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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 253 records · Page 14

Nonequilibrium kinetic freeze-out properties in relativistic heavy ion collisions from energies employed at the RHIC beam energy scan to those available at the LHC

In this paper, we investigate the kinetic freeze-out properties in relativistic heavy ion collisions at different collision energies. We present a study of standard Boltzmann-Gibbs blast-wave (BGBW) fits and Tsallis blast-wave (TBW) fits performed on the transverse momentum spectra of identified hadrons produced in Au + Au collisions at collision energies of $\sqrt{s_{\rm{NN}}}=$7.7 –200 GeV at the Relativistic Heavy Ion Collider (RHIC), and in Pb + Pb collisions at collision energies of $\sqrt{s_{\rm{NN}}}=$ 2.76 and 5.02 TeV at the Large Hadron Collider (LHC). The behavior of strange and multistrange particles is also investigated. We found that the TBW model describes data better than the BGBW one overall, and the contrast is more prominent as the collision energy increases as the degree of nonequilibrium of the produced system is found to increase. From TBW fits, the kinetic freeze-out temperature at the same centrality shows a weak dependence of collision energy between 7.7 and 39 GeV, while it decreases as collision energy continues to increase up to 5.02 TeV. The radial flow is found to be consistent with zero in peripheral collisions at RHIC energies but sizable at LHC energies and central collisions at all RHIC energies. We also observed that the strange hadrons, with higher temperature and similar radial flow, approach equilibrium more quickly from peripheral to central collisions than light hadrons. The dependence of temperature and flow velocity on nonequilibrium parameter (q - 1) is characterized by two second-order polynomials. Both a and dξ from the polynomials fit, related to the influence of the system bulk viscosity, increase toward lower RHIC energies.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Employing ternary fission of Pu 242 as a probe of very neutron-rich matter

Detailed assessments of the ability of recent theoretical approaches to modeling existing experimental data for ternary fission confirm earlier indications that the dominant mode of cluster formation in ternary fission is clusterization in very neutron rich, very low density, essentially chemically equilibrated, nucleonic matter. An extended study and comparison of these approaches applied to ternary fission yields in the thermal neutron induced reaction 241 Pu(n th ,f) has been undertaken to refine the characterization of the source matter. Here, the resonance gas approximation has been improved taking in-medium effects on the binding energies into account. A temperature of 1.29 MeV, density of 6.7 × 10 -5 nucleons/fm 3 and proton fraction Y p = 0.035 are found to provide a good representation of yields of the ternary emitted light particles and clusters. In particular, results for Z = 1 and 2 isotopes are presented. Isotopes with larger Z are discussed, and the roles of medium and continuum effects, even at very low density are illustrated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A high transmission tender X-ray monochromator employing a matched pair of multilayer grating and mirror

It is now well established that multilayer coated gratings may offer high diffraction efficiencies over the tender X-ray range, from about 1 keV to 5 keV, covering the gap between single layer coated grating monochromators and crystal monochromators. Nevertheless, few beamlines in the world are using such gratings in their monochromator. The successful implementation of a multilayer grating monochromator requires producing a matched pair of a multilayer grating and a multilayer mirror, and this matching is not straightforward as it must account for different incidence angles and refraction effects on each element. Here we review the realization of the multilayer grating monochromator of the SIRIUS beamline which has been successfully in service for several years. We show how, by alternating computer simulation with our diffraction code and measurements, we could optimize the monochromator transmission on a very wide energy range. After the grating was coated, it was found that the angle of optimal efficiency versus photon energy was significantly different from what was predicted by a simple conformal model of binary layers. Layer interdiffusion and profile smoothing during the deposition process must be added to the multilayer model to reproduce the measured data. The critical adjustment of the mirror multilayer period is achieved by the lateral translation of the mirror, which was given a small transverse period gradient. The monochromator is thus providing high transmission efficiency in the 1 to 5 keV energy range, more than 30% over 2.5 keV and up to 46% at 4.6 keV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Novel High-Power Microwave Circulator Employing Circularly Polarized Waves

A novel four-port circulator is presented which uses an inline ferromagnetic element to allow for transmission or reflection depending on the sense of the incident circularly polarized wave. This configuration has been shown to reduce the dependency on ferrite anisotropy and support higher power, low rf loss, operation. An analytic analysis of this device is presented here alongside corroborating cold test data of the first prototype. High-power operation was performed at 2.856 GHz, with input power levels up to 8 MW for 3.5 μs in a pressurized nitrogen environment. The results from this research not only demonstrate ability to eliminate the use of greenhouse insulators, such as SF6, but also provide conceptual groundwork for a new class of ultrahigh power (50 MW+) nonreciprocal networks including circulators, isolators, phase shifters, and rf switches.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Employing Interacting Qubits for Distributed Microgrid Control

To empower flexible and scalable operations, distributed control of multi-inverter microgrids, based on classical communication networks among distributed energy resources, has attracted considerable attention as it can guarantee synchronization and provide suitable remedies to the problem of improper power sharing. Notwithstanding this, resilience of the current schemes on classical communication makes microgrids vulnerable to cyber attacks. Inspired by recent revolutionary breakthroughs in quantum communication, in this paper, we devise a novel synchronization mechanism. We extend the synchronization framework utilized in distributed control algorithms to networks of quantum systems by generating pinning terms and coupling mechanism for the new synchronization rule via exploiting proper quantum jump operators and observables, and show that the quantum system will converge to a time-variant target state. Our devised quantum distributed controller (QDC) gives rise to a novel quantum communication scheme for distributed control of microgrids and enables microgrids to exploit the state-of-the-art quantum communication frameworks as communication infrastructure. Finally, test results on two representative AC and DC networked microgrids validate the efficacy and universality of the quantum distributed control.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

Employing sequential experiments to gain insights on the interaction between creep and fatigue damage in Ni‐base superalloys

Abstract The interaction between creep and fatigue damage in Ni‐base superalloy CMSX‐8 was explored using a sequential workflow that decouples creep and fatigue steps to quantify how accumulated creep damage interacts with subsequent isothermal low‐cycle fatigue (LCF) and vice versa. Two workflows were considered: creep followed by LCF and LCF followed by creep. For the first workflow, the subsequent LCF was evaluated at temperatures of 20°C, 750°C, and 1100°C. It was found that the extent of deleterious interaction of prior creep on LCF depended on increasing subsequent fatigue test temperature. For the LCF followed by creep, fatigue tests were first conducted at 20°C and 1100°C to 60% of life, and then creep was conducted at 800°C, where primary creep is promoted, or 900°C, where primary creep is absent. LCF damage accumulated at 1100°C accelerated creep and decreased ductility, while fatigue damage at room temperature had minimal effect on the creep behavior.

Gorgannejad, Sanam↗

Ultra-Long Distance BOTDA Sensor System Employing Hybrid Amplification and Advanced Noise Reduction Techniques

Brillouin Optical Time Domain Analysis (BOTDA) sensor system play a pivotal role in distributed sensing, which enables precise measurements of strain and temperature across extensive fiber lengths. Nonetheless, challenges emerge as distances grow due to signal attenuation and noise interference resulting in measurement errors. This research offers a comprehensive strategy to extend the sensing range of BOTDA systems beyond 10’s of kilometers while maintaining high spatial resolutions. Such enhanced sensing is realized through the integration of distributed Raman amplification, inline amplification using erbium-doped fiber amplifiers (EDFA), and advanced noise reduction techniques. Leveraging inherent redundancy in measured data as a function of frequency and fiber distance, the non-local means (NLM) filter removes noise while preserving essential physical information. This approach proves particularly advantageous in BOTDA systems, where accurate measurement of Brillouin scattering signals is paramount for long-range sensing, while concurrently safeguarding high spatial resolutions. In summary, this research has shown a holistic exploration of extending BOTDA's distance sensing capabilities up to 150 km with spatial resolutions of 8 meters.

Bhatta, Hari↗

Q-BEEP: Quantum Bayesian Error Mitigation Employing Poisson Modeling over the Hamming Spectrum

Quantum computing technology has grown rapidly in recent years, with new technologies being explored, error rates being reduced, and quantum processor’s qubit capacity growing. However, near-term quantum algorithms are still unable to be induced without compounding consequential levels of noise, leading to non-trivial erroneous results. Quantum Error Correction (in-situ error mitigation) and Quantum Error Mitigation (post-induction error mitigation) are promising fields of research within the quantum algorithm scene, aiming to alleviate quantum errors, increasing the overall fidelity and hence the overall quality of circuit induction. Earlier this year, a pioneering work, namely HAMMER, published in ASPLOS-22 demonstrated the existence of a latent structure regarding post-circuit induction errors when mapping to the Hamming spectrum. However, they intuitively assumed that errors occur in local clusters, and that at higher average Hamming distances this structure falls away. In this work, we show that such a correlation structure is not only local but extends certain non-local clustering patterns which can be precisely described by a Poisson distribution model taking the input circuit, the device run time status (i.e., calibration statistics) and qubit topology into consideration. Using this quantum error characterizing model, we developed an iterative algorithm over the generated Bayesian network state-graph for post-induction error mitigation. Thanks to more precise modeling of the error distribution latent structure and the new iterative method, our Q-Beep approach provides state of the art performance and can boost circuit execution fidelity by up to 234.6% on Bernstein-Vazirani circuits and on average 71.0% on QAOA solution quality, using 16 practical IBMQ quantum processors. For other benchmarks such as those in QASMBench, the fidelity improvement is up to 17.8%. Q-Beep is a light-weight post-processing technique that can be performed offline and remotely, making it a useful tool for quantum vendors to integrate and provide more reliable circuit induction results.

Stein, Samuel A.↗

Employing artificial intelligence to steer exascale workflows with colmena

Computational workflows are a common class of application on supercomputers, yet the loosely coupled and heterogeneous nature of workflows often fails to take full advantage of their capabilities. We created Colmena to leverage the massive parallelism of a supercomputer by using Artificial Intelligence (AI) to learn from and adapt a workflow as it executes. Colmena allows scientists to define how their application should respond to events (e.g., task completion) as a series of cooperative agents. In this paper, we describe the design of Colmena, the challenges we overcame while deploying applications on exascale systems, and the science workflows we have enhanced through interweaving AI. The scaling challenges we discuss include developing steering strategies that maximize node utilization, introducing data fabrics that reduce communication overhead of data-intensive tasks, and implementing workflow tasks that cache costly operations between invocations. These innovations coupled with a variety of application patterns accessible through our agent-based steering model have enabled science advances in chemistry, biophysics, and materials science using different types of AI. In conclusion, our vision is that Colmena will spur creative solutions that harness AI across many domains of scientific computing.

Workflows↗

Laser-induced damage-growth threshold at 351 nm in the nanosecond regime in dielectric coatings employing different high-index materials

The laser-damage performance of HfO 2 /SiO 2 and Al 2 O 3 /SiO 2 mirrors was investigated at a laser wavelength of 351 nm with nanosecond pulse durations. A method was developed to quantify the laser-induced damage-growth threshold under conditions relevant to high-repetition-rate, large-aperture laser systems. The results suggest that the damage-growth performance cannot be inferred from the corresponding damage-initiation threshold that is commonly used to evaluate the performance of optical materials. Here, a systematic difference was also observed in the performance between these two groups of high-index materials, with the Al 2 O 3 /SiO 2 mirrors exhibiting about twofold improvement in the damage-growth threshold.

36 MATERIALS SCIENCE↗

Improving the laser performance of ion beam sputtered dielectric thin films through the suppression of nanoscale defects by employing a xenon sputtering gas

Laser damage-prone precursors in high index materials such as hafnia are believed to be the primary limiter in the performance of dielectric multilayer films to advance ultra-high power and energy laser applications. Removing or suppressing these precursors is the key to fabricating laser damage resistant thin films for the enabling technologies. Early work has revealed that nanobubbles formed by entrapped argon (Ar) working gas in ion beam sputtering (IBS) produced hafnia films are primarily responsible for the onset of laser damage upon exposure to UV, ns-laser pulses. In this study, we demonstrate that the UV ns-laser damage onset of IBS produced hafnia films can be improved to 3.1 +/- 0.2 J/cm 2 by substituting the conventional Ar working gas with xenon (Xe), a nearly 1 J/cm 2 increase from that of the Ar produced hafnia films. In addition to the suppression of the overall point-defect density of the hafnia films, the reduction of the Xe entrapment eliminates the nanobubbles and the generation of plasmas that initiates the laser damage. The defect suppression and its correlation to the increase in laser damage threshold is revealed by the combined analysis of Rutherford backscattering spectroscopy, electron paramagnetic resonance spectroscopy, transmission electron microscopy, and laser damage testing. Monte Carlo simulations suggest a much smaller entrapment of Xe gas by comparison to Ar, which is attributed to the significant difference in the energy of the reflected neutrals (3X) which are likely to be implanted. These results provide an effective process route with a fundamental understanding for producing high laser damage resistant dielectric films for high power and high energy laser applications.

36 MATERIALS SCIENCE↗

Operando bulk and interfacial characterization for electrochemical energy storage: Case study employing isothermal microcalorimetry and X-ray absorption spectroscopy

Abstract The global shift to electricity as the main energy carrier will require innovation in electrochemical energy storage (EES). EES systems are the key to the “electron energy economy,” minimizing losses and increasing reliability between energy supply and demand. However, steep challenges such as cost, cycle/calendar life, energy density, material availability, and safety limit widespread adoption of batteries for large-scale grid and vehicle applications. Battery innovation that meets today’s challenges will require new chemistries, which can originate from understanding charge transport phenomena at multiple time and length scales. The advancement of operando characterization can expedite this progress as changes can be observed during battery function. This article highlights progress in bulk and interfacial operando characterization of batteries. Specifically, a case study involving Fe 3 O 4 is provided demonstrating that combining X-ray absorption spectroscopy and isothermal microcalorimetry can provide real-time characterization of productive faradaic redox processes and parasitic interfacial reactions during (de)lithiation. Graphic abstract

36 MATERIALS SCIENCE↗

Feasibility Study of Replacing the R/V Robert Gordon Sproul with a Hybrid Vessel Employing Zero-emission Propulsion Technology

This project is a natural "follow-on" to the 2017 MARAD-funded project establishing the technical, regulatory, and economic feasibilities of a zero-emission hydrogen fuel-cell coastal research vessel named the Zero-V. In this follow-on project, we examine the applicability of hydrogen fuel-cell propulsion technology for a different kind of vessel, namely a smaller coastal/local research vessel targeted as a replacement for the Scripps Institution of Oceanography (SIO) R/V Robert Gordon Sproul, which is approaching the end of its service life.

08 HYDROGEN↗