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This presentation covers design, execution, and early results for the EUCLID experiment. Unresolved compensating errors for Pu-239 and the Joint uncertainty problems are discussed. Various tools and design implementations are discussed along with upcoming work. Additional slides compare EUCLID calculations to experiment for several nuclear data libraries. ENDF/B-VIII.1β2 is named e81b2.
A new set of critical experiments exploring the temperature-dependence of the reactivity in a critical assembly is described. In the experiments, the temperature of the critical assembly will be varied to determine the temperature that produces the highest reactivity in the assembly. This temperature is the inversion point of the isothermal reactivity coefficient of the assembly. An analysis of relevant configurations is presented. Existing measurements are described and an analysis of these experiments presented. The overall experimental approach is described as are the modifications to the critical assembly needed to perform the experiments.
Unconstrained physics spaces between two or more nuclear data observables in a library occur when their values can be simultaneously adjusted without violating the uncertainties in either differential information or simulations of relevant integral experiments. Differential data are often too imprecise to fully bound all nuclear data observables of interest for application simulations. Integral data are simulated with combinations of nuclear data so that an error in one observable may be hidden by a counterbalancing error in another. In this manner compensating errors may lurk within nuclear data libraries and these errors have the potential to undermine the predictive power of neutron transport simulations, particularly in situations where there is no conclusive validation experiment that resembles the application of interest. The EUCLID project (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) developed a preliminary workflow to identify these unconstrained physics spaces by bringing together results from a large collection of integral experiments with their simulated counter-parts as well as differential information that have a one-to-one correspondence to nuclear data. This wealth of information is processed by machine learning tools for subsequent refinement by human experts. Here, we show how the EUCLID work-flow is executed by applying it first to 239 Pu and then to 9 Be nuclear data in ENDF/B-VIII.0.
Nuclear criticality safety is an extremely important part of the work at Los Alamos National Laboratory (LANL). As part of the work LANL performs to continue to keep criticality safety a top priority, LANL has developed and regularly teaches nuclear criticality safety training classes for both the United States Department of Energy Nuclear Criticality Safety Program as well as internal trainings for LANL employees. A portion of the training classes is comprised of hands-on demonstrations, where students get the opportunity to handle special nuclear material at the National Criticality Experiments Research Center (NCERC). One hands-on demonstration uses the “Class foils,” thin HEU foils which are stacked with lucite moderator plates. A hand-stack is performed until the multiplication reaches the “three-quarters rule,” where the demonstration is continued remotely on a vertical lift assembly up until the system is critical. This hands-on demonstration eventually achieves a critical configuration and follows the ANS-1 guidelines on an approach to critical. Another hands-on demonstration involves handling clad plutonium and neptunium spheres, and follows procedures using criticality safety evaluations to ensure that the hands-on demonstrations remain subcritical.This hands-on demonstration also involves the use of polyethylene shells around the plutonium sphere to demonstrate how additional reflector increases the criticality of a system. This paper is focused on developing a new hands-on demonstration using Zero Power Physics Reactor (ZPPR) plates. This new hands-on demonstration will follow the ANS-8 standards as it is not desired to achieve criticality with the ZPPR plates during the hands-on demonstration. A hands-on demonstration using multiple plutonium parts will likely be more applicable to personnel who handle plutonium on a daily basis, such as LANL glovebox operators.
Computational modeling programs are invaluable tools that allow us to understand systems, safely develop new processes, and make reliable predictions about future designs. However, the effectiveness of these codes is limited by the degree to which their parameters match the real world. In the field of nuclear engineering, cross section data is one of these vital parameters. Accurate cross section data on important fissile and fissionable isotopes promotes the design of safer and more efficient fabrication, transportation, storage, and stockpiling of nuclear fuel. Unfortunately, there are knowledge gaps in data on key isotopes. In 2011, a multinational meeting hosted by the US Department of Energy Nuclear Criticality Safety Program ranked the priority of certain cross section data needs. In response, Lawrence Livermore National Lab (LLNL) designed the Thermal and Epithermal eXperiment (TEX) series of benchmark experiments. Benchmark experiments are used to validate current cross section data. They validate data by comparing the results of an actual experiment to the predicted results from a computational model. The data a benchmark applies to depends on the isotope and energy range the experiment’s neutron multiplication factor ( k eff ) is most sensitive to. The development and testing of the TEX High 240 Plutonium Benchmark will help validate 240 Pu cross section data. The configuration and materials of this benchmark are designed to be most sensitive to 240 Pu's intermediate energy range (from 0.625 ev to 100 keV ). MCNP® models of the assembly have been developed by LLNL and the results have been written in the final design report. In order for the discrepancies between benchmark models and experiments to be attributed to cross section inaccuracies, the accuracy of the models needs to be verified. The goal of this project is to verify of the results of LLNL's modeling by creating a new set of MCNP models and comparing the results.
Since 1945, Los Alamos National Laboratory (LANL) has performed critical experiments, primarily at the Los Alamos Critical Experiments Facility (LACEF) at Technical Area 18 (TA-18). Since 2011, these experiments have been conducted by the National Criticality Experiments Research Center (NCERC), operated by LANL, at the Device Assembly Facility (DAF) in the Nevada National Security Site (NNSS). These experiments utilize various types of Special Nuclear Material (SNM). Some of these experiments utilize what is referred to as the Rocky Flat Shells, which are called such as they came from the Rocky Flats Plant. These concentric hemi-shells are made of Highly Enriched Uranium (HEU), which is 93 w/o 235U. Fig. 1. Subset of the Rocky Flat Shells LANL is designing a new subcritical hands-on experiment with the goal of achieving a neutron multiplication in the range of 50 to 200, which correlates to Keff values of 0.98 to 0.995. ANSI/ANS-1 is the standard for Conduct of Critical Experiments which governs critical operations at NCERC. Section 3.9 of ANSI/ANS-1 states that when manipulating a critical assembly by hand, the predicted k eff of a known configuration should not exceed 0.95 (a neutron multiplication of 20). This presents a challenge, as this system would have a higher multiplication than 20 and the assembly would have to remain subcritical in normal and credible accident scenarios. To ensure the safety of such an assembly, the different normal and abnormal conditions that could alter the criticality 1 MCNP® and Monte Carlo N-Particle® are registered trademarks owned by Triad National Security, LLC, manager and operator of Los Alamos National Laboratory. Any third party use of such registered marks should be properly of the system must be considered and analyzed. If such a condition is deemed to be credible, it will be further investigated using the Monte Carlo N-Particle (MCNP) transport code. If the results of these simulations show that a k eff larger than one could be possible, modifications to the assembly will be made until such an event is deemed no longer possible.
The Neptunium Subcritical Observation (NeSO) experiment was a subcritical integral benchmark experiment. This experiment was designed in 2017-2018 and was performed at the National Criticality Experiments Research Center (NCERC) in 2019. Eight different subcritical configurations were measured with varying Nickel reflector thickness. For all configurations, a 3 He detection system was used to record neutron events. The focus of this work is to share neutron noise results of the measured data.
The HEU Jemima plates have been utilized in numerous International Criticality Safety Benchmark Evaluation Project (ICSBEP) evaluations. ICSBEP evaluations are a vital com ponent of nuclear data validation for applications across the nuclear community. In the past, different combinations of mass, caliper measurements, and drawing dimensions have been used to define the HEU Jemima plates in ICSBEP evaluations. Some of these combinations result in large density ranges (17 g/cm 3 to 19 g/cm 3 ) or unrealistic densities (greater than 19 g/cm 3 ). Additionally, oxidation of the plates has led to questioning the flatness of each plate, which can add additional gaps in experiment configurations. This work proposes a standardized method of defining the commonly used HEU Jemima plates across different experiments.
This report documents the experimental configurations and measurements for IER-518: Joint LLNL, LANL, SNL, and IRSN High Multiplication Subcritical (Multiplicity) Benchmark Experiments. These measurements involved a series of subcritical configurations at the Sandia Critical Experiments (SCX) facility at Sandia National Laboratories (SNL). The purpose of these measurements was to produce time tagged neutron count data of configurations that exceed a subcritical multiplication of 20, which is the high end of the fundamental physics benchmarks currently available in the International Criticality Safety Benchmark Evaluation Project Handbook (ICSBEP). These measurements leverage experimental configurations 1 and detector systems 2 from previously accepted ICSBEP benchmark evaluations, allowing evaluations of these measurements to be performed at greatly reduced cost.
This report incorporates our work carried out during our 5-month internship at LANL under an internship agreement with EAMEA (École des Applications Militaires de l’Énergie Atomique). After outlining the context in which we worked, we present our work as aid to modeling and predicting the neutronic behavior of nuclear systems, with a view to carrying out criticality experiments qualifying the MCNP code as part of innovative projects. Fourth generation reactors will enable to tackle a lot of issues such as environmental crisis, affordable energy access, and nuclear waste management. They seem to be one of the keys for a sustainable future. Most of the projects that emerge nowadays include the use of HALEU (high assay low enriched uranium) or MOX recycled fuels. Our projects are part of this dynamic and addresses concrete scientific research issues in the nuclear field. Studies of HALEU package are essential to anticipate the need, therefore the Optimus L (OPTImal Modular Universal Shipping cask technology) designed by NAC (Nuclear Assurance Corporation) international but filled with 20 % enriched uranium dioxide (UO 2 ) will be studied to support safe transportation. However, it seems there is no benchmark with a high correlation with the combination of this fuel and this package to validate MCNP simulations. As such, the study will focus on the development of new criticality safety benchmarks for this case. On the other hand, there is a great need for critical benchmarks in the intermediate energy range with MOX fuel. An IER (Integral Experiment Request) has then be requested to answer it through a partnership between French institution IRSN and U.S. Department of Energy's Nuclear Criticality Safety Program (NCSP). This experience planned for 2025 requires to gather calculated data through a MCNP model to be realized safely. Finally, a presentation of our one-week experience at the DAF as part of our discovery of criticality experiments will be introduced in Appendix 1: Week at the DAF (Device Assembly Facility)
The Chlorine Worth Studies (CWS) experiments with polyvinyl chloride (PVC with chemical formula (C 2 H 3 Cl) n ), chlorinated polyvinyl chloride (CPVC with chemical formula (C 9 H 11 Cl 7 ) n ), and high density polyethylene (HDPE with chemical formula (CH 2 ) n ) were a series of measurements performed at the National Criticality Experiments Research Center (NCERC). The purpose of the CWS experiments was to perform integral experiments that were highly sensitive to the thermal 35 Cl(n,γ) reaction and matched the sensitivities of aqueous chloride operations at the plutonium facility at Los Alamos National Laboratory (LANL). The CWS experiments were performed on the Planet critical assembly machine at NCERC and utilized weapons grade plutonium (WGPu) plates as fuel. The design process and design of the CWS experiment were discussed previously. This paper discusses the benchmark evaluation of the experiment, intended for the International Criticality Safety Benchmark Evaluation Project (ICSBEP). Criticality calculations were performed with MCNP version 6.3. Results presented here are preliminary, as the benchmark has not yet been submitted to the ICSBEP.
This presentation discusses the benchmark of the IER 498: Godiva-IV criticality accident alarm system (CAAS). It details the goal of the project which is to create a CAAS benchmark capability for Godiva-IV in order to create a shielding benchmark for NCSP software and data, to add geometrically diverse benchmark/benchmarks to the ICSBEP Handbook, to enable more precise measurements at NCERC, and to help assure CAAS performance is as-stated. It also states that work was completed on CED-1 in 2019 and that future work includes the completion of CED-2 in 2020.
A lack of intermediate molybdenum benchmarks in the ICSBEP has been identified by LANL, Y-12, and IRSN. This lacking adversely effects criticality safety operations and leaves new differential molybdenum data unvalidated. NCERC is proposing a series of intermediate integral experiments to better the understanding of molybdenum systems. Using MCNP6.2 with the ENDF/B-VIII.0 nuclear data library a single unmoderated and four moderated system designs were identified using a sensitivity optimization method. Each proposed system was found to be at least twice as sensitive to the 95 Mo capture cross section in the URR as the sole existing intermediate molybdenum benchmark in the ISCBEP handbook. The addition of a new molybdenum sensitive intermediate system would improve future nuclear data evaluations.
Two critical experiments with HEU-Lucite were performed using the Planet Universal Critical Assembly Machine at Los Alamos National Laboratory in 2019. HEU foils were interleaved with Lucite in a column stack for moderation and reflection from the square Lucite plates. The evaluation of the experiments is presented. A Monte-Carlo (MCNP6) calculation model was developed for the determination of uncertainties and their effect on the multiplication factor. Experimental uncertainties were found to be low with the overall uncertainty in k eff approximately 240 pcm. The comparison of calculations with experimental data is presented.
The International Criticality Safety Benchmark Evaluation Project (ICSBEP) has continued its work generating evaluations of new and historical criticality benchmark experiments since the last update to the nuclear criticality safety community at the 11th International Conference on Nuclear Criticality Safety (ICNC 2019) in Paris, France. Three additional versions of the ICSBEP Handbook have been published since that update, and the Technical Review Group (TRG) held two in-person (in 2019 and 2023) and three virtual (2020 and 2021) meetings to review and approve additional benchmarks. The 2019 edition of the ICSBEP Handbook included five new evaluations with 79 new configurations, the 2020 version of the ICSBEP Handbook contained five new evaluations totaling 76 new configurations, and the 2021 version of the ICSBEP handbook contained five new evaluations with a total of 57 different configurations. The ICSBEP TRG met in October and December 2021, to review benchmarks for potential inclusion in the 2022 ICSBEP Handbook, with seven evaluations receiving provisional approval pending resolution of review group comments. Final comment resolution for some of these evaluations is currently underway and handbook publication should be completed soon. The ICSBEP TRG met again in person in April 2023 to review benchmarks for the 2023 ICSBEP Handbook, provisionally approving 7 new evaluations. The ICSBEP continues to deliver high-quality, peer reviewed evaluations of experiments relevant to the nuclear criticality safety community.
The US Department of Energy Nuclear Criticality Safety Program (NCSP) convened a multinational Thermal Epithermal eXperiments (TEX) meeting in July of 2011 to discuss the data and experimental needs of criticality safety practitioners. The number one and two priority integral experiment data needs were for 239 Pu and 240 Pu, with special emphasis on cross section performance in the intermediate energy range (from 0.625 eV to 100 keV). LLNL measured five critical configurations with LANL for the plutonium test bed (IER-184) and published the experiments as International Criticality Safety Benchmark Evaluation Project evaluation PUMET-MIXED-002. Modeling of the benchmark configurations using ENDF/B-VIII.0 nuclear data showed significant overprediction of reactivity for configurations that had a large percentage of fissions in the intermediate energy regime. This report documents a variation on the TEX plutonium test bed to provide a test of 240 Pu cross sections, with sensitivity of the configuration to 240 Pu radiative capture and fission cross sections a priority for the design.
Resolved resonance region evaluations of the major isotopes of natural lead, 206 Pb, 207 Pb, 208 Pb, have been per formed to support the development of Generation IV reactors. In this study, validation of nuclear data for lead fast reactors was performed with simulations of shielding benchmarks, integral critical benchmarks, and quasi-differential scattering measurements. Sensitivity analyses of these systems showed that elastic scattering reactions above 100 keV were the dominant reactions driving system performance. The resolved resonance regions (RRRs) of the lead isotopes extend past 100 keV, making the RRR an ideal starting point to evaluate lead cross sections. Since the R-matrix requires knowledge of bound, distant, and observed resonances, it was necessary to evaluate from 10 -5 eV up to the respective limit of the RRR. The 208 Pb RRR evaluation was extended to 1.5 MeV in order to obtain resonance parameters used to calculate new elastic scattering angular distributions up to 1.5 MeV. Resonance parameter uncertainties and covariance were generated using the R-matrix code SAMMY. The new RRR parameters show a direct improvement to the scattering kernel below 1.5 MeV which in turn greatly improves fast critical experiments over ENDF/B-VIII.0.
Neutron multiplicity counting (NMC) is a technique for the assay of fissile material. In this work, three detection systems are utilized for active interrogation assay of shells of the Rocky Flats shells (highly enriched uranium, 93% 235U) stacked from 13.25-54.92 kg assemblies. The singles ($R_1$) and doubles ($R_2$) rates are calculated with each system to estimate two sample parameters: $M_L$- the leakage multiplication and F - the sample fission rate. The estimated mass, m, is found by dividing F by a constant activity per unit mass. Since we are interrogating HEU, the α ratio of (α; n) to fission neutrons is taken to be zero. The system of equations to calculate these quantities was originally derived. The Neutron Multiplicity 3 He Array Detector (NOMAD) consists of 15 3 He tubes inside polyethylene and is the traditional, capture-based detection system for NMC. The polyethylene moderates incoming neutrons for thermal capture in individual tubes. The low gamma background, discrete capture signals, and high efficiency of the NOMAD are beneficial for NMC. However, the time to slow down neutrons to thermal energies leads to a system die away time on the scale of microseconds. Comparatively, the Rossi-alpha Measurements – Rapid Organic (n, γ) Discrimination Detector (RAMRODD) and the Organic Scintillator Array (OSCAR) are scatter-based detection systems. RAMRODD consists of 8, 5.08 by 5.08 cm EJ-309 liquid scintillators in 4 pairs, evenly-spaced with 90 degrees separation about the center of each assembly. OSCAR consists of a single array of 12, 5.08 by 5.08 cm trans-stilbene crystals aligned with the center of the assembly. Scatter-based systems detect fast neutrons without any moderation, leading to system die away times on the scale of tens of nanoseconds. This allows much shorter timing gate widths compared to thermal systems, thus increasing counting statistics of true correlated fission events. However, scatter-based systems are susceptible to neutron cross-talk when an incident neutron scatters off one detector and interacts in an adjacent detector, causing two seemingly correlated detection signals. The equations developed adjust for cross-talk to conduct NMC with scatter-based systems.