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NASA NTRS1995

Condensed Water in Tropical Cyclone "Oliver", 8 February 1993

On February 8, 1993, the NASA DC-8 aircraft profiled from 10,000 to 37,000 feet (3.1-11.3 km) pressure altitude in a stratified section of tropical cyclone "Oliver" over the Coral Sea northeast of Australia. Size, shape and phase of cloud and precipitation particles were measured with a 2-D Greyscale probe. Cloud/precipitation particles changed from liquid to ice as soon as the freezing level was reached near 17,000 feet (5.2 km) pressure altitude. The cloud was completely glaciated at -5 C. There was no correlation between ice particle habit and ambient temperature. In the liquid phase, the precipitation-cloud drop concentration was 4.0 x 10(exp 3)/cu m, the geometric mean diameter D(sub g) = 0.5-0.7 mm, and the liquid water content 0.7-1.9 g m(exp-3). The largest particles anywhere in the cloud, dominated by fused dendrites at concentrations similar to that of raindrops (2.5 x 10(exp 3) m(exp -3)) but a higher condensed water content(5.4 g/cu m estimated) were found in the mixed phase; condensed water is removed very effectively from the mixed layer due to high settling velocities of the large mixed particles. The highest number concentration (4.9 x 10(exp 4)/cu m, smallest size (D(sub g) = 0.3-0.4 mm), largest surface area (up to 2.6 x 10 (exp 2) sq cm/cu m at 0.4- 1.0 g/cu m of condensate) existed in the ice phase at the coldest temperature (- 40 C) at 35,000 feet ( 10.7 km). Each cloud contained aerosol (haze particles) in addition to cloud particles. The aerosol total surface area exceeded that of the cirrus particles at the coldest temperature. Thus, aerosols must play a significant role in the upscattering of solar radiation. Light extinction (6.2/km) and backscatter (0.8/sr/km) was highest in the coldest portion of the cirrus cloud at the highest altitude.

Pueschel, R. F.↗

NASA NTRS1990

A parameterization for the shortwave transmissivity of stratiform water clouds based on empirical data and radiative transfer theory

Surface measurements of solar flux and total integrated liquid-water content, radiosonde data, and infrared satellite images are analyzed in conjunction with radiative transfer calculations to derive an empirical parameterization for the shortwave transmissivity of continental stratiform water clouds. The data were collected near Denver, Colorado, over a period of six years. A multiple reflection radiative transfer model is employed to estimate stratus cloud transmissivity in terms of the measurable liquid-water path (LWP). A nonlinear fit of estimated transmissivities to the corresponding observations of LWP yields close agreement with a previous, more complicated parameterization. The derived expression for cloud transmissivity is used to predict mean daily surface fluxes for 61 days during which periods of stratiform clouds were observed over the Denver area. A comparison between predicted and measured fluxes shows agreement to within + or - 4 percent, with best agreement for clouds of moderate optical thickness. Potential sources of error are identified with sensitivity studies.

Derr, V. E.↗

DOE OSTI2023

Insights into the relation between vertical cloud structure and dynamics of three polar lows: Observations from COMBLE

The vertical structure of three polar lows is described using profiling radar, lidar, and passive remote sensors deployed at a coastal site in northern Norway. The data were collected as part of the Cold-air Outbreaks in the Marine Boundary Layer Experiment (COMBLE). These data are examined in the context of satellite imagery, operational weather radar reflectivity imagery, and output from the AROME-Arctic model. A comparison to satellite images shows that AROME-Arctic captured the polar lows well. All three polar lows form in marine cold-air outbreaks and are surrounded by open-cellular convection typical of such outbreaks. Two of the lows form in a forward shear environment, and one under reverse shear. Initially, the three polar lows are comma-shaped; two of them transition to be more spirali-form at their mature stage and have mostly cloud-free warm cores. The warm cores are the result of a warm-seclusion process. All three lows have stratiform precipitation bands, marked by little cloud liquid water, and rather high surface precipitation rate. The vertical drafts and turbulence in these stratiform clouds are generally weak. In conclusion, all three lows also have convective clouds, which have stronger vertical drafts, stronger turbulence, and pockets of high liquid water content.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2011

Understanding Effective Diameter and Its Application to Terrestrial Radiation in Ice Clouds

The cloud property known as "effective diameter" or "effective radius", which in essence is the cloud particle size distribution (PSD) volume at bulk density divided by its projected area, is used extensively in atmospheric radiation transfer, climate modeling and remote sensing. This derives from the assumption that PSD optical properties can be uniquely described in terms of their effective diameter, D(sub e), and their cloud water content (CWC), henceforth referred to as the D(sub e)-CWC assumption. This study challenges this assumption, showing that while the D(sub e)-CWC assumption appears generally valid for liquid water clouds, it appears less valid for ice clouds in regions where (1) absorption is not primarily a function of either the PSD ice water content (IWC) or the PSD projected area, and (2) where wave resonance (i.e. photon tunneling) contributes significantly to absorption. These two regions often strongly coincide at terrestrial wavelengths when De less than ~60 m, which is where this D(sub e)-CWC assumption appears poorest. Treating optical properties solely in terms of D(sub e) and IWC may lead to errors up to 24%, 26% and 20% for terrestrial radiation in the window region regarding the absorption and extinction coefficients and the single scattering albedo, respectively. Outside the window region, errors may reach 33% and 42% regarding absorption and extinction. The magnitude and sign of these errors can change rapidly with wavelength, which may produce significant errors in climate modeling, remote sensing and other applications concerned with the wavelength dependence of radiation. Where the D(sub e)-CWC assumption breaks down, ice cloud optical properties appear to depend on D(sub e), IWC and the PSD shape. Optical property parameterizations in climate models and remote sensing algorithms based on historical PSD measurements may exhibit errors due to previously unknown PSD errors (i.e. the presence of ice artifacts due to the shattering of larger ice particles on the probe inlet tube during sampling). More recently developed cloud probes are designed to mitigate this shattering problem. Using realistic PSD shapes for a given temperature (and/or IWC) and cloud type may minimize errors associated with PSD shape in ice optics parameterizations and remote sensing algorithms. While this topic was investigated using two ice optics schemes (the Yang et al., 2005 database and the modified anomalous diffraction approximation, or MADA), a physical understanding of the limitations of the D(sub e)-IWC assumption was made possible by using MADA. MADA allows one to approximate the contribution of photon tunneling to absorption relative to other optical processes, which reveals that part of the error regarding the D(sub e)-IWC assumption can be associated with tunneling. By relating the remaining error to the radiation penetration depth in bulk ice (DELTA L) due to absorption, the domain where the D(sub e)-IWC assumption is weakest was described in terms of D(sub e) and DELTA L.

Mitchell, D. L.↗

DOE OSTI2022

The FastEddy® Resident-GPU Accelerated Large-Eddy Simulation Framework: Moist Dynamics Extension, Validation and Sensitivities of Modeling Non-Precipitating Shallow Cumulus Clouds

Herein we describe the moist dynamics formulation implemented within the graphics processing unit-resident large-eddy simulation FastEddy® model, which includes a simple saturation adjustment scheme for condensation and evaporation processes. Two LES model intercomparison exercises for non-precipitating shallow cumulus clouds are simulated in order to validate this model extension, including a static forcing and a time-dependent forcing case. Overall, we find our dynamical, thermodynamical and microphysical quantities, along with turbulence variability and fluxes, to be commensurate with the corresponding model intercomparison results. In addition, sensitivities to specific model settings are investigated. Among these settings, it is shown that boundary layer and cloud layer structure and characteristics are sensitive to use of higher-order advection schemes impacting the vertical distribution of cloud content and associated turbulence statistics. Increasing the timescale of the saturation scheme leads to enhanced liquid water presence and decreases vertical velocity variance within the cloud deck. In some cases, these sensitivities agree with the model-to-model variability reported in the intercomparison exercises, highlighting the important role of specific model implementation choices in the context of shallow cumulus convection simulations. These analyses and findings also provide the basis for future extensions and applications of FastEddy® for modeling moist convection and precipitation scenarios.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1990

Microwave (SSM/I) Estimates of the Precipitation Rate to Improve Numerical Atmospheric Model Forecasts

Delay in the spin-up of precipitation early in numerical atmospheric forecasts is a deficiency correctable by diabatic initialization combined with diabatic forcing. For either to be effective requires some knowledge of the magnitude and vertical placement of the latent heating fields. Until recently the best source of cloud and rain water data was the remotely sensed vertical integrated precipitation rate or liquid water content. Vertical placement of the condensation remains unknown. Some information about the vertical distribution of the heating rates and precipitating liquid water and ice can be obtained from retrieval techniques that use a physical model of precipitating clouds to refine and improve the interpretation of the remotely sensed data. A description of this procedure and an examination of its 3-D liquid water products, along with improved modeling methods that enhance or speed-up storm development is discussed.

Raymond, William H.↗

NASA NTRS1994

Simulations of the effects of water vapor, cloud liquid water, and ice on AMSU moisture channel brightness temperatures

Radiative transfer simulations are performed to determine how water vapor and nonprecipitating cloud liquid water and ice particles within typical midlatitude atmospheres affect brightness temperatures T(sub B)'s of moisture sounding channels used in the Advanced Microwave Sounding Unit (AMSU) and AMSU-like instruments. The purpose is to promote a general understanding of passive top-of-atmosphere T(sub B)'s for window frequencies at 23.8, 89.0, and 157.0 GHz, and water vapor frequencies at 176.31, 180.31, and 182.31 GHz by documenting specific examples. This is accomplished through detailed analyses of T(sub B)'s for idealized atmospheres, mostly representing temperate conditions over land. Cloud effects are considered in terms of five basic properties: droplet size distribution, phase, liquid or ice water content, altitude, and thickness. Effects on T(sub B) of changing surface emissivity also are addressed. The brightness temperature contribution functions are presented as an aid to physically interpreting AMSU T(sub B)'s. Both liquid and ice clouds impact the T(sub B)'s in a variety of ways. The T(sub B)'s at 23.8 and 89 GHz are more strongly affected by altostratus liquid clouds than by cirrus clouds for equivalent water paths. In contrast, channels near 157 and 183 GHz are more strongly affected by ice clouds. Higher clouds have a greater impact on 157- and 183-GHz T(sub B)'s than do lower clouds. Clouds depress T(sub B)'s of the higher-frequency channels by suppressing, but not necessarily obscuring, radiance contributions from below. Thus, T(sub B)'s are less closely associated with cloud-top temperatures than are IR radiometric temperatures. Water vapor alone accounts for up to 89% of the total attenuation by a midtropospheric liquid cloud for channels near 183 GHz. The Rayleigh approximation is found to be adequate for typical droplet size distributions; however, Mie scattering effects from liquid droplets become important for droplet size distribution functions with modal radii greater than 20 micrometers near 157 and 183 GHz, and greater than 30-40 micrometers at 89 GHz. This is due mainly to the relatively small concentrations of droplets much larger than the mode radius. Orographic clouds and tropical cumuli have been observed to contain droplet size distributions with mode radii in the 30-40 micrometers range. Thus, as new instruments bridge the gap between microwave and infrared to frequencies even higher than 183 GHz, radiative transfer modelers are cautioned to explicitly address scattering characteristics of such clouds.

Muller, Bradley M.↗

DOE OSTI2024

Partition between supercooled liquid droplets and ice crystals in mixed-phase clouds based on airborne in situ observations

Abstract. The onset of ice nucleation in mixed-phase clouds determines the lifetime and microphysical properties of ice clouds. In this work, we develop a novel method that differentiates between various phases of mixed-phase clouds, such as clouds dominated by pure liquid or pure ice segments, compared with those having ice crystals surrounded by supercooled liquid water droplets or vice versa. Using this method, we examine the relationship between the macrophysical and microphysical properties of Southern Ocean mixed-phase clouds at −40 to 0 °C (e.g. stratiform and cumuliform clouds) based on the in situ aircraft-based observations during the US National Science Foundation Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) flight campaign. The results show that the exchange between supercooled liquid water and ice crystals from a macrophysical perspective, represented by the increasing spatial ratio of regions containing ice crystals relative to the total in-cloud region (defined as ice spatial ratio), is positively correlated with the phase exchange from a microphysical perspective, represented by the increasing ice water content (IWC), decreasing liquid water content (LWC), increasing ice mass fraction, and increasing ice particle number fraction (IPNF). The mass exchange between liquid and ice becomes more significant during phase 3 when pure ice cloud regions (ICRs) start to appear. Occurrence frequencies of cloud thermodynamic phases show a significant phase change from liquid to ice at a similar temperature (i.e. −17.5 °C) among three types of definitions of mixed-phase clouds based on ice spatial ratio, ice mass fraction, or IPNF. Aerosol indirect effects are quantified for different phases using number concentrations of aerosols greater than 100 or 500 nm (N>100 and N>500, respectively). N>500 shows stronger positive correlations with ice spatial ratios compared with N>100. This result indicates that larger aerosols potentially contain ice-nucleating particles (INPs), which facilitate the formation of ice crystals in mixed-phase clouds. The impact of N>500 is also more significant in phase 2 when ice crystals just start to appear in the mixed phase compared with phase 3 when pure ICRs have formed, possibly due to the competing aerosol indirect effects on primary and secondary ice production in phase 3. The thermodynamic and dynamic conditions are quantified for each phase. The results show stronger in-cloud turbulence and higher updraughts in phases 2 and 3 when liquid and ice coexist compared with pure liquid or ice (phases 1 and 4, respectively). The highest updraughts and turbulence are seen in phase 3 when supercooled liquid droplets are surrounded by ice crystals. These results indicate both updraughts and turbulence support the maintenance of supercooled liquid water amongst ice crystals. Overall, these results illustrate the varying effects of aerosols, thermodynamics, and dynamics through various stages of mixed-phase cloud evolution based on this new method that categorizes cloud phases.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRSDate not supplied

Observing Ice Phase Clouds and Precipitation with Millimeter- and Submillimeter-wave Radiometry during the IMPACTS field campaign: Algorithm Development for the Emerging Class of Microwave Radiometers

Millimeter- and submillimeter-wave (mmWave, submm) radiometers provide significant information content on atmospheric water in liquid, ice, and vapor phases. Recent sensors, such as the Global Precipitation Measurement (GPM) or the Temporal Experiment for Storms and Tropical Systems Technology – Demonstration (TEMPEST-D), use mmWave bands to improve estimation of ice-phase precipitation, and future missions, such as the Atmosphere Observing System (AOS), will extend to submm to provide additional information on thinner ice clouds, linking clouds and precipitation and therefore elucidating the links between weather, climate, and the water cycle. To support the expanded use of mmWave/submm radiometry and exploit the available information content on condensed water mass, we demonstrate ice and liquid water path retrievals for NASA Goddard Space Flight Center's airborne radiometers the Conical Scanning Millimeter-wave Imaging Radiometer (CoSMIR) and the Configurable Scanning Submillimeter-wave Instrument/Radiometer (CoSSIR, formerly the Compact Scanning Submillimeter Imaging Radiometer). The analysis is based on data collected during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS) field campaign. A simulation study compares and contrasts retrievals for CoSMIR and CoSSIR, with CoSSIR demonstrating higher skill in ice retrievals, particularly for thin clouds, and the CoSMIR frequencies performing better for liquid. Additionally, we look at dual-polarized radiances observed by CoSMIR during the first two IMPACTS deployments to understand the polarization signatures induced by oriented hydrometeors. Results will be presented in the context of upcoming missions and sensors including AOS and the Ice Cloud Imager (ICI). We will describe the objectives for the expected first flight of the newly upgraded CoSSIR during the final IMPACTS deployment, and we will share novel science investigations we plan to undertake with CoSSIR's new capabilities. Popular Summary: Ice in clouds and falling snow is an important component of weather, climate, and water resources. To better use a new class of sensors that provide information on atmospheric ice, we developed an approach to measure ice clouds and falling snow using airborne data taken during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Storms (IMPACTS), a field campaign to study winter storms. We look at the results for two similar instruments to understand how those differences affect these measurements of clouds and snow, and we further investigate the information the sensors can provide on properties of the clouds and snow.

Ian S Adams↗

NASA NTRSDate not supplied

Observing Ice Phase Clouds and Precipitation with Millimeter- and Submillimeter-wave Radiometry during the IMPACTS field campaign: Algorithm Development for the Emerging Class of Microwave Radiometers

Ian S Adams↗

NASA NTRS2001

Icing Cloud Calibration of the NASA Glenn Icing Research Tunnel

The icing research tunnel at the NASA Glenn Research Center underwent a major rehabilitation in 1999, necessitating recalibration of the icing clouds. This report describes the methods used in the recalibration, including the procedure used to establish a uniform icing cloud and the use of a standard icing blade technique for measurement of liquid water content. The instruments and methods used to perform the droplet size calibration are also described. The liquid water content/droplet size operating envelopes of the icing tunnel are shown for a range of airspeeds and compared to the FAA icing certification criteria. The capabilities of the IRT to produce large droplet icing clouds is also detailed.

Ide, Robert F.↗

DOE OSTI2024

Droplet Growth or Evaporation Does Not Buffer the Variability in Supersaturation in Clean Clouds

Abstract Water vapor supersaturation in clouds is a random variable that drives activation and growth of cloud droplets. The Pi Convection–Cloud Chamber generates a turbulent cloud with a microphysical steady state that can be varied from clean to polluted by adjusting the aerosol injection rate. The supersaturation distribution and its moments, e.g., mean and variance, are investigated for varying cloud microphysical conditions. High-speed and collocated Eulerian measurements of temperature and water vapor concentration are combined to obtain the temporally resolved supersaturation distribution. This allows quantification of the contributions of variances and covariances between water vapor and temperature. Results are consistent with expectations for a convection chamber, with strong correlation between water vapor and temperature; departures from ideal behavior can be explained as resulting from dry regions on the warm boundary, analogous to entrainment. The saturation ratio distribution is measured under conditions that show monotonic increase of liquid water content and decrease of mean droplet diameter with increasing aerosol injection rate. The change in liquid water content is proportional to the change in water vapor concentration between no-cloud and cloudy conditions. Variability in the supersaturation remains even after cloud droplets are formed, and no significant buffering is observed. Results are interpreted in terms of a cloud microphysical Damköhler number (Da), under conditions corresponding to , i.e., the slow-microphysics regime. This implies that clouds with very clean regions, such that is satisfied, will experience supersaturation fluctuations without them being buffered by cloud droplet growth. Significance Statement The saturation ratio (humidity) in clouds controls the growth rate and formation of cloud droplets. When air in a turbulent cloud mixes, the humidity varies in space and time throughout the cloud. This is important because it means cloud droplets experience different growth histories, thereby resulting in broader size distributions. It is often assumed that growth and evaporation of cloud droplets buffers out some of the humidity variations. Measuring these variations has been difficult, especially in the field. The purpose of this study is to measure the saturation ratio distribution in clouds with a range of conditions. We measure the in-cloud saturation ratio using a convection cloud chamber with clean to polluted cloud properties. We found in clouds with low concentrations of droplets that the variations in the saturation ratio are not suppressed.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Cloud microphysical structure analysis based on high-resolution insitu measurements

This study investigates the microphysical parameters and shapes of droplet size distributions (DSDs) along three aircraft traverses of developing convective clouds during Cloud Aerosol Interactions and Precipitation Enhancement Experiment (CAIPEEX) Phase III 2015 at a sampling frequency of 25 Hz. The droplet number concentration (Nc, cm -3 ), and liquid water content (LWC, g m -3 ) present steep gradients within zones of a few tens of meters near the cloud edges and relatively gentle gradients in the strong updraft zones. Sometimes, the horizontal LWC distribution resembles a trapezoidal shape with steep LWC and Nc gradients near the cloud edges. The LWC maximums (LWC max ) are lower than the adiabatic LWCs, but the high adiabatic fractions in the cloud core indicate low dilution. High LWC/LWC max , largest droplets, and narrow and similarly shaped DSDs are found in the regions of high updrafts. Zones of low LWC/LWC max are found close to the cloud edges, where DSDs are highly diverse, containing both large and small droplets. Finally, we analyze the mixing diagrams. Significant in-phase turbulent fluctuations in LWC and N c were found. The effective radii change slightly across cloud updraft zones but decrease at the zone of low LWC/LWC max ratio close to cloud edges. The spectra of LWC and N c obey Kolmogorov -5/3 turbulence law. The radii of the correlation of LWC and N c in updraft zones are of several tens of meters. Filaments up to 120–175 m in size are also noticed.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1992

Performance of the Phase Doppler Particle Analyzer icing cloud droplet sizing probe in the NASA Lewis Icing Research Tunnel

The design, development, and testing of an icing cloud droplet sizing probe based upon the Phase Doppler Particle Analyzer (PDPA) are discussed. This probe is an in-situ laser interferometry based single particle measuring device capable of determining size distributions. The probe is designed for use in harsh environments such as icing tunnels and natural icing clouds. From the measured size distribution, Median Volume Diameter (MVD) and Liquid Water Content (LWC) may be determined. Both the theory of measurement and the mechanical aspects of the probe design and development are discussed. The MVD results from the probe are compared to an existing calibration based upon different instruments in a series of tests in the NASA Lewis Icing Research Tunnel. Agreement between the PDPA probe and the existing calibration is close for MVDs between 15 to 30 microns, but the PDPA results are considerably smaller for MVDs under 15 microns.

Rudoff, R. C.↗

NASA NTRS1972

Microwave radiometric measurements of atmospheric temperature and water from an aircraft.

A five-channel microwave spectrometer operating near the 1.35-cm wavelength water vapor and the 5-mm wavelength oxygen resonances was flown in the NASA Convair 990 aircraft at altitudes near 12 km and used to infer layer thicknesses and water vapor and liquid water abundances in the troposphere. The calibration of the spectrometer and a multiple regression method of interpretation of the data obtained from the flights are described. Possible errors from clouds and from the terrestrial surface are discussed. Values of atmospheric layer thicknesses, water vapor content, and liquid water content inferred from microwave data obtained over two frontal systems are presented. The inferred values of 1000- to 500-mb and 500- to 250-mb thicknesses agree with directly measured values to within 15 meters at the places where the direct measurements were made. This agreement is equivalent to errors of less than 1 K in mean temperature.

Rosenkranz, P. W.↗

NASA NTRS1949

Investigation of Meteorological Conditions Associated with Aircraft Icing in Layer-Type Clouds for 1947-48 Winter

Rotating-cylinder measurements of the icing conditions encountered in flight during the winter of 1947-48 are presented. Liquid water content, drop size, and temperature data are shown to be consistent with previously measured conditions and with proposed maximum icing conditions in supercooled layer-type clouds. Cumulative frequency graphs of meteorological parameters indicate the frequency with which various icing conditions have been encountered in the Great Lakes area and surrounding states.

WATER, SUPERCOOLED↗

NASA NTRS2007

Multi-Layer Arctic Mixed-Phase Clouds Simulated by a Cloud-Resolving Model: Comparison with ARM Observations and Sensitivity Experiments

A cloud-resolving model (CRM) is used to simulate the multiple-layer mixed-phase stratiform (MPS) clouds that occurred during a three-and-a-half day subperiod of the Department of Energy-Atmospheric Radiation Measurement Program s Mixed-Phase Arctic Cloud Experiment (M-PACE). The CRM is implemented with an advanced two-moment microphysics scheme, a state-of-the-art radiative transfer scheme, and a complicated third-order turbulence closure. Concurrent meteorological, aerosol, and ice nucleus measurements are used to initialize the CRM. The CRM is prescribed by time-varying large-scale advective tendencies of temperature and moisture and surface turbulent fluxes of sensible and latent heat. The CRM reproduces the occurrences of the single- and double-layer MPS clouds as revealed by the M-PACE observations. However, the simulated first cloud layer is lower and the second cloud layer thicker compared to observations. The magnitude of the simulated liquid water path agrees with that observed, but its temporal variation is more pronounced than that observed. As in an earlier study of single-layer cloud, the CRM also captures the major characteristics in the vertical distributions and temporal variations of liquid water content (LWC), total ice water content (IWC), droplet number concentration and ice crystal number concentration (nis) as suggested by the aircraft observations. However, the simulated mean values differ significantly from the observed. The magnitude of nis is especially underestimated by one order of magnitude. Sensitivity experiments suggest that the lower cloud layer is closely related to the surface fluxes of sensible and latent heat; the upper cloud layer is probably initialized by the large-scale advective cooling/moistening and maintained through the strong longwave (LW) radiative cooling near the cloud top which enhances the dynamical circulation; artificially turning off all ice-phase microphysical processes results in an increase in LWP by a factor of 3 due to interactions between the excessive LW radiative cooling and extra cloud water; heating caused by phase change of hydrometeors could affect the LWC and cloud top height by partially canceling out the LW radiative cooling. It is further shown that the resolved dynamical circulation appears to contribute more greatly to the evolution of the MPS cloud layers than the parameterized subgrid-scale circulation.

Luo, Yali↗

DOE OSTI2021

Ice and Supercooled Liquid Water Distributions over the Southern Ocean based on In Situ Observations and Climate Model Simulations

Three climate models are evaluated using in situ airborne observations from the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) campaign. The evaluation targets cloud phases, microphysical properties, thermodynamic conditions, and aerosol indirect effects from –40°C to 0°C. Compared with 580-s averaged observations (i.e., 100 km horizontal scale), the Community Atmosphere Model version 6 (CAM6) shows the most similar result for cloud phase frequency distribution and allows more liquid-containing clouds below –10°C compared with its predecessor—CAM5. The Energy Exascale Earth System Model (E3SM) underestimates (overestimates) ice phase frequencies below (above) –20°C. CAM6 and E3SM show liquid and ice water contents (i.e., LWC and IWC) similar to observations from –25°C to 0°C, but higher LWC and lower IWC than observations at lower temperatures. Simulated in-cloud RH shows higher minimum values than observations, possibly restricting ice growth during sedimentation. As number concentrations of aerosols larger than 500 nm (Na 500 ) increase, observations show increases of LWC, IWC, liquid, and ice number concentrations (N liq , N ice ). Number concentrations of aerosols larger than 100 nm (Na 100 ) only show positive correlations with LWC and N liq . From –20°C to 0°C, higher aerosol number concentrations are correlated with lower glaciation ratio and higher cloud fraction. From –40°C to –20°C, large aerosols show positive correlations with glaciation ratio. CAM6 shows small increases of LWC and N liq with Na 500 and Na 100 . E3SM shows small increases of N ice with Na 500 . Altogether, CAM6 and E3SM underestimate aerosol indirect effects on ice crystals and supercooled liquid droplets over the Southern Ocean.

54 ENVIRONMENTAL SCIENCES↗