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At least 271 records · Page 15

Testing Lunar Permanently Shadowed Regions for Water Ice: LEND Results from LRO

We use measurements from the Lunar Exploration Neutron Detector (LEND) collimated sensors during more than one year of the mapping phase of NASA's Lunar Reconnaissance Orbiter (LRO) mission to make estimates of the epithermal neutron flux within known large Permanently Shadowed Regions (PSRs). These are compared with the local neutron background measured outside PSRs in sunlit regions. Individual and collective analyses of PSR properties have been performed. Only three large PSRs, Shoemaker and Cabeus in the south and Rozhdestvensky U in the north, have been found to manifest significant neutron suppression. All other PSRs have much smaller suppression, only a few percent, if at all. Some even display an excess of neutron emission in comparison to the sunlit vicinity around them. Testing PSRs collectively, we have not found any average suppression for them. Only the group of 18 large PSRs, with area >200 square kilometers, show a marginal effect of small average suppression, approx. 2%, with low statistical confidence. An approx. 2% suppression corresponds to approx. 125 ppm of hydrogen taking into account the global neutron suppression near the lunar poles and assuming a homogeneous H distribution in depth in the regolith. This means that all PSRs, except those in Shoemaker, Cabeus and Rozhdestvensky U craters, do not contain any significant amount of hydrogen in comparison with sunlit areas around them at the same latitude.

LEND↗

Application of recoil-imaging time projection chambers to directional neutron background measurements in the SuperKEKB accelerator tunnel

Gaseous time projection chambers (TPCs) with high readout segmentation are capable of reconstructing detailed 3D ionization distributions of nuclear recoils resulting from elastic neutron scattering. Here, using a system of six compact TPCs with pixel ASIC readout, filled with a 70:30 mixture of He:CO 2 gas, we analyze the first directional measurements of beam-induced neutron backgrounds in the tunnel regions surrounding the Belle II detector at the SuperKEKB e + e – collider. With the use of 3D recoil tracking, we show that these TPCs are capable of maintaining nearly 100% nuclear recoil purity to reconstructed ionization energies (E reco ) as low as 5 keV ee . Using a large sample of Monte-Carlo (MC)-simulated 4 He, 12 C, and 16 O recoil tracks, we find consistency between predicted and measured recoil energy spectra in five of the six TPCs, providing useful validation of the neutron production mechanisms modeled in simulation. Restricting this sample to 4 He recoil tracks with E reco > 40 keV ee , we further demonstrate axial angular resolutions within 8° and we introduce a procedure that under suitable conditions, correctly assigns the vector direction to 91% of these simulated 4 He recoils. Applying this procedure to assign vector directions to measured 4 He recoil tracks, we observe consistency between the angular distributions of observed and simulated recoils, providing first experimental evidence of localized neutron “hotspots” in the accelerator tunnel. Observed rates of nuclear recoils in these TPCs suggest that simulation overestimates the neutron flux from these hotspots. Despite this, we estimate these hotspots to produce the majority of neutron backgrounds in the accelerator tunnel at SuperKEKB’s target luminosity of 6.3 x 10 35 cm –2 s –1 , making them important regions to continue to monitor.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Variance reduction techniques for Monte Carlo neutron noise simulations

The small fluctuations of the neutron flux caused by small perturbations of the macroscopic cross-sections take the name of neutron noise. Advanced Monte Carlo methods have been recently proposed in order to solve the neutron noise equations in the frequency domain, which allows establishing reference solutions to validate faster but approximate deterministic solvers. Due to the presence of particles carrying two statistical weights (for the real and imaginary components of the noise field), both of which may be positive or negative, Monte-Carlo simulations of neutron noise pose distinct challenges in terms of variance reduction. In this work we investigate two variance-reduction techniques, namely branchless collisions and weight cancellation, and probe their effectiveness for a benchmark con- figuration concerning the noise field induced by a pin with oscillating cross sections in a fuel assembly.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

High Flux Isotope Reactor Neutron Spectrum Shape Estimation From Activation Experiment Data

Here, this article provides a comprehensive review of historical irradiation dosimetry available for different locations within the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL). This article includes a summary of the available measured activation target data covering a span of over 15 years and 39 experimental campaigns, including 200 individual sample locations evaluated. Using this broad set of data, we reconstruct historic average neutron spectra shapes for HFIR at various locations, including within the flux trap region, beryllium reflectors, and hydraulic tube (HT) regions, at both the 100- and 85-MW operational power. Our findings indicate that the general axial flux distribution shows a relatively small change in transition from 100- to 85-MW operating power, with differences of -6% to +15% for the thermal energy range and around -16% to +8% for the fast range, indicating a sharper drop-off of the thermal neutron flux away from the axial center. Compared with historical dosimetry estimates of the HFIR flux shape, we generally find a moderately broader axial profile shape for thermal neutrons in the interior target regions for the 100-MW samples evaluated but relatively close agreement for the present 85-MW flux shape for both thermal and fast fluxes.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Westcott g factors extended to arbitrary neutron energy spectra

Westcott 𝑔 factors are used in Neutron Activation Analysis (NAA) and Prompt Gamma-ray Activation Analysis (PGAA) to evaluate the impact of non-1∕𝑣 behavior in the neutron-capture cross sections of certain nuclei on activation product yields. This non-1∕𝑣 behavior arises from the presence of neutron resonances in the neutron- capture cross sections that overlap with the source neutron spectrum at low (< 5 eV) energies. Historically, Westcott 𝑔 factors that have been cataloged for NAA and PGAA applications are the result of calculations that assume a Maxwellian neutron flux distribution with a given temperature. In this work, we use this approach with updated neutron-capture cross sections from the Evaluated Nuclear Data File, version VIII.1 (ENDF/B-VIII.1) to tabulate Westcott 𝑔 factor values for a broad range of Maxwellian distribution temperatures, comparing the results against currently-available 𝑔 factors from International Atomic Energy Agency tables and other sources. Here, it was discovered during this analysis that the use of guided thermal and cold-neutron beams at certain facilities necessitates an approach for evaluating Westcott 𝑔 factors based on arbitrary non-Maxwellian spectra. In this paper, we present an approach for calculating 𝑔 factors with user-specified neutron spectra, and we demonstrate these methods to obtain Westcott 𝑔-factors for guided- and cold-neutron beams at the Budapest Research Reactor and the Forschungsreaktor München II reactor. As part of this work, open-source software has been developed that can be used to perform these calculations for applications in PGAA and NAA experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Leveraging the High Flux Isotope Reactor for nuclear fuel development: a review of experiments, facilities, and capabilities

Materials testing reactors (MTRs) have been used to develop in-core nuclear fuels and materials since the outset of the nuclear power industry. However, the closure of prominent MTRs worldwide and protracted construction timelines for new facilities have increased reliance on existing infrastructure for near-term irradiation testing needs. One facility that can support these needs is the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. HFIR boasts the highest steady-state neutron flux in the Western Hemisphere and, among other roles, has been used to rapidly administer high fluences on fuels and materials for fission and fusion reactor applications. This paper reviews HFIR facilities and infrastructure, fuel-bearing irradiation experiments conducted in HFIR, and select nonfueled experiments that demonstrate advanced techniques transferable to fuels experiments. Collectively, these examples underscore HFIR's potential role as a nuclear fuels testbed supporting both the existing reactor fleet and advanced reactor fuel development.

Fuel qualification↗

Advancing neutron diffraction for accurate structural measurement of light elements at megabar pressures

Over the last 60 years, the diamond anvil cell (DAC) has emerged as the tool of choice in high pressure science because materials can be studied at megabar pressures using X-ray and spectroscopic probes. In contrast, the pressure range for neutron diffraction has been limited due to low neutron flux even at the strongest sources and the resulting large sample sizes. Here, we introduce a neutron DAC that enables break-out of the previously limited pressure range. Key elements are ball-bearing guides for improved mechanical stability, gem-quality synthetic diamonds with novel anvil support and improved in-seat collimation. We demonstrate a pressure record of 1.15 Mbar and crystallographic analysis at 1 Mbar on the example of nickel. Additionally, insights into the phase behavior of graphite to 0.5 Mbar are described. These technical and analytical developments will further allow structural studies on low-Z materials that are difficult to characterize by X-rays.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Validation of neutron emission and neutron energy spectrum calculations on a Mega Ampere Spherical Tokamak with directional relativistic spectrum simulator

The recently developed directional relativistic spectrum simulator (DRESS) code has been validated for the first time against numerical calculations and experimental measurements performed on the Mega Ampere Spherical Tokamak . In this validation, the neutron emissivities and rates computed by DRESS are benchmarked against TRANSP/NUBEAM predictions while the neutron energy spectra provided by DRESS taking as input TRANSP/NUBEAM and ASCOT/BBNBI in Gyro-Orbit mode fast ion distributions are validated against proton pulse height spectra measured by the neutron flux monitor. Finally, excellent agreement was found between DRESS and TRANSP/NUBEAM predictions of local and total neutron emission.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Q1 Report for FY25 Theory and Simulation Performance Target: Development of an integrated modeling framework for fusion reactor design and assessment

This report describes the work and activities carried out towards the completion of each of the following milestones in FY25 Q1: 1. Demonstrate workflow for generating self-consistent CESOL plasma profiles + first wall and divertor loading prediction and generate the CAT plasma and neutron loading needed for further engineering analysis: $/circ$ Initially run CESOL with SOLPS and map heat flux using simple HEAT method: ▪ Generate SOLPS grid for CAT reference case, ▪ Implement and apply ‘lower’ fidelity method of using HEAT-like analytic method to map SOLPS heat flux from charged particles to first wall, and ▪ Provide initial heat flux + neutron loading for further engineering analysis. 2. Demonstrate multiphysics magnet analysis: $/circ$ Demonstrate validation of the Elmer workflow by comparing induced stresses due to EM forces generated by TF coils using multiple codes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Theoretical Yields for 188 W Production in the High Flux Isotope Reactor

Accurately predicting the production yield of 188 W and 191 Os from enriched 186W metal rings irradiated in HFIR is not straightforward. Two key factors can lead to significant uncertainty or inaccuracy in yield predictions: The effect of neutron flux depression in the dense tungsten metal target. Inaccuracy of the currently published 187 W thermal neutron absorption cross section. This manuscript reports the calculated yields for 188 W, 191 Os, and total osmium mass for the NM-888 target that was irradiated in High Flux Isotope Reactor (HFIR) Cycles 487 and 488. Three different yield calculation methods were used and are described herein. The results are presented in terms of total yield and in terms of yield per target mass. This allows for an approximate estimation of yields for future targets of varying mass loading but with similar irradiation profiles. For more accurate prediction yields, target-specific models that account for target loading, target positioning within HFIR, and accurate HFIR cycle data are required.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Energetic particle transport and loss induced by helically-trapped energetic-ion-driven resistive interchange modes in the Large Helical Device

Here, energetic-ion confinement and loss due to energetic-ion driven magnetohydrodynamic modes are studied using comprehensive neutron diagnostics and orbit-following numerical simulations for the Large Helical Device (LHD). The neutron flux monitor is employed in order to obtain global confinement of energetic ions and two installed vertical neutron cameras (VNCs) viewing different poloidal cross-sections are utilized in order to measure the radial profile of energetic ions. A strong helically-trapped energetic-ion-driven resistive interchange mode (EIC) excited in relatively low-density plasma terminated high-temperature state in LHD. Changes in the neutron emission profile due to the EIC excitation are clearly visualized by the VNCs. The reduction in the neutron signal for the helical ripple valley increases with EIC amplitude, which reaches approximately 50%. In addition to the EIC experiment, orbit-following simulations using the DELTA5D code with EIC fluctuations were performed to assess the energetic-ion transport and loss. Two-dimensional temporal evolution results show that the neutron emissivity at the helical ripple decreases significantly due to the EIC. The rapid reduction in neutron emissivity shows that the helically-trapped beam ions immediately escape from the plasma. The reduction in the VNC signals for the helical ripple valley and the total neutron emission rate increase with increasing EIC amplitude, as observed in the experiment. Calculated line-integrated neutron emission results show that the profile measured by VNC1 has one peak, whereas the profile measured by VNC2 has two peaks, as observed in the experiment. Although the neutron emission profile for VNC2 has a relatively wide peak compared with the experimental results, the significant decrease in neutron signal corresponding to the helical ripple valley was successfully reproduced.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Neutron-gamma techniques for planetary exploration

Chemical analysis of planetary surfaces is necessary for the understanding of the origin and evolutionary processes of the solar system. Orbital lunar geochemical experiments performed during the Apollo 15 and 16 demonstrated that even with a low neutron flux (fast and thermal), reliable results could be extracted. The possibility of using a compact 14 MeV neutron generator for geochemical analysis of planetary surfaces, comets and asteroids is currently studied. This method allows the determination of bulk chemical composition, even in the presence of an atmosphere. This would be possible on the surface of Venus, for example, where alternate methods such as sample return are impractical. This method can be used for continuous monitoring of elemental abundances from a roving vehicle, for example, on the surface of Mars.

Johnson, R. G.↗

A Workflow to Optimize Fast Neutron Irradiation in A Thermal Neutron Spectrum Test Reactor Leveraging Open-Source Tools

The Advanced Test Reactor (ATR) located at Idaho National Laboratory (INL) is one of the key nuclear engineering research and testing facilities within the US Department of Energy (DOE). The ATR is one of few high-power research reactors in the world with different application including accelerated testing of nuclear fuel, materials irradiation in a very high neutron flux environment, and medical radioisotope production [1]. Also, the ATR offers opportunities for testing fast spectrum fission and fusion reactor materials. The key challenges in this area are in further detailing and optimizing a fast spectrum environment within a thermal test reactor. This challenge involves researching, developing, and testing novel concepts for the multiplying of neutron populations into ever higher energy spectra in high flux test reactors like ATR. The main objective of this work is to investigate candidate materials for establishing a fast neutron experiment irradiation in thermal neutron spectrum test reactors which can be accomplished by filtering thermal and epithermal neutrons and boosting fast neutrons at designated irradiation positions. However, adding these filters will render the neutron spectrum and the criticality of the system. The selection of the thickness and material layers should be accomplished by developing an optimization design algorithm that is applicable for ATR to enhance the fast neutron spectrum irradiation utilizing high-fidelity Monte Carlo methods along with advanced machine learning capabilities. This paper presents workflow for design optimization to enhance fast neutron irradiation in the ATR. The workflow leverages open-source tools to develop an algorithm that is viable to ATR and can be leveraged in other reactors. The following sections discuss the development of the experiment design optimization workflow and its application to ATR irradiation positions.

42 - ENGINEERING↗

Automated reactor physics analysis framework of High Flux Isotope Reactor low-enriched uranium silicide dispersion fuel designs

The High Flux Isotope Reactor (HFIR) is a versatile research reactor that provides one of the highest steady-state neutron fluxes of any reactor in the world. The HFIR reactor physics team investigated the conversion of the current 93 wt% highly enriched uranium U 3 O 8 -Al dispersion fuel to a 19.75% low-enriched uranium (LEU) U 3 Si 2 -Al dispersion fuel. The team continuously develops a Python module to streamline the analysis steps required for an LEU core design to ensure reproducible and agile design iteration. The Python module automates the data processing between analysis steps and automates the input perturbation for branch calculations and design changes. The automated framework has proven to significantly increase the efficiency and reproducibility of the reactor physics team to design High Flux Isotope Reactor (HFIR) LEU cores and thoroughly analyze performance metrics, safety metrics, and thermal safety margins. Consequently, the team can now respond rapidly to fuel fabrication engineer and thermal-hydraulic-structural analyst requests. Numerous combinations of LEU fuel designs are explored, of which two LEU fuel designs are presented here in this paper: a low density silicide design, and a high-density silicide design. Results show that both designs meet or exceed safety and performance metrics with exception for minor differences caused by the hardened spectrum from LEU.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Insulation Activation and Contamination in Low-Power Experiments

Among the diverse advanced nuclear reactor concepts being developed are designs that expect to operate at much higher temperatures than conventional light-water reactors, and therefore require alternative materials for components capable of withstanding these extreme temperatures. Insulation is one such component where alternative high-temperature industrial composites are being considered. Low-power experiments can provide an opportunity for advancing our understanding of material behavior under irradiation; however, these experiments are not without occupational hazards. The focus of this paper is the potential for activation of insulating composites when exposed to neutron fluence during reactor experiments, and to discuss the subsequent contamination of the testing area. This paper will also discuss practical measures for preventing the creation and inhalation of activated particulate matter (i.e., dust), such as engineering and administrative controls and personal protective equipment. This paper evaluates the suitability of several insulation materials for use in reactor experiments based on their activation from neutron irradiation. The materials considered are Pyrogel XTE by Aspen Aerogel, Cerablanket and Kaowool by Morgan Advanced Materials, Thermo-12 Gold by Johns Manville, and Maxsil CF6-2000 by McAllister Mills. Although these materials are not yet widely used in the nuclear industry, they are common in other industries due to their thermal insulating properties. These materials produce dust while handling that can pose health and safety hazards, which could be further exacerbated by activation. The analysis presented in this paper utilizes a deterministic method developed to predict the activation source term of the provided insulation materials. The method calculates the atomic density of each element within the composites and simulates their exposure to a specified neutron flux density representative of low power experimental conditions. During the irradiation phase and throughout the extensive cooling period, neutron absorptions and nuclear decays are tracked for relevant isotopes. The residual activity within each composite is then assessed to identify the material with the lowest potential radiological hazard to workers. Dust will be created during installation and removal of insulating materials and may also be generated during the experiment. Contamination of surrounding surfaces due to dispersion is highly likely unless preventative measures are taken. The results of this analysis are used to estimate an internal dose from inhalation of activated dust, which is significantly lower than the allowable whole-body dose. However, the risk of internal exposure may increase if the dust becomes a transport vector for nuclear material. The goals of this paper are to enhance the understanding of the potential activation and contamination hazards from the use of these insulating materials in low-power nuclear experiments and to foster safer work environments through informed decision-making and strategic planning. This work ultimately contributes to a broader understanding of how new non-nuclear materials for advanced reactors impact the radiological safety of co-located workers, helping to ensure the responsible management of radioactive materials during installation and decommissioning activities.

12 - MGMT OF RADIOACTIVE AND NON-RADIOACTIVE WASTE↗

AGC-4 As-Run Uncertainty Analysis

The concept of measuring neutron flux (or fluence rate) with activation foils has existed since the late 1940s and is a well-used methodology. Activation foils are selected for their unique isotopic cross sections that create reaction products with desirable properties: relatively simple radioactive decay scheme, measurable quantities of gamma-rays or betas, and half-lives appropriate for the irradiation and decay durations of the experiment. The activation materials, deemed flux wires, fluence wires, dosimeters, or flux foils, are fabricated to have a mass appropriate for the irradiation as well so the measurement using a radiation detector following the irradiation is sufficient but not overwhelming in terms of total activity. Activation measurement results are expressed in terms of reaction rate, which can then be used to “adjust” the neutron spectrum. The Advanced Graphite Creep (AGC)-4 experiment contained 26 flux wire packages, each containing an iron and a niobium wire inside a vanadium capsule. For all stackup positions, the value of fast to thermal neutrons is higher than expected, but the total neutron fluence is near the predicted value of ~2 x 1022 n/cm2. As compared to the predicted neutron spectrum, there are four takeaways in the results as compared to the predicted ATR irradiation: 1) Additional fast (fission) neutrons present, 2) Spectrum hardening due to temperature, 3) Spectrum hardening due to container attenuation, 4) Total neutron fluence is close to predicted values. Since the neutron energy spectrum is a key parameter when attributing neutron damage in materials, the adjusted energy-dependent spectrum and the total neutron fluence results from the dosimeters can be incorporated for future calculations.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High average-flux laser-driven neutron source

Laser-driven neutron generation is an attractive alternative to more established methods for compact, short-pulse-duration neutron sources with applications in medical science, material science and imaging. Despite extensive investigation of various techniques, achieving performance comparable to nuclear reactors or conventional accelerators remains challenging. In this work, we generate a stable, high-repetition-rate laser-driven neutron source reaching a record average flux of 7.8 × 10 7 n/sr/s, improving on other existing laser-based sources by more than one order of magnitude. Our approach is based on a two-step process where electrons are accelerated to relativistic energies via laser wakefield acceleration (LWFA), and subsequently generate neutrons through Bremsstrahlung emission followed by photonuclear reactions in a tungsten converter. Experimental results, supported by Monte Carlo simulations, show a neutron flux of 3.0 × 10 7 n/cm 2 /s near the target, on par with some compact accelerator-based neutron sources. Additionally, a direct comparison with the target-normal sheath acceleration (TNSA) pitcher-catcher scheme, performed on the same laser system, reveals a significantly higher total neutron yield of 3.9 × 10 8 neutrons per shot, outperforming the TNSA scheme by several orders of magnitude. These findings represent a significant advancement towards the development of practical laser-driven neutron sources and highlight the advantages of LWFA-based neutron generation for future applications.

Vallières, Simon [Institut National de la Recherch↗

Development of Large Bore Rabbit Capsules in Support of BWR Cladding Irradiations in HFIR

The High Flux Isotope Reactor (HFIR) is an ideal tool for materials irradiation testing because of its intense steady-state neutron flux. Many programs take advantage of HFIR’s central flux trap for irradiation experiments using capsules, also known as rabbits, to support advanced materials development and reactor design. The facility that makes up the HFIR flux trap has recently undergone a design change that increases the HFIR primary coolant volumetric flow rate by removing restrictions in the system. As a result, the usable cross-sectional area within the facility increased, opening the door to increase the cross-sectional area of the rabbit capsules that fill the facility. This report documents a new large-diameter rabbit housing that increases the usable volume within the rabbit capsule by 22.6%. However, challenges arise with increasing the capsule size, such as establishing a new maximum capsule operating pressure and determining the thermal-hydraulic characteristics. This report addresses those challenges with previously adopted HFIR safety methods. The rupture pressure of the rabbit housings is demonstrated while verifying that capsule swelling during and after rupture will not block coolant flow. Then, a safety factor is applied to ascertain an administrative operating pressure. Additionally, the thermal-hydraulic performance of the HFIR facility filled with large-diameter rabbit capsules is shown to not violate previously determined safety criteria. Next, heat transfer coefficients are determined for use in design calculations. Furthermore, this report gives an example of internal configurations for the new, larger rabbit capsules that use relevant boiling water reactor (BWR) cladding geometry. Finally, this report documents an example thermal design performance for a rabbit capsule containing six gauge-curved tensile tube specimens. The thermal performance gives predicted temperature distributions within the capsule and shows the expected temperature of the passive thermometers for post-irradiation temperature comparisons.

99 GENERAL AND MISCELLANEOUS↗