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At least 271 records · Page 15

Comparison of graphite, aluminum, and TransHab shielding material characteristics in a high-energy neutron field

Space radiation transport models clearly show that low atomic weight materials provide a better shielding protection for interplanetary human missions than high atomic weight materials. These model studies have concentrated on shielding properties against charged particles. A light-weight, inflatable habitat module called TransHab was built and shown to provide adequate protection against micrometeoroid impacts and good shielding properties against charged particle radiation in the International Space Station orbits. An experiment using a tissue equivalent proportional counter, to study the changes in dose and lineal energy spectra with graphite, aluminum, and a TransHab build-up as shielding, was carried out at the Los Alamos Nuclear Science Center neutron facility. It is a continuation of a previous study using regolith and doped polyethylene materials. This paper describes the results and their comparison with the previous study. Published by Elsevier Science Ltd.

NASA Center JSC↗

Mortality among workers at the Rocky Flats Plant, 1951–2017

The Rocky Flats (RFs) Plant operated from 1951–1989 as part of the U.S. Department of Energy (DOE) nuclear complex. Its primary mission was weapons component fabrication, whereby workers were potentially exposed to radioactive and non-radioactive hazards. RF worker mortality was compared to the general population, and dose-response relationships between mortality and radiation organ doses were examined. RF workers first employed between 1951 and 1979 for ⩾30 d were identified (n = 9397). Vital status was determined using national and state death records up to 2017. Organ doses from external photons and neutrons irritation and internalised plutonium (Pu), americium (Am), and uranium (U) were modelled as cumulative lagged total doses per year. Beryllium exposure was evaluated as an effect modifier using data from the DOE Nationwide Beryllium Medical Program. Statistical analyses included standardised mortality ratios (SMRs), Cox proportional hazard models, and excess relative risk (ERR) models. Approximately 53.2% of workers were deceased by the end of the study. Nearly 90% were monitored for radiation exposure, with a mean weighted absorbed dose of 59.0 mGy for the lungs. Nearly 45% of workers had intakes of alpha-particle emitting radionuclides, and 46.7% were monitored for neutrons. Leading causes of death included ischemic heart disease (n = 999) and lung cancer (n = 361). The highest SMRs were observed for berylliosis (SMR: 176.9; 95% CI: 76.2, 348.7; n < 10) and asbestosis (SMR: 4.65; 95% CI: 2.23, 8.55; n = 10). Dose-response analyses showed no statistical increase in risk from low-dose radiation including lung cancer (ERR per 100 mGy: −0.02; 95% CI: −0.11, 0.08; n = 361) and Parkinson’s disease (ERR per 100 mGy: 0.13; 95% CI: −0.26, 0.31; n = 57). Approximately 45% of workers were monitored for beryllium, with a weak non-significant indication of effect modification for lung cancer risk. The RF cohort showed no evidence of a statistically significant increase in mortality from occupational radiation exposure. However, this study was limited by low statistical power, which inhibits the ability to detect effects. Future pooling of Million Person Study (MPS) cohorts will provide further insights, particularly regarding Pu as a carcinogen.

61 RADIATION PROTECTION AND DOSIMETRY↗

Ash loading and insolation at Hanford, Washington during and after the eruption of Mount St. Helens

The effects of volcanic ash suspended in the atmosphere on the incident solar radiation was monitored at the Hanford Meteorological Station (HMS) subsequent to the major eruption of Mount St. Helens on May 18, 1980. Passage of the ash plume over Hanford resulted in a very dramatic decrease of solar radiation intensity to zero. A reduction in visibility to less than 1 km was observed, as great quantities of ash fell out of the plume onto the ground. Ash loading in the atmosphere remained very high for several days following the eruption, primarily as a result of resuspension from the surface. Visibilities remained low (2 to 8 km) during this period. Estimates of atmospheric turbidity were made from the ratio of diffuse-to-direct solar radiation; these turbidities were used to estimate extinction along a horizontal path, a quantity which can be related to visibility. Comparisons of observed and estimated visibilities were very good, in spite of the rather coarse approximations used in the estimates. Atmospheric clarity and visibility improved to near pre-eruption conditions following a period of rain showers. The diffuse-to-direct ratio of solar radiation provided a useful index for estimating volcanic ash loading of the atmosphere.

Laulainen, N. S.↗

Simulated Performance of the Micro-Pocket Fission Detector in the Advanced Test Reactor Critical Facility

The Micro-Pocket Fission Detector (MPFD) is a small-form–factor real-time fission chamber. MPFD performance has been simulated in the Advanced Test Reactor Critical Facility (ATRC), located at Idaho National Laboratory (INL). Here, the neutron and gamma-ray flux profiles and magnitudes were simulated using Monte Carlo N-Particle (MCNP) in the near-core B-8 irradiation position. These simulations were performed at 69 discrete axial locations inside the B-8 position for three separate orientations of the nearby hafnium outer shim control cylinders and at a power level of 700 Wth. The resulting neutron and gamma-ray flux values were used to determine the MPFD response for various fissile masses and detector gas pressures. The optimal gas-operating pressure was determined to be between 30 and 60 psig. The required fissile-layer mass was determined to be between 1–2 µg of 235 U. Additionally, the gamma-ray to fission-fragment interaction rate was determined to be 4.42 × 10 -3 with average energy deposition for gamma rays and fission fragments in 30 psig argon gas to be 1 keV and 9.5 MeV, respectively.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

A 400 kilowatt argon arc lamp for solar simulation

A 400 kilowatt argon arc lamp for a solar simulator has been designed, operated, and evaluated. The lamp is designed to produce one solar constant on a test area 4.6 by 9.2 meters when used with a collimator. The divergence angle of the beam is about 1 deg. The lamp is designed to operate completely within a vacuum environment. Over 80 kilowatt of directed radiation was monitored and measured for a 25-hour period during a recent test. In another test, an arc was operated at 400 kilowatt for 110 hours without removal or refurbishing of the electrodes. These tests have proven the cleanliness and integrity of the radiation source.

Decker, A. J.↗

Simultaneous measurement of multiple radiation-induced protein expression profiles using the Luminex(TM) system

Space flight results in the exposure of astronauts to a mixed field of radiation composed of energetic particles of varying energies, and biological indicators of space radiation exposure provides a better understanding of the associated long-term health risks. Current methods of biodosimetry have employed the use of cytogenetic analysis for biodosimetry, and more recently the advent of technological progression has led to advanced research in the use of genomic and proteomic expression profiling to simultaneously assess biomarkers of radiation exposure. We describe here the technical advantages of the Luminex(TM) 100 system relative to traditional methods and its potential as a tool to simultaneously profile multiple proteins induced by ionizing radiation. The development of such a bioassay would provide more relevant post-translational dynamics of stress response and will impart important implications in the advancement of space and other radiation contact monitoring. c2004 COSPAR. Published by Elsevier Ltd. All rights reserved.

NASA Center JSC↗

Crystal Growth Scale-Up and Stability of RbSr 2 X 5 :Eu Scintillators

The discovery and development of new scintillation materials support national security needs. In these applications, large volumes of scintillator crystals are needed to achieve efficient screening for contraband. Therefore, one important step in the discovery of new scintillator compositions is testing their feasibility for scale-up and their stability. In this work, high-quality Ø22 mm crystals of two new scintillators RbSr 2 Br 5 :Eu and RbSr 2 I 5 :Eu were grown via the Vertical Bridgman method, and their scintillation properties were characterized. Here, the Ø22 mm RbSr 2 I 5 :Eu crystals could be grown with fast translation rates up to 3.5 mm/h. Both RbSr 2 Br 5 :Eu and RbSr 2 I 5 :Eu had high scintillation performance, including light yields of 46,000 and 61,000 ph/MeV, respectively, for Ø22 × 35 mm crystals. Additionally, properties related to physical stability were investigated, including the coefficients of thermal expansion via high-temperature X-ray diffraction (HTXRD) as well as moisture sensitivity. HTXRD confirmed the absence of solid–solid phase transitions and showed that RbSr 2 Br 5 had minimal thermal expansion anisotropy compared to RbSr 2 I 5 and some other inorganic metal halide scintillators, which favors the growth of large-sized crystals.

36 MATERIALS SCIENCE↗

Search for effects of Comet S-L 9 fragment impacts on low radio frequency emission from Jupiter

Decametric radio observations of Jupiter were made before, during, and after the impacts of the fragments of the comet S-L 9 with the planet, from the University of Florida Radio Observatory, the Maipu Radio Astronomy Observatory of the University of Chile, and the Owens Valley Radio Observatory of the California Institute of Technology. The decametric radiation was monitored at frequencies from 16.7 to 32 MHz. The minimum detectable flux densities were on the order of 30 kJy, except for that of the large 26.3 MHz array in Florida, which was about 1 kJy. There was no significant enhancement or suppression of the decametric L-burst or S-burst emission with respect to normal activity patterns that might be attributed to the fragment entries. A burst of left-hand elliptically polarized radiation having a considerably longer duration than an L-burst was observed almost simultaneously with the impact of the large fragment Q2, and another with right-hand elliptical polarization was observed simultaneously with Q1. We consider the possibility that these two bursts were emitted just above the local electron cyclotron frequencies from the southern and northern ends, respectively, of magnetic flux tubes that had been excited in some way by the proximity of fragments Q2 and Q1. A search was conducted for possible comet-enhanced Jovian synchrotron radiation at 45 MHz using a large dipole antenna array at the observatory in Chile.

Carr, T. D.↗

Fission Product Gas Monitoring During Fuel Drying Operations - 20094

The goal of the project was to devise and implement a method of accurately qualifying any noble gas emitted during fuel drying operations (part of the dry fuel storage process) in order to provide the data needed to validate the off-site dose calculations. The imputes of the project was the NRC publishing Information Notice 18-01, 'Noble Fission Gas Releases During Spent Fuel Cask Loading Operations' in February 2018. The information notice describes some industry events that occurred during vacuum drying operations as part of a dry fuel campaign. The solution was devised by Fort Calhoun Station staff in partnership with Mirion Technologies technical staff. The monitoring was accomplished by directing all the effluent from the fuel storage cask vacuum drying machine through a sample chamber containing a compact ISOCS characterized CZT based gamma spectrometer connected to a Mirion Data Analyst. This resulted near real-time quantification of the radionuclides of concern. (authors)

07 ISOTOPE AND RADIATION SOURCES↗

Monitoring Temperatures of Tires Using Luminescent Materials

A method of noncontact, optical monitoring of the surface temperature of a tire has been devised to enable the use of local temperature rise as an indication of potential or impending failures. The method involves the use of temperature-sensitive paint (or filler): Temperature-sensitive luminescent dye molecules or other luminescent particles are incorporated into a thin, flexible material coating the tire surface of interest. (Alternatively, in principle, the luminescent material could be incorporated directly into the tire rubber, though this approach has not yet been tested.) The coated surface is illuminated with shorter-wavelength light to excite longer-wavelength luminescence, which is observed by use of a charge-coupled-device camera or a photodetector (see Figure 1). If temporally constant illumination is used, then the temperature can be deduced from the known temperature dependence of the intensity response of the luminescence. If pulsed illumination is used, then the temperature can be deduced from the known temperature dependence of the time or frequency response of the luminescence. If sinusoidally varying illumination is used, then the temperature can be deduced from the known temperature dependence of the phase response of the luminescence. Unlike a prior method of monitoring the temperature at a fixed spot on a tire by use of a thermocouple, this method is not restricted to one spot and can, therefore, yield information on the spatial distribution of temperature: in particular, it enables the discovery of newly forming hot spots where damage may be starting. Also unlike in the thermocouple method, the measurements in this method are not vulnerable to breakage of wires in repeated flexing of the tire. Moreover, unlike in another method in which infrared radiation is monitored as an indication of surface temperature, the luminescence measurements in this method are not significantly affected by changes in infrared emissivity. This method has been demonstrated in application to the outside surface of a tire (see Figure 2), using both constant and pulsed light sources for illumination and cooled, slow-scan, gated CCD cameras for detection. For observing the temperature of the inside surface of a tire (this has not yet been done), it would probably be necessary to use fiber optics and/or windows for coupling excitation light into, and coupling luminescence out of, the interior volume.

Bencic, Timothy J↗

Fast, Large Area, Wide Band GAP UV Photodetector for Cherenkov Light Detection

A solid-state radiation detector includes a pattern of conductive metal on a zinc oxide substrate. The pattern provides an arrangement of interdigitated electrode fingers. The wide band gap substrate is sensitive to UV light, which can cause a conductivity change in the substrate. The electrode fingers are configured to sense a difference in substrate conductivity resulting from UV light. The detector has a fast response time, which enables it to detect Cherenkov light. The compact detector provides savings on size, weight, and required power. Thus, the solid-state detector can be used to replace photomultiplier tubes in Cherenkov detectors. The features of the novel detector allow for an improved system to detect and monitor UV radiation, especially during deep space missions.

Wrbanek, John D.↗

Lessons Learned in the Development of Industry Guidance - 20279

The availability of industry guidance on different aspects of waste management forms a valuable reference for waste practitioners. The guidance typically details the principles, processes and practices that should be consulted during each stage of the relevant activities. It also includes relevant regulatory and international requirements, appropriate case studies and examples of best practices to illustrate technical concepts and make the information available to the reader in an accessible manner. Over recent years Wood have developed (or are developing) a number of industry guidance documents on a range of topics including Solid Waste Characterization, Routine Water Quality Monitoring on Nuclear Sites: Pipeline Characterization: Determining Background Radioactivity for Land Quality Assessment: Interim Storage and Aqueous Waste Management. This talk provides an overview of lessons learned along the way including: - the importance of stakeholder engagement through the process: - how to identify 'good practice'; - the importance of iterative development; and - the selection of illustrative and informative case studies. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Achieving the End State for the Pahute Mesa Corrective Action Units at the Nevada National Security Site - 20355

Underground nuclear testing at the Nevada National Security Site (NNSS) ended in 1992. To address the impact of radionuclide contamination from underground nuclear testing on the groundwater resources of Nevada, the U.S. Department of Energy (DOE) Environmental Management (EM) Nevada Program created the Underground Test Area (UGTA) activity to characterize the radionuclides in groundwater, understand the nature and extent of radionuclide migration, and forecast the distribution of radionuclides in groundwater for 1,000 years. The UGTA activity is regulated by the Federal Facility Agreement and Consent Order (FFACO), an agreement negotiated between the Nevada Division of Environmental Protection (NDEP), DOE, and the U.S. Department of Defense (DoD). DOE is close to achieving the end state (closure in place with monitoring and institutional control) for three of the five UGTA corrective action units (CAUs) on the NNSS. A number of challenges remain to achieve the end state of the other two CAUs, both located on Pahute Mesa. Pahute Mesa was the location of 82 underground nuclear tests, less than 10% of the total number of tests on the NNSS. Yet, Pahute Mesa contains slightly more than 60% of the total radionuclides (in curies). Based on groundwater sampling in monitoring wells, two radionuclide plumes have migrated several kilometers (km) in groundwater from selected test cavities and have crossed the boundary of the NNSS (yet remain within the boundaries of Federally controlled land). The path to achieve the end state continues to evolve as more data are collected and a better understanding of radionuclide migration in groundwater is developed. DOE has invested in drilling and sampling more than 50 characterization and monitoring groundwater wells over the past 25 years. The data indicate that the primary radionuclide of concern is tritium as it is about 89% of the total radionuclide inventory (in curies). As well, only tritium has been measured in groundwater outside of cavities at concentrations exceeding the Safe Drinking Water Act (SDWA) standard. For one of the tritium plumes that has migrated across the NNSS boundary, the average rate of migration has been measured as about 45 meters (m) per year with the rate of migration at the leading edge of the plume of about 85 meters per year. At that rate of migration, the tritium plume will decay to safe levels and not reach the publicly accessible environment at concentrations above the SDWA standard. Other radionuclides, at concentrations below the SDWA standards, will be monitored to ensure they remain at safe levels. Consequently, the end state path forward for Pahute Mesa has evolved to take full advantage of the data from the monitoring network to constrain uncertainty in model forecasts and to reduce reliance on probabilistic simulations. The focus of the end state approach relies on developing a monitoring well network that is protective of human health by increasing confidence that no radionuclide plume in the groundwater will migrate undetected to the accessible environment, located about 22 km from the nearest up-gradient underground nuclear test. Using the measured data to remove uncertainty, the evaluation of radionuclide migration from Pahute Mesa is directed toward meeting the goals of the end state. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Tensioned metastable fluid detector sensing technology for multifarious-multiscale applications in the nuclear fuel cycle

The nuclear fuel cycle presents formidable 10 30+ multiscale challenges for high-efficiency spectroscopic sensing of alpha-neutron-fission radiation signatures amidst extreme gamma-beta radiation backgrounds at various stages of the cycle; it involves diverse arenas ranging from continuous/pulsed power production, security/safeguards, spent fuel, environmental remediation, and personnel health-dosimetry. This paper discusses the novel tensioned metastable fluid detector (TMFD) sensor technology. It discusses the results of studies demonstrating extreme (10 4 Sv/h) gamma-beta field blind high intrinsic efficiencies (80–100%) for neutron-alpha-fission radiation spectrometric detection. Example studies discussed in this paper include Neutron detection with spectroscopy; H*10 neutron radiation dosimetry upwards from ultra-low10 −2 µSv/h levels; Air and/or liquid-borne trace (10 –3 Bq/mL) quantity, 1 keV energy resolved alpha/fission spectroscopy for Rn/Po/U/Pu/Am environmental isotope assays at 106:1 (β:α) ratios; Directional-position enabled extended standoff tracking of neutron emitting (shielded/unshielded) special nuclear materials while stationary or moving at highway speeds; and, U.S. Department of Energy nuclear complex wide nuclear waste reprocessing, criticality safety, health physics, and environmental applications.

Alpha-fission-neutron spectrometry↗

Final Report on Radiation Measurements Performed Inside of the BEAM Module

Measurements of the radiation environment inside of the Bigelow Expandable Activity Module (BEAM) have been made on a pseudo-continuous basis since June 6, 2016 using both passive and active instrumentation. Passive detectors yield a single cumulative dose value (or average daily dose) over the measurement period from deploy to return to ground. Active Radiation Environment Monitor (REM) sensors yield dose rate, Linear Energy Transfer (LET) spectra, and particle-specific dose, all on a 1-minute cadence. From the initial install in 2016 until early 2018, BEAM was an empty module. In 2018, further testing was approved and stowage began to be moved into BEAM. As a result, it was decided to stop measurements with RAM detectors to avoid potential difficulties with access after stowage was added. The REM sensors remained however in the original deploy locations.

radiation exposure↗

Application of On-Line Monitoring and Real-Time Characterization of Low Level Waste Samples from Hanford Tanks - 20380

Waste and treatment stream characterization is an essential part of safe, efficient, and cost-effective processing of Hanford materials. The demand for materials characterization, including chemical, radionuclide, and physical attributes during waste management, transfer, and staging operations in the Hanford tank farms, is expected to significantly increase as the U.S. Department of Energy Office of River Protection (ORP) progresses toward Hanford waste treatment and immobilization. The application of on-line monitoring can greatly improve operation time frames and reduce costs by providing real-time data and supporting the reduction of necessary grab sample collection. Recently, our team applied Raman online monitoring and chemometric modeling to the supernate of Hanford tank 241-AP-105, and demonstrated the quantitative measurement of nine analytes within this waste. Application of this method has been expanded to additional Hanford tank wastes, AW-102 and AP-107. The performance of the process monitoring instruments and the accuracy of the chemometric models will be assessed. On-line monitoring results will be compared to anion results determined from the current standard, ion-chromatographic and inductively coupled plasma mass spectrometry methods. Comparisons of both determined values and uncertainties of results will be presented. Results will be shared with personnel working on flowsheet interfaces for the Direct-Feed Low Activity Waste mission at Hanford. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Low Level Radon Concentration and Radon Daughter Dose Monitoring in an Arid-zone Waste Store - 20081

Radioactive waste containing predominantly soil and rubble from the clean-up of a former uranium and thorium minerals processing research facility is currently stored at the Woomera Test Range in South Australia awaiting final disposal. Prior to commencing any manipulation of the nearly 10,000 waste drums (205 L or 55 gallon each), radon concentration monitoring and radon daughter dosimetry has been undertaken to (i) gain understanding of the temporal and spatial variation of radon and its daughters within the storage facility, which could provide insights into the radiological source term and (ii) confirm that radiological risks to workers are below the guideline values. A time series of nearly 12 months of detailed observations shows low level radon concentrations with annual average values that are slightly above the average radon concentrations in Australian homes. Peak values in summer are about three times higher than the annual average based on the CRM measurements. Both radon concentrations and annual effective dose are well below the regulatory limits. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Monitoring the Possible Effects of Corroding Fuel Cladding in Nuclear Ponds: a Modified ROV for Storage Ponds - 20144

Nuclear ponds are used worldwide to store radioactive nuclear material, often for extended periods of time. The pond water conditions need to be closely monitored so that mitigation strategies can be put in place should any leakage of radioactive material occur. This paper describes the selection, development and on-site deployment of a bespoke system whose design was based on of-the-shelf components. The system is able to identify, locate and differentiate the leakage of radioactive material stored in nuclear ponds from the background activity of the water in the pond. The selection of an appropriate detector and monitoring geometry was supported by MCNP modelling which allowed a high degree of confidence in the proposed design. The development of the system allowed a real-time indication of the canister integrity, without incurring the increased operator doses from manual sampling operations that were previously used on site. The benefits of the developed system include the fact that the system is lightweight, easily deployable, retrievable, decontaminable and results in negligible waste products. Moreover, it is able to analyse the samples in-situ, in this way reducing the time needed to manually collect and send the samples to a laboratory for lengthy analysis. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗