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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 253 records · Page 14

Bridging the academic and industrial metrics for next-generation practical batteries

Batteries have shaped the modern world to an extent far beyond that of other technologies. This success is the result of the intense collaboration between Academia and Industry that took shape in the past several decades culminating with the advent and improvements of rechargeable Li-ion batteries. However, as applications are getting more demanding, stunted growth in the performance of commercial batteries risks to slow down the adoption of important technologies, such as electric vehicles. Yet, the scientific literature is full of reports describing material designs with allegedly superior performances. A large gap needs to be filled if we wish these lab-based achievements reach commercialization. In this Perspective we discuss some of the most relevant testing parameters that are often overlooked in academic literature, but that are critical for the practical applicability of lab-scale research. Metrics, such as anode energy density, voltage hysteresis, mass of the non-active cell components and anode/cathode mass ratio, will be explained and recommendation for future reporting will be made at the end of each section. We hope that this Perspective, together with other similar guiding principles that have recently started to emerge, will aid the transition from lab-scale research to next-generation practical batteries

Cao, Yuliang↗

Hybrid approach for estimating dynamic states of synchronous generators

Accurate and robust estimation of dynamic states is essential for monitoring and controlling a power grid. To achieve higher accuracy and robustness, this paper proposes a hybrid estimation approach to estimate the dynamic states of synchronous generators using multiple models, classified into a set of local models and a wide-area model. The proposed estimation approach, first, estimates dynamic states using the extended Kalman filter (EKF) based on a local model and a wide-area model. Then, at each time step, probability indexes, which quantify the likelihood of both local and wide-area models, are determined using hypothesis testing based on measurements innovations. Finally, using the weighted fix approach, the states estimated from the local and wide-area models are combined based on their probability indexes. Simulation studies using the two-area four-machine system shows that the proposed approach can improve estimation accuracy and increase robustness against model errors.

Akhlaghi, Shahrokh↗

Analyses of the plasma generated by laser irradiation on sputtered target for determination of the thickness used for plasma generation

In Brookhaven National Laboratory, laser ion source has been developed to provide heavy ion beams by using plasma generation with 1064 nm Nd:YAG laser irradiation onto solid targets. The laser energy is transferred to the target material and creates a crater on the surface. However, only the partial material can be turned into plasma state and the other portion is considered to be just vaporized. Since heat propagation in the target material requires more than typical laser irradiation period, which is typically several ns, only the certain depth of the layers may contribute to form the plasma. As a result, the depth is more than 500 nm because the base material Al ions were detected. On the other hand, the result of comparing each carbon thickness case suggests that the surface carbon layer is not contributed to generate plasma.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Efficient Raman generation in a waveguide: A route to ultrafast quantum random number generation

The inherent uncertainty in quantum mechanics offers a source of true randomness which can be used to produce unbreakable cryptographic keys. We discuss the development of a high-speed random number generator based on the quantum phase fluctuations in spontaneously initiated stimulated Raman scattering (SISRS). We utilize the tight confinement and long interaction length available in a Potassium Titanyl Phosphate waveguide to generate highly efficient SISRS using nanojoule pulse energies, reducing the high pump power requirements of the previous approaches. We measure the random phase of the Stokes output using a simple interferometric setup to yield quantum random numbers at 145 Mbps.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

An ITPA joint experiment to study runaway electron generation and suppression

Recent results from an ITPA joint experiment to study the onset, growth, and decay of relativistic electrons (REs) indicate that loss mechanisms other than collisional damping may play a dominant role in the dynamics of the RE population, even during the quiescent I{sub p} flattop. Understanding the physics of RE growth and mitigation is motivated by the theoretical prediction that disruptions of full-current (15 MA) ITER discharges could generate up to 10 MA of REs with 10–20 MeV energies. The ITPA MHD group is conducting a joint experiment to measure the RE detection threshold conditions on a number of tokamaks under quasi-steady-state conditions in which V{sub loop}, n{sub e}, and REs can be well-diagnosed and compared to collisional theory. Data from DIII-D, C-Mod, FTU, KSTAR, and TEXTOR have been obtained so far, and the consensus to date is that the threshold E-field is significantly higher than predicted by relativistic collisional theory, or conversely, the density required to damp REs is significantly less than predicted, which could have significant implications for RE mitigation on ITER.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Generation and focusing of electron beams with initial transverse-longitudinal correlation

In charged particle beams, one of the roles played by space charge is to couple the transverse and longitudinal dynamics of the beam. This can lead to very complex phenomena which are generally studied using computer simulations. However, in some cases models based on phenomenological or analytic approximations can provide valuable insight into the system behavior. In this paper, we employ such approximations to investigate the conditions under which all the slices of a space charge dominated electron beam with slowly varying current could be focused to a waist with the same radius and at the same location, independent of slice current, and show that this can be accomplished approximately if the initial transverse-longitudinal correlation introduced onto the beam by the electron gun is chosen to compensate for the transverse-longitudinal correlation introduced onto the beam in the drift section. The validity of our approximations is assessed by use of progressively more realistic calculations. We also consider several design elements of electron guns that affect the initial correlations in the beams they generate.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Slowing of Femtosecond Laser-Generated Nanoparticles in a Background Gas

The slowing of Pt nanoparticles in argon background gas was characterized by Rayleigh scattering imaging using a plume of nanoparticles generated by femtosecond laser through thin film ablation (fs-TTFA) of 20 nanometers-thick Pt films. The ablation was performed at threshold laser energy fluences for complete film removal to provide a well-defined plume consisting almost entirely of nanoparticles traveling with a narrow velocity distribution, providing a unique system to unambiguously characterize the slowing of nanoparticles during interaction with background gases. Nanoparticles of ~200 nm diameter were found to decelerate in background Ar gas with pressures less than 50 Torr in good agreement with a linear drag model in the Epstein regime. Based on this model, the stopping distance of small nanoparticles in the plume was predicted and tested by particle collection in an off-axis geometry, and size distribution analysis by transmission electron microscopy. These results permit a basis to interpret nanoparticle propagation through background gases in laser ablation plumes that contain mixed components.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Visible light carrier generation in co-doped epitaxial titanate films

Perovskite titanates such as SrTiO{sub 3} (STO) exhibit a wide range of important functional properties, including ferroelectricity and excellent photocatalytic performance. The wide optical band gap of titanates limits their use in these applications; however, making them ill-suited for integration into solar energy harvesting technologies. Our recent work has shown that by doping STO with equal concentrations of La and Cr, we can enhance visible light absorption in epitaxial thin films while avoiding any compensating defects. In this work, we explore the optical properties of photoexcited carriers in these films. Using spectroscopic ellipsometry, we show that the Cr{sup 3+} dopants, which produce electronic states immediately above the top of the O 2p valence band in STO reduce the direct band gap of the material from 3.75 eV to 2.4–2.7 eV depending on doping levels. Transient reflectance spectroscopy measurements are in agreement with the observations from ellipsometry and confirm that optically generated carriers are present for longer than 2 ns. Finally, through photoelectrochemical methylene blue degradation measurements, we show that these co-doped films exhibit enhanced visible light photocatalysis when compared to pure STO.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Gigawatt-class radiation generated by a Ka-band overmoded Cherenkov-type high power millimeter wave generator

Particle simulation and experimental results are presented about a Ka-band overmoded Cherenkov-type high power millimeter wave generator in this paper. The relativistic electron beam with peak current of 8.4 kA was generated by a pulsed power accelerator working at the voltage of 625 kV, which was guided by an axial magnetic field of 1.05 T and transported through the beam-wave interaction structures. After careful calibration, the microwave power radiated in the far field was as high as about 500 MW, with a frequency of 32.1 GHz and a pulse width of 20 ns. The radiation mode was well controlled to be TM{sub 0n} mode.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Positron generation using laser-wakefield electron sources

Positron generation, using wakefield-accelerated electrons driven into a converter target, was investigated experimentally and through Monte Carlo simulations. Using experimentally measured initial electron distributions from a 60 fs laser system, modeling shows that a collimated wakefield electron beam of moderate energy (50–200 MeV) produces a large number of positrons (~10 7 ), which are emitted from the rear of a mm-scale, high-Z target with divergence angles between 50 and 150 mrad. The large perpendicular momentum of the positrons was found to be dominated by contributions from multiple small angle Coulomb scattering. Positrons were not observed above background noise for a range of targets where simulations indicate a 5–30× increase in the beam charge was necessary to exceed threshold detection. These results provide new understanding to the fundamental limitations of creating narrow-divergence, high-density positron beams from laser-wakefield platforms for use in future laboratory pair plasma experiments.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Small scale coherent vortex generation in drift wave-zonal flow turbulence

We present a paradigm for the generation of small scale coherent vortex (SSCV) in drift wave-zonal flow (DW-ZF) turbulence. We demonstrate that phases of DWs can couple coherently, mediated by the ZF shearing. A SSCV is formed when the phases of the DWs are “attracted” to form a stable “phase cluster.” We show that the ZF shearing induces asymmetry between “attractive” and “repulsive” phase couplings, so that a net attractive phase coupling results. The turbulent DWs will (partially)synchronize into a stable SSCV at locations, where the attractive phase coupling induced by the ZF shearing exceeds the “detuning” effects by the DW dispersion and random phase scattering. We also discuss the “self-binding” effect of the newly formed SSCV.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Thermal generation of spin current in epitaxial CoFe 2 O 4 thin films

The longitudinal spin Seebeck effect (LSSE) has been investigated in high-quality epitaxial CoFe 2 O 4 (CFO) thin films. The thermally excited spin currents in the CFO films are electrically detected in adjacent Pt layers due to the inverse spin Hall effect (ISHE). The LSSE signal exhibits a linear increase with increasing temperature gradient, yielding a LSSE coefficient of –100 nV/K at room temperature. The temperature dependence of the LSSE is investigated from room temperature down to 30 K, showing a significant reduction at low temperatures, revealing that the total amount of thermally generated magnons decreases. Moreover, we demonstrate that the spin Seebeck effect is an effective tool to study the magnetic anisotropy induced by epitaxial strain, especially in ultrathin films with low magnetic moments.

36 MATERIALS SCIENCE↗

Robust and compact entanglement generation from diode-laser-pumped four-wave mixing

Four-wave-mixing processes are now routinely used to demonstrate multi-spatial-mode Einstein-Podolsky-Rosen entanglement and intensity difference squeezing. Diode-laser-pumped four-wave mixing processes have recently been shown to provide an affordable, compact, and stable source for intensity difference squeezing, but it was unknown if excess phase noise present in power amplifier pump configurations would be an impediment to achieving quadrature entanglement. Here, we demonstrate the operating regimes under which these systems are capable of producing entanglement and under which excess phase noise produced by the amplifier contaminates the output state. We show that Einstein-Podolsky-Rosen entanglement in two mode squeezed states can be generated by a four-wave-mixing source deriving both the pump field and the local oscillators from a tapered-amplifier diode-laser. This robust continuous variable entanglement source is highly scalable and amenable to miniaturization, making it a critical step toward the development of integrated quantum sensors and scalable quantum information processors, such as spatial comb cluster states.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Characterization of mechanical deformation in aluminum by optical second harmonic generation

Second harmonic generation (SHG), a laser-based surface technique, was used to characterize near-surface defect evolution associated with mechanical deformation in 2024-T3 aluminum due to tensile loads. Electron backscatter diffraction (EBSD) measurements were also performed to determine the geometrically necessary dislocation density before and after tensile deformation. Comparison of the EBSD and SHG results found that dislocation density and SHG signal are inversely proportional; tensile deformation in the plastic regime led to an increase in dislocation density and a decrease in SHG response. A similar trend was seen in the SHG results on as-received (unpolished) Al samples; SHG response decreases with extent of plastic deformation. Furthermore, this study suggests that SHG has potential as a nondestructive evaluation technique.

36 MATERIALS SCIENCE↗

Search for pair-produced third-generation squarks decaying via charm quarks or in compressed supersymmetric scenarios in p p collisions at s = 8 TeV with the ATLAS detector

Results of a search for supersymmetry via direct production of third-generation squarks are reported, using 20.3 fb -1 of proton-proton collision data at $ \sqrt{s} $=8 TeV recorded by the ATLAS experiment at the LHC in 2012. Two different analysis strategies based on monojetlike and c-tagged event selections are carried out to optimize the sensitivity for direct top squark-pair production in the decay channel to a charm quark and the lightest neutralino ($ \tilde{t} $ -1 →c+ $ \tilde{χ} ^0_1 $) across the top squark-neutralino mass parameter space. No excess above the Standard Model background expectation is observed. The results are interpreted in the context of direct pair production of top squarks and presented in terms of exclusion limits in the (m $ \tilde{t} $ -1 , m $ \tilde{χ} ^0_1 $ ) parameter space. A top squark of mass up to about 240 GeV is excluded at 95% confidence level for arbitrary neutralino masses, within the kinematic boundaries. Top squark masses up to 270 GeV are excluded for a neutralino mass of 200 GeV. In a scenario where the top squark and the lightest neutralino are nearly degenerate in mass, top squark masses up to 260 GeV are excluded. The results from the monojetlike analysis are also interpreted in terms of compressed scenarios for top squark-pair production in the decay channel $ \tilde{t} $ -1 → b + ff' +$ \tilde{χ} ^0_1 $ and sbottom pair production with $ \tilde{b} $ 1 → b +$ \tilde{χ} ^0_1 $, leading to a similar exclusion for nearly mass-degenerate third-generation squarks and the lightest neutralino. The results in this paper significantly extend previous results at colliders.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗