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At least 271 records · Page 15

Harmonic and reactive behavior of the quasiparticle tunnel current in SIS junctions

In this paper, we show theoretically and experimentally that the reactive quasiparticle tunnel current of the superconductor tunnel junction could be directly measured at specific bias voltages for the higher harmonics of the quasiparticle tunnel current. We used the theory of quasiparticle tunneling to study the higher harmonics of the quasiparticle tunnel current in superconducting tunnel junction in the presence of rf irradiation. The impact of the reactive current on the harmonic behavior of the quasiparticle tunnel current was carefully studied by implementing a practical model with four parameters to model the dc I-V characteristics of the superconducting tunnel junction. The measured reactive current at the specific bias voltage is in good agreement with our theoretically calculated reactive current through the Kramers-Kronig transform. This study also shows that there is an excellent correspondence between the behavior of the predicted higher harmonics using the previously established theory of quasiparticle tunnel current in superconducting tunnel junctions by J.R. Tucker and M.J. Feldman and the measurements presented in this paper.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Generation of harmonics and supercontinuum in nematic liquid crystals

Nonlinear optical properties of nematic liquid crystals (NLC) have been investigated. A technique for efficient laser frequency conversion in a microscopic NLC volume deposited on an optical fibre end face is experimentally demonstrated. An efficient design of a compact NLC-based IR frequency converter with a fibre input and achromatic collimator is proposed and implemented. Simultaneous generation of the second and third harmonics is obtained for the first time under pumping NLC by a 1.56-mm femtosecond fibre laser. The second-harmonic generation efficiency is measured to be about 1 %, while the efficiency of third-harmonic generation is several tenths of percent. A strong polarisation dependence of the third-harmonic generation efficiency is revealed. When pumping NLC by a cw laser, generation of spectral supercontinua (covering the visible and near-IR spectral ranges) is observed. The nonlinear effects revealed can be due to the light-induced change in the orientational order in liquid crystals, which breaks the initial symmetry and leads to formation of disclination structures. The NLC optical nonlinearity is believed to be of mixed orientationalelectronic nature as a whole. (laser optics 2012)

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Bright circularly polarized soft X-ray high harmonics for X-ray magnetic circular dichroism

Significance The new ability to generate circularly polarized coherent (laser-like) beams of short wavelength high harmonics in a tabletop-scale setup is attracting intense interest worldwide. Although predicted in 1995, this capability was demonstrated experimentally only in 2014. However, all work to date (both theory and experiment) studied circularly polarized harmonics only in the extreme UV (EUV) region of the spectrum at wavelengths >18 nm. In this new work done in a broad international collaboration, we demonstrate the first soft X-ray high harmonics with circular polarization to wavelengths λ < 8 nm and the first tabletop soft X-ray magnetic circular dichroism (XMCD) measurements, and also uncover new X-ray light science that will inspire many more studies of circular high-harmonic generation (HHG).

36 MATERIALS SCIENCE↗

Attosecond synchronization of extreme ultraviolet high harmonics from crystals

The interaction of strong near-infrared (NIR) laser pulses with wide-bandgap dielectrics produces high harmonics in the extreme ultraviolet (XUV) wavelength range. These observations have opened up the possibility of attosecond metrology in solids, which would benefit from a precise measurement of the emission times of individual harmonics with respect to the NIR laser field. In this work, we show that, when high-harmonics are detected from the input surface of a magnesium oxide crystal, a bichromatic probing of the XUV emission shows a clear synchronization largely consistent with a semiclassical model of electron–hole recollisions in bulk solids. On the other hand, the bichromatic spectrogram of harmonics originating from the exit surface of the 200 μm-thick crystal is strongly modified, indicating the influence of laser field distortions during propagation. Our tracking of sub-cycle electron and hole re-collisions at XUV energies is relevant to the development of solid-state sources of attosecond pulses.

74 ATOMIC AND MOLECULAR PHYSICS↗

Macroscopic scaling of high-order harmonics generated by two-color optimized waveforms in a hollow waveguide

We present the macroscopic scaling of high harmonics generated by two-color laser pulses interacting with Ne gas in a hollow waveguide. We demonstrate that the divergence of harmonics is inversely proportional to the waveguide radius and harmonic yields are proportional to the square of the waveguide radius when the gas pressure and waveguide length are chosen to meet the phase-matching condition. We also show that harmonic yields are inversely proportional to the ionization level of the optimized two-color waveform with proper gas pressure if waveguide radius and length are fixed. These scaling relations would help experimentalists find phase-matching conditions to efficiently generate tabletop high-flux coherent soft x rays for applications.

74 ATOMIC AND MOLECULAR PHYSICS↗

Generation of circularly polarized XUV and soft-x-ray high-order harmonics by homonuclear and heteronuclear diatomic molecules subject to bichromatic counter-rotating circularly polarized intense laser fields

Recently, studies of bright circularly polarized high-harmonic beams from atoms in the soft-x-ray region as a source for x-ray magnetic circular dichroism measurement in a tabletop-scale setup have received considerable attention. In this paper, we address the problem with molecular targets and perform a detailed quantum study of H 2 +, CO, and N 2 molecules in bichromatic counter-rotating circularly polarized laser fields where we adopt wavelengths (1300 and 790 nm) and intensities (2 × 10 14 W/cm 2 ) reported in a recent experiment [Proc. Natl. Acad. Sci. USA 112, 14206 (2015)]. Our treatment of multiphoton processes in homonuclear and heteronuclear diatomic molecules is nonperturbative and based on the time-dependent density-functional theory for multielectron systems. The calculated radiation spectrum contains doublets of left and right circularly polarized harmonics with high-energy photons in the XUV and soft-x-ray ranges. Overall, our results reveal intriguing and substantially different nonlinear optical responses for homonuclear and heteronuclear diatomic molecules subject to circularly polarized intense laser fields. We study in detail the below- and above-threshold harmonic regions and analyze the ellipticity and phase of the generated harmonic peaks.

74 ATOMIC AND MOLECULAR PHYSICS↗

Controlling electron quantum paths for generation of circularly polarized high-order harmonics by H 2 + subject to tailored (ω, 2ω) counter-rotating laser fields

Recently, studies of high-order harmonics (HHG) from atoms driven by bichromatic counter-rotating circularly polarized laser fields as a source of coherent circularly polarized extreme ultraviolet (XUV) and soft-x-ray beams in a tabletop-scale setup have received considerable attention. Here, we demonstrate the ability to control the electron recollisions giving three returns per one cycle of the fundamental frequency ω by using tailored bichromatic (ω, 2ω) counter-rotating circularly polarized laser fields with a molecular target. The full control of the electronic pathway is first analyzed by a classical trajectory analysis and then extended to a detailed quantum study of H 2 + molecules in bichromatic (ω, 2ω) counter-rotating circularly polarized laser fields. The radiation spectrum contains doublets of left- and right-circularly polarized harmonics in the XUV ranges. Finally, we study in detail the below-, near-, and above-threshold harmonic regions and describe how excited-state resonances alter the ellipticity and phase of the generated harmonic peaks.

74 ATOMIC AND MOLECULAR PHYSICS↗

Harmonic Modeling, Data Generation and Analysis of Power Electronics-Interfaced Residential Loads

The share of electronics-based residential load is expected to rise as devices such as variable frequency drives (VFDs), electric vehicle chargers, and inverter-based distributed energy resources (DERs), e.g., photovoltaic (PV) systems become more common. These loads may introduce significant harmonics into power networks that need to be closely studied in order to perform accurate load modeling and forecasting. However, it can be difficult to obtain harmonic-rich voltage and current data - necessary for identifying accurate load models - for residential electrical loads. Recognizing this need, we identify and model a set of electronics-based end-use loads and DERs in an electromagnetic transients program (EMTP) tool for a residence with a single- phase split-phase supply. Further, a procedure is developed to model harmonic interactions between end-use loads connected to the same non-ideal supply voltage in a residential setting. Finally, a harmonic-rich dataset produced via the proposed procedure is utilized to identify frequency coupling matrix (FCM) based load model. Numerical results demonstrate the accuracy of the model, and explore model identifiability with limited data points.

harmonics, power quality, load modeling↗

High-efficiency, large-aperture fifth-harmonic: Generation of 211-nm pulses in ammonium dihydrogen phosphate crystals for fusion diagnostics

High-energy ultraviolet (UV) sources are required to probe hot dense plasmas from fusion experiments by using Thomson scattering resulting from the lower self-generated background from the plasma in the 180 to 230-nm spectral region. Although recently we demonstrated efficient, joule-class fifth harmonic conversion of 1053-nm pulses using a cesium lithium borate (CLBO) crystal, larger crystals are necessary for increased UV energy. This paper presents an alternative approach for fifth-harmonic generation of a large-aperture neodymium laser using ammonium dihydrogen phosphate (ADP). An Nd:YLF laser was optimized to produce square pulses with a flattop, square beam profile (1053 nm, 1 to 2.8 ns, 12 x 12 mm, ≤1.5 J, ≤5 Hz). Noncritical phase matching in ADP suitable for sum–frequency mixing the fourth harmonic with residual fundamental light was achieved by cooling the crystal (65 x 65 x 10 mm) in a two-chamber cryostat to 200 K. The crystal chamber used helium (1 atm) as the thermally conductive medium between the crystal and the crystal chamber, which in turn was surrounded by a high-vacuum chamber that contained a liquid nitrogen reservoir to cool the crystal chamber. Temperature variation of 0.4 K across the crystal aperture was obtained using two 50-W heaters with active feedback. The total conversion efficiency from the fundamental to the fifth harmonic, including surface losses and absorption, was 26%.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Spectroscopic study of carbon plasma produced by the first (1064 nm) and second (532 nm) harmonics of Nd:YAG laser

In this research work, spectroscopic studies of carbon (C) plasma by using laser-induced breakdown spectroscopy (LIBS) are presented. The plasma was produced by the first (1064 nm) and second (532 nm) harmonics of a Q-switched Nd:YAG (Quantel Brilliant) pulsed laser having a pulse duration of 5 ns and 10-Hz repetition rate, which is capable of delivering 400 mJ at 1064 nm and 200 mJ at 532 nm. The laser beam was focused on the target material (100% carbon) by placing it in air at atmospheric pressure. The experimentally observed line profiles of five neutral carbon (C I) lines at 247.85, 394.22, 396.14, 588.95, and 591.25 nm were used to extract the electron temperature T{sub e} by using the Boltzmann plot method and determine its value, 9880 and 9400 K, respectively, for the fundamental and second harmonics of the laser, whereas the electron density N{sub e} was determined from the Stark broadening profile of neutral carbon line at 247.85 nm. The values of N{sub e} at a distance of 0.05 mm from the target surface for the fundamental-harmonic laser with a pulse energy of 130 mJ and the second-harmonic laser with a pulse energy of 72 mJ are 4.68 × 10{sup 17} and 5.98 × 10{sup 17} cm{sup −3}, respectively. This extracted information on T{sub e} and N{sub e} is useful for the deposition of carbon thin films by using the pulsed laser deposition technique. Moreover, both plasma parameters (T{sub e} and N{sub e}) were also calculated by varying the distance from the target surface along the line of propagation of the plasma plume and also by varying the laser irradiance.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Exciton Spectroscopy of Semiconductors by the Method of Optical Harmonics Generation (Review)

Nonlinear optical phenomena are widely used for the study of semiconductor materials. The paper presents an overview of experimental and theoretical studies of excitons by the method of optical second and third harmonics generation in various bulk semiconductors (GaAs, CdTe, ZnSe, ZnO, Cu{sub 2}O, (Cd,Mn)Te, EuTe, EuSe), and low-dimensional heterostructures ZnSe/BeTe. Particular attention is paid to the role of external electric and magnetic fields that modify the exciton states and induce new mechanisms of optical harmonics generation. Microscopic mechanisms of harmonics generation based on the Stark effect, the spin and orbital Zeeman effects, and on the magneto-Stark effect specific for excitons moving in an external magnetic field are considered. This approach makes it possible to study the properties of excitons and to obtain new information on their energy and spin structure that is not available when the excitons are investigated by linear optical spectroscopy. As a result of these studies, a large amount of information was obtained, which allows us to conclude on the establishing of a new field of research—exciton spectroscopy by the method of optical harmonics generation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

High-harmonic generation in ZnO driven by self-compressed mid-infrared pulses

Progress in attosecond science has relied on advancements in few-cycle pulse generation technology and its application to high-order harmonic generation. Traditionally, self-phase modulation in bulk solids has been used for the compression of moderate-energy pulses, additionally exhibiting favorable dispersion properties for mid-infrared (mid-IR) pulses. For this study, we use the anomalous dispersion of Y 3 Al 5 O 12 (YAG) to self-compress many-cycle pulses from a 50 kHz mid-IR OPA down to produce sub-three-cycle 10 μJ pulses and further use them to generate high-order harmonics in a ZnO crystal. In agreement with theoretical predictions, we observe a boost in the harmonic yield by a factor of two, and spectral broadening of above-gap harmonics, compared to longer driving pulses. The enhanced yield results from an increase in the intensity for the self-compressed pulses.

36 MATERIALS SCIENCE↗

Lorentz drift compensation in high harmonic generation in the soft and hard X-ray regions of the spectrum

Here, we present a semi-classical study of the effects of the Lorentz force on electrons during high harmonic generation in the soft and hard X-ray regions driven by near- and mid-infrared lasers with wavelengths from 0.8 to 20 μm, and at intensities below 10 15 W/cm 2 . The transverse extent of the longitudinal Lorentz drift is compared for both Gaussian focus and waveguide geometries. Both geometries exhibit a longitudinal electric field component that cancels the magnetic Lorentz drift in some regions of the focus, once each full optical cycle. We show that the Lorentz force contributes a super-Gaussian scaling which acts in addition to the dominant high harmonic flux scaling of λ -(5-6) due to quantum diffusion. We predict that the high harmonic yield will be reduced for driving wavelengths > 6 μm, and that the presence of dynamic spatial mode asymmetries results in the generation of both even and odd harmonic orders. Remarkably, we show that under realistic conditions, the recollision process can be controlled and does not shut off completely even for wavelengths >10 μm and recollision energies greater than 15 keV.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Enhancing high-order harmonic generation by controlling the diffusion of the electron wave packet

We experimentally study the enhancement of high-order harmonic generation (HHG) driven by synthesized ω <#comment/> − <#comment/> 3 ω <#comment/> laser fields, where we control whether the ionization rate or the electron wave packet’s diffusion is the dominant enhancement mechanism. When minimizing the electron wave packet’s diffusion, the excursion times of the corresponding electron trajectories are reduced by a factor of 2 or more. This result is important for imaging techniques that use the returning electron wave packet to probe the remaining ion. Furthermore, we achieve a 10 × <#comment/> to 3800 × <#comment/> enhancement of the harmonic yield driven by the bichromatic fields relative to that of an optimized single-color field, showing that the bichromatic fields improve HHG’s capability as a light source. We also measure that the two-color field’s harmonics have half the divergence angle compared to their single-color counterpart, suggesting that the “short” electron trajectories play a more prominent role compared to their “long” trajectory counterparts, thus improving the wavefront of the emerging harmonic beam.

74 ATOMIC AND MOLECULAR PHYSICS↗

Fenestration system energy performance research, implementation, and international harmonization

The research conducted by the NFRC and its contractors adds significantly to the understanding of several areas of investigation. NFRC enables manufacturers to rate fenestration energy performance to comply with building energy codes, participate in ENERGY STAR, and compete fairly. NFRC continuously seeks to improve its ratings and also seeks to simplify the rating process. Several research projects investigated rating improvement potential such as • Complex Product VT Rating Research • Window 6 and Therm 6 Validation Research Project • Complex Product VT Rating Research Conclusions from these research projects led to important changes and increased confidence in the existing NFRC rating process. Conclusions from the Window 6/Therm 6 project will enable window manufacturers to rate an expanded array of products and improve existing ratings. Some research lead to an improved new rating method called the Component Modeling Approach. A primary goal of the CMA was a simplification of the commercial energy rating process to increase participation and make the commercial industry more competitive and code compliant. The project below contributed towards CMA development: • Component Modeling Approach Condensation Resistance Research NFRC continues to implement the Component Modeling Approach program. The program includes the CMA software tool, CMAST, and several procedural documents to govern the certification process. This significant accomplishment was a response the commercial fenestration industry’s need for a simplification of the present NFRC energy rating method (named site built). To date, most commercial fenestration is self-rated by a variety of techniques. The CMA enables commercial fenestration manufacturers to rate according to the NFRC 100/200 as most commercial energy codes require. International Harmonization NFRC achieved significant international harmonization success by continuing its licensing agreements with the Australian Fenestration Rating Council and the Association of Architectural Aluminum Manufacturers of South Africa (AAAMSA) to produce NFRC certified product ratings in their respective nations. NFRC worked in several other nations to introduce the NFRC ratings system: • India • China • Japan • Canada • Thailand • South Africa • Brazil • Korea NFRC attended or hosted several meetings in each of these nations establishing academic, commercial, industrial, and governmental contacts. NFRC presented the NFRC process and then necessary infrastructure steps necessary to achieve harmonization with the NFRC labeling system. NFRC looks forward to continued work toward harmonization in these nations and potentially others.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Propagation And Damping Of High Harmonic Fast Waves And Electron Cyclotron Waves In The Nstx-U-Device

For the spherical torus and for conventional tokamaks to be viable means of producing fusion energy there are two important requirements. The first is to heat the plasma in the experimental devices to high temperatures; preferably, to fusion relevant temperatures. The second is to drive a current in the plasma so that the fusion device operates in a steady-state mode. A pulsed fusion reactor for energy production is not desirable. A favored means to achieve both of these requirements is through the use of microwaves, commonly referred to as radio frequency waves. This proposal was to understand observations from the National Spherical Torus Experiment Upgrade (NSTX-U) device on radio frequency wave heating of the confined plasma during operations with high harmonic fast waves. The proposed research was also directed toward assisting in the optimization of the experimental modes of operation so as to maximize the heating efficiency. A detailed analysis of the experiments has shown that about one-third of the input radio frequency power does not make it into the core region of the plasma where heating is required. The losses are believed to occur primarily in the edge region where the radio frequency power is initially coupled into the plasma. Using sophisticated computational codes and theoretical models, that have been developed for the NSTX-U experimental program, this research quantified the physical processes which occur in the edge plasma and lead to a decrease in the heating efficiency. The effect of edge turbulence on the scattering of radio frequency waves was studied for waves in the ion cyclotron and electron cyclotron range of frequencies. For high harmonic fast waves in the ion cyclotron range of frequencies, simulations were carried out using a full-wave solver that was extended to the vacuum vessel wall. These simulations successfully reproduced trends that were observed experimentally. This simulation capability was also used to study the interaction of high harmonic fast waves with the scrape-off layer plasma. More recently, a new technique has been developed for the calculation of radio frequency waves in toroidal geometry that enables the simultaneous incorporation of antenna geometry, plasma facing components, the scrape off-layer, and core propagation in the high harmonic fast wave regime. The effect of turbulent plasmas on the mode conversion of extraordinary electromagnetic waves in the electron cyclotron range of frequencies in the NSTX-U plasma has been studied theoretically. In the over-dense plasmas of NSTX-U, the traditional electromagnetic waves are not effective for delivering energy and momentum to the core plasma. However, electron Bernstein waves generated by mode conversion are efficient carriers of wave energy and momentum to the core. The mode conversion occurs in the turbulent edge region. A theory for mode conversion in such plasmas has been developed. The parameters that can optimize the mode conversion can be readily determined. Also, the model is useful for experimentalists to analyze observation on a shot-to-shot basis.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Propagation And Damping Of High Harmonic Fast Waves And Electron Cyclotron Waves In The Nstx-U-Device

For the spherical torus and for conventional tokamaks to be viable means of producing fusion energy there are two important requirements. The first is to heat the plasma in the experimental devices to high temperatures; preferably, to fusion relevant temperatures. The second is to drive a current in the plasma so that the fusion device operates in a steady-state mode. A pulsed fusion reactor for energy production is not desirable. A favored means to achieve both of these requirements is through the use of microwaves, commonly referred to as radio frequency waves. This proposal was to understand observations from the National Spherical Torus Experiment Upgrade (NSTX-U) device on radio frequency wave heating of the confined plasma during operations with high harmonic fast waves. The proposed research was also directed toward assisting in the optimization of the experimental modes of operation so as to maximize the heating efficiency. A detailed analysis of the experiments has shown that about one-third of the input radio frequency power does not make it into the core region of the plasma where heating is required. The losses are believed to occur primarily in the edge region where the radio frequency power is initially coupled into the plasma. Using sophisticated computational codes and theoretical models, that have been developed for the NSTX-U experimental program, this research quantified the physical processes which occur in the edge plasma and lead to a decrease in the heating efficiency. The effect of edge turbulence on the scattering of radio frequency waves was studied for waves in the ion cyclotron and electron cyclotron range of frequencies. For high harmonic fast waves in the ion cyclotron range of frequencies, simulations were carried out using a full-wave solver that was extended to the vacuum vessel wall. These simulations successfully reproduced trends that were observed experimentally. This simulation capability was also used to study the interaction of high harmonic fast waves with the scrape-off layer plasma. More recently, a new technique has been developed for the calculation of radio frequency waves in toroidal geometry that enables the simultaneous incorporation of antenna geometry, plasma facing components, the scrape off-layer, and core propagation in the high harmonic fast wave regime. The effect of turbulent plasmas on the mode conversion of extraordinary electromagnetic waves in the electron cyclotron range of frequencies in the NSTX-U plasma has been studied theoretically. In the over-dense plasmas of NSTX-U, the traditional electromagnetic waves are not effective for delivering energy and momentum to the core plasma. However, electron Bernstein waves generated by mode conversion are efficient carriers of wave energy and momentum to the core. The mode conversion occurs in the turbulent edge region. A theory for mode conversion in such plasmas has been developed. The parameters that can optimize the mode conversion can be readily determined. Also, the model is useful for experimentalists to analyze observation on a shot-to-shot basis.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Harmonization of experimental approach and data collection to streamline analysis of biomass composition from algae in an inter-laboratory setting

In order to establish and design long-term algae cultivation experiments, inter-laboratory projects need to harmonize the requirements of techno-economic and life-cycle analysis models, with standardized data inputs. In order to provide a consistent foundation and allow for integration and analysis of the results in computational technical and resource analysis models, we implemented closely coordinated, harmonized and objective analytical protocols along with a common language for measuring growth and productivity for the major algal components. We describe here the process by which we developed a harmonization framework for analysis across five geographically diverse testbed sites. Our goal was to align analytical procedures to ensure consistent reporting on biomass and lipid content, quality and yields to eliminate measurement variability as a source of uncertainty in production data. Developing standards for analysis that streamline reporting on composition and expected fuel yields from biomass is one of the major outcomes of this work and this provides a starting place for further advanced characterization of algae to support the techno-economical process analyses and account for the mass balance accounting of algal biomass. In conclusion, initial analysis of data obtained from field studies shows trends in compositional shifts of lipid and protein content of the biomass that are in support of the physiological experiments demonstrated in the first geographically distributed unified outdoor cultivation trials.

09 BIOMASS FUELS↗