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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Mass measurements of neutron-rich gallium isotopes refine production of nuclei of the first r -process abundance peak in neutron-star merger calculations

We report mass measurements of neutron-rich Ga isotopes 80–85 Ga with TRIUMF's Ion Trap for Atomic and Nuclear science. The measurements determine the masses of 80–83 Ga in good agreement with previous measurements. Here, the masses of 84 Ga and 85 Ga were measured for the first time. Uncertainties between 25 and 48 keV were reached. The new mass values reduce the nuclear uncertainties associated with the production of A ≈ 84 isotopes by the r-process for astrophysical conditions that might be consistent with a binary neutron star (BNS) merger producing a blue kilonova. Our nucleosynthesis simulations confirm that BNS merger may contribute to the first abundance peak under moderate neutron-rich conditions with electron fractions Y e = 0.35–0.38.

59 ≤ A ≤ 89↗
DOE OSTI2021

Integral Measurement of the 237 Np($n$, γ) 238 Np Cross Section with Fast Neutrons

Accurate knowledge of the 237 Np($n$; γ) 238 Np cross section at fast neutron energies is important for applied nuclear science. The presently available experimental data has large disagreements in the fast neutron region. A measurement of the 237 Np($n$; γ) 238 Np cross section was performed using a well characterized fast neutron source and the results was compared with previous measurements and current nuclear data evaluations. This will provide an integral measurement that can be used as a benchmark for current evaluations. Multiple samples of 237 Np were irradiated in the Godiva-IV critical assembly. Following the irradiation, the samples placed in a γ-ray counting setup and the γ-rays emitted from the decay of 238 Np were measured over a time period of approximately 7 days. Multiple γ-ray decay branches of 238 Np were observed. The observed activity of 238 Np was used to calculate the amount of 238 Np produced during the irradiation via the 237 Np($n$; γ) 238 Np and an integral cross section of 359(10) mb was measured. The 238 Np half-life has been measured with a result of 50.34(7) hours. An integral measurement of the 237 Np($n$; γ) 238 Np cross section has been measured. This result has been compared to the calculated integral cross section using the ENDF/BVIII.0 and JENDL-4.0 evaluated cross sections and found to be in good agreement with ENDF/BVIII.0 value of 367 mb. The JENDL-4.0 evaluation yields a value of 312 mb, which is significantly lower than the measured cross section.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Enabling Nuclear Systems Through Demonstrations

DOE program launched in October 2019 Authorized by the Nuclear Energy Innovation Capabilities Act (NEICA) DOE-Office of Nuclear Energy; INL Nuclear Science & Tech Partner with industry to bridge the gap between research and commercial deployment Leverage national lab expertise and infrastructure

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2021

Hyperstoichiometric Uranium Dioxides: Rapid Synthesis and Irradiation-Induced Structural Changes

Uranium dioxide (UO 2 ), the primary fuel for commercial nuclear reactors, incorporates excess oxygen forming a series of hyperstoichiometric oxides. Thin layers of these oxides, such as UO 2.12 , form readily on the fuel surface and influence its properties, performance, and potentially geologic disposal. This work reports a rapid and straightforward combustion process in uranyl nitrate–glycine–water solutions to prepare UO 2.12 nanomaterials and thin films. We also report on the investigation of the structural changes induced in the material by irradiation. Despite the simple processing aspects, the combustion synthesis of UO 2.12 has a sophisticated chemical mechanism involving several exothermic steps. Raman spectroscopy and single-crystal X-ray diffraction (XRD) measurements reveal the formation of a complex compound containing the uranyl moiety, glycine, H 2 O, and NO 3 – groups in reactive solutions and dried combustion precursors. Combustion diagnostic methods, gas-phase mass spectroscopy, differential scanning calorimetry (DSC), and extracted activation energies from DSC measurements show that the rate-limiting step of the process is the reaction of ammonia with nitrogen oxides formed from the decomposition of glycine and uranyl nitrate, respectively. However, the exothermic decomposition of the complex compound determines the maximum temperature of the process. In situ transmission electron microscopy (TEM) imaging and electron diffraction measurements show that the decomposition of the complex compound directly produces UO 2 . The incorporation of oxygen at the cooling stage of the combustion process is responsible for the formation of UO 2.12 . Spin coating of the solutions and brief annealing at 670 K allow the deposition of uniform films of UO 2.12 with thicknesses up to 300 nm on an aluminum substrate. Irradiation of films with Ar 2+ ions (1.7 MeV energy, a fluence of up to 1 × 10 17 ions/cm 2 ) shows unusual defect-simulated grain growth and enhanced chemical mixing of UO 2.12 with the substrate due to the high uranium ion diffusion in films. As a result, the method described in this work allows the preparation of actinide oxide targets for fundamental nuclear science research and studies associated with stockpile stewardship.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2024

TEX-HEU: Integral Experiment Execution with Polyethylene at Very Low Temperatures

The low-temperature variant of the TEX HEU (called Low-Temperature TEX or sometimes LT TEX) campaign is a highly anticipated and necessary experimental series by the greater nuclear science community. Fundamentally, the need for low-temperature integral experiments is required to perform validation of cross sections below room temperature. There has been substantial international interest in low-temperature benchmarks to validate below room temperature cross sections, namely talks given at the 2019 International Conference on Nuclear Criticality (ICNC): UK (Watson, 2019), France (Milin, 2019), and UK (Gan & Wilson, 2019). Additionally, NCSP funded thermal scattering laws (TSLs) were produced by North Carolina State University and require low-temperature benchmarks to validate them. Validation of low-temperature cross sections is also necessary for criticality safety applications. One particularly important application is to ensure that during transportation, fissile materials must remain subcritical under normal ambient conditions which is defined as temperatures down to -40°C/°F by the United States 10 CRF 71 as well as a regulation put forward by the International Atomic Energy Agency (IAEA).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

ENDF/B-VIII.1

The ENDF/B-VIII.1 release is the newest evaluated nuclear data library produced, distributed, and recommended by CSEWG for use in nuclear science and technology applications. Among the many key advances, relative to the previous version ENDF/B-VIII.0, are: re-evaluation of 239Pu file by a joint international effort; updated 16,18O, 19F, 28-30Si, 50-54Cr, 55Mn, 54,56,57Fe, 63,65Cu, 139La, 233,235,238U, and 240,241Pu neutron nuclear data by the IAEA-coordinated INDEN collaboration; significant changes for 3He, 6Li, 9Be, 51V, 88Sr, 103Rh, 140,142Ce, Dy, 181Ta, Pt, 206-208Pb, and 234,236U neutron data; new nuclear data for the photo-nuclear, being 196 adopted from the IAEA2019 Photonuclear Data Library and one new file from JENDL-5; and new evaluations for the charged-particle and atomic sublibraries. Numerous thermal neutron scattering kernels were re-evaluated or provided for the very first time. Additionally, new covariance testing was implemented. ENDF/B-VIII.1 reduced bias in the simulations of many integral experiments with particular progress noted for fluorine, copper and stainless steel containing benchmarks. Data issues which had hindered the deployment of ENDF/B-VIII.0 for commercial nuclear power applications in high burn-up situations, were addressed. ENDF/B-VIII.1 data are distributed in both ENDF-6 and GNDS formats.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Perspectives on Potential Advanced Construction Technologies for Nuclear Energy

NRIC Enables Nuclear Reactor Tests & Demonstrations Authorized by the Nuclear Energy Innovation Capabilities Act (NEICA) DOE-Office of Nuclear Energy; INL Nuclear Science & Tech Partner with industry to bridge the gap between research and commercial deployment Leverage national lab expertise and infrastructure

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2022

Uncertainty Quantification of a Light Water Pulsed-Neutron Die-Away Experiment to Thermal Neutron Scattering Laws

Thermal neutron scattering laws are important nuclear data for many nuclear science and engineering applications. Validation helps to ensure that a thermal neutron scattering law has a high quality and often employs critical benchmarks as integral experiments. Recently, pulsed-neutron die-away benchmarks have been used as an experiment to validate thermal neutron scattering laws. Herein, we evidence how this alternative integral experiment has a high sensitivity to these nuclear data by performing an uncertainty quantification analysis. The analysis randomly sampled the nuclear model parameters associated with hydrogen bound in light water thermal neutron scattering law and sampled other nuclear data that influenced the experiment’s integral parameter (e.g., elastic scattering, absorption in hydrogen and oxygen) from their respective covariance matrices. The thermal neutron scattering law caused an uncertainty in the integral parameter that reached 2.67%, which exceeds by an order of magnitude the uncertainties induced in commonly used thermal solution critical benchmarks. The validation performed here, although limited due to a poor description of the historical experiment, indicated that the ENDF/B-VIII.0 thermal neutron scattering law well predicted the integral parameter. These results motivate further benchmark and validation efforts using pulsed-neutron die-away experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Covariant Density Functional Theory in Nuclear Physics and Astrophysics

How does subatomic matter organize itself? Neutron stars are cosmic laboratories uniquely poised to answer this fundamental question that lies at the heart of nuclear science. Newly commissioned rare isotope facilities, telescopes operating across the entire electromagnetic spectrum, and ever more sensitive gravitational wave detectors will probe the properties of neutron-rich matter with unprecedented precision over an enormous range of densities. A coordinated effort between observation, experiment, and theoretical research is of paramount importance for realizing the full potential of these investments. Theoretical nuclear physics provides valuable insights into the properties of neutron-rich matter in regimes that are not presently accessible to experiment or observation. In particular, nuclear density functional theory is likely the only tractable framework that can bridge the entire nuclear landscape by connecting finite nuclei to neutron stars. This compelling connection is the main scope of the present review.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1999

Proton Effects and Test Issues for Satellite Designers: Ionization Effects - Section 4

This portion of the Short Course is divided into two segments to separately address the two major proton-related effects confronting satellite designers: ionization effects and displacement damage effects. While both of these topics are deeply rooted in "traditional" descriptions of space radiation effects, there are several factors at play to cause renewed concern for satellite systems being designed today. For example, emphasis on Commercial Off-The-Shelf (COTS) technologies in both commercial and government systems increases both Total Ionizing Dose (TID) and Single Event Effect (SEE) concerns. Scaling trends exacerbate the problems, especially with regard to SEEs where protons can dominate soft error rates and even cause destructive failure. In addition, proton-induced displacement damage at fluences encountered in natural space environments can cause degradation in modern bipolar circuitry as well as in many emerging electronic and opto-electronic technologies. A crude, but nevertheless telling, indication of the level of concern for proton effects follows from surveying the themes treated in papers presented at this conference. The table lists themes found in the IEEE Transaction on Nuclear Science (TNS) December issue from the past year and compares them with the December issue's content a decade earlier. Ten years ago there were nine papers, or about 10% of the total, dealing with the four indicated topics. At that time, single event effects from protons were the primary concern, and these were thought to be possible only when a nuclear reaction initiated energetic recoil atoms. This is shown in the table as the 'traditional" SEE subject. A decade later, submissions addressing this topic had doubled, while papers devoted to displacement damage studies had increased from one to nine! More importantly, displacement damage effects in the natural space environments have become a concern for degradation in modern devices (other than solar cells), and this was not so ten years earlier.

Marshall, Paul W.↗
DOE OSTI2021

Materials and Fuels Complex Human Performance and Nuclear Safety Culture Pocket Guide

The facilities at the Materials and Fuels Complex (MFC) contain a diverse collection of nuclear research and development capabilities which enable experiments and engineering to drive the world’s nuclear energy future. It is our responsibility to ensure safe, efficient, and reliable operation of MFC facilities to support INL’s nuclear science and technology and national security missions. The MFC management plan makes it clear that safely achieving this takes the right people using good processes.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2023

Epithermal and Fast Neutron Radiography Facility HFIR Futures – Enhanced Capabilities Series (Vol. 8)

The Sustaining and Enhancing Nuclear Science Initiative at Oak Ridge National Laboratory (ORNL) was created to explore potential enhancements to scientific capabilities in the High Flux Isotope Reactor as part of a reactor pressure vessel replacement project. One proposed scientific enhancement included creation of an epithermal and fast neutron radiography station on the HB-3 beam tube with the capability to image highly radioactive specimens such as irradiated nuclear fuel rods, isotope production targets, or spallation neutron target materials. This document summarizes findings and recommendations from a working group of ORNL staff tasked with conceptualizing such a facility and includes a background of similar instruments at other research facilities, technical specifications, and an estimate of procurement cost and schedule.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2023

Cross sections for neutron-induced reactions from surrogate data: Reexamining the Weisskopf-Ewing approximation for ( n , n ' ) and ( n , 2 n ) reactions

Background: Modeling nuclear reaction networks for nuclear science applications and for simulations of astrophysical environments relies on cross section data for a vast number of reactions, many of which have never been measured. Cross sections for neutron-induced reactions on unstable nuclei are particularly scarce, since they are the most difficult to measure. Consequently, we must rely on theoretical predictions or indirect measurements to obtain the requisite reaction data. For compound nuclear reactions, the surrogate reaction method can be used to determine many cross sections of interest. Purpose: Earlier work has demonstrated that cross sections for neutron-induced fission and radiative neutron capture can be determined from a combination of surrogate reaction data and theory. For the fission case, it was shown that the Weisskopf-Ewing approximation, which significantly simplifies the implementation of the surrogate method, can be employed. Capture cross sections cannot be obtained, and require a detailed description of the surrogate reaction process. Here, we examine the validity of the Weisskopf-Ewing approximation for determining unknown (n, n') and (n, 2n) cross sections from surrogate data. Methods: Using statistical reaction calculations with realistic parametrizations, we investigate first whether the assumptions underlying the Weisskopf-Ewing approximation are valid for (n, n') and (n, 2n) reactions on representative target nuclei. We then produce simulated surrogate reaction data and assess the impact of applying the Weisskopf-Ewing approximation when extracting (n, n') and (n, 2n) cross sections in situations where the approximation is not strictly justified. Results: We find that peak cross sections can be estimated using the Weisskopf-Ewing approximation, but the shape of the (n, n') and (n, 2n) cross sections, especially for low neutron energies, cannot be reliably determined without accounting for the angular-momentum differences between the neutron-induced and surrogate reaction. Conclusions: To obtain reliable (n, n') and (n, 2n) cross sections from surrogate reaction data, a detailed description of the surrogate reaction mechanisms is required. To do so for the compound-nucleus energies and decay channels relevant to these reactions, it becomes necessary to extend current modeling capabilities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Building surrogate models of nuclear density functional theory with Gaussian processes and autoencoders

From the lightest Hydrogen isotopes up to the recently synthesized Oganesson (Z = 118), it is estimated that as many as about 8,000 atomic nuclei could exist in nature. Most of these nuclei are too short-lived to be occurring on Earth, but they play an essential role in astrophysical events such as supernova explosions or neutron star mergers that are presumed to be at the origin of most heavy elements in the Universe. Understanding the structure, reactions, and decays of nuclei across the entire chart of nuclides is an enormous challenge because of the experimental difficulties in measuring properties of interest in such fleeting objects and the theoretical and computational issues of simulating strongly-interacting quantum many-body systems. Nuclear density functional theory (DFT) is a fully microscopic theoretical framework which has the potential of providing such a quantitatively accurate description of nuclear properties for every nucleus in the chart of nuclides. Thanks to high-performance computing facilities, it has already been successfully applied to predict nuclear masses, global patterns of radioactive decay like β or γ decay, and several aspects of the nuclear fission process such as, e.g., spontaneous fission half-lives. Yet, predictive simulations of nuclear spectroscopy—the low-lying excited states and transitions between them—or of nuclear fission, or the quantification of theoretical uncertainties and their propagation to basic or applied nuclear science applications, would require several orders of magnitude more calculations than currently possible. However, most of this computational effort would be spent into generating a suitable basis of DFT wavefunctions. Such a task could potentially be considerably accelerated by borrowing tools from the field of machine learning and artificial intelligence. In this paper, we review different approaches to applying supervised and unsupervised learning techniques to nuclear DFT.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

A.I. for nuclear physics

Nuclear science is concerned with the understanding of the nature of matter, its basic constituents and their interaction to form the elements and the properties we observe. This includes the forms of matter we see around us and also exotic forms such as those that existed in the first moments after the Big Bang and that exist today inside neutron stars. The techniques, tools, and expertise needed for nuclear physics (NP) research are therefore diverse in nature. State-of-the art accelerators are being developed to illuminate the dynamical basis of the core of the atom in terms of the fundamental constituents called quarks and gluons and to increase the number of isotopes with known properties. This scientific infrastructure is reaching scales and complexities that require computational methods for tasks such as anomaly detection in operational data. New methodologies are needed to detect anomalies and to optimize operating parameters, predict failures as well as to discover new optimization algorithms.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

FY 2021 Mid-Year HPC Utilization Report M3UF-21IN0701018

Idaho National Laboratory (INL), supported by the Department of Energy Office of Nuclear Energy (DOE-NE) through the Nuclear Science User Facilities, provides access to supercomputer systems and data storage along with support staff for system management, software installation, cybersecurity and user support to the broader DOE-NE user community. Users include individuals at universities, industry, and government laboratories enabling a wide range of research and development and mission-supporting activities. The availability of high-performance computing (HPC) capabilities is a key foundation of collaboration and innovation in nuclear energy systems research. HPC resources and INL directly support the mission and objectives of DOE-NE. From October 2020 through March 2021, INL HPC capabilities were utilized by a diverse set of computing and applied researchers, for a wide range of research and engineering activities. This report focuses on current INL HPC systems and utilization from October 1, 2020 through March 31, 2021.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2024

FY24 accomplishments in preparation for startup of Activated Materials Laboratory (AML)

The Activated Materials Laboratory (AML) will be a new radiological facility at the Advanced Photon Source (APS) in Argonne National Laboratory (ANL), adjacent to the high-energy x-ray microscopy (HEXM) beamline in the long beamline building (LBB) constructed under the APS-upgrade (APS-U) project. The AML is a centralized facility to facilitate the safe conduct of experiments on activated materials at the APS. This report provides an overview of the status of the AML as a Nuclear Science User Facilities (NSUF) partner user facility in preparation for the general user access in 2025 upon the commissioning of the APS-U beamlines. The AML's scope, functionality and components are detailed. The NSUF partner beamlines’ commissioning status in the post-APS-U era is provided, along with the AML’s operational updates and operational plan.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗