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At least 253 records · Page 14

The Gallium Anomaly and the BEST Experiment [Slides]

The measurements of the charged-current capture rate of neutrinos on 71 Ga from strong radioactive sources have yielded results below those expected, based on the known strength of the principal transition supplemented by theory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Paragenetic controls on CO 2 -fluid-rock interaction and weakening in a macroporous-dominated sandstone

The injection and storage of anthropogenic CO 2 in the subsurface is being deployed as a climate change mitigation tool; however, diagenetic-paragenetic heterogeneity in sandstone reservoirs often contributes to interval specific chemomechanical changes that affect injection and can increase leakage risk.In this paper we address reservoir heterogeneities’ impact on chemomechanical changes in a macroporous-dominated lithofacies of Morrow B sandstone, a formation containing several diagenetically-distinct hydraulic facies while undergoing enhanced oil recovery (EOR) and carbon dioxide (CO 2 ) sequestration. We performed three flow-through experiments using a CO 2 -charged or uncharged formation water combined with four indirect tensile strength tests per post-test sample. We then used the microstructure and paragenetic sequence to understand chemomechanical weakening with key observations as follows: dissolution of carbonates and feldspars changed porosity; increased permeability led to reclassifying each sample in a different hydraulic flow unit; decreased ultrasonic velocity; and did not lead to a loss of tensile strength. Tensile strength maintenance occurred due to the low abundance and minor dissolution of siderite, the stability of quartz, and the relative position of diagenetic ankerite within feldspar. This macroporous-dominated lithofacies is the primary reservoir for the Morrow B Sandstone, and is analogous to other porous sandstone reservoirs. It represents an end-member of a chemomechanically low-risk siliceous CO 2 sequestration and CO 2 -EOR reservoir.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Charged-current non-standard neutrino interactions at Daya Bay

The full data set of the Daya Bay reactor neutrino experiment is used to probe the effect of the charged current non-standard interactions (CC-NSI) on neutrino oscillation experiments. Two different approaches are applied and constraints on the corresponding CC-NSI parameters are obtained with the neutrino flux taken from the Huber-Mueller model with a 5% uncertainty. For the quantum mechanics-based approach (QM-NSI), the constraints on the CC-NSI parameters $ϵ_{eα}$ and $ϵ^s_{eα}$ are extracted with and without the assumption that the effects of the new physics are the same in the production and detection processes, respectively. The approach based on the weak effective field theory (WEFT-NSI) deals with four types of CC-NSI represented by the parameters [ε X ] eα . For both approaches, the results for the CC-NSI parameters are shown for cases with various fixed values of the CC-NSI and the Dirac CP-violating phases, and when they are allowed to vary freely. We find that constraints on the QM-NSI parameters $ϵ_{eα}$ and $ϵ^s_{eα}$ from the Daya Bay experiment alone can reach the order O(0.01) for the former and O(0.1) for the latter, while for WEFT-NSI parameters [ε X ] eα , we obtain O(0.1) for both cases.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

CISME report on experiments with HMX powder, PBX 9501 prills, and heated PBX 9501

The ability to predict post-ignition explosive response is relevant to explosives safety, particularly weapons assembly/disassembly operations that must operate under a sufficiently conservative safety basis to meet risk mitigation criteria for inadvertent nuclear detonation (IND). In particular, hazard determinations hinge on whether the PBX 9501 main charge can ultimately attain detonation from an initial, non-shock, ignition stimulus. The CISME experiment uses a spherical explosive charge, which is thermally ignited in the center using a fiber-delivered infrared laser pulse. This ignition mechanism - i.e. a localized thermal hotspot - is representative of the ignition-causing insults typical in accident scenarios, including low-velocity impact, drop, skid, and punch events. In fiscal year 2018 CISME experiments were conducted with pristine PBX 9501 spheres, confined and unconfined. Sub-detonative, low-violence reactions were observed. Here we report experiments conducted since 2018. The explosive charge was varied: experiments were conducted with room temperature pour-density HMX powder and prills of PBX 9501, and heated, thermally damaged PBX 9501. Experiments were conducted in a confined configuration, with two 4 mm-thick stainless-steel hemispherical shells bolted around the sphere. Detonation, via DDT (deflagration-to-detonation transition) was observed in the 3-inch diameter powdered HMX and the 6-inch diameter heated and thermally-damaged PBX 9501 tests. No transition to DDT was observed in smaller diameters for those configurations, and no DDT was observed for pour-density prills of PBX 9501 of any diameter. The original test series demonstrated that the response of pristine, undamaged PBX 9501 to a central ignition is relatively benign. This new test series shows that increased porosity, lack of polymer binders and thermal damage can greatly increase the violence of the post-ignition response, up to and including detonation. These results bridge the explosive response of PBX 9501 from sub-detonative through detonation as a function of diameter and provide valuable test cases for modeling efforts that strive to capture the DDT threshold. By exploring explosive response in a more representative 3D geometry, we can also benchmark these new results to more plentiful DDT datasets generated from testing in 1D tube confinement (the historical test configuration)–the configuration upon which almost all DDT models were developed.

42 ENGINEERING↗

The physics potential of a reactor neutrino experiment with Skipper-CCDs: searching for new physics with light mediators

In this work, we explore the sensitivity to new physics of the recently proposed vIOLETA experiment: a 10 kg Skipper Charged Coupled Device detector deployed 12 meters away from a commercial nuclear reactor core. We investigate two broad classes of models which benefit from the very low energy recoil threshold of these detectors, namely neutrino magnetic moments and light mediators coupled to neutrinos and quarks or electrons. We find that this experimental setup is very sensitive to light, weakly coupled new physics, and in particular that it could probe potential explanations of the event excess observed in XENON1T. We also provide a detailed study on the dependence of the sensitivity on the experimental setup assumptions and on the neutrino flux systematic uncertainties.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Robustness of the smartpixels classifier for different simulated sensor geometries and non-ideal detector conditions

Pixel tracking detectors at upcoming collider experiments will see unprecedented charged-particle densities. Real-time data reduction on the detector will enable higher granularity and faster readout, possibly enabling the use of the pixel detector in high-rate online event selection, such as the ATLAS or CMS first-level trigger systems. This data reduction can be accomplished with a neural network (NN) in the readout chip bonded with the sensor that recognizes and rejects tracks with low transverse momentum (p T ) based on the geometrical shape of the charge deposition (“cluster”). To design viable detectors for deployment, the dependence of the NN as a function of the sensor geometry, external magnetic field, irradiation, and noise must be understood. In this paper, we present first studies of the efficiency and data reduction for planar pixel sensors exploring these parameters. For the CMS HL-LHC sensor geometry, we obtain a signal efficiency of (91.9 ± 0.7)% and a data reduction of (29.7 ± 1.0)%. A smaller sensor pitch in the bending direction improves the p T discrimination, but a larger pitch can be partially compensated with detector thickness. Any accumulated radiation damage also changes the cluster shape, reducing the signal efficiency compared to the baseline by approximately 30–60% in absolute terms, but nearly all of the performance can be recovered through retraining of the network and updating the weights. Finally, the impact of noise was investigated, and retraining the network on noise-injected datasets was found to maintain performance within 6% of the baseline network trained and evaluated on noiseless data. •ASIC-compatible track-momentum classifier is robust in realistic detector conditions.•About 90% signal efficiency and 30% data reduction per layer for CMS HL-LHC geometry.•Single-layer signal efficiency increases for smaller pixel pitch or thicker sensors.•Performance with noise or after radiation damage mostly recovered by retraining.

Shekar, Danush [Illinois U., Chicago] (ORCID:00000↗

Acid–Base Chemistry of a Model IrO 2 Catalytic Interface

Iridium oxide (IrO 2 ) is one of the most efficient catalytic materials for the oxygen evolution reaction (OER), yet the atomic scale structure of its aqueous interface is largely unknown. Herein, the hydration structure, proton transfer mechanisms and acid-base properties of the rutile IrO 2 (110)-water interface are investigated using ab-initio based deep neural-network potentials and enhanced sampling simulations. The proton affinities of the different surface sites are characterized by calculating their acid dissociation constants, which yield a point of zero-charge in good agreement with experiments. A large fraction (≈ 80%) of adsorbed water dissociation is observed, together with a short lifetime (≈ 0.5 ns) of the resulting terminal hydroxy groups, due to rapid proton exchanges between adsorbed H 2 O and adjacent OH species. As a result, this rapid surface proton transfer supports the suggestion that the rate-determining step in the OER may not involve proton transfer across the double layer into solution, as indicated by recent experiments.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Explosively driven Richtmyer–Meshkov instability jet suppression and enhancement via coupling machine learning and additive manufacturing

The ability to control the behavior of fluid instabilities at material interfaces, such as the shock-driven Richtmyer–Meshkov instability, is a grand technological challenge with a broad number of applications ranging from inertial confinement fusion experiments to explosively driven shaped charges. In this work, we use a linear-geometry shaped charge as a means of studying methods for controlling material jetting that results from the Richtmyer–Meshkov instability. A shaped charge produces a high-velocity jet by focusing the energy from the detonation of high explosives. The interaction of the resulting detonation wave with a hollowed cavity lined with a thin metal layer produces the unstable jetting effect. By modifying the characteristics of the detonation wave prior to striking the lined cavity, the kinetic energy of the jet can be enhanced or reduced. Modifying the geometry of the liner material can also be used to alter jetting properties. We apply optimization methods to investigate several design parameterizations for both enhancing or suppressing the shaped-charge jet. This is accomplished using 2D and 3D hydrodynamic simulations to investigate the design space that we consider. We also apply new additive manufacturing methods for producing the shaped-charge assemblies, which allow for the experimental testing of complicated design geometries obtained through computational optimization. We present a direct comparison of our optimized designs with experimental results carried out at the High Explosives Application Facility at Lawrence Livermore National Laboratory.

36 MATERIALS SCIENCE↗

Discrimination of electronic recoils from nuclear recoils in two-phase xenon time projection chambers

We present a comprehensive analysis of electronic recoil vs. nuclear recoil discrimination in liquid/gas xenon time projection chambers, using calibration data from the 2013 and 2014-16 runs of the Large Underground Xenon (LUX) experiment. We observe strong charge-to-light discrimination enhancement with increased event energy. For events with S1 = 120 detected photons, i.e. equivalent to a nuclear recoil energy of ~100 keV, we observe an electronic recoil background acceptance of <10 –5 at a nuclear recoil signal acceptance of 50%. We also observe modest electric field dependence of the discrimination power, which peaks at a field of around 300 V/cm over the range of fields explored in this study (50-500 V/cm). In the WIMP search region of S1 = 1-80 phd, the minimum electronic recoil leakage we observe is (7.3 ± 0.6) 10 –4 , which is obtained for a drift field of 240-290 V/cm. Pulse shape discrimination is utilized to improve our results, and we find that, at low energies and low fields, there is an additional reduction in background leakage by a factor of up to 3. We develop an empirical model for recombination fluctuations which, when used alongside the Noble Element Scintillation Technique (NEST) simulation package, correctly reproduces the skewness of the electronic recoil data. We use this updated simulation to study the width of the electronic recoil band, finding that its dominant contribution comes from electron-ion recombination fluctuations, followed in magnitude of contribution by fluctuations in the S1 signal, fluctuations in the S2 signal, and fluctuations in the total number of quanta produced for a given energy deposition.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Quadrilateral particle arrangement within shocks in a two-dimensional dusty plasma

The microscopic structure within a two-dimensional shock was studied using data from a dusty plasma experiment. A single layer of charged microparticles, levitated in a glow-discharge plasma, was perturbed by an electrically floating wire that was moved at a steady supersonic speed to excite a compressional shock. A rearrangement of particles was observed, from a hexagonal lattice in the preshock into a quadrilateral microstructure on the front side of the shock. This quadrilateral structure would not be stable in a monolayer of identical repulsive particles, under equilibrium conditions. Glaser-Clark polygon analysis of the microstructure helped in identifying quadrilaterals. Voronoi analysis was used to characterize the defect fraction behind the shock, as an indication of shock-induced melting. Published by the American Physical Society 2025

Kananovich, Anton (ORCID:0000000225374952)↗

Computational Elucidation of Mechanical Degradation in NMC Cathodes: Impact on Cell Performance

Next-generation lithium ion batteries are expected to demonstrate superior energy and power density with longer cycle life for successful electrification of the automobile, aviation, and marine industries. Adoption of lithium metal anodes with solid electrolytes can help to achieve that goal given that the dendrite-related issues are solved eventually. Another possibility is to use Ni-rich high-capacity NMC cathode materials with liquid and/or solid electrolytes, which presently experiences rapid capacity fade while charged to higher voltages. Several mechanical and chemical degradation mechanisms are active within these NMC-based cathode particles. Recent experimental research activities attempted to correlate the mechanical damage with the capacity fade experienced by Ni-rich LiNi x Mn y Co z O 2 (x+y+z = 1) (NMC) cathodes. Here, a computational framework is developed in this study capable of quantifying the evolution of inter primary particle and cathode/electrolyte interfacial fracture experienced by the poly- and single-crystalline NMC cathodes during charge/discharge operation. Influences of mechanical degradation on the overall cell capacity, while operating with liquid and/or solid electrolytes, are successfully characterized. Decreasing the size of the cathode primary particles, or the size of the single-crystalline cathodes, can mitigate the overall mechanical degradation, and subsequent capacity fade, experienced by NMC cathodes. The developed theoretical methodology can help the engineers and scientists to better understand the mechanical degradation mechanism prevalent in Ni-rich NMC cathodes and build superior lithium ion-based energy storage devices for the application in next-generation devices.

25 ENERGY STORAGE↗

A data-driven method to constrain the $\bar{p}$ background in Mu2e

The Mu2e experiment will search for the charged lepton flavour violating process of neutrinoless coherent muon to electron conversion in the field of an Al nucleus. The expected signal is a 104.97 MeV/c electron. One of the expected backgrounds is due to ¯ps produced by the proton beam at the Production Target and annihilating in the Stopping Target (ST). The background from ¯p annihilation is not a dominant one, but it has a large uncertainty and it cannot be suppressed by the timing cuts used to reduce the prompt background. However at Mu2e energies, p¯p annihilation is the only source of events with multiple simultaneous tracks coming from the ST. We exploit this unique feature and reconstruct the multi-track events to estimate the ¯p background.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

ELECTRON COOLING USING A PULSED AND DITHERING BEAM FROM AN ELECTROSTATIC ELECTRON COOLER

Electron cooling continues to be an invaluable technique to reduce and maintain the emittance in hadron storage rings such as the EIC and EICC where stochastic cooling is inefficient and radiative cooling is negligible. Extending the energy range of electron coolers beyond what is feasible with the conventional, electrostatic approach necessitates the use of RF fields for acceleration and, thus, a bunched electron beam. To experimentally investigate how the relative time structure of the two beams affects the cooling properties, we have set up a pulsed-beam cooling device by adding a synchronized pulsing circuit to the conventional electron source of the CSRm cooler at Institute of Modern Physics. Using both constant and modulated synchronization between electron pulses and ion bunches, we have measured the effects of the electron bunch length and longitudinal ion focusing strength on the temporal evolution of the longitudinal and transverse ion beam profile and demonstrated the detrimental effect of timing jitter as predicted by space-charge theory and simulations. Our experiment suggests a need for further investigations of specific aspects of bunched cooling such as synchro-betatron coupling and phase dithering effects when using short electron bunches to cool longer ion bunches. However, given the comparatively long IBS lifetime of higher-energy proton storage rings like the EIC, slow dithering could potentially provide an option to save cost on the electron cooler linac.

Wang, Haipeng↗

Summer 2021 Co-op Report: X-Ray Scintillation Detector (A Co-op Work Experience Report)

The M-3 team was in need of a detector that could be used properly characterize their X-Ray machines. It can also be used to diagnose the X-ray in the case that problems arise before or during an experiment. They put me in charge of designing, ordering, and constructing said detector. After doing research, I found that scintillation-based detectors would be the best diagnostic tool for this purpose. It will allow the team to collect a full photon count of the X-ray pulse as well as provide spectroscopy functions with which we can view photon counts at different energy levels. This will also allow them to calculate an accurate dose given from the machine. Due to lead times, the crystals are still in manufacturing, thus the detector could not be completed. Although the designs and calculations needed to construct and operate the scintillator have been completed which is what I will be presenting in this document. Compared to the detectors being used before, my design offers a cheaper and far more efficient alternative.

42 ENGINEERING↗

Thermionic Sources for Electron Cooling at IOTA

We are designing and fabricating two new thermionic sources of magnetized electrons for use in the electron lens project in the Integrable Optics Test Accelerator (IOTA) at Fermilab. These electron sources will be used for cooling 2.5 MeV protons. One source will be used to compensate for emittance growth due to Intra Beam Scattering in experiments with weak space-charge, while the other source will be used to research the interplay between electron cooling and intense space charge. In this paper we present the progress made so far and the upcoming steps for the thermionic electron sources.

43 PARTICLE ACCELERATORS↗

EIC hadron ring longitudinal stability simulations at injection

At the EIC injection energy (23.8 GeV for protons), the hadron beam experiences a relatively strong space charge field. The corresponding wakefield, in conjunction with the wakes from the RF cavities (i.e. the geometrical wakes), may become the cause of single-bunch instabilities, both longitudinal and transverse. In this report, we focus on the longitudinal stability aspect of this picture, using a simplified model for the ring.

43 PARTICLE ACCELERATORS↗

Breaking the Limit of Size-Dependent CO2RR Selectivity in Ag Nanoparticle Electrocatalysts through Electronic Metal-Carbon Interactions: Insights from Computational Hydrogen Electrode Calculations

This poster highlights the use of computational hydrogen electrode approach to explain the improved activity and selectivity of Ag nanoparticle catalysts for CO2 to CO conversion observed in the experiments. The calculations predict a charge transfer from the Ag nanoparticle to a defective carbon surface, stabilizing the *COOH intermediate through reduced antibonding orbital overlap, significantly reducing the *COOH formation energy barrier, and improving CO2-to-CO conversion selectivity compared with Ag nanocluster on defect-free carbon. These results provide new insights into carbon-supported electrocatalysts for CO2RR and introduce a new approach for creating active and selective nanocatalysts.

electrocatalysis↗