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At least 271 records · Page 15

Raman DIAL measurements of stratospheric ozone in the presence of volcanic aerosols

Since the eruption of Mt. Pinatubo in June, 1991, measurements of atmospheric species which depend on Rayleigh scattering of radiation, have been severely compromised where the volcanic aerosol cloud exists. For the GSFC stratospheric ozone lidar, this has meant that ozone determination has been impossible below approximately 30 km. The GSFC lidar has been modified to detect Raman scattering from nitrogen molecules from transmitted laser wavelengths. The instrument transmits two laser wavelengths at 308 nm and 351 nm, and detects returns at four wavelengths; 308 nm, 332 nm, 351 nm, and 382 nm. Using this technique in conjunction with the Rayleigh DIAL measurement, ozone profiles have been measured between 15 and 50 km.

Mcgee, Thomas J.↗

Mariner 9 ultraviolet spectrometer experiment - Scattering properties of Hellas

A least-squares analysis of 709 Mariner 9 UV spectra obtained over Hellas from Revolution 140 to 214 (Jan. 22, 1972, to Feb. 28, 1972) showed the extinction optical depth of the atmosphere above Hellas to be 0.5 plus or minus 0.2. This is evidence of lingering dust in the Hellas basin. An atmospheric model, combining dust and Rayleigh scattering, was used to make an apparent pressure map of Hellas. Anomalously high pressures are interpreted as clouds developing over the southern part of Hellas near the time of autumnal equinox. The blue ratio (reflectance at 2680 A divided by reflectance at 3050 A) showed a 20% increase from Revolution 40 to Revolution 74, attributed to the decay of the dust storm. Thereafter, the blue ratio remained essentially constant through Revolution 214, which implies that the rate of clearing in Hellas was much slower than that planetwide.

Ajello, J. M.↗

Use of an Improved Radiation Amplification Factor to Estimate the Effect of Total Ozone Changes on Action Spectrum Weighted Irradiances and an Instrument Response Function

Multiple scattering radiative transfer results are used to calculate action spectrum weighted irradiances and fractional irradiance changes in terms of a power law in ozone OMEGA, U(OMEGA/200)(sup -RAF), where the new radiation amplification factor (RAF) is just a function of solar zenith angle. Including Rayleigh scattering caused small differences in the estimated 30 year changes in action spectrum-weighted irradiances compared to estimates that neglect multiple scattering. The radiative transfer results are applied to several action spectra and to an instrument response function corresponding to the Solar Light 501 meter. The effect of changing ozone on two plant damage action spectra are shown for plants with high sensitivity to UVB (280-315 run) and those with lower sensitivity, showing that the probability for plant damage for the latter has increased since 1979, especially at middle to high latitudes in the Southern Hemisphere. Similarly, there has been an increase in rates of erythemal skin damage and pre-vitamin D3 production corresponding to measured ozone decreases. An example conversion function is derived to obtain erythemal irradiances and the UV index from measurements with the Solar Light 501 instrument response function. An analytic expressions is given to convert changes in erythemal irradiances to changes in CIE vitamin-D action spectrum weighted irradiances.

Herman, Jay R.↗

Saturn - UBV photoelectric pinhole scans of the disk

UBV photoelectric pinhole scans of Saturn's disk are reported. The data are interpreted by using elementary radiative-transfer models to describe scattering in the atmosphere above the visible haze layer. Limits are placed on the optical thickness of the region above the haze, and the results are discussed in terms of the probable structure of Saturn's upper atmosphere. It is shown that a model involving conservative Rayleigh scattering by hydrogen molecules above an opaque haze or cloud deck provides a satisfactory quantitative description of the scattering properties of Saturn's upper atmosphere.

Franz, O. G.↗

Aerosol analysis with the Coastal Zone Color Scanner - A simple method for including multiple scattering effects

A method for studying aerosols over the ocean using Nimbus-7 CZCS data is proposed which circumvents having to perform radiative transfer computations involving the aerosol properties. The method is applied to the CZCS band 4 at 670 nm, and yields the total radiance (L sub t) backscattered from the top of a stratified atmosphere containing both stratospheric and tropospheric aerosols and the the Rayleigh scattered radiance (L sub r). The radiance which the aerosol would produce in the single scattering approximation is retrieved from (L sub t) - (L sub r) with an error of not greater than 5-7 percent.

Gordon, Howard R.↗

Data analysis and interpretation of lunar dust exosphere

The lunar horizon glow observed by Apollo astronauts and recorded during the Surveyor missions is believed to result from the scattering of sunlight off lunar fines suspended in a dust layer above the lunar surface. For scale heights of tens of kilometers, theory and astronaut's observations suggest that the size of the dust particles will be smaller than 0.1 microns in radius and will act as Rayleigh scatters. This means that the dust scattered light will be 100 percent polarized at a 90 degree scattering angle and will depend on wavelength to the inverse fourth power ('bluing'). Believing these signatures to be observable from ground based telescopes, observational data in the form of CCD images has been collected from McDonald Observatory's 36 in. telescope, and the reduction and analysis of this data is the focus of the present report.

Andrews, George A., Jr.↗

A multi-layer discrete-ordinate method for vector radiative transfer in a vertically-inhomogeneous, emitting and scattering atmosphere. I - Theory. II - Application

A theory is developed for discretizing the vector integro-differential radiative transfer equation including both solar and thermal radiation. A complete solution and boundary equations are obtained using the discrete-ordinate method. An efficient numerical procedure is presented for calculating the phase matrix and achieving computational stability. With natural light used as a beam source, the Stokes parameters from the model proposed here are compared with the analytical solutions of Chandrasekhar (1960) for a Rayleigh scattering atmosphere. The model is then applied to microwave frequencies with a thermal source, and the brightness temperatures are compared with those from Stamnes'(1988) radiative transfer model.

Weng, Fuzhong↗

Atmospheric Multiple Scattering Effects on GLAS Altimetry: Calculations of Single Pulse Bias - Part 1

Estimates of the effect of pulse stretching on satellite laser altimetry in particular the Geoscience Laser Altimeter System (GLAS), by cloud multiple scattering were made from an analytical method and from Monte Carlo calculations. The path delay of the return pulse was found to be largest for low-level clouds with particle radii (3-20 microns). The magnitude of the path delay was affected by several factors including cloud height, cloud optical depth, cloud particle size, particle shape, and receiver field of view. Polar aerosol and Rayleigh scattering usually added less than 1 cm to the overall path delay. Path delay estimates for all cloud conditions would be less if a simple Gaussian fit of the return pulse peak were used to measure the pulse's centroid. However, care must be taken in determining the centroid as factors such as pulse width, surface slope and the fitting method used will affect the estimate. A planned application for laser altimetry is high precision monitoring of the height change of polar ice sheets. In the absence of a correction algorithm, the required GLAS altimetry accuracies will not be achieved unless atmospheric channel information is used to remove profiles that are likely to be heavily contaminated by multiple scattering.

Duda, David P.↗

The OMPS Limb Profiler Instrument: An Alternative Data Analysis and Retrieval Algorithm

The upcoming Ozone Mapper and Profiler Suite (OMPS), which will be launched on the NPOESS Preparatory Project (NPP) platform in early 2011, will continue monitoring the global distribution of the Earth's middle atmosphere ozone and aerosol. OMPS is composed of three instruments, namely the Total Column Mapper (heritage: TOMS, OMI), the Nadir Profiler (heritage: SBUV) and the Limb Profiler (heritage: SOLSE/LORE, OSIRIS, SCIAMACHY, SAGE III). The ultimate goal of the mission is to better understand and quantify the rate of stratospheric ozone recovery. The focus of the paper will be on the Limb Profiler (LP) instrument. The LP instrument will measure the Earth fs limb radiance (which is due to the scattering of solar photons by air molecules, aerosol and Earth surface) in the ultra-violet (UV), visible and near infrared, from 285 to 1000 nm. The LP simultaneously images the whole vertical extent of the Earth's limb through three vertical slits, each covering a vertical tangent height range of 100 km and each horizontally spaced by 250 km in the cross-track direction. The focal plane of the LP spectrometer is a two ]dimensional CCD array comprised of 340 x 740 pixels. Several data analysis tools are presently being constructed and tested to retrieve ozone and aerosol vertical distribution from limb radiance measurements. The primary NASA algorithm is based on earlier algorithms developed for the SOLSE/LORE and SAGE III limb scatter missions. The paper will describe an alternative algorithm which will retrieve ozone density and aerosol extinction directly from radiance data collected on individual CCD pixels. This alternative method uses an optimal estimation approach to retrieve ozone and aerosol in the 10-60 km range from the information contained within an ensemble of about 50000 down-linked pixels. Tangent height registration is performed using the Rayleigh Scattering Attitude Sensor (RSAS) technique applied to columns of pixels in the 340-360 nm range. Cloud height is determined by analyzing the radiance first derivative along pixel columns at longer wavelengths. Wavelength registration is performed using rows of pixels and identifying Fraunhofer solar lines within the measured spectra. Special attention is given to stray-light decontamination and modeling of the measured finite spectral/spatial line shape functions.

Rault, Didier F.↗

Absolute intensity and polarization of rotational Raman scattering from N2, O2, and CO2

An experimental examination of the absolute intensity, polarization, and relative line intensities of rotational Raman scattering (RRS) from N2, O2, and CO2 is reported. The absolute scattering intensity for N2 is characterized by its differential cross section for backscattering of incident light at 647.1 nm, which is calculated from basic measured values. The ratio of the corresponding cross section for O2 to that for N2 is 2.50 plus or minus 5 percent. The intensity recent for N2, O2, and CO2 are shown to compare favorably to values calculated from recent measurements of the depolarization of Rayleigh scattering plus RRS. Measured depolarizations of various RRS lines agree to within a few percent with the theoretical value of 3/4. Detailed error analyses are presented for intensity and depolarization measurements. Finally, extensive RRS spectra at nominal gas temperatures of 23 C, 75 C, and 125 C are presented and shown to compare favorably to theoretical predictions.

Penney, C. M.↗

NASA TROPOMI Aerosol Products: Algorithmic Upgrades and Preliminary Evaluation

This poster presentation describes an expanded NASA TROPOMI (Tropospheric Monitoring Instrument)aerosol algorithm (N-TROPOMAER) that takes advantage of TROPOMI observations in the ultraviolet and visible spectral regions. The availability of the Oxygen B-band observations, and the unprecedentedly high spatial resolution (3.5 km X 5.5 km) for a hyper-spectral sensor are significant improvements for aerosol properties retrieval. The heritage N-TROPOMAER aerosol algorithm uses near-ultraviolet radiances at 354 nm and 388 nm from Sentinel 5 Precursor-TROPOMI for simultaneously retrieving aerosol optical depth (AOD), single-scattering albedo (SSA), aerosol absorption optical depth (AAOD), and above-cloud aerosol optical depth(ACAOD) at 388 nm, along with the qualitative UV aerosol index (UVAI). We have expanded the inversion capability beyond the UV, to retrieve AOD at 466 nm and 680 nm. Surface reflectance effects at466 nm are accounted for using a recently developed geometry-dependent surface Lambertian-equivalent reflectivity (GLER) product, which is derived from the top-of-atmosphere radiance computed with Rayleigh scattering and surface bidirectional reflectance distribution function (BRDF) for the exact viewing geometry at the sensor’s spatial resolution. Aerosol layer height (ALH) and 680 nm AOD are simultaneously derived from observations at 680 nm and at the Oxygen-B band (688 nm). Another important upgrade is the use of time averaged total column carbon monoxide from the NASA GEOS-CF(Global Earth Observing System Composition Forecast) as a tracer of carbonaceous aerosols.

TROPOMI↗

100-kHz Rate Rayleigh Imaging for Combustion and Flow Diagnostics

Two-dimensional (2D) Rayleigh scattering (RS) imaging at an ultrahigh repetition rate of 100 kHz is demonstrated in non-reacting and reacting flows employing a high-energy burst-mode laser system. Image sequences of flow mixture fraction were directly derived from high-speed RS images. Additionally, a 2D instantaneous flow velocity field at 100 kHz was obtained through optical-flow-based analysis of the RS images. The technique was also applied to study turbulent flames having a near-constant Rayleigh cross section. The demonstrated high-speed RS technique in conjunction with optical-flow-based analysis provides non-intrusive, simultaneous measurements of the flow mixing and velocity field, extending the measurement capability of the RS technique to high-speed non-reacting and reacting flows.

Jiang, Naibo↗

Gaseous hydrogen/oxygen injector performance characterization

Results are presented of spontaneous Raman scattering measurements in the combustion chamber of a 110 N thrust class gaseous hydrogen/oxygen rocket. Temperature, oxygen number density, and water number density profiles at the injector exit plane are presented. These measurements are used as input profiles to a full Navier-Stokes computational fluid dynamics (CFD) code. Predictions of this code while using the measured profiles are compared with predictions while using assumed uniform injector profiles. Axial and radial velocity profiles derived from both sets of predictions are compared with Rayleigh scattering measurements in the exit plane of a 33:1 area ratio nozzle. Temperature and number density Raman scattering measurements at the exit plane of a test rocket with a 1:1.36 area ratio nozzle are also compared with results from both sets of predictions.

Degroot, W. A.↗

Aerosol scattering of ultraviolet sunlight in the tropical maritime atmosphere

The effects of atmospheric aerosol scattering on the vertical profile of solar ultraviolet radiation are investigated. Measurements of diffuse and total ultraviolet radiation were made using a rocketborne optical sonde in the marine atmosphere of Antigua. During observations, the sun was at zenith. Vertical profiles of directly transmitted solar radiation were calculated by subtraction of the diffuse component from the total radiance. Using these values of direct downward solar UV-flux, the optical thickness of the atmosphere was derived as a function of altitude. Absorption by ozone was also considered. In the troposphere the values of observed optical thickness were in general equal to or lower than those expected theoretically from Rayleigh scattering alone. The measured radiation profiles were compared with those computed for a multiple scattering model atmosphere. Some computations regarding the interaction of UV-sunlight with maritime aerosols are presented.

Ghazi, A.↗

An x ray scatter approach for non-destructive chemical analysis of low atomic numbered elements

A non-destructive x-ray scatter (XRS) approach has been developed, along with a rapid atomic scatter algorithm for the detection and analysis of low atomic-numbered elements in solids, powders, and liquids. The present method of energy dispersive x-ray fluorescence spectroscopy (EDXRF) makes the analysis of light elements (i.e., less than sodium; less than 11) extremely difficult. Detection and measurement become progressively worse as atomic numbers become smaller, due to a competing process called 'Auger Emission', which reduces fluorescent intensity, coupled with the high mass absorption coefficients exhibited by low energy x-rays, the detection and determination of low atomic-numbered elements by x-ray spectrometry is limited. However, an indirect approach based on the intensity ratio of Compton and Rayleigh scattered has been used to define light element components in alloys, plastics and other materials. This XRS technique provides qualitative and quantitative information about the overall constituents of a variety of samples.

Ross, H. Richard↗

Evaluation of Brightness Temperature Sensitivity to Snowpack Physical Properties Using Coupled Snow Physics and Microwave Radiative Transfer Models

There are multiple existing microwave radiative transfer models (RTMs) to simulate the brightness temperature (Tb) of snowpacks. It is still challenging to have consistent Tb responses from RTMs due to individual physical formulations of the snowpack scattering process. This article examines three of the widely-used multi-layer RTMs: 1) the microwave emission model of layered snowpacks (MEMLS); 2) the dense media radiative transfer based on the quasi-crystalline approximation (QCA) of Mie scattering of densely packed sticky spheres (DMRTQMS); and 3) the Helsinki University of Technology (HUT) model. Interestingly, these models yield slightly different Tb responses when driven by the same physical snowpack properties. Tb variations, dependent on the choice of RTMs, are then evaluated to improve the understanding of model differences in microwave emission from a snowpack. We first perform a sensitivity study of the Tb predictions from the three RTMs as a function of snow grain sizes, densities, and depths. While Tb from all three RTMs decreases with increasing snow grain sizes, it is found that a scaling factor is required to have the same amount of Tb attenuation for small grain sizes within the Rayleigh scattering regime. For larger grain sizes, however, a scaling coefficient is not enough to match the model outputs due to the different scattering assumptions of the RTMs. For a single snow layer with increasing snow depths and densities, all three RTMs exhibit Tb attenuations arising from the increase in path lengths and optical depths. Further evaluations are conducted by feeding the three RTMs with the output of a snow physics model driven by in situ weather forcing in a coupled simulation. Outputs of this coupled model include snowpack physical properties and Tbs. By using snow stratigraphy observations, another set of Tb simulation is also conducted with RTMs driven by in situ snowpit observations. The snow physics outputs from the coupled case are compared against in situ snow stratigraphy observations.

Do Hyuk Kang↗

IPRT Polarized Radiative Transfer Model Intercomparison Project-Phase A

The polarization state of electromagnetic radiation scattered by atmospheric particles such as aerosols, cloud droplets, or ice crystals contains much more information about the optical and microphysical properties than the total intensity alone. For this reason an increasing number of polarimetric observations are performed from space, from the ground and from aircraft. Polarized radiative transfer models are required to interpret and analyse these measurements and to develop retrieval algorithms exploiting polarimetric observations. In the last years a large number of new codes have been developed, mostly for specific applications. Benchmark results are available for specific cases, but not for more sophisticated scenarios including polarized surface reflection and multi-layer atmospheres. The International Polarized Radiative Transfer (IPRT) working group of the International Radiation Commission (IRC) has initiated a model intercomparison project in order to fill this gap. This paper presents the results of the first phase A of the IPRT project which includes ten test cases, from simple setups with only one layer and Rayleigh scattering to rather sophisticated setups with a cloud embedded in a standard atmosphere above an ocean surface. All scenarios in the first phase A of the intercomparison project are for a one-dimensional plane-parallel model geometry. The commonly established benchmark results are available at the IPRT website

radiative transfer↗

Interpretation of Dynamics Explorer far UV images of the quiet time thermosphere

A selected set of far ultra violet images of Earth have been analyzed quanitatively to establish their validity for studying thermospheric weather. The set of images chosen for the study was restricted to mostly geomagnetically quiet conditions in order to obtain a baseline understanding of the relationship between the observations and thermospheric phenomenology. The images included low to modrerate solar activity levels. A new model was developed to generate global dayglow images using first principles methods. The mass Spectrometer/incoherent scatter (MSIS-86) model was used to predict the thermospheric concentrations. The analyses of thermospheric images observed in the 123 to 160-nm nominal passband show that the spectral composition for observations on the projected earth disk is dominated by O I 130.4-nm radiation (85-90%), with concentrations from O I 135.6-nm and N2 Lyman-Birge-Hopefield (LBH) bands of about 5-8% each. The synthetic images reproduce the global features of the observed images rather well. Differences between the model and the data are attributed to real atmospheric effects, such as atomic oxygen depletions which are not well reproduced by the MSIS model when geomagnetic activity is elevated. The absoute values recorded were 38-54% higher than predicted. We attribute this discrepancy to low values of the solar extreme ultraviolet irradiances used in the model. Images obtained in the 136 to 165-nm nominal passband are a factor of 2.7 greater than the model. The excess signal observed is most likely due to a long wavelength tail in the instrument sensitivity which allowed Rayleigh scattered sunlight between 180and 250nm to be detected. The understanding of the Dynamics Explorer (DE 1) images gained by this study provides the basis for future work on the global response of the theremosphere to geomagnetic forcing.

Meier, R. R.↗