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At least 271 records · Page 15

Thermal stability of the deep ultraviolet emission from AlGaN/AlN Stranski-Krastanov quantum dots

We report on the structural and optical properties of AlGaN/AlN quantum dot (QD) superlattices synthesized by plasma-assisted molecular-beam epitaxy. Modifying the composition and geometry of the QDs, the peak emission wavelength can be shifted from 320 nm to 235 nm while keeping the internal quantum efficiency larger than 30%. The efficient carrier confinement is confirmed by the stability of the photoluminescence (PL) intensity and decay time, from low temperature up to 100 K. Above this threshold, the PL intensity decreases and the radiative lifetime increases due to carrier thermalization. We also identified the intraband electronic transition between the ground level of the conduction band and the first excited state confined along the growth axis (s-p{sub z}).

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Ozone generation by rock fracture: Earthquake early warning?

We report the production of up to 10 ppm ozone during crushing and grinding of typical terrestrial crust rocks in air, O{sub 2} and CO{sub 2} at atmospheric pressure, but not in helium or nitrogen. Ozone is formed by exoelectrons emitted by high electric fields, resulting from charge separation during fracture. The results suggest that ground level ozone produced by rock fracture, besides its potential health hazard, can be used for early warning in earthquakes and other catastrophes, such as landslides or land shifts in excavation tunnels and underground mines.

54 ENVIRONMENTAL SCIENCES↗

Metallization Effect during Compression of Inert Gases

We consider the effect of metallization of inert gas vapors, which is observed under their shock compression in the plasma fluid region. We propose that the jumpwise increase in the conductivity be explained by a decrease in the ionization potential of atoms associated with broadening of the ground level due to the formation of dielectric jelly. The behavior of the plasma fluid conductivity acquires features of semiconductor conductivity. The composition and conductivity of dense inert gas vapors are calculated using the modified “3+” model. Comparative analysis is carried out for the effect in metal and inert gas vapors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Applications of TIERRAS for underground particle cascade simulations

In this communication we present some example applications of TIERRAS, a software package for the simulation of High Energy particle cascades underground and underwater. The examples illustrate how this package can be used to study the phenomenology of particle cascades from Extended Air Showers propagated several meters underground, including the effect of the surface ''albedo'' particles that are generated when a cascade reaches ground level. These up-going particles can have a measurable effect on surface or shallow underground detectors. Finally, to show the package ability ro perform simulations of particle cascades in ice, an application for neutrino radio detection is briefly introduced.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Airborne and ground-based measurements of the trace gases and particles emitted from prescribed fires in the United States

We measured the emission factors for 19 trace gas species and particulate matter (PM2.5) from 14 prescribed fires in chaparral and oak savanna in the southwestern US, as well as pine forest understory in the southeastern US and Sierra Nevada mountains of California. These are likely the most extensive emission factor field measurements for temperate biomass burning to date and the only published emission factors for temperate oak savanna fuels. This study helps close the gap in emissions data available for temperate zone fires relative to tropical biomass burning. We present the first field measurements of the biomass burning emissions of glycolaldehyde, a possible precursor for aqueous phase secondary organic aerosol formation. We also measured the emissions of phenol, another aqueous phase secondary organic aerosol precursor. Our data confirm previous suggestions that urban deposition can impact the NOx emission factors and thus subsequent plume chemistry. For two fires, we measured the emissions in the convective smoke plume from our airborne platform at the same time the unlofted residual smoldering combustion emissions were measured with our ground-based platform after the flame front passed through. The smoke from residual smoldering combustion was characterized by emission factors for hydrocarbon and oxygenated organic species that were up to ten times higher than in the lofted plume, including significant 1,3-butadiene and isoprene concentrations which were not observed in the lofted plume. This should be considered in modeling the air quality impacts of smoke that disperses at ground level, and we show that the normally-ignored unlofted emissions can also significantly impact estimates of total emissions. Preliminary evidence of large emissions of monoterpenes was seen in the residual smoldering spectra, but we have not yet quantified these emissions. These data should lead to an improved capacity to model the impacts of biomass burning in similar ecosystems.

09 BIOMASS FUELS↗

A Data Processing Workflow for Fixed-wing Drone Based Radiation Mapping in the Chornobyl Exclusion Zone (CEZ) - 20119

April 2020 marks the 34. anniversary of the high-profile radiological release from the Chornobyl Nuclear Power Plant (ChNPP). The release of radioactive material from reactor number four began on the 26 April 1986 and continued over a period of about 10 days, releasing approximately 1700 PBq of radioactive material (including 85 PBq of 137-Cs) into the environment. To this day, the accident remains the most significant release of radioactive material since civil nuclear power generation began. In the years since the accident, automated and remote radiation monitoring technologies have advanced significantly in their capabilities. One such example of this is the use of unmanned aerial vehicles (UAVs) in radiation mapping investigations. In April 2019, a team of scientists from the University of Bristol showcased a novel radiation mapping system within the CEZ, specifically aiming to map radiation over a large portion of the area immediately surrounding the ChNPP. Over six days of data collection, the system flew a total distance of 583.8 km, covering an area of 14.6 sq.km with an exceptional spatial resolution (sub 20 m/pixel). The work presented herein outlines and explains the data processing procedure to convert the raw data into 137-Cs activity (kBq/sq.m) and cesium-equivalent dose-rate (CED) at 1 m above ground level (μSv/hr). A demonstration of the validity of the method is demonstrated through the successful reduction of the raw data into a single linear relationship between the measured {sup 137}Cs net peak intensity and the {sup 137}Cs activity. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Using Regionalized Air Quality Model Performance and Bayesian Maximum Entropy Data Fusion to Map Global Surface Ozone Concentration and Associated Uncertainty

Estimates of ground-level ozone concentrations have been improved through data fusion of observations and atmospheric chemistry models. Our previous global ozone estimates for the Global Burden of Disease study corrected for bias uniformly across continents and then corrected near monitoring stations using the Bayesian Maximum Entropy (BME) framework for data fusion. Here, we use the Regionalized Air Quality Model Performance (RAMP) framework to correct model bias over a much larger spatial range than BME can, accounting for the spatial inhomogeneity of bias and nonlinearity as a function of modeled ozone. RAMP bias correction is applied to a composite of 9 global chemistry-climate models, based on the nearest set of monitors. These estimates are then fused with observations using BME, which matches observations at measurement stations, with the influence of observations declining with distance in space and time. We create global ozone maps for each year from 1990 to 2017 at fine spatial resolution. RAMP is shown to create unrealistic discontinuities due to the spatial clustering of ozone monitors, which we overcome by applying a weighting for RAMP based on the number of monitors nearby. Incorporating RAMP before BME has little effect on model performance near stations, but strongly increases R 2 by 0.15 at locations farther from stations, shown through a checkerboard cross-validation. Corrections to estimates differ based on location in space and time, confirming heterogeneity. We quantify the likelihood of exceeding selected ozone levels, finding that parts of the Middle East, India, and China are most likely to exceed 55 parts per billion (ppb) in 2017. About 96% of the global population was exposed to ozone levels above the World Health Organization guideline of 60 µg m −3 (30 ppb) in 2017. Our annual fine-resolution ozone estimates may be useful for several applications including epidemiology and assessments of impacts on health, agriculture, and ecosystems.

Ozone↗

Solar Cosmic Ray Acceleration by a Shock Wave in the Lower Solar Corona on November 22, 1977

Based on the theory of diffusive shock acceleration of charged particles, we have investigated the spectra of protons recorded in the solar cosmic ray event near the Earth’s orbit on November 22, 1977 (ground level enhancement no. 30, GLE30). The proton flux data from the CPME instrument installed on the IMP-8 spacecraft and the worldwide network of neutron monitors have been used to analyze the event. Using GLE30 as an example, we have shown for the first time that solar cosmic rays of relativistic energies can be produced by a shock wave with a relatively low speed of 560 km s{sup –1} in the lower solar corona at a distance up to 1.6R{sub ⊙} (R{sub ⊙} is the solar radius) within 615 s. The calculated proton spectra satisfactorily reproduce the measurements in the Earth’s orbit.

79 ASTRONOMY AND ASTROPHYSICS↗

Cryogenic vertical test facility for the SRF cavities at BNL

A vertical test facility has been constructed to test SRF cavities and can be utilized for other applications. The liquid helium volume for the large vertical dewar is approximate 2.1m tall by 1m diameter with a clearance inner diameter of 0.95m after the inner cold magnetic shield installed. For radiation enclosure, the test dewar is located inside a concrete block structure. The structure is above ground, accessible from the top, and equipped with a retractable concrete roof. A second radiation concrete facility, with ground level access via a labyrinth, is also available for testing smaller cavities in 2 smaller dewars. The cryogenic transfer lines installation between the large vertical test dewar and the cryo plant's sub components is currently near completion. Controls and instrumentations wiring are also nearing completion. The Vertical Test Facility will allow onsite testing of SRF cavities with a maximum overall envelope of 0.9 m diameter and 2.1 m height in the large dewar and smaller SRF cavities and assemblies with a maximum overall envelope of 0.66 m diameter and 1.6 m height.

43 PARTICLE ACCELERATORS↗

GLIDES – Efficient Energy Storage from ORNL

The research shown in this video features the GLIDES (Ground-Level Integrated Diverse Energy Storage) project, which has been under development at Oak Ridge National Laboratory (ORNL) since 2013. GLIDES can store energy via combined inputs of electricity and heat, and deliver dispatchable electricity. Supported by ORNL’s Laboratory Director’s Research and Development (LDRD) fund, this energy storage system is low-cost, and hybridizes compressed air and pumped-hydro approaches to allow for storage of intermittent renewable energy at high efficiency. A U.S. patent application for this novel energy storage concept has been submitted, and research findings suggest it has the potential to be a flexible, low-cost, scalable, high-efficiency option for energy storage, especially useful in residential and commercial buildings.

25 ENERGY STORAGE↗

Weekly periodicities of aerosol properties observed at an urban location in India

Multi-year (~7 years) observations of aerosol optical and microphysical properties were conducted at a tropical urban location in Bangalore, India. As a consequence of rapid urbanization, Bangalore presents high local atmospheric emissions, which makes it an interesting site to study the effect of anthropogenic activities on aerosol properties. It has been found that both column (aerosol optical depth, AOD) and ground-level measurements (black carbon (BC) and composite aerosol mass) exhibit a weekly cycle with low aerosol concentrations on weekends. In comparison to the weekdays, the weekend reductions of aerosol optical depth, black carbon and composite aerosol mass concentrations were ~15%, 25% and 24%, respectively. The magnitude of weekend reduction of black carbon is as much as ~1 μg m -3 . The similarity in the weekly cycle between the column and surface measurements suggests that the aerosol column loading at this location is governed by local anthropogenic emissions. The strongest weekly cycle in composite aerosol mass concentration was observed in the super micron mass range (>1 μm). The weekly cycle of composite aerosol mass in the sub micron mass range (<1 μm) was weak in comparison to the super micron aerosol mass.

54 ENVIRONMENTAL SCIENCES↗

Cosmic Ray Interactions in Shielding Materials

This document provides a detailed study of materials used to shield against the hadronic particles from cosmic ray showers at Earth’s surface. This work was motivated by the need for a shield that minimizes activation of the enriched germanium during transport for the MAJORANA collaboration. The materials suitable for cosmic-ray shield design are materials such as lead and iron that will stop the primary protons, and materials like polyethylene, borated polyethylene, concrete and water that will stop the induced neutrons. The interaction of the different cosmic-ray components at ground level (protons, neutrons, muons) with their wide energy range (from kilo-electron volts to giga-electron volts) is a complex calculation. Monte Carlo calculations have proven to be a suitable tool for the simulation of nucleon transport, including hadron interactions and radioactive isotope production. The industry standard Monte Carlo simulation tool, Geant4, was used for this study. The result of this study is the assertion that activation at Earth’s surface is a result of the neutronic and protonic components of the cosmic-ray shower. The best material to shield against these cosmic-ray components is iron, which has the best combination of primary shielding and minimal secondary neutron production.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Evaluation of Stratospheric Intrusions and Biomass Burning Plumes on the Vertical Distribution of Tropospheric Ozone Over the Midwestern U.S.

Naturally occurring ozone rich Stratosphere-to-Troposphere Transport (STT) intrusions and biomass burning plumes reaching the surface can contribute to exceedances of the U.S. National Ambient Air Quality Standards (NAAQS) for ground-level ozone (70 ppbv implemented in 2015). In addition, fires can inject significant pollution into the free troposphere where it can be transported long distances. The combined air quality impacts from these sources on ozone has only been analyzed in a few case studies for the Midwest U.S. Here we study ozone impacts in a major Midwestern city, for the first time in St. Louis, Missouri, using a series of ozonesonde profiles taken during the SEAC4RS (Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys) field campaign in August-September 2013. All ozonesondes showed some enhancements above the background profile levels (~55 ppbv) throughout each tropospheric column. Two models were used to estimate and quantify ozone origins within the columns. A chemical transport model identified enhancements from STT equivalent to 10to15 ppbv over the background with a 10 to15% contribution overall to the column. Two FLEXPART-WRF simulations, one with smoke in the boundary layer and the other with smoke above, identified enhancements from biomass burning equivalent to 10to 80 ppbv. Overall, the total biomass burning contribution is 15to 30% of the total column. Five ozonesondes showed signatures of mixed biomass burning plumes and STT intrusions. During this study period, biomass burning in the western U.S. contributed 70% to ozone enhancements in the total column compared to 3% from the central U.S and 27% from other areas.

National Ambient Air Quality Standards for ground‐↗

Investigation of the solar influence on the cosmic muon flux using WILLI detector

A fesibility study to explore the capability of the WILLI detector to observe the solar events/activity by recording the muon intensity at ground level is presented.The WILLI detector, set up in National Institute of Physics and Nuclear Engineering, Bucharest, is a 1 m{sup 2} incident area sampling calorimeter. It can measure simultaneously muon events with the muon energy {>=}0.4 GeV and, if the muons are stopped in the detector, and muon energy between 0.4<E{sub {mu}<}0.6 GeV, if the muons pass the minimum of 2 plates of the detector stack.Taking into account muon events with energy {>=}0.4 GeV, a modulation of the muon intensity as a diurnal variation is observed. Muon events for a smaller energy range (0.4-0.6 GeV) seem to exhibit an aperiodic variation of the muon intensity, which could be correlated with magnetic activity indicated by the planetary K{sub p} index.

79 ASTRONOMY AND ASTROPHYSICS↗

Sound Radiation from a Supersonic Jet Passing Through a Partially Open Exhaust Duct

The radiation of sound from a perfectly expanded Mach 2.5 cold supersonic jet of 25.4 mm exit diameter flowing through a partially open rigid-walled duct with an upstream i-deflector has been studied experimentally. In the experiments, the nozzle is mounted vertically, with the nozzle exit plane at a height of 73 jet diameters above ground level. Relative to the nozzle exit plane (NEP), the location of the duct inlet is varied at 10, 5, and -1 jet diameters. Far-field sound pressure levels were obtained at 54 jet diameters above ground with the aid of acoustic sensors equally spaced around a circular arc of radius equal to 80 jet diameters from the jet axis. Data on the jet acoustic field for the partially open duct were obtained and compared with those with a free jet and with a closed duct. The results suggest that for the partially open duct the overall sound pressure level (OASPL) decreases as the distance between the NEP and the duct inlet plane decreases, while the opposite trend is observed for the closed duct. It is also concluded that the observed peak frequency in the partially open duct increases above the free jet value as the angle from the duct axis is increased, and as the duct inlet plane becomes closer to the NEP.

Kandula, Max↗

Molecular response of poplar to single and combined ozone and drought

High concentration in ground-level ozone (O 3 ) and water deficit affect forest ecosystems service. Earlier we found intercellular CO 2 concentration and isoprene emission were affected by the combination of O 3 and drought, but the molecular mechanisms controlling these phenotypes are still open questions. In this study, we examined the stomatal conductance (g s ) and transcriptome changes in an O 3 -sensitive hybrid poplar exposed to two O 3 levels [charcoal-filtered ambient air (CF) and non-filtered ambient air plus 40 ppb (NF40)] and two water conditions [well-watered (W) and moderate drought (D)]. NF40 reduced the g s more under D than W. We identified the differentially expressed genes (DEGs) from pairwise comparisons and found the poplar's molecular response to drought was counteracted by elevated O 3 . From nine clusters obtained through K-means clustering, 12 core transcription factors were identified. DEGs involved in isoprene biosynthesis and phytohormones signal pathways indicate the molecular response and stomatal closure of poplar under O 3 and/or drought might be through MEP/DOXP and ABA-dependent pathways. In addition, 102 Helitrons capturing DEGs were involved in response to O 3 and/or drought and related with ABA-dependent pathway. This integrated analysis provides multi-dimensional insights to understand the molecular response to the combination of O 3 and drought.

59 BASIC BIOLOGICAL SCIENCES↗

Observation Targeting for the Tehachapi Pass and Mid-Columbia Basin: WindSENSE Phase III Project Summary Report

The overall goal of this multi-phased research project known as WindSENSE is to develop an observation system deployment strategy that would improve wind power generation forecasts. The objective of the deployment strategy is to produce the maximum benefit for 1- to 6-hour ahead forecasts of wind speed at hub-height (~80 m). In Phase III of the project, the focus was on the Mid-Columbia Basin region which encompasses the Bonneville Power Administration (BPA) wind generation area shown in Figure 1 that includes Klondike, Stateline, and Hopkins Ridge wind plants. The typical hub height of a wind turbine is approximately 80-m above ground level (AGL). So it would seem that building meteorological towers in the region upwind of a wind generation facility would provide data necessary to improve the short-term forecasts for the 80-m AGL wind speed. However, this additional meteorological information typically does not significantly improve the accuracy of the 0- to 6-hour ahead wind power forecasts because processes controlling wind variability change from day-to-day and, at times, from hour-to-hour. It is also important to note that some processes causing significant changes in wind power production function principally in the vertical direction. These processes will not be detected by meteorological towers at off-site locations. For these reasons, it is quite challenging to determine the best type of sensors and deployment locations. To address the measurement deployment problem, Ensemble Sensitivity Analysis (ESA) was applied in the Phase I portion of the WindSENSE project. The ESA approach was initially designed to produce spatial fields that depict the sensitivity of a forecast metric to a set of prior state variables selected by the user. The best combination of variables and locations to improve the forecast was determined using the Multiple Observation Optimization Algorithm (MOOA) developed in Phase I. In Zack et al. (2010a), the ESA-MOOA approach was applied and evaluated for the wind plants in the Tehachapi Pass region for a period during the warm season. That research demonstrated that forecast sensitivity derived from the dataset was characterized by well-defined, localized patterns for a number of state variables such as the 80-m wind and the 25-m to 1-km temperature difference prior to the forecast time. The sensitivity patterns produced as part of the Tehachapi Pass study were coherent and consistent with the basic physical processes that drive wind patterns in the Tehachapi area. In Phase II of the WindSENSE project, the ESA-MOOA approach was extended and applied to the wind plants located in the Mid-Columbia Basin wind generation area of Washington-Oregon during the summer and to the Tehachapi Pass region during the winter. The objective of this study was to identify measurement locations and variables that have the greatest positive impact on the accuracy of wind forecasts in the 0- to 6-hour look-ahead periods for the two regions and to establish a higher level of confidence in ESA-MOOA for mesoscale applications. The detailed methodology and results are provided in separate technical reports listed in the publications section below. Ideally, the data assimilation scheme used in the Phase III experiments would have been based upon an ensemble Kalman filter (EnKF) that was similar to the ESA method used to diagnose the Mid-Columbia Basin sensitivity patterns in the previous studies. However, running an EnKF system at high resolution is impractical because of the very high computational cost. Thus, it was decided to use a three-dimensional variational (3DVAR) analysis scheme that is less computationally intensive. The objective of this task is to develop an observation system deployment strategy for the mid Columbia Basin (i.e. the BPA wind generation region) that is designed to produce the maximum benefit for 1- to 6-hour ahead forecasts of hub-height (~80 m) wind speed with a focus on periods of large changes in wind speed. There are two tasks in the current project effort designed to validate the ESA observational system deployment approach in order to move closer to the overall goal: (1) Perform an Observing System Experiment (OSE) using a data denial approach. (2) Conduct a set of Observing System Simulation Experiments (OSSE) for the Mid-Columbia basin region.

17 WIND ENERGY↗

Photoacoustic optical properties at UV, VIS, and near IR wavelengths for laboratory generated and winter time ambient urban aerosols

We present the laboratory and ambient photoacoustic (PA) measurement of aerosol light absorption coefficients at ultraviolet wavelength (i.e., 355 nm) and compare with measurements at 405, 532, 870, and 1047 nm. Simultaneous measurements of aerosol light scattering coefficients were achieved by the integrating reciprocal nephelometer within the PA's acoustic resonator. Absorption and scattering measurements were carried out for various laboratory generated aerosols, including salt, incense, and kerosene soot to evaluate the instrument calibration and gain insight on the spectral dependence of aerosol light absorption and scattering. Ambient measurements were obtained in Reno, Nevada, between 18 December 2009 and 18 January 2010. The measurement period included days with and without strong ground level temperature inversions, corresponding to highly polluted (freshly emitted aerosols) and relatively clean (aged aerosols) conditions. Particulate matter (PM) concentrations were measured and analyzed with other tracers of traffic emissions. The temperature inversion episodes caused very high concentration of PM{sub 2.5} and PM{sub 10} (particulate matter with aerodynamic diameters less than 2.5 {mu}m and 10 {mu}m, respectively) and gaseous pollutants: carbon monoxide (CO), nitric oxide (NO), and nitrogen dioxide (NO{sub 2}). The diurnal change of absorption and scattering coefficients during the polluted (inversion) days increased approximately by a factor of two for all wavelengths compared to the clean days. The spectral variation in aerosol absorption coefficients indicated a significant amount of absorbing aerosol from traffic emissions and residential wood burning. The analysis of single scattering albedo (SSA), Angstrom exponent of absorption (AEA), and Angstrom exponent of scattering (AES) for clean and polluted days provides evidences that the aerosol aging and coating process is suppressed by strong temperature inversion under cloudy conditions. In general, measured UV absorption coefficients were found to be much larger for biomass burning aerosol than for typical ambient aerosols.

09 BIOMASS FUELS↗