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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 271 records · Page 15
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

A New Candidate Laser Dye Based 1,4-Bis[β-(2-Naphthothiazolyle)Vinyl]Benzene. Spectroscopic Behavior, Laser Parameters and Excitation Energy Transfer

A new candidate laser dye based 1,4-bis[β-(2-naphthothisolyl) vinyl] benzene (BNTVB) were prepared, and characterized in various organic solvents. The center polarity is less sensitive than electronic absorption. A red shift was noticed in the fluorescence spectra (ca. 40 nm) with increment in the solvent’s polarity, this means that BNTVB’s polarity appreciates upon excitation. The dipole moment of ground state (μ{sub g}) and the excited singlet state dipole moment (μ{sub e}) are determined from Kawski – Chamma and Bakshiev–Viallet equations using the disparity of Stokes shift with solvent polarity function of ε (dielectric constant) and n (refractive index) of the solvent. The result was found to be 0.019D and 5.13D for ground and exited state, in succession. DFT/TD-DFT manners were used to understand the electronic structures and geometric of BNTVB in other solvents. The experimental and theoretical results showed a good agreement. The photochemical quantum yield (Ф{sub c}) of BNTVB was calculated in variable organic reagents such as Dioxane, CHCl{sub 3}, EtOH and MeOH at room temperature. The values of φ{sub c} were calculated as 2.3 × 10{sup −4}, 3.3 × 10{sup −3}, 9.7 × 10{sup −5} and 6.2 × 10{sup −5} in Dioxane, CHCl{sub 3}, EtOH and MeOH, respectively. The dye solutions (2 × 10{sup −4} M) in DMF, MeOH and EtOH give laser emission in the blue-green region. The green zone is excited by nitrogen pulse 337.1 nm. The tuning range, gain coefficient (α) and cross – section emission (σ{sub e}) of laser were also estimated. Excitation energy transfer from BNTVB to rhodamine-6G (R6G) and N,N-bis(2,6-dimethyphenyl)-3,4:9,10-perylenebis-(dicarboximide) (BDP) was also studied in EtOH to increase the laser emission output from R6G and BDP when excited by nitrogen laser. The dye-transfer power laser system (ETDL) obeys the Foster Power Transmission (FERT) mechanism with a critical transmission distance, R{sub o} of 40 and 32 A and k{sub ET} equals 2.6 × 10{sup 13} and 1.06 × 10{sup 13} M{sup −1} s{sup −1} for BNTVB / R6G and BNTVB / BDP pair, respectively.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2021

End-gas autoignition fraction and flame propagation rate in laser-ignited primary reference fuel mixtures at elevated temperature and pressure

Knock in spark-ignited (SI) engines is initiated by autoignition of the unburned gasses upstream of spark-ignited, propagating, turbulent premixed flames. Knock propensity of fuel/air mixtures is typically quantified using research octane number (RON), motor octane number (MON), or methane number (MN; for gaseous fuels), which are measured using single-cylinder, variable compression ratio engines. In this study, knock propensity of SI fuels was quantified via observations of end-gas autoignition (EGAI) in unburned gasses upstream of laser-ignited, premixed flames at elevated pressures and temperatures in a rapid compression machine. Stoichiometric primary reference fuel (PRF; n-heptane/isooctane) blends of varying reactivity (50 ≤ PRF ≤ 100) were ignited using an Nd:YAG laser over a range of temperatures and pressures, all in excess of 545 K and 16.1 bar. Laser ignition produced outwardly-propagating premixed flames. High-speed pressure measurements and schlieren images indicated the presence of EGAI. The fraction of the total heat release attributed to EGAI (i.e., EGAI fraction) varied with fuel reactivity (i.e., octane number) and the time-integrated temperature of the end-gas prior to ignition. Flame propagation rates, which were measured using schlieren images, were only weakly correlated with octane number but were affected by turbulence caused by variation in piston timing. Under conditions of low turbulence, measured flame propagation rates approached one-dimensional premixed laminar flame speed computations performed at the same conditions. Experiments were simulated with a three-dimensional CONVERGE™ model using reduced chemical kinetics (121 species, 538 reactions). The simulations accurately captured the measured flame propagation rates, as well as the variation in EGAI fraction with fuel reactivity and time-integrated end-gas temperature. The simulations also revealed low-temperature heat release as well as formaldehyde and hydrogen peroxide formation in the end-gas upstream of the propagating flame, which increased the temperature and degree of chain branching in the end-gas, ultimately leading to EGAI.

42 ENGINEERING↗
DOE OSTI2019

Tripled yield in direct-drive laser fusion through statistical modelling [Tripling the yield in direct-drive laser fusion via predictive statistical modeling]

Focusing laser light onto a very small target can produce the conditions for laboratory-scale nuclear fusion of hydrogen isotopes. The lack of accurate predictive models, which are essential for the design of high-performance laser-fusion experiments, is a major obstacle to achieving thermonuclear ignition. Here we report a statistical approach that was used to design and quantitatively predict the results of implosions of solid deuterium–tritium targets carried out with the 30-kilojoule OMEGA laser system, leading to tripling of the fusion yield to its highest value so far for direct-drive laser fusion. When scaled to the laser energies of the National Ignition Facility (1.9 megajoules), these targets are predicted to produce a fusion energy output of about 500 kilojoules—several times larger than the fusion yields currently achieved at that facility. As a result, this approach could guide the exploration of the vast parameter space of thermonuclear ignition conditions and enhance our understanding of laser-fusion physics.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Optimization of laser-target parameters for the production of stable lithium beam

A laser ion source coupled with a radio frequency quadrupole linac accelerator is being proposed as a suitable system for the production of a low energy, high-current stable lithium beam. In order to maximize the lithium yield, plasmas generated by laser ablation of different materials based on lithium (Li, LiOH, and LiNbO3) have been characterized by using a Faraday cup and an electrostatic ion analyzer in the time of flight configuration. A wide range of laser power density has been investigated (109–1012 W/cm2) using two Nd:YAG lasers operating at different wavelengths (1064 nm and 532 nm), pulse durations (6 ns and 17 ns), and maximum energies (1400 mJ and 210 mJ). This paper outlines the pros and cons of the investigated materials by studying how the ion energy, yields, and charge state distributions are modified when the laser power density is changed. Considerable attention has been paid to the higher charge states of oxygen, which may occur with the same mass-to-charge ratio of Li3+. The analysis has evidenced that LiNbO3 represents a valid target since it allows minimizing the O6+/7Li3+ ratio down to 2.5% by using a laser power density of 1.8 × 1010 W/cm2. For such a condition, a Li3+ current of 1.4 mA/cm2 has been measured.

Cannavò, A. (ORCID:0000000309759630)↗
DOE OSTI2021

Absolute laser energy absorption measurement of relativistic 0.7 ps laser pulses in nanowire arrays

Laser absorption is one of the most important parameters governing laser–matter interactions. The laser energy absorption on nanowire array targets is measured for the first time in the relativistic regime at intensities of 10 19 W=cm 2 and compared to foil targets. The results show that the laser energy absorption of 0.7 ps frequency doubled (527 nm) pulses on Au nanowire targets varies widely with nanowire parameters, reaching laser energy absorption values up to 71% of the incident energy, significantly exceeding those of solid flat targets obtained in similar irradiation conditions. The analysis shows that the increase in absorption strongly correlates with larger effective target surface area over a broad range of nanowire parameters explored. These direct absorption measurements provide valuable data to benchmark simulations of the relativistic laser pulse interactions with nanostructures.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Planar laser induced fluorescence mapping of a carbon laser produced plasma

We present measurements of ion velocity distribution profiles obtained by laser induced fluorescence (LIF) on an explosive laser produced plasma. The spatiotemporal evolution of the resulting carbon ion velocity distribution was mapped by scanning through the Doppler-shifted absorption wavelengths using a tunable, diode-pumped laser. The acquisition of these data was facilitated by the high repetition rate capability of the ablation laser (1 Hz), which allowed for the accumulation of thousands of laser shots in short experimental times. By varying the intensity of the LIF beam, we were able to explore the effects of fluorescence power against the laser irradiance in the context of evaluating the saturation vs the non-saturation regime. The small size of the LIF beam led to high spatial resolution of the measurement compared to other ion velocity distribution measurement techniques, while the fast-gate operation mode of the camera detector enabled the measurement of the relevant electron transitions.

Instruments & Instrumentation↗
DOE OSTI2025

Demonstration of full-scale spatiotemporal diagnostics of solid-density plasmas driven by an ultra-short relativistic laser pulse using an X-ray free-electron laser

Understanding the complex plasma dynamics in ultra-intense relativistic laser–solid interactions is of fundamental importance for applications of laser–plasma-based particle accelerators, the creation of high-energy-density matter, understanding planetary science, and laser-driven fusion energy. However, experimental efforts in this regime have been limited by the lack of accessibility of over-critical densities and the poor spatiotemporal resolution of conventional diagnostics. Over the last decade, the advent of femtosecond brilliant hard X-ray free-electron lasers (XFELs) has opened new horizons to overcome these limitations. Here, for the first time, we present full-scale spatiotemporal measurements of solid-density plasma dynamics, including preplasma generation with tens of nanometer scale length driven by the leading edge of a relativistic laser pulse, ultrafast heating and ionization at the main pulse arrival, the laser-driven blast wave, and transient surface return current-induced compression dynamics up to hundreds of picoseconds after interaction. These observations are enabled by utilizing a novel combination of advanced X-ray diagnostics including small-angle X-ray scattering, resonant X-ray emission spectroscopy, and propagation-based X-ray phase-contrast imaging simultaneously at the European XFEL-HED beamline station.

Huang, Lingen [Helmholtz-Zentrum Dresden-Rossendor↗
DOE OSTI2018

On-Chip Laser-Power Delivery System for Dielectric Laser Accelerators

We propose an on-chip optical-power delivery system for dielectric laser accelerators based on a fractal “tree-network” dielectric waveguide geometry. Here, this system replaces experimentally demanding free-space manipulations of the driving laser beam with chip-integrated techniques based on precise nanofabrication, enabling access to orders-of-magnitude increases in the interaction length and total energy gain for these miniature accelerators. Based on computational modeling, in the relativistic regime, our laser delivery system is estimated to provide 21 keV of energy gain over an acceleration length of 192 μm with a single laser input, corresponding to a 108-MV/m acceleration gradient. The system may achieve 1 MeV of energy gain over a distance of less than 1 cm by sequentially illuminating 49 identical structures. These findings are verified by detailed numerical simulation and modeling of the subcomponents, and we provide a discussion of the main constraints, challenges, and relevant parameters with regard to on-chip laser coupling for dielectric laser accelerators.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Role of Direct Laser Acceleration of Electrons in a Laser Wakefield Accelerator with Ionization Injection

We show the first experimental demonstration that electrons being accelerated in a laser wakefield accelerator operating in the forced or blowout regimes gain significant energy from both the direct laser acceleration (DLA) and the laser wakefield acceleration mechanisms. Supporting full-scale 3D particle-in-cell simulations elucidate the role of the DLA of electrons in a laser wakefield accelerator when ionization injection of electrons is employed. An explanation is given for how electrons can maintain the DLA resonance condition in a laser wakefield accelerator despite the evolving properties of both the drive laser and the electrons. The produced electron beams exhibit characteristic features that are indicative of DLA as an additional acceleration mechanism.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Laser and optical transport line for laser-based ion beam diagnostics and control in the SNS linear accelerator

We report our recent upgrade of the laser and optical transport line for the laser-based ion beam diagnostics (laser wire) system at the linear accelerator (linac) of the Spallation Neutron Source (SNS). A new light source based on diodepumped solid-state laser amplifiers has been developed to provide near diffraction-limited laser beam with a variety of pulse structures. The free-space optical transport line has been modified to include image relay optics with remote control, which greatly improved the laser beam quality and position stability at individual measurement stations. The upgraded system enables novel beam diagnostics/control capabilities including longitudinal profile measurement and high-energy proton beam extraction from the SNS linac.

Liu, Yun↗
DOE OSTI2021

Advanced laser development and plasma-physics studies on the multiterawatt laser

The Multi-Terawatt (MTW) laser, built initially as the prototype front-end for a petawatt laser system, is a 1053-nm hybrid system with gain from optical parametric chirped-pulse amplification (OPCPA) and Nd:glass. Here, compressors and target chambers were added, making MTW a complete laser facility (output energy up to 120 J, pulse duration from 20 fs to 2.8 ns) for studying high-energy-density physics and developing short-pulse laser technologies and target diagnostics. Further extensions of the laser support ultrahigh-intensity laser development of an all-OPCPA system and a Raman plasma amplifier. A short summary of the variety of scientific experiments conducted on MTW is also presented.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

Experimental longitudinal emittance manipulation using laser-based photoionization in the Fermilab Linac

A series of simulations and beam studies were conducted at Fermilab’s linear accelerator to evaluate the effectiveness of longitudinal emittance control via laser-induced photoionization. While similar laser techniques have been employed at Fermilab to enhance injection and extraction efficiency into the Booster, the work presented here focuses on extending these methods to bunch-by-bunch manipulation. This approach utilizes fine-scale correction of the H- bunches’ longitudinal spatial distribution. In theory, loosely confined particles in longitudinal phase space contribute to emittance growth during acceleration. By selectively removing these outlying particles through laser scraping (H- + γ → H + e-), this growth can be reduced. This report presents experimental results from both symmetric and asymmetric longitudinal scraping of H⁻ bunches in the Fermilab linac, which were subsequently injected into Booster, and evaluates the broader applicability of this method for future high-intensity accelerator operations.

Landon, Parker [Boston U.; Fermilab]↗
DOE OSTI2018

X-Ray Diffraction Measurements on Laser-Compressed Polycrystalline Samples Using a Short-Pulse Laser Generated X-Ray Source

Existing models for most materials do not describe phase transformations and associated lattice dy- namics (kinetics) under extreme conditions of pressure and temperature. Dynamic x-ray diffraction (DXRD) allows material investigations in situ on an atomic scale due to the correlation between solid-state structures and their associated diffraction patterns. In this LDRD project we have devel- oped a nanosecond laser-compression and picosecond-to-nanosecond x-ray diffraction platform for dynamically-compressed material studies. A new target chamber in the Target Bay in building 983 was commissioned for the ns, kJ Z-Beamlet laser (ZBL) and the 0.1 ns, 250 J Z-Petawatt (ZPW) laser systems, which were used to create 8-16 keV plasma x-ray sources from thin metal foils. The 5 ns, 15 J Chaco laser system was converted to a high-energy laser shock driver to load material samples to GPa stresses. Since laser-to-x-ray energy conversion efficiency above 10 keV is low, we employed polycapillary x-ray lenses for a 100-fold fluence increase compared to a conventional pinhole aperture while simultaneously reducing the background significantly. Polycapillary lenses enabled diffraction measurements up to 16 keV with ZBL as well as diffraction experiments with ZPW. This x-ray diffraction platform supports experiments that are complementary to gas guns and the Z facility due to different strain rates. Ultimately, there is now a foundation to evaluate DXRD techniques and detectors in-house before transferring the technology to Z. This page intentionally left blank.

36 MATERIALS SCIENCE↗
DOE OSTI2022

A study of sacrificial mirrors for use prior to a laser wakefield accelerator driven by the Z-Petawatt laser

Many experiments at Sandia’s Z Pulsed Power Facility require x-ray backlighting diagnostics to understand experiment performance. Due to limitations in present-day source/detection modalities, most x-ray diagnostics at Z are restricted to photon energies <20 keV, ultimately limiting the density, amount, and atomic number of targets diagnosable in experiments. These limitations force the use of low-Z materials like Beryllium, and they prevent acquisition of important backlighting data for materials/densities that are opaque to soft x-rays and where background emission from the Z load and transmission lines overwhelm diagnostics. In this LDRD project, we have investigated the design and development of a laser wakefield acceleration platform driven by the Z-Petawatt laser – a platform that would enable the generation of a pulsed, collimated beam of high energy x-rays up to 100 keV. Geometrical considerations for implementation on the Z Machine require the use of sacrificial mirrors, which have been tested in offline experiments in the Chama target chamber in building 983. Our results suggest the use of sacrificial mirrors would not necessarily inhibit the laser wakefield x-ray process, particularly with the benefits stemming from planned laser upgrades. These conclusions support the continuation of laser wakefield source research and the development of the necessary infrastructure to deliver the Z-Petawatt laser to the Z center section along the appropriate lines of sight. Ultimately, this new capability will provide unprecedented views through dense states of matter, enabling the use of previously incompatible target materials/designs, and uncovering a new set of observables accessible through diffraction and spectroscopy in the hard x-ray regime. These will amplify the data return on precious Z shots and enhance Sandia’s ability to investigate fundamental physics in support of national security.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Ion Channel Laser Based on Direct Laser Acceleration of a Shaped Beam Driver (Final Technical Report)

The main focus of our research was to understand the synergies between an electron bunch and a laser pulse when the two co-propagate through the plasma. We have clearly demonstrated using theoretical and computational modeling that the propagation distance of both the bunch and the laser pulse could be extended. The ability of the combined bunch/pulse system to extend the propagation distance and the size of the plasma bubble enables highly-efficient sources of relativistic electrons. As pointed out by the Plasma Decadal Study, such electron sources can be used for generating extremely bright x-rays for a variety of applications can serve as probes and diagnostics for other plasma experiments: high energy density (HED) sciences, inertial confinement fusion (ICF), and potentially Fusion Materials and Technology (FM&T). Development of advanced diagnostics of plasma-based accelerators is yet another key area identified by recent reports. Even broader security and medical applications of compact accelerator-based radiation sources, such as very high energy electron (VHEE) sources for FLASH radiobiology, have been identified by a recent multi-agency panel. A number of key technical issues were considered and successfully resolved during the course of the grant. Those include: beam loading effect of both the driver and witness bunches on the wake, laser channeling by the bunch, and the direct laser acceleration (DLA) of the driver bunch by the laser pulse. To demonstrate clear synergy, we were able to ascertain that the total energy gain of a witness bunch in the wake of the combined bunch/laser complex is large than the sum of the energy gains in the wake of the laser pulse alone, and the driver bunch alone. We have also demonstrated that not only the energy gain is improved, but the energy spread is not sacrificed. To carry out these simulations, we have to develop a range of in-house computational tools, including a fully-3D code WAND-PIC.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Analysis of High-Power Diode Laser Heating Effects on HY-80 Steel for Laser Assisted Friction Stir Welding Applications

In this research, several conditions of high power diode laser heated HY-80 steel were characterized to determine the viability of using such lasers as a preheating source before friction stir welding in order to reduce frictional forces thereby reducing tool wear and increasing welding speeds. Differences in microstructures within heat affected zones were identified at specific laser powers and traverse speeds. Vickers hardness values were recorded and analyzed to validate the formation of additional martensite in diode laser heated regions of HY-80 steel. Conditions that produced little to no additional martensite were identified and relationships among high power diode laser power, traverse speed, and martensite formation were determined. The development of heat affected zones, change in grain structure, and creation of additional martensite in HY-80 can be prevented through the optimization of laser amperage and transverse speed.

36 MATERIALS SCIENCE↗
NASA NTRS1973

Laser scanning methods and a phase comparison, modulated laser range finder for terrain sensing on a Mars roving vehicle

Two areas of a laser range finder for a Mars roving vehicle are investigated: (1) laser scanning systems, and (2) range finder methods and implementation. Several ways of rapidly scanning a laser are studied. Two digital deflectors and a matrix of laser diodes, are found to be acceptable. A complete range finder scanning system of high accuracy is proposed. The problem of incident laser spot distortion on the terrain is discussed. The instrumentation for a phase comparison, modulated laser range finder is developed and sections of it are tested.

Herb, G. T.↗