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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

3D xRAGE simulation of inertial confinement fusion implosion with imposed mode 2 laser drive asymmetry

Low-mode asymmetries represent an important obstacle to achieving high-gain inertial confinement fusion implosions. As a step in learning how to control such effects, an OMEGA experiment with imposed mode 2 laser drive asymmetries was done to study the expected signatures of this type of asymmetry [M. Gatu Johnson et al., PRE 2018]. In the present work, a 3D xRAGE simulation including the stalk mount has been brought to bear on the data from that experiment. Furthermore, comprehensive comparisons between simulated and measured observables are made. Good agreement between simulated and measured x-ray image-inferred shell trajectories, bang times and neutron emission widths are seen, showing that the hydrodynamics are well captured in the simulation. Asymmetries seen in simulated and measured time-resolved and time-integrated x-ray images and areal densities also compare well, showing impact of both stalk and mode 2. On the other hand, important differences in measured and simulated neutron emission histories, yield, and ion temperature (T ion ) asymmetries are seen, suggesting that the simulation is overestimating shock yield. Overall, the results clearly demonstrate the importance of considering all asymmetry sources when interpreting measured signatures of asymmetry.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Benchmark calculations of infinite neutron matter with realistic two- and three-nucleon potentials

In this study, we present the equation of state of infinite neutron matter as obtained from highly realistic Hamiltonians that include nucleon-nucleon and three-nucleon coordinate-space potentials. We benchmark three independent many-body methods: Brueckner-Bethe-Goldstone (BBG), Fermi hypernetted chain/single-operator chain (FHNC/SOC), and auxiliary-field diffusion Monte Carlo (AFDMC). We find them to provide similar equations of state when the Argonne v 18 and the Argonne v' 6 nucleon-nucleon potentials are used in combination with the Urbana IX three-body force. Only at densities larger than about 1.5 the nuclear saturation density ( ρ 0 =0.16 fm ⁻3 ) the FHNC/SOC energies are appreciably lower than the other two approaches. The AFDMC calculations carried out with all of the Norfolk potentials fitted to reproduce the experimental trinucleon ground-state energies and nd doublet scattering length yield unphysically bound neutron matter, associated with the formation of neutron droplets. Including tritium β decay in the fitting procedure, as in the second family of Norfolk potentials, mitigates but does not completely resolve this problem. An excellent agreement between the BBG and AFDMC results is found for the subset of Norfolk interactions that do not make neutron-matter collapse, while the FHNC/SOC equations of state are moderately softer.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Mass-asymmetric fission of 205,207,209 Bi at energies close to the fission barrier using proton bombardment of 204,206,208 Pb

Background: Recent observation of mass-asymmetric fission in neutron-deficient Hg and Pt nuclei has reignited interest in fission fragment mass distributions close to Pb. Investigations at energies close to the fission barrier, where mass-asymmetric fission is expected to be most obvious and the sensitivity to shell effects is maximized, are limited in this mass region. Purpose: To measure fission mass distributions for 205,207,209 Bi nuclei at the lowest possible excitation energies to determine how the mass distributions change with excitation energy and the neutron number of the compound nucleus. Method: Proton beams bombarding targets of 204,206,208 Pb were used to study the fission of 205,207,209 Bi at energies from just above to 10 MeV above their fission barriers. Fission fragments were measured using the CUBE fission spectrometer. Fission fragment mass distributions were determined using a newly developed time difference analysis method. Mass distributions were characterized by triple-Gaussian fits to determine the systematic trends across each isotope with excitation energy. Results: Measured mass distributions of all three Bi isotopes exhibit a component of mass-asymmetric fission at all energies studied. The probability of mass-asymmetric fission decreases significantly with increasing excitation energy, from ≈70 to ≈40% over a 10-MeV range. Comparisons between the three Bi isotopes hint at an increase in the mass-symmetric fission yield with increasing neutron number, which could be due to a decrease in the difference between the symmetric and asymmetric fission barriers. The centroids of the mass-asymmetric peaks suggest that several deformed shell gaps in the fission fragments could be contributing to the presence of the mass-asymmetric fission mode with Z light ≃ 38, Z heavy ≃ 45, and N light ≃ 56 all present in the fission fragments. Conclusions: Measurements of fission mass distributions at the lowest possible excitation energies above the fission barrier provide an excellent platform to investigate the origins of the mass-asymmetric fission mode. Finally, further systematic measurements at these energies offer an opportunity to rigorously test new models of fission in this mass region.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Reviewing Incident Neutron Energy assignments in 238 U(n,f) Fission Yield Data

Fission yield evaluations rely not only on precise measurements, but also on clear documentation of experimental conditions especially the energy of incident neutrons inducing fission. In the EXFOR database, following the convention adopted in past evaluations, the incident neutron energy has traditionally been divided in only three energy groups: thermal, fast and 14 MeV. The information is stored in the EN-DUMMY field, which often serves as a placeholder in the presence of broad-spectrum or reactor-based sources. This work reviews 238 U(n,f) entries in EXFOR that use EN-DUMMY, identifying cases where better energy estimates can be made based on the original publications, facility characteristics, or reconstructed neutron spectra. We assign new cross-section-weighted average energies where possible. The revised independent and cumulative fission yield data are compiled for future use in model development and evaluation efforts.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Complex Structural Disorder in a Polar Orthorhombic Perovskite Observed through the Maximum Entropy Method/Rietveld Technique

Ambient pressure stable perovskite oxides with all Bi3+ on the A-site are rare, with only four examples known. Due to the lone pair on Bi 3+ , these materials are seen as the best alternative to Pb-based piezoelectrics, which are used widely in society. The industry standard piezoelectric, Pb (Zr 1 – x Ti x )O 3 , relies on the [001] polarization of PbTiO 3 , but there are currently no ambient pressure stable Bi-based perovskites with this polarization vector, preventing the creation of an analogous system. We present the full structural analysis of the orthorhombic phase of (1 – x)Bi (Ti 3/8 Fe 2/8 Mg 3/8 )O 3 – x CaTiO 3 , which crystallizes in Pna2 1 symmetry with [001] polarization. This symmetry is rare and has only been reported twice for perovskites at ambient conditions. Analysis of maximum entropy method (MEM) models using synchrotron radiation powder X-ray diffraction reveals a disordered A-site configuration, and the MEM/Rietveld technique generates a structural model of this extreme disorder. Combined Rietveld analysis of X-ray and neutron diffraction data yields an accurate description of the local A-site configuration, which we use to understand our dielectric, ferroelectric, and piezoelectric measurements. These results give insight into how to stabilize this unique symmetry and inspire new design principles for Bi-based piezoelectrics.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Efficiency enhancement of thermonuclear DD reaction in femtosecond laser plasma with the use of structured low-average-density targets

An increase in the yield of fast neutrons is experimentally demonstrated by exciting a nuclear DD reaction in the interaction of a relativistically intense (over 10{sup 18} W cm{sup −2}) ultrashort laser pulse with a deuterated low-average-density target volume-structured at the wavelength scale. It is shown that decreasing the average target density from 0.78 to 0.35 g cm{sup −3} doubles the neutron flux, which reaches 7 × 10{sup 4} particles per 1 J of input energy. The effect may be associated with an increase in the number of accelerated deuterium ions due to the three dimensional expansion of individual elements of the target structure. (paper)

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Nucleosynthesis in outflows of compact objects and detection prospects of associated kilonovae

ABSTRACT We perform a comparative analysis of nucleosynthesis yields from binary neutron star (BNS) mergers, black hole-neutron star (BHNS) mergers, and core-collapse supernovae (CCSNe) with the goal of determining which are the most dominant sources of r-process enrichment observed in stars. We find that BNS and BHNS binaries may eject similar mass distributions of robust r-process nuclei post-merger (up to third peak and actinides, A ∼ 200−240), after accounting for the volumetric event rates. Magnetorotational (MR) CCSNe likely undergo a weak r-process (up to A ∼ 140) and contribute to the production of light element primary process (LEPP) nuclei, whereas typical thermal, neutrino-driven CCSNe only synthesize up to first r-process peak nuclei (A ∼ 80−90). We also find that the upper limit to the rate of MR CCSNe is $\lesssim 1~{{\ \rm per\ cent}}$ the rate of typical thermal CCSNe; if the rate was higher, then weak r-process nuclei would be overproduced. Although the largest uncertainty is from the volumetric event rate, the prospects are encouraging for confirming these rates in the next few years with upcoming surveys. Using a simple model to estimate the resulting kilonova light curve from mergers and our set of fiducial merger parameters, we predict that ∼7 BNS and ∼2 BHNS events will be detectable per year by the Vera C. Rubin Observatory (LSST), with prior gravitational wave (GW) triggers.

Astronomy & Astrophysics↗
DOE OSTI2022

LLE Diagnostic Resource Team for Innovative Fusion Concepts (Final Report)

The LLE Diagnostic Resource Team for Innovative Fusion Concepts provided travelling neutron diagnostics, consultancy on neutron diagnostics, and consultancy on tritium handling to fusion companies. An existing neutron detector was recalibrated for low yields and two detectors were built based on designs proven on the Omega Laser Facility. The three detectors allow measurements over a wide range of yields (from 10 to 1E7 incident neutrons). The detectors were calibrated for DD neutrons on a dedicated OMEGA shot day. Neutron detectors from the company MIFTI were also calibrated on OMEGA. MIFTI is currently using their detectors and two of our detectors on staged Z-pinch experiments at UCSD. The Team acted as consultants for the development of a liquid scintillator array to detect neutrons from muon induced fusion by NK Labs. Segments of NK Labs’ detector were tested at the LLE using radioactive sources and a DD neutron generator. The Team also acted as consultants for the design of a tritium handling system for NK Labs. A new type of neutron spectrometer was designed and built, and has completed preliminary testing.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1985

The secondary radiation under Saturn's A-B-C rings produced by cosmic ray interactions

On the basis of a study of spacecraft data of Saturn, Chenette et al. (1980) concluded that highly relativistic galactic cosmic ray nuclei with magnetic rigidities greater than the Stoermer rigidity cutoff in the plane of Saturn's A-B-C rings along the Pioneer 11 trajectory produced a secondary population of charged particles. The existence of this secondary particle population was confirmed by Randall (1982). Cooper and Simpson (1980) further developed this concept of secondary production of nucleons by cosmic ray nuclei to estimate the yield of secondary neutrons which might, through decay, populate the radiation belt with low-energy electrons and protons. Cooper (1983) reported quantitative Monte Carlo calculations of neutron production in the rings and their decay in the magnetosphere. The present investigation is concerned with a confirmation of the earlier work, and an extension of the studies on the basis of improved spectra for the proton and electron components.

Cooper, J. F.↗
NASA NTRS2002

Nuclear model calculations and their role in space radiation research

Proper assessments of spacecraft shielding requirements and concomitant estimates of risk to spacecraft crews from energetic space radiation requires accurate, quantitative methods of characterizing the compositional changes in these radiation fields as they pass through thick absorbers. These quantitative methods are also needed for characterizing accelerator beams used in space radiobiology studies. Because of the impracticality/impossibility of measuring these altered radiation fields inside critical internal body organs of biological test specimens and humans, computational methods rather than direct measurements must be used. Since composition changes in the fields arise from nuclear interaction processes (elastic, inelastic and breakup), knowledge of the appropriate cross sections and spectra must be available. Experiments alone cannot provide the necessary cross section and secondary particle (neutron and charged particle) spectral data because of the large number of nuclear species and wide range of energies involved in space radiation research. Hence, nuclear models are needed. In this paper current methods of predicting total and absorption cross sections and secondary particle (neutrons and ions) yields and spectra for space radiation protection analyses are reviewed. Model shortcomings are discussed and future needs presented. c2002 COSPAR. Published by Elsevier Science Ltd. All right reserved.

NASA Center JSC↗
DOE OSTI2022

Neutronic design and fuel cycle analysis of a fluoride salt-cooled High Temperature Reactor (FHR)

The Fluoride salt-cooled High temperature Reactor (FHR) is a new Gen IV reactor concept that can operate under near atmospheric pressure circumstances and further enhance the inherent safety. In this study, an FHR core design with 165 megawatts of thermal output (MWth) is proposed. The reactor core employs tri-structural-isotropic (TRISO) particle fuel within prismatic graphite blocks as the basic fuel form, FLiBe (2 {sup 7}LiF-BeF{sub 2}) as the primary coolant, and a three-batch fuel cycle scheme. Sensitivity analyses on various parameters were performed to optimize the cycle length and neutronic parameters. The fuel cycle of this core design was evaluated in detail from 4 aspects: cycle length, power peaking factor (PPF), discharge burnup, and temperature coefficient. It was found that larger fuel channel pitch (FCP) would have a relatively harder neutron spectrum, and yield relatively longer cycle length, lower, better fuel temperature coefficient (FTC), and moderator temperature coefficient (MTC). In addition, burnable poison (BP), Er{sub 2}O{sub 3}, can effectively reduce PPF, hold down the multiplication factor, and more importantly it can improve the MTC. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2021

Top-level physics requirements and simulated performance of the MRSt on the National Ignition Facility

The time-resolving Magnetic Recoil Spectrometer (MRSt) for the National Ignition Facility (NIF) has been identified by the US National Diagnostic Working Group as one of the transformational diagnostics that will reshape the way inertial confinement fusion (ICF) implosions are diagnosed. The MRSt will measure the time-resolved neutron spectrum of an implosion, from which the time-resolved ion temperature, areal density, and yield will be inferred. Top-level physics requirements for the MRSt were determined based on simulations of numerous ICF implosions with varying degrees of alpha heating, P2 asymmetry, and mix. Synthetic MRSt data were subsequently generated for different configurations using Monte–Carlo methods to determine its performance in relation to the requirements. The system was found to meet most requirements at current neutron yields at the NIF. This work was supported by the DOE and LLNL.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Fission Product Yields of 233 U and 239 Pu by Neutron-Induced Fission at Neutron Energies from 0.18-140 MeV [Slides]

Nuclear fission is an important process with applications in astrophysics, nuclear reactors, and stockpile stewardship. Despite having been discovered over 80 years ago, fission is not fully described by a predictive model. This study will show fission product mass yields and total kinetic energies (TKE) across a large range of incident neutron energies for future refinement of fission models. 233U(n,f) data is used to verify features and structures on a previous experiment and compared against fission models. 239Pu(n,f) data will be analyzed to show new data at higher neutron energies using techniques to handle fission in the presence of alphas. 252Cf(sf) data will be used for calibration and benchmarking with a thin-backed target.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2021

Top-level physics requirements and simulated performance of the MRSt on the National Ignition Facility

The time-resolving Magnetic Recoil Spectrometer (MRSt) for the National Ignition Facility (NIF) has been identified by the US National Diagnostic Working Group as one of the transformational diagnostics that will reshape the way inertial confinement fusion (ICF) implosions are diagnosed. The MRSt will measure the time-resolved neutron spectrum of an implosion, from which the time-resolved ion temperature, areal density, and yield will be inferred. Top-level physics requirements for the MRSt were determined based on simulations of numerous ICF implosions with varying degrees of alpha heating, P2 asymmetry, and mix. Synthetic MRSt data were subsequently generated for different configurations using Monte–Carlo methods to determine its performance in relation to the requirements. The system was found to meet most requirements at current neutron yields at the NIF. This work was supported by the DOE and LLNL.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Characterization of D-T Generator Neutron Flux Spectrum for Cyclic Neutron Activation Analysis Experiments

Improving nuclear data for short-lived fission product yields will further our fundamental understanding of fission, which is needed across various scientific fields and applications. One method of attaining the needed product yield data is through cyclic neutron activation, which allows a target to be irradiated in a neutron environment and then transported for counting of the radionuclides produced, typically via g spectroscopy. Recently, such a system has been constructed and commissioned at Pacific Northwest National Laboratory. Targets are shuttled between the head of a D-T neutron generator and a counting station with a transit time of 2 seconds. As part of the characterization of this system, the neutron flux was studied using two activation targets. The neutron flux from the deuterium-tritium fusion generator was determined to be 9.95(33) x10^8 n/cm2-s with a peak energy of 14.9 MeV and a spread of approximately 4 decades between the epithermal and 14 MeV peak group flux.

cyclic neutron activation, gamma-ray spectroscopy,↗
DOE OSTI2023

Impact of temperature on light yield and pulse shape discrimination of polysiloxane-based organic scintillators formulated with commercial resins

This work investigates how increased temperature affects neutron/ discrimination and light yield (LY) in several different polysiloxane-based scintillators doped with either 9,9-dimethyl-2-phenylflourene (PhF) or 2,5-diphenyloxazole (PPO) as a primary fluorophore and 9,9-dimethyl-2,7-di((E)-styryl) fluorene (SFS) as the secondary fluorophore. The polysiloxane matrices were prepared from the commercial resins Wacker Lumisil 579 or Shin-Etsu KER-6000. Control scintillators were prepared from poly(vinyltoluene) (PVT), the industry standard matrix, as a reference point for LY and pulse shape discrimination (PSD) measurements. Samples with PhF and PPO dopant concentrations of 1 wt% and 5 wt% in the polysiloxanes and 3 wt% and 5 wt% in the PVT samples were tested at 20 °C, 35 °C, and 50 °C. In the polysiloxane samples, the KER-6000 resin outperformed the Wacker 579 and PhF proved to be a better dopant than PPO in both LY and PSD capabilities. Polysiloxane scintillators showed slight decreases in LY and increases in neutron/discrimination at increased temperatures, while PVT scintillators showed a similar LY decrease with little to no improvement in neutron/discrimination at increased temperatures. Altogether, polysiloxane scintillators may not require recalibration in applications where temperatures increase up to 50 °C.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Measuring the β-decay Properties of Neutron-rich Exotic Pm, Sm, Eu, and Gd Isotopes to Constrain the Nucleosynthesis Yields in the Rare-earth Region

Abstract The β -delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing β -decay half-life ( T 1/2 ) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and β -delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A ≈ 160 in the r -process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of 168 Sm and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167–172.

79 ASTRONOMY AND ASTROPHYSICS↗