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At least 253 records · Page 14

Acousto-Optical Imaging Spectropolarimeter

Imaging spectropolarimeter designed around acousto-optical tunable filter (AOTF) takes polarization-specific spectral images of solid surfaces, aerosols, and absorption and emission phenomena in gas phase, at wavelengths from 500 to 1,000 nm. Produces side-by-side spectral images in two mutually perpendicular polarizations, one corresponding to ordinary, other corresponding to extraordinary waves in acousto-optical material. Offers large aperture, high resolving power, and rapid tunability, with no moving parts.

Saif, Babak↗

The Cloud Slicing Technique-Measuring the Unmeasureable

In satellite remote sensing clouds are usually considered an annoying interference. Satellite investigators go to unusual lengths to try to avoid clouds or to correct for their effects, and satellite data users routinely exclude cloudy data from analysis. Yet it was shown about a decade ago using TOMS data that for the study of tropospheric constituents, such as ozone, clouds can play a very beneficial role by allowing one to measure what otherwise cannot be directly measured from space. We call this technique "cloud Slicing". The so-called Convective Cloud Differential (CCD) method is one particular application of cloud slicing that has been applied successfully to data from TOMS and other similar satellite instruments to study the behavior of tropical tropospheric ozone at variety of spatial and temporal scales. However, there has been considerable confusion in the literature as to what exactly one measures from reflected sunlight instruments such as TOMS in cloudy atmospheres. We will discuss recently completed analysis of data taken by the Ozone Monitoring Instrument (OMI) on the Aura satellite in conjunction with several other instruments on the A-train satellite constellation to present new insight on how clouds affect absorption by aerosols and trace gases at reflected wavelengths (UV-SWIR). We will show several examples to illustrate how this insight is helping us to study the behavior of trace gases and aerosols in the atmosphere that cannot be studied by focusing only on cloud-free scenes.

Bhartia, P.↗

Development of the Global Ozone Lidar Demonstrator (GOLD) Instrument for Deployment on the NASA Global Hawk

A compact ozone (O3) and aerosol lidar system is being developed for conducting global atmospheric investigations from the NASA Global Hawk Uninhabited Aerial Vehicle (UAV) and for enabling the development and test of a space-based O3 and aerosol lidar. GOLD incorporates advanced technologies and designs to produce a compact, autonomously operating O3 and aerosol Differential Absorption Lidar (DIAL) system for a UAV platform. The GOLD system leverages advanced Nd:YAG and optical parametric oscillator laser technologies and receiver optics, detectors, and electronics. Significant progress has been made toward the development of the GOLD system, and this paper describes the objectives of this program, basic design of the GOLD system, and results from initial ground-based atmospheric tests.

Hair, Jonathan W.↗

Agricultural Fires in the Southeastern U.S. During SEAC4RS: Emissions of Trace Gases and Particles and Evolution of Ozone, Reactive Nitrogen, and Organic Aerosol

Emissions from 15 agricultural fires in the southeastern U.S. were measured from the NASA DC-8 research aircraft during the summer 2013 Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) campaign. This study reports a detailed set of emission factors (EFs) for 25 trace gases and 6 fine particle species. The chemical evolution of the primary emissions in seven plumes was examined in detail for ~1.2 h. A Lagrangian plume cross-section model was used to simulate the evolution of ozone (O3), reactive nitrogen species, and organic aerosol (OA). Observed EFs are generally consistent with previous measurements of crop residue burning, but the fires studied here emitted high amounts of SO2 and fine particles, especially primary OA and chloride. Filter-based measurements of aerosol light absorption implied that brown carbon (BrC) was ubiquitous in the plumes. In aged plumes, rapid production of O3, peroxyacetyl nitrate (PAN), and nitrate was observed with (Delta)O3/(Delta)CO, (Delta)PAN/(Delta)NOy, and (Delta)nitrate/(Delta)NOy reaching approx. 0.1, approx. 0.3, and approx.0.3. For five selected cases, the model reasonably simulated O3 formation but underestimated PAN formation. No significant evolution of OA mass or BrC absorption was observed. However, a consistent increase in oxygen-to-carbon (O/C) ratios of OA indicated that OA oxidation in the agricultural fire plumes was much faster than in urban and forest fire plumes. Finally, total annual SO2, NOx, and CO emissions from agricultural fires in Arkansas, Louisiana, Mississippi, and Missouri were estimated (within a factor of approx. 2) to be equivalent to approx. 2% SO2 from coal combustion and approx. 1% NOx and approx. 9% CO from mobile sources.

OA mass or BrC absorption↗

Evaluation of the Land Surface Reflectance Fundamental Climate Data Record

The land surface reflectance is a fundamental climate data record at the basis of the derivation of other climate data records (Albedo, LAI/Fpar, Vegetation indices) and has been recognized as a key parameter in the understanding of the land-surface-climate processes. In this presentation, we present the validation of the Land surface reflectance used for MODIS, VIIRS, Landsat 8 and Sentinel 2 data. This methodology uses the 6SV Code and data from the AERONET network. The overall accuracy clearly reaches the satellite specifications. To understand how to improve the validation, we developed an exhaustive error budget. Results show an impact of the absorption of aerosol and of the fine mode volume concentration.

Atmospheric correction↗

Evaluation of Spectral Band Adjustment Factors for Cross-Calibration of Visible Imagers

The NASA CERES EBAF dataset provides TOA SW and LW fluxes for long-term monitoring of the Earth’s energy balance and to validate climate models. The EBAF products, based on the Terra, Aqua, and NOAA20 CERES instrument observed radiances, rely on coincident measurements from the onboard MODIS or VIIRS imagers to determine cloud properties used for angular distribution model scene selection, which is required to convert the CERES observed radiances into flux values. Furthermore, CERES utilizes geostationary imager (GEO) hourly fluxes and clouds to infer the regional averaged daily flux in the SYN1deg product. A seamless transition of fluxes and clouds can only occur if the analogous MODIS, VIIRS, and GEO channels are properly inter-calibrated. The analogous band SRFs differ noticeably and require scene dependent spectral band adjustment factors (SBAF) for proper radiometric scaling between them. Given their disparate but overlapping SRFs, the coincident VIIRS I1 and M5 band TOA reflectance measurements provide the optimal opportunity to validate SBAFs over many surface and cloud conditions. The CERES project maintains SCIAMACHY, GOME-2, and Hyperion scene-stratified hyper-spectral reflectance measurements that can be convolved with sensor pair SRFs to compute the corresponding SBAF. This study highlights the SCIAMACHY, GOME-2, and Hyperion based SBAFs for different MODIS, VIIRS, and GEO inter-calibration targets, including all-sky tropical ocean (ATO), Libya-4, Dome-C, and deep convective clouds. To mitigate the observed sensor radiance fluctuations due to atmospheric absorption and aerosol variations, the Earth target observed radiances are correlated with multiple atmospheric parameters, such as precipitable water and ozone. The remaining M5 and I1 mean spectral band radiance difference should be resolved by the SBAF correction. The formulation of hyper-spectral sensor based SBAFs and validation methods can be verified in future utilizing high-accuracy, SI-traceable hyper-spectral measurements from CLARREO Pathfinder.

David R Doelling↗

Local and Regional Diurnal Variability of Aerosol Properties Retrieved by DSCOVR/EPIC UV Algorithm

The diurnal variability of aerosol optical depth retrieved from L1 point satellite radiance measurements closely matches surface observations. Seasonal variability of retrieved single scattering albedo is in good qualitative agreement with equivalent ground-based observations. EPIC aerosol products can be used in the qualitative and quantitative monitoring of extraordinary aerosol events resulting from wildfires and desert dust storms.

Aerosols, Absorption, Satellite retrieval↗

Ultraviolet DIAL measurements of O3 profiles in regions of spatially inhomogeneous aerosols

The differential absorption lidar (DIAL) technique generally assumes that atmospheric optical scattering is the same at the two laser wavelengths used in the DIAL measurement of a gas concentration profile. Erros can arise in this approach when the wavelengths are significantly separated, and there is a range dependence in the aerosol scattering distribution. This paper discusses the errors introduced by large DIAL wavelength separations and spatial inhomogeneity of aerosols in the atmosphere. A Bernoulli solution for determining the relative distribution of aerosol backscattering in the UV region is presented, and scattering ratio boundary values for these solutions are discussed. The results of this approach are used to derive a backscatter correction to the standard DIAL analysis method. It is shown that for the worst cases of severe range dependence in aerosol backscattering, the residual errors in the corrected DIAL O3 measurements were less than 10 ppbv for DIAL wavelengths at 286 and 300 nm.

Browell, E. V.↗

Identification of Absorbing Aerosol Types at a Site in the Northern Edge of Indo-Gangetic Plain and a Polluted Valley in the Foothills of the Central Himalayas

Identification of atmospheric aerosol types and characterization of absorbing aerosols, based on AErosol RObotic NETwork (AERONET) data collected during 2013–2014 over two sites in Nepal: Lumbini in the northernmost part of central Indo-Gangetic Plain (IGP) and Kathmandu Valley in foothills of the central Himalayas, have been conducted in the present study. The relationship between four aerosol parameters; Extinction Angstrom Exponent (EAE), Absorption Angstrom Exponent (AAE), Single Scattering Albedo (SSA) and Real Refractive Index (RRI) was analyzed to study the aerosol types. This resulted in the identification of two types of aerosols concerning their origin: biomass burning and urban/industrial mix. Furthermore, to understand the absorbing aerosol types, the relationship between aerosol size parameters; Fine Mode Fraction (FMF) and Angstrom Exponent (AE), and aerosol absorption characteristics; SSA and AAE were investigated. In regards to the absorbing aerosol types, ‘Mostly BC’ was the dominant absorbing aerosol, over both sites, with comparatively negligible contribution from other absorbing aerosol types such as dust. The aerosol subtypes obtained from satellite-borne CALIPSO instrument supported the results derived from the AERONET data. The CALIPSO images also indicated that the aerosols over the foothills of the Himalayas could extend to the height of >5 km above the ground, which could be transported towards the Himalayan and Tibetan Plateau (HTP) region with sensitive ecosystems. The multi-sites based study of long-term records is required to elucidate the nature and trends of aerosols in the HTP region and any perturbation to the atmospheric environment and other environments in this region.

Aerosol types↗

Atmospheric processing and aerosol aging responsible for observed increase in absorptivity of long-range-transported smoke over the southeast Atlantic

Biomass burning aerosol (BBA) from agricultural fires in southern Africa contributes about one-third of the global carbonaceous aerosol load. These particles have strong radiative effects in the southeast Atlantic (SEA), which depend in part on the radiative contrast between the aerosol layer in the free troposphere (FT) and the underlying cloud layer. However, there is large disagreement in model estimates of aerosol-driven climate forcing due to uncertainties in the vertical distribution, optical properties, and life cycle of these particles. This study applies a novel method combining remote sensing observations with regional model outputs to investigate the aging of the BBA and its impact on the optical properties during transatlantic transport from emission sources in Africa to the SEA. Results show distinct variations in extinction Ångström exponent (EAE) and single-scattering albedo (SSA) as aerosols age. Near the source, fresh aerosols are characterized by low mean SSA (0.84) and high EAE (1.85), indicating smaller, highly absorbing particles. By isolating marine contributions from the total column during BBA transport across the SEA, our analysis reveals an initial decrease in BBA absorptivity, with mean FT SSA of 0.87 after 6–7 d, followed by increased absorptivity with mean FT SSA of 0.84 after 10 d, suggesting enhanced absorption due to chemical aging. These findings indicate that BBA becomes more absorbing during extended transport across the SEA, with implications for reducing model uncertainties. Our remote-sensing-based results agree well with previous in situ studies and offer new insights into aerosol–radiation interactions and the energy balance over the SEA.

54 ENVIRONMENTAL SCIENCES↗

Effect of Tropospheric Aerosols in Satellite-Based Trace Gas Retrieval

Scattering and absorption by tropospheric aerosol particles have an effect on the airmass factor (AMF), a fundamental quantity for trace gas concentration retrieval by inversion of satellite measurements. The interference effect depends on the aerosols micro-physical and optical properties as well as the relative distribution of the tropospheric trace gas and aerosol load. Quantifying the aerosol impact on trace gas retrieval requires a sensitivity study using radiative transfer calculations. In this presentation we will describe a recently initiated effort to characterize the aerosol-related error in trace gas retrievals when the presence of aerosol particles is not accounted in the inversion procedure. A general description of the project will be presented and preliminary results on aerosol effects on SO2 retrieved concentrations will be discussed.

Krotkov, Nickolay↗

Calculations of Aerosol Radiative Forcing in the SAFARI Region from MODIS Data

SAFARI 2000 provided the opportunity to validate MODIS aerosol retrievals and to correct any assumptions in the retrieval process. By comparing MODIS retrievals with ground-based sunphotometer data, we quantified the degree to which the MODIS algorithm underestimated the aerosol optical thickness. This discrepancy was attributed to underestimating the degree of light absorption by the southern African smoke aerosol. Correcting for this underestimation of absorption, produces more realistic aerosol retrievals that allow various applications of the MODIS aerosol products. One such application is the calculation of the aerosol radiative forcing at the top and bottom of the atmosphere. The combination of MODIS accuracy, coverage, resolution and the ability to separate fine and coarse mode make this calculation substantially advanced over previous attempts with other satellites. We focus on the oceans adjacent to southern Africa and use a solar radiative transfer model to perform the flux calculations. The forcing at the top of atmosphere is calculated to be 10 W/sq m, while the forcing at the surface is -26 W/sq m. These results resemble those calculated from INDOEX data, and are most sensitive to assumptions of aerosol absorption, the same parameter that initially interfered with our retrievals.

Remer, L. A.↗

Realistic operation of two residential cordwood-fired outdoor hydronic heater appliances—Part 3: Optical properties of black and brown carbon emissions

Residential biomass combustion is a source of carbonaceous aerosol. Inefficient combustion, particularly of solid fuels produces large quantities of black and brown carbon (BC and BrC). These particle types are important as they have noted effects on climate forcing and human health. One method of measuring these quantities is by measurement of aerosol light-absorption and scattering, which can be performed using an aethalometer and nephelometer, respectively. These instruments are widely deployed in the study of ambient air and are frequently used in air quality modeling and source apportionment studies. In this study, we will describe (1) a method for measuring primary BC and BrC emissions from two residential log-fired wood hydronic heaters and (2) the BC and BrC emission from these devices over a wide range of operating conditions, such as cold-starts, warm-starts, four different levels of output ranging from 15% to 100% maximum rated output, and periods of repeated cycling. The range in flue-gas BC concentrations, measured using an aethalometer at the 880 nanometer (nm) wavelength, were between 5.09 × 10 2 and 2.24 × 10 4 micrograms per cubic meter (µg/m 3 ) while the scattering coefficient of the flue-gas, measured by a nephelometer at 880 nm, ranged between 2.20 × 10 3 and 8.56 × 10 5 inverse megameters (Mm –1 ). The BrC concentrations, measured using the 370 nm wavelength of an aethalometer, were between 9.10 × 10 1 and 3.56 × 10 4 µg/m 3 . The calculated Angstrom Absorption Exponent (AAE) of the flue-gas aerosol ranged between 1.54 and 3.63. Performing a comparison between the measured BC concentration and an external particulate matter (PM) concentration showed that overall BC makes up roughly a quarter of the PM emitted by either of the two appliances. Further for both appliances, the cold-start and the test phase immediately following it had the highest BC and BrC concentrations, the highest measured scattering coefficient, as well as a low AAE.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗

Detecting Layer Height of Smoke and Dust Aerosols Over Vegetated Land and Water Surfaces Via Oxygen Absorption Bands

We present an algorithm for retrieving aerosol layer height (ALH) and aerosol optical depth (AOD) for smoke and dust over vegetated land and water surfaces from measurements of the Earth Polychromatic Imaging Camera (EPIC) onboard the Deep Space Climate Observatory (DSCOVR). Our algorithm uses EPIC atmospheric window bands to determine AOD and then takes advantage of oxygen A and B bands to derive ALH. We applied this algorithm on several dust and smoke events. Validation shows our results are of high accuracy.

Jing Zeng↗

Direct Radiative Effects of Aerosols Over South Asia From Observations and Modeling

Quantitative assessment of the seasonal variations in the direct radiative effect (DRE) of composite aerosols as well as the constituent species over the Indian sub continent has been carried out using a synergy of observations from a dense network of ground based aerosol observatories and modeling based on chemical transport model simulations. Seasonal variation of aerosol constituents depict significant influence of anthropogenic aerosol sources in winter and the dominance of natural sources in spring, even though the aerosol optical depth doesn't change significantly between these two seasons. A significant increase in the surface cooling and atmospheric warming has been observed as season changes from winter DRE(sub SUR) = −28 +/- 12 W m(exp −2) and DRE(sub ATM) = +19.6 +/- 9 W m(exp −2) to spring DRE(sub SUR) = −33.7 +/- 12 W m(exp −2) and DRE(sub ATM) = +27 +/- 9 W m(exp−2). Interestingly, springtime aerosols are more absorptive in nature compared to winter and consequently the aerosol induced diabatic heating of the atmosphere goes as high as approximately 1 K day(exp -1) during spring, especially over eastern India. The atmospheric DRE due to dust aerosols (+14 +/- 7 W m(exp 2) during spring overwhelms that of black carbon DRE (+11.8 +/- 6 W m(exp -2) during winter. The DRE at the top of the atmosphere is mostly governed by the anthropogenic aerosols during all the seasons. The columnar aerosol loading, its anthropogenic fraction and radiative effects shows a steady increase with latitude across Indian mainland leading to a larger aerosol-induced atmospheric warming during spring than in winter.

dust aerosols↗

Algorithm for Atmospheric Corrections of Aircraft and Satellite Imagery

A simple and fast atmospheric correction algorithm is described which is used to correct radiances of scattered sunlight measured by aircraft and/or satellite above a uniform surface. The atmospheric effect, the basic equations, a description of the computational procedure, and a sensitivity study are discussed. The program is designed to take the measured radiances, view and illumination directions, and the aerosol and gaseous absorption optical thickness to compute the radiance just above the surface, the irradiance on the surface, and surface reflectance. Alternatively, the program will compute the upward radiance at a specific altitude for a given surface reflectance, view and illumination directions, and aerosol and gaseous absorption optical thickness. The algorithm can be applied for any view and illumination directions and any wavelength in the range 0.48 micron to 2.2 micron. The relation between the measured radiance and surface reflectance, which is expressed as a function of atmospheric properties and measurement geometry, is computed using a radiative transfer routine. The results of the computations are presented in a table which forms the basis of the correction algorithm. The algorithm can be used for atmospheric corrections in the presence of a rural aerosol. The sensitivity of the derived surface reflectance to uncertainties in the model and input data is discussed.

Fraser, Robert S.↗