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At least 253 records · Page 14

Magnetic field generation in core-sheath jets via the kinetic Kelvin-Helmholtz instability

We have investigated magnetic field generation in velocity shears via the kinetic Kelvin-Helmholtz instability (kKHI) using a relativistic plasma jet core and stationary plasma sheath. Our three-dimensional particle-in-cell simulations consider plasma jet cores with Lorentz factors of 1.5, 5, and 15 for both electron-proton and electron-positron plasmas. For electron-proton plasmas, we find generation of strong large-scale DC currents and magnetic fields that extend over the entire shear surface and reach thicknesses of a few tens of electron skin depths. For electron-positron plasmas, we find generation of alternating currents and magnetic fields. Jet and sheath plasmas are accelerated across the shear surface in the strong magnetic fields generated by the kKHI. The mixing of jet and sheath plasmas generates a transverse structure similar to that produced by the Weibel instability.

79 ASTRONOMY AND ASTROPHYSICS↗

Atomic site sensitivity of the energy loss magnetic chiral dichroic spectra of complex oxides

The quantitative analysis of magnetic oxide core level spectra can become complicated when the magnetic atoms are located at several nonequivalent atomic sites in the crystal. This is, for instance, the case for Fe atoms in magnetite, which are located in tetrahedral and octahedral atomic sites; in this case, the x-ray magnetic circular dichroic (XMCD) spectra recorded at the L{sub 2,3} edge of Fe contain contributions from the different nonequivalent atomic sites, which unfortunately cannot be separated. Energy loss magnetic chiral dichroic (EMCD) spectra are the transmission electron microscope analogies of the XMCD spectra. One of the important differences between these two techniques of magnetic analysis is that EMCD uses a fast electron beam instead of polarized light. The fast electrons behave like Bloch states in the sample, and the fine structure of the EMCD spectra is strongly influenced by channeling and dynamical diffraction effects. These effects can be adjusted by changing the experimental configuration. We use theoretical calculations, which include dynamical diffraction effects and in which electronic transitions are treated in the atomic multiplet formalism, to show that the relative weight of the Fe atoms in different nonequivalent atomic sites can be changed by a proper choice of the position of the detector and of the magnetite sample orientation and thickness. We conclude that EMCD spectra could be used to isolate the magnetic contribution of atoms in each of the nonequivalent atomic sites, which would not be possible with XMCD techniques.

36 MATERIALS SCIENCE↗

DERIVATION OF THE MAGNETIC FIELD IN A CORONAL MASS EJECTION CORE VIA MULTI-FREQUENCY RADIO IMAGING

The magnetic field within the core of a coronal mass ejection (CME) on 2010 August 14 is derived from analysis of multi-wavelength radio imaging data. This CME's core was found to be the source of a moving type IV radio burst, whose emission is here determined to arise from the gyrosynchrotron process. The CME core's true trajectory, electron density, and line-of-sight depth are derived from stereoscopic observations, constraining these parameters in the radio emission models. We find that the CME carries a substantial amount of mildly relativistic electrons (E < 100 keV) in a strong magnetic field (B < 15 G), and that the spectra at lower heights are preferentially suppressed at lower frequencies through absorption from thermal electrons. We discuss the results in light of previous moving type IV burst studies, and outline a plan for the eventual use of radio methods for CME magnetic field diagnostics.

79 ASTRONOMY AND ASTROPHYSICS↗

Unusual high B{sub s} for Fe-based amorphous powders produced by a gas-atomization technique

Fe-based alloy powders with a high Fe content of about 81 at.% were produced by a gas-atomization technique. Powders of Fe{sub 81}Si{sub 1.9}B{sub 5.7}P{sub 11.4} (at.%) alloy showed a good glass forming ability and exhibited unusual high saturation magnetic flux density of 1.57 T. The core-loss property at a frequency of 100 kHz for the compacted core made of the Fe{sub 81}Si{sub 1.9}B{sub 5.7}P{sub 11.4} powder is evaluated to be less than 500 kW/m{sup 3} under a maximum induction of 100 mT. Moreover, good DC-superposition characteristic of the core was also confirmed. These results suggest that the present Fe-based alloy powder is promising for low-loss magnetic-core materials and expected to contribute in miniaturization of electric parts in the near future.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Ion irradiation of Fe-Fe oxide core-shell nanocluster films: Effect of interface on stability of magnetic properties

A cluster deposition method was used to produce films of loosely aggregated nanoclusters (NCs) of Fe core-Fe{sub 3}O{sub 4} shell or fully oxidized Fe{sub 3}O{sub 4}. Films of these NC on Si(100) or MgO(100)/Fe{sub 3}O{sub 4}(100) were irradiated to 10{sup 16} Si{sup 2+}/cm{sup 2} near room temperature using an ion accelerator. Ion irradiation creates structural change in the NC film with corresponding chemical and magnetic changes which depend on the initial oxidation state of the cluster. Films were characterized using magnetometry (hysteresis, first order reversal curves), microscopy (transmission electron, helium ion), and x-ray diffraction. In all cases, the particle sizes increased due to ion irradiation, and when a core of Fe is present, irradiation reduces the oxide shells to lower valent Fe species. These results show that ion irradiated behavior of the NC films depends strongly on the initial nanostructure and chemistry, but in general saturation magnetization decreases slightly.

36 MATERIALS SCIENCE↗

Magnetic Interactions in Substitutional Core-Doped Graphene Nanoribbons

The design of a spin imbalance within the crystallographic unit cell of bottom-up engineered 1D graphene nanoribbons (GNRs) gives rise to nonzero magnetic moments within each cell. Here, we demonstrate the bottom-up assembly and spectroscopic characterization of a one-dimensional Kondo spin chain formed by a chevron-type GNR (cGNR) physisorbed on Au(111). Substitutional nitrogen core doping introduces a pair of low-lying occupied states per monomer within the semiconducting gap of cGNRs. Charging resulting from the interaction with the gold substrate quenches one electronic state for each monomer, leaving behind a 1D chain of radical cations commensurate with the unit cell of the ribbon. In this work, scanning tunneling microscopy (STM) and spectroscopy (STS) reveal the signature of a Kondo resonance emerging from the interaction of $\textit{S}$ = 1/2 spin centers in each monomer core with itinerant electrons in the Au substrate. STM tip lift-off experiments locally reduce the effective screening of the unpaired radical cation being lifted, revealing a robust exchange coupling between neighboring spin centers. First-principles DFT-LSDA calculations support the presence of magnetic moments in the core of this GNR when it is placed on Au.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

MAGNETIC FIELD STRUCTURE AROUND LOW-MASS CLASS 0 PROTOSTARS: B335, L1527, AND IC348-SMM2

We report new 350 {mu}m polarization observations of the thermal dust emission from the cores surrounding the low-mass, Class 0 young stellar objects L1527, IC348-SMM2, and B335. We have inferred magnetic field directions from these observations and have used them together with results in the literature to determine whether magnetically regulated core-collapse and star formation models are consistent with the observations. These models predict a pseudo-disk with its symmetry axis aligned with the core magnetic field. The models also predict a magnetic field pinch structure on a scale less than or comparable to the infall radii for these sources. In addition, if the core magnetic field aligns (or nearly aligns) the core rotation axis with the magnetic field before core collapse, then the models predict the alignment (or near alignment) of the overall pinch field structure with the bipolar outflows in these sources. We show that if one includes the distorting effects of bipolar outflows on magnetic fields, then in general the observational results for L1527 and IC348-SMM2 are consistent with these magnetically regulated models. We can say the same for B335 only if we assume that the distorting effects of the bipolar outflow on the magnetic fields within the B335 core are much greater than for L1527 and IC348-SMM2. We show that the energy densities of the outflows in all three sources are large enough to distort the magnetic fields predicted by magnetically regulated models.

79 ASTRONOMY AND ASTROPHYSICS↗

Advances in Processing, Manufacturing, and Applications of Magnetic Materials

Magnetic materials are increasingly important for many green energy technologies. Probably, the best known of these are permanent magnets. They are used to supply a magnetic field and are widely used in actuators, motors, generators, data storage, and sensors. These are “hard magnets,” meaning that they retain a large permanent magnetization (difficult to be demagnetized), which is what makes them so useful in motors where an opposing magnetic field can be used to push against them. A coercivity (resistance to demagnetization) of ~400 Oe (32,000 A/m) or more is typically the threshold value for a hard magnet and is typical of isotropic sintered ferrite (SrFe 12 O 19 ) such as found in many “refrigerator magnets.” Comparably important soft magnets are useful for directing magnetic fields and can be very easily (de)magnetized. As such, they typically have a coercivity < 12.5 Oe (1000 A/m), and specialized very soft magnets can have coercivities < 0.00125 Oe (1 A/m). Some common applications include coil cores, transformer cores, and magnetic shielding. Additionally, they are important for many AC electrical applications such as inductors, filters, and resonators, particularly at high frequencies up to and including microwaves.

36 MATERIALS SCIENCE↗

ENABLING STAR FORMATION VIA SPONTANEOUS MOLECULAR DIPOLE ORIENTATION IN ICY SOLIDS

It is shown here how new experimental data, for the electrical properties of solid CO, can be used to fill important gaps in our understanding of the evolution of prestellar cores. Dust grains with a mantle of CO lead to a reduction in the degree of ionization in these cores by a factor of between 5 and 6. The lifetimes for expulsion of magnetic fields from cores, a process generally necessary for gravitational collapse, are reduced from current estimates of several megayears, by a similar factor. This removes a major inconsistency, since lifetimes now tally with typical ages of prestellar cores of a few hundred thousand to 10{sup 6} yr, derived from observations. With the reduced timescales, cores also escape disruption by Galactic supernova remnants. Our results provide a natural mechanism for the generation of so-called magnetically supercritical cores, in which the magnetic field alone cannot prevent gravitational collapse. In addition, we find a minimum value for the density of prestellar cores of ≥(1.1 ± 0.1) × 10{sup 4} H{sub 2} cm{sup −3}, in agreement with observations.

79 ASTRONOMY AND ASTROPHYSICS↗

SLOSHING OF THE MAGNETIZED COOL GAS IN THE CORES OF GALAXY CLUSTERS

X-ray observations of many clusters of galaxies reveal the presence of edges in surface brightness and temperature, known as 'cold fronts'. In relaxed clusters with cool cores, these edges have been interpreted as evidence for the 'sloshing' of the core gas in the cluster's gravitational potential. The smoothness of these edges has been interpreted as evidence for the stabilizing effect of magnetic fields 'draped' around the front surfaces. To check this hypothesis, we perform high-resolution magnetohydrodynamics simulations of magnetized gas sloshing in galaxy clusters initiated by encounters with subclusters. We go beyond previous works on the simulation of cold fronts in a magnetized intracluster medium by simulating their formation in realistic, idealized mergers with high resolution ({Delta}x {approx} 2 kpc). Our simulations sample a parameter space of plausible initial magnetic field strengths and field configurations. In the simulations, we observe strong velocity shears associated with the cold fronts amplifying the magnetic field along the cold front surfaces, increasing the magnetic field strength in these layers by up to an order of magnitude, and boosting the magnetic pressure up to near-equipartition with thermal pressure in some cases. In these layers, the magnetic field becomes strong enough to stabilize the cold fronts against Kelvin-Helmholtz instabilities, resulting in sharp, smooth fronts as those seen in observations of real clusters. These magnetic fields also result in strong suppression of mixing of high- and low-entropy gases in the cluster, seen in our simulations of mergers in the absence of a magnetic field. As a result, the heating of the core due to sloshing is very modest and is unable to stave off a cooling catastrophe.

79 ASTRONOMY AND ASTROPHYSICS↗

Enrichment of magnetic alignment stimulated by {gamma}-radiation in core-shell type nanoparticle Mn-Zn ferrite

Core shell type nanoparticle Mn{sub x}Zn{sub 1-x}Fe{sub 2}O{sub 4} systems with x=0.55, 0.65 and 0.75 were prepared using autocombustion method. The systems were characterized using tools like XRD and IR for structure confirmation. Magnetic parameter measurements like Saturation magnetization and coercivity were obtained from hysteresis loop which exhibited a symmetry shift due to core shell nature of the nanoparticles. Nanoparticles of particle size between 21.2nm to 25.7nm were found to show 20 percent shrinkage after being radiated by the {gamma}-radiation. This is due to variation in the cation distribution which also affects the cell volume of the cubic cell. Lattice constant reduction observed is reflected in the magnetic properties of the samples. A considerable hike in the saturation magnetization of the samples was observed due to enrichment of magnetic alignment in the magnetic core of the particles. Samples under investigation were irradiated with gamma radiation from Co{sup 60} source for different time intervals.

36 MATERIALS SCIENCE↗

DOES MAGNETIC-FIELD-ROTATION MISALIGNMENT SOLVE THE MAGNETIC BRAKING CATASTROPHE IN PROTOSTELLAR DISK FORMATION?

Stars form in dense cores of molecular clouds that are observed to be significantly magnetized. In the simplest case of a laminar (non-turbulent) core with the magnetic field aligned with the rotation axis, both analytic considerations and numerical simulations have shown that the formation of a large, 10{sup 2} AU scale, rotationally supported protostellar disk is suppressed by magnetic braking in the ideal MHD limit for a realistic level of core magnetization. This theoretical difficulty in forming protostellar disks is termed the ''magnetic braking catastrophe''. A possible resolution to this problem, proposed by Hennebelle and Ciardi and Joos et al., is that misalignment between the magnetic field and rotation axis may weaken the magnetic braking enough to enable disk formation. We evaluate this possibility quantitatively through numerical simulations. We confirm the basic result of Joos et al. that the misalignment is indeed conducive to disk formation. In relatively weakly magnetized cores with dimensionless mass-to-flux ratio {approx}> 4, it enabled the formation of rotationally supported disks that would otherwise be suppressed if the magnetic field and rotation axis are aligned. For more strongly magnetized cores, disk formation remains suppressed, however, even for the maximum tilt angle of 90 Degree-Sign . If dense cores are as strongly magnetized as indicated by OH Zeeman observations (with a mean dimensionless mass-to-flux ratio {approx}2), it would be difficult for the misalignment alone to enable disk formation in the majority of them. We conclude that, while beneficial to disk formation, especially for the relatively weak field case, misalignment does not completely solve the problem of catastrophic magnetic braking in general.

79 ASTRONOMY AND ASTROPHYSICS↗

Early Solar Wind and Dynamo Magnetic Field Topology Predictions for (16) Psyche and Other Asteroids

Abstract Asteroid (16) Psyche is a metal‐rich body that might record an ancient coherent magnetization if some relict crust or mantle is preserved. Herein, we use magnetohydrodynamic simulations to predict (16) Psyche's field topology for several distinct pathways: (i) an early solar wind‐induced magnetization imparted after a larger body was impacted, forming the present‐day asteroid, (ii) a core dynamo magnetization imparted in an asteroid that is either presently largely intact or was a rubble pile, and (iii) magnetization in the turbulent solar nebula disk. For pathway (i) we find the field to be predominantly dipolar and spin axis‐aligned. For pathway (ii) we find the field to be either dipolar and spin axis‐misaligned, or highly multipolar. We also find that (iii) a field produced earlier before the solar nebula cleared, would be highly multipolar. In cases (i) and (ii) we also place constraints on the field strength. Simple detection of a magnetic field without constraining its topology and temporal variability would be insufficient to confirm a remanent source, due to the influence of the present‐day solar wind, electromagnetic induction, and (16) Psyche's high obliquity. For sufficiently strong fields however, the field topology and orientation may reveal key observable consequences of the nature and history of (16) Psyche. Our framework is also broadly applicable to the study of magnetic fields from other asteroids.

79 ASTRONOMY AND ASTROPHYSICS↗

Application of Chebyshev Formalism to Identify Nonlinear Magnetic Field Components in Beam Transport Systems

An experiment was conducted at Jefferson Lab's Continuous Electron Beam Accelerator Facility to develop a beam-based technique for characterizing the extent of the nonlinearity of the magnetic fields of a beam transport system. Horizontally and vertically oriented pairs of air-core kicker magnets were simultaneously driven at two different frequencies to provide a time-dependent transverse modulation of the beam orbit relative to the unperturbed reference orbit. Fourier decomposition of the position data at eight different points along the beamline was then used to measure the amplitude of these frequencies. For a purely linear transport system one expects to find solely the frequencies that were applied to the kickers with amplitudes that depend on the phase advance of the lattice. In the presence of nonlinear fields one expects to also find harmonics of the driving frequencies that depend on the order of the nonlinearity. Chebyshev polynomials and their unique properties allow one to directly quantify the magnitude of the nonlinearity with the minimum error. A calibration standard was developed using one of the sextupole magnets in a CEBAF beamline. The technique was then applied to a pair of Arc 1 dipoles and then to the magnets in the Transport Recombiner beamline to measure their multipole content as a function of transverse position within the magnets.

43 PARTICLE ACCELERATORS↗

Exchange-Spring Magnets: Nanocomposite Exchange-Spring Magnets for Motor and Generator Applications

REACT Project: ANL will develop a cost-effective exchange-spring magnet to use in the electric motors of wind generators and EVs that uses no rare earth materials. This ANL exchange-spring magnet combines a hard magnetic outer shell with a soft magnetic inner core—coupling these together increases the performance (energy density and operating temperature). The hard and soft magnet composite particles would be created at the molecular level, followed by consolidation in a magnetic field. This process allows the particles to be oriented to maximize the magnetic properties of low-cost and abundant metals, eliminating the need for expensive imported rare earths. The ultimate goal of this project is to demonstrate this new type of magnet in a prototype electric motor.

ARPA-E↗

Templated Mesoporous Silica Outer Shell for Controlled Silver Release of a Magnetically Recoverable and Reusable Nanocomposite for Water Disinfection

Here, we encapsulated Fe 3 O 4 @SiO 2 @Ag (MS-Ag), a bifunctional magnetic silver core–shell structure, with an outer mesoporous silica (mS) shell to form an Fe 3 O 4 @SiO 2 @ 2 Ag@mSiO 2 (MS-Ag-mS) nanocomposite using a cationic CTAB (cetyltrimethylammonium bromide) micelle templating strategy. The mS shell acts as protection to slow down the oxidation and detachment of the AgNPs and incorporates channels to control the release of antimicrobial Ag + ions. Results of TEM, STEM, HRSEM, EDS, BET, and FTIR showed the successful formation of the mS shells on MS-Ag aggregates 50–400 nm in size with highly uniform pores ~4 nm in diameter that were separated by silica walls ~2 nm thick. Additionally, the mS shell thickness was tuned to demonstrate controlled Ag + release; an increase in shell thickness resulted in an increased path length required for Ag + ions to travel out of the shell, reducing MS-Ag-mS’ ability to inhibit E. coli growth as illustrated by the inhibition zone results. Through a shaking test, the MS-Ag-mS nanocomposite was shown to eradicate 99.99+% of a suspension of E. coli at 1 × 10 6 CFU/mL with a silver release of less than 0.1 ppb, well under the EPA recommendation of 0.1 ppm. This high biocidal efficiency with minimal silver leach is ascribed to the nanocomposite’s mS shell surface characteristics, including having hydroxyl groups and possessing a high degree of structural periodicity at the nanoscale or “smoothness” that encourages association with bacteria and retains high Ag + concentration on its surface and in its close proximity. Furthermore, the nanocomposite demonstrated consistent antimicrobial performance and silver release levels over multiple repeated uses (after being recovered magnetically because of the oxidation-resistant silica-coated magnetic Fe 3 O 4 core). It also proved effective at killing all microbes from Long Island Sound surface water. The described MS-Ag-mS nanocomposite is highly synergistic, easy to prepare, and readily recoverable and reusable and offers structural tunability affecting the bioavailability of Ag + , making it excellent for water disinfection that will find wide applications.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Magnetics, Inc. 0077894A7 (Datasheet)

Description of Core Under Test (CUT). Magnetics, Inc. 0077894A7 is a powder core material having low loss and high saturation fields. Known for the marketing name Kool Mu, was transformed by taking the known magnetic material, Sendust, and altered the manufacturing process to lower core losses. Possessing these specific properties makes it ideal for power factor correction circuits as well Pulse and Flyback Transformers. In-Line Noise Filters and Inductors are also common due to the near zero magnetostriction. Exhibits a potential saturation induction of 1 T.

36 MATERIALS SCIENCE↗