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At least 253 records · Page 14

Measurement of the bulk radioactive contamination of detector-grade silicon with DAMIC at SNOLAB

We present measurements of bulk radiocontaminants in the high-resistivity silicon CCDs from the DAMIC experiment at SNOLAB. We utilize the exquisite spatial resolution of CCDs to discriminate between α and β decays, and to search with high efficiency for the spatially-correlated decays of various radioisotope sequences. Using spatially-correlated β decays, we measure a bulk radioactive contamination of 32 Si in the CCDs of 140 ± 30 μBq/kg, and place an upper limit on bulk 210 Pb of < 160 μBq/kg. Using similar analyses of spatially-correlated α and β decays, we set upper limits of < 11 μBq/kg (0.9 ppt) on 238 U and < 7.3 μBq/kg (1.8 ppt) on 232 Th in the bulk silicon. The ability of DAMIC CCDs to identify and reject spatially-coincident backgrounds, particularly from 32 Si, has significant implications for the next generation of silicon-based dark matter experiments, where β's from 32 Si decay will likely be a dominant background.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Isomeric and beta-decay spectroscopy of 173,174 Ho

β-decay spectroscopy of 173,174 Ho (Z = 67, N = 106,107) was conducted at Radioactive Isotope Beam Factory at RIKEN by using in-flight fission of a 345-MeV/u 238 U primary beam. A previously unreported isomeric state at 405 keV with half-life of 3.7(12) μs and a spin and parity of (3/2 + ) is identified in 173 Ho. Moreover, a new state with a spin and parity of 9 - was discovered in 174 Er. The experimental log ft values of 5.84(20) and 5.25(18) suggest an allowed-hindered β decay from the ground state of 174 Ho to the K π = 8 - isomeric state in 174 Er. Configuration-constrained potential energy surface (PES) calculations were performed and the predictions are in reasonable agreement with the experimental results.

150 ≤ A ≤ 189↗

Harvesting 62 Zn from an aqueous cocktail at the NSCL

“Isotope harvesting” is a technique that offers access to exotic radionuclides created as by-products during nuclear science research. Ongoing exploratory work at the National Superconducting Cyclotron Laboratory (NSCL) is directed towards the production and extraction of rare radionuclides from a flowing-water target and intends to pave the way for future harvesting efforts at the upcoming Facility for Rare Isotope Beams (FRIB). Here in this paper, we present the collection of 62 Zn from an aqueous matrix irradiated with a 150 MeV/nucleon 78Kr beam, while synergistically capturing other gaseous reaction products. In addition to the production rate for 62 Zn (9.08(30)E-5 62 Zn per incoming 78 Kr), the rates of formation for several other radionuclides were determined as well. The purification of 62 Zn from a large number of co-produced radionuclides was performed by anion exchange chromatography, allowing the isolation of 80.5(5.2) % of the generated 62 Zn. With the decay of 62 Zn the radioactive daughter 62 Cu is generated, and with the isolation of pure 62 Cu eluate, the principle of a medical radionuclide generator could be demonstrated. To illustrate the applicability of the obtained 62 Zn, the isolated product was used in free and DTPA-labelled form in a proof of principle plant uptake study with garden cress employing phosphor imaging for visualization.

07 ISOTOPE AND RADIATION SOURCES↗

First principles calculations in support of Pu aging: calculating the effects of lattice imperfections on thermodynamics

Plutonium (Pu) has, in theory, well defined crystal structures: its atoms are arranged in regular spatial patterns. But Pu is radioactive, and as its nuclei decay those regular spatial patterns are interrupted. The interruptions are lattice imperfections, which are known to affect how materials respond to their environment. To adequately model Pu, we need to know which lattice imperfections are present, how they interact with each other, and how they affect the material’s response to its environment. The work presented here aims to use density functional theory (DFT) calculations to begin to answer the latter, in particular, how individual lattice imperfections affect measurable effects including thermal expansion (the change in volume in response to a change in temperature), heat capacity (the amount of thermal energy needed to change a material’s temperature), and elastic moduli (a material’s resistance to applied stresses). Pu poses many computational challenges. The $\textit{f}$ electrons require special attention. Of all the elements, Pu has the largest number of electrons that must be included in the calculations. Thermal effects require calculating the phonons (the lattice vibrations), which for systems containing lattice imperfections demand large, complex computational cells - but computational resources limit the size and complexity. With careful restructuring of how the calculations are performed, all these challenges have been met to enable calculations that provide insight into how lattice imperfections affect Pu’s response to its environment. Reported here are the computational challenges and the advances developed to meet them, along with the first results showing the strong effect that one prototype lattice imperfection (an interstitial Pu atom in a delta-phase Pu lattice) has on Pu’s response to its environment.

36 MATERIALS SCIENCE↗

High-temperature 205 Tl decay clarifies 205 Pb dating in early Solar System

Radioactive nuclei with lifetimes on the order of millions of years can reveal the formation history of the Sun and active nucleosynthesis occurring at the time and place of its birth. Among such nuclei whose decay signatures are found in the oldest meteorites, 205 Pb is a powerful example, as it is produced exclusively by slow neutron captures (the s process), with most being synthesized in asymptotic giant branch (AGB) stars. However, making accurate abundance predictions for 205 Pb has so far been impossible because the weak decay rates of 205 Pb and 205 Tl are very uncertain at stellar temperatures. To constrain these decay rates, we measured for the first time the bound-state β - decay of fully ionized 205 Tl 81+ , an exotic decay mode that only occurs in highly charged ions. The measured half-life is 4.7 times longer than the previous theoretical estimate and our 10% experimental uncertainty has eliminated the main nuclear-physics limitation. With new, experimentally backed decay rates, we used AGB stellar models to calculate 205 Pb yields. Propagating those yields with basic galactic chemical evolution (GCE) and comparing with the 205 Pb/ 204 Pb ratio from meteorites, we determined the isolation time of solar material inside its parent molecular cloud. We find positive isolation times that are consistent with the other s-process short-lived radioactive nuclei found in the early Solar System. Our results reaffirm the site of the Sun’s birth as a long-lived, giant molecular cloud and support the use of the 205 Pb– 205 Tl decay system as a chronometer in the early Solar System.

79 ASTRONOMY AND ASTROPHYSICS↗

KATRIN background due to surface radioimpurities

The goal of the KArlsruhe TRItrium Neutrino (KATRIN) experiment is the determination of the effective electron antineutrino mass with a sensitivity of 0.2 eV/c 2 at 90 % C.L. 1 . This goal can only be achieved with a very low background level in the order of 10 mcps 2 in the detector region of interest. A possible background source are α-decays on the inner surface of the KATRIN Main Spectrometer. Rydberg atoms, produced in sputtering processes accompanying the α-decays, are not influenced by electric or magnetic fields and freely propagate inside the vacuum of the Main Spectrometer. Here, they can be ionized by thermal radiation and the released electrons directly contribute to the KATRIN background. Two α-sources, 223 Ra and 228 Th, were installed at the Main Spectrometer with the purpose of temporarily increasing the background in order to study α-decay induced background processes. In this paper, we present a possible background generation mechanism and measurements performed with these two radioactive sources. Our results show a clear correlation between α-activity on the inner spectrometer surface and background from the volume of the spectrometer. Two key characteristics of the Main Spectrometer background – the dependency on the inner electrode offset potential, and the radial distribution – could be reproduced with this artificially induced background. These findings indicate a high contribution of α-decay induced events to the residual KATRIN background.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Investigation of the excited states of 114 Sn using the GRIFFIN spectrometer at TRIUMF

The semi-magic 110-122 Sn isotopes display signs of shape coexistence in their excited 0 + states, which, in contrast to the spherical 0+ ground states, are deformed. Here, this paper investigates the nuclear structure of 114 Sn using the competing β + decay and electron capture of a radioactive beam of 114 Sb produced at the TRIUMF-ISAC facility using the GRIFFIN spectrometer. This study will allow for an in-depth understanding of the excited 0 + states in 114 Sn, by focusing on their decay patterns. In the present experiment, transitions at 856.2-keV and 1405.0-keV, which were observed in an earlier β + decay study but not placed in the 114 Sn level scheme, have been Physics, assigned to the level scheme in connection to the 0$^+_3$ level at 2156.0-keV. Properly assigning these transitions refines the level scheme and enhances our understanding of the nuclear structure in 114 Sn.

GRIFFIN↗

Ion Manipulation from Liquid Xe to Vacuum: Ba-Tagging for a nEXO Upgrade and Future 0 νββ Experiments

Neutrinoless double beta decay (0𝜈𝛽𝛽) provides a way to probe physics beyond the Standard Model of particle physics. The upcoming nEXO experiment will search for 0𝜈𝛽𝛽 decay in 136 Xe with a projected half-life sensitivity exceeding 10 28 years at the 90% confidence level using a liquid xenon (LXe) Time Projection Chamber (TPC) filled with 5 tonnes of Xe enriched to ∼90% in the 𝛽𝛽-decaying isotope 136 Xe. In parallel, a potential future upgrade to nEXO is being investigated with the aim to further suppress radioactive backgrounds and to confirm 𝛽𝛽-decay events. This technique, known as Ba-tagging, comprises extracting and identifying the 𝛽𝛽-decay daughter 136 Ba ion. One tagging approach being pursued involves extracting a small volume of LXe in the vicinity of a potential 𝛽𝛽-decay using a capillary tube and facilitating a liquid-to-gas phase transition by heating the capillary exit. The Ba ion is then separated from the accompanying Xe gas using a radio-frequency (RF) carpet and RF funnel, conclusively identifying the ion as 136 Ba via laser-fluorescence spectroscopy and mass spectrometry. Simultaneously, an accelerator-driven Ba ion source is being developed to validate and optimize this technique. The motivation for the project, the development of the different aspects, along with the current status and results, are discussed here.

a-tagging↗

Choosing the Best Modeling Platform for Radiological Risk Assessment Models - 20468

Radiological risk assessments, in the form of performance or safety assessments, are often required under regulations or guidance for remediation of contaminated land, decommissioning of contaminated buildings or structures, and radioactive waste disposal. These risk assessments are usually supported by fate and transport models that address decay and ingrowth of radionuclides, as well as their movement through engineered systems and the natural environment. These models are often projected thousands, or more, years into the future, largely because the radioactive species change through decay and ingrowth, and hence the magnitude of the radioactive effect changes with time. There are many computer codes that are available to address this type of modeling. They range from addressing specific pathways or processes such as infiltration of water, groundwater, surface water, air, biota, diffusion and advection of water and gases, to those that try to couple all processes together to evaluate the impact of fate and transport through the entire system to places in space and time to which access is assumed. These different types of codes are sometimes separated with the monikers process-level and systems-level codes, although it is often not clear that this separation does justice to the capabilities of the many codes that are available to evaluate fate and transport of radionuclides. The focus of this paper is the latter group of modeling codes. Several systems level modeling codes exist and are used. There are differences between these codes in terms of utility, flexibility, complexity and cost. The purpose of this paper is to compare a few of these codes in the context of work currently being performed by the International Atomic Energy Agency (IAEA) Modeling and Data for Radiological Impact Assessments (MODARIA) II Working Group 1 (WG1). The MODARIA II WG1's main focus is how stakeholder engaged decision analysis can, or should, be applied to radiological contamination problems so that better, longstanding, sustainable, solutions are reached. However, the WG1 also recognizes the potential impact of the modeling tools that are chosen to address radiological risk, which is often a primary objective of decision making for radiological problems. Other objectives might also be important, such as constraining costs, obtaining financing, minimizing impact on ecosystems, saving cultural resources, saving jobs, farmland, environmental justice, etc., in a full decision analysis for a given radiological contamination problem, but none of these other objectives have the same types of complex modeling needs as minimize radiological dose. Consequently, a further focus of WG1 is to evaluate the potential impacts on decision making of the choice of fate and transport, and risk assessment, modeling codes that are used to support decision making. The WG1 will produce a report at the end of 2020 that will focus on an approach to effective decision making and stakeholder engagement. The report will also consider the role that performance assessment modeling should play in the decision-making process, including the impact of the choice of modeling tools or computer codes on risk-informed decision making. Several sites around the World have been made available by Member States for these model comparisons, and several modeling tools have been considered. However, the focus of this paper is on two of the sites, one in Belgium and one in Ukraine, and on three of the tools: NORMALYSA (NORM And Legacy Site Assessment); GoldSim{sup C}, and AMBER{sup C}. The final report from this working group will also cover other modeling tools, including RESRAD, and PC-Cream{sup R}. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Implications of Underground Nuclear Explosion Cavity Evolution for Radioxenon Isotopic Composition

Abstract Isotopic ratios of radioxenons sampled in the atmosphere or subsurface can be used to verify the occurrence of an underground nuclear explosion (UNE). Differences in the half-lives of radioactive xenon precursors and their decay-chain networks produce different time-dependent concentration profiles of xenon isotopes allowing isotopic ratios to be used for tracking UNE histories including estimating the time of detonation. In this study, we explore the potential effects of post-detonation cavity processes: precipitation of iodine precursors, gas seepage, and prompt venting on radioxenon isotopic evolution which influences UNE histories. Simplified analytical models and closed-form solutions yielding a potentially idealized radioactive decay/ingrowth chain in a closed and well-mixed system typically have limited application by not including the partitioning of the radionuclide inventory between a gas phase and rock melt created by the detonation and by ignoring gas transport from the cavity to host rock or ground surface. In reality, either subsurface transport or prompt release that is principally responsible for gas signatures violates the closed-system (or batch-mode) assumption. A closed-form solution representing time-dependent source-term activities is extended by considering the cavity partitioning process, slow seepage, and/or prompt release of gases from the cavity and applied to realistic systems.

Sun, Yunwei (ORCID:0000000194801439)↗

A laserball calibration device for the SNO+ scintillator phase

Located 2 km underground in SNOLAB, Sudbury, Canada, SNO+ is a large scale liquid scintillator experiment that primarily aims to search for neutrinoless double beta decay. Whilst SNO+ has light and radioactive calibration sources external to the inner volume, an internally deployed optical source is necessary for the full characterization of the detector model. A laser diffuser ball developed for SNO has previously demonstrated to be an effective optical calibration device for both SNO and SNO+ water phase. Since the introduction of liquid scintillator for SNO+, the material compatibility, cleanliness, and radiopurity requirements of any materials in contact with the internal medium have increased. Improving on the original SNO laserball design, a new laserball calibration device has been developed for the SNO+ scintillator phase with the goal of measuring the optical properties of the detector and performing routine PMT gain and timing calibrations. Simulations have been written to model the diffusion properties to optimise optical and temporal performance for calibration. Prototype laserballs have been built and characterised, demonstrating sub-ns timing resolution and a quasi-isotropic light distribution.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

High-isospin multiplets in 𝐴=15 and 16 nuclei

Isospin quartets (T=3/2) and quintets (T=2) have been investigated for A=15 and A=16 nuclei, respectively. Data from an invariant-mass experiment, with a 17 Ne beam, were reanalyzed and the T=3/2 and T=2 states in 15 O and 16 F, associated with p+ 14 N and 2p+ 14 N exit channels respectively, were found. In some cases, γ-ray gating was used to tag on events that decay to the excited 0 + , T=1 state in 14 N rather than the ground state. With the new states, the lowest-energy 1/2 + and 5/2 + quartets for A=15 and the 0 + and 2 + quintets for A=16 are completed. In addition, members of these multiplets in 15 F and 16 Ne decaying to the p+ 14 O and 2p+ 14 O channels are reevaluated by gating on events where the 14 O fragment recoils perpendicular to beam axis in the parent reference frame. Such transverse-decay events have the best invariant-mass resolution. No evidence for deviations from a quadratic dependence of the mass on the isospin projection was found for the A=15 quartets. However for the A=16 0 + and 2 + quintets, evidence for deviations were found.

Coulomb energies↗

3 He +𝛼 resonances in 7 Be

Resonances in 7 Be which decay into the 3 He+α exit channel have been measured with improved precision using preexisting data sets. The energy and width of the J π =7/2 - state have been extracted from an invariant-mass study of projectile-breakup products originating from interactions of an E/A=10.7-MeV 10 C beam on Be and C targets. The excitation energy of this state (from the pole of the S-matrix) is determined to be E*=4.545(6)~MeV, a factor of 8 improvement in precision as compared to the ENSDF value. This improvement is enabled by fine tuning the detector calibrations using calibration resonances in 6 Li, 7 Li, 6 Be, 9 B, and 12 C whose decay energies are known to high precision. The J π =7/2- resonance in 7 Be can now itself be used as a calibration resonance in invariant-mass experiments. This utility is particularly helpful for 3 He energy calibrations of CsI(Tl) detectors which are often used in detector arrays employed for measurements with fast beams. This utility is demonstrated with a data set associated with E/A=70 MeV 7 Be beams which are inelastically excited to the 7/2 - and 5/2 - 1 resonances. Again using the pole of the S-matrix as the definition of the resonance parameters, the fitted excitation energy of the 5/2 - 1 resonance is 6.376(17) MeV, approximately 300 keV lower than the ENSDF value. Finally, its width of 565(4) keV is roughly half of the ENSDF value.

energy levels↗

Single-nucleon knockout cross sections for reactions producing resonance states at or beyond the drip line

Single-nucleon knockout cross sections from fast secondary beams of the proton-drip-line nuclei 9 C, 13 O, and 17 Ne on a 9 Be target have been studied with emphasis on the production of resonance states. These states were identified by their invariant mass, and resonances with two-, three-, and five-body exit channels were examined. The measured cross sections for these states were compared with eikonal-model predictions using shell-model or variational Monte Carlo spectroscopic factors. The experimental yields were found to be suppressed relative to the model predictions, especially when a well-bound neutron or proton is removed. This suppression exceeds that found systematically in measured inclusive cross sections to particle-bound final states. In neutron knockout from 9 C and 13 O projectiles, this suppression of the unbound ground-state residuals yield is a factor of two to three times larger than that found in the bound final-state studies. Modifications to the structure of these systems due to coupling of the shell-model configurations to the continuum is expected to contribute to this extra suppression, especially when the final state is a near-threshold resonance. Furthermore, other considerations including the role of nuclear dynamics may be required to explain all the observed trends.

6 ≤ A ≤ 19↗

Fission and the r -process nucleosynthesis of translead nuclei in neutron star mergers

In this report we study the impact of fission on the production and destruction of translead nuclei during the r-process nucleosynthesis occurring in neutron-star mergers. Abundance patterns and rates of nuclear energy production are obtained for different ejecta conditions using three sets of stellar reaction rates, one of which is based on microscopic and consistent calculations of nuclear masses, fission barriers, and collective inertias. We show that the accumulation of fissioning material during the r process can strongly affect the free neutron abundance after the r-process freeze-out. This leads to a significant impact on the abundances of heavy nuclei that undergo α decay or spontaneous fission, affecting the radioactive energy production by the ejecta at timescales relevant for kilonova emission.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Using spin alignment of inelastically excited nuclei in fast beams to assign spins: The spectroscopy of 13 O as a test case

Excited states in O 13 were investigated using inelastic scattering of an E / A = 69.5 MeV O 13 beam off of a Be 9 target. The excited states were identified in the invariant-mass spectra of the decay products. Both single-proton and sequential two-proton decays of the excited states were examined. Furthermore, for a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave Born-approximation calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced O 13 level scheme is compared to ab initio no-core shell model with continuum predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1 s 1 / 2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Spectroscopy of 10 N with the invariant-mass method

Proton decays of $^{10}$N states has been investigated with the invariant-mass technique using data from two reactions. In the first experiment, $^{10}$N states were created via multi-nucleon knockout from a fast $^{13}$O beam. The second experiment involved proton pickup from a $^9$Be target to a fast $^9$C beam. Both data sets produce similar distributions with a peak centered at a decay energy of 2.8 MeV and a width of $\approx 2.5$ MeV. This result is consistent with a previous study using multi-nucleon transfer reaction which was originally fit with an $\ell$ = 0 resonance but later interpreted as an $\ell$=1 resonance. This later interpretation is affirmed as the proton pickup reaction should favor $\ell$ = 1. This strength is located near the predicted energies of two $\ell$ = 1 resonances in calculations using complex scaling and the Gamow shell model. Furthermore, the multi-nucleon knockout data also show excess strength below the main peak which is interpreted as contributions from one or more $\ell$ = 0 resonances.

6 ≤ A ≤ 19↗

Decay spectroscopy of 160 Eu: Quasiparticle configurations of excited states and structure of K π = 4 + bandheads in 160 Gd

Background: Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. Purpose: We aim to improve the understanding of the nuclear structure of 160 Gd, specifically the K π = 4 + bands, as well as study the β decay of 160 Eu into 160 Gd. Methods: High-statistics decay spectroscopy of 160 Gd resulting from the β-decay of 160 Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. Results: Two new excited states and ten new transitions were observed in 160 Gd. The β-decaying half-lives of the low- and high-spin isomers in 160 Eu were determined, and the low-spin state's half-life was measured to be t 1/2 = 26.0 (8) s, ≈ 16% shorter than previous measurements. Lifetimes of the two K π = 4 + bandheads in 160 Gd were measured for the first time, as well as γ – γ angular correlations and mixing ratios of intense transitions out of those bandheads. Conclusions: Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the K π = 4 + bandheads in 160 Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0-keV state in 160 Gd heavily populated in β decay is shown to have positive parity, which raises questions regarding the structure of the high-spin β-decaying state in 160 Eu.

150 ≤ A ≤ 189↗