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All sourcesNASA NTRSDOE OSTI
NASA NTRS1995

SeaWiFS Technical Report Series: The SeaWiFS CZCS-Type Pigment Algorithm - Volume 29

The Sea-viewing Wide Field-of-view Sensor (SeaWiFS) mission will provide operational ocean color that will be superior to the previous Coastal Zone Color Sensor (CZCS) proof-of-concept mission. An algorithm is needed that exploits the full functionality of SeaWiFS whilst remaining compatible in concept with algorithms used for the CZCS. This document describes the theoretical rationale of radiance band-ratio methods for determining chlorophyll-a and other important biogeochemical parameters, and their implementation for the SeaWIFS mission. Pigment interrelationships are examined to explain the success of the CZCS algorithms. In the context where chlorophyll-a absorbs only weakly at 520 nm, the success of the 520 nm to 550 nm CZCS band ratio needs to be explained. This is explained by showing that in pigment data from a range of oceanic provinces chlorophyll-a (absorbing at less than 490 nm), carotenoids (absorbing at greater than 460 nm), and total pigment are highly correlated. Correlations within pigment groups particularly photoprotectant and photosynthetic carotenoids are less robust. The sources of variability in optical data are examined using the NIMBUS Experiment Team (NET) bio-optical data set and bio-optical model. In both the model and NET data, the majority of the variance in the optical data is attributed to variability in pigment (chlorophyll-a), and total particulates, with less than 5% of the variability resulting from pigment assemblage. The relationships between band ratios and chlorophyll is examined analytically, and a new formulation based on a dual hyperbolic model is suggested which gives a better calibration curve than the conventional log-log linear regression fit. The new calibration curve shows the 490:555 ratio is the best single-band ratio and is the recommended CZCS-type pigment algorithm. Using both the model and NET data, a number of multiband algorithms are developed; the best of which is an algorithm based on the 443:555 and 490:555 ratios. From model data, the form of potential algorithms for other products, such as total particulates and dissolved organic matter (DOM), are suggested.

Hooker, Stanford B.↗
NASA NTRS1993

Effect of marine stratocumulus in TOMS ozone

The algorithm used to correct total O3 from the total ozone mapping spectrometer (TOMS) for cloud effects is based on the measured reflectivity, a climatological cloud top height, and an assumed tropospheric O3 column amount below clouds. In regions of persistent subtropical marine stratocumulus it is assumed that this introduces a positive error into total O3 because these clouds are lower than the assumed mean cloud height used in the algorithm. This appears to be confirmed by high correlation between Nimbus 7 TOMS total O3 and reflectivity data for typical regimes of persistent stratus, as identified by the international satellite cloud climatology project (ISCCP) observations. The TOMS total O3 overestimate has been computed using Nimbus 7/solar backscattered ultraviolet total O3 derived using temperature humidity infrared radiometer (THIR) data for years 1979-1984. A functional relationship between the THIR/non-THIR total O3 difference and reflectivity is used with TOMS reflectivity to modify Nimbus 7 TOMS O3 data for selected regions and periods. The correction diminishes or eliminates a number of apparent O3 maxima, with reductions of up to 20 Dobson units (DU) in total O3 on daily maps and approximately 5 DU on monthly mean O3 maps. Significant correlation between corrected TOMS O3 and reflectivity data remains because low-altitude O3 is retrieved more efficiently over a high-albedo surface. It is also possible that dynamical influences leading to stratocumulus formation bring O3-enriched air into the area. These results imply that although good arguments can be made for the use of TOMS total O3 as a proxy for tropospheric O3 in the tropics, caution must be exercised in the use of daily and even monthly O3 maps in the vicinity of clouds. Further research into the TOMS algorithm in cloudy regions is required to derive reliable estimates of tropospheric O3.

Thompson, A. M.↗
NASA NTRS2023

Decoupling in the Vertical Shape of HCHO During a Sea Breeze Event: the Effect on Trace Gas Satellite Retrievals and Column-to-Surface Translation

The effect of sea breeze circulation on stratification of the vertical formaldehyde (HCHO) concentration vertical profiles is explored using a regional atmospheric chemical transport model (CTM) for three synoptically stagnant days focused on the east coast of the U.S in June 2018. During this event, a significant thermal contrast between the Atlantic Ocean and the terrestrial regions (12–17 °C), observed by moderate resolution imaging spectroradiometer (MODIS) and well-captured by the WRF-CMAQ model (15–18 °C), is conducive to monsoon-like flow, perpendicular to the shorelines, carrying clean marine air masses over the land within a few hundreds of meters above the surface. In contrast, the westerly continental polluted air masses prevail in higher altitudes. These two conflicting flows result in atypical vertical shapes of HCHO concentrations increasing with altitude. This decoupling pattern is so pronounced that we observe total column HCHO negatively correlate with surface concentrations. Comparisons of an accredited global model, GEOS-CF, to surface wind measurements and MODIS skin temperature indicate its poor representation of the sea breeze timing and strength, resulting in GEOS-CF HCHO vertical shapes being drastically different from the WRF-CMAQ. Based on radiative transfer calculations, the differences in the vertical distribution of HCHO between the WRF-CMAQ and that of GEOS-CF in the first 3 km are sufficient to induce a 20–30% error in air mass factors (thus total vertical HCHO column abundances). Through an experiment involving converting HCHO total columns to surface mixing ratios, we demonstrate that GEOS-CF allocates noticeably more HCHO molecules (40–150%) to the surface layer due to the misrepresentation of the vertical shape of HCHO during the sea breeze event. It is known that a significant fraction of the human population lives in coastal areas prone to detrimental effects caused by air pollution, and elevated pollutant concentrations usually occur in synoptically stagnant atmospheric conditions when local circulation patterns come into play; accordingly, our experiments emphasize the importance of the effect a priori profiles can have on satellite-derived applications under such conditions. To ensure that the quantitative representation of satellite-based trace gas retrievals on a daily basis is trustworthy and useable for air quality applications, atmospheric models providing a priori profiles for satellite retrievals should be well-tuned to reproduce complex local circulation such as sea-land breezes.

sea breeze↗
NASA NTRS1986

October Antarctic temperature and total ozone trends from 1979-1985

The morphology of temperature trends in the south polar stratosphere from 1979-1985 is detailed. A significant cooling has occurred in the stratosphere over this period. South polar October mean temperatures have declined 18 K at 24 km over the seven-year period. A large fraction of this decline occurs as a result of including 1979 temperatures in the trend. The years 1979 and 1982 differ from other years in that they include large mid-October wave events which produce significantly warmer polar temperatures. Nevertheless, a significant temperature decline has still occurred in the stratosphere even when the dynamically active years are not included. Comparing two relatively dynamically quiet years, 1980 and 1985, the largest temperature decrease in the 30 mb temperature field occurs not at the pole but in the subpolar temperature maximum centered near 60 deg S. The changes in temperature of both the maximum and the polar low regions correlate fairly well with total ozone changes observed by the Total Ozone Mapping Spectrophotometer.

Newman, Paul A.↗
DOE OSTI2019

Homeostatic maintenance of nonstructural carbohydrates during the 2015-2016 El Niño drought across a tropical forest precipitation gradient

Non-structural carbohydrates (NSCs) are essential for maintenance of plant metabolism, and may be sensitive to both short- and long-term climatic variation. The NSC variation in NSCs in moist tropical forests has only rarely been studied, however, so regulation of NSCs in these systems is poorly understood. We measured foliar and branch NSC content in 23 tree species at three sites located across a large precipitation gradient in Panama during the 2015-2016 El Niño to examine how short- and long-term climatic variation impacts carbohydrate dynamics. Across all sites, leaf NSCs increased over diurnal time-periods. There was no significant difference in total NSCs over as the progression of the drought progressed (leaf p=0.32, branch p=0.30), nor across the rainfall gradient (leaf p=0.91, branch p=0.96). The Foliar soluble sugars decreased while starch increased :starch ratio did decrease over the duration of the dry period, suggesting greater partitioning of NSCs to storage than metabolism or transport as drought progressed. There was large variation across species at all sites, but total foliar NSCs were positively correlated with leaf mass per area, while branch sugars were positively related to leaf temperature and negatively correlated with daily photosynthesis and wood density. The NSC homeostasis across a wide range of conditions suggests that NSCs are an allocation priority in moist tropical forests.

Dickman, Lee T.↗
DOE OSTI2021

Hubble Space Telescope UV and Hα Measurements of the Accretion Excess Emission from the Young Giant Planet PDS 70 b

Recent discoveries of young exoplanets within their natal disks offer exciting opportunities to study ongoing planet formation. In particular, a planet’s mass accretion rate can be constrained by observing the accretion-induced excess emission. So far, planetary accretion is only probed by the Hα line, which is then converted to a total accretion luminosity using correlations derived for stars. However, the majority of the accretion luminosity is expected to emerge from hydrogen continuum emission, and is best measured in the ultraviolet (UV). In this paper, we present HST/WFC3/UVIS F336W (UV) and F656N (Hα) high-contrast imaging observations of PDS 70. Applying a suite of novel observational techniques, we detect the planet PDS 70 b with signal-to-noise ratios of 5.3 and 7.8 in the F336W and F656N bands, respectively. This is the first time that an exoplanet has been directly imaged in the UV. Our observed Hα flux of PDS 70 b is higher by 3.5σ than the most recent published result. However, the light curve retrieved from our observations does not support greater than 30% variability in the planet’s Hα emission in six epochs over a five month timescale. We estimate a mass accretion rate of 1.4±0.2×10{sup −8}M{sub Jup} yr{sup −1}. Hα accounts for 36% of the total accretion luminosity. Such a high proportion of energy released in line emission suggests efficient production of Hα emission in planetary accretion, and motivates using the Hα band for searches of accreting planets. These results demonstrate HST/WFC3/UVIS’s excellent high-contrast imaging performance and highlight its potential for planet formation studies.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Measuring Black Hole Light Echoes with Very Long Baseline Interferometry

Light passing near a black hole can follow multiple paths from an emission source to an observer due to strong gravitational lensing. Photons following different paths take different amounts of time to reach the observer, which produces an echo signature in the image. The characteristic echo delay is determined primarily by the mass of the black hole, but it is also influenced by the black hole spin and inclination to the observer. In the Kerr geometry, echo images are demagnified, rotated, and sheared copies of the direct image and lie within a restricted region of the image. Echo images have exponentially suppressed flux, and temporal correlations within the flow make it challenging to directly detect light echoes from the total light curve. In this Letter, we propose a novel method to search for light echoes by correlating the total light curve with the interferometric signal at high spatial frequencies, which is a proxy for indirect emission. We explore the viability of our method using numerical general relativistic magnetohydrodynamic simulations of a near-face-on accretion system scaled to M87-like parameters. We demonstrate that our method can be used to directly infer the echo delay period in simulated data. An echo detection would be clear evidence that we have captured photons that have circled the black hole, and a high-fidelity echo measurement would provide an independent measure of fundamental black hole parameters. Our results suggest that detecting echoes may be achievable through interferometric observations with a modest space-based very long baseline interferometry mission.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2005

Characterization of AIRS temperature and water vapor measurement capability using correlative observations

In this presentation we address several fundamental issues in the measurement of temperature and water vapor by AIRS: accuracy, precision, vertical resolution and biases as a function of cloud amount. We use two correlative data sources. First we compare AIRS total water vapor with that from the Advanced microwave Sounding Radiometer for EOS (AMSR-E) instrument, also onboard the Aqua spacecraft. AMSRE uses a mature methodology with a heritage including the operational Special Sensor Microwave Imager (SSM/I) instruments. AIRS and AMSR-E observations are collocated and simultaneous, providing a very large data set for comparison: about 200,000 over-ocean matches daily. We show small cloud-dependent biases between AIRS and AMSR-E total water vapor for several oceanic regions. Our second correlative data source is several hundred dedicated radiosondes launched during AIRS overpasses.

meteorology↗
DOE OSTI2018

A new method for calculating normal boiling point of liquids

A method for predicting normal boiling points (NBPs) of pure liquids based on linear free energy relationships (LFERs) and thermodynamics formulas is proposed. For 15 classes of chemical compounds (a total of 683 substances), correlation equations relating NBPs to molecular descriptors were obtained using stepwise regression. For all equations, the mean relative deviations (MD) lie between 0.89% and 2.83%, being mostly less than 2%. The correlation coefficients of 13 equations are larger than 0.98. The correlation equations obtained are simple, have clear physical sense, wide applicability range and provide rather high predictive power and accuracy of calculations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Synchrotron-based X-ray fluorescence microscopy mapping the ionome of a toxic freshwater cyanobacterium

Harmful algal blooms (HABs) pose a major environmental concern across the globe. In abundance, cyanobacteria, or so-called green-blue algae can produce extremely dangerous cyanotoxins that harm humans and animals. This study focused on the mapping and distribution of intracellular macro-and micronutrients of the widespread freshwater cyanobacteria Microcystis aeruginosa (M. aeruginosa). Towards a better understanding of trace metal uptake and homeostasis throughout the cell cycle, we quantitatively mapped the spatial distribution of the elements P, K, Fe, Ca, Zn, Mn, and Cu across the ultrastructure of frozen-hydrated single cells using state-of-theart X-ray nanofluorescence imaging at the Advanced Photon Source (APS) at Argonne National Laboratory. Further, bulk cellular nutrient and trace metal content correlated well with the total intracellular elemental content in individual cells obtained by quantitative synchrotron X-ray fluorescence measurements. Multi-dimensional mappings showed P and K atoms colocalized as discrete semicircular hotspots that were analyzed with respect to their stoichiometry. Elevated Cu and Ca concentrations were detected along division plane of cells. P and K were found to have similar spatial elemental distribution with about 65% and 69% of the total cellular P and K, respectively, located at the hotspots. The P and K colocalization were refined further using nanotomography, showing a K envelope surrounding the P core. Inorganic P and organic P compounds were specified using solution-state 31 P nuclear magnetic resonance (NMR) spectroscopy from M. aeruginosa. Of the total extracted P determined by 31 P NMR spectroscopy, 47% were found to be nucleotides while only 11% were polyphosphates. Multimodal X-ray imaging provides a better understanding of intracellular biochemical processes in cyanobacteria, helping us monitor and combat an emerging environmental threat.

31P NMR spectroscopy↗
DOE OSTI2020

Spent fuel nondestructive assay integrated characterization from active neutron, passive neutron, and passive gamma

Spent nuclear fuel comprises a wide range of irradiated isotopic material compositions, and characterization through nondestructive measurements is beneficial in verifying declared parameters before the fuel is placed in storage, final disposal, and/or reprocessed. This paper discusses results from three nondestructive assay instruments, including passive gamma, passive neutron, and active neutron methods, that measured fifty spent fuel assemblies at the Clab interim storage facility in Sweden. Here, integrated analysis of the measurements from the three different instruments allowed parametric assessments of cooling time, burnup, neutron multiplication, fissile mass, initial enrichment, and decay heat of each individual fuel assembly. Passive gamma measurements were found to be the most beneficial in predicting cooling time, passive neutron for determining burnup, active neutron in estimating initial enrichment, and both passive and total neutron for multiplication correlations. Fissile mass was best estimated using any combination of any two of the instruments such that corrections for isotopic changes in the fuel could be accounted for with the first set of measurements and multiplication of the assembly in the second. In conclusion, the nondestructive assay technologies demonstrated through this effort enhance the characterization of spent nuclear fuel assemblies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Influences from solvents on charge storage in titanium carbide MXenes

We report that pseudocapacitive energy storage in supercapacitor electrodes differs significantly from the electrical double-layer mechanism of porous carbon materials, which requires a change from conventional thinking when choosing appropriate electrolytes. Here we show how simply changing the solvent of an electrolyte system can drastically influence the pseudocapacitive charge storage of the two-dimensional titanium carbide, Ti 3 C 2 (a representative member of the MXene family). Measurements of the charge stored by Ti 3 C 2 in lithium-containing electrolytes with nitrile-, carbonate- and sulfoxide-based solvents show that the use of a carbonate solvent doubles the charge stored by Ti 3 C 2 when compared with the other solvent systems. We find that the chemical nature of the electrolyte solvent has a profound effect on the arrangement of molecules/ions in Ti 3 C 2 , which correlates directly to the total charge being stored. Finally, having nearly completely desolvated lithium ions in Ti 3 C 2 for the carbonate-based electrolyte leads to high volumetric capacitance at high charge–discharge rates, demonstrating the importance of considering all aspects of an electrochemical system during development.

25 ENERGY STORAGE↗
DOE OSTI2021

Stochastic evaluation of fourth-order many-body perturbation energies

A scalable, stochastic algorithm evaluating the fourth-order many-body perturbation (MP4) correction to energy is proposed. Three hundred Goldstone diagrams representing the MP4 correction are computer generated and then converted into algebraic formulas expressed in terms of Green’s functions in real space and imaginary time. They are evaluated by the direct (i.e., non-Markov, non-Metropolis) Monte Carlo (MC) integration accelerated by the redundant-walker and control-variate algorithms. The resulting MC-MP4 method is efficiently parallelized and is shown to display O(n 5.3 ) size-dependence of cost, which is nearly two ranks lower than the O(n 7 ) dependence of the deterministic MP4 algorithm. Furthermore, it evaluates the MP4/aug-cc-pVDZ energy for benzene, naphthalene, phenanthrene, and corannulene with the statistical uncertainty of 10 mE h (1.1% of the total basis-set correlation energy), 38 mE h (2.6%), 110 mE h (5.5%), and 280 mE h (9.0%), respectively, after about 10 9 MC steps.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2022

A refined assessment of nuclear data target accuracy requirements for ALFRED

The interest in target accuracy assessment has been recently renewed within the OECD/NEA Working Party on International Nuclear Data Evaluation Cooperation with an update exercise, thanks to the invaluable initiative of Massimo Salvatores. This work, moving from evaluations on the main core integral parameters of the Advanced Lead-cooled Fast Reactor European Demonstrator (ALFRED), and the identification of the associated target accuracies needed for improving its design, approaches the retrieval of target accuracy requirements for nuclear data, as the inverse problem of uncertainty quantification. The preliminary results obtained in a previous work are here refined by explicitly taking into account the total contribution due to correlations among variables in the optimization constraint, while its various components are evaluated individually. Moreover, three different sets of cost parameters are considered to introduce a bias in the solution in order to take in due account the relative difficulties in the execution of new differential experiments as needed for achieving the proposed target accuracies. By this, the obtained results are deemed usefully informative, and proposed for the update of a High Priority List which identifies the isotopes-reaction couples of most interest for future refinement experiments, especially when integrated with further analogous information collected on other advanced nuclear systems. Among the cross-sections whose refinement contributes the most to the reduction of the multiplication factor, the fission of Pu{sup 239} was found, which needs to be fixed below 1% in the range of interest for ALFRED (2 keV-4 MeV). Another contribution for the amelioration of the multiplication factor calculation accuracy, is due to the capture channel of Pu{sup 239}, for which the initial high uncertainty (around 15%) can be significantly reduced resorting to easily practicable experiments. The same occurs for the inelastic of Pb{sup 207}, for which the initial uncertainty value of around 50% can be drastically reduced up to target values between 4% and 7%.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2020

Multi-Trait Regressor Stacking Increased Genomic Prediction Accuracy of Sorghum Grain Composition

Genomic prediction has enabled plant breeders to estimate breeding values of unobserved genotypes and environments. The use of genomic prediction will be extremely valuable for compositional traits for which phenotyping is labor-intensive and destructive for most accurate results. We studied the potential of Bayesian multi-output regressor stacking (BMORS) model in improving prediction performance over single trait single environment (STSE) models using a grain sorghum diversity panel (GSDP) and a biparental recombinant inbred lines (RILs) population. A total of five highly correlated grain composition traits—amylose, fat, gross energy, protein and starch, with genomic heritability ranging from 0.24 to 0.59 in the GSDP and 0.69 to 0.83 in the RILs were studied. Average prediction accuracies from the STSE model were within a range of 0.4 to 0.6 for all traits across both populations except amylose (0.25) in the GSDP. Prediction accuracy for BMORS increased by 41% and 32% on average over STSE in the GSDP and RILs, respectively. Prediction of whole environments by training with remaining environments in BMORS resulted in moderate to high prediction accuracy. Our results show regression stacking methods such as BMORS have potential to accurately predict unobserved individuals and environments, and implementation of such models can accelerate genetic gain.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Ironsand (Titanomagnetite-Titanohematite): Chemistry, Magnetic Properties and Direct Applications for Wireless Power Transfer

Ironsand is an abundant and inexpensive magnetic mineral resource. However, the magnetic properties of unprocessed ironsand are often inadequate for any practical applications. In this work, the applicability of ironsand for use as a component in a soft magnetic composite for large-scale inductive power transfer applications was investigated. After magnetic separation, the chemical, structural and magnetic properties of ironsand sourced from different locations were compared. Differences observed in the DC magnetic properties were consistent with changes in the chemical compositions obtained from X-ray Absorption Near-Edge Spectroscopy (XANES), which suggests varying the titanohematite to titanomagnetite content. Increased content in titanomagnetite and magnetic permeability correlated well with the total Fe content in the materials. The best-performing ironsand with the highest permeability and lowest core losses was used alongside Mn,Zn-Ferrite particles (ranging from ~100 μm to 2 mm) to fabricate toroid cores with varying magnetic material loading. It was shown that ironsand can be used to replace up to 15 wt.% of the magnetic materials with minimal impact on the composite magnetic performance, thus reducing the cost. Ironsand was also used as a supporting material in a single-rail wireless power transfer system, effectively increasing the power transfer, demonstrating potential applications to reduce flux leakage.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Uranium and Nickel Partitioning in a Contaminated Riparian Wetland

Uranium (U) and nickel (Ni) released 50 years ago have been immobilized in the Tims Branch wetlands located on the Savannah River Site in the United States. Sediments were collected from seven locations to identify the factors responsible for this attenuation. Ni and U contents in the solids were significantly correlated, suggesting that depositional as opposed to chemical processes contributed to their spatial distribution. Based on sequential extractions, 63 ± 16% of the U was partitioned into the organic fraction, whereas Ni was distributed between several sediment fractions. An inverse pH-organic matter (OM) correlation and positive correlations of OM with total U and organic-bound U/Ni suggest that increased OM preservation and binding to the mineral surfaces were likely responsible for Ni- and especially U-sediment retention (Tims Branch pH = 4.84 ± 0.68). EXAFS analysis indicated the predominance of U(VI) coordinated with clay minerals (~65%), together with ~35% coordinated to either OM (in areas with elevated OM levels) or iron oxides. The desorption-Kd coefficients of U (3972 ± 1370 L/kg) and Ni (30 ± 8 L/kg) indicate that dissolved Ni poses a greater long-term risk than dissolved U for migrating downstream. This study suggests that a delicate balance of geochemical properties controls whether wetlands behave as sinks or sources of contaminants.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗
NASA NTRS1972

A theoretical and experimental investigation of the hypersonic turbulent boundary layer subject to normal and longitudinal pressure gradients and cross flow along a windward plane of symmetry.

A theoretical and experimental investigation for the hypersonic turbulent boundary layer undergoing both normal and longitudinal pressure gradients and cross flow along the plane of symmetry on the windward side of a body of revolution is presented. The purpose of this investigation is to provide a method for calculating boundary layers that occur on the centerline of symmetry of an inlet. The three-dimensional compressible integral equations are written along the symmetry plane and integrated numerically, and the effect of the cross flow on the behavior of the boundary layer is also studied. The experiments were performed at Mach number 6 and Reynolds number of 44,000,000/ft for the axisymmetric case and for the case with cross flow. The velocity profiles and the boundary layer parameters agree relatively well with theoretical values with and without cross flow effects. The presence of the cross flow alters significantly the value of the profiles. Total temperature-velocity correlations deviate from the linear Crocco distribution. Heat transfer rates agree with theoretical values and values obtained by the flat plate reference enthalpy method. Cross flow influence on the heat transfer rates is of minor relevance.

Zakkay, V.↗