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DOE OSTI2023

Role of nanoscale coherent precipitates on the thermo-mechanical response of martensitic materials (Final Report)

Coherent second phases can have a profound effect on the properties and performance of martensitic materials, and we lack a comprehensive, mechanistic understanding of the underlying processes. This limits our ability to rationally design second phases to tailor the response of martensitic materials. To address this situation, this project sought to develop a mechanistic, predictive understanding of the thermal and mechanical response of martensitic materials with nanoscale coherent heterogeneities. A synergistic combination of atomistic simulations and experiments was used to relate the local properties of each phase (in particular, their free energy landscape) and the material nanostructure (volume fraction, shape and size of second phase precipitates, and defects that may disrupt coherency) to the overall materials response. The focus was on second phases expected to induce phenomena or properties not otherwise achievable: second order martensitic transformation in SMAs, ultra-low stiffness, increased control of transition temperatures, and fatigue resistance.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Undulator Radiation of Single Electrons: Coherence Length and Quantum-Optical Properties

The aims of the CLARA experiment at the Fermilab Integrable Optics Test Accelerator (IOTA) were to directly measure the coherence length of undulator radiation emitted by a single electron and to test whether the radiation is in a pure classical Glauber coherent state or in a quantum mixture of coherent and Fock states. We used a Mach-Zehnder interferometer (MZI) to study visible radiation generated by 150-MeV electrons circulating in the ring. The relative delay between the two arms of the MZI was adjusted by varying the length of one of them with a resolution of 10 nm. The intensity of the circulating beam spanned several orders of magnitude, down to single electrons. A pair of single-photon avalanche diodes (SPADs) was placed at the output of the MZI arms to detect photocounts with high efficiency and timing resolution. We describe the observed interference patterns and photocount rates as a function of interferometer delay and discuss their implications.

43 PARTICLE ACCELERATORS↗

DOE OSTI2022

Search for Anomalous Neutral Current Coherent-Like Single-Photon Production in MicroBooNE

MicroBooNE is a liquid argon time projection chamber (TPC) detector which offers excellent spatial and energy resolution and the ability to distinguish electrons from photons. In this note we present preliminary results from a dedicated search for neutral current (NC) single-photon production, with a focus on forward-going photons and no visible hadronic activity, both of which are key characteristics of “coherent-like” electromagnetic shower production. A total efficiency for SM-predicted NC coherent 1$\gamma$ events of 12.5% is obtained, defined relative to simulated events in the entire MicroBooNE active TPC. Relative to the Pandora-reconstructed single-shower event selection, the analysis achieves a 95% rejection of non-coherent NC 1π 0 background events and a 99.97% rejection of cosmic background events, while maintaining a signal efficiency of approximately 45%.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Search for anomalous neutral current coherent-like single-photon production in MicroBooNE

This note describes progress towards the first experimental search for neutrino-induced neutral current coherent single-photon production (NC coherent 1γ). The search makes use of data from the MicroBooNE’s 85-tonne active mass liquid argon time projection chamber detector, situated in Fermilab’s Booster Neutrino Beam, with an average neutrino energy of $\langle$E ν $\rangle$ ~ 0.8 GeV. A selection targeted on candidate neutrino interactions with a single photon-like electromagnetic shower in the final state and no visible vertex activity was developed to search for this rare NC coherent 1γ process.

43 PARTICLE ACCELERATORS↗

DOE OSTI2022

Search for anomalous neutral current coherent-like single-photon production in MicroBooNE

MicroBooNE is a liquid argon time projection chamber (TPC) detector which offers excellent spatial and energy resolution and the ability to distinguish electrons from photons. In this note we present preliminary results from a dedicated search for neutral current (NC) single-photon production, with a focus on forward-going photons and no visible hadronic activity, both of which are key characteristics of “coherent-like” electromagnetic shower production. A total efficiency for SM-predicted NC coherent 1γ events of 12.5% is obtained, defined relative to simulated events in the entire MicroBooNE active TPC. Relative to the Pandora-reconstructed single-shower event selection, the analysis achieves a 95% rejection of non-coherent NC 1π 0 background events and a 99.97% rejection of cosmic background events, while maintaining a signal efficiency of approximately 45%.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

SQMS Nanofabrication Taskforce: Towards Fabrication of High Coherence Superconducting Qubits

SQMS Nanofabrication Taskforce, which brings together experts in nanofabrication and materials science at the SQMS Center, has been launched to implement novel materials, substrates, and fabrication techniques for high coherence superconducting quantum devices. In a first coordinated effort, the Nanofabrication Taskforce developed fabrication processes to eliminate the lossy materials at surfaces and interfaces of superconducting qubits to enhance qubit coherence. The initial results of this study demonstrated T1 enhancement by almost an order of magnitude with best T1 s reaching ~ 600 $\mu$s. [1] We attribute this improvement to the replacement of lossy native Nb oxide layer with native Ta oxide, which is thinner and less disordered. we are now currently working on strategies with an aim towards moving qubit coherence times to millisecond timescales and beyond. The results of a systematic study will be presented to address substrate preparation, alternative materials as low loss platforms (Nb, Ta, and Re), novel non-oxide forming low loss capping layers such as proximitized Au, optimized qubit designs, and optimized Josephson junction materials, processing, and design.

Bal, Mustafa↗

DOE OSTI2025

Charged Current Coherent Pion Production Cross-Section Measurement at MicroBooNE

Coherent pion production, characterized by a neutrino interacting with an entire nucleus without breaking it apart, results in a forward-going muon, pion, and a low-momentum recoil nucleus. By leveraging an improved understanding of particle identification and background parameterization, we aim to achieve a new level of sensitivity to coherent interactions at low neutrino energy. The outcome of this analysis will contribute to ongoing efforts to model neutrino nucleus interactions accurately in neutrino oscillation studies and beyond Standard Model searches in MicroBooNE and future experiments, such as DUNE. We present progress towards a measurement of charged current coherent pion production cross-section on argon with the MicroBooNE liquid argon time projection chamber detector. This measurement will use MicroBooNE's full dataset collected from the Booster Neutrino Beam with a total exposure of $ 1.3 \times 10^{21} $ protons-on-target and average neutrino energy of 0.8 GeV.

Hussain, Adil [Kansas State U.]↗

DOE OSTI2025

External Radiation and Magnetic-Field Effects on the Coherence and Stability of Transmon Qubits

Superconducting transmon qubits are a central building block of modern quantum computing architectures, yet their coherence properties remain sensitive to external influences that can limit performance or introduce temporal instabilities. In this talk, I will discuss two experimental studies aimed at quantifying these effects. First, I will examine how ionizing radiation impacts qubit relaxation. Using the same transmon device operated at two locations with dramatically different radiation backgrounds—the above-ground SQMS facility at Fermilab (USA) and the deep-underground Gran Sasso Laboratory (Italy)—we observe a higher rate of radiation-induced decay events above ground, even though intrinsic noise remains the dominant source of single-shot errors. I will also discuss the detection efficiency of a radiation detector made using such a device. Second, I will present results on how small magnetic fields, applied either during cooldown or at millikelvin temperatures, influence device stability. We find that fixed-frequency transmons maintain robust coherence up to approximately 600 mG of trapped out-of-plane field, and that controlled application of magnetic field can reduce temporal fluctuations in T1. Together, these studies provide insight into how external environments shape transmon coherence and offer potential pathways for improving qubit stability in scalable quantum processors.

Roy, Tanay [Fermilab]↗

DOE OSTI2025

Multidimensional Coherent Spectroscopy of van der Waals materials and heterostructures (Final Technical Report)

This project advanced multidimensional coherent spectroscopy (MDCS) and related spectroscopic-imaging methods as quantitative probes of many-body optical excitations in two-dimensional (2D) van der Waals (vdW) semiconductors and their heterostructures. Monolayer transition-metal dichalcogenides (TMDs) such as MoSe 2 and WSe 2 provide a uniquely strong platform for excitonic physics due to reduced dielectric screening, which enhances Coulomb interactions and makes higher-order correlated states (e.g., biexcitons and exciton–trion correlations) more prominent than in conventional bulk semiconductors. At the same time, the same sensitivity that enables strong interactions also increases susceptibility to spatial inhomogeneity—e.g., strain gradients, wrinkles, nanoscale disorder potentials, and charge puddling—which can broaden resonances, obscure interaction signatures, and complicate device-to-device reproducibility. The work reported here addressed this dual opportunity and challenge by: (i) developing and deploying coherent multidimensional methods (including double-quantum MDCS) capable of isolating interaction signals with reduced background, (ii) integrating electrostatic control to tune carrier populations and interaction strengths in situ, and (iii) introducing complementary spatially resolved photoluminescence (PL) techniques—hyperspectral PL imaging and polarization-/field-dependent PL lineshape analysis—to directly quantify disorder, strain, and localization that govern the coherent response.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Progress toward differential cross-section measurements of coherent charged-pion production in charged-current muon neutrino interactions on argon with SBND

Coherent charged pion production in charged-current muon neutrino–nucleus interactions provides a clean experimental signature and enables an excellent estimate of the neutrino energy, making it particularly valuable for neutrino flux constraints and oscillation analyses in future long-baseline experiments. Despite its importance, theoretical modeling of this process remains challenging, especially in the low-energy region below 1 GeV and its dependence on the nuclear target. The Short-Baseline Near Detector (SBND) offers a unique opportunity to study coherent charged pion production using neutrinos in the few-hundred-MeV energy range from the Booster Neutrino Beam (BNB) interacting with an argon target (A = 40), with unprecedented statistics expected to yield approximately three thousand signal events in SBND’s BNB data with 3.5 x 10^20 protons on target. This analysis aims to achieve the first differential cross-section measurement of charged-current coherent charged pion production on argon, as well as the first measurement of this process using BNB neutrinos.

Oh, Sungbin [Fermilab]↗

DOE OSTI2022

The DREAM Endstation at the Linac Coherent Light Source

Free-electron lasers (FEL), with their ultrashort pulses, ultrahigh intensities, and high repetition rates at short wavelength, have provided new approaches to Atomic and Molecular Optical Science. One such approach is following the birth of a photo electron to observe ion dynamics on an ultrafast timescale. Such an approach presents the opportunity to decipher the photon-initiated structural dynamics of an isolated atomic and molecular species. It is a fundamental step towards understanding single- and non-linear multi-photon processes and coherent electron dynamics in atoms and molecules, ultimately leading to coherent control following FEL research breakthroughs in pulse shaping and polarization control. A key aspect for exploring photoinduced quantum phenomena is visualizing the collective motion of electrons and nuclei in a single reaction process, as dynamics in atoms/ions proceed at femtosecond (10 –15 s) timescales while electronic dynamics take place in the attosecond timescale (10 –18 s). Here, we report on the design of a Dynamic Reaction Microscope (DREAM) endstation located at the second interaction point of the Time-Resolved Molecular and Optical (TMO) instrument at the Linac Coherent Light Source (LCLS) capable of following the photon–matter interactions by detecting ions and electrons in coincidence. The DREAM endstation takes advantage of the pulse properties and high repetition rate of LCLS-II to perform gas-phase soft X-ray experiments in a wide spectrum of scientific domains. With its design ability to detect multi-ions and electrons in coincidence while operating in step with the high repetition rate of LCLS-II, the DREAM endstation takes advantage of the inherent momentum conservation of reaction product ions with participating electrons to reconstruct the original X-ray photon–matter interactions. In this report, we outline in detail the design of the DREAM endstation and its functionality, with scientific opportunities enabled by this state-of-the-art instrument.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

Subhalos in Galaxy Clusters: Coherent Accretion and Internal Orbits

Subhalo dynamics in galaxy cluster host halos govern the observed distribution and properties of cluster member galaxies. We use the IllustrisTNG simulation to investigate the accretion and orbits of subhalos found in cluster-size halos. We find that the median change in the major axis direction of cluster-size host halos is approximately 80° between a ∼ 0.1 and the present day. We identify coherent regions in the angular distribution of subhalo accretion, and ∼68% of accreted subhalos enter their host halo through ∼38% of the surface area at the virial radius. The majority of galaxy clusters in the sample have ∼2 such coherent regions. We further measure angular orbits of subhalos with respect to the host major axis and use a clustering algorithm to identify distinct orbit modes with varying oscillation timescales. The orbit modes correlate with subhalo accretion conditions. Subhalos in orbit modes with shorter oscillations tend to have lower peak masses and accretion directions somewhat more aligned with the major axis. One orbit mode, exhibiting the least oscillatory behavior, largely consists of subhalos that accrete near the plane perpendicular to the host halo major axis. Our findings are consistent with expectations from inflow from major filament structures and internal dynamical friction: most subhalos accrete through coherent regions, and more massive subhalos experience fewer orbits after accretion. Our work offers a unique quantification of subhalo dynamics that can be connected to how the intracluster medium strips and quenches cluster galaxies.

galaxy clusters↗

DOE OSTI2025

First Search for Neutral Current Coherent Single-Photon Production in MicroBooNE

This article presents the first search for neutrino-induced neutral current coherent single-photon production (NC coherent 1$\gamma$). The search makes use of data from the MicroBooNE 85-tonne active volume liquid argon time projection chamber detector, situated in the Fermilab Booster Neutrino Beam (BNB), with an average neutrino energy of $\langle E_{\nu}\rangle \sim 0.8$ GeV. A targeted selection of candidate neutrino interactions with a single photon-like electromagnetic shower in the final state and no visible vertex activity was developed to search for the NC coherent 1$\gamma$ process, along with two auxiliary selections used to constrain the dominant background from NC$\pi^0$ production. With an integrated exposure of $6.87 \times 10^{20}$ protons on target delivered by the BNB, we set the world's first limit for this rare process, corresponding to an upper limit on the flux-averaged cross section of $\sigma<1.49 \times 10^{-41}\text{cm}^2$ at 90% C.L.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Quantum coherent devices with reduced energy dissipation

The disclosed technology can be used to increase lifetimes of quantum coherent devices such as qubits including transmons and xmons and to reduce the losses in resonators. Energy stored in superconducting devices can be lost by emission of phonons that couple to the environment. Defects in one or more materials in the quantum coherent device can cause the coupling to phonons. Patterning one or more of the layers creates a phononic bandgap that reduces or eliminates the emission of the phonons to the environment. The energy then couples back to the quantum coherent device.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2021

On the Phase Grouping Mechanism for a Magnetron Coherent Oscillation

CW magnetrons, developed for industrial heaters, but driven by an injection-locking signal were suggested to power Superconducting RF (SRF) cavities due to higher efficiency and lower cost of generated RF power per Watt than traditionally used RF sources (klystrons, IOTs, solid-state amplifiers). When the magnetrons are intended to feed Room Temperature (RT) cavities, the injected phase or frequency locking signal may provide required phase or frequency stability of the accelerating field. However, when the magnetron RF sources are intended to feed high Q-factor SRF cavities, the sources must be controlled in phase and power in a wide bandwidth to compensate parasitic phase and amplitude modulations caused by microphonics. In dependence on parameters of magnetron and the injection-locking signal one can choose regime most suitable for feeding SRF cavities, enabling magnetron almost coherent oscillation at the wide bandwidth of control. A novel approach considering magnetrons as quasi-coherent or coherent RF generators enables choosing the tube parameters and operation most suitable for various SRF accelerators.

43 PARTICLE ACCELERATORS↗

DOE OSTI2023

Renewal: Coherent control of spin states in organic electronics – discovery and investigation of complex room-temperature magnetic quantum excitations

In the course of four funding cycles of this project, its research focused on the exploration and understanding of spin-dependent electronic processes in organic semiconductors. It aimed to investigate the potential of harnessing the spin degree of freedom in organic materials for various applications such as spin electronics, quantum information, sensors, and as well as quantum coherent spin phenomena of charge carrier states in organic semiconductors, with the aim to develop room-temperature-based quantum applications. Specifically, the project aimed to: Apply new diagnostic tools, i.e. spin spectroscopy techniques, for paramagnetic charge carrier states in organic semiconductors, based on coherent control with pulsed electron spin resonance to understand spin relaxation and spin mixing mechanisms in organic semiconductor materials and devices such as OLEDs. Explore the nature of charge carrier spin-coupling and pathways for its manipulation to control the physical behaviors of these materials. This involves investigating spin interactions through materials structure, composition, morphological dependencies, isotopic effects, and externally applied electric and magnetic fields, with the goal to manipulate electrical and optical material properties by adjusting spin-orbit, spin-dipolar, spin-exchange, as well as spin-hyperfine interactions to open up this materials class for new applications. Study spin-dependent charge carrier transport and recombination and how these observables are governed by spin-propagation, especially coherent spin propagation as well as collective spin-effects such as the spin-Dicke effect and resonant multi-photon magnetic dipole transitions. The project utilized pulsed electrically detected magnetic resonance (pEDMR) and pulsed optically detected magnetic resonance (pODMR) techniques over a wide frequency range. These techniques enabled the observation and quantification of various spin-spin coupling types, including spin-exchange, spin-dipolar, hyperfine, and spin-orbit interactions. The project will leverage low- to mid-frequency pEDMR/pODMR facilities and collaboration with the National High Magnetic Field Laboratory.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Measurement Of The Total Cross-Section Of Muon Neutrino Charged-Current Coherent Pion Production in NOvA Near Detector

Charged Current (CC) coherent neutrino-nucleus pion production is characterized by small momentum transferred to the nucleus, which is left in its ground state. Despite the relatively large uncertainties on the production cross-section, coherent production of mesons by neutrinos represents an important process, as it can shed light on the structure of the weak current and can also constitute a potential source of background for modern neutrino oscillation experiments and searches for Beyond Standard Model (BSM) physics. This Ph.D. thesis presents a new measurement of CC coherent pion production in the NOvA near detector at the Fermi National Accelerator Laboratory (Fermilab). The analysis is based on the use of both particle identification and kinematic selection criteria based on Convolutional Neural Networks (CNN) to achieve a selection purity of 60%. Given the energy range 1-5 GeV accessible with the available NOvA exposure in the NuMI beam, the results will also be relevant for f uture neutrino experiments like the Deep Underground Neutrino Experiment (DUNE).

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

νBDX: a Coherent Elastic Neutrino Nucleus Scattering (CEνNS) experiment at Jefferson Lab

Particle physics is an ever-changing field seeking to explain phenomena that lie at the limits of our current knowledge. Among discovered and hypothesized interactions, Coherent Elastic Neutrino-Nucleus Scattering (CE?NS) stands out as a fascinating and elusive phenomenon, offering a unique window into the nature of neutrinos and their interactions with matter. CE?NS, a process predicted by the Standard Model, represents one of the subtle ways in which neutrinos can interact with atomic nuclei. Unlike other neutrinonucleus interactions, CE?NS occurs coherently, meaning that the entire nucleus collectively responds to the neutrino-mediated weak force, resulting in small energy transfers to the nucleus as a whole. The extremely rare nature of CE?NS events presents a formidable challenge to experimenters seeking to detect and study these interactions. Recent advances in detector technologies and the implementation of large-scale experiments, such as coherent neutrino scattering experiments at research facilities around the world, have opened up new avenues for exploring this elusive phenomenon. These experiments aim not only to observe CE?NS directly but also to extract valuable information on neutrino properties, nuclear structure, and potential deviations from the Standard Model. This thesis aims to study the feasibility of an experiment to study CE?NS at The Thomas Jefferson National Accelerator Facility, Newport News, VA, USA. This would be an experiment that exploits the production of neutrinos by an electron beam dumped on a thick target (the beam dump). The large quantity of neutrinos produced and their energy profile are well suited to the purpose of studying the CE?NS. In my thesis, I will start from previous studies on CE?NS and from theoretical considerations regarding the process, then quantify the expected events for a hypothetical experiment and possible backgrounds through simulations aimed at optimizing the geometry of the future detector. I will also show some tests on selected detector components that will be part of a first prototype.

Grazzi, Stefano↗