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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Magnetization reversal in magnetic dot arrays: Nearest-neighbor interactions and global configurational anisotropy

Various proposals for future magnetic memories, data processing devices, and sensors rely on a precise control of the magnetization ground state and magnetization reversal process in periodically patterned media. In finite dot arrays, such control is hampered by the magnetostatic interactions between the nanomagnets, leading to the non-uniform magnetization state distributions throughout the sample while reversing. In this paper, we evidence how during reversal typical geometric arrangements of dots in an identical magnetization state appear that originate in the dominance of either Global Configurational Anisotropy or Nearest-Neighbor Magnetostatic interactions, which depends on the fields at which the magnetization reversal sets in. Based on our findings, we propose design rules to obtain the uniform magnetization state distributions throughout the array, and also suggest future research directions to achieve non-uniform state distributions of interest, e.g., when aiming at guiding spin wave edge-modes through dot arrays. Our insights are based on the Magneto-Optical Kerr Effect and Magnetic Force Microscopy measurements as well as the extensive micromagnetic simulations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Search for giant magnetic anisotropy in transition-metal dimers on defected hexagonal boron nitride sheet

Structural and magnetic properties of many transition-metal dimers embedded in a defected hexagonal boron nitride monolayer are investigated through density functional calculations to search for systems with magnetic anisotropy energies (MAEs) larger than 30meV. In particular, Ir–Ir@Dh–BN is found to have both large MAE (∼126 meV) and high structural stability against dissociation and diffusion, and it hence can serve as magnetic unit in spintronics and quantum computing devices. This giant MAE mainly results from the spin orbit coupling and the magnetization of the upper Ir atom, which is in a rather isolated environment.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

NONTHERMALLY DOMINATED ELECTRON ACCELERATION DURING MAGNETIC RECONNECTION IN A LOW-β PLASMA

By means of fully kinetic simulations, we investigate electron acceleration during magnetic reconnection in a nonrelativistic proton–electron plasma with conditions similar to solar corona and flares. We demonstrate that reconnection leads to a nonthermally dominated electron acceleration with a power-law energy distribution in the nonrelativistic low-β regime but not in the high-β regime, where β is the ratio of the plasma thermal pressure and the magnetic pressure. The accelerated electrons contain most of the dissipated magnetic energy in the low-β regime. A guiding-center current description is used to reveal the role of electron drift motions during the bulk nonthermal energization. We find that the main acceleration mechanism is a Fermi-type acceleration accomplished by the particle curvature drift motion along the electric field induced by the reconnection outflows. Although the acceleration mechanism is similar for different plasma β, low-β reconnection drives fast acceleration on Alfvénic timescales and develops power laws out of thermal distribution. The nonthermally dominated acceleration resulting from magnetic reconnection in low-β plasma may have strong implications for the highly efficient electron acceleration in solar flares and other astrophysical systems.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Evolution of magnetic interactions in Sb-substituted MnBi 2 Te 4

The Mn(Bi 1–x Sb x ) 2 Te 4 series is purported to span from an antiferromagnetic (AF) topological insulator at x = 0 to a trivial AF insulator at x = 1. Here we report on neutron diffraction and inelastic neutron scattering studies of the magnetic interactions across this series. All compounds measured possess ferromagnetic (FM) triangular layers and we find a crossover from AF to FM interlayer coupling near x = 1 for our samples. The large spin gap at x = 0 closes rapidly and the average FM exchange interactions within the triangular layer increase with Sb substitution. Similar to a previous study of MnBi 2 Te 4 , we find severe spectral broadening which increases dramatically across the compositional series. In addition to broadening, we observe an additional sharp magnetic excitation in MnSb 2 Te 4 that may indicate the development of local magnetic modes originating from antisite disorder between Mn and Sb sublattices. Here, the results suggest that both substitutional and antisite disorder contribute substantially to the magnetism in Mn(Bi 1–x Sb x ) 2 Te 4 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Novel Transformer with Variable Leakage and Magnetizing Inductances

This paper introduces the concept of a novel variable inductance transformer (VIT) whose leakage and magnetizing inductances can be varied dynamically and independently to aid the advancement of research in isolated power electronic converters. In this transformer, the leakage inductance can be varied by varying the length of overlap between the primary and secondary windings, while the magnetizing inductance can be varied by varying the air gap between the core legs. Individual controls for the two inductances ensure that one can be varied independent of the other, as needed to satisfy different power conversion objectives. In this paper, the analytical models of the variable leakage and magnetizing inductances are presented. Analytical results are compared with those obtained from Finite Element Method (FEM) and an experimental prototype of a VIT. Analytical solutions of the variable leakage inductance present an error of less than 2.35 % when compared to FEM solutions, while the analytical solutions of the variable magnetizing inductance present a maximum error of 1.82 % when compared to experimental measurements.

image method, leakage inductance, magnetizing indu↗
DOE OSTI2024

Effect of different grain boundary diffusion alloys on magnetic properties of Dy-free sintered NdFeB magnet

Dy-free sintered magnets were fabricated by blending Neo powder with different grain boundary diffusion alloy powders. Cu, CeAl and CeAlCu have a negative effect on H cj of magnets, while PrAlCu and AlCuGa have a positive effect. The PrAlCu-added magnet achieves the best magnetic properties among all magnets with the additions of different diffusion alloys. With increasing PrAlCu from 0-10 wt.%, H cj of the magnets gradually increases from the original 14.5 kOe to 19.2 kOe. The magnet with 7.5 wt.% PrAlCu obtains a H cj of 18 kOe and (BH) max of 39.1 MGOe. It is found that Pr and Cu in PrAlCu alloy is mainly distributed at grain boundary and triple junctions, leading to a reduced coupling among grains, thus an enhanced H cj . Here, the grain boundary engineering by adding an appropriate alloy is an effective method to improve H cj of Dy-free NdFeB magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Effect of Exchange Interaction Constants on the Magnetization Reversal in a Hard/Soft Magnetic Bilayer Model

A model is developed to study a hard/soft magnetic bilayer in an external magnetic field by the Monte Carlo method. The influence of the constants of the exchange intralayer and interlayer interactions of the hard magnetic and soft magnetic layers on the magnetization reversal in the magnetic bilayer is investigated. The formation of a spin spring is shown to be mainly determined by the exchange interaction in the soft magnetic layer. Phase diagrams are plotted for the magnetic bilayer.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Formation of gapless Z{sub 2} spin liquid phase manganites in the (Sm{sub 1–y}Gd{sub y}){sub 0.55}Sr{sub 0.45}MnO{sub 3} system in zero magnetic field: Topological phase transitions to states with low and high density of 2D-vortex pairs induced by the magnetic field

The evolution of the ground state of the manganese spin ensemble in the (Sm{sub 1–y}Gd{sub y}){sub 0.55}Sr{sub 0.45}MnO{sub 3} in the case of isovalent substitution of rare-earth samarium ions with large radii with gadolinium ions with significantly smaller radii is studied. The measured temperature dependences of the ac magnetic susceptibility and the field dependences of the dc magnetizations are analyzed using the Heisenberg–Kitaev model describing the transition from the ordered spin state with classical isotropic AFM exchange to the frustrated spin state with quantum highly anisotropic FM exchange. A continuous transition from the 3D ferromagnetic state of manganese spins in the initial sample with y = 0 to zigzag AFM ordering of CE-type spins in ab planes for y = 0.5, coexisting in samples with y = 0.5, 0.6, and 0.7 at temperatures below T{sub N} ≅ 48.5 K with a disordered phase such as a quantum Griffiths phase is identified. As the gadolinium concentration further increases, the CE-type zigzag AFM structure is molten, which leads to the appearance of an unusual phase in Gd{sub 0.55}Sr{sub 0.45}MnO{sub 3} in the temperature range close to the absolute zero. This phase has characteristic features of a gapless Z{sub 2} quantum spin liquid in zero external magnetic field. The step changes in the magnetization isotherms measured at 4.2 K in the field range of ±75 kOe are explained by quantum phase transitions of the Z{sub 2} spin liquid to a phase with topological order in weak magnetic fields and a polarized phase in strong fields. The significant difference between critical fields and magnetization jumps in isotherms indicates the existence of hysteretic phenomena in quantum spin liquid magnetization–demagnetization processes caused by the difference between localization–delocalization of 2D vortex pairs induced by a magnetic field in a quantum spin liquid with disorder.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Strategic coating of NdFeB magnets with Dy to improve the coercivity of permanent magnets

Here, we present a method, supported by theoretical analysis, for optimizing the usage of the critical rare earth element dysprosium in Nd 2 Fe 14 B (NdFeB)-based permanent magnets. In this method, we use Dy selectively in locations such as magnet edges and faces, where demagnetization factors are most significant, rather than uniformly throughout the bulk sample. A 200 nm thick Dy film was sputtered onto commercial N-38, NdFeB magnets with a thickness of 3 mm and post-annealed at temperatures from 600 - 700 C. Magnets displayed enhanced coercivities after post-annealing. Furthermore, our experimental results indicate as large as a 5 percent increase in the energy product of NdFeB magnets, achieved for a total Dy weight percentage of 0.06 percent, much less than that used in commercial grade Dy-NdFeB magnets. Finally, by assuming all Dy diffused into NdFeB magnets, the improvement in energy product corresponds to a saving of over 1% Dy (critical element). Magnets manufactured using this technique will therefore be higher performing and significantly less expensive than those made presently.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Collaborative Research: Effects of the magnetic field shear and flow shear on the kinetic physics and particle acceleration in relativistic magnetic reconnection (Final Report)

Magnetic reconnection is a fundamental plasma process that allows rapid changes of magnetic field topology and the conversion of magnetic energy into plasma kinetic energy. There has been a strong surge of interest in relativistic reconnection over the past few years in plasma astrophysics, but the rich physics of collisionless reconnection and its associated particle acceleration in the relativistic regime remain less studied compared to the non-relativistic counterparts. Magnetic reconnection in a realistic system is often accompanied with the magnetic field shear and shear flows. This setting is more general and likely the more common situation where most reconnection takes place. Within the past few decades, researchers had made significant progress in understanding how magnetic reconnection works under these conditions in the non-relativistic regime. However, how the effect of special relativity, among other effects, influences the dynamics of reconnection in the strongly magnetized astrophysical plasmas under these conditions is largely unknown. Our proposed research is to use fully kinetic simulations to understand kinetic physics and particle acceleration in relativistic magnetic reconnection in more realistic configurations and physical conditions. The primary goal of this project is to identify the fundamental effects caused by special relativity under the presence of field shear and flow shear.

43 PARTICLE ACCELERATORS↗
DOE OSTI2016

POLARIZATION SIGNATURES OF RELATIVISTIC MAGNETOHYDRODYNAMIC SHOCKS IN THE BLAZAR EMISSION REGION. I. FORCE-FREE HELICAL MAGNETIC FIELDS

The optical radiation and polarization signatures in blazars are known to be highly variable during flaring activities. It is frequently argued that shocks are the main driver of the flaring events. However, the spectral variability modelings generally lack detailed considerations of the self-consistent magnetic field evolution modeling; thus, so far the associated optical polarization signatures are poorly understood. We present the first simultaneous modeling of the optical radiation and polarization signatures based on 3D magnetohydrodynamic simulations of relativistic shocks in the blazar emission environment, with the simplest physical assumptions. By comparing the results with observations, we find that shocks in a weakly magnetized environment will largely lead to significant changes in the optical polarization signatures, which are seldom seen in observations. Hence an emission region with relatively strong magnetization is preferred. In such an environment, slow shocks may produce minor flares with either erratic polarization fluctuations or considerable polarization variations, depending on the parameters; fast shocks can produce major flares with smooth polarization angle rotations. In addition, the magnetic fields in both cases are observed to actively revert to the original topology after the shocks. All these features are consistent with observations. Future observations of the radiation and polarization signatures will further constrain the flaring mechanism and the blazar emission environment.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Magnetic structure and magnetodielectric behavior of the chiral magnet CoTeMoO 6

We investigate the magnetic structure and magnetodielectric behavior of the chiral magnet CoTeMoO 6 (CTMO) through neutron diffraction, magnetization, and magnetodielectric measurements, complemented by density functional theory (DFT) calculations. Our findings reveal a canted magnetic structure with moments confined to the ab plane, giving rise to weak ferromagnetism under an external magnetic field. Additionally, we observe magnetodielectric coupling that strongly correlates with the magnetic ordering temperature and magnetic structure. Furthermore, these results are discussed in the context of potential mechanisms involving spin-dependent p-d hybridization and spin-phonon coupling.

Canted magnetism↗
DOE OSTI2018

Model-free reconstruction of magnetic correlations in frustrated magnets

Frustrated magnetic systems exhibit extraordinary physical properties, but quantification of their magnetic correlations poses a serious challenge to experiment and theory. Current insight into frustrated magnetic correlations relies on modelling techniques such as reverse Monte-Carlo methods, which require knowledge about the exact ordered atomic structure. Here, we present a method for direct reconstruction of magnetic correlations in frustrated magnets by three-dimensional difference pair distribution function analysis of neutron total scattering data. The methodology is applied to the disordered frustrated magnet bixbyite, (Mn 1– x Fe x ) 2 O 3 , which reveals nearest-neighbor antiferromagnetic correlations for the metal sites up to a range of approximately 15 Å. Pertinently, this technique allows for magnetic correlations to be determined directly from the experimental data without any assumption about the atomic structure.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Magnetic order in the structurally disordered helicoidal magnet Cr{sub 1/3}NbS{sub 2}: NMR at {sup 53}Cr nuclei

The Cr{sub 1/3}NbS{sub 2} magnet is studied by nuclear magnetic resonance (NMR) at {sup 53}Cr nuclei in a zero applied magnetic field. The following two frequency ranges are distinguished in the {sup 53}Cr NMR spectrum at T = 4.2 K: ν{sub 1} = 64–68 MHz and ν{sub 2} = 49–51 MHz. They can be related to two valence states of chromium ions, namely, Cr{sup 4+} and Cr{sup 3+}. The components of the electric field gradient, the hyperfine fields, and the magnetic moment at chromium atoms are determined. The NMR data demonstrate that the magnetic moments of chromium lie in plane ab and form a magnetic structure consisting of regions with a helicoidal magnetic order and regions where this order is broken.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Magnetic Solitons and Thickness‐Dependent Magnetization Reversal in Interconnected Helical Nanowire Arrays

By expanding magnetic nanostructures into the third dimension, it is possible to introduce new interactions and realize new forms of magnetic textures and emergent phenomena. Consequently, this unlocks new opportunities for applications in data storage, unconventional computing and sensing by utilizing 3D devices with enhanced functionalities. Connected magnetic nanowires offer a unique platform for applications such as neuromorphic computing due to their tunability and the presence of multiple transport pathways. However to realize this promise, it is necessary to further our understanding of how to locally control the magnetization in 3D, nanowire-based geometries. In this work we show the formation of magnetic domain walls, vortices, anti-vortices, and linked vortex-anti-vortex pairs in interconnected helical nanowire arrays. We show how wire diameter and 3D geometric design can control the states that form and reveal the magnetization reversal mechanism. Hence, we demonstrate this to be a highly tunable system, where the magnetization can be readily reconfigured by an external magnetic field.

3D Nanomagnetism↗
DOE OSTI2020

Tunable Magnetic Exchange between Rare-Earth Metal 5d and Iron 3d States: A Case Study of the Multiple Magnetic Transitions in Gd 6 FeBi 2 and the Solid Solutions Dy 6– x Gd x FeBi 2 (1 ≤ x ≤ 5) with Curie Temperatures in the Range 120–350 K

In this paper, the room-temperature magnet Gd 6 FeBi 2 was comprehensively characterized by means of temperature-dependent single-crystal X-ray diffraction, magnetization measurements, and experimental electron density and electronic structure computations. This work explores the electron-spin effects of Fe on this structure and suggests that Gd6FeBi2 shows structural features and exchange interactions, which are clearly distinguishable from other analogues, including the solid solutions Dy 6–x Gd x FeBi 2 (0 ≤ x ≤ 5). The unique traits of Gd 6 FeBi 2 and its derivatives encompass abnormal variations of lattice parameters with the temperature, as well as the presence of multiple magnetic transitions of complex nature. Based on the comprehensive analyses, it can be suggested that the unique magnetic response in this material is the result from tunable Fe spin states, which are coupled with strong Gd 5d–Fe 3d interactions, which differ from other members of this large, structural family. In the ground state, according to density functional theory calculations, the Fe atom carries two net electrons, whose spins are coupled in an antiparallel fashion to the spins of the Gd electrons. Near the Curie temperature, the Fe net moment is reduced intermittently, coupled with a multiple of magnetic transitions. The magnetic correlations are manifested in unexpected variations of the lattice parameters as a function of temperature, suggesting spin–lattice interactions. Furthermore, this study emphasizes the important role of Gd 5d electrons in tuning Fe 3d-based magnetic contribution, which enables better understanding on the spin coupling in other related compounds and sheds light on the development of new magnetic and spintronic compounds.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Canting of the Magnetic Moments on the Octahedral Site of an Iron Oxide Garnet in Response to Diamagnetic Cation Substitution

Using neutron powder diffraction and magnetic susceptibility measurements, we report on the preparation and characterization of the temperature- and field-dependent properties of CaY2ZrFe4O12, a composition closely related to the high-temperature ferrimagnet Y3Fe5O12. By diluting the concentration of paramagnetic ions on the octahedral sublattice of the garnet structure, we find temperature-dependent canting of the magnetic moments. This reflects the importance of the octahedral sublattice in mediating the magnetic interactions between the tetrahedral sites and offers insight into a large number of competing magnetic interactions in the garnet structure.

Milam-Guerrero, JoAnna↗
DOE OSTI2024

Magnetic Solitons in Hierarchical 3D Magnetic Nanoarchitectures of Nanoflower Shape

Curvilinear magnetism emerged as a new route to tailor properties of magnetic solitons by the choice of geometry and topology of a magnetic architecture. Here, we develop an anodized aluminum oxide template-based approach to realize hierarchical 3D magnetic nanoarchitectures of nanoflower shape. The technique provides defect-free regular arrays of magnetic nanoflowers of tunable shape with a period of 400 nm over cm 2 areas. We combined advanced magnetic imaging methods with micromagnetic simulations to study complex magnetic states in nanoflowers originating due to magnetostatics-driven symmetry break in curvilinear nanomembranes. An interaction between surface and volume magnetostatic charges in 3D curved nanoflowers leads to the stabilization of asymmetric and shifted vortices as well as states with two Bloch lines. Ordered large area arrays of complex-shaped magnetic nanoarchitectures developed in this work are relevant for prospective research on 3D magnonics and spintronics.

3D nanoarchitectures↗