, including crystal lattice mismatch with ice, carbon number, and insolubility in water. In conclusion, we suggest that the presence of these organic solids in atmospheric aerosols may promote atmospheric ice nucleation at warm temperatures.

Clouds↗

NASA NTRS1979

Analysis of radiation patterns of interaction tones generated by inlet rods in the JT15D engine

Interaction tones were intentionally generated by circumferential arrays of equally spaced rods that protrude radially from the inlet wall near the face of the 28-blade fan. Arrays of 28 and 41 rods, selected to give specific far field radiation properties, were tested. The expected properties were readily apparent in the measured radiation patterns. A more detailed analysis of the test data showed both the precision and limitations of the applied acoustic theory. Rods protruding 23 percent of the radius predominantly generated only lowest radial order modes, as expected. Measured and predicted radiation patterns were generally in good agreement. The agreement, however, depended on a significant degree of implied refraction due to inlet velocity gradients. Refraction, if present, would impact static-flight noise comparisons.

Heidmann, M. F.↗

NASA NTRS1985

Solar maximum thermal surface assessment

The inflight repair of the Solar Maximum Spacecraft provided the first opportunity to make actual measurements of thermal control surfaces after 4 years exposure in low Earth orbit. Defective hardware was replaced by astronauts and returned to Earth while protected from reentry damage in the Shuttle Payload bay. A preliminary thermal surface assessment was made soon after retrieval in support of Space Telescope and other current spacecraft programs. This included visual examination and measurement of Kapton and Teflon film to determine change in thermal radiative properties after 4 years exposure to solar radiation and reaction with atomic oxygen. Comparative measurements were made with a portable solar reflectometer used for inspection of spacecraft hardware. Post flight measurements and observations reveal significant surface changes that further confirm Kapton mass loss predictions made prior to Solar Maximum repair. Details of thermal surface application, measurements and experimental results are presented and discussed.

Rhoads, G. D.↗

NASA NTRS1995

On the Calculation of Anisotropic Extinction Coefficients for Rigid Fibrous Ceramic Insulations

The specific anisotropic extinction coefficient e* couples the effective Radiative properties of a fibrous insulation into the radiation diffusion equation. This coefficient can be calculated using Mie scattering theory if fiber diameters, refractive indices and fiber orientation distributions are known. In general, fiber orientation distributions are not readily accessible and past calculations have considered fibers as either randomly distributed or normal to the heat flow direction. In certain rigid fibrous ceramic insulations neither of these cases apply well and a simple procedure is described for approximating e* from values calculated for the random and normal orientation cases. The intrinsic error associated with this scaling procedure is investigated. Numerical computations for several test structures and fiber materials show the average error to be less than 5% for net heat flux and radiation conductivity calculations.

Marshall, Jochen↗

NASA NTRS1993

Application of Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) to Determination of Atmospheric Aerosol Optical Depth and Precipitable Water Content

This paper focuses on determination of the temporal and spatial gas absorption and aerosol scattering properties of the atmosphere itself including the radiative properties of clouds, specifically derivation of estimates of aerosol optical depth, atmospheric water vapor, and oxygen pressure surface altitude form upwelling near-TOA spectral radiance measurements obtained with the AVIRIS.

Remote SensingAVIRIS↗